A self-powered HgTe quantum dots/PBDB-T:Y6 bipolar broadband photodetector for logic gates.

IF 12.2 2区 材料科学 Q1 CHEMISTRY, MULTIDISCIPLINARY Materials Horizons Pub Date : 2025-02-13 DOI:10.1039/d4mh01925c
Wenxin Zeng, Zaihua Duan, Yichen Bu, Haichao Yu, Changhong Wang, Xing Tang, Jingwen Yang, Zhen Yuan, Yadong Jiang, Huiling Tai
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Abstract

Optoelectronic logic gates (OELGs) have become one of the excellent candidates for logic devices in the post Moore era, with great potential for complex optical computing, secure optical communication, and image processing. As an important component of OELGs, bipolar photodetectors (BPDs) face problems such as limited logic functionality, narrow response range, slow response speed, and high-power consumption. Here, we propose a self-powered BPD with a back-to-back structure based on HgTe quantum dot (QD) and organic material PBDB-T:Y6 stacking. The results show that the BPD exhibits a broadband bipolar photoresponse (300-1800 nm) under a bias voltage of 0 V, with a rapid response speed in the microsecond range. By modulating the device with three light sources within the positive and negative photoresponse wavelength ranges, the HgTe QDs/PBDB-T:Y6 BPD successfully achieves five logic gate operations ("OR", "AND", "NAND", "NOR", and "NOT"). Based on excellent fast and broadband bipolar optoelectronic response, we further confirm the potential application of the HgTe QDs/PBDB-T:Y6 BPD in broadband optical communication encryption. This work provides a useful reference for the combination of QDs and organic materials in the development of high-performance BPDs.

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Materials Horizons
Materials Horizons CHEMISTRY, MULTIDISCIPLINARY-MATERIALS SCIENCE, MULTIDISCIPLINARY
CiteScore
18.90
自引率
2.30%
发文量
306
审稿时长
1.3 months
期刊介绍: Materials Horizons is a leading journal in materials science that focuses on publishing exceptionally high-quality and innovative research. The journal prioritizes original research that introduces new concepts or ways of thinking, rather than solely reporting technological advancements. However, groundbreaking articles featuring record-breaking material performance may also be published. To be considered for publication, the work must be of significant interest to our community-spanning readership. Starting from 2021, all articles published in Materials Horizons will be indexed in MEDLINE©. The journal publishes various types of articles, including Communications, Reviews, Opinion pieces, Focus articles, and Comments. It serves as a core journal for researchers from academia, government, and industry across all areas of materials research. Materials Horizons is a Transformative Journal and compliant with Plan S. It has an impact factor of 13.3 and is indexed in MEDLINE.
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