A sulfur dioxide detection platform based on photoacoustic spectroscopy and a 266.22 nm high-power stabilized LD-pumped solid-state Q-switched laser

IF 6.8 1区 医学 Q1 ENGINEERING, BIOMEDICAL Photoacoustics Pub Date : 2025-04-01 Epub Date: 2025-02-18 DOI:10.1016/j.pacs.2025.100702
Xiaowen Shen , Yixin Zhang , Ruyue Cui , Donghe Tian , Ming Cheng , Pietro Patimisco , Angelo Sampaolo , Chaofeng Sun , Xukun Yin , Vincenzo Spagnolo , Lei Dong , Hongpeng Wu
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Abstract

A ppb-level sulfur dioxide (SO2) monitoring platform was developed by exploiting standard photoacoustic spectroscopy and a novel, highly stable UV laser. A 266.22 nm LD-pumped solid-state, acousto-optic modulator Q-switched laser with high beam quality (M2 =1.0275) and excellent output optical power stability (δ ˂ 1 % ∼24 h) was selected as light source of the photoacoustic sensor. The performance of the SO2 sensor was evaluated in terms of gas flow rate, pressure, and detection sensitivity. An ultimate detection limit of 3 ppb for SO2 detection in N2 was demonstrated with 1 s integration time, in laboratory environment. Continuous outdoor monitoring for five days verified the excellent stability and reliability of the reported SO2 photoacoustic sensor.
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基于光声光谱和266.22 nm大功率稳定ld泵浦固态调q激光器的二氧化硫检测平台
利用标准光声光谱和新型高稳定紫外激光器,研制了ppb级二氧化硫(SO2)监测平台。选择266.22 nm的ld泵浦固态声光调制器调q激光器作为光声传感器的光源,该激光器具有高光束质量(M2 =1.0275)和良好的输出光功率稳定性(δPσ小于1 % ~ 24 h)。从气体流速、压力和检测灵敏度等方面对SO2传感器的性能进行了评价。在实验室环境下,以1 s的积分时间,对N2中SO2的最终检出限为3 ppb。连续5天的室外监测验证了所报道的SO2光声传感器的优异稳定性和可靠性。
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来源期刊
Photoacoustics
Photoacoustics Physics and Astronomy-Atomic and Molecular Physics, and Optics
CiteScore
11.40
自引率
16.50%
发文量
96
审稿时长
53 days
期刊介绍: The open access Photoacoustics journal (PACS) aims to publish original research and review contributions in the field of photoacoustics-optoacoustics-thermoacoustics. This field utilizes acoustical and ultrasonic phenomena excited by electromagnetic radiation for the detection, visualization, and characterization of various materials and biological tissues, including living organisms. Recent advancements in laser technologies, ultrasound detection approaches, inverse theory, and fast reconstruction algorithms have greatly supported the rapid progress in this field. The unique contrast provided by molecular absorption in photoacoustic-optoacoustic-thermoacoustic methods has allowed for addressing unmet biological and medical needs such as pre-clinical research, clinical imaging of vasculature, tissue and disease physiology, drug efficacy, surgery guidance, and therapy monitoring. Applications of this field encompass a wide range of medical imaging and sensing applications, including cancer, vascular diseases, brain neurophysiology, ophthalmology, and diabetes. Moreover, photoacoustics-optoacoustics-thermoacoustics is a multidisciplinary field, with contributions from chemistry and nanotechnology, where novel materials such as biodegradable nanoparticles, organic dyes, targeted agents, theranostic probes, and genetically expressed markers are being actively developed. These advanced materials have significantly improved the signal-to-noise ratio and tissue contrast in photoacoustic methods.
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