Recent advances in transition metal carbides and nitrides (MXenes): Characteristics, environmental remediation and challenges

IF 13.3 1区 工程技术 Q1 ENGINEERING, CHEMICAL Chemical Engineering Journal Pub Date : 2021-08-15 DOI:10.1016/j.cej.2021.129296
You Wu , Xiaoming Li , Hui Zhao , Fubing Yao , Jiao Cao , Zhuo Chen , Xiaoding Huang , Dongbo Wang , Qi Yang
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引用次数: 54

Abstract

MXenes, as newly emerging two-dimensional (2D) transition metal carbides and nitrides, have become promising candidates for environmental remediation and detection due to their hydrophilicity, metallic conductivity, versatile surface chemistry and 2D layered atomic structure. Nevertheless, little attention has been paid to the relationship between the properties of MXenes and their environmental performances. Herein, based on the recent experimental and theoretical research, a systematic review about the environmental applications of MXenes and MXenes-based materials including the removal and detection of toxic metal ions and organic contaminants, capture and mitigation of gas, hydrogen production, membrane- based separation, and disinfection has been done. Various design strategies of MXenes on ameliorating application performance are mentioned, and their suitability in multifarious environmental applications is thoroughly discussed. Based on the specific requirements of the final environmental applications, a targeted description between their properties and their abilities for environmental application is provided. Finally, current challenges and perspectives in this field are proposed from our personal insights. Particular emphasis in this review is directed toward the importance of understanding ultimate the aim and the required attributes to develop the proper materials for specific applications, and facilitates the further evolution of MXenes in environmental applications.

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过渡金属碳化物和氮化物(MXenes)的最新进展:特征、环境修复和挑战
MXenes作为新兴的二维(2D)过渡金属碳化物和氮化物,由于其亲水性、金属导电性、多样的表面化学性质和二维层状原子结构,已成为环境修复和检测的有希望的候选者。然而,很少有人关注MXenes的性质与其环境性能之间的关系。本文基于近年来的实验和理论研究,对MXenes及其基材料在有毒金属离子和有机污染物的去除和检测、气体的捕获和减排、制氢、膜分离和消毒等方面的环境应用进行了系统综述。介绍了MXenes在提高应用性能方面的各种设计策略,并深入讨论了它们在各种环境应用中的适用性。根据最终环境应用的具体要求,对其特性和环境应用能力进行了有针对性的描述。最后,从个人的角度提出了当前该领域面临的挑战和前景。本综述特别强调了了解最终目的和所需属性的重要性,以开发适合特定应用的材料,并促进MXenes在环境应用中的进一步发展。
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来源期刊
Chemical Engineering Journal
Chemical Engineering Journal 工程技术-工程:化工
CiteScore
21.70
自引率
9.30%
发文量
6781
审稿时长
2.4 months
期刊介绍: The Chemical Engineering Journal is an international research journal that invites contributions of original and novel fundamental research. It aims to provide an international platform for presenting original fundamental research, interpretative reviews, and discussions on new developments in chemical engineering. The journal welcomes papers that describe novel theory and its practical application, as well as those that demonstrate the transfer of techniques from other disciplines. It also welcomes reports on carefully conducted experimental work that is soundly interpreted. The main focus of the journal is on original and rigorous research results that have broad significance. The Catalysis section within the Chemical Engineering Journal focuses specifically on Experimental and Theoretical studies in the fields of heterogeneous catalysis, molecular catalysis, and biocatalysis. These studies have industrial impact on various sectors such as chemicals, energy, materials, foods, healthcare, and environmental protection.
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