Impact of agricultural straw open-field burning on concentrations of six criteria air pollutants in China

IF 7.3 2区 环境科学与生态学 Q1 ENVIRONMENTAL SCIENCES Environmental Pollution Pub Date : 2025-05-15 Epub Date: 2025-03-25 DOI:10.1016/j.envpol.2025.126109
Hao-Neng Huang , Zhou Yang , Yuming Guo , Jia-Jun Ma , Bo-Wen Ming , Jun Yang , Cui Guo , Li Li , Chun-Quan Ou
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Abstract

Agricultural straw open-field burning (ASOB) is a major source of fine particles and carbonaceous aerosols, particularly in China, India, and Southeast Asia. However, the exposure-lag-response relationship between straw burning and urban air pollution in China remains insufficiently investigated. This study compiled satellite-based ASOB data along with daily meteorological and air pollution monitoring data for 156 Chinese cities from 2015 to 2020. The ASOB points detected by the Moderate Resolution Imaging Spectroradiometer (MODIS) were identified as exposure events, and their exposure-lag-response relationships with daily pollutant levels were elucidated using distributed lag nonlinear models. The nation-level estimate of the impact of ASOB points on urban air quality was obtained by a meta-analysis. The results revealed significant short-term elevation in the daily concentrations of six pollutants. Each increase of 10 straw burning points is associated with an increase of 8.89, 8.52, 8.17, 2.43, and 0.84 μg/m3 in PM10, O3, PM2.5, NO2, and SO2, respectively, and an increase of 0.048 mg/m3 in CO with a lag of 0–3 days. Regional and seasonal ASOB variations and their effects were observed, revealing a pronounced effect in East China, particularly from October to December. ASOB contributed 4.54 % of O3 and 2.72 % of PM2.5 concentrations in air pollution waves in the high-intensity ASOB burning seasons. This study highlights the adverse impact of open-field straw burning on air quality, even under China's strict ASOB ban, providing scientific evidence for future assessments of the cost-effectiveness of straw-burning bans and policy refinements.

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农用秸秆露天焚烧对中国六项指标大气污染物浓度的影响
农业秸秆露天焚烧(ASOB)是细颗粒和含碳气溶胶的主要来源,特别是在中国、印度和东南亚。然而,秸秆焚烧与中国城市大气污染之间的暴露滞后反应关系研究尚不充分。该研究汇编了2015年至2020年156个中国城市的卫星ASOB数据以及每日气象和空气污染监测数据。将中分辨率成像光谱仪(MODIS)检测到的ASOB点确定为暴露事件,并利用分布滞后非线性模型阐明其与日污染物水平的暴露滞后响应关系。通过荟萃分析获得了ASOB点对城市空气质量影响的国家水平估计。结果显示,六种污染物的日浓度在短期内显著升高。每增加10个秸秆燃烧点,PM10、O3、PM2.5、NO2和SO2分别增加8.89、8.52、8.17、2.43和0.84 μg/m3, CO增加0.048 mg/m3,滞后时间为0 ~ 3 d。观测到ASOB的区域和季节变化及其影响,其中东部地区的影响最为明显,特别是10 - 12月。在ASOB高强度燃烧季节,ASOB对大气污染波中O3和PM2.5浓度的贡献分别为4.54%和2.72%。本研究强调了即使在中国严格的ASOB禁令下,露天秸秆焚烧对空气质量的不利影响,为未来评估秸秆焚烧禁令的成本效益和政策完善提供了科学依据。
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来源期刊
Environmental Pollution
Environmental Pollution 环境科学-环境科学
CiteScore
16.00
自引率
6.70%
发文量
2082
审稿时长
2.9 months
期刊介绍: Environmental Pollution is an international peer-reviewed journal that publishes high-quality research papers and review articles covering all aspects of environmental pollution and its impacts on ecosystems and human health. Subject areas include, but are not limited to: • Sources and occurrences of pollutants that are clearly defined and measured in environmental compartments, food and food-related items, and human bodies; • Interlinks between contaminant exposure and biological, ecological, and human health effects, including those of climate change; • Contaminants of emerging concerns (including but not limited to antibiotic resistant microorganisms or genes, microplastics/nanoplastics, electronic wastes, light, and noise) and/or their biological, ecological, or human health effects; • Laboratory and field studies on the remediation/mitigation of environmental pollution via new techniques and with clear links to biological, ecological, or human health effects; • Modeling of pollution processes, patterns, or trends that is of clear environmental and/or human health interest; • New techniques that measure and examine environmental occurrences, transport, behavior, and effects of pollutants within the environment or the laboratory, provided that they can be clearly used to address problems within regional or global environmental compartments.
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