首页 > 最新文献

Nuclear Energy and Technology最新文献

英文 中文
Ensuring radiation safety during dismantling, transportation and long-term storage of the SM-3 research reactor core 确保 SM-3 研究堆芯拆卸、运输和长期储存期间的辐射安全
Pub Date : 2024-03-29 DOI: 10.3897/nucet.10.123054
Anton N. Yusupov, Pavel A. Mikhailov, V. D. Kizin, Mikhail O. Gromov, Aleksei V. Kusovnikov, Vasilii V. Avdonin
Described shortly here is a procedure of demounting, removal, transport and long-term storage of the SM-3 core, based on the previous experience of reactor refurbishment undertaken in 1991. Prior to performing refurbishment, computations and calculated data analysis were performed to prove radiation safety of this work, which included estimation of the activity level for activation products in the structural materials of the nuclear research reactor core and the radiation conditions at different stages of its handling. As evidenced by the calculated data, the activity of the main dose-forming radionuclide 60Co attains equilibrium in about 12 years of radiation exposure. Taking into account the fact that the time period between two refurbishments was longer than 12 years, the calculated values of the equivalent dose rate were normalized to the radiation monitoring data obtained during the previous refurbishment, taking into account the calculated activity of 60Co radionuclide. The normalization made it possible to confirm reliability of estimates. The obtained activity data of activation products and taking into account the time spent during the SM-3 refurbishment in 1991, the radiation impact on personnel was estimated. Calculated values of the anticipated effective radiation exposure doses to the personnel engaged in the refurbishment revealed that the main limits of the personnel radiation exposure established in accordance with NRB-99/2009 were not exceeded. Comparison of the results of calculating the equivalent dose rate with the results of radiation monitoring at various points allowed us to establish that during the calculation and analytical justification of the radiation safety of work, the assessment of reflected radiation was significantly underestimated. But the radiation monitoring data, personal radiation monitoring, as well as recorded data of automatic radiation monitoring system show that all work was performed in compliance with the requirements of regulatory documents in the field of radiation safety.
根据 1991 年反应堆翻新的经验,在此简要介绍 SM-3 堆芯的拆卸、移除、运输和长期储 存程序。在进行翻新之前,进行了计算和计算数据分析,以证明这项工作的辐射安全性,其中包 括估计核研究反应堆堆芯结构材料中活化产物的活度水平,以及处理反应堆堆芯的不同 阶段的辐射条件。计算数据表明,主要剂量形成放射性核素 60Co 的放射性活度在大约 12 年的辐照时间内达到平衡。考虑到两次整修之间的间隔时间长于 12 年,等效剂量率的计算值与前一次整修期间获得的辐射监测数据进行了归一化处理,同时考虑到计算得出的 60Co 放射性核素活度。通过归一化处理,可以确认估算值的可靠性。根据所获得的活化产物活度数据,并考虑到 1991 年 SM-3 翻修期间所用的时间,估算 了对人员的辐射影响。对参与整修的人员的预期有效辐射照射剂量的计算值表明,没有超出根据 NRB-99/2009 确定的人员辐射照射的主要限值。将等效剂量率的计算结果与各点的辐射监测结果进行比较后,我们可以确定,在计算 和分析工作辐射安全的理由时,对反射辐射的评估被大大低估了。但是,辐射监测数据、个人辐射监测以及自动辐射监测系统的记录数据表明,所有工作都是按照辐射安全领域监管文件的要求进行的。
{"title":"Ensuring radiation safety during dismantling, transportation and long-term storage of the SM-3 research reactor core","authors":"Anton N. Yusupov, Pavel A. Mikhailov, V. D. Kizin, Mikhail O. Gromov, Aleksei V. Kusovnikov, Vasilii V. Avdonin","doi":"10.3897/nucet.10.123054","DOIUrl":"https://doi.org/10.3897/nucet.10.123054","url":null,"abstract":"Described shortly here is a procedure of demounting, removal, transport and long-term storage of the SM-3 core, based on the previous experience of reactor refurbishment undertaken in 1991. Prior to performing refurbishment, computations and calculated data analysis were performed to prove radiation safety of this work, which included estimation of the activity level for activation products in the structural materials of the nuclear research reactor core and the radiation conditions at different stages of its handling. As evidenced by the calculated data, the activity of the main dose-forming radionuclide 60Co attains equilibrium in about 12 years of radiation exposure. Taking into account the fact that the time period between two refurbishments was longer than 12 years, the calculated values of the equivalent dose rate were normalized to the radiation monitoring data obtained during the previous refurbishment, taking into account the calculated activity of 60Co radionuclide. The normalization made it possible to confirm reliability of estimates. The obtained activity data of activation products and taking into account the time spent during the SM-3 refurbishment in 1991, the radiation impact on personnel was estimated. Calculated values of the anticipated effective radiation exposure doses to the personnel engaged in the refurbishment revealed that the main limits of the personnel radiation exposure established in accordance with NRB-99/2009 were not exceeded.\u0000 Comparison of the results of calculating the equivalent dose rate with the results of radiation monitoring at various points allowed us to establish that during the calculation and analytical justification of the radiation safety of work, the assessment of reflected radiation was significantly underestimated. But the radiation monitoring data, personal radiation monitoring, as well as recorded data of automatic radiation monitoring system show that all work was performed in compliance with the requirements of regulatory documents in the field of radiation safety.","PeriodicalId":509190,"journal":{"name":"Nuclear Energy and Technology","volume":"22 2","pages":""},"PeriodicalIF":0.0,"publicationDate":"2024-03-29","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"140365339","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Analysis of radwaste accumulation in various scenarios of NP development 对核燃料发展的各种情况下的放射性废物积累进行分析
Pub Date : 2024-03-29 DOI: 10.3897/nucet.10.118046
Andrey A. Kashirsky, Vladimir M. Solomatin, Sergey A. Panov, E. A. Rodina, Alexander V. Egorov, Sergey A. Dmitriev, Alexey Y. Shulga
Within the framework of “Proryv” project a radiation-equivalent approach to radioactive waste management is being envisioned with U and Pu recycling and MA transmutation. Successful industry-wide implementation of the design approaches should be planned in order to avoid considerable financial and radiological encumbrances caused by the NFC final stage for two-component nuclear power system (NPS) under formation on the basis of thermal and fast reactors. In order to ensure a successful industry-wide implementation of the approaches being developed, the back-end of the NFC should not constitute considerable a financial and radiological burden for the emerging two-component nuclear power system (NPS). This article addresses the problems concerning justification of radiological and technical-and-economic feasibility of MA partitioning and subsequent transmutation in FNR. The extent of MA accumulation as a result of TNR SNF reprocessing confirms the need for the introduction of MA partitioning technologies not only at all reprocessing plants planned for commissioning, but also at the plants now in operation. Based on available data, the study has shown that the implementation of the closed NFC with FNR contributes to significant reduction in the cost of disposal of radwaste compared to the scenario based exclusively on the development of VVER and open fuel cycle technologies. Recycling plutonium in fast reactors should be implemented in conjunction with MA to address environmental, non-proliferation and economic concerns of the back-end of advanced NFC. Within the scale of the future nuclear power system in Russia, an option such as this can only be realized on the basis of developing a FNR fleet.
在 "Proryv "项目的框架内,设想了一种放射性废物管理的辐射等效方法,即铀和钚的再循环以及 MA 的嬗变。应计划在全行业成功实施这些设计方法,以避免在热堆和快堆基础上正在形成的双组分核电系统(NPS)的 NFC 最后阶段造成巨大的财政和放射性负担。为确保在全行业范围内成功实施正在开发的方法,NFC 的后端不应对正在形成的双组分核电系统(NPS)构成相当大的财务和放射性负担。本文探讨了在 FNR 中对 MA 进行分区和随后的嬗变在辐射和技术经济上是否可行的问题。TNR SNF 后处理造成的 MA 累积程度证明,不仅计划投产的所有后处理厂需要采用 MA 分离技术,而且目前正在运行的后处理厂也需要采用这种技术。根据现有数据,研究表明,与完全基于开发 VVER 和开放式燃料循环技术的方案相比,实施封闭式 NFC 和 FNR 有助于大幅降低放射性废物的处置成本。在快堆中回收钚应与千年生态系统评估一起实施,以解决先进核燃料循环后端的环境、防扩散和经济问题。在俄罗斯未来核电系统的规模范围内,只有在发展快堆群的基础上才能实现这样的方案。
{"title":"Analysis of radwaste accumulation in various scenarios of NP development","authors":"Andrey A. Kashirsky, Vladimir M. Solomatin, Sergey A. Panov, E. A. Rodina, Alexander V. Egorov, Sergey A. Dmitriev, Alexey Y. Shulga","doi":"10.3897/nucet.10.118046","DOIUrl":"https://doi.org/10.3897/nucet.10.118046","url":null,"abstract":"Within the framework of “Proryv” project a radiation-equivalent approach to radioactive waste management is being envisioned with U and Pu recycling and MA transmutation. Successful industry-wide implementation of the design approaches should be planned in order to avoid considerable financial and radiological encumbrances caused by the NFC final stage for two-component nuclear power system (NPS) under formation on the basis of thermal and fast reactors. In order to ensure a successful industry-wide implementation of the approaches being developed, the back-end of the NFC should not constitute considerable a financial and radiological burden for the emerging two-component nuclear power system (NPS).\u0000 This article addresses the problems concerning justification of radiological and technical-and-economic feasibility of MA partitioning and subsequent transmutation in FNR. The extent of MA accumulation as a result of TNR SNF reprocessing confirms the need for the introduction of MA partitioning technologies not only at all reprocessing plants planned for commissioning, but also at the plants now in operation. Based on available data, the study has shown that the implementation of the closed NFC with FNR contributes to significant reduction in the cost of disposal of radwaste compared to the scenario based exclusively on the development of VVER and open fuel cycle technologies. Recycling plutonium in fast reactors should be implemented in conjunction with MA to address environmental, non-proliferation and economic concerns of the back-end of advanced NFC. Within the scale of the future nuclear power system in Russia, an option such as this can only be realized on the basis of developing a FNR fleet.","PeriodicalId":509190,"journal":{"name":"Nuclear Energy and Technology","volume":"57 5","pages":""},"PeriodicalIF":0.0,"publicationDate":"2024-03-29","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"140367351","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Computational substantiation of technological characteristics of the closure stage of nuclear fuel cycle using code VIZART 利用 VIZART 代码对核燃料循环关闭阶段的技术特征进行计算论证
Pub Date : 2024-03-29 DOI: 10.3897/nucet.10.123052
Inga R. Makeyeva, Vasiliy Yu. Pugachev, Olga V. Shmidt, A. А. Rykunova, Andrey Yu. Shadrin
There exist different variants of organizing the closure of nuclear fuel cycle (CNFC) depending on fast reactor type, fuel types, station or centralized allocation of closed nuclear fuel cycle stages. One of the ways to verify and estimate engineering solution is mathematical modeling of radiochemical technology which in the end will allow to optimize composite technological process in order to increase effectiveness and reduce cost. In order to calculate the balance of material flows of process circuits and individual production sections in the stationary and dynamic modes, with taking into account the isotopic composition evolution, a software package VIZART (Virtual Plant of Radiochemical Technologies) was developed, allowing the user to assemble the required sequence of operations for any part of the process scheme and perform the calculation of material balance for all flows of the circuit, as well as to optimize the equipment operating modes and provide the necessary data to justify the safety of certain limits and the entire process circuit. The following capabilities of code VIZART for computational substantiation of CNFC technology design and characteristics are considered: material balance calculation, cyclogram creation, determination of the most loaded parts of processing lines, estimation of fissile materials accumulating in devices and intermediate vessels, optimization of productivity of nodes and devices.
根据快堆类型、燃料类型、站或集中分配核燃料循环闭合阶段,核燃料循环闭合(CNFC)有不同的组织形式。对放射化学技术进行数学建模是验证和估算工程解决方案的方法之一,最终可以优化复合技术流程,以提高效率和降低成本。为了计算工艺回路和单个生产部分在静态和动态模式下的物料流平衡,同时考虑到同位素成分的演变,开发了一个软件包 VIZART(放射化学技术虚拟工厂),允许用户为工艺方案的任何部分组合所需的操作顺序,并对回路的所有物料流进行物料平衡计算,以及优化设备运行模式,并提供必要的数据来证明某些限制和整个工艺回路的安全性。VIZART 代码在计算证明 CNFC 技术设计和特性方面具有以下功能:物料平衡计算、循环图创建、确定加工生产线中负荷最大的部分、估算设备和中间容器中积聚的裂变材料、优化节点和设备的生产率。
{"title":"Computational substantiation of technological characteristics of the closure stage of nuclear fuel cycle using code VIZART","authors":"Inga R. Makeyeva, Vasiliy Yu. Pugachev, Olga V. Shmidt, A. А. Rykunova, Andrey Yu. Shadrin","doi":"10.3897/nucet.10.123052","DOIUrl":"https://doi.org/10.3897/nucet.10.123052","url":null,"abstract":"There exist different variants of organizing the closure of nuclear fuel cycle (CNFC) depending on fast reactor type, fuel types, station or centralized allocation of closed nuclear fuel cycle stages. One of the ways to verify and estimate engineering solution is mathematical modeling of radiochemical technology which in the end will allow to optimize composite technological process in order to increase effectiveness and reduce cost. In order to calculate the balance of material flows of process circuits and individual production sections in the stationary and dynamic modes, with taking into account the isotopic composition evolution, a software package VIZART (Virtual Plant of Radiochemical Technologies) was developed, allowing the user to assemble the required sequence of operations for any part of the process scheme and perform the calculation of material balance for all flows of the circuit, as well as to optimize the equipment operating modes and provide the necessary data to justify the safety of certain limits and the entire process circuit. The following capabilities of code VIZART for computational substantiation of CNFC technology design and characteristics are considered: material balance calculation, cyclogram creation, determination of the most loaded parts of processing lines, estimation of fissile materials accumulating in devices and intermediate vessels, optimization of productivity of nodes and devices.","PeriodicalId":509190,"journal":{"name":"Nuclear Energy and Technology","volume":"33 4","pages":""},"PeriodicalIF":0.0,"publicationDate":"2024-03-29","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"140367385","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
An analysis of the “Fast” noise measurements of the dynamic VVER processes 动态 VVER 过程的 "快速 "噪声测量分析
Pub Date : 2024-03-29 DOI: 10.3897/nucet.10.123398
G. V. Arkadov, V. Pavelko, M. T. Slepov
Studies of maneuverable modes of VVER to confirm the possibility of participation of nuclear power plants in the mode of daily carrying capacity have been conducted for quite a long time. Tests at various nuclear power plants with VVER-1000 (Zaporizhzhia NPP in 1998, Khmelnitsky NPP in 2005, Tianwan NPP in 2007) have shown the practical possibility of NPP participation in the daily schedule of carrying capacity, however, the commissioning of nuclear power plants with VVER-1200 requires similar work on all new units with VVER-1200: NVAES-2, LNPP-2 Belarusian NPP. The article presents some aspects of the use of noise control methods for analyzing the condition of equipment and the core. Since the emergence of the technology of noise analysis of signals from VVER reactor installations, researchers have formulated several criteria for obtaining results of appropriate quality. The fundamental requirement for conducting noise experiments was the registration of data in stationary modes of operation of power units, since any non-stationarity made significant changes in spectral estimates, which ultimately complicated the work and “distorted” the results obtained. This requirement was included in the operating instructions of various diagnostic systems using noise signal analysis methods (the SUS system, manufactured by Siemens). For a long period of time, the current situation suited both developers of various diagnostic systems and NPP personnel operating them at power units. On the one hand, this was due to the imperfection of the technical means used (low speed of analog-to-digital converters, limited storage capacity, bulky equipment, etc.), on the other hand, the use of domestic NPP power units only in the base load mode without tracking daily power fluctuations in the power system. The standard archives of the upper block level system, the in-reactor control system and additionally produced multi-channel “fast” measurements with a frequency of 1 kHz for the analysis of maneuverable mode 95-55-95% of the VVER-1200 reactor plant were analyzed. Global disturbances of the core have been detected after one step of the regulatory body of the control and protection system, which attenuates within one second if the next step of the control and protection system has not occurred during this time. Such fast neutron processes can be controlled only by neutron-noise measurements with an upper frequency of at least 20 Hz.
为确认核电站参与日常运载能力模式的可能性而对 VVER 的可操纵模式进行的研究已经进行了很长时间。在各核电站进行的 VVER-1000 试验(1998 年在 Zaporizhzhia 核电站、2005 年在 Khmelnitsky 核电站、2007 年在田湾核电站)表明,核电站参与日常运载能力计划是切实可行的,但是,VVER-1200 核电站的调试需要对所有新的 VVER-1200 机组进行类似的工作:NVAES-2、LNPP-2 白俄罗斯核电厂。文章介绍了使用噪声控制方法分析设备和堆芯状况的一些方面。自 VVER 反应堆装置信号噪声分析技术出现以来,研究人员已制定了获得适当质量结果的若干标准。进行噪声实验的基本要求是在动力装置的静态运行模式下登记数据,因为任何非静态都会使频谱估计值发生重大变化,最终使工作复杂化并 "扭曲 "所获得的结果。这一要求已被纳入使用噪声信号分析方法的各种诊断系统(西门子公司生产的 SUS 系统)的操作说明书中。在很长一段时间内,目前的状况既适合各种诊断系统的开发人员,也适合在发电厂操作这些系统的国家核电厂工作人员。一方面,这是由于所使用的技术手段不完善(模数转换器速度低、存储容量有限、设备笨重等),另一方面,国内核电厂机组仅在基本负荷模式下使用,而不跟踪电力系统的日常功率波动。为了分析 VVER-1200 反应堆厂房 95-55-95% 的可操纵模式,分析了上部模块级系统的标准档案、反应堆内控制系统以及额外制作的频率为 1 kHz 的多通道 "快速 "测量。在控制和保护系统的调节机构执行一个步骤后,堆芯的全局扰动被检测到,如果控制和保护系统的下一个步骤在此期间没有发生,扰动会在一秒钟内减弱。这种快中子过程只能通过频率上限至少为 20 赫兹的中子噪声测量来控制。
{"title":"An analysis of the “Fast” noise measurements of the dynamic VVER processes","authors":"G. V. Arkadov, V. Pavelko, M. T. Slepov","doi":"10.3897/nucet.10.123398","DOIUrl":"https://doi.org/10.3897/nucet.10.123398","url":null,"abstract":"Studies of maneuverable modes of VVER to confirm the possibility of participation of nuclear power plants in the mode of daily carrying capacity have been conducted for quite a long time. Tests at various nuclear power plants with VVER-1000 (Zaporizhzhia NPP in 1998, Khmelnitsky NPP in 2005, Tianwan NPP in 2007) have shown the practical possibility of NPP participation in the daily schedule of carrying capacity, however, the commissioning of nuclear power plants with VVER-1200 requires similar work on all new units with VVER-1200: NVAES-2, LNPP-2 Belarusian NPP. The article presents some aspects of the use of noise control methods for analyzing the condition of equipment and the core.\u0000 Since the emergence of the technology of noise analysis of signals from VVER reactor installations, researchers have formulated several criteria for obtaining results of appropriate quality. The fundamental requirement for conducting noise experiments was the registration of data in stationary modes of operation of power units, since any non-stationarity made significant changes in spectral estimates, which ultimately complicated the work and “distorted” the results obtained. This requirement was included in the operating instructions of various diagnostic systems using noise signal analysis methods (the SUS system, manufactured by Siemens). For a long period of time, the current situation suited both developers of various diagnostic systems and NPP personnel operating them at power units. On the one hand, this was due to the imperfection of the technical means used (low speed of analog-to-digital converters, limited storage capacity, bulky equipment, etc.), on the other hand, the use of domestic NPP power units only in the base load mode without tracking daily power fluctuations in the power system.\u0000 The standard archives of the upper block level system, the in-reactor control system and additionally produced multi-channel “fast” measurements with a frequency of 1 kHz for the analysis of maneuverable mode 95-55-95% of the VVER-1200 reactor plant were analyzed. Global disturbances of the core have been detected after one step of the regulatory body of the control and protection system, which attenuates within one second if the next step of the control and protection system has not occurred during this time. Such fast neutron processes can be controlled only by neutron-noise measurements with an upper frequency of at least 20 Hz.","PeriodicalId":509190,"journal":{"name":"Nuclear Energy and Technology","volume":"13 8","pages":""},"PeriodicalIF":0.0,"publicationDate":"2024-03-29","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"140367457","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Experience in the production of 99Mo from low enriched uranium at the VVR-ts research nuclear facility 在 VVR-ts 研究核设施利用低浓铀生产 99Mo 的经验
Pub Date : 2024-03-26 DOI: 10.3897/nucet.10.122284
O. Kochnov, Valery I. Stepanov, D. A. Pakholik, Valery V. Kolesov, Evgeny V. Nikulin
The key industrial method for producing 99Mo is production of the radionuclide as one of the 235U fission fragments. 235U is irradiated with neutrons in a nuclear reactor (both heterogeneous and homogeneous nuclear reactors can be used) and then processed in radiochemical laboratories, where 99Mo is chemically extracted from fission products. Both highly enriched uranium (HEU) and low enriched uranium (LEU) can be used to produce 99Mo by the fragmentation method. To date, almost all world producers, with the exception of Russia, are either in the final stages of transferring production from highly enriched uranium to low enriched uranium, or are already producing 99Mo using LEU. This is due to the problems of non-proliferation of nuclear materials and the prevention of the likelihood of terrorist threats. A number of experimental studies have been carried out on the basis of the VVR-ts research reactor. Experimental studies included the study of the effect of LEU targets on the reactivity reserve of the VVR-ts reactor, irradiation of these targets in experimental channels and separation of 99Mo from them. The paper presents the results of producing and separating 99Mo from targets with LEU material. It is shown that it is necessary to improve the processing technology to increase the production of fragmented 99Mo from LEU.
生产 99Mo 的主要工业方法是生产作为 235U 裂变碎片之一的放射性核素。235U 在核反应堆(可使用异质和均质核反应堆)中接受中子辐照,然后在放射化学实验室进行处理,从裂变产物中化学提取 99Mo。高浓缩铀(HEU)和低浓缩铀(LEU)都可用于通过破碎法生产 99Mo。迄今为止,除俄罗斯外,世界上几乎所有生产国要么正处于从高浓铀向低浓铀转移生产的最后阶段,要么已经在使用低浓铀生产 99Mo。这是由于核材料的不扩散问题和防止恐怖主义威胁的可能性。在 VVR-ts 研究反应堆的基础上进行了多项实验研究。实验研究包括研究 LEU 靶件对 VVR-ts 反应堆反应储备的影响、在实验通道中辐照这些靶件以及从中分离 99Mo。论文介绍了用低浓铀材料从靶件中生产和分离 99Mo 的结果。结果表明,有必要改进处理技术,以提高从 LEU 中生产碎片 99Mo的能力。
{"title":"Experience in the production of 99Mo from low enriched uranium at the VVR-ts research nuclear facility","authors":"O. Kochnov, Valery I. Stepanov, D. A. Pakholik, Valery V. Kolesov, Evgeny V. Nikulin","doi":"10.3897/nucet.10.122284","DOIUrl":"https://doi.org/10.3897/nucet.10.122284","url":null,"abstract":"The key industrial method for producing 99Mo is production of the radionuclide as one of the 235U fission fragments. 235U is irradiated with neutrons in a nuclear reactor (both heterogeneous and homogeneous nuclear reactors can be used) and then processed in radiochemical laboratories, where 99Mo is chemically extracted from fission products. Both highly enriched uranium (HEU) and low enriched uranium (LEU) can be used to produce 99Mo by the fragmentation method. To date, almost all world producers, with the exception of Russia, are either in the final stages of transferring production from highly enriched uranium to low enriched uranium, or are already producing 99Mo using LEU. This is due to the problems of non-proliferation of nuclear materials and the prevention of the likelihood of terrorist threats. A number of experimental studies have been carried out on the basis of the VVR-ts research reactor. Experimental studies included the study of the effect of LEU targets on the reactivity reserve of the VVR-ts reactor, irradiation of these targets in experimental channels and separation of 99Mo from them. The paper presents the results of producing and separating 99Mo from targets with LEU material. It is shown that it is necessary to improve the processing technology to increase the production of fragmented 99Mo from LEU.","PeriodicalId":509190,"journal":{"name":"Nuclear Energy and Technology","volume":"121 43","pages":""},"PeriodicalIF":0.0,"publicationDate":"2024-03-26","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"140380062","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Enhancing the efficiency of the MOX fuel cycle for VVER-1200 using burnable absorbers 利用可燃吸收剂提高 VVER-1200 的 MOX 燃料循环效率
Pub Date : 2023-11-16 DOI: 10.3897/nucet.9.98689
Joy Ozoani, Yuri Volkov
Margin adoption in a nuclear power plant (NPP) design is a frequent approach to strengthen the design’s robustness and provide an efficient way to handle uncertainties. However, the current trend of increasing fuel enrichment, including the use of MOX fuel to achieve a higher burnup, leads to non-uniformity in the energy release (power peaking factor) at the level of the fuel rod lattice, thereby causing a great effect on the reactor margins. One of the ways to reduce the power peaking factor is the use of burnable absorbers (BAs) which helps to minimize the power peaking factor. This work aims at enhancing the efficiency of the MOX fuel cycle for VVER-1200 reactor by replacing the Gadolinium burnable absorber to Erbia burnable absorber.
在核电站(NPP)设计中采用裕度是加强设计稳健性的常用方法,也是处理不确定性的有效途径。然而,当前燃料浓缩度不断提高的趋势,包括使用 MOX 燃料以获得更高的燃烧度,导致燃料棒晶格层面的能量释放(功率峰值因数)不均匀,从而对反应堆裕度产生了巨大影响。降低功率峰值因数的方法之一是使用可燃吸收剂(BA),这有助于最大限度地降低功率峰值因数。这项工作旨在通过将钆可燃吸收剂替换为埃比亚可燃吸收剂,提高 VVER-1200 反应堆 MOX 燃料循环的效率。
{"title":"Enhancing the efficiency of the MOX fuel cycle for VVER-1200 using burnable absorbers","authors":"Joy Ozoani, Yuri Volkov","doi":"10.3897/nucet.9.98689","DOIUrl":"https://doi.org/10.3897/nucet.9.98689","url":null,"abstract":"Margin adoption in a nuclear power plant (NPP) design is a frequent approach to strengthen the design’s robustness and provide an efficient way to handle uncertainties. However, the current trend of increasing fuel enrichment, including the use of MOX fuel to achieve a higher burnup, leads to non-uniformity in the energy release (power peaking factor) at the level of the fuel rod lattice, thereby causing a great effect on the reactor margins. One of the ways to reduce the power peaking factor is the use of burnable absorbers (BAs) which helps to minimize the power peaking factor. This work aims at enhancing the efficiency of the MOX fuel cycle for VVER-1200 reactor by replacing the Gadolinium burnable absorber to Erbia burnable absorber.","PeriodicalId":509190,"journal":{"name":"Nuclear Energy and Technology","volume":"11 5","pages":""},"PeriodicalIF":0.0,"publicationDate":"2023-11-16","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"139268644","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
期刊
Nuclear Energy and Technology
全部 Acc. Chem. Res. ACS Applied Bio Materials ACS Appl. Electron. Mater. ACS Appl. Energy Mater. ACS Appl. Mater. Interfaces ACS Appl. Nano Mater. ACS Appl. Polym. Mater. ACS BIOMATER-SCI ENG ACS Catal. ACS Cent. Sci. ACS Chem. Biol. ACS Chemical Health & Safety ACS Chem. Neurosci. ACS Comb. Sci. ACS Earth Space Chem. ACS Energy Lett. ACS Infect. Dis. ACS Macro Lett. ACS Mater. Lett. ACS Med. Chem. Lett. ACS Nano ACS Omega ACS Photonics ACS Sens. ACS Sustainable Chem. Eng. ACS Synth. Biol. Anal. Chem. BIOCHEMISTRY-US Bioconjugate Chem. BIOMACROMOLECULES Chem. Res. Toxicol. Chem. Rev. Chem. Mater. CRYST GROWTH DES ENERG FUEL Environ. Sci. Technol. Environ. Sci. Technol. Lett. Eur. J. Inorg. Chem. IND ENG CHEM RES Inorg. Chem. J. Agric. Food. Chem. J. Chem. Eng. Data J. Chem. Educ. J. Chem. Inf. Model. J. Chem. Theory Comput. J. Med. Chem. J. Nat. Prod. J PROTEOME RES J. Am. Chem. Soc. LANGMUIR MACROMOLECULES Mol. Pharmaceutics Nano Lett. Org. Lett. ORG PROCESS RES DEV ORGANOMETALLICS J. Org. Chem. J. Phys. Chem. J. Phys. Chem. A J. Phys. Chem. B J. Phys. Chem. C J. Phys. Chem. Lett. Analyst Anal. Methods Biomater. Sci. Catal. Sci. Technol. Chem. Commun. Chem. Soc. Rev. CHEM EDUC RES PRACT CRYSTENGCOMM Dalton Trans. Energy Environ. Sci. ENVIRON SCI-NANO ENVIRON SCI-PROC IMP ENVIRON SCI-WAT RES Faraday Discuss. Food Funct. Green Chem. Inorg. Chem. Front. Integr. Biol. J. Anal. At. Spectrom. J. Mater. Chem. A J. Mater. Chem. B J. Mater. Chem. C Lab Chip Mater. Chem. Front. Mater. Horiz. MEDCHEMCOMM Metallomics Mol. Biosyst. Mol. Syst. Des. Eng. Nanoscale Nanoscale Horiz. Nat. Prod. Rep. New J. Chem. Org. Biomol. Chem. Org. Chem. Front. PHOTOCH PHOTOBIO SCI PCCP Polym. Chem.
×
引用
GB/T 7714-2015
复制
MLA
复制
APA
复制
导出至
BibTeX EndNote RefMan NoteFirst NoteExpress
×
0
微信
客服QQ
Book学术公众号 扫码关注我们
反馈
×
意见反馈
请填写您的意见或建议
请填写您的手机或邮箱
×
提示
您的信息不完整,为了账户安全,请先补充。
现在去补充
×
提示
您因"违规操作"
具体请查看互助需知
我知道了
×
提示
现在去查看 取消
×
提示
确定
Book学术官方微信
Book学术文献互助
Book学术文献互助群
群 号:481959085
Book学术
文献互助 智能选刊 最新文献 互助须知 联系我们:info@booksci.cn
Book学术提供免费学术资源搜索服务,方便国内外学者检索中英文文献。致力于提供最便捷和优质的服务体验。
Copyright © 2023 Book学术 All rights reserved.
ghs 京公网安备 11010802042870号 京ICP备2023020795号-1