Pub Date : 2023-01-24DOI: 10.1021/acssuschemeng.2c07413
Chengfeng Shen, Xue Zhao, Yuwei Long, Wenli An, Xuelian Zhou, Xuehui Liu, Shimei Xu, Yu-zhong Wang
{"title":"Approach for the Low Carbon Footprint of Biodegradable Plastic PBAT: Complete Recovery of Its Every Monomer via High-Efficiency Hydrolysis and Separation","authors":"Chengfeng Shen, Xue Zhao, Yuwei Long, Wenli An, Xuelian Zhou, Xuehui Liu, Shimei Xu, Yu-zhong Wang","doi":"10.1021/acssuschemeng.2c07413","DOIUrl":"https://doi.org/10.1021/acssuschemeng.2c07413","url":null,"abstract":"","PeriodicalId":131518,"journal":{"name":"ACS Sustainable Chemistry & Engineering","volume":"98 ","pages":"0"},"PeriodicalIF":0.0,"publicationDate":"2023-01-24","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"117432929","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2023-01-19DOI: 10.1021/acssuschemeng.2c06668
Harald Silau, A. Melas, K. Dam‐Johansen, Hao Wu, A. Daugaard, M. Høj
{"title":"Solvent Fractionation and Depolymerization Provide Liquid Lignin Fractions Exploited as Bio-based Aromatic Building Blocks in Epoxies","authors":"Harald Silau, A. Melas, K. Dam‐Johansen, Hao Wu, A. Daugaard, M. Høj","doi":"10.1021/acssuschemeng.2c06668","DOIUrl":"https://doi.org/10.1021/acssuschemeng.2c06668","url":null,"abstract":"","PeriodicalId":131518,"journal":{"name":"ACS Sustainable Chemistry & Engineering","volume":"177 39","pages":"0"},"PeriodicalIF":0.0,"publicationDate":"2023-01-19","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"117436510","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2023-01-18DOI: 10.1021/acssuschemeng.2c06876
Luoxi Tan, H. L. Scott, M. Smith, S. Pingali, H. O’Neill, J. Morrell-Falvey, J. Katsaras, Jeremy C. Smith, B. Davison, J. Elkins, J. Nickels
{"title":"Amphiphilic Co-Solvents Modulate the Structure of Membrane Domains","authors":"Luoxi Tan, H. L. Scott, M. Smith, S. Pingali, H. O’Neill, J. Morrell-Falvey, J. Katsaras, Jeremy C. Smith, B. Davison, J. Elkins, J. Nickels","doi":"10.1021/acssuschemeng.2c06876","DOIUrl":"https://doi.org/10.1021/acssuschemeng.2c06876","url":null,"abstract":"","PeriodicalId":131518,"journal":{"name":"ACS Sustainable Chemistry & Engineering","volume":"70 1","pages":"0"},"PeriodicalIF":0.0,"publicationDate":"2023-01-18","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"117615476","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2023-01-11DOI: 10.1021/acssuschemeng.2c05936
H. Jo, Hanna Yu, Huijin Cheon, Jun-Hong Kim, G. Kim, Byoung Sik Kim, Jeong-Sun Kim, Jin‐Byung Park
{"title":"Multilayer Engineering of an Escherichia coli-Based Biotransformation System to Exclusively Produce Glycolic Acid from Formaldehyde","authors":"H. Jo, Hanna Yu, Huijin Cheon, Jun-Hong Kim, G. Kim, Byoung Sik Kim, Jeong-Sun Kim, Jin‐Byung Park","doi":"10.1021/acssuschemeng.2c05936","DOIUrl":"https://doi.org/10.1021/acssuschemeng.2c05936","url":null,"abstract":"","PeriodicalId":131518,"journal":{"name":"ACS Sustainable Chemistry & Engineering","volume":"164 1","pages":"0"},"PeriodicalIF":0.0,"publicationDate":"2023-01-11","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"119753894","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2022-12-23DOI: 10.1021/acssuschemeng.2c06266
Heather O. LeClerc, Jeffrey R. Page, G. Tompsett, Sydney F. Niles, A. McKenna, J. Valla, M. Timko, Andrew R. Teixeira
GC-MS Methodology. Gas chromatography mass spectrometry was performed using an Agilent 6890N gas chromatogram equipped with an Agilent 5973N mass spectrometer. Samples were diluted 1:100 in acetone before injection of 0.5µL at a 25:1 split ratio with constant flow of helium carrier gas. Inlet temperature was set to 270 °C. The oven was initially heated to 40 °C and utilized a ramp of 10 °C/min to a temperature of 170 °C before reducing the ramp rate to 3 °C until a final temperature of 270 °C was reached. The column utilized was an HP-5. (+) APPI FT-ICR MS Methodology. Biocrude (and aqueous) samples were diluted in (50/50, by volume) toluene/tetrahydrofuran (THF) to a concentration of 125 µg/mL for analysis by positive-ion (+) atmospheric pressure photoionization (APPI) Fourier transform ion cyclotron resonance mass spectrometry (FT-ICR MS) at 21 tesla. Toluene and THF increased the ionization efficiency of nonpolar aromatic compounds 1, 2 through charge exchange, 3, 4 and proton transfer 5 reactions between ionized toluene molecules and neutral analyte molecules. An atmospheric pressure photoionization (APPI) source (Thermo-Fisher Scientific, San Jose, CA) was coupled to the first stage
gc - ms方法。气相色谱质谱分析使用安捷伦6890N气相色谱仪和安捷伦5973N质谱仪。样品在丙酮中稀释1:100后，以25:1的分割比注入0.5µL，恒流氦气载气。入口温度设置为270°C。烘箱最初加热到40°C，并利用10°C/min的斜坡温度到170°C，然后将斜坡速度降低到3°C，直到达到270°C的最终温度。所使用的色谱柱是HP-5。(+) APPI FT-ICR质谱方法。生物原油(和水溶液)样品在甲苯/四氢呋喃(THF)中(按体积计算为50/50)稀释至125µg/mL，采用21特斯拉正离子(+)大气压光电离(APPI)傅立叶变换离子回旋共振质谱(FT-ICR MS)进行分析。甲苯和四氢呋喃通过电离后的甲苯分子与中性分析物分子之间的电荷交换、3、4和质子转移5反应，提高了非极性芳香族化合物1、2的电离效率。一个大气压光电离(APPI)源(thermofisher Scientific, San Jose, CA)耦合到第一级
{"title":"Emergent Chemical Behavior in Mixed Food and Lignocellulosic Green Waste Hydrothermal Liquefaction","authors":"Heather O. LeClerc, Jeffrey R. Page, G. Tompsett, Sydney F. Niles, A. McKenna, J. Valla, M. Timko, Andrew R. Teixeira","doi":"10.1021/acssuschemeng.2c06266","DOIUrl":"https://doi.org/10.1021/acssuschemeng.2c06266","url":null,"abstract":"GC-MS Methodology. Gas chromatography mass spectrometry was performed using an Agilent 6890N gas chromatogram equipped with an Agilent 5973N mass spectrometer. Samples were diluted 1:100 in acetone before injection of 0.5µL at a 25:1 split ratio with constant flow of helium carrier gas. Inlet temperature was set to 270 °C. The oven was initially heated to 40 °C and utilized a ramp of 10 °C/min to a temperature of 170 °C before reducing the ramp rate to 3 °C until a final temperature of 270 °C was reached. The column utilized was an HP-5. (+) APPI FT-ICR MS Methodology. Biocrude (and aqueous) samples were diluted in (50/50, by volume) toluene/tetrahydrofuran (THF) to a concentration of 125 µg/mL for analysis by positive-ion (+) atmospheric pressure photoionization (APPI) Fourier transform ion cyclotron resonance mass spectrometry (FT-ICR MS) at 21 tesla. Toluene and THF increased the ionization efficiency of nonpolar aromatic compounds 1, 2 through charge exchange, 3, 4 and proton transfer 5 reactions between ionized toluene molecules and neutral analyte molecules. An atmospheric pressure photoionization (APPI) source (Thermo-Fisher Scientific, San Jose, CA) was coupled to the first stage","PeriodicalId":131518,"journal":{"name":"ACS Sustainable Chemistry & Engineering","volume":"237 1","pages":"0"},"PeriodicalIF":0.0,"publicationDate":"2022-12-23","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"118071361","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2022-12-02DOI: 10.1021/acssuschemeng.2c04954
A. M. Borrero-López, A. Celzard, V. Fierro
{"title":"Eco-Friendly Production of Hyper-Cross-Linked Polymers Using Mechanosynthesis and Bioresources: A Critical Review","authors":"A. M. Borrero-López, A. Celzard, V. Fierro","doi":"10.1021/acssuschemeng.2c04954","DOIUrl":"https://doi.org/10.1021/acssuschemeng.2c04954","url":null,"abstract":"","PeriodicalId":131518,"journal":{"name":"ACS Sustainable Chemistry & Engineering","volume":"54 1","pages":"0"},"PeriodicalIF":0.0,"publicationDate":"2022-12-02","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"119566966","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
{"title":"A Simple, Low-Cost, and Green Method for Preparing Strong, Tough, and Ductile Poly(lactic acid) Materials with Good Transparency and Heat Resistance","authors":"Tairong Kuang, Jingbing Zhang, F. Chen, Yanpei Fei, Hongfu Zhou, Yunxuan Weng, Tong Liu, Jintao Yang, Mingqiang Zhong","doi":"10.1021/acssuschemeng.2c05613","DOIUrl":"https://doi.org/10.1021/acssuschemeng.2c05613","url":null,"abstract":"","PeriodicalId":131518,"journal":{"name":"ACS Sustainable Chemistry & Engineering","volume":"64 2 1","pages":"0"},"PeriodicalIF":0.0,"publicationDate":"2022-11-30","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"119466849","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2022-11-29DOI: 10.1021/acssuschemeng.2c04327
Haiqiu Jiang, Lingling Wang, Qian Liu, Q. Lu, R. Cheng, Keming Zhan, Hui Wan, Long Yang, G. Du, Wei Gao
{"title":"Superhydrophobic Poplar Scrimber Via In Situ Synthesis of Cu7Cl4(OH)10·H2O Heterostructure Inspired by Pine Cone with Superultraviolet Resistance","authors":"Haiqiu Jiang, Lingling Wang, Qian Liu, Q. Lu, R. Cheng, Keming Zhan, Hui Wan, Long Yang, G. Du, Wei Gao","doi":"10.1021/acssuschemeng.2c04327","DOIUrl":"https://doi.org/10.1021/acssuschemeng.2c04327","url":null,"abstract":"","PeriodicalId":131518,"journal":{"name":"ACS Sustainable Chemistry & Engineering","volume":"7 1","pages":"0"},"PeriodicalIF":0.0,"publicationDate":"2022-11-29","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"120631993","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2022-11-23DOI: 10.1021/acssuschemeng.2c05094
Tian Fei, H. Yi, R. Zboray, Xiao-Qiang Yan, Si-Si Song, Lei Ren, Huizhang Guo, Yuanyan Jiang
{"title":"Bioinspired Enzymatic Mineralization Incorporates CaCO3 Mesocrystals in Wood for Surface Reinforcement and Flame-Retardancy","authors":"Tian Fei, H. Yi, R. Zboray, Xiao-Qiang Yan, Si-Si Song, Lei Ren, Huizhang Guo, Yuanyan Jiang","doi":"10.1021/acssuschemeng.2c05094","DOIUrl":"https://doi.org/10.1021/acssuschemeng.2c05094","url":null,"abstract":"","PeriodicalId":131518,"journal":{"name":"ACS Sustainable Chemistry & Engineering","volume":"17 1","pages":"0"},"PeriodicalIF":0.0,"publicationDate":"2022-11-23","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"119965551","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
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