Isotopes in Environmental and Health Studies最新文献

In Germany, river monitoring for tritium started in the early 1970s. Today this monitoring network consists of 50 stations and includes stable isotopes. The stable isotope time series to the end of 2021 are at least four years and for some stations up to 30 years long. Daily river water samples were collected during an extraordinary dry season from October 2018 until end of January 2019 from six selected stations of the Rhine and five stations of the Elbe basin. The most dominating stable isotope effects in river water are the seasonal and altitude effects, but also a continental effect is visible. The isotopes indicate snow and ice melt contributions in the Rhine and Danube during the summer months and a consecutive dilution of these signals by mixing with tributary rivers. Close to the coasts in northern Germany, stable isotope patterns reflect influence of seawater and tides. Daily patterns during the dry season 2018/2019 surprisingly do not exhibit extreme changes but rather trends of enhanced groundwater contribution. Long-term continual data across scales are important for comparing and identifying hydrological processes in German river basins of different size and mean catchment altitudes, and highlight the benefits of a co-organized national network.

Although stable hydrogen (δ²H) and carbon (δ¹³C) isotopic compositions of bird feathers have been increasingly used to understand the migration of birds through assignment of individuals to established isoscapes, far less is known about the structure of feather isoscapes based on stable sulphur isotope (δ³⁴S) assays. While δ²H isoscapes have been used to investigate the migratory origins of the Globe Skimmer (Pantala flavescens) dragonfly in India, no isotope studies have been applied to avian migration patterns in that region. Here, based on museum collections, we report the feather δ³⁴S values of 13 avian species that included marine birds with expected ³⁴S enriched feathers, resident birds throughout India and a single migratory species, Bar-headed Goose (Anser indicus). Feathers from the marine birds were the most enriched (20.6 ± 1.2 ‰, n = 10; range = 4.4 ‰) in ³⁴S but terrestrial resident species also showed unexpectedly high δ³⁴S values (11.7 ± 4.8 ‰, n = 74; range = 19.9 ‰) throughout most of India but the Himalayan region and Gangetic plain typically showed δ³⁴S values less than 6.4 ‰. Our results show the utility of feather δ³⁴S studies to decipher avian and other animal migration between these two regions.

Soil gas radon and indoor radon measurements have been carried out in Mayo-Louti and Benoué Divisions in northern Cameroon. Concentrations of radon in soil have been measured using Markus 10 at the depth of about 1 m. Radon concentration in soil varies from 0.9 to 13.8 kBq m^-3 with a mean value of 4.6 kBq m^-3. Average daily indoor radon concentrations measured with RadonEye+² detectors vary from 7 to 60 Bq m^-3 with an average of 17 Bq m^-3. Indoor radon concentrations measured with passive RADTRAK detectors range between 15 and 104 Bq m^-3 with a geometric value of 38 Bq m^-3 and a geometric standard deviation of 1.5. This geometric value is lower than the value of 30 Bq m^-3 given by UNSCEAR. Indoor radon inhalation dose ranges between 0.28 and 1.97 mSv a^-1 with geometric value of 0.72 mSv a^-1 (at 0.03 standard deviation). Outdoor radon inhalation ranges between 0.02 and 0.26 mSv a^-1 with a mean value of 0.09 mSv a^-1. The total annual effective dose due to indoor and outdoor radon exposure for this study area is 0.81 mSv a^-1, less than 1.15 mSv a^-1 the world average value given by UNSCEAR. There is no significant radiological risk for the inhabitants.

The isotope biogeochemistry of bioindicators has widely demonstrated its added value in environmental issues by allowing to precisely identify sources of contamination. Most of the studies are based on studying one or two isotope systematics. Here, we are presenting an innovative multi-proxy approach that combines chemistry with both stable (C, S, N) and radiogenic (Pb) isotope systematics. Using Hypogymnia physodes bioindicators, we evaluated air quality in the complex environment of the Świętokrzyski National Park (ŚNP, Poland) with the ultimate objective of isotopically identifying the sources responsible for the observed contamination. Combining the isotope systematics showed that home heating is a major source of contamination in winter, whereas the contribution of road traffic increases during the summer. Pb isotope ratios identified industrial activities as the major source of this metal in the atmosphere.

North-central Ukraine is vulnerable to temperature increases and precipitation pattern changes associated with climate change. With water management becoming increasingly important, information on current water sources and moisture recycling is critically needed. Isotope ratios of oxygen (δ¹⁸O) and hydrogen (δ²H) in precipitation are sensitive to these variables and allow comparisons across the region. The δ²H and δ¹⁸O values from collected precipitation in Kyiv and Cherkasy in 2020 and published ³H data for Kyiv from the year 2000 show an influence of the North Atlantic Oscillation (NAO) and provide information about processes affecting precipitation along the storm trajectory. The δ¹⁸O values also show a correlation with temperature, indicating that precipitation patterns may be affected by the rising temperatures in the region, as predicted by recent regional studies using Representative Concentration Pathway scenarios and the global climate model GFDL-ESM2M. When compared to backtracked storm trajectory and NAO data, clear relationships emerged between water isotope ratios, storm paths, and likely moisture recycling. Overall, δ²H, δ¹⁸O, ³H, and backtracked storm trajectory data provide more regional and local information on water vapour processes, improving climate-change-driven precipitation forecasts in Ukraine.