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The multi-isotope biogeochemistry (S, C, N and Pb) of Hypogymnia physodes lichens: air quality approach in the Świętokrzyski National Park, Poland. 多同位素生物地球化学(S、C、N和Pb):波兰Świętokrzyski国家公园空气质量研究
IF 1.3 4区 环境科学与生态学 Q4 CHEMISTRY, INORGANIC & NUCLEAR Pub Date : 2022-08-01 DOI: 10.1080/10256016.2022.2110591
Monika Maria Ciężka, Maciej Górka, Agnieszka Trzyna, Magdalena Modelska, Anna Łubek, David Widory

The isotope biogeochemistry of bioindicators has widely demonstrated its added value in environmental issues by allowing to precisely identify sources of contamination. Most of the studies are based on studying one or two isotope systematics. Here, we are presenting an innovative multi-proxy approach that combines chemistry with both stable (C, S, N) and radiogenic (Pb) isotope systematics. Using Hypogymnia physodes bioindicators, we evaluated air quality in the complex environment of the Świętokrzyski National Park (ŚNP, Poland) with the ultimate objective of isotopically identifying the sources responsible for the observed contamination. Combining the isotope systematics showed that home heating is a major source of contamination in winter, whereas the contribution of road traffic increases during the summer. Pb isotope ratios identified industrial activities as the major source of this metal in the atmosphere.

生物指标的同位素生物地球化学已广泛显示其在环境问题上的附加价值,因为它可以精确地识别污染源。大多数研究都是基于对一两个同位素系统的研究。在这里,我们提出了一种创新的多代理方法,将化学与稳定(C, S, N)和放射性成因(Pb)同位素系统相结合。使用Hypogymnia physodes生物指标,我们评估了Świętokrzyski国家公园(ŚNP,波兰)复杂环境中的空气质量,最终目的是同位素确定造成观察到的污染的来源。结合同位素系统分析表明,家庭供暖是冬季污染的主要来源,而道路交通的贡献在夏季增加。铅同位素比率确定工业活动是大气中这种金属的主要来源。
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引用次数: 2
Better understand past, present and future climate variability by linking water isotopes and conventional hydrometeorology: summary and recommendations from the International Atomic Energy Agency and World Meteorological Organization. 通过将水同位素与传统水文气象学联系起来,更好地了解过去、现在和未来的气候变率:国际原子能机构和世界气象组织的摘要和建议。
IF 1.3 4区 环境科学与生态学 Q4 CHEMISTRY, INORGANIC & NUCLEAR Pub Date : 2022-08-01 DOI: 10.1080/10256016.2022.2108418
Yuliya Vystavna, Johannes Cullmann, Keith Hipel, Jodie Miller, David X Soto, Astrid Harjung, Andrew Watson, Alexandra Mattei, Seifu Kebede, Maksym Gusyev
Better understand past, present and future climate variability by linking water isotopes and conventional hydrometeorology: summary and recommendations from the International Atomic Energy Agency and World Meteorological Organization Yuliya Vystavna , Johannes Cullmann, Keith Hipel, Jodie Miller, David X. Soto, Astrid Harjung, Andrew Watson, Alexandra Mattei, Seifu Kebede f and Maksym Gusyev Isotope Hydrology Section, International Atomic Energy Agency (IAEA), Vienna International Centre, Vienna, Austria; World Meteorological Organization (WMO), Geneva, Switzerland; Department of Systems Design Engineering, University of Waterloo, Waterloo, Canada; School for Climate Studies, Stellenbosch University, Matieland, South Africa; UMR 6134 SPE, CNRS, University of Corsica, Corte, France; Center for Water Resources Research, University of KwaZulu Natal, Pietermaritzburg, South Africa; Institute of Environmental Radioactivity, Fukushima University, Fukushima, Japan
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引用次数: 4
Use of isotopes in examining precipitation patterns in north-central Ukraine. 同位素在检验乌克兰中北部降水模式中的应用。
IF 1.3 4区 环境科学与生态学 Q4 CHEMISTRY, INORGANIC & NUCLEAR Pub Date : 2022-08-01 DOI: 10.1080/10256016.2022.2131781
Elizabeth Avery, Olena Samonina, Lidiia Kryshtop, Iryna Vyshenska, Alan E Fryar, Andrea M Erhardt

North-central Ukraine is vulnerable to temperature increases and precipitation pattern changes associated with climate change. With water management becoming increasingly important, information on current water sources and moisture recycling is critically needed. Isotope ratios of oxygen (δ18O) and hydrogen (δ2H) in precipitation are sensitive to these variables and allow comparisons across the region. The δ2H and δ18O values from collected precipitation in Kyiv and Cherkasy in 2020 and published 3H data for Kyiv from the year 2000 show an influence of the North Atlantic Oscillation (NAO) and provide information about processes affecting precipitation along the storm trajectory. The δ18O values also show a correlation with temperature, indicating that precipitation patterns may be affected by the rising temperatures in the region, as predicted by recent regional studies using Representative Concentration Pathway scenarios and the global climate model GFDL-ESM2M. When compared to backtracked storm trajectory and NAO data, clear relationships emerged between water isotope ratios, storm paths, and likely moisture recycling. Overall, δ2H, δ18O, 3H, and backtracked storm trajectory data provide more regional and local information on water vapour processes, improving climate-change-driven precipitation forecasts in Ukraine.

乌克兰中北部容易受到与气候变化相关的温度升高和降水模式变化的影响。随着水资源管理变得越来越重要,迫切需要有关当前水资源和水分循环的信息。降水中氧(δ18O)和氢(δ2H)的同位素比值对这些变量很敏感,可以在整个区域内进行比较。基辅和切尔卡西收集的2020年降水的δ2H和δ18O值以及基辅2000年公布的3H数据显示了北大西洋涛动(NAO)的影响,并提供了沿风暴轨迹影响降水过程的信息。δ18O值也与温度相关,表明该地区降水模式可能受到温度上升的影响,这与最近使用代表性浓度路径情景和全球气候模式GFDL-ESM2M的区域研究结果一致。当与回溯的风暴轨迹和NAO数据进行比较时,水同位素比率、风暴路径和可能的水分再循环之间出现了明确的关系。总的来说,δ2H、δ18O、3H和回溯的风暴轨迹数据提供了更多关于水汽过程的区域和当地信息,改善了乌克兰气候变化驱动的降水预报。
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引用次数: 1
Subterranean carbon flows from source to stygofauna: a case study on the atyid shrimp Stygiocaris stylifera (Holthuis, 1960) from Barrow Island (WA) 地下碳从碳源到海鞘动物群的流动:以巴罗岛(WA)的不腐虾Stygiocaris stylifera (Holthuis, 1960)为例
IF 1.3 4区 环境科学与生态学 Q4 CHEMISTRY, INORGANIC & NUCLEAR Pub Date : 2022-05-04 DOI: 10.1080/10256016.2022.2071873
M. Saccò, W. Humphreys, N. Stevens, Matthew R. Jones, Fiona Takulis, E. Thomas, A. Blyth
ABSTRACT Groundwater biota are crucial for the ecological functioning of subterranean ecosystems. However, while knowledge of the taxonomic diversity of groundwater invertebrates (stygofauna) is increasing, functional ecological information is still limited. Here, we investigate seldom empirically tested assumptions around stygofaunal trophic plasticity in coping with oligotrophic habitats. We focus on Barrow Island (Western Australia), an ideal natural laboratory due to the occurrence of natural oil seeps in association with aquifers. The trophic position and food source use of the endemic atyid shrimp Stygiocaris stylifera (Holthuis, 1960) were assessed via δ 13C and δ 15N stable isotope analysis (SIA). Background information on the environmental conditions was gathered through hydrochemical data and δ 13C SIA combined with 14C data from dissolved inorganic/organic carbon and particulate organic carbon from groundwater samples. Our results indicate carbon enrichment in proximity to the natural oil seepage coupled with changes in trophic positions of S. stylifera from higher consumers/predators to biofilm grazers/decomposers. These results are consistent with an increased involvement of hydrocarbon seeps and associated microbial communities in the carbon flows and confirm potential for the trophic flexibility in stygofauna. Further investigations involving other trophic groups will help elucidate the functioning of the ecosystems at a community level.
地下水生物群对地下生态系统的生态功能至关重要。然而,尽管地下水无脊椎动物(丛动物群)的分类多样性正在增加,但功能生态信息仍然有限。在这里,我们调查了很少经过实证检验的关于水生动物营养可塑性应对贫营养栖息地的假设。我们的重点是巴罗岛(西澳大利亚),一个理想的天然实验室,因为与含水层有关的天然石油渗漏的发生。采用δ 13C和δ 15N稳定同位素分析(SIA)对Holthuis, 1960年养殖的stylifera (Stygiocaris stylifera)虾的营养地位和食物来源利用进行了评价。通过水化学数据和δ 13C SIA数据,结合地下水样品中溶解无机/有机碳和颗粒有机碳的14C数据,收集了环境条件的背景信息。我们的研究结果表明,在天然油渗漏附近存在碳富集,并且花柱草的营养地位从较高的消费者/捕食者转变为生物膜食草者/分解者。这些结果与碳流中碳氢化合物渗漏和相关微生物群落的增加参与一致,并证实了stylo动物群营养灵活性的潜力。对其他营养类群的进一步调查将有助于在群落水平上阐明生态系统的功能。
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引用次数: 3
Assessing land use influences on isotopic variability and stream water ages in urbanising rural catchments 评估土地利用对城市化农村集水区同位素变率和河流年龄的影响
IF 1.3 4区 环境科学与生态学 Q4 CHEMISTRY, INORGANIC & NUCLEAR Pub Date : 2022-05-04 DOI: 10.1080/10256016.2022.2070615
Jamie Lee Stevenson, J. Geris, C. Birkel, D. Tetzlaff, C. Soulsby
ABSTRACT Stable water isotopes are invaluable in helping understand catchment functioning and are widely used in experimental catchments, with higher frequency data becoming increasingly common. Such datasets incur substantial logistical costs, reducing their feasibility for use by decision makers needing to understand multi-catchment, landscape-scale functioning over a relatively short period to assess the impact of proposed land use change. Instead, reconnaissance style surveys (high spatial resolution across the landscape at a lower temporal frequency, over a relatively short period) offer an alternative, complementary approach. To test if such sampling could identify heterogeneities in hydrological functioning, and associated landscape controls, we sampled 27 stream sites fortnightly for one year within a peri-urban landscape undergoing land use change. Visual examination of raw data and application of mean transit time and young water fraction models indicated urbanisation, agriculture and responsive soils caused more rapid cycling of precipitation to stream water, whereas mature forestry provided attenuation. We were also able to identify contiguous catchments which functioned fundamentally differently, meaning their response to land use alteration would also be different. This study demonstrated how stable water isotopes can be a valuable, low-cost addition to tools available for environmental decision makers by providing local, process-based information.
稳定水同位素在帮助了解流域功能方面具有不可估量的价值,并且在实验流域中得到广泛应用,高频数据变得越来越普遍。这些数据集产生了大量的物流成本,降低了决策者使用这些数据集的可行性,因为决策者需要在相对较短的时间内了解多流域、景观尺度的功能,以评估拟议的土地利用变化的影响。相反,侦察式调查(在相对较短的时间内,以较低的时间频率在整个景观中实现高空间分辨率)提供了一种替代的补充方法。为了测试这种采样是否可以识别水文功能的异质性,以及相关的景观控制,我们在经历土地利用变化的城郊景观中每两周采样27个河流站点,持续一年。对原始数据的目视检查以及平均传输时间和年轻水组分模型的应用表明,城市化、农业和响应性土壤导致降水到水流的更快循环,而成熟的林业则提供了衰减。我们还能够识别出功能根本不同的连续集水区,这意味着它们对土地利用改变的反应也会不同。这项研究表明,稳定的水同位素可以通过提供当地的、基于过程的信息,成为环境决策者可用工具的一种有价值的、低成本的补充。
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引用次数: 5
A straightforward approach for assessing the effectiveness of membrane materials as radon (222Rn) barriers 一种评估膜材料作为氡(222Rn)屏障有效性的直接方法
IF 1.3 4区 环境科学与生态学 Q4 CHEMISTRY, INORGANIC & NUCLEAR Pub Date : 2022-05-04 DOI: 10.1080/10256016.2022.2058500
M. Schubert, Diana Altendorf, H. Weiss
ABSTRACT The ubiquitous presence of the radioisotope radon (222Rn) and its short-lived progeny (218Po, 214Pb, 214Bi, 214Po) is challenging in two respects: (i) Radon is a major issue regarding health-related problems due to potentially elevated radiation exposure of humans in dwellings, and (ii) due to the mobility of radon the short-lived progeny may cause complications in radionuclide detection in laboratories. Polymer membranes are an appropriate means for effectively preventing unwanted radon migration. However, most of the published literature focusses on robust membranes made for the large-scale sealing of dwelling substructures. Membranes that are suitable (at small-scale) for sealing purposes in radionuclide detection applications are only rarely discussed. In this paper, we present a straightforward practical approach that allows the effectiveness of any membrane to be assessed for any purpose related to radon sealing. Executing the approach requires only (i) a suitable container with inlet and outlet ports, (ii) a mobile radon detector, and (iii) any type of radon source material. The approach provides a tool that allows testing any available membrane for its applicability as radon barrier sheeting.
摘要放射性同位素氡(222Rn)及其短命子代(218Po、214Pb、214Bi、214Po)的普遍存在在两个方面具有挑战性:(i)由于人类在住宅中的辐射暴露可能增加,氡是与健康相关的主要问题,以及(ii)由于氡的流动性,短命的子代可能会导致实验室放射性核素检测的复杂性。聚合物膜是有效防止不必要的氡迁移的合适手段。然而,大多数已发表的文献都集中在为住宅下部结构的大规模密封而制造的坚固膜上。适用于放射性核素检测应用中密封目的(小规模)的膜很少被讨论。在本文中,我们提出了一种简单实用的方法,可以评估任何膜的有效性,用于与氡密封相关的任何目的。执行该方法只需要(i)一个带入口和出口的合适容器,(ii)一个移动氡探测器,以及(iii)任何类型的氡源材料。该方法提供了一种工具,可以测试任何可用的膜是否适用于氡气挡板。
{"title":"A straightforward approach for assessing the effectiveness of membrane materials as radon (222Rn) barriers","authors":"M. Schubert, Diana Altendorf, H. Weiss","doi":"10.1080/10256016.2022.2058500","DOIUrl":"https://doi.org/10.1080/10256016.2022.2058500","url":null,"abstract":"ABSTRACT The ubiquitous presence of the radioisotope radon (222Rn) and its short-lived progeny (218Po, 214Pb, 214Bi, 214Po) is challenging in two respects: (i) Radon is a major issue regarding health-related problems due to potentially elevated radiation exposure of humans in dwellings, and (ii) due to the mobility of radon the short-lived progeny may cause complications in radionuclide detection in laboratories. Polymer membranes are an appropriate means for effectively preventing unwanted radon migration. However, most of the published literature focusses on robust membranes made for the large-scale sealing of dwelling substructures. Membranes that are suitable (at small-scale) for sealing purposes in radionuclide detection applications are only rarely discussed. In this paper, we present a straightforward practical approach that allows the effectiveness of any membrane to be assessed for any purpose related to radon sealing. Executing the approach requires only (i) a suitable container with inlet and outlet ports, (ii) a mobile radon detector, and (iii) any type of radon source material. The approach provides a tool that allows testing any available membrane for its applicability as radon barrier sheeting.","PeriodicalId":14597,"journal":{"name":"Isotopes in Environmental and Health Studies","volume":"58 1","pages":"301 - 310"},"PeriodicalIF":1.3,"publicationDate":"2022-05-04","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"42799854","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 1
How do precipitation events modify the stable isotope ratios in leaf water at Lhasa on the southern Tibetan Plateau? 降水事件如何改变青藏高原南部拉萨地区叶片水的稳定同位素比率?
IF 1.3 4区 环境科学与生态学 Q4 CHEMISTRY, INORGANIC & NUCLEAR Pub Date : 2022-05-03 DOI: 10.1080/10256016.2022.2062343
Yong Wang, Wusheng Yu, Lun Luo, Minghui Li, Xiaoming Liu, Rong Guo, Yaoming Ma, Baiqing Xu, Guangjan Wu, Chengyi Zhao, Zhaowei Jing, Feili Wei, J. Cui, Jingyi Zhang, D. Qu
ABSTRACT Serving as a medium between source water and cellulose, leaf water contributes to the isotope ratios (δ 18O, δ 2H) of plant organic matter, which can be used for paleoclimate reconstruction. This study is the first to examine the diurnal variations in the δ 18O and δ 2H of leaf water on the southern Tibetan Plateau. The δ 18O and δ 2H of leaf water were relatively low when precipitation events occurred. In particular, 18O and 2H of leaf water became extremely depleted 5 h after the precipitation event. Our findings demonstrate that precipitation can modify the isotope ratios of leaf water from external and internal causes. First, precipitation events affect meteorological elements, lead to decreases in leaf transpiration, and immediately weaken the isotope enrichment of leaf water (‘rapid effect’ of precipitation). Second, precipitation events affect the internal plant–soil water cycle process, causing the plant to preferentially use deeper soil water, and the corresponding isotope ratios of leaf water exhibit extremely low values 5 h after precipitation events (‘delay effect’ of precipitation). This study suggests that researchers need to be cautious in separating the signals of precipitation and hydrological processes when interpreting isotope records preserved in tree-ring cellulose archives from the Tibetan Plateau.
摘要叶水作为水源水和纤维素之间的介质,对植物有机质的同位素比值(δ18O,δ2H)有贡献,可用于古气候重建。本研究首次对青藏高原南部叶水δ18O和δ2H的日变化进行了研究。降水事件发生时,叶片水分的δ18O和δ2H相对较低。特别是,在降水事件后5小时,18O和2H的叶水变得极度枯竭。我们的研究结果表明,降水可以从外部和内部原因改变叶片水的同位素比率。首先,降水事件影响气象要素,导致叶片蒸腾减少,并立即削弱叶片水分的同位素富集(降水的“快速效应”)。其次,降水事件影响植物-土壤内部的水循环过程,导致植物优先利用深层土壤水,并且在降水事件发生5小时后,叶片水的相应同位素比率表现出极低的值(降水的“延迟效应”)。这项研究表明,研究人员在解释青藏高原树木年轮纤维素档案中保存的同位素记录时,需要谨慎地分离降水和水文过程的信号。
{"title":"How do precipitation events modify the stable isotope ratios in leaf water at Lhasa on the southern Tibetan Plateau?","authors":"Yong Wang, Wusheng Yu, Lun Luo, Minghui Li, Xiaoming Liu, Rong Guo, Yaoming Ma, Baiqing Xu, Guangjan Wu, Chengyi Zhao, Zhaowei Jing, Feili Wei, J. Cui, Jingyi Zhang, D. Qu","doi":"10.1080/10256016.2022.2062343","DOIUrl":"https://doi.org/10.1080/10256016.2022.2062343","url":null,"abstract":"ABSTRACT Serving as a medium between source water and cellulose, leaf water contributes to the isotope ratios (δ 18O, δ 2H) of plant organic matter, which can be used for paleoclimate reconstruction. This study is the first to examine the diurnal variations in the δ 18O and δ 2H of leaf water on the southern Tibetan Plateau. The δ 18O and δ 2H of leaf water were relatively low when precipitation events occurred. In particular, 18O and 2H of leaf water became extremely depleted 5 h after the precipitation event. Our findings demonstrate that precipitation can modify the isotope ratios of leaf water from external and internal causes. First, precipitation events affect meteorological elements, lead to decreases in leaf transpiration, and immediately weaken the isotope enrichment of leaf water (‘rapid effect’ of precipitation). Second, precipitation events affect the internal plant–soil water cycle process, causing the plant to preferentially use deeper soil water, and the corresponding isotope ratios of leaf water exhibit extremely low values 5 h after precipitation events (‘delay effect’ of precipitation). This study suggests that researchers need to be cautious in separating the signals of precipitation and hydrological processes when interpreting isotope records preserved in tree-ring cellulose archives from the Tibetan Plateau.","PeriodicalId":14597,"journal":{"name":"Isotopes in Environmental and Health Studies","volume":"58 1","pages":"229 - 246"},"PeriodicalIF":1.3,"publicationDate":"2022-05-03","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"41724333","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Measurement of age-dependent radiation ingestion doses due to gross alpha and gross beta exposure from medicinal plants. 测量药用植物总α和总β照射引起的随年龄变化的辐射摄入剂量。
IF 1.3 4区 环境科学与生态学 Q4 CHEMISTRY, INORGANIC & NUCLEAR Pub Date : 2022-05-01 Epub Date: 2022-02-08 DOI: 10.1080/10256016.2022.2032691
Muhammad Rafique, Chand Shahzadi, Abdul Jabbar, Mumtaz Khan, Saeed Ur Rahman, Syed Shujahat Hussain Bukhari, Shahab Ahmed Abbasi, Nasar Ahmed

This article presents the results of a study conducted to measure the gross alpha, gross beta activities in medicinal plant samples collected from different districts of Azad Kashmir, Pakistan. The ASC-950-DP gasless high-speed counter was used for the measurement of gross α/β activities. Measured activities have been used to assess age-dependent annual effective doses for infants, one-, five-, ten-, and fifteen-year-old and adult people. For a medicinal plant consumption rate (MPCR) of 1.8 kg a-1, the average gross alpha and beta annual committed effective dose (ACED) delivered to one-, five-, ten-, fifteen-year-olds and adults fall below the WHO recommended level (290 µSv a-1) and that reported in the UNSCEAR 2000 (0.3 mSv a-1) report. Results obtained for the current study show that the radiological hazard related to the consumption of natural radionuclides in medicinal plants is inconsequential with exception of the ACED delivered to infants at an MPCR of 1.8 g a-1 and higher values.

本文介绍了一项研究的结果,以测量从巴基斯坦阿扎德克什米尔不同地区收集的药用植物样品中的总α,总β活性。采用ASC-950-DP无气高速计数器测定总α/β活性。测量的活度已被用来评估婴儿、1岁、5岁、10岁、15岁和成年人的年有效剂量与年龄有关。对于1.8 kg a-1的药用植物消耗率(MPCR), 1岁、5岁、10岁、15岁儿童和成年人的平均总α和β年承诺有效剂量(ced)低于世卫组织建议水平(290µSv a-1)和2000年联合国科委会报告的水平(0.3 mSv a-1)。目前的研究结果表明,除了MPCR为1.8 g a-1及更高值的婴儿接受的放射性核素外,与食用药用植物中的天然放射性核素有关的辐射危害是无关紧要的。
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引用次数: 1
Stable hydrogen and oxygen isotope abundance of major bottled water brands sold in the United Kingdom. 在英国销售的主要瓶装水品牌氢、氧同位素丰度稳定。
IF 1.3 4区 环境科学与生态学 Q4 CHEMISTRY, INORGANIC & NUCLEAR Pub Date : 2022-05-01 Epub Date: 2021-12-16 DOI: 10.1080/10256016.2021.2005041
Vasile Ersek, Jamie Sharples, William Thomas

Bottled water in the UK has a ∼20 % share of the soft drinks market with a sales value of >£1.5 billion. Bottled water is susceptible to fraud and it is important to characterise the chemical signature of aquifers used by the bottled water industry. Measuring 18O/16O and 2H/1H ratios in bottled water is one important step in fraud prevention and aquifer characterisation as these ratios in groundwater tend to be stable or change very slowly through time. Here we characterise the isotopic signature of 30 brands of bottled water sold in the UK. The average δ18O of bottled waters is -7.4 and -48.4 for δ2H. This isotopic composition is closely related to that of the annual rainfall and follows latitudinal and longitudinal gradients which combine to explain 77 % of the δ18O variance.

瓶装水在英国软饮料市场中占有20%的份额,销售额超过15亿英镑。瓶装水很容易受到欺诈,瓶装水工业使用的含水层的化学特征特征是很重要的。测量瓶装水中的18O/16O和2H/1H比率是防止欺诈和描述含水层特征的重要一步,因为地下水中的这些比率随着时间的推移趋于稳定或变化非常缓慢。在这里,我们描述了在英国销售的30个品牌瓶装水的同位素特征。瓶装水δ18O平均值为-7.4,δ2H平均值为-48.4。该同位素组成与年降雨量密切相关,并遵循纬度和纵向梯度,这两者结合起来解释了77%的δ18O方差。
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引用次数: 1
Quantifying the contribution of evaporation from Lake Taihu to precipitation with an isotope-based method 用同位素法量化太湖蒸发量对降水的贡献
IF 1.3 4区 环境科学与生态学 Q4 CHEMISTRY, INORGANIC & NUCLEAR Pub Date : 2022-04-05 DOI: 10.1080/10256016.2022.2056599
Yongbo Hu, W. Xiao, Jingyuan Wang, L. Welp, Chengyu Xie, H. Chu, Xuhui Lee
ABSTRACT Moisture recycling plays a crucial role in regional hydrological budgets. The isotopic composition of precipitation has long been considered as a good tracer to investigate moisture recycling. This study quantifies the moisture recycling fractions (f r) in the Lake Taihu region using spatial variations of deuterium excess in precipitation (d P) and surface water vapour flux (d E). Results show that d P at a site downwind of the lake was higher than that at an upwind site, indicating the influence of lake moisture recycling. Spatial variations in d P after sub-cloud evaporation corrections were 2.3, 1.4 and 3.2 ‰, and d E values were 27.4, 32.3 and 31.4 ‰ for the first winter monsoon, the summer monsoon and the second winter monsoon, respectively. Moisture recycling fractions were 0.48 ± 0.13, 0.07 ± 0.03 and 0.38 ± 0.05 for the three monsoon periods, respectively. Both using the lake parameterization kinetic fractionation factors or neglecting sub-cloud evaporation would decrease f r, and the former has a larger influence on the f r calculation. The larger f r in the winter monsoon periods was mainly caused by lower specific humidity of airmasses but comparable moisture uptake along their trajectories compared to the summer monsoon period.
摘要水分循环利用在区域水文预算中起着至关重要的作用。长期以来,降水的同位素组成一直被认为是研究水分循环的良好示踪剂。本研究利用降水中氘过量(dP)和地表水蒸气通量(dE)的空间变化来量化太湖地区的水分循环分数(fr)。结果表明,湖泊下风处的dP高于上风处,表明湖泊水分循环的影响。第一次冬季风、夏季风和第二次冬季风经云底蒸发校正后的dP空间变化分别为2.3、1.4和3.2‰,dE值分别为27.4、32.3和31.4‰。水分回收率为0.48 ± 0.130.07 ± 0.03和0.38 ± 三个季风期分别为0.05。无论是使用湖泊参数化动力学分馏因子还是忽略亚云蒸发都会降低f r,前者对f r的计算影响较大。冬季风期较大的f r主要是由于气团的比湿度较低,但与夏季风期相比,其轨迹上的吸湿量相当。
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引用次数: 1
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Isotopes in Environmental and Health Studies
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