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Ein multiples interaktives Kontinuumsmodell (MINC) zur Simulation des reaktiven Stofftransports in einem Bergbaufolgegebiet: Eine Fallstudie über das Ibbenbürener Westfeld 多层连续模式模型(MINC)用于模拟煤矿地区的被动物料运输:本文针对西博尼亚半岛的研究
4区 环境科学与生态学 Q2 Earth and Planetary Sciences Pub Date : 2023-06-01 DOI: 10.1007/s10230-023-00938-2
Diego Bedoya-Gonzalez, Timo Kessler, Thomas Rinder, Sylke Hilberg, Zsuzsanna Szabó-Krausz, Maria-Theresia Schafmeister
Abstract We tested the suitability of the multiple interactive continua approach (MINC) to simulate reactive mass transport in a disturbed post-mining coal zone. To the authors’ knowledge, this approach has not been employed in such mining settings despite its relative success in other environmental fields. To this end, TOUGHREACT software was used to set up a MINC model of the unsaturated overburden of the Ibbenbüren Westfield. With it, we examined and evaluated water–rock interactions in both the fractured and porous continua as the main driver of elevated hydrogen, iron, sulfate, and chloride concentrations in the coal mine groundwater. Long and seasonal geochemical signatures were obtained by formulating and applying a five-stage modelling process that depicts the mining history of the area. The simulation results agree well with the concentrations and discharge trends measured in the mine drainage. Oxygen and meteoric water flow through the fractured continuum, leading to a high and steady release of hydrogen, iron, and sulfate ions derived from pyrite oxidation in the matrix continua closest to the fractures. Likewise, high chloride concentrations resulted from the mixing and gradual release of relatively immobile solutes in the matrix as they interacted with percolating water in the fracture. In both cases, the use of a multiple continua approach was essential to resolve sharp gradients for advection and faster kinetic reactions, while reducing the model’s dependence on block size for diffusive transport at the fracture–matrix interface. The model further allows for the calculation and analysis of solute exchange and transport in the unsaturated overburden resulting from rebound and imbibition processes, something pioneering when compared to other models in the field.
摘要本文测试了多重交互连续体方法(MINC)在扰动采煤后区域反应性物质输运模拟中的适用性。据作者所知,尽管这种方法在其他环境领域取得了相对的成功,但尚未在这种采矿环境中采用。为此,利用TOUGHREACT软件建立了ibbenb西油田非饱和覆盖层的MINC模型。有了它,我们检查和评估了裂缝和多孔连续体中的水岩相互作用,作为煤矿地下水中氢、铁、硫酸盐和氯化物浓度升高的主要驱动因素。通过制定和应用描述该地区采矿历史的五阶段建模过程,获得了长期和季节性的地球化学特征。模拟结果与实测的矿井水浓度和排放趋势吻合较好。氧气和大气水流经断裂连续体,导致最靠近裂缝的基质连续体中黄铁矿氧化产生的氢、铁和硫酸盐离子大量稳定释放。同样,高氯化物浓度是由于基质中相对不流动的溶质与裂缝中的渗透水相互作用时混合并逐渐释放而产生的。在这两种情况下,使用多重连续方法对于解决平流的急剧梯度和更快的动力学反应是必不可少的,同时减少了模型对裂缝-基质界面扩散输运块大小的依赖。该模型进一步允许计算和分析非饱和覆盖层中由反弹和吸胀过程引起的溶质交换和运移,与该领域的其他模型相比,这是一个开创性的成果。
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引用次数: 0
基于化学和水同位素组份揭示芬兰基斯塔拉Kittilä矿井水来源和演化 基于化学和水同位素组份揭示芬兰基斯塔拉Kittilä矿井水来源和演化
4区 环境科学与生态学 Q2 Earth and Planetary Sciences Pub Date : 2023-06-01 DOI: 10.1007/s10230-023-00935-5
V. Milesi, J. Declercq, W. Harding, T. Jarman, O. Baas, J. Saukkoriipi, A. van Wageningen, R. Bowell
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引用次数: 0
Dear Reader 亲爱的读者
4区 环境科学与生态学 Q2 Earth and Planetary Sciences Pub Date : 2023-06-01 DOI: 10.1007/s10230-023-00940-8
Robert Kleinmann
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引用次数: 0
Eine praktische Methode für die Vorhersage von Sohlwassereinbrüchen unter Verwendung eines Hybridmodells aus künstlicher Intelligenz und GIS 这是用人工智慧和信息技术混合模型预测严重自发性突水事故的实用方法
4区 环境科学与生态学 Q2 Earth and Planetary Sciences Pub Date : 2023-06-01 DOI: 10.1007/s10230-023-00932-8
Weitao Liu, Mengke Han
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引用次数: 0
含水煤样力学损伤与变形破坏试验研究 含水煤样力学损伤与变形破坏试验研究
4区 环境科学与生态学 Q2 Earth and Planetary Sciences Pub Date : 2023-05-27 DOI: 10.1007/s10230-023-00933-7
Qiangling Yao, Liqiang Yu, Changhao Shan, Ze Xia, Ning Chen, Hongxin Xie, Liu Zhu
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引用次数: 0
Effect of Temperature on Arsenic Treatment and Mobility in Mine Influenced Water 温度对砷在矿井水中的处理及迁移率的影响
IF 2.8 4区 环境科学与生态学 Q2 Earth and Planetary Sciences Pub Date : 2023-05-24 DOI: 10.1007/s10230-023-00931-9
Drummond Earley
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引用次数: 0
海水中产生的水滑石用于修复酸性金属矿井排水和海底安置的评估 海水中产生的水滑石用于修复酸性金属矿井排水和海底安置的评估
4区 环境科学与生态学 Q2 Earth and Planetary Sciences Pub Date : 2023-05-20 DOI: 10.1007/s10230-023-00934-6
Ni Made Sri Suliartini, Cynthia A. Joll, Grant B. Douglas
Abstract Uncontrolled release of acid mine drainage (AMD) causes widespread detrimental impacts on the receiving environment. Thus, effective treatment to neutralise AMD effluent pH and capture a suite of metals is required. In-situ hydrotalcite (HTC) precipitation is an emerging technology for AMD remediation. HTC has an inherent capacity to accommodate a range of cations and anions during in situ formation, offering a method of broad-spectrum contaminant removal. This study explored the feasibility of using seawater as an Mg source and synthetic AMD in HTC formation. The HTC was formed from a stoichiometric combination of synthetic AMD and seawater. While three initial stoichiometric M 2+ :M 3+ ratios of 2:1, 3:1, and 4:1 were investigated, only HTC with an M 2+ :M 3+ ratio of 2:1 was generated, as confirmed by both mineralogical and geochemical analyses. Importantly, the HTC was demonstrated to effectively remove a suite of metals present in AMD such as Cu, Zn, Al, and Mn with removal rates of between 99.97 to 99.99%. The HTC precipitate contained ≈6.6% Cu and 4.1% Zn, and thus shows the potential, if required, for future metal recovery. Since submarine placement is often used in metal mining and processing operations proximal to the coast, the stability of the HTC precipitate in seawater was also investigated. Importantly, only 0.2% of the Cu and 1.1% of the Zn within the HTC were subsequently leaching in decreasing increments into seawater over 30 days with decreasing increments after the initial seven days. This indicates robust element retention and confirms the potential of HTC for AMD remediation with direct submarine placement.
酸性矿井水的无节制排放对接收环境造成了广泛的危害。因此,需要有效的处理来中和AMD废水的pH值并捕获一套金属。原位水滑石(HTC)沉淀法是一种新兴的AMD修复技术。HTC在原位形成过程中具有容纳一系列阳离子和阴离子的固有能力,提供了一种广谱污染物去除方法。本研究探讨了以海水为镁源,在HTC地层中合成AMD的可行性。HTC是由合成AMD和海水的化学计量组合形成的。虽然研究了三种初始化学计量m2 +: m3 +比例分别为2:1、3:1和4:1,但矿物学和地球化学分析均证实,只生成了m2 +: m3 +比例为2:1的HTC。重要的是,HTC被证明可以有效地去除AMD中存在的一系列金属,如Cu, Zn, Al和Mn,去除率在99.97到99.99%之间。HTC沉淀物含有≈6.6%的Cu和4.1%的Zn,因此,如果需要的话,它显示出未来金属回收的潜力。由于潜艇经常用于靠近海岸的金属采矿和加工作业,因此还研究了海水中HTC沉淀物的稳定性。重要的是,在30天内,HTC中只有0.2%的Cu和1.1%的Zn浸出到海水中,浸出量逐渐减少,在最初的7天之后,浸出量逐渐减少。这表明了强大的元素保留,并证实了HTC通过直接潜艇安置进行AMD修复的潜力。
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引用次数: 0
Mine Wastewater Treatment with Upflow Anaerobic Fixed Film Reactors 上流式厌氧固定膜反应器处理矿山废水
IF 2.8 4区 环境科学与生态学 Q2 Earth and Planetary Sciences Pub Date : 2023-05-17 DOI: 10.1007/s10230-023-00929-3
Islamud Din, S. Khan, A. Hesham, Sidra Irum, Cang Daqiang
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引用次数: 0
Eine Methode zur Kontrolle von Wassergefahren in Deckschichten von tiefen Jurakohlen, welche auf der sedimentären Fazies begründet ist 法基夫妇的技术,如笛法所指出的
4区 环境科学与生态学 Q2 Earth and Planetary Sciences Pub Date : 2023-04-07 DOI: 10.1007/s10230-023-00930-w
Yang Wang, Yonghui Wu, Qin Ge, Zhiguo Pu, Jinhui Liu, Yanhong Zhang, Xiangjian Xie
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引用次数: 1
Editor's Note 编者按
IF 2.8 4区 环境科学与生态学 Q2 Earth and Planetary Sciences Pub Date : 2023-03-01 DOI: 10.1007/s10230-001-8073-4
Red Washburn
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引用次数: 0
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Mine Water and the Environment
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