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Sensitivity enhancement of time-gated Raman spectroscopy by reducing the systematic noise of residual fluorescence background. 通过降低残余荧光背景的系统噪声,提高时间门控拉曼光谱的灵敏度。
IF 3.1 2区 物理与天体物理 Q2 OPTICS Pub Date : 2024-12-15 DOI: 10.1364/OL.540236
Zhenyou Wang, Guangyou Fang

Fluorescence interference is a pervasive challenge in Raman spectroscopy, often limiting its broader application. Time-gated Raman spectroscopy offers a more universal solution by temporally separating Raman signals from fluorescence; however, it faces significant challenges when dealing with samples that exhibit short fluorescence lifetimes. Achieving high time resolution to effectively distinguish these signals typically requires advanced detectors that are not only costly but also difficult to source commercially, often resulting in substantial residual fluorescence that diminishes overall signal quality. In this work, we identified that the dominant noise in time-gated Raman spectroscopy is wavelength-to-wavelength fluctuation noise, which cannot be reduced by simply extending the collection time. Through our analysis, we discovered that this noise is linearly proportional to the fluorescence background and remains consistent across different time windows when collected using the time-correlated single-photon counting (TCSPC) technology. Recognizing this consistent pattern, we developed a novel, to the best of our knowledge, method to effectively remove this noise by leveraging the time-resolved fluorescence spectrum. For example, in the case of sesame oil excited with a 532 nm laser, it is typically difficult to obtain a recognizable Raman spectrum when the gate width exceeds 300 ps. However, using our method, we were able to achieve a decent signal even with a gate width of 4 ns. By correcting the Raman spectrum using the captured pure fluorescence spectrum, we achieve up to a 23-fold improvement in the signal-to-noise ratio (SNR). This innovation significantly reduces the dependence on high-cost, high-time-resolution detectors, potentially expanding the adoption and applicability of time-gated Raman spectroscopy across various fields.

荧光干扰是拉曼光谱学中普遍存在的难题,往往限制了拉曼光谱学的广泛应用。时间门控拉曼光谱通过在时间上分离拉曼信号和荧光,提供了一种更通用的解决方案;然而,在处理荧光寿命较短的样品时,时间门控拉曼光谱面临着巨大的挑战。要实现有效区分这些信号的高时间分辨率,通常需要先进的检测器,而这些检测器不仅成本高昂,而且很难从市场上采购,这往往会导致大量荧光残留,从而降低整体信号质量。在这项工作中,我们发现在时间门控拉曼光谱中占主导地位的噪声是波长间波动噪声,这种噪声无法通过简单地延长采集时间来降低。通过分析,我们发现这种噪声与荧光背景成线性比例,并且在使用时间相关单光子计数(TCSPC)技术采集时,在不同的时间窗口中保持一致。认识到这种一致的模式后,我们开发了一种新颖的方法,据我们所知,这种方法可以利用时间分辨荧光光谱有效地去除这种噪声。例如,在用 532 nm 激光激发芝麻油的情况下,当栅宽超过 300 ps 时,通常很难获得可识别的拉曼光谱。然而,使用我们的方法,即使栅极宽度为 4 毫微秒,我们也能获得像样的信号。通过使用捕获的纯荧光光谱对拉曼光谱进行校正,我们将信噪比(SNR)提高了 23 倍。这一创新大大降低了对高成本、高时间分辨率探测器的依赖,有可能扩大时间门控拉曼光谱在各个领域的应用范围。
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引用次数: 0
High-efficiency single-mode erbium-doped lithium niobate microring laser with milliwatt output power. 输出功率达毫瓦的高效单模掺铒铌酸锂微光激光器。
IF 3.1 2区 物理与天体物理 Q2 OPTICS Pub Date : 2024-12-15 DOI: 10.1364/OL.544271
Chao Sun, Youting Liang, Jian Liu, Yuan Zhou, Zhihao Zhang, Jinming Chen, Zhaoxiang Liu, Zhiwei Fang, Min Wang, Haisu Zhang, Ya Cheng

Erbium-doped thin-film lithium niobate (TFLN) lasers have attracted great interest in recent years due to their compatibility with high-speed electro-optic (EO) modulation on the same platform. In this work, high-efficiency single-mode erbium-doped microring lasers with milliwatt output powers were demonstrated. Monolithic lithium niobate microring resonators using pulley-waveguide-coupling were fabricated by the photolithography assisted chemo-mechanical etching (PLACE) technique. The maximum single-mode laser power of 1.26 mW with the side-mode suppression ratio (SMSR) of 50 dB was achieved around the wavelength of 1562 nm, as well as the maximum laser slope efficiency of 2.51% and the minimum laser linewidth of 30 kHz. Besides, the lasing band was easily switched by the pulley-coupler with variable waveguide widths. The demonstrated milliwatt-level on-chip microlasers hold great promise as bright light sources for various integrated devices on the TFLN platform such as EO modulators and combs.

近年来,掺铒铌酸锂薄膜(TFLN)激光器因其与高速光电(EO)调制在同一平台上的兼容性而备受关注。在这项工作中,演示了输出功率为毫瓦的高效单模掺铒微oring 激光器。采用光刻辅助化学机械蚀刻(PLACE)技术,制造出了使用脉冲波导耦合的铌酸锂单片微孔谐振器。在波长 1562 nm 附近实现了 1.26 mW 的最大单模激光功率和 50 dB 的侧模抑制比(SMSR),以及 2.51% 的最大激光斜率效率和 30 kHz 的最小激光线宽。此外,通过波导宽度可变的滑轮耦合器,还能轻松切换激光波段。所展示的毫瓦级片上微激光器有望成为 TFLN 平台上各种集成设备(如 EO 调制器和梳状器)的明亮光源。
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引用次数: 0
300 mW 45 MHz fundamental mode-locking all-fiber ring Mamyshev oscillator at 1 µm. 300 mW 45 MHz 基本模式锁定全光纤环形马梅雪夫振荡器,波长 1 µm。
IF 3.1 2区 物理与天体物理 Q2 OPTICS Pub Date : 2024-12-15 DOI: 10.1364/OL.541931
Corentin Delangle, Florent Scol, Clemens Hönninger, Geraud Bouwmans, Olivier Vanvincq, Emmanuel Hugonnot

In this Letter, we present an experimental demonstration of an all-fiber ring Mamyshev oscillator (MO) that delivers a 300 mW optical power at a repetition rate of 45 MHz. Numerical design has shown that more than 70 MHz repetition rate is achievable in a ring cavity configuration using standard step-index fibers and components. Interest of WDM type filtering on pulse duration is especially shown. This demonstration of a high repetition rate ring Mamyshev oscillator working with the simplest transmission filter paves the way to very simple and cost-effective all-standard-PM-fiber Mamyshev oscillators.

在这封信中,我们介绍了一种全光纤环形马梅雪夫振荡器(MO)的实验演示,它能以 45 MHz 的重复频率提供 300 mW 的光功率。数值设计表明,使用标准阶梯指数光纤和元件,在环形腔配置中可以实现超过 70 MHz 的重复率。波分复用型滤波器对脉冲持续时间的影响尤为明显。利用最简单的传输滤波器实现高重复率环形马迈雪夫振荡器的演示,为实现非常简单和经济高效的全标准 PM 光纤马迈雪夫振荡器铺平了道路。
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引用次数: 0
Compressed computational imaging based on optical differentiation. 基于光学分辨的压缩计算成像。
IF 3.1 2区 物理与天体物理 Q2 OPTICS Pub Date : 2024-12-15 DOI: 10.1364/OL.535063
An Wang, Junfan Zhu, Jiguo Wu, Ling Ye, Xiong Liu, Yinghang Jiang, Yifan Wang, Yurong Liu, Rongchun Ge, Jinglei Du, Zhiyou Zhang

In computational imaging, getting better imaging quality with shorter time usage is always a challenging problem. The powerful compressed sensing functions as a backend algorithm, which leaves room for us to develop a methodology of compression in imaging systems. Optical differentiation was widely utilized in direct imaging to highlight the features of an image. We apply optical differentiation to compress information in the correlated imaging system. The experimental results indicate a significant improvement in the signal-to-noise ratio and imaging speed. In addition, this scheme enables phase imaging from the second-order correlation. Our work can spark potential applications in biological microscopic and scattering media imaging.

在计算成像领域,如何在更短的时间内获得更好的成像质量始终是一个具有挑战性的问题。功能强大的压缩传感作为一种后端算法,为我们在成像系统中开发压缩方法提供了空间。光学微分技术被广泛应用于直接成像,以突出图像的特征。我们在相关成像系统中应用光学分辨来压缩信息。实验结果表明,信噪比和成像速度都有显著提高。此外,该方案还能通过二阶相关性实现相位成像。我们的研究成果有望应用于生物显微成像和散射介质成像。
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引用次数: 0
Intelligent open-set MIMO recognition in OWC using a Siamese neural network.
IF 3.1 2区 物理与天体物理 Q2 OPTICS Pub Date : 2024-12-15 DOI: 10.1364/OL.543826
Yinan Zhao, Chen Chen, Hailin Cao, Zhihong Zeng, Min Liu, Harald Haas

Multiple-input multiple-output (MIMO) technology, a core component of 6G, has been widely adopted in optical wireless communication (OWC) systems. Accurate recognition of different MIMO types is essential for MIMO selection and demodulation. In this Letter, we propose an open-set MIMO recognition method for OWC systems using a Siamese neural network (SNN). Simulation results show that the SNN significantly outperforms other recognition approaches, including convolutional neural networks (CNNs) and traditional machine learning techniques. For SNN-based recognition, over 90% accuracy is achieved with training based on only nine fixed sampling points in both 2 × 2 and 4 × 4 MIMO-OWC systems.

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引用次数: 0
Metasurface-based functional optical splitter for a spatially parallelized dual-polarization coherent modulator.
IF 3.1 2区 物理与天体物理 Q2 OPTICS Pub Date : 2024-12-15 DOI: 10.1364/OL.541473
Chun Ren, Kento Komatsu, Go Soma, Yoshiaki Nakano, Takuo Tanemura

We propose a surface-normal dual-polarization in-phase and quadrature modulator (DP-IQM) that employs a thin dielectric metasurface (MS) layer inserted on a high-speed electro-absorptive modulator array. The metasurface provides the functionalities of all the passive components necessary for a DP-IQM, including a polarization beam splitter/combiner and an interferometric circuit, to a normal-incident beam. A dielectric metasurface composed of silicon nanoposts is designed and fabricated to experimentally demonstrate polarization and beam splitting functionalities with a phase error of less than 0.08 rad and a power imbalance of less than 0.9 dB. These small errors correspond to an error-vector magnitude of less than 7% when it is used to generate dual-polarization quaternary phase-shift-keying (DP-QPSK) or 16 quadrature amplitude modulation (DP-16QAM) signals. The surface-normal configuration of our scheme allows scaling to a large two-dimensional (2D) array to generate spatially parallelized DP coherent signals for various applications, including optical communication, computing, and sensing.

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引用次数: 0
Observing high dependence of red luminescence on localized symmetry in Mn4+ activated inverse spinel phosphors.
IF 3.1 2区 物理与天体物理 Q2 OPTICS Pub Date : 2024-12-15 DOI: 10.1364/OL.544994
Chenyang Li, Yimin Zhou, Fei Tang

Localized symmetry has been shown to significantly impact the luminescence behavior of Mn4+ ions through the electron-phonon coupling process. Building on this characteristic, three types of inverse spinel structure oxides (Mg2XO4, where X = Ti, Ti/Ge, Ge) doped with Mn4+ were developed, exhibiting strong red emission when exposed to UV and blue light. A thorough examination reveals that the symmetric improvement of the Mn4+ sites within the octahedral environment leads to significant changes in their luminescence behavior, including a suppression of zero-phonon-line (ZPL) emission, a blueshift, and an extension of the luminescence lifetime. Moreover, variable-temperature PL spectra of phosphors are carefully measured. Low-temperature PL spectra demonstrate three distinct sharp emission peaks for Mg2GeO4:Mn4+, while Mg2TiO4:Mn4+ exhibits a broad emission band. The average primary phonon energies involved in the vibronic processes are determined through theoretical fitting of temperature-dependent PL intensities. Lastly, the luminescence dynamics associated with anti-Stokes, ZPL, and Stokes emissions are analyzed. The observed increase in luminescence lifetime indicates a significant impact of the localized environment on luminescence properties.

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引用次数: 0
Ultra-sensitive liquid crystal-coated microbubble resonator based on a whispering gallery mode for penicillin G detection.
IF 3.1 2区 物理与天体物理 Q2 OPTICS Pub Date : 2024-12-15 DOI: 10.1364/OL.542428
Peiyao An, Xiaolei Hao, Shanshan Zhang, Mengxiao Li, Chuan Wang, Mingxiang Yang, Miao Yu, Jun Ren, Rensheng Shen, Zhenlin Wu

Penicillin G detection is of great significance in medical research and disease diagnosis. Liquid crystal (LC), as a branch of sensitive materials, has a broad application prospect in the field of biosensing. Herein, a liquid crystal-coated silica microbubble resonator (LC-MBR), with high sensitivity for penicillin G detection, has been proposed and demonstrated. Whispering gallery mode (WGM) spectra with a Q factor exceeding 106 were excited through the coupling between tapered fiber and LC-MBR. The orientation transition of the LC molecules, combined with WGM resonance, amplified target information and triggered wavelength blueshifts. LC-MBR was then applied in pH detection, achieving a sensitivity of 2.51 nm/pH within a pH range of 3.8-8.5. This resonator was also successfully employed to detect enzymatic reactions of penicillinase, with a detection limit of 6 × 103 U/mL. The fabricated sensor offers significant advantages, including a simple structure, improved stability, and higher sensitivity across a wide pH detection range, making it a promising candidate for future biomedical applications.

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引用次数: 0
Experimental retrieval of metaholographic images via evanescent wave using a single-layer nanostructure for encryption.
IF 3.1 2区 物理与天体物理 Q2 OPTICS Pub Date : 2024-12-15 DOI: 10.1364/OL.542690
Yingxin Xie, Tian Huang, Zhiwei Huang, Yongquan Zeng, Zile Li, Guoxing Zheng

Metasurfaces have demonstrated significant potential in optical encryption and anti-counterfeiting due to their incredible capability of manipulating various light properties. However, previous metasurface-encryption methods did not sufficiently explore the spatial frequency aspect, particularly regarding evanescent waves. Here, we propose an encryption scheme by introducing evanescent waves into the encoding and decoding processes. Different parts of the target image are individually encoded at distinct spatial frequencies within the evanescent-wave region. Only when an evanescent wave with a specific transverse wave vector (TWV) serves as the key can the complete target image be retrieved. Our work exemplifies a thorough exploration of the mathematical framework underlying metasurface-based holography. It enables the feasibility of a single metasurface in concealing and retrieving information in the evanescent-wave region, thus opening up a new, to our knowledge, methodology for high-security optical information encryption.

由于元表面具有令人难以置信的操纵各种光特性的能力,因此在光学加密和防伪方面显示出巨大的潜力。然而,以往的元表面加密方法并没有充分探索空间频率方面的问题,尤其是有关蒸发波的问题。在此,我们提出一种加密方案,在编码和解码过程中引入蒸发波。目标图像的不同部分分别以不同的空间频率在频散波区域内进行编码。只有当具有特定横波矢量(TWV)的蒸发波作为密钥时,才能检索到完整的目标图像。我们的工作体现了对基于元表面的全息技术的数学框架的深入探索。它使单个元表面在隐蔽和检索渐隐波区域信息方面具有可行性,从而为我们所知的高安全性光学信息加密开辟了一种新方法。
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引用次数: 0
Skin effect enhancement through symmetry breaking in reciprocal photonic crystals.
IF 3.1 2区 物理与天体物理 Q2 OPTICS Pub Date : 2024-12-15 DOI: 10.1364/OL.545841
Jinhong Xu, Ran Hao

Enhancing the skin effect in non-Hermitian photonic crystals has traditionally required alternating materials with different gain and loss characteristics inside the basic unit, which not only increases fabrication complexity but also faces limitations due to different material compatibility and material integrations. In this paper, a novel method is proposed that requires only one material but enables significant enhancement of the skin effect intensity by introducing spatial rotational symmetry breaking in two-dimensional reciprocal photonic crystals. Our result has shown a 306.09% improvement in skin effect intensity with just one material, if compared to previous designs. Our finding not only may broaden the theoretical framework of non-Hermitian optics but also demonstrates significant potential for practical applications in photonic integration, optical sensing, and laser design, thus opening up new possibilities for future photonic device innovations.

增强非赫米提光子晶体的趋肤效应传统上需要在基本单元内交替使用具有不同增益和损耗特性的材料,这不仅增加了制造复杂性,还面临着不同材料兼容性和材料集成度的限制。本文提出了一种新方法,只需要一种材料,但通过在二维互易光子晶体中引入空间旋转对称破缺,可显著增强集肤效应强度。结果表明,与之前的设计相比,只需一种材料,集肤效应强度就能提高 306.09%。我们的发现不仅可以拓宽非赫米提光学的理论框架,而且在光子集成、光学传感和激光器设计的实际应用中也显示出巨大的潜力,从而为未来光子设备的创新开辟了新的可能性。
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引用次数: 0
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Optics letters
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