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2018 IEEE ISAF-FMA-AMF-AMEC-PFM Joint Conference (IFAAP)最新文献

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Origins of Conduction at Domain Boundaries, LaAlO3/SrTiO3 and Surface for Depolarization & Size Effect 畴边界导电的起源,LaAlO3/SrTiO3和表面的退极化和尺寸效应
Pub Date : 2018-09-11 DOI: 10.1109/ISAF.2018.8463221
Yukio Watanabe, D. Matsumoto, Y. Urakami, M. Okano, A. Masuda
The conductions at domain boundaries due to ferroelectric polarization and LaAlO3/SrTiO3found by Ohtomo and Hwang [Nature 427, 423 (2004)] are intriguing. If these conductions are different from the conventional conductions at domain boundaries and oxide interfaces due to defects, they prove the earlier predictions [Phys. Rev. Lett. 86, 332(2001); Phys. Rev. B57, 789(1998)]. That is, when these conductions are primarily due to ferroelectric polarization as predicted, the foundations of mesoscale and nanoscale ferroelectrics should change. Considering conventional mechanisms including the high field effect as in the resistance switching (RRAM), we examine their origin and discuss these implications.
Ohtomo和Hwang发现的由铁电极化和LaAlO3/ srtio3引起的畴边界电导非常有趣[Nature 427, 423(2004)]。如果这些电导由于缺陷而与畴边界和氧化物界面的常规电导不同,它们就证明了早期的预测[物理学家]。Rev. Lett. 86, 332(2001);理论物理。Rev. B57, 789(1998)]。也就是说,当这些导电主要是由铁电极化引起时,中尺度和纳米尺度铁电体的基础应该改变。考虑到传统的机制,包括电阻开关(RRAM)中的高场效应,我们研究了它们的起源并讨论了这些影响。
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引用次数: 0
Domain Switching by Applied Electric Field in (001) and (111)-epitaxial (K0.5Na0.5)NbO3Films 外加电场在(001)和(111)-外延(K0.5Na0.5) nbo3薄膜中的畴切换
Pub Date : 2018-07-10 DOI: 10.1109/ISAF.2018.8463311
M. Kawano, T. Yamada, S. Matsuo, M. Yoshino, T. Nagasaki, O. Sakata, Y. Imai
(K1-xNax)NbO3 (KNN) is especially paid attention to as a lead-free piezoelectric material. It is known that KNN has a morphotropic phase boundary (MPB) at $xsim 0.5$, which shows a high piezoelectric property. However, it has not been fully clarified how the domain structure of KNN changes by applied electric field. In this study, we observed electric field-induced strain and domain fraction change of KNN films by synchrotron X-ray diffraction.
(K1-xNax)NbO3 (KNN)作为一种无铅压电材料尤其受到关注。已知KNN在$xsim 0.5$处具有向晶相边界(MPB),表现出较高的压电性能。然而,对于外加电场如何改变KNN的畴结构,目前还没有完全阐明。在本研究中,我们用同步x射线衍射观察了KNN薄膜的电场致应变和畴分数变化。
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引用次数: 0
Data-Mining Driven Design for Novel Perovskite-type Piezoceramics 新型钙钛矿型压电陶瓷的数据挖掘驱动设计
Pub Date : 2018-05-01 DOI: 10.1109/ISAF.2018.8463245
Jian Yu, Jun Yu Li, Yinglong Jiang, J. Chu
Materials Genome Initiative is envisioning the discovery, development, manufacturing and deployment of advanced materials twice as fast and at a fraction of cost. High throughput computation and experimentation will generate big data, which underscores the emergence of the fourth paradigm data science. In contrast to machine-learning needing big-data, data-mining assisted by domain knowledge and expertise works well with a limited number of data. In this presentation, data-mining based on material genome approach were performed in field of perovskite-type oxides. New ferroelectric ceramics based on BiFeO3 for high temperature piezoelectric applications are realized with piezoresponse of 1.5~4.0 times the present commercial non-perovskite counterpart. Our essay demonstrates data-mining driven searching sure able to reduce time-to-insight and human effort on synthesization, accelerating new materials discovery and deployment.
“材料基因组计划”(Materials Genome Initiative)正在设想以两倍的速度和一小部分成本发现、开发、制造和部署先进材料。高通量计算和实验将产生大数据,这强调了第四种范式数据科学的出现。与需要大数据的机器学习不同,由领域知识和专业知识辅助的数据挖掘可以很好地处理有限数量的数据。本文在钙钛矿型氧化物领域进行了基于材料基因组方法的数据挖掘。基于BiFeO3的新型铁电陶瓷实现了高温压电应用,其压电响应是目前商用非钙钛矿同类产品的1.5~4.0倍。我们的论文展示了数据挖掘驱动的搜索确实能够减少洞察时间和人工合成的工作量,加速新材料的发现和部署。
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引用次数: 1
Control of Leakage Current through BaTiO3 Film by Cumulative Cycle of Applied Voltage Scanning for ReRAM or Neuromorphic Application 应用累积周期电压扫描法控制BaTiO3薄膜泄漏电流的研究
Pub Date : 2018-05-01 DOI: 10.1109/ISAF.2018.8463232
S. Maejima, M. Uchida, M. Noda
We found a new phenomenon that shows a large change in leakage current through BaTiO3(BTO) film with the maximum ratio of 107 to 109 observed in this work by changing cumulative cycle of voltage scan applied on the film capacitor. These leakage phenomena are thought to depend on several factors such as BTO film thickness, concentration of $V_{0}^{+}$, bias voltage, its sweep rate and so on, because trapping/detrapping of carrier electron into/from oxygen vacancy would be a competition dependent on their rates and concentrations. These results imply that the leakage current can be controlled by some sequences or protocols of applied voltage scan, leading to use for ReRAM or neuromorphic applications.
通过改变扫描电压的累积周期,我们发现通过BaTiO3(BTO)薄膜的漏电流发生了较大的变化,最大比值为107比109。这些泄漏现象被认为取决于几个因素,如BTO膜厚度,$V_{0}^{+}$的浓度,偏置电压,其扫描速率等,因为载流子电子进入/从氧空位中捕获/脱出将是一种依赖于它们的速率和浓度的竞争。这些结果表明,泄漏电流可以通过施加电压扫描的某些序列或协议来控制,从而用于ReRAM或神经形态应用。
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引用次数: 0
Piezoelectric Ultrasonic Microsensors on Buckled Diaphragms Using Sol-Gel Derived PZT Films 基于溶胶-凝胶衍生PZT薄膜的屈曲膜片压电超声微传感器
Pub Date : 2018-05-01 DOI: 10.1109/ISAF.2018.8463278
K. Yamashita, Shōta Nakajima, Jo Shiomi, M. Noda, P. Muralt
Piezoelectric ultrasonic microsensors with a PZT (lead-zirconate-titanate) capacitor on a buckled diaphragm were fabricated and deposition condition of the sol-gel derived PZT films was investigated from the viewpoint of high mechano-electrical conversion efficiency. The buckling of the diaphragm affects the conversion efficiency in the geometrical aspect and is influenced by the residual stress of the diaphragm. The films were deposited through various thermal treatment in the sol-gel process; four pyrolysis temperatures and two first-crystallized gel film thickness, and were evaluated in their stress and ferroelectric property. The thickness of the gel film affected the crystallographic orientation, (100) or (111), of the film, and dominated the film stress and remanent polarization, e.g., the stress and polarization of the (100)-oriented films were smaller than those of the (lll)-oriented films, meaning the (100) orientation is better in the stress but worse in the remanent polarization than (111) orientation. The pyrolysis temperature was then precisely controlled and finally orientation-distributed samples were fabricated and evaluated. The samples with mixed orientation of (100) and (111) in around 50% showed intermediate stress and remanent polarization, and their sensitivity was enhanced by 1.4-4 times to those with (100) or (111) single oriented films.
制作了一种带压电薄膜的压电超声微传感器,并从高机电转换效率的角度研究了溶胶-凝胶PZT薄膜的沉积条件。膜片的屈曲在几何方面影响着转换效率,并受膜片残余应力的影响。采用溶胶-凝胶法对薄膜进行各种热处理;研究了四种热解温度和两种初晶凝胶膜厚度,并对其应力和铁电性能进行了评价。凝胶膜的厚度影响膜的晶体取向(100)或(111),并支配膜的应力和残余极化,例如(100)取向的膜的应力和极化小于(ll)取向的膜,说明(100)取向比(111)取向的应力好,但残余极化差。然后精确控制热解温度,最终制备出取向分布的样品并进行评价。(100)和(111)混合取向在50%左右的样品表现出中等应力和残余极化,其灵敏度比(100)或(111)单一取向的样品提高了1.4 ~ 4倍。
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引用次数: 1
Vibration Mode Analyses for Circular Wedge Acoustic Waveguides 圆楔声波导振动模态分析
Pub Date : 2018-05-01 DOI: 10.1109/ISAF.2018.8463226
Tai-Ho Yu
A bi-dimensional finite element model based on Hamilton's principle and the finite element method is developed in this study to analyze the dispersive characteristics and mode shapes of normal modes for circular wedge acoustic waveguides. The dispersion curves of phase velocities for guided waves and their corresponding resonant frequencies for a circular wedge waveguide were also evaluated by 3D finite element analysis (FEA) using the commercial ANSYS code. The convergence of guided waves was discussed. The 3D FEA was limited in terms of calculating for higher normal modes due to constraints in the available number of elements. The bi-dimensional finite element method is based on the separation of variables, with the wave propagation factor being separated from cross-sectional vibrations of the acoustic waveguides. The present method has advantages in terms of being able to determine phase velocities and mode shapes up to higher normal modes and in a wide range of frequencies without loss of accuracy. The phase velocities of the anti-symmetric flexural (ASF) guided waves in circular wedge waveguides were found to be slower than the Rayleigh wave speed. Furthermore, the calculated results in the range of higher wave numbers were in good agreement with the empirical formula provided by Lagasse [1]. The ASF waves in circular cylindrical wedge-typed waveguides were found to have faster and frequency-dependent phase velocities in the range of lower wave numbers. This phenomenon results from the boundary conditions on the bottom of waveguides, which are different from the ideal wedge problem considered in Lagasse's work. In addition, the curvatures of the acoustic waveguides were found to increase the phase velocities of higher normal modes only.
基于Hamilton原理和有限元方法建立了楔形圆波导的二维有限元模型,分析了楔形圆波导正模的色散特性和模态振型。利用商用ANSYS软件对楔形圆波导进行了三维有限元分析,得到了导波相速度的色散曲线及其对应的谐振频率。讨论了导波的收敛性。由于可用单元数量的限制,三维有限元分析在计算较高正态模态方面受到限制。二维有限元法基于变量分离,将声波传播因子与声波导的截面振动分离。本方法的优点在于能够在不损失精度的情况下确定高阶正态模态和宽频率范围内的相速度和模态形状。在楔形圆波导中,发现反对称弯曲导波的相速度比瑞利波速慢。在较高波数范围内的计算结果与Lagasse[1]提供的经验公式吻合较好。在较低波数范围内,发现圆柱楔形波导中的ASF波具有更快且与频率相关的相速度。这种现象的产生是由于波导底部的边界条件不同于Lagasse工作中考虑的理想楔形问题。此外,发现声波导的曲率只会增加高正法模的相速度。
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引用次数: 1
Piezoelectric Resonating Force Sensor in the Second Vibration Mode 第二振型压电谐振力传感器
Pub Date : 2018-05-01 DOI: 10.1109/ISAF.2018.8463273
K. Yamashita, P. Muralt
A resonating force sensor is studied, which is composed of a metal bridge coated with a piezoelectric film for force detection. It is thought to operate the sensor at the second flexural vibration mode having one node at the center of the bridge. Resonance frequency and piezoelectric coupling are investigated in the frame of an analytical model, and compared with finite element analysis (FEA) in a desired force range. The resonance frequency-force relation derived from the analytical model is close the the FEA result in the force range. The coupling factor-force relation from the analytical model agrees with the one from FEA in the small force region, but it shows lower coupling than the FEA result in the large force region.
研究了一种谐振式力传感器,该传感器是在金属桥上涂覆一层压电薄膜,用于力检测。它被认为在第二弯曲振动模式下操作传感器,在桥梁中心有一个节点。在解析模型框架下研究了谐振频率和压电耦合,并在期望的力范围内与有限元分析(FEA)进行了比较。解析模型得到的共振频率-力关系在力范围内与有限元分析结果接近。解析模型的耦合系数-力关系在小力区与有限元分析结果一致,但在大力区与有限元分析结果的耦合较低。
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引用次数: 0
An Ag Decorated P(VDF-CTFE)/BT@HBP@PDA Nanocomposites with Double-Shell Core Structure for High Dielectric Performance 高介电性能Ag修饰P(VDF-CTFE)/BT@HBP@PDA纳米复合材料
Pub Date : 2018-05-01 DOI: 10.1109/ISAF.2018.8463253
W. Xia, Yalin Yin, Junhong Xing, Ning Zhang, Zhuo Xu
A core-shell inorganic/polymer materials with abundant compositions and multiple shapes have attracted many attentions recently for their harmonious interfacial compatibility, high dielectric performance, and thereby the prospect of applications in energy storage devices. In this work, for improving the interfacial compatibility of in organiclpolymer nanocomposites, the BaTiO3 (BT) nano-powders are coated successively by using double shell polyamide (HBP) and dopamine (PDA) that is decorated with nanoscale Ag particles. In addition, a P(VDF-CTFE) with high breakdown electric field and proper dielectric permittivity are selected as the polymer matrix, and the flexible 0–3 nanocomposite of Ag decorated P(VDF-CTFE)/BT@HBP@PDA films with ~20μm in thickness are obtained through spin-casting method. The morphologies from FESEM show that the interface between BaTiO3 and P(VDF-CTFE) has been improved significantly and BaTiO3 is homogeneous dispersion in the polymer matrix. Consequently, the multicomponent nanocomposites possess the large dielectric permittivity (εr~40) and a low dielectric loss tangent (0.1 Hz) since the ionic polarization of BaTiO3 and the penetration effect of electrons. The result provides an effective way of interfacial improving that through various mutual promoting mediums to achieve high dielectric performance composite materials for their potential applications in energy storage areas.
一种成分丰富、形状多样的核壳无机高分子材料以其和谐的界面相容性和高介电性能,在储能器件中具有广阔的应用前景,近年来备受关注。为了提高有机聚合物纳米复合材料的界面相容性,本文采用双壳聚酰胺(HBP)和多巴胺(PDA)包覆BaTiO3 (BT)纳米粉末,并以纳米级银粒子装饰。此外,选择具有高击穿电场和适当介电常数的P(VDF-CTFE)作为聚合物基体,通过自旋浇铸法制备了厚度约20μm的Ag修饰P(VDF-CTFE)/BT@HBP@PDA薄膜的柔性0-3纳米复合材料。FESEM形貌分析表明,BaTiO3与P(VDF-CTFE)之间的界面明显改善,BaTiO3在聚合物基体中均匀分散。由于BaTiO3的离子极化和电子的穿透作用,复合材料具有较大的介电常数(εr~40)和较低的介电损耗正切(0.1 Hz)。研究结果为通过多种介质相互促进实现高介电性能复合材料在储能领域的潜在应用提供了一条有效的界面改善途径。
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引用次数: 1
Ferromagnetism in barium titanate nanoparticles. Effect of annealing in hydrogen atmosphere on magnetic properties 钛酸钡纳米颗粒的铁磁性。氢气氛退火对磁性能的影响
Pub Date : 2018-05-01 DOI: 10.1109/ISAF.2018.8463349
N. A. Emelianov, L. Korotkov, W. M. Al Mandalawi, M. Kashirin, J. Roldan López, T. N. Korotkova
Dependences of magnetization on magnetic field strength were studied for both the nanostructured and the bulk ferroelectric barium titanate. It has been found that nanostructured barium titanate demonstrates ferroelectric, ferromagnetic and diamagnetic properties simultaneously. The annealing of nanostructured barium titanate in hydrogen atmosphere under experimental conditions leads to a significant increase of the spontaneous magnetization and decrease of the diamagnetic response. Analysis of experimental results shows that defects in grains surfaces of the barium titanate nanoparticles (probably oxygen vacancies) are mainly responsible for electron states, which produce ferromagnetic and diamagnetic responses.
研究了纳米结构铁电钛酸钡和块状铁电钛酸钡的磁化强度与磁场强度的关系。纳米钛酸钡同时具有铁电性、铁磁性和抗磁性。在实验条件下,将纳米钛酸钡在氢气气氛中退火后,其自发磁化强度显著提高,抗磁响应显著降低。实验结果分析表明,钛酸钡纳米颗粒表面的缺陷(可能是氧空位)是电子态产生的主要原因,这些电子态产生铁磁和抗磁响应。
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引用次数: 3
Investigating the effects of losses of a piezoelectric transducer in temperature varying environment through Finite Element Analysis 通过有限元分析研究了变温环境下压电换能器损耗的影响
Pub Date : 2018-05-01 DOI: 10.1109/ISAF.2018.8463347
T. Meurisse, Dragan Damjanovic
Piezoelectric ultrasonic transducers are used in many situations, including system and structural health monitoring and for non-destructive testing. For this, a piezoelectric resonator is used to actuate a structure and produce the sound waves that interact with the system under investigation and are then analysed. The behavior of such transducers is dependent on their environment, e.g., on the temperature. The mechanical parameters of the metals can be significantly changed if the temperature modification is large. Furthermore, the piezoelectric materials have their coefficients and losses modified by temperature changes. While the temperature behavior of the piezoelectric and metal can be independently determined experimentally, the role of the temperature change on the transducer performance and generated sound level is not well understood. In this paper, a simple transducer intended for high-temperature applications is investigated using Finite Element Analysis. A piezoelectric disc resonator is glued under a fixed stainless steel membrane, with parameters for the glue considered as those of gold. Effects of losses on the fundamental resonance of the admittance of the transducer and on the sound level it produces are investigated between 20°C and 300°C. Increasing the temperature reduces the resonance frequency of the transducer while maintaining the sound level at resonance. An error of one order of magnitude in input elastic losses of the piezoelectric material will have a stronger effect on the transducer admittance at every frequency than a similar error in the input dielectric and piezoelectric losses.
压电超声换能器应用于许多场合,包括系统和结构健康监测以及无损检测。为此,使用压电谐振器来驱动结构并产生声波,这些声波与所研究的系统相互作用,然后进行分析。这种换能器的性能取决于它们的环境,例如温度。当温度变化较大时,金属的力学参数会发生明显的变化。此外,压电材料的系数和损耗随温度的变化而变化。虽然压电和金属的温度行为可以通过实验独立确定,但温度变化对换能器性能和产生声级的作用尚不清楚。本文研究了一种用于高温应用的简单换能器。将压电圆盘谐振器粘在固定的不锈钢膜下,胶的参数与黄金一样。在20°C和300°C之间,研究了损耗对换能器导纳的基本共振及其产生的声级的影响。升高温度降低了换能器的共振频率,同时保持了共振时的声级。压电材料输入弹性损耗的一个数量级误差对换能器在每个频率上的导纳的影响比输入介电和压电损耗的类似误差更大。
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引用次数: 1
期刊
2018 IEEE ISAF-FMA-AMF-AMEC-PFM Joint Conference (IFAAP)
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