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Innovative carbon nanotubes-bridging strategy valorizes plastic waste into high-quality H2-rich syngas while suppressing CO2 emissions 创新性碳纳米管桥接战略可将塑料废弃物转化为高质量的富含 H2- 的合成气,同时抑制二氧化碳排放
IF 16.2 1区 环境科学与生态学 Q1 ENVIRONMENTAL SCIENCES Pub Date : 2024-05-06 DOI: 10.1016/j.oneear.2024.04.005
Xuesong Zhang, Ge Kong, Yuan Jiang, Linling Zhou, Kejie Wang, Xin Zhang, Guanya Ji, Lujia Han

Plastic waste disposal is mounting, with consequences for both environmental and human wellbeing. Addressing the plastic waste challenge through chemically upcycling waste to other products is gaining momentum but can have trade-offs. For example, the conversion of plastic waste into hydrogen rich gas can be achieved via catalytic steam, but this process can release large quantities of CO2 (∼12 kg CO2 per 1 kg H2 production). High-performance bifunctional catalysts, such as carbon nanotubes (CNTs), offer a potential solution, but suppressing CO2 emissions without compromising H2-rich gas yield remains challenging. Here, we synthesize a new CNTs-bridging nanocomposite by integrating Ni nanoparticles with HY zeolite. Employing this bifunctional CNTs-bridging nanocomposite in the catalytic steam reforming of polyethylene can achieve high-quality H2 yields of up to 2,340 mL/gplastic and a 77% reduction in CO2 emissions (1.68 g CO2 per 1 g H2 production). This work introduces an innovative CNTs-bridging strategy to valorize plastic waste into high-quality H2-rich syngas while suppressing CO2 emissions.

塑料垃圾的处理量不断增加,对环境和人类福祉都造成了影响。通过将废弃物转化为其他产品的化学升级再循环方法来应对塑料废弃物挑战的势头日益强劲,但这一方法可能会产生一些利弊。例如,可通过催化蒸汽将塑料垃圾转化为富氢气体,但这一过程会释放大量二氧化碳(每生产 1 千克氢气释放 12 千克二氧化碳)。高性能双功能催化剂,如碳纳米管(CNT),提供了一种潜在的解决方案,但在不影响富氢气体产量的情况下抑制二氧化碳排放仍然具有挑战性。在这里,我们通过将镍纳米颗粒与 HY 沸石相结合,合成了一种新型 CNT 桥接纳米复合材料。在聚乙烯催化蒸汽转化过程中使用这种双功能 CNTs-桥接纳米复合材料,可获得高达 2,340 mL/gplastic 的高质量 H2 产率,并减少 77% 的 CO2 排放(每生产 1 g H2 产生 1.68 g CO2)。这项工作介绍了一种创新的碳纳米管桥接策略,可将塑料废弃物转化为富含高质量 H2- 的合成气,同时抑制二氧化碳排放。
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引用次数: 0
Accelerating social tipping points in sustainable behaviors: Insights from a dynamic model of moralized social change 加速可持续行为的社会临界点:道德化社会变革动态模型的启示
IF 16.2 1区 环境科学与生态学 Q1 ENVIRONMENTAL SCIENCES Pub Date : 2024-05-03 DOI: 10.1016/j.oneear.2024.04.004
Madeline Judge, Thijs Bouman, Linda Steg, Jan Willem Bolderdijk

To address the climate crisis, it is important to accelerate social tipping points in the adoption of sustainable behaviors. Social tipping points describe the process whereby small changes trigger self-perpetuating feedback loops and produce a fundamental transformation in the social system. The current literature does not adequately address how the moralized nature of sustainable behaviors could lead to unique tipping trajectories. In this Perspective, we propose a dynamic model of moralized social change that provides insights on how novel sustainable behaviors spread over society and how to speed up this process. Although moralization may initially generate social friction that delays tipping points, it can accelerate change at later stages by increasing social pressure on laggards. By implementing early system-level changes, policymakers can help reduce the initial inertia created by moralization and accelerate social tipping points. We discuss how our model can inform the decisions of activists, policymakers, professionals, and researchers.

为了应对气候危机,必须加快可持续行为的社会临界点。社会临界点描述了这样一个过程:微小的变化会引发自我持续的反馈循环,并在社会系统中产生根本性的转变。目前的文献没有充分论述可持续行为的道德化性质如何导致独特的临界点轨迹。在本视角中,我们提出了一个道德化社会变革的动态模型,为新型可持续行为如何在社会中传播以及如何加快这一过程提供了见解。虽然道德化最初可能会产生社会摩擦,从而推迟临界点的出现,但它可以通过增加对落后者的社会压力来加速后期阶段的变革。通过尽早实施系统层面的变革,政策制定者可以帮助减少道德化最初产生的惰性,加速社会临界点的到来。我们将讨论我们的模型如何为活动家、决策者、专业人士和研究人员的决策提供参考。
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引用次数: 0
Global spatially explicit carbon emissions from land-use change over the past six decades (1961–2020) 过去六十年(1961-2020 年)土地利用变化产生的全球空间显性碳排放
IF 16.2 1区 环境科学与生态学 Q1 ENVIRONMENTAL SCIENCES Pub Date : 2024-04-30 DOI: 10.1016/j.oneear.2024.04.002
Zhangcai Qin, Yakun Zhu, Josep G. Canadell, Min Chen, Tingting Li, Umakant Mishra, Wenping Yuan

Land-use change (LUC) is a major source of global anthropogenic carbon emissions that contribute to climate change. However, current estimates of LUC-induced emissions vary widely with differences in data and models, making it challenging to identify and manage emissions hotspots by location and LUC activity. Here, we estimated spatially explicit carbon fluxes associated with global major gross land-use transitions based on a new bookkeeping model (i.e., LUCE). Between 1961 and 2020, LUC induced 215 and 142 Pg C of global carbon emissions and removals, respectively, resulting in average net emissions (ELUC) of 1.21 Pg C year−1. Latin America, Southeast Asia, and Sub-Saharan Africa dominated global ELUC with 69% of 60-year cumulative emissions, or about 86% between 2001 and 2020. Forest-related LUC activities (e.g., deforestation, reforestation) contributed largely to both regional and global carbon fluxes. Our findings shed new light on identifying LUC-induced emissions hotspots and managing land for climate mitigation and conservation.

土地利用变化(LUC)是导致气候变化的全球人为碳排放的主要来源。然而,由于数据和模型的差异,目前对土地利用变化引起的排放的估计差别很大,这使得按地点和土地利用变化活动来识别和管理排放热点具有挑战性。在此,我们基于一个新的簿记模型(即 LUCE)估算了与全球主要土地利用总转变相关的空间明确碳通量。从 1961 年到 2020 年,土地利用变化引起的全球碳排放量和碳清除量分别为 215 和 142 Pg C,平均净排放量(ELUC)为每年 1.21 Pg C。拉丁美洲、东南亚和撒哈拉以南非洲在全球碳排放和碳清除中占主导地位,占 60 年累计排放量的 69%,或 2001 至 2020 年间的约 86%。与森林相关的土地利用变化活动(如毁林、重新造林)在很大程度上造成了地区和全球的碳通量。我们的研究结果为识别土地利用变化引起的排放热点以及管理土地以减缓和保护气候提供了新的思路。
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引用次数: 0
Enhanced but highly variable biodiversity outcomes from coastal restoration: A global synthesis 海岸恢复带来的生物多样性成果得到了加强,但差异很大:全球综述
IF 16.2 1区 环境科学与生态学 Q1 ENVIRONMENTAL SCIENCES Pub Date : 2024-04-19 DOI: 10.1016/j.oneear.2024.02.013
Michael Sievers, Rod M. Connolly, Kimberly A. Finlayson, Michaela E. Kitchingman, Andria Ostrowski, Ryan M. Pearson, Mischa P. Turschwell, Maria F. Adame, Ana B. Bugnot, Ellen Ditria, Robin Hale, Brian R. Silliman, Stephen E. Swearer, Stephanie R. Valdez, Christopher J. Brown
Coastal ecosystems are being restored to combat environmental degradation and biodiversity loss. Colonization of restored sites by non-habitat-forming animals improves outcomes for ecosystems and society, yet there has been no review of how animals respond to coastal restoration. Here, we extracted 5,133 response ratios from 160 studies to show how coastal ecosystem restoration benefits animals as individuals, populations, and communities. Abundances and diversity at restored sites were greater than at degraded (61% and 35%, respectively) and unstructured (42% and 37%) control sites and similar to those at natural reference sites (both within 2%). Individuals in restored sites were similar in condition to those within control and reference sites. However, responses among projects were highly variable and rarely related to restored site maturity or characteristics, presenting a challenge for predicting outcomes and highlighting the need to improve restoration techniques, monitoring, and reporting. Nevertheless, studies so far suggest coastal restoration benefits biodiversity.
为了应对环境退化和生物多样性丧失,人们正在恢复沿海生态系统。非栖息地动物在恢复地点的定殖改善了生态系统和社会的结果,但目前还没有关于动物如何对海岸恢复做出反应的综述。在此,我们从 160 项研究中提取了 5,133 个响应比率,以说明海岸生态系统恢复如何使动物个体、种群和群落受益。恢复地点的丰度和多样性高于退化(分别为 61% 和 35%)和非结构化(分别为 42% 和 37%)对照地点,与自然参照地点的丰度和多样性相似(均在 2% 以内)。恢复地点的个体状况与对照地点和参考地点的个体状况相似。然而,各项目之间的反应差异很大,而且很少与恢复地点的成熟度或特征有关,这对预测结果提出了挑战,并突出了改进恢复技术、监测和报告的必要性。不过,迄今为止的研究表明,海岸恢复有利于生物多样性。
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引用次数: 0
Understanding insect movements through space and time is vital for safeguarding global ecosystem services 了解昆虫的时空移动对保护全球生态系统服务至关重要
IF 16.2 1区 环境科学与生态学 Q1 ENVIRONMENTAL SCIENCES Pub Date : 2024-04-19 DOI: 10.1016/j.oneear.2024.03.007
Tomas Roslin
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引用次数: 0
Insect vectors on the move 移动中的昆虫病媒
IF 16.2 1区 环境科学与生态学 Q1 ENVIRONMENTAL SCIENCES Pub Date : 2024-04-19 DOI: 10.1016/j.oneear.2024.03.012
Manju Rahi, Henk van den Berg, Indra Vythilingam, Raman Velayudhan
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引用次数: 0
How climate change might impact insect movement via physiological mechanisms 气候变化如何通过生理机制影响昆虫的活动
IF 16.2 1区 环境科学与生态学 Q1 ENVIRONMENTAL SCIENCES Pub Date : 2024-04-19 DOI: 10.1016/j.oneear.2024.03.008
John S. Terblanche, Susana Clusella-Trullas, Philipp Lehmann
Climate change is altering the abundance and geographic distributions of insects, with potential consequences for human health, sustainable agriculture, and ecosystem function. How insects will be affected during their routine movements by climate-change-associated warming remains poorly understood. Here, we therefore review the potential impacts of, and mechanisms involved in coping with, heat stress during movement from an ecophysiological perspective. Within a movement ecology framework, we propose key ecophysiology attributes that support insect movement with warming conditions. By identifying major knowledge gaps and focusing on movement-related traits discussed here, future studies can further strengthen mechanistic links between functional traits and insect redistribution under climate change and, therefore, provide more robust forecasting tools.
气候变化正在改变昆虫的数量和地理分布,可能对人类健康、可持续农业和生态系统功能产生影响。人们对昆虫在日常活动中如何受到气候变化相关变暖的影响仍然知之甚少。因此,我们在此从生态生理学的角度回顾了热应激在昆虫运动过程中的潜在影响和应对机制。在运动生态学框架内,我们提出了在气候变暖条件下支持昆虫运动的关键生态生理学属性。通过确定主要的知识差距并关注本文讨论的与运动相关的特征,未来的研究可以进一步加强功能特征与气候变化下昆虫重新分布之间的机理联系,从而提供更可靠的预测工具。
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引用次数: 0
The global reach of citizen science for monitoring insects 公民科学监测昆虫的全球影响力
IF 16.2 1区 环境科学与生态学 Q1 ENVIRONMENTAL SCIENCES Pub Date : 2024-04-19 DOI: 10.1016/j.oneear.2024.03.009
Helen E. Roy, Angeliki F. Martinou, Michael J.O. Pocock, Victoria Werenkraut, David B. Roy
Biodiversity is declining rapidly. The most important causes of biodiversity loss are climate change, land- and sea-use change, invasive alien species, pollution, and overexploitation of natural resources. This unprecedented deterioration of the biosphere has profound and far-reaching consequences for insects, who play many important roles within ecosystems, including pollination and decomposition. Declines in the abundance and distribution of insects threaten these essential ecosystem functions. While there is no doubt that urgent and immediate measures are needed to address biodiversity loss and climate change, monitoring of insects is a priority to underpin and inform ongoing conservation action. Citizen science has emerged as an important tool for monitoring insects. In this primer, we explain the application of citizen science for monitoring insects and emerging approaches using digital technologies.
生物多样性正在迅速减少。造成生物多样性丧失的最重要原因是气候变化、土地和海洋使用的变化、外来物种入侵、污染和自然资源的过度开发。生物圈前所未有的恶化对昆虫产生了深远的影响,因为昆虫在生态系统中发挥着许多重要作用,包括授粉和分解。昆虫数量和分布的减少威胁着这些重要的生态系统功能。毫无疑问,我们需要立即采取紧急措施来应对生物多样性的丧失和气候变化,而对昆虫的监测则是支持和指导当前保护行动的当务之急。公民科学已成为监测昆虫的重要工具。在这篇入门文章中,我们将介绍公民科学在监测昆虫方面的应用,以及利用数字技术的新兴方法。
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引用次数: 0
Insect diversity for agroecosystem resilience in a changing climate 昆虫多样性促进农业生态系统在不断变化的气候中的恢复能力
IF 16.2 1区 环境科学与生态学 Q1 ENVIRONMENTAL SCIENCES Pub Date : 2024-04-19 DOI: 10.1016/j.oneear.2024.03.003
Ingolf Steffan-Dewenter, Rachel Bezner Kerr, Marcell Karl Peters
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引用次数: 0
Q&A with Dr. Stanley Burgiel 斯坦利-伯吉尔博士问答
IF 16.2 1区 环境科学与生态学 Q1 ENVIRONMENTAL SCIENCES Pub Date : 2024-04-19 DOI: 10.1016/j.oneear.2024.03.014
Stanley Burgiel
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引用次数: 0
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One Earth
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