Pub Date : 2024-09-02DOI: 10.1134/S1063778824700534
Yu. Senichev, A. Aksentyev, S. Kolokolchikov, A. Melnikov, N. Nikolaev, V. Ladygin, E. Syresin
To search for proton Electric Dipole Moments (EDM) using proton storage ring with purely electrostatic elements, the concept of frozen spin method has been proposed by Brookhaven National Laboratory. This method is based on two facts: in the equation of spin precession, the magnetic field dependence is entirely eliminated, and at the ‘‘magic’’ energy, the spin precession frequency coincides with the precession frequency of the particle momentum. In case of deuteron, we have to use the electrical and magnetic field simultaneously, keeping the frozen spin direction along the momentum as in the pure electrostatic ring. Later, Yu. Senichev proposed the concept of quasi-frozen spin, in which the spin oscillates around the direction of the pulse within half the value of the advanced phase of rotation in magnetic arcs, each time returning back in deflectors with an electrostatic field. Due to the low value of the anomalous magnetic moment of deuteron, an effective contribution to the expected EDM effect is reduced only by a few percent compared with frozen spin method. In this work, we consider the adapted structure of the NICA and Nuclotron synchrotrons, in which the ‘‘quasi-frozen spin’’ option can be implemented. The advantage of the ‘‘quasi-frozen spin’’ concept is the possibility of using synchrotrons already existing in the world that are not focused on studying EDM, which makes this method the only one possible for the accelerators of the NICA complex.
摘要 为了利用纯静电元素的质子贮存环来寻找质子电偶极矩(EDM),布鲁克海文国家实验室提出了冷冻自旋法的概念。这种方法基于两个事实:在自旋前驱方程中,磁场依赖性被完全消除;在 "神奇 "能量下,自旋前驱频率与粒子动量的前驱频率重合。对于氘核,我们必须同时使用电场和磁场,像在纯静电环中一样保持沿动量的冻结自旋方向。后来,尤.塞尼切夫提出了准冻结自旋的概念,在这种情况下,自旋在磁弧中围绕脉冲方向振荡,振荡幅度不超过旋转提前阶段值的一半,每次振荡都会在带有静电场的偏转器中返回。由于氘核的反常磁矩值较低,与冷冻自旋法相比,对预期放电加工效应的有效贡献只减少了百分之几。在这项工作中,我们考虑了 NICA 和 Nuclotron 同步加速器的调整结构,在这种结构中可以实施 "准冻结自旋 "选项。准冷冻自旋''概念的优点是可以使用世界上现有的不专注于研究电火花放电的同步加速器,这使得这种方法成为 NICA 综合加速器唯一可能的方法。
{"title":"NICA Facilities for the Search for EDM Light Nuclei","authors":"Yu. Senichev, A. Aksentyev, S. Kolokolchikov, A. Melnikov, N. Nikolaev, V. Ladygin, E. Syresin","doi":"10.1134/S1063778824700534","DOIUrl":"10.1134/S1063778824700534","url":null,"abstract":"<p>To search for proton Electric Dipole Moments (EDM) using proton storage ring with purely electrostatic elements, the concept of frozen spin method has been proposed by Brookhaven National Laboratory. This method is based on two facts: in the equation of spin precession, the magnetic field dependence is entirely eliminated, and at the ‘‘magic’’ energy, the spin precession frequency coincides with the precession frequency of the particle momentum. In case of deuteron, we have to use the electrical and magnetic field simultaneously, keeping the frozen spin direction along the momentum as in the pure electrostatic ring. Later, Yu. Senichev proposed the concept of quasi-frozen spin, in which the spin oscillates around the direction of the pulse within half the value of the advanced phase of rotation in magnetic arcs, each time returning back in deflectors with an electrostatic field. Due to the low value of the anomalous magnetic moment of deuteron, an effective contribution to the expected EDM effect is reduced only by a few percent compared with frozen spin method. In this work, we consider the adapted structure of the NICA and Nuclotron synchrotrons, in which the ‘‘quasi-frozen spin’’ option can be implemented. The advantage of the ‘‘quasi-frozen spin’’ concept is the possibility of using synchrotrons already existing in the world that are not focused on studying EDM, which makes this method the only one possible for the accelerators of the NICA complex.</p>","PeriodicalId":728,"journal":{"name":"Physics of Atomic Nuclei","volume":"87 4","pages":"436 - 441"},"PeriodicalIF":0.3,"publicationDate":"2024-09-02","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://link.springer.com/content/pdf/10.1134/S1063778824700534.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142198570","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2024-09-02DOI: 10.1134/S106377882470042X
L. P. Kaptari, O. P. Solovtsova
We present a new relativistic expression for the Sommerfeld–Gamow–Sakharov factor ((S)-factor) of a composite system of two spin-1/2 particles of arbitrary masses interacting via a via a Coulomb-like chromodynamical potential. The analysis is performed in the framework of a relativistic quasipotential approach based on the Hamiltonian formulation of the covariant quantum field theory in the relativistic configuration representation suggested by A.A. Logunov, A.N. Tavkhelidze and V.G. Kadyshevsky. The pseudoscalar, vector and pseudovector systems are considered and the behavior of the (S)-factor near the threshold and in the relativistic limit is investigated in detail. It is argued that at the threshold the contribution of spins significantly reduces the Sommerfeld effect, while at ultrarelativistic velocities their role diminishes and the (S)-factor becomes basically the same as for the spinless systems.
{"title":"Spin Effects in the Sommerfeld–Gamow–Sakharov Factor","authors":"L. P. Kaptari, O. P. Solovtsova","doi":"10.1134/S106377882470042X","DOIUrl":"10.1134/S106377882470042X","url":null,"abstract":"<p>We present a new relativistic expression for the Sommerfeld–Gamow–Sakharov factor (<span>(S)</span>-factor) of a composite system of two spin-1/2 particles of arbitrary masses interacting via a via a\u0000Coulomb-like chromodynamical potential. The analysis is performed in the framework of a relativistic quasipotential approach based on the Hamiltonian formulation of the covariant quantum field theory in the relativistic configuration representation suggested by A.A. Logunov, A.N. Tavkhelidze and V.G. Kadyshevsky. The pseudoscalar, vector and pseudovector systems are considered and the behavior of the <span>(S)</span>-factor near the threshold and in the relativistic limit is investigated in detail. It is argued that at the threshold the contribution of spins significantly reduces the Sommerfeld effect, while at ultrarelativistic velocities their role diminishes and the <span>(S)</span>-factor becomes basically the same as for the spinless systems.</p>","PeriodicalId":728,"journal":{"name":"Physics of Atomic Nuclei","volume":"87 4","pages":"476 - 482"},"PeriodicalIF":0.3,"publicationDate":"2024-09-02","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142198576","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2024-09-02DOI: 10.1134/S1063778824700480
I. N. Borzov, S. V. Tolokonnikov
The strength distributions of charge exchange spin-dipole excitations are calculated in the continuum quasiparticle random-phase approximation based on the Fayans density functional with modified isovector part. An impact of the isovector parameter (h_{2}^{-}) of the DF3-f functional on the strength functions of charge-exchange spin-dipole excitations ((0^{-}), (1^{-}), (2^{-})) are studied for ({}^{208})Pb, ({}^{132})Sn and ({}^{90})Zr. The sum rules are calculated using both ground state radii and direct integration of the total SD strength distributions. A comparison with the experimental SD sum rule in ({}^{90})Zr gives one a possibility to check previously estimated (h_{2}^{-}) values which described well the recent combined estimate for (Delta R_{np}) in ({}^{208})Pb and corresponding equation of state parameters – symmetry energy (J_{0}=J(rho_{0})) and a slope parameter (L_{0}=L(rho_{0})).
{"title":"Spin-Dipole Strengths and Neutron Skin Thickness of ({}^{{90}})Zr, ({}^{{132}})Sn, ({}^{{208}})Pb","authors":"I. N. Borzov, S. V. Tolokonnikov","doi":"10.1134/S1063778824700480","DOIUrl":"10.1134/S1063778824700480","url":null,"abstract":"<p>The strength distributions of charge exchange spin-dipole excitations are calculated in the continuum quasiparticle random-phase approximation based on the Fayans density functional with modified isovector part. An impact of the isovector parameter <span>(h_{2}^{-})</span> of the DF3-f functional on the strength functions of charge-exchange spin-dipole excitations (<span>(0^{-})</span>, <span>(1^{-})</span>, <span>(2^{-})</span>) are studied for <span>({}^{208})</span>Pb, <span>({}^{132})</span>Sn and <span>({}^{90})</span>Zr. The sum rules are calculated using both ground state radii and direct integration of the total SD strength distributions. A comparison with the experimental SD sum rule in <span>({}^{90})</span>Zr gives one a possibility to check previously estimated <span>(h_{2}^{-})</span> values which described well the recent combined estimate for <span>(Delta R_{np})</span> in <span>({}^{208})</span>Pb and corresponding equation of state parameters – symmetry energy <span>(J_{0}=J(rho_{0}))</span> and a slope parameter <span>(L_{0}=L(rho_{0}))</span>.</p>","PeriodicalId":728,"journal":{"name":"Physics of Atomic Nuclei","volume":"87 4","pages":"541 - 547"},"PeriodicalIF":0.3,"publicationDate":"2024-09-02","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://link.springer.com/content/pdf/10.1134/S1063778824700480.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142198587","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2024-09-02DOI: 10.1134/S1063778824700479
N. N. Nikolaev, F. Rathmann, J. Slim
A measurement of the spin observables in external target and storage ring experiments requires a comparison of interactions of oppositely polarized beams. The ideal way to reduce systematic effects is to store bunches of opposite polarization in the same fill. Here we discuss how such bunches can be organized based on the extended pilot-bunch principle.
{"title":"Alternating Spin Polarity Bunches in Storage Rings","authors":"N. N. Nikolaev, F. Rathmann, J. Slim","doi":"10.1134/S1063778824700479","DOIUrl":"10.1134/S1063778824700479","url":null,"abstract":"<p>A measurement of the spin observables in external target and storage ring experiments requires a comparison of interactions of oppositely polarized beams. The ideal way to reduce systematic effects is to store bunches of opposite polarization in the same fill. Here we discuss how such bunches can be organized based on the extended pilot-bunch principle.</p>","PeriodicalId":728,"journal":{"name":"Physics of Atomic Nuclei","volume":"87 4","pages":"442 - 446"},"PeriodicalIF":0.3,"publicationDate":"2024-09-02","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142198578","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2024-09-02DOI: 10.1134/S1063778824700406
A. V. Karpishkov, V. A. Saleev, K. K. Shilyaev
The production of polarized (J/psi) mesons at the NICA (Nuclotron based Ion Collider fAcility) energy of (sqrt{s}=27) GeV is studied on the basis of the generalized parton model in the leading order of perturbative QCD. The hadronization of a (cbar{c}) quark pair to a (J/psi) meson is described within the model of nonrelativistic QCD. Nonperturbative model parameters are determined on the basis of a comparison with available experimental data on the production of prompt (J/psi) mesons at the energies of (sqrt{s}=19.4) GeV (NA3) and (sqrt{s}=200) GeV (PHENIX).
Abstract The production of polarized (J/psi) mesons at the NICA (Nuclotron based Ion Collider fAcility) energy of (sqrt{s}=27) GeV is studied on the basis of the generalized parton model in the leading order of perturbative QCD.在非相对论QCD模型中描述了一个(cbar{c})夸克对到一个(J/psi)介子的强子化。非微扰模型参数是在与能量为 (sqrt{s}=19.4) GeV (NA3)和 (sqrt{s}=200) GeV (PHENIX)时产生瞬时 (J/psi) 介子的现有实验数据进行比较的基础上确定的。
{"title":"Production of Polarized ({J/}psi) Mesons within Nonrelativistic QCD and Generalized Parton Model","authors":"A. V. Karpishkov, V. A. Saleev, K. K. Shilyaev","doi":"10.1134/S1063778824700406","DOIUrl":"10.1134/S1063778824700406","url":null,"abstract":"<p>The production of polarized <span>(J/psi)</span> mesons at the NICA (Nuclotron based Ion Collider fAcility) energy of <span>(sqrt{s}=27)</span> GeV is studied on the basis of the generalized parton model in the leading order of perturbative QCD. The hadronization of a <span>(cbar{c})</span> quark pair to a <span>(J/psi)</span> meson is described within the model of nonrelativistic QCD. Nonperturbative model parameters are determined on the basis of a comparison with available experimental data on the production of prompt <span>(J/psi)</span> mesons at the energies of <span>(sqrt{s}=19.4)</span> GeV (NA3) and <span>(sqrt{s}=200)</span> GeV (PHENIX).</p>","PeriodicalId":728,"journal":{"name":"Physics of Atomic Nuclei","volume":"87 4","pages":"494 - 497"},"PeriodicalIF":0.3,"publicationDate":"2024-09-02","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142198579","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2024-09-02DOI: 10.1134/S1063778824700492
O. V. Selyugin, O. V. Teryaev
Taking into account the recent parameterizations of parton distribution functions (PDFs), the momentum transfer dependence of generalized parton distributions (GPDs) of nucleons is obtained in the limit (xito 0). The gravitational quark and gluon form factors of nucleons are calculated. It is shown that the gluon gravitational radius of the nucleon is comparable to the electromagnetic radius of the proton. The power dependence of form factors is investigated. As a result, it was obtained that the quark gravitational form factor is reproduced by the dipole form, while the form of the gluon gravitation form factor corresponds to the triple form.
{"title":"GPDs and Gravitational Form Factors of Nucleons (Quark and Gluon Contributions)","authors":"O. V. Selyugin, O. V. Teryaev","doi":"10.1134/S1063778824700492","DOIUrl":"10.1134/S1063778824700492","url":null,"abstract":"<p>Taking into account the recent parameterizations of parton distribution functions (PDFs), the momentum transfer dependence of generalized parton distributions (GPDs) of nucleons is obtained in the limit <span>(xito 0)</span>. The gravitational quark and gluon form factors of nucleons are calculated. It is shown that the gluon gravitational radius of the nucleon is comparable to the electromagnetic radius of the proton. The power dependence of form factors is investigated. As a result, it was obtained that the quark gravitational form factor is reproduced by the dipole form, while the form of the gluon gravitation form factor corresponds to the triple form.</p>","PeriodicalId":728,"journal":{"name":"Physics of Atomic Nuclei","volume":"87 4","pages":"518 - 522"},"PeriodicalIF":0.3,"publicationDate":"2024-09-02","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://link.springer.com/content/pdf/10.1134/S1063778824700492.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142198582","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2024-09-02DOI: 10.1134/S1063778824700509
D. M. Rodkin, Yu. M. Tchuvil’sky
Based on the ab initio scheme developed by the authors for calculating the asymptotic characteristics of decay channels of nuclear states—the method of orthogonal functions of cluster channels—an approach has been created that makes it possible to directly implement the results of ab initio calculations of (A)-nucleon wave functions, as well as the partial decay widths of resonant states of compound nucleus obtained through their use, into calculations of cross sections for resonance nuclear reactions. Both calculated and reliably measured resonance energies can be employed in these calculations. Using the examples of such a theoretical analysis of the reaction cross sections for ({}^{7}textrm{Li}(p,{}^{4}textrm{He})^{4})He and ({}^{7}textrm{Be}(n,{}^{4}textrm{He}){}^{4})He, the efficiency of this approach and the wide prospects of its use in nuclear spectroscopy are demonstrated.
{"title":"Calculation of Cross Sections for Resonance Nuclear Reactions Based on Ab Initio Computations of Spectral Characteristics of Light Nuclei Levels","authors":"D. M. Rodkin, Yu. M. Tchuvil’sky","doi":"10.1134/S1063778824700509","DOIUrl":"10.1134/S1063778824700509","url":null,"abstract":"<p>Based on the ab initio scheme developed by the authors for calculating the asymptotic characteristics of decay channels of nuclear states—the method of orthogonal functions of cluster channels—an approach has been created that makes it possible to directly implement the results of ab initio calculations of <span>(A)</span>-nucleon wave functions, as well as the partial decay widths of resonant states of compound nucleus obtained through their use, into calculations of cross sections for resonance nuclear reactions. Both calculated and reliably measured resonance energies can be employed in these calculations. Using the examples of such a theoretical analysis of the reaction cross sections for <span>({}^{7}textrm{Li}(p,{}^{4}textrm{He})^{4})</span>He and <span>({}^{7}textrm{Be}(n,{}^{4}textrm{He}){}^{4})</span>He, the efficiency of this approach and the wide prospects of its use in nuclear spectroscopy are demonstrated.</p>","PeriodicalId":728,"journal":{"name":"Physics of Atomic Nuclei","volume":"87 4","pages":"548 - 560"},"PeriodicalIF":0.3,"publicationDate":"2024-09-02","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142198611","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2024-09-02DOI: 10.1134/S1063778824700364
P. O. Kazinski, A. A. Sokolov
An explicit expression for the probability of twisted-photon absorption by an atomic nucleus is obtained. It is found that photoabsorption by nuclei lying in the vicinity of the axis along which a twisted photon propagates obeys the selection rule (jgeqslant|m_{gamma}|), where (m_{gamma}) is the projection of the photon total angular momentum and (j) is the multipolarity of the nuclear transition. In the long-wavelength limit, the (j=|m_{gamma}|) multipole transition makes a dominant contribution to the probability for twisted-photon absorption. The absorption coefficient for twisted photons is found for a target that consists of many nuclei.
{"title":"Excitation of Multipolar Transitions in Nuclei by Twisted Photons","authors":"P. O. Kazinski, A. A. Sokolov","doi":"10.1134/S1063778824700364","DOIUrl":"10.1134/S1063778824700364","url":null,"abstract":"<p>An explicit expression for the probability of twisted-photon absorption by an atomic nucleus is obtained. It is found that photoabsorption by nuclei lying in the vicinity of the axis along which a twisted photon propagates obeys the selection rule <span>(jgeqslant|m_{gamma}|)</span>, where <span>(m_{gamma})</span> is the projection of the photon total angular momentum and <span>(j)</span> is the multipolarity of the nuclear transition. In the long-wavelength limit, the <span>(j=|m_{gamma}|)</span> multipole transition makes a dominant contribution to the probability for twisted-photon absorption. The absorption coefficient for twisted photons is found for a target that consists of many nuclei.</p>","PeriodicalId":728,"journal":{"name":"Physics of Atomic Nuclei","volume":"87 4","pages":"561 - 569"},"PeriodicalIF":0.3,"publicationDate":"2024-09-02","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142198613","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2024-09-02DOI: 10.1134/S1063778824700285
A. Melnikov, A. Aksentyev, Yu. Senichev, S. Kolokolchikov
The main features of the quasi-frozen spin lattice were calculated in the spinor formalism, such as a spin-tune and a direction of the invariant spin axis. As the radial field perturbations play a crucial role in the EDM measurement procedure, the difference of frozen and quasi-frozen spin lattices was investigated in this regard.
{"title":"Quasi-Frozen Spin Concept at NICA for EDM Search and Its Matrix Analysis","authors":"A. Melnikov, A. Aksentyev, Yu. Senichev, S. Kolokolchikov","doi":"10.1134/S1063778824700285","DOIUrl":"10.1134/S1063778824700285","url":null,"abstract":"<p>The main features of the quasi-frozen spin lattice were calculated in the spinor formalism, such as a spin-tune and a direction of the invariant spin axis. As the radial field perturbations play a crucial role in the EDM measurement procedure, the difference of frozen and quasi-frozen spin lattices was investigated in this regard.</p>","PeriodicalId":728,"journal":{"name":"Physics of Atomic Nuclei","volume":"87 4","pages":"447 - 450"},"PeriodicalIF":0.3,"publicationDate":"2024-09-02","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142198574","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
The nuclear tracks created in poly allyl diglycol carbonate (PADC type CR-39) due to exposure to (alpha) particles for specific times followed by chemical etching for definite time periods at 4, 7, 11, and 13 hours are prepared. The measured IR spectrum for investigated films clarified a decrease in peak intensity against increase in etched layer thickness (ELT). This is argued to the formation of free radicals due to etching. Furthermore, pyrolysis of the investigated films displayed that the actual structural variation occurs in the second and third stages of degradation. The calculated activation energy values for thermal decomposition of studied PADC exhibited an increase against etching time periods. Other thermal parameters such as enthalpy, Gibbs free energy, and entropy are calculated and discussed. Moreover, the two nonlinear optical parameters, second-order index of refraction ((n_{2})) and third-order nonlinear optical susceptibility, (chi^{(3)}), are also calculated and displayed that (n_{2}) and (chi^{(3)}) increase by one order of magnitude against the irradiation times which is attributed to the structural damage due to irradiation by (alpha) particle.
Abstract The nuclear track created in poly allyl diglycol carbonate (PADC type CR-39) is prepared due to exposure to (α) particles for specific times followed by chemical etching for definite time periods at 4, 7, 11, and 13 hours.所测得的红外光谱表明,随着蚀刻层厚度(ELT)的增加,峰值强度也在降低。这与蚀刻过程中自由基的形成有关。此外,所研究薄膜的热分解显示,实际的结构变化发生在降解的第二和第三阶段。所研究的 PADC 的热分解活化能计算值随着蚀刻时间的延长而增加。计算并讨论了其他热参数,如焓、吉布斯自由能和熵。此外,还计算了两个非线性光学参数:二阶折射率((n_{2})和三阶非线性光学感度((chi^{(3)}),结果表明(n_{2})和(chi^{(3)})随着辐照时间的延长而增加了一个数量级,这归因于(alpha)粒子辐照造成的结构损伤。
{"title":"Dependence of Structure Variation, Pyrolysis, and Nonlinear Optical Dispersion on the Chemical Etching of Poly Allyl Diglycol Carbonate (PADC) Irradiated with ({alpha})-Particles","authors":"Heba Abdelmaksoud, Nabil El-Faramawy, Fathy Abdel-Wahab","doi":"10.1134/S1063778824700303","DOIUrl":"10.1134/S1063778824700303","url":null,"abstract":"<p>The nuclear tracks created in poly allyl diglycol carbonate (PADC type CR-39) due to exposure to <span>(alpha)</span> particles for specific times followed by chemical etching for definite time periods at 4, 7, 11, and 13 hours are prepared. The measured IR spectrum for investigated films clarified a decrease in peak intensity against increase in etched layer thickness (ELT). This is argued to the formation of free radicals due to etching. Furthermore, pyrolysis of the investigated films displayed that the actual structural variation occurs in the second and third stages of degradation. The calculated activation energy values for thermal decomposition of studied PADC exhibited an increase against etching time periods. Other thermal parameters such as enthalpy, Gibbs free energy, and entropy are calculated and discussed. Moreover, the two nonlinear optical parameters, second-order index of refraction (<span>(n_{2})</span>) and third-order nonlinear optical susceptibility, <span>(chi^{(3)})</span>, are also calculated and displayed that <span>(n_{2})</span> and <span>(chi^{(3)})</span> increase by one order of magnitude against the irradiation times which is attributed to the structural damage due to irradiation by <span>(alpha)</span> particle.</p>","PeriodicalId":728,"journal":{"name":"Physics of Atomic Nuclei","volume":"87 4","pages":"399 - 413"},"PeriodicalIF":0.3,"publicationDate":"2024-09-02","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142198569","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}