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Unraveling the mechanism of catalytic water oxidation via de novo synthesis of reactive intermediate 通过重新合成反应中间体揭示催化水氧化的机理
Pub Date : 2020-03-06 DOI: 10.1021/jacs.9b10265.s001
A. K. Ravari
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引用次数: 0
Poking and buckling of pressurized spherical shells 受压球壳的戳戳和屈曲
Pub Date : 2020-03-05 DOI: 10.26226/morressier.5f5f8e69aa777f8ba5bd6016
A. Abbasi, Dong Yan, M. Pezzulla, P. Reis
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引用次数: 0
Morphological Control of Multifunctional Melting Gel Coatings via Electrospray Deposition 多功能熔融凝胶涂层的电喷涂形态学控制
Pub Date : 2020-03-05 DOI: 10.7282/T3-YT1J-R755
A. Gamboa, Lin Lei, J. Mercado, J. Guzmán, L. Klein, A. Jitianu, J. Singer
{"title":"Morphological Control of Multifunctional Melting Gel Coatings via Electrospray Deposition","authors":"A. Gamboa, Lin Lei, J. Mercado, J. Guzmán, L. Klein, A. Jitianu, J. Singer","doi":"10.7282/T3-YT1J-R755","DOIUrl":"https://doi.org/10.7282/T3-YT1J-R755","url":null,"abstract":"","PeriodicalId":9375,"journal":{"name":"Bulletin of the American Physical Society","volume":"90 1","pages":""},"PeriodicalIF":0.0,"publicationDate":"2020-03-05","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"83934133","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
A truly-programmable mechanical metamaterial using magnetic actuation 一种真正可编程的机械超材料,采用磁驱动
Pub Date : 2020-03-05 DOI: 10.26226/morressier.5f5f8e69aa777f8ba5bd608f
Tian Chen
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引用次数: 0
Electric field modulation of magnetism in ferrimagnetic Heusler heterostructures 铁磁Heusler异质结构中磁场的电场调制
Pub Date : 2020-03-05 DOI: 10.1103/physrevb.101.134419
Qilong Sun, Sohee Kwon, M. Stamenova, S. Sanvito, N. Kioussis
To date the realization of magnetoresistive random access memory (RAM) and magnetoelectric RAM (MeRAM) devices relies primarily on ultrathin ferromagnetic-based (FeCoB/MgO) magnetic tunnel junctions. On the other hand, the Heusler family of intermetallics is considered very promising for spintronic applications. Nevertheless, the voltage controlled magnetic anisotropy (VCMA) in ultrathin Heusler-based magnetic-tunnel junction stacks remains unexplored. Here, using the ferrimagnetic Heusler ${mathrm{Mn}}_{3}mathrm{Ga}$ as a prototype system, we report ab initio calculations of the electric field modulation of magnetism in the $mathrm{Ir}/{mathrm{Mn}}_{3}mathrm{Ga}$/MgO heterostructure. The trilayer structures with one and three monolayer Ir caps and Mn-Mn termination exhibit large perpendicular magnetic anisotropy in contrast to those with Mn-Ga termination which yield in-plane magnetization orientation. We predict giant VCMA coefficients the magnitude and sign of which depend on both the interface termination and the Ir cap thickness. The underlying atomistic mechanism lies on the electric-field-induced shifts of the spin-orbit coupling energies of the spin-polarized $mathrm{Ir}/d$ orbitals with different orbital angular momentum symmetries. Our paper paves the way for exploiting the unique magnetic properties of ferrimagnetic Heusler compounds for next generation MeRAM devices.
迄今为止,磁阻随机存取存储器(RAM)和磁电RAM (MeRAM)器件的实现主要依赖于超薄铁磁(FeCoB/MgO)磁隧道结。另一方面,Heusler族金属间化合物被认为是非常有前途的自旋电子应用。然而,超薄heusler基磁隧道结堆的电压控制磁各向异性(VCMA)仍未被探索。本文以铁磁Heusler ${mathrm{Mn}}_{3}mathrm{Ga}$为原型系统,从头计算了$mathrm{Ir}/{mathrm{Mn}}_{3}mathrm{Ga}$/MgO异质结构中的电场调制磁场。具有一个和三个单层Ir帽和Mn-Mn端部的三层结构表现出较大的垂直磁各向异性,而具有Mn-Ga端部的结构则产生平面内磁化取向。我们预测了巨大的VCMA系数,其大小和符号取决于界面终端和Ir帽厚度。潜在的原子机制在于具有不同轨道角动量对称的自旋极化$ mathm {Ir}/d$轨道的自旋轨道耦合能的电场诱导位移。我们的论文为下一代MeRAM器件开发铁磁性Heusler化合物的独特磁性铺平了道路。
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引用次数: 10
Electrospray deposition of nanowire forests through spinodal gelation 电喷雾沉积纳米线森林通过spinodinal gelation
Pub Date : 2020-03-05 DOI: 10.1021/scimeetings.0c03444
Lin Lei, Catherine J. Nachtigal, Shensheng Chen, Tyler F. Moy, Xin Yong, J. Singer
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引用次数: 0
3D self-replication of DNA nanostructures DNA纳米结构的三维自我复制
Pub Date : 2020-03-04 DOI: 10.1021/scimeetings.0c01581
Feng Zhou, Heng Ni, R. Sha, N. Seeman, P. Chaikin
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引用次数: 0
Magneto-elastic coupling in multiferroic metal-organic framework [(CH3)2NH2]Co(HCOO)3 多铁金属-有机骨架[(CH3)2NH2]Co(HCOO)3的磁弹性耦合
Pub Date : 2020-03-04 DOI: 10.1063/9.0000147
K. Thirunavukkuarasu, R. Richardson, Zhengguang Lu, D. Smirnov, Nan Huang, N. Combs, G. Pokharel, D. Mandrus
Metal-organic frameworks based on metal-formates have emerged as a intriguing class of multiferroics with wide range of applications. In this work, we present magneto-Raman spectroscopic investigations on [(CH3)2NH2]Co(HCOO)3 belonging to this family. The spectroscopic studies were performed at magnetic fields up to 31 T at the temperature of 2.3 K. It was observed that the formate bending mode at around 798 cm−1 shifts to higher energies with increasing magnetic field. The magneto-response of the phonon also exhibits anomalies at magnetic fields of 14.5 T and 23.5 T corresponding to magnetic phase transitions. Based on our results, we conclude that the formate bending mode does play a role in facilitating the saturation of magnetic states similar to its Mn and Ni analogs.
基于金属甲酸盐的金属有机骨架是一类具有广泛应用前景的多铁材料。在这项工作中,我们对属于该家族的[(CH3)2NH2]Co(HCOO)3进行了磁拉曼光谱研究。在2.3 K的温度下,在31 T的磁场下进行光谱研究。结果表明,在798 cm−1附近,随着磁场的增加,甲酸盐弯曲模式向高能量方向转变。声子的磁响应在14.5 T和23.5 T的磁场下也表现出与磁相变相对应的异常。基于我们的研究结果,我们得出结论,甲酸盐弯曲模式确实在促进类似于Mn和Ni类似物的磁态饱和方面发挥了作用。
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引用次数: 0
Broadband sensitivity improvement via coherent quantum feedback with PT-symmetry 利用pt对称的相干量子反馈提高宽带灵敏度
Pub Date : 2020-03-04 DOI: 10.1117/12.2586469
Xiang Li, M. Goryachev, Yiqiu Ma, M. Tobar, Chunnong Zhao, R. Adhikari, Yanbei Chen
A conventional resonant detector is often subject to a trade-off between bandwidth and peak sensitivity that can be traced back to quantum Cramer-Rao Bound. Anomalous dispersion has been shown to improve it by signal amplification and is thus more robust against decoherence, while it leads to instabilities. We propose a stable quantum amplifier applicable to linear systems operating at the fundamental detection limits, enabled by two-mode non-degenerate parametric amplification. At threshold, one mode of the amplifier forms a PT-symmetric system of original detector mode. Sensitivity improvements are shown for laser-interferometric gravitational-wave detectors and microwave cavity axion detectors.
传统的谐振探测器通常需要在带宽和峰值灵敏度之间进行权衡,这可以追溯到量子Cramer-Rao边界。反常色散已被证明可以通过信号放大来改善它,因此对退相干具有更强的鲁棒性,但它会导致不稳定性。我们提出了一种稳定的量子放大器,适用于在基本检测极限下工作的线性系统,通过双模非简并参数放大实现。在阈值处,放大器的一个模式形成原始检测器模式的pt对称系统。激光干涉引力波探测器和微波腔轴子探测器的灵敏度得到了提高。
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引用次数: 11
(Invited) 2D NC-FET, FE-FET and FeS-FET
Pub Date : 2020-03-04 DOI: 10.1149/ma2020-01241370mtgabs
P. Ye
{"title":"(Invited) 2D NC-FET, FE-FET and FeS-FET","authors":"P. Ye","doi":"10.1149/ma2020-01241370mtgabs","DOIUrl":"https://doi.org/10.1149/ma2020-01241370mtgabs","url":null,"abstract":"","PeriodicalId":9375,"journal":{"name":"Bulletin of the American Physical Society","volume":"16 1","pages":""},"PeriodicalIF":0.0,"publicationDate":"2020-03-04","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"82150491","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
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