首页 > 最新文献

Green Energy and Resources最新文献

英文 中文
Corrigendum to “Effect of rich-MgO from low-calcium limestone on the calcination and properties of C4A3$-C2S clinker” [Green energy and Resources 2 (2024) 100099] “低钙石灰石中富mgo对C4A3$-C2S熟料煅烧和性能的影响”的勘误表[绿色能源与资源2 (2024)100099]
Pub Date : 2026-01-24 DOI: 10.1016/j.gerr.2025.100166
Yiping Qiu , Chengming Li , Yiqun Zhang , Yuan Feng , Sergei Leonovich , Piqi Zhao , Shoude Wang
{"title":"Corrigendum to “Effect of rich-MgO from low-calcium limestone on the calcination and properties of C4A3$-C2S clinker” [Green energy and Resources 2 (2024) 100099]","authors":"Yiping Qiu , Chengming Li , Yiqun Zhang , Yuan Feng , Sergei Leonovich , Piqi Zhao , Shoude Wang","doi":"10.1016/j.gerr.2025.100166","DOIUrl":"10.1016/j.gerr.2025.100166","url":null,"abstract":"","PeriodicalId":100597,"journal":{"name":"Green Energy and Resources","volume":"4 1","pages":"Article 100166"},"PeriodicalIF":0.0,"publicationDate":"2026-01-24","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"146039939","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Flamelet/progress variable modelling of turbulent non-premixed cool flames of dimethyl-ether/methane mixtures 二甲醚/甲烷混合物湍流非预混冷火焰的小火焰/进度变量模型
Pub Date : 2025-12-20 DOI: 10.1016/j.gerr.2025.100163
Weilin Zeng , Zeyang Pan , Xujiang Wang , Kai Hong Luo
In present work, the turbulent non-premixed cool flames of dimethyl-ether (DME)/methane mixtures are studied within the framework of flamelet/progress variable modelling and chemical kinetic analyses. The numerical setup is based on the Princeton CARAT burner configuration, and the accuracy of the hpmech-V3.3 chemistry to model turbulent low-temperature combustion is validated against the reference experiments and DNS. The simulation results reveal that turbulent cool flame structures are modified (lifted) by methane addition owing to the decline of cool flame extinction limits. The different flame regions associated with differing thermochemical characteristics for the dual-fuel lifted cool flames are uncovered. The DME/methane consumption trends suggest that methane addition inhibits the DME low-temperature oxidation. Through the kinetic analyses, the mechanisms are identified to be two-fold: methane competes with the DME H-abstraction reaction for OH radicals and the reaction of QOOH <=> O2 + 2CH2O is significantly slowed down with the methane addition. The mechanisms also kinetically explain the finding that the formation of CH2O, CO, CO2 in cool flames decline in response to the increase of methane blending ratios. The correlation between temperature and key intermediate formation is discovered.
本文在火焰/进程变量模型和化学动力学分析的框架下,对二甲醚/甲烷混合物的湍流非预混冷火焰进行了研究。数值模拟采用普林斯顿CARAT燃烧器结构,通过参考实验和DNS验证了hpmech-V3.3化学模型模拟湍流低温燃烧的准确性。模拟结果表明,甲烷的加入使冷火焰熄灭极限降低,从而改变(提升)了湍流冷火焰结构。揭示了与双燃料提升冷火焰不同热化学特性相关的不同火焰区域。二甲醚/甲烷消耗趋势表明,甲烷的加入抑制了二甲醚的低温氧化。通过动力学分析,确定了其机理有两方面:甲烷与二甲醚抽氢反应竞争OH自由基;甲烷的加入使QOOH <;=>; O2 + 2CH2O的反应明显减慢。该机理还从动力学上解释了在低温火焰中CH2O、CO、CO2的生成随甲烷混合比例的增加而减少的发现。发现了温度与关键中间地层的相关性。
{"title":"Flamelet/progress variable modelling of turbulent non-premixed cool flames of dimethyl-ether/methane mixtures","authors":"Weilin Zeng ,&nbsp;Zeyang Pan ,&nbsp;Xujiang Wang ,&nbsp;Kai Hong Luo","doi":"10.1016/j.gerr.2025.100163","DOIUrl":"10.1016/j.gerr.2025.100163","url":null,"abstract":"<div><div>In present work, the turbulent non-premixed cool flames of dimethyl-ether (DME)/methane mixtures are studied within the framework of flamelet/progress variable modelling and chemical kinetic analyses. The numerical setup is based on the Princeton CARAT burner configuration, and the accuracy of the hpmech-V3.3 chemistry to model turbulent low-temperature combustion is validated against the reference experiments and DNS. The simulation results reveal that turbulent cool flame structures are modified (lifted) by methane addition owing to the decline of cool flame extinction limits. The different flame regions associated with differing thermochemical characteristics for the dual-fuel lifted cool flames are uncovered. The DME/methane consumption trends suggest that methane addition inhibits the DME low-temperature oxidation. Through the kinetic analyses, the mechanisms are identified to be two-fold: methane competes with the DME H-abstraction reaction for OH radicals and the reaction of QOOH &lt;=&gt; O<sub>2</sub> + 2CH<sub>2</sub>O is significantly slowed down with the methane addition. The mechanisms also kinetically explain the finding that the formation of CH<sub>2</sub>O, CO, CO<sub>2</sub> in cool flames decline in response to the increase of methane blending ratios. The correlation between temperature and key intermediate formation is discovered.</div></div>","PeriodicalId":100597,"journal":{"name":"Green Energy and Resources","volume":"4 1","pages":"Article 100163"},"PeriodicalIF":0.0,"publicationDate":"2025-12-20","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"146039938","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
OpenFOAM-based study on near-field formation and mixing of high nozzle pressure ratio hydrogen jets from leakages 基于openfoam的高喷嘴压比泄漏氢射流近场形成与混合研究
Pub Date : 2025-12-18 DOI: 10.1016/j.gerr.2025.100164
Rui Jovan Yeo , T.H. New , W.L. Chan
A gas stored at high-pressure leaking through a small hole forms a complex series of shock structures as it accelerates and expands to ambient conditions. The near-field region of the jet includes the initial jet expansion, Mach disc formation, and starting vortices, all of which can affect hydrogen mixing with the surrounding air and have an associated combustion risk. Through the use of a modified OpenFOAM solver, simulations of hydrogen stored at 10 and 100 bar leaking into atmospheric conditions through 1.5 mm diameter circular nozzles were performed to determine the transient temperature profile, shock locations, and hydrogen mixing profiles of the hydrogen jet in its initial expansion and propagation stages. From these transient simulations, it was shown that starting vortices form pockets of mixed hydrogen and air that are within hydrogen flammability limits. This new simulation data shows mixed hydrogen pockets can linger in the nozzle near-field region and present a flammability risk that is not easily accounted for when using existing numerical models optimized for far-field flame behavior, showing this new open-source tool can resolve hydrogen mixing behavior in the nozzle near-field region without compromising on shock resolution capabilities.
储存在高压下的气体通过小孔泄漏,在加速膨胀到环境条件时,会形成一系列复杂的激波结构。射流的近场区域包括初始射流膨胀、马赫盘形成和起始涡,所有这些都会影响氢气与周围空气的混合,并具有相关的燃烧风险。通过使用改进的OpenFOAM求解器,模拟了储存在10和100 bar的氢气通过直径1.5 mm的圆形喷嘴泄漏到大气条件下,以确定氢气射流在初始膨胀和传播阶段的瞬态温度分布、激波位置和氢气混合分布。从这些瞬态模拟中可以看出,开始的涡流形成了氢和空气混合的小袋,这些小袋在氢可燃性的限制范围内。新的模拟数据显示,混合氢穴可以在喷嘴近场区域停留,并且在使用现有的远场火焰行为优化数值模型时,不容易解释可燃性风险,这表明这个新的开源工具可以解决喷嘴近场区域的氢混合行为,而不会影响冲击分辨率。
{"title":"OpenFOAM-based study on near-field formation and mixing of high nozzle pressure ratio hydrogen jets from leakages","authors":"Rui Jovan Yeo ,&nbsp;T.H. New ,&nbsp;W.L. Chan","doi":"10.1016/j.gerr.2025.100164","DOIUrl":"10.1016/j.gerr.2025.100164","url":null,"abstract":"<div><div>A gas stored at high-pressure leaking through a small hole forms a complex series of shock structures as it accelerates and expands to ambient conditions. The near-field region of the jet includes the initial jet expansion, Mach disc formation, and starting vortices, all of which can affect hydrogen mixing with the surrounding air and have an associated combustion risk. Through the use of a modified OpenFOAM solver, simulations of hydrogen stored at 10 and 100 bar leaking into atmospheric conditions through 1.5 mm diameter circular nozzles were performed to determine the transient temperature profile, shock locations, and hydrogen mixing profiles of the hydrogen jet in its initial expansion and propagation stages. From these transient simulations, it was shown that starting vortices form pockets of mixed hydrogen and air that are within hydrogen flammability limits. This new simulation data shows mixed hydrogen pockets can linger in the nozzle near-field region and present a flammability risk that is not easily accounted for when using existing numerical models optimized for far-field flame behavior, showing this new open-source tool can resolve hydrogen mixing behavior in the nozzle near-field region without compromising on shock resolution capabilities.</div></div>","PeriodicalId":100597,"journal":{"name":"Green Energy and Resources","volume":"4 1","pages":"Article 100164"},"PeriodicalIF":0.0,"publicationDate":"2025-12-18","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"146081282","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Mushroom-based high-efficiency solar evaporator for water harvesting 以蘑菇为基础的高效太阳能蒸发器
Pub Date : 2025-12-10 DOI: 10.1016/j.gerr.2025.100162
Hongjun Fu , Enhui Ma , Xinyang He , Chunyi Li , Jiahui Zhu , Qi Feng , Xinyi Liao , Wenxin Liu , Xiaodan Huang , Rongtai Yu
Solar-driven interfacial evaporation represents an innovative and highly promising strategy to address global freshwater scarcity and enhance water purification technologies. The distinctive structure of natural mushrooms, comprising a pileus and stipe, offers a feasible pathway for designing efficient and low-cost solar evaporators. In this work, natural mushrooms were employed as solar evaporators to evaluate their performance in evaporating seawater and sewage. Under 3.9 suns illumination, evaporation rates of 4.89, 4.57, and 3.73 kg·m−2·h−1 were achieved for sewage, deionized water, and seawater, respectively. Under natural sunlight conditions (0.5 sun), the mushroom evaporator attained rates of 2.62 and 2.13 kg·m−2·h−1 for sewage and seawater, respectively. The mushroom-based evaporator demonstrates not only exceptional photothermal conversion performance but also remarkable cycling stability and durability.
太阳能驱动的界面蒸发是解决全球淡水短缺和提高水净化技术的一种创新和非常有前途的战略。天然蘑菇的独特结构,包括菌柄和柱头,为设计高效、低成本的太阳能蒸发器提供了可行的途径。本研究以天然蘑菇作为太阳能蒸发器,考察其对海水和污水的蒸发性能。在3.9个太阳光照下,污水、去离子水和海水的蒸发速率分别为4.89、4.57和3.73 kg·m−2·h−1。在自然光照条件下(0.5太阳),蘑菇蒸发器对污水和海水的蒸发率分别为2.62和2.13 kg·m−2·h−1。该蒸发器不仅具有优异的光热转换性能,而且具有显著的循环稳定性和耐用性。
{"title":"Mushroom-based high-efficiency solar evaporator for water harvesting","authors":"Hongjun Fu ,&nbsp;Enhui Ma ,&nbsp;Xinyang He ,&nbsp;Chunyi Li ,&nbsp;Jiahui Zhu ,&nbsp;Qi Feng ,&nbsp;Xinyi Liao ,&nbsp;Wenxin Liu ,&nbsp;Xiaodan Huang ,&nbsp;Rongtai Yu","doi":"10.1016/j.gerr.2025.100162","DOIUrl":"10.1016/j.gerr.2025.100162","url":null,"abstract":"<div><div>Solar-driven interfacial evaporation represents an innovative and highly promising strategy to address global freshwater scarcity and enhance water purification technologies. The distinctive structure of natural mushrooms, comprising a pileus and stipe, offers a feasible pathway for designing efficient and low-cost solar evaporators. In this work, natural mushrooms were employed as solar evaporators to evaluate their performance in evaporating seawater and sewage. Under 3.9 suns illumination, evaporation rates of 4.89, 4.57, and 3.73 kg·m<sup>−2</sup>·h<sup>−1</sup> were achieved for sewage, deionized water, and seawater, respectively. Under natural sunlight conditions (0.5 sun), the mushroom evaporator attained rates of 2.62 and 2.13 kg·m<sup>−2</sup>·h<sup>−1</sup> for sewage and seawater, respectively. The mushroom-based evaporator demonstrates not only exceptional photothermal conversion performance but also remarkable cycling stability and durability.</div></div>","PeriodicalId":100597,"journal":{"name":"Green Energy and Resources","volume":"4 1","pages":"Article 100162"},"PeriodicalIF":0.0,"publicationDate":"2025-12-10","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"146081281","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Review of carbon capture and conversion with reactive magnesia cement materials 活性镁水泥材料碳捕集与转化研究进展
Pub Date : 2025-12-01 DOI: 10.1016/j.gerr.2025.100154
Yisong Liu , Linglin Xu , Zhiyuan Zhang , Changzai Ren , Dandan Sun , Yi Bao , Kai Wu
The high carbon emissions associated with the cement industry underscore the urgent need for low-carbon alternative materials. Compared with other alternatives, Reactive Magnesia Cement (RMC) offers the potential to absorb CO2. However, current research on RMC remains fragmented, lacking a systematic overview of its complete processing route. This review summarizes the carbonation mechanism of RMC and provides a comprehensive discussion of evaluation methods for its carbonation degree. In addition, the review provides an in-depth analysis of factors influencing carbonation and strategies to enhance it. Specifically, we categorize the mechanisms and evaluate the effectiveness of various methods, with an emphasis on environmentally friendly production processes to identify the most optimal approaches. Finally, the study highlights the carbon footprint of RMC and discusses the challenges associated with achieving low-carbon RMC production.
与水泥行业相关的高碳排放凸显了对低碳替代材料的迫切需求。与其他替代材料相比,活性镁水泥(RMC)具有吸收二氧化碳的潜力。然而,目前对RMC的研究仍然是碎片化的,缺乏对其完整加工路线的系统概述。综述了RMC的碳酸化机理,并对RMC碳酸化程度的评价方法进行了全面探讨。此外,本文还对影响碳酸化的因素和提高碳酸化的策略进行了深入分析。具体来说,我们对机制进行了分类,并评估了各种方法的有效性,重点是环境友好型生产过程,以确定最优方法。最后,该研究强调了RMC的碳足迹,并讨论了实现低碳RMC生产相关的挑战。
{"title":"Review of carbon capture and conversion with reactive magnesia cement materials","authors":"Yisong Liu ,&nbsp;Linglin Xu ,&nbsp;Zhiyuan Zhang ,&nbsp;Changzai Ren ,&nbsp;Dandan Sun ,&nbsp;Yi Bao ,&nbsp;Kai Wu","doi":"10.1016/j.gerr.2025.100154","DOIUrl":"10.1016/j.gerr.2025.100154","url":null,"abstract":"<div><div>The high carbon emissions associated with the cement industry underscore the urgent need for low-carbon alternative materials. Compared with other alternatives, Reactive Magnesia Cement (RMC) offers the potential to absorb CO<sub>2</sub>. However, current research on RMC remains fragmented, lacking a systematic overview of its complete processing route. This review summarizes the carbonation mechanism of RMC and provides a comprehensive discussion of evaluation methods for its carbonation degree. In addition, the review provides an in-depth analysis of factors influencing carbonation and strategies to enhance it. Specifically, we categorize the mechanisms and evaluate the effectiveness of various methods, with an emphasis on environmentally friendly production processes to identify the most optimal approaches. Finally, the study highlights the carbon footprint of RMC and discusses the challenges associated with achieving low-carbon RMC production.</div></div>","PeriodicalId":100597,"journal":{"name":"Green Energy and Resources","volume":"3 4","pages":"Article 100154"},"PeriodicalIF":0.0,"publicationDate":"2025-12-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145684552","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Experimental verification of electrode activation for improved performance in vanadium redox flow batteries 电极活化提高钒氧化还原液流电池性能的实验验证
Pub Date : 2025-12-01 DOI: 10.1016/j.gerr.2025.100155
Zhi Zhuge , Zebo Huang , Osamah Ibrahim Khalaf , Longxing Wu
Vanadium redox flow batteries (VRFBs) have held significant promise in large-scale energy storage applications due to their advantages, including long cycle life, high safety, and the ability to independently design power and capacity. However, the relatively low power density has remained a critical bottleneck for further development. As a key material in VRFB power units, enhancing the performance of graphite felt electrodes has represented an effective strategy for achieving high-power battery technology. To improve the activity of graphite felt electrodes, this study has employed an experimental verification approach to investigate battery performance parameters under various activation temperatures and durations, thereby identifying the optimal activation conditions. In contrast to prior studies that exclusively targeted 400°C without systematically optimizing activation duration, this study has systematically evaluated five activation temperatures and four activation durations to clarify the synergistic influence of these parameters on VRFB performance. Specifically, experiments have been conducted at room temperature using activation temperatures of 300, 350, 400, 450, and 500°C, as well as activation durations of 24, 11, 7, and 3 ​h. The results have indicated that an activation temperature of 400°C yielded notable improvements in charge/discharge performance, internal resistance, efficiency, and capacity retention. Notably, energy efficiency has increased by 5.06%, 5.94%, 3.67%, and 4.72% under these conditions. This study has identified the optimal activation conditions of “400°C for 7 ​h” and has provided the corresponding performance data, which can help reduce research costs associated with electrode activation in future investigations. This study has provided valuable insights into electrode activation and has offered guidance for enhancing VRFB performance.
钒氧化还原液流电池(vrfb)由于其循环寿命长、安全性高、能够独立设计功率和容量等优点,在大规模储能应用中具有重要的前景。然而,相对较低的功率密度仍然是进一步发展的关键瓶颈。石墨毡电极作为VRFB动力装置的关键材料,提高其性能是实现大功率电池技术的有效策略。为了提高石墨毡电极的活性,本研究采用实验验证的方法研究了不同活化温度和持续时间下的电池性能参数,从而确定了最佳的活化条件。与以往的研究只针对400°C而没有系统优化激活时间不同,本研究系统地评估了5种激活温度和4种激活时间,以阐明这些参数对VRFB性能的协同影响。具体来说,实验在室温下进行,激活温度分别为300、350、400、450和500℃,激活时间分别为24、11、7和3小时。结果表明,激活温度为400°C时,电池的充放电性能、内阻、效率和容量保持率均有显著提高。能效分别提高了5.06%、5.94%、3.67%和4.72%。本研究确定了“400°C 7 h”的最佳活化条件,并提供了相应的性能数据,有助于在未来的研究中降低与电极活化相关的研究成本。该研究为电极活化提供了有价值的见解,并为提高VRFB性能提供了指导。
{"title":"Experimental verification of electrode activation for improved performance in vanadium redox flow batteries","authors":"Zhi Zhuge ,&nbsp;Zebo Huang ,&nbsp;Osamah Ibrahim Khalaf ,&nbsp;Longxing Wu","doi":"10.1016/j.gerr.2025.100155","DOIUrl":"10.1016/j.gerr.2025.100155","url":null,"abstract":"<div><div>Vanadium redox flow batteries (VRFBs) have held significant promise in large-scale energy storage applications due to their advantages, including long cycle life, high safety, and the ability to independently design power and capacity. However, the relatively low power density has remained a critical bottleneck for further development. As a key material in VRFB power units, enhancing the performance of graphite felt electrodes has represented an effective strategy for achieving high-power battery technology. To improve the activity of graphite felt electrodes, this study has employed an experimental verification approach to investigate battery performance parameters under various activation temperatures and durations, thereby identifying the optimal activation conditions. In contrast to prior studies that exclusively targeted 400°C without systematically optimizing activation duration, this study has systematically evaluated five activation temperatures and four activation durations to clarify the synergistic influence of these parameters on VRFB performance. Specifically, experiments have been conducted at room temperature using activation temperatures of 300, 350, 400, 450, and 500°C, as well as activation durations of 24, 11, 7, and 3 ​h. The results have indicated that an activation temperature of 400°C yielded notable improvements in charge/discharge performance, internal resistance, efficiency, and capacity retention. Notably, energy efficiency has increased by 5.06%, 5.94%, 3.67%, and 4.72% under these conditions. This study has identified the optimal activation conditions of “400°C for 7 ​h” and has provided the corresponding performance data, which can help reduce research costs associated with electrode activation in future investigations. This study has provided valuable insights into electrode activation and has offered guidance for enhancing VRFB performance.</div></div>","PeriodicalId":100597,"journal":{"name":"Green Energy and Resources","volume":"3 4","pages":"Article 100155"},"PeriodicalIF":0.0,"publicationDate":"2025-12-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145684515","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
A review on comprehensive strategies for decarbonizing bioethanol production process 生物乙醇生产过程脱碳综合策略综述
Pub Date : 2025-10-06 DOI: 10.1016/j.gerr.2025.100153
Treerat Vacharanukrauh , Apinan Soottitantawat , Nuttha Thongchul , Worapon Kiatkittipong , Nopphon Weeranoppanant , Suttichai Assabumrungrat
Bioethanol plays a crucial role in the global transition to sustainability, serving as a renewable fuel especially in the transportation sector, and a versatile renewable chemical precursor in industries, mitigating greenhouse gas (GHG) emissions. Although bioethanol is renewable, its production is still carbon-intensive, with most emissions arising from fermentation and cogeneration. Despite significant advancements, existing works on bioethanol have largely focused on individual decarbonization elements (e.g., CCU, CCS in bioenergy, and process intensification in ethanol production). Few studies link these strategies together to show how they could collectively move bioethanol toward carbon-negative production. This review aims to fill that gap by systematically analyzing the evolution of bioethanol production processes, identifying key sources of CO2 emissions, and critically evaluating state-of-the-art strategies—including process optimization, CCU, and CCS—within a unified framework. Overall, this review underscores that integrating process optimization, CCU, and CCS can transform bioethanol production from a low-carbon fuel into a negative-emission technology, reinforcing its pivotal role in global decarbonization efforts.
生物乙醇在全球向可持续发展的过渡中发挥着至关重要的作用,它是一种可再生燃料,特别是在交通运输部门,也是一种多用途的可再生化学前体,可以减少温室气体(GHG)的排放。虽然生物乙醇是可再生的,但其生产仍然是碳密集型的,大部分排放来自发酵和热电联产。尽管取得了重大进展,但现有的生物乙醇工作主要集中在个别脱碳元素上(例如,生物能源中的CCU, CCS和乙醇生产中的过程强化)。很少有研究将这些策略联系在一起,以显示它们如何共同将生物乙醇推向负碳生产。本综述旨在通过系统地分析生物乙醇生产过程的演变,确定二氧化碳排放的主要来源,并在统一的框架内批判性地评估最先进的策略,包括过程优化,CCU和ccs,来填补这一空白。总之,这篇综述强调,整合工艺优化、CCU和CCS可以将生物乙醇生产从低碳燃料转变为负排放技术,加强其在全球脱碳努力中的关键作用。
{"title":"A review on comprehensive strategies for decarbonizing bioethanol production process","authors":"Treerat Vacharanukrauh ,&nbsp;Apinan Soottitantawat ,&nbsp;Nuttha Thongchul ,&nbsp;Worapon Kiatkittipong ,&nbsp;Nopphon Weeranoppanant ,&nbsp;Suttichai Assabumrungrat","doi":"10.1016/j.gerr.2025.100153","DOIUrl":"10.1016/j.gerr.2025.100153","url":null,"abstract":"<div><div>Bioethanol plays a crucial role in the global transition to sustainability, serving as a renewable fuel especially in the transportation sector, and a versatile renewable chemical precursor in industries, mitigating greenhouse gas (GHG) emissions. Although bioethanol is renewable, its production is still carbon-intensive, with most emissions arising from fermentation and cogeneration. Despite significant advancements, existing works on bioethanol have largely focused on individual decarbonization elements (e.g., CCU, CCS in bioenergy, and process intensification in ethanol production). Few studies link these strategies together to show how they could collectively move bioethanol toward carbon-negative production. This review aims to fill that gap by systematically analyzing the evolution of bioethanol production processes, identifying key sources of CO<sub>2</sub> emissions, and critically evaluating state-of-the-art strategies—including process optimization, CCU, and CCS—within a unified framework. Overall, this review underscores that integrating process optimization, CCU, and CCS can transform bioethanol production from a low-carbon fuel into a negative-emission technology, reinforcing its pivotal role in global decarbonization efforts.</div></div>","PeriodicalId":100597,"journal":{"name":"Green Energy and Resources","volume":"3 4","pages":"Article 100153"},"PeriodicalIF":0.0,"publicationDate":"2025-10-06","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145467489","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Methane hydrate formation using high gravity equipment: A new method for recovery of associated gas in offshore oilfields 利用高重力设备形成甲烷水合物:海上油田开采伴生气的新方法
Pub Date : 2025-10-04 DOI: 10.1016/j.gerr.2025.100151
Qi Nie , Jianlu Zhu , Liang Hao , Yuxing Li
For deep-sea oil exploitation far away from land, there is inevitably the generation of oilfield-associated gas. It is a new method for recover oilfield associated gas by using a high-gravity device to generate hydrate. In this paper, the methane hydrate formation process of different packings in the high-gravity machine was studied. By comparing the structural morphology of varying packings and the characteristics of the hydrate in the high-gravity machine, a new type of layered packing is designed and manufactured. The volumetric storage capacity, normalized gas consumption rates and methane absorption time of foam metal packing, metal mesh packing, 3D printing spiral packing, and new layered packing were investigated experimentally. The results show that the new layered packing has significant advantages. The maximum volumetric storage capacity, normalized gas consumption rate, and the shortest methane absorption time are 239265 mol/(m3·min), and 74 min, respectively. It exhibits an excellent methane hydrate formation effect and the advantage of small equipment size. It is very suitable for the recovery of oilfield-associated gas produced in the process of offshore oil exploitation.
对于远离陆地的深海石油开采,不可避免地会产生油田伴生气。利用高重力装置生成水合物是开采油田伴生气的一种新方法。本文研究了不同填料在高重力机器中的甲烷水合物形成过程。通过比较不同填料的结构形态和高重力机器中水合物的特性,设计并制造了一种新型分层填料。实验研究了泡沫金属填料、金属网状填料、3D打印螺旋填料和新型分层填料的储气量、标准化气体消耗率和甲烷吸收时间。结果表明,新型分层填料具有明显的优越性。最大储气量为239265 mol/(m3·min),标准化气体消耗率为74 min,甲烷吸收时间最短。它具有良好的甲烷水合物生成效果和设备体积小的优点。它非常适合于海上石油开采过程中产生的油田伴生气的开采。
{"title":"Methane hydrate formation using high gravity equipment: A new method for recovery of associated gas in offshore oilfields","authors":"Qi Nie ,&nbsp;Jianlu Zhu ,&nbsp;Liang Hao ,&nbsp;Yuxing Li","doi":"10.1016/j.gerr.2025.100151","DOIUrl":"10.1016/j.gerr.2025.100151","url":null,"abstract":"<div><div>For deep-sea oil exploitation far away from land, there is inevitably the generation of oilfield-associated gas. It is a new method for recover oilfield associated gas by using a high-gravity device to generate hydrate. In this paper, the methane hydrate formation process of different packings in the high-gravity machine was studied. By comparing the structural morphology of varying packings and the characteristics of the hydrate in the high-gravity machine, a new type of layered packing is designed and manufactured. The volumetric storage capacity, normalized gas consumption rates and methane absorption time of foam metal packing, metal mesh packing, 3D printing spiral packing, and new layered packing were investigated experimentally. The results show that the new layered packing has significant advantages. The maximum volumetric storage capacity, normalized gas consumption rate, and the shortest methane absorption time are 239265 mol/(m<sup>3</sup>·min), and 74 min, respectively. It exhibits an excellent methane hydrate formation effect and the advantage of small equipment size. It is very suitable for the recovery of oilfield-associated gas produced in the process of offshore oil exploitation.</div></div>","PeriodicalId":100597,"journal":{"name":"Green Energy and Resources","volume":"3 4","pages":"Article 100151"},"PeriodicalIF":0.0,"publicationDate":"2025-10-04","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145323997","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Accounting the life cycle carbon footprint for TOD project: An example from the China SH TOD project TOD项目生命周期碳足迹核算:以中国上海TOD项目为例
Pub Date : 2025-10-02 DOI: 10.1016/j.gerr.2025.100152
Jingxiao Zhang , Lei Gao , Xin Liu , Martin Skitmore
Transit-Oriented Development (TOD) has emerged as a critical strategy for advancing the green transformation of China's low-carbon cities. Conducting carbon footprint research on TOD from a whole life cycle perspective holds profound significance for achieving the Dual Carbon Goals. This study constructs five carbon footprint calculation models based on life cycle assessment theory. Setting four residential travel scenario assumptions thoroughly examines the whole life cycle carbon emissions of China SH TOD project and the carbon reduction achieved through transportation during the operation phase. Results indicate that total carbon emissions in the study area amount to 2.9902 million tons. Considering solely the carbon reduction effect from shifts in resident travel modes under the TOD model, the total carbon reduction reaches 203600 tons, with a carbon reduction effectiveness evaluation index of 6.81%. Compared to the continuous increase in carbon footprint observed after the operation of traditional residential and commercial projects, the carbon reduction effect is notably significant. Furthermore, the study identified key high-emission stages within the lifecycle through model-based calculations and proposed targeted mitigation strategies. These findings provide recommendations for energy conservation, carbon reduction, and sustainable development in TOD projects.
交通导向发展(TOD)已成为推动中国低碳城市绿色转型的关键战略。从全生命周期角度对TOD进行碳足迹研究,对于实现双碳目标具有重要意义。本研究基于生命周期评价理论构建了5个碳足迹计算模型。通过设定四种住宅出行情景假设,深入考察了中国SH TOD项目全生命周期的碳排放,以及运行阶段通过运输实现的碳减排。结果表明,研究区碳排放总量为299.02万吨。仅考虑TOD模型下居民出行方式转换的减碳效果,总减碳量达到203600吨,减碳效果评价指标为6.81%。与传统住宅和商业项目运行后碳足迹的持续增加相比,减碳效果显著。此外,该研究通过基于模型的计算确定了生命周期内的关键高排放阶段,并提出了有针对性的缓解战略。研究结果为TOD项目的节能减排和可持续发展提供了建议。
{"title":"Accounting the life cycle carbon footprint for TOD project: An example from the China SH TOD project","authors":"Jingxiao Zhang ,&nbsp;Lei Gao ,&nbsp;Xin Liu ,&nbsp;Martin Skitmore","doi":"10.1016/j.gerr.2025.100152","DOIUrl":"10.1016/j.gerr.2025.100152","url":null,"abstract":"<div><div>Transit-Oriented Development (TOD) has emerged as a critical strategy for advancing the green transformation of China's low-carbon cities. Conducting carbon footprint research on TOD from a whole life cycle perspective holds profound significance for achieving the Dual Carbon Goals. This study constructs five carbon footprint calculation models based on life cycle assessment theory. Setting four residential travel scenario assumptions thoroughly examines the whole life cycle carbon emissions of China SH TOD project and the carbon reduction achieved through transportation during the operation phase. Results indicate that total carbon emissions in the study area amount to 2.9902 million tons. Considering solely the carbon reduction effect from shifts in resident travel modes under the TOD model, the total carbon reduction reaches 203600 tons, with a carbon reduction effectiveness evaluation index of 6.81%. Compared to the continuous increase in carbon footprint observed after the operation of traditional residential and commercial projects, the carbon reduction effect is notably significant. Furthermore, the study identified key high-emission stages within the lifecycle through model-based calculations and proposed targeted mitigation strategies. These findings provide recommendations for energy conservation, carbon reduction, and sustainable development in TOD projects.</div></div>","PeriodicalId":100597,"journal":{"name":"Green Energy and Resources","volume":"3 4","pages":"Article 100152"},"PeriodicalIF":0.0,"publicationDate":"2025-10-02","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145467490","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Insight into the occurrence relationships between Pb, As, Zn and Cr with minerals phases in the coal gangue: A novel quantitative dissociation method 煤矸石中Pb、As、Zn、Cr与矿物相赋存关系的研究:一种新的定量解离方法
Pub Date : 2025-09-01 DOI: 10.1016/j.gerr.2025.100143
Yichao Chen , Wanyao Li , Haofei Li , Yuhong Qin , Shugang Guo , Bin Fang , Yujia Du , Jin Yuan , Leteng Lin
Establishing the quantitative relationships between heavy metals and mineral phases in coal gangue is essential for its comprehensive landfill and refined utilization. In this study, the Guandi coal gangue was subjected to a stepwise dissociation method using seven concentration gradients (0.1, 1.0, 4.0, 6.0, 8.0, 10.0, 12.0 ​mol/L) of aqua regia and hydrofluoric acid. Combined with the Rietveld refinement method, inverse matrix calculations of residual fractions of mineral phases and dissociation degrees of heavy metals after dissociation, the quantitative relationships between Pb, As, Zn, Cr and the mineral phases were determined. The results show that kaolinite, quartz, pyrite, and the amorphous phase are the primary host phases for Pb, As, Zn, and Cr, with their contents in crystalline phases ranging from 71.36% to 87.68%. Validation via the standard addition method demonstrates that the relative standard deviation of the stepwise dissociation for Pb, As, Zn, and Cr is ​≤7.23%, with spike recovery rates ranging from 85.43% to 112.85%, indicating favorable test results. Sequential chemical leaching demonstrates that heavy metals are mainly distributed in stable aluminosilicate-bound state and carbonate or oxide-bound state. The toxicity characteristic leaching procedure test indicated that Cr exhibited high toxicity and thus required long-term monitoring. The results of this study provide important theoretical guidance for the comprehensive landfilling and resource utilization of Guandi coal gangue, and the established analytical method can be extended to studies on quantitative relationships between heavy metals and mineral phases in other tailings.
建立煤矸石中重金属与矿物相的定量关系,对煤矸石的综合填埋和精细化利用具有重要意义。采用王水和氢氟酸7个浓度梯度(0.1、1.0、4.0、6.0、8.0、10.0、12.0 mol/L)对官地煤矸石进行了分步解离实验。结合Rietveld精细化法、矿相残留分数逆矩阵计算和重金属解离度计算,确定了Pb、As、Zn、Cr与矿相的定量关系。结果表明:Pb、As、Zn、Cr的主要寄主相为高岭石、石英、黄铁矿和非晶相,其晶相含量在71.36% ~ 87.68%之间;标准加入法验证Pb、As、Zn、Cr逐步解离的相对标准偏差≤7.23%,峰回收率为85.43% ~ 112.85%,试验结果良好。序贯化学浸出表明,重金属主要以稳定的铝硅酸盐结合态和碳酸盐或氧化物结合态分布。毒性特征浸出过程试验表明,铬具有高毒性,需要长期监测。研究结果为官地煤矸石的综合填埋和资源化利用提供了重要的理论指导,所建立的分析方法也可推广到其他尾矿中重金属与矿相定量关系的研究中。
{"title":"Insight into the occurrence relationships between Pb, As, Zn and Cr with minerals phases in the coal gangue: A novel quantitative dissociation method","authors":"Yichao Chen ,&nbsp;Wanyao Li ,&nbsp;Haofei Li ,&nbsp;Yuhong Qin ,&nbsp;Shugang Guo ,&nbsp;Bin Fang ,&nbsp;Yujia Du ,&nbsp;Jin Yuan ,&nbsp;Leteng Lin","doi":"10.1016/j.gerr.2025.100143","DOIUrl":"10.1016/j.gerr.2025.100143","url":null,"abstract":"<div><div>Establishing the quantitative relationships between heavy metals and mineral phases in coal gangue is essential for its comprehensive landfill and refined utilization. In this study, the Guandi coal gangue was subjected to a stepwise dissociation method using seven concentration gradients (0.1, 1.0, 4.0, 6.0, 8.0, 10.0, 12.0 ​mol/L) of aqua regia and hydrofluoric acid. Combined with the Rietveld refinement method, inverse matrix calculations of residual fractions of mineral phases and dissociation degrees of heavy metals after dissociation, the quantitative relationships between Pb, As, Zn, Cr and the mineral phases were determined. The results show that kaolinite, quartz, pyrite, and the amorphous phase are the primary host phases for Pb, As, Zn, and Cr, with their contents in crystalline phases ranging from 71.36% to 87.68%. Validation via the standard addition method demonstrates that the relative standard deviation of the stepwise dissociation for Pb, As, Zn, and Cr is ​≤7.23%, with spike recovery rates ranging from 85.43% to 112.85%, indicating favorable test results. Sequential chemical leaching demonstrates that heavy metals are mainly distributed in stable aluminosilicate-bound state and carbonate or oxide-bound state. The toxicity characteristic leaching procedure test indicated that Cr exhibited high toxicity and thus required long-term monitoring. The results of this study provide important theoretical guidance for the comprehensive landfilling and resource utilization of Guandi coal gangue, and the established analytical method can be extended to studies on quantitative relationships between heavy metals and mineral phases in other tailings.</div></div>","PeriodicalId":100597,"journal":{"name":"Green Energy and Resources","volume":"3 3","pages":"Article 100143"},"PeriodicalIF":0.0,"publicationDate":"2025-09-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145120980","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
期刊
Green Energy and Resources
全部 Acc. Chem. Res. ACS Applied Bio Materials ACS Appl. Electron. Mater. ACS Appl. Energy Mater. ACS Appl. Mater. Interfaces ACS Appl. Nano Mater. ACS Appl. Polym. Mater. ACS BIOMATER-SCI ENG ACS Catal. ACS Cent. Sci. ACS Chem. Biol. ACS Chemical Health & Safety ACS Chem. Neurosci. ACS Comb. Sci. ACS Earth Space Chem. ACS Energy Lett. ACS Infect. Dis. ACS Macro Lett. ACS Mater. Lett. ACS Med. Chem. Lett. ACS Nano ACS Omega ACS Photonics ACS Sens. ACS Sustainable Chem. Eng. ACS Synth. Biol. Anal. Chem. BIOCHEMISTRY-US Bioconjugate Chem. BIOMACROMOLECULES Chem. Res. Toxicol. Chem. Rev. Chem. Mater. CRYST GROWTH DES ENERG FUEL Environ. Sci. Technol. Environ. Sci. Technol. Lett. Eur. J. Inorg. Chem. IND ENG CHEM RES Inorg. Chem. J. Agric. Food. Chem. J. Chem. Eng. Data J. Chem. Educ. J. Chem. Inf. Model. J. Chem. Theory Comput. J. Med. Chem. J. Nat. Prod. J PROTEOME RES J. Am. Chem. Soc. LANGMUIR MACROMOLECULES Mol. Pharmaceutics Nano Lett. Org. Lett. ORG PROCESS RES DEV ORGANOMETALLICS J. Org. Chem. J. Phys. Chem. J. Phys. Chem. A J. Phys. Chem. B J. Phys. Chem. C J. Phys. Chem. Lett. Analyst Anal. Methods Biomater. Sci. Catal. Sci. Technol. Chem. Commun. Chem. Soc. Rev. CHEM EDUC RES PRACT CRYSTENGCOMM Dalton Trans. Energy Environ. Sci. ENVIRON SCI-NANO ENVIRON SCI-PROC IMP ENVIRON SCI-WAT RES Faraday Discuss. Food Funct. Green Chem. Inorg. Chem. Front. Integr. Biol. J. Anal. At. Spectrom. J. Mater. Chem. A J. Mater. Chem. B J. Mater. Chem. C Lab Chip Mater. Chem. Front. Mater. Horiz. MEDCHEMCOMM Metallomics Mol. Biosyst. Mol. Syst. Des. Eng. Nanoscale Nanoscale Horiz. Nat. Prod. Rep. New J. Chem. Org. Biomol. Chem. Org. Chem. Front. PHOTOCH PHOTOBIO SCI PCCP Polym. Chem.
×
引用
GB/T 7714-2015
复制
MLA
复制
APA
复制
导出至
BibTeX EndNote RefMan NoteFirst NoteExpress
×
0
微信
客服QQ
Book学术公众号 扫码关注我们
反馈
×
意见反馈
请填写您的意见或建议
请填写您的手机或邮箱
×
提示
您的信息不完整,为了账户安全,请先补充。
现在去补充
×
提示
您因"违规操作"
具体请查看互助需知
我知道了
×
提示
现在去查看 取消
×
提示
确定
Book学术官方微信
Book学术文献互助
Book学术文献互助群
群 号:604180095
Book学术
文献互助 智能选刊 最新文献 互助须知 联系我们:info@booksci.cn
Book学术提供免费学术资源搜索服务,方便国内外学者检索中英文文献。致力于提供最便捷和优质的服务体验。
Copyright © 2023 Book学术 All rights reserved.
ghs 京公网安备 11010802042870号 京ICP备2023020795号-1