Pub Date : 2024-09-21DOI: 10.1080/09593330.2024.2405662
Yue Yang, Xiaoli Zhou, Zixun Zhou, Xiujuan Qian, Jie Zhou, Minjiao Chen, Weiliang Dong, Min Jiang
With the increasing focus on environmental friendliness and sustainable development, extensive research has been conducted on the biodegradation of plastics. The non-hydrolyzable, highly hydrophobic, and high-molecular-weight properties of polyethylene (PE) pose challenges for cell interaction and biodegradation of PE substrates. To overcome these obstacles, PE films were treated with low-temperature plasma before biodegradation. The morphology, surface chemistry, molecular weight, and weight loss of PE films after plasma treatment and biodegradation were studied. The plasma treatment decreased the surface water contact angle, formed C-O and C = O groups, and decreased the molecular weight of PE films. With the increased pretreatment time, the biodegradation efficiency rose to 2.6% from 0.63% after 20 days of incubation. The mechanism was proposed that the surface oxygen-containing groups formed by plasma treatment can facilitate the bio-accessibility and be further decomposed and utilised by the microbes. This study provided an effective and rapid pretreatment strategy for improving biodegradation of PE.
随着对环境友好和可持续发展的日益关注，人们对塑料的生物降解进行了广泛的研究。聚乙烯（PE）具有不可水解、高度疏水和高分子量的特性，这给聚乙烯基底的细胞相互作用和生物降解带来了挑战。为了克服这些障碍，在生物降解前用低温等离子体处理聚乙烯薄膜。研究了等离子处理和生物降解后聚乙烯薄膜的形态、表面化学、分子量和重量损失。等离子体处理降低了聚乙烯薄膜的表面水接触角，形成了 C-O 和 C = O 基团，并降低了聚乙烯薄膜的分子量。随着预处理时间的延长，培养 20 天后的生物降解效率从 0.63% 上升到 2.6%。其机理是等离子体处理形成的表面含氧基团可促进生物进入，并被微生物进一步分解和利用。这项研究为改善聚乙烯的生物降解提供了一种有效而快速的预处理策略。
{"title":"The effect of low-temperature plasma pretreatment on the biodegradability of polyethylene films.","authors":"Yue Yang, Xiaoli Zhou, Zixun Zhou, Xiujuan Qian, Jie Zhou, Minjiao Chen, Weiliang Dong, Min Jiang","doi":"10.1080/09593330.2024.2405662","DOIUrl":"https://doi.org/10.1080/09593330.2024.2405662","url":null,"abstract":"<p><p>With the increasing focus on environmental friendliness and sustainable development, extensive research has been conducted on the biodegradation of plastics. The non-hydrolyzable, highly hydrophobic, and high-molecular-weight properties of polyethylene (PE) pose challenges for cell interaction and biodegradation of PE substrates. To overcome these obstacles, PE films were treated with low-temperature plasma before biodegradation. The morphology, surface chemistry, molecular weight, and weight loss of PE films after plasma treatment and biodegradation were studied. The plasma treatment decreased the surface water contact angle, formed C-O and C = O groups, and decreased the molecular weight of PE films. With the increased pretreatment time, the biodegradation efficiency rose to 2.6% from 0.63% after 20 days of incubation. The mechanism was proposed that the surface oxygen-containing groups formed by plasma treatment can facilitate the bio-accessibility and be further decomposed and utilised by the microbes. This study provided an effective and rapid pretreatment strategy for improving biodegradation of PE.</p>","PeriodicalId":12009,"journal":{"name":"Environmental Technology","volume":null,"pages":null},"PeriodicalIF":2.2,"publicationDate":"2024-09-21","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142282403","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2024-09-19DOI: 10.1080/09593330.2024.2404646
Oshrat Levy-Ontman, Shir Nagar, Ofra Paz-Tal, Adi Wolfson
Renewable and biodegradable polysaccharides attract attention as environmentally friendly adsorbents for the removal of heavy metals from wastewater. One such group, is carrageenan, of which were recently successfully employed to adsorb representative lanthanide and actinide ions. Herein, iota-carrageenan-based hydrogels were used to adsorb europium ions (Eu3+) from water solutions, followed by desorption of the ions from the hydrogel beads and recycling of the beads three times. It was found that sorption yields from a 500 mg/L Eu3+ ion solution with beads that were prepared with 1 or 2 wt/v% aqueous solution of iota-carrageenan with CaCl2 (0.5 M) reached maximum sorption yield of 50% and 65%, correspondingly, after 1 h. In addition, the sorption kinetics followed the pseudo second-order model controlled by chemisorption. Desorption yields in the first cycle using NaNO3 (1 M) with both preparations were 57% and 74%, respectively. The sorption yields increased during the second and third cycles and were efficient in the overall pH range. Cryo-SEM, SEM, SEM-EDS and TGA analyses verified the adsorption and desorption of Eu3+ ions to and from the iota beads and that the Ca2+ ions that initially crosslinked the hydrogel were replaced during the cycles by Eu3+ or Na+ ions. In addition, the beads were stable and easily reusable for several sorption/desorption cycles. Furthermore, after sorption, the beads were characterised by a porous structure, such that beads prepared with a 2 wt/v% aqueous solution of iota-carrageenan yielded a more porous, ordered structure, and after desorption, the bead textures became even more porous.
{"title":"Iota-carrageenan as a regenerating system for Eu<sup>3+</sup> recovery: adsorption/desorption cycles.","authors":"Oshrat Levy-Ontman, Shir Nagar, Ofra Paz-Tal, Adi Wolfson","doi":"10.1080/09593330.2024.2404646","DOIUrl":"https://doi.org/10.1080/09593330.2024.2404646","url":null,"abstract":"<p><p>Renewable and biodegradable polysaccharides attract attention as environmentally friendly adsorbents for the removal of heavy metals from wastewater. One such group, is carrageenan, of which were recently successfully employed to adsorb representative lanthanide and actinide ions. Herein, iota-carrageenan-based hydrogels were used to adsorb europium ions (Eu<sup>3+</sup>) from water solutions, followed by desorption of the ions from the hydrogel beads and recycling of the beads three times. It was found that sorption yields from a 500 mg/L Eu<sup>3+</sup> ion solution with beads that were prepared with 1 or 2 wt/v% aqueous solution of iota-carrageenan with CaCl<sub>2</sub> (0.5 M) reached maximum sorption yield of 50% and 65%, correspondingly, after 1 h. In addition, the sorption kinetics followed the pseudo second-order model controlled by chemisorption. Desorption yields in the first cycle using NaNO<sub>3</sub> (1 M) with both preparations were 57% and 74%, respectively. The sorption yields increased during the second and third cycles and were efficient in the overall pH range. Cryo-SEM, SEM, SEM-EDS and TGA analyses verified the adsorption and desorption of Eu<sup>3+</sup> ions to and from the iota beads and that the Ca<sup>2+</sup> ions that initially crosslinked the hydrogel were replaced during the cycles by Eu<sup>3+</sup> or Na<sup>+</sup> ions. In addition, the beads were stable and easily reusable for several sorption/desorption cycles. Furthermore, after sorption, the beads were characterised by a porous structure, such that beads prepared with a 2 wt/v% aqueous solution of iota-carrageenan yielded a more porous, ordered structure, and after desorption, the bead textures became even more porous.</p>","PeriodicalId":12009,"journal":{"name":"Environmental Technology","volume":null,"pages":null},"PeriodicalIF":2.2,"publicationDate":"2024-09-19","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142282401","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2024-09-18DOI: 10.1080/09593330.2024.2405033
Youfei Zhou, Peilin Guo, Yi Liu, Weijie Hu, Tianfeng Wang
The impact of four nano-bubble water (NBW) additions on the hydrolysis rate, methane yield, and microbial community of co-digestion of cabbage waste (CW) and cow manure (CM) under mesophilic and th...
{"title":"Effects of nano-bubble water on anaerobic co-digestion of cabbage waste and cow manure under mesophilic and thermophilic conditions","authors":"Youfei Zhou, Peilin Guo, Yi Liu, Weijie Hu, Tianfeng Wang","doi":"10.1080/09593330.2024.2405033","DOIUrl":"https://doi.org/10.1080/09593330.2024.2405033","url":null,"abstract":"The impact of four nano-bubble water (NBW) additions on the hydrolysis rate, methane yield, and microbial community of co-digestion of cabbage waste (CW) and cow manure (CM) under mesophilic and th...","PeriodicalId":12009,"journal":{"name":"Environmental Technology","volume":null,"pages":null},"PeriodicalIF":2.8,"publicationDate":"2024-09-18","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142264479","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2024-09-18DOI: 10.1080/09593330.2024.2404648
Alfredo Córdova Lizama, Cristian Carrera Figueiras, Alejandro Zepeda Pedreguera, Noori M. Cata Saady, Juan Enrique Ruiz Espinoza
This work evaluated the effects of cobalt nanoparticles (CoNPs) (0.025–7 mg/gVS) on the intensification of sewage sludge anaerobic digestion (AD) using biochemical methane potential (BMP) tests. Th...
{"title":"Improving the anaerobic digestion of sewage sludge by adding cobalt nanoparticles","authors":"Alfredo Córdova Lizama, Cristian Carrera Figueiras, Alejandro Zepeda Pedreguera, Noori M. Cata Saady, Juan Enrique Ruiz Espinoza","doi":"10.1080/09593330.2024.2404648","DOIUrl":"https://doi.org/10.1080/09593330.2024.2404648","url":null,"abstract":"This work evaluated the effects of cobalt nanoparticles (CoNPs) (0.025–7 mg/gVS) on the intensification of sewage sludge anaerobic digestion (AD) using biochemical methane potential (BMP) tests. Th...","PeriodicalId":12009,"journal":{"name":"Environmental Technology","volume":null,"pages":null},"PeriodicalIF":2.8,"publicationDate":"2024-09-18","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142264689","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2024-09-18DOI: 10.1080/09593330.2024.2402097
Burçin Yıldız Sevgili
To degrade phenol with the heterogeneous Fenton-like process and to compare the results, micro-scale zero-valent iron particles (mZVI) and nickel-coated iron bimetallic particles (Ni/Fe) were used....
{"title":"The effect of use of Ni/Fe and mZVI on phenol removal with the heterogenous fenton process and in-situ generation of H2O2","authors":"Burçin Yıldız Sevgili","doi":"10.1080/09593330.2024.2402097","DOIUrl":"https://doi.org/10.1080/09593330.2024.2402097","url":null,"abstract":"To degrade phenol with the heterogeneous Fenton-like process and to compare the results, micro-scale zero-valent iron particles (mZVI) and nickel-coated iron bimetallic particles (Ni/Fe) were used....","PeriodicalId":12009,"journal":{"name":"Environmental Technology","volume":null,"pages":null},"PeriodicalIF":2.8,"publicationDate":"2024-09-18","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142264688","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2024-09-16DOI: 10.1080/09593330.2024.2401644
Z. Wu, B.V.N. Sewwandi, Xing Chen, G. Perera, L. Jayarathna, A.C.A. Jayasundara, Rohan Weerasooriya
Thin-film nanocomposite (TFN) membranes with a polyamide (PA) active layer modified with carbon nanotubes (CNTs) hold promise for water desalination and wastewater reuse via forward osmosis (FO). W...
{"title":"Forward osmosis membrane with lightweight functionalised multiwall carbon nanotube nanofillers","authors":"Z. Wu, B.V.N. Sewwandi, Xing Chen, G. Perera, L. Jayarathna, A.C.A. Jayasundara, Rohan Weerasooriya","doi":"10.1080/09593330.2024.2401644","DOIUrl":"https://doi.org/10.1080/09593330.2024.2401644","url":null,"abstract":"Thin-film nanocomposite (TFN) membranes with a polyamide (PA) active layer modified with carbon nanotubes (CNTs) hold promise for water desalination and wastewater reuse via forward osmosis (FO). W...","PeriodicalId":12009,"journal":{"name":"Environmental Technology","volume":null,"pages":null},"PeriodicalIF":2.8,"publicationDate":"2024-09-16","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142264691","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2024-09-12DOI: 10.1080/09593330.2024.2381644
Litao Wang, Hong Liang, Xuran Du, Guanyu Chen, Weijian Lai, Ye Liu, Ming Li, Dawen Gao
Polycyclic aromatic hydrocarbons (PAHs) are pervasive and persistent pollutants in contaminated soil, posing a severe health and environmental threat. Enzymatic bioremediation presents a viable sol...
{"title":"Enzymatic bioremediation of polycyclic aromatic hydrocarbons (PAHs) in contaminated soil: a study on the recombinant laccase TVL","authors":"Litao Wang, Hong Liang, Xuran Du, Guanyu Chen, Weijian Lai, Ye Liu, Ming Li, Dawen Gao","doi":"10.1080/09593330.2024.2381644","DOIUrl":"https://doi.org/10.1080/09593330.2024.2381644","url":null,"abstract":"Polycyclic aromatic hydrocarbons (PAHs) are pervasive and persistent pollutants in contaminated soil, posing a severe health and environmental threat. Enzymatic bioremediation presents a viable sol...","PeriodicalId":12009,"journal":{"name":"Environmental Technology","volume":null,"pages":null},"PeriodicalIF":2.8,"publicationDate":"2024-09-12","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142264476","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2024-09-11DOI: 10.1080/09593330.2024.2401158
Ni Liao,Furong Li,Xiuli Huang,Yi Zhang
In this work, a kind of novel Chitosan (Cs)-doped zeolite imidazole framework (ZIF-8@Cs) with a larger surface area and a smaller pore size was synthesised via a facial solvothermal approach and applied to remove Cu2+ from mine wastewater. Compared to nondoped ZIF-8, ZIF-8@Cs exhibited a stronger adsorption performance and removal efficiency. The reason was that ZIF-8@Cs doped by the Cs could suppress the aggregation and increase the monodispersity of ZIF-8. Using the high-performance ZIF-8@Cs, as a novel adsorbent, was successfully developed for the efficient removal of Cu2+ from mine wastewater. Various parameters, such as contact time, initial Cu2+ concentration, adsorbent dosage, and pH, were investigated. The results showed that a removal efficiency of 85% was obtained at 4 h contact time for a Cu2+ concentration of 30 mg/L at the optimum pH of 6.0. Equilibrium data were analysed using different isothermal models and kinetic models, analytic results indicated that the capture of Cu2+ by ZIF-8@Cs could favourably comply with the pseudo-first-order kinetic model and Langmuir isotherm model. The single-layer adsorption of Cu2+ on ZIF-8@Cs was dominated by diffusional mass transfer. Additionally, the results of the thermodynamic analysis indicated that the adsorption of Cu2+ by ZIF-8/Cs was a spontaneous, exothermic, and ordered process. Overall, the results reported herein indicated that ZIF-8/Cs with high adsorption efficiency are very attractive and imply a potential practical application for the removal of potentially toxic elements in wastewater.
{"title":"Synthesis of ZIF-8/chitosan composites for Cu2+ removal from water.","authors":"Ni Liao,Furong Li,Xiuli Huang,Yi Zhang","doi":"10.1080/09593330.2024.2401158","DOIUrl":"https://doi.org/10.1080/09593330.2024.2401158","url":null,"abstract":"In this work, a kind of novel Chitosan (Cs)-doped zeolite imidazole framework (ZIF-8@Cs) with a larger surface area and a smaller pore size was synthesised via a facial solvothermal approach and applied to remove Cu2+ from mine wastewater. Compared to nondoped ZIF-8, ZIF-8@Cs exhibited a stronger adsorption performance and removal efficiency. The reason was that ZIF-8@Cs doped by the Cs could suppress the aggregation and increase the monodispersity of ZIF-8. Using the high-performance ZIF-8@Cs, as a novel adsorbent, was successfully developed for the efficient removal of Cu2+ from mine wastewater. Various parameters, such as contact time, initial Cu2+ concentration, adsorbent dosage, and pH, were investigated. The results showed that a removal efficiency of 85% was obtained at 4 h contact time for a Cu2+ concentration of 30 mg/L at the optimum pH of 6.0. Equilibrium data were analysed using different isothermal models and kinetic models, analytic results indicated that the capture of Cu2+ by ZIF-8@Cs could favourably comply with the pseudo-first-order kinetic model and Langmuir isotherm model. The single-layer adsorption of Cu2+ on ZIF-8@Cs was dominated by diffusional mass transfer. Additionally, the results of the thermodynamic analysis indicated that the adsorption of Cu2+ by ZIF-8/Cs was a spontaneous, exothermic, and ordered process. Overall, the results reported herein indicated that ZIF-8/Cs with high adsorption efficiency are very attractive and imply a potential practical application for the removal of potentially toxic elements in wastewater.","PeriodicalId":12009,"journal":{"name":"Environmental Technology","volume":null,"pages":null},"PeriodicalIF":2.8,"publicationDate":"2024-09-11","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142216035","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2024-09-11DOI: 10.1080/09593330.2024.2402099
Shanzhu Jiang,Zhaobo Wang,Yangjie Qin,Ruan Chi,Shengchao Huang,Huijuan Ma,Zhongjun Li
In order to promote the high-value utilization of waste phosphogypsum (PG), hydroxyapatite was directly synthesized from PG by acid precipitation-hydrothermal method (PGHAP), which was used for the adsorption of bovine serum albumin (BSA) and lysozyme (LYS). The synthesized PGHAP was characterized by XRD, SEM, FTIR and BET, and the effects of various factors on protein adsorption capacity were studied. The results showed that PGHAP exhibits a clear needle-like morphology, high crystallinity, and an average size of about 200 nm. The pH had the greatest effect on the adsorption of protein, and the highest adsorption capacity was obtained at pH 4.0. In addition, the adsorption mechanism of protein on PGHAP was explored by adsorption kinetics and adsorption isotherm. The adsorption of protein on PGHAP conforms to the Intra-particle diffusion model kinetic model, the maximum adsorption capacity of protein on PGHAP can reach 31 mg/g, which is comparable to other adsorbents in this field. In addition, the adsorption behaviour of PGHAP on protein is more appropriately described by Langmuir isotherm model, which indicates that the binding site with uniform energy on the surface of PGHAP realizes the monolayer adsorption of protein. The main adsorption mechanisms are ion exchange, co-precipitation, complexation reaction and so on. Therefore, the needle-like PGHAP synthesized from waste PG is a protein adsorbent with industrial application potential.
{"title":"Acid precipitation-hydrothermal synthesis of needle-like hydroxyapatite for protein adsorption from waste phosphogypsum.","authors":"Shanzhu Jiang,Zhaobo Wang,Yangjie Qin,Ruan Chi,Shengchao Huang,Huijuan Ma,Zhongjun Li","doi":"10.1080/09593330.2024.2402099","DOIUrl":"https://doi.org/10.1080/09593330.2024.2402099","url":null,"abstract":"In order to promote the high-value utilization of waste phosphogypsum (PG), hydroxyapatite was directly synthesized from PG by acid precipitation-hydrothermal method (PGHAP), which was used for the adsorption of bovine serum albumin (BSA) and lysozyme (LYS). The synthesized PGHAP was characterized by XRD, SEM, FTIR and BET, and the effects of various factors on protein adsorption capacity were studied. The results showed that PGHAP exhibits a clear needle-like morphology, high crystallinity, and an average size of about 200 nm. The pH had the greatest effect on the adsorption of protein, and the highest adsorption capacity was obtained at pH 4.0. In addition, the adsorption mechanism of protein on PGHAP was explored by adsorption kinetics and adsorption isotherm. The adsorption of protein on PGHAP conforms to the Intra-particle diffusion model kinetic model, the maximum adsorption capacity of protein on PGHAP can reach 31 mg/g, which is comparable to other adsorbents in this field. In addition, the adsorption behaviour of PGHAP on protein is more appropriately described by Langmuir isotherm model, which indicates that the binding site with uniform energy on the surface of PGHAP realizes the monolayer adsorption of protein. The main adsorption mechanisms are ion exchange, co-precipitation, complexation reaction and so on. Therefore, the needle-like PGHAP synthesized from waste PG is a protein adsorbent with industrial application potential.","PeriodicalId":12009,"journal":{"name":"Environmental Technology","volume":null,"pages":null},"PeriodicalIF":2.8,"publicationDate":"2024-09-11","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142216032","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2024-09-11DOI: 10.1080/09593330.2024.2401645
Wenxiao Wang,Xiaojing Zhang,Bingbing Ma,Han Zhang,Qiong Wang,Yali Song,Yongpeng Ma
Partial nitrification (PN) is a prerequisite step for the short-cut nitrogen removal process, which is crucial to provide stable nitrite accumulation for subsequent units. The present study innovatively proposed a new strategy for the rapid establishment of PN by adopting short-term anoxic starvation combined with high free ammonia inhibition. The sludge obtained from the secondary sedimentation tank of a municipal wastewater treatment plant was starved for 7 days under anoxic conditions, and then wastewater with high ammonia nitrogen (400 mg L-1) was introduced. Within 17 days, stable nitrite accumulation was achieved in the sequencing batch reactor, and the nitrite accumulation rate reached more than 95.0%. The activity of ammonia monooxygenase enzyme increased from 0.0364 ± 0.0074 to 0.1275 ± 0.0021 μg NO2--N·mg-1 protein min-1, while that of hydroxylamine oxidoreductase enzyme increased from 1.5350 ± 0.0208 to 6.3852 ± 0.0400 EU g-1 SS. The relative abundance of Nitrosomonas increased from 0.10% to 25.90%, while that of Nitrospira consistently remained below 0.04%. And the relative abundance of short-cut denitrifying bacteria, including Truepera, OLB8, and OLB13 all increased. The results proved that the short-term anoxic starvation combined with high free ammonia inhibition was an effective strategy for rapid establishment of PN.
{"title":"Rapid achievement of partial nitrification process by adopting the combined strategy of anoxic starvation and free ammonia inhibition.","authors":"Wenxiao Wang,Xiaojing Zhang,Bingbing Ma,Han Zhang,Qiong Wang,Yali Song,Yongpeng Ma","doi":"10.1080/09593330.2024.2401645","DOIUrl":"https://doi.org/10.1080/09593330.2024.2401645","url":null,"abstract":"Partial nitrification (PN) is a prerequisite step for the short-cut nitrogen removal process, which is crucial to provide stable nitrite accumulation for subsequent units. The present study innovatively proposed a new strategy for the rapid establishment of PN by adopting short-term anoxic starvation combined with high free ammonia inhibition. The sludge obtained from the secondary sedimentation tank of a municipal wastewater treatment plant was starved for 7 days under anoxic conditions, and then wastewater with high ammonia nitrogen (400 mg L-1) was introduced. Within 17 days, stable nitrite accumulation was achieved in the sequencing batch reactor, and the nitrite accumulation rate reached more than 95.0%. The activity of ammonia monooxygenase enzyme increased from 0.0364 ± 0.0074 to 0.1275 ± 0.0021 μg NO2--N·mg-1 protein min-1, while that of hydroxylamine oxidoreductase enzyme increased from 1.5350 ± 0.0208 to 6.3852 ± 0.0400 EU g-1 SS. The relative abundance of Nitrosomonas increased from 0.10% to 25.90%, while that of Nitrospira consistently remained below 0.04%. And the relative abundance of short-cut denitrifying bacteria, including Truepera, OLB8, and OLB13 all increased. The results proved that the short-term anoxic starvation combined with high free ammonia inhibition was an effective strategy for rapid establishment of PN.","PeriodicalId":12009,"journal":{"name":"Environmental Technology","volume":null,"pages":null},"PeriodicalIF":2.8,"publicationDate":"2024-09-11","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142216034","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
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