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Complex analysis of heavy metals mobility in the soils of the border town of Blagoveshchensk (Far East, Russia) 边境城镇布拉戈维申斯克(俄罗斯远东)土壤重金属迁移的复杂分析
IF 0.7 4区 环境科学与生态学 Q4 ENVIRONMENTAL SCIENCES Pub Date : 2019-11-21 DOI: 10.1504/ijep.2019.103750
V. Radomskaya, N. Borodina, L. M. Pavlova
A comprehensive assessment of the degree of heavy metals mobility in the soils of Blagoveshchensk was carried out, based on research on HM fractional composition and mathematical statistics. It was shown that the majority of Cu, Cr, Ni, Co and Pb accumulates in residual fraction components and that Mn, Cd and Zn accumulate in Fe- and Mn-hydroxides and the residual fraction. Under the increased technogenic addition of Zn contaminants, Pb was fixed in soil due to unstable specific absorption, Cd due to specific absorption and in hydroxide fraction. Cu was bound to an organic fraction, and Cr, Co and Ni to organic and hydroxide fractions. In urban soils compared to background soil, there was increased potential for the mobility of Zn, Pb, Ni, Cu, Cr and Cd. Among the elements studied, Zn, Mn and Cd, whose potential mobility corresponds to a high level of danger, posed the greatest danger.
在HM分数组成和数理统计研究的基础上,对布拉戈维申斯克土壤中重金属的迁移程度进行了综合评价。结果表明,Cu、Cr、Ni、Co和Pb主要富集在残余组分中,Mn、Cd和Zn主要富集在Fe和Mn的氢氧化物和残余组分。在增加Zn污染物的工艺添加下,Pb因比吸收不稳定而固定在土壤中,Cd因比吸收而固定在氢氧化物部分中。Cu与有机馏分结合,Cr、Co和Ni与有机馏分和氢氧化物馏分结合。与背景土壤相比,城市土壤中Zn、Pb、Ni、Cu、Cr和Cd的迁移潜力增加。在所研究的元素中,Zn、Mn和Cd的潜在迁移率对应于高水平的危险,构成了最大的危险。
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引用次数: 0
Numerical modelling of transient dispersion of air pollution in perpendicular urban street intersection with detail inclusion of traffic dynamics 包含交通动力学细节的垂直城市街道交叉口空气污染瞬态扩散的数值模拟
IF 0.7 4区 环境科学与生态学 Q4 ENVIRONMENTAL SCIENCES Pub Date : 2019-08-27 DOI: 10.1504/IJEP.2019.10023400
J. Pospíšil, M. Jicha
In this study, the authors focus on the utilisation of computer modelling for the detailed identification of transient pollutants' dispersion in a perpendicular intersection equipped with traffic lights. Passenger cars are considered as the main source of the air pollution in the intersection. Car movement is at the same time a major driving force affecting the air flow in the crossroad area. A model based on an Eulerian-Lagrangian approach to moving objects has been integrated into a commercial CFD software package StarCD. The inclusion of traffic dynamics is used for a correct description of dispersion processes. The air pollution concentration fields were obtained from numerical predictions for traffic light switching periods of 60, 90, and 120 s. The correctness of the developed dispersion model was assessed on the base of NOx concentration measurements carried out in a real city intersection with similar geometry as in the numerical model.
在这项研究中,作者专注于利用计算机建模来详细识别配备红绿灯的垂直交叉口中的瞬态污染物扩散。客车被认为是十字路口空气污染的主要来源。汽车运动同时也是影响十字路口空气流动的主要驱动力。基于欧拉-拉格朗日方法的运动物体模型已集成到商业CFD软件包StarCD中。包含交通动力学用于正确描述分散过程。空气污染浓度场是从60、90和120秒的红绿灯切换期的数值预测中获得的。基于在与数值模型中几何形状相似的真实城市交叉口中进行的NOx浓度测量,评估了所开发的分散模型的正确性。
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引用次数: 3
The coupled chemistry-meteorology model BOLCHEM: an application to air pollution in the Po Valley (Italy) hot spot 化学-气象耦合模型BOLCHEM在意大利波谷热点地区空气污染中的应用
IF 0.7 4区 环境科学与生态学 Q4 ENVIRONMENTAL SCIENCES Pub Date : 2019-08-27 DOI: 10.1504/IJEP.2019.10023397
R. Cesari, T. Landi, A. Maurizi
We present the model performance of the online air quality model BOLCHEM on seasonal period (year 2010) in an air pollution hot spot located in Northern Italy. Simulated surface concentrations of pollutants are compared with those measured at background AirBase stations. Particulate matter (PM10 and PM2.5) is investigated for winter and summer period. The correlation coefficient R is 0.6 for both pollutants and in both seasons. In the winter period, the PM2.5 ground concentration is underestimated by 6.5% on average, the PM10 ground concentration is underestimated by 7.8% on average. In the summer period, the PM2.5 average ground concentration is underestimated by 0.7% on average, while the PM10 average ground concentration is underestimated by 20% on average. The last result suggests that PM10 from Saharan dust storms is underestimated. Ozone (O3) ground concentration is considered only in summer period. It is well reproduced, the correlation coefficient R is 0.7.
我们展示了在线空气质量模型BOLCHEM在意大利北部一个空气污染热点季节(2010年)的模型性能。模拟的表面污染物浓度与在背景空军基地站测得的污染物浓度进行了比较。研究了冬季和夏季的颗粒物(PM10和PM2.5)。两种污染物和两个季节的相关系数R均为0.6。冬季PM2.5地面浓度平均低估6.5%,PM10地面浓度平均高估7.8%。在夏季,PM2.5平均地面浓度平均低估了0.7%,而PM10平均地面浓度则平均低估了20%。最后一个结果表明撒哈拉沙尘暴的PM10被低估了。臭氧(O3)地面浓度仅在夏季考虑。它被很好地再现,相关系数R为0.7。
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引用次数: 4
Effects of increasing the surface reflectance over air quality levels using WRF-BEM/AEMM/CMAQ: application over the city of Madrid 使用WRF-BEM/AEMM/CMAQ增加地表反射率对空气质量水平的影响:在马德里市的应用
IF 0.7 4区 环境科学与生态学 Q4 ENVIRONMENTAL SCIENCES Pub Date : 2019-08-27 DOI: 10.1504/IJEP.2019.10023406
M. A. González, R. Arasa, P. Gámez, Miquel Picanyol, P. Campra
The effects of increasing the surface reflectance by albedo modifications have been evaluated using an air quality modelling system. We have evaluated the influence over pollutant concentrations of increasing from 0.20 to 0.55 the roof surface albedo (scenario called Albedo1) and increasing from 0.15 to 0.30 the ground surface albedo and from 0.20 to 0.55 the roof surface albedo for all urban categories (scenario called Albedo2). To obtain a better representation of the local processes we have considered very high resolution (333.33 m) and up to 10 different urban categories. Changes in albedo cause changes in different meteorological parameters (planetary boundary layer height, radiation and temperature), modifying the pollutant concentration in every single scenario. Results show that this mitigation measure is effective during summer periods, providing not high NO2 increments and O3 reduction on the urban areas of the city of Madrid. Whilst during winter periods the measure induces NO2 increments over polluted areas with high NOx emissions. In this way, the benefits of the measure, from the point of view of urban heat island effects, are greater than the detriments during summer periods, in comparison with air quality effects.
已经使用空气质量建模系统评估了通过反照率修改来增加表面反射率的影响。我们评估了所有城市类别的屋顶表面反照率从0.20增加到0.55(情景称为“反照率1”)、地面反照率由0.15增加到0.30以及屋顶表面反射率从0.20提高到0.55对污染物浓度的影响。为了更好地反映局部过程,我们考虑了非常高的分辨率(333.33米)和多达10个不同的城市类别。反照率的变化会导致不同气象参数(行星边界层高度、辐射和温度)的变化,从而改变每种情况下的污染物浓度。结果表明,这种缓解措施在夏季是有效的,在马德里市的城市地区提供了不高的NO2增量和O3减少。而在冬季,该措施会导致NOx排放量高的污染地区的NO2增加。这样,从城市热岛效应的角度来看,与空气质量影响相比,该措施在夏季的好处大于坏处。
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引用次数: 2
A new bottom-up emissions estimation approach for aircraft sources in support of air quality modelling for community-scale assessments around airports. 一种新的自下而上的飞机排放估算方法,以支持机场周围社区规模评估的空气质量模型。
IF 0.7 4区 环境科学与生态学 Q4 ENVIRONMENTAL SCIENCES Pub Date : 2019-08-22 DOI: 10.1504/IJEP.2019.101832
S. Arunachalam, Brian Naess, Catherine Seppanen, Alejandro Valencia, J. Brandmeyer, A. Venkatram, J. Weil, Vlad Isakov, T. Barzyk
Transportation infrastructure (including roadway traffic, ports, and airports) is critical to the nation's economy. With a growing economy, aircraft activity is expected to grow across the world. In the US, airport-related emissions, while generally small, are not an insignificant source of air pollution and related adverse health effects. However, currently there is a lack of tools that can easily be applied to study near-source pollution and explore the benefits of improvements to air quality and exposures. Screening-level air quality modelling is a useful tool for examining urban-scale air quality impacts of airport operations. Spatially-resolved aircraft emissions are needed for the screening-level modelling. In order to create spatially-resolved aircraft emissions, we developed a bottom-up emissions estimation methodology that includes data from a global chorded inventory dataset from the aviation environmental design tool (AEDT). The initial implementation of this method was performed for Los Angeles International Airport (LAX). This paper describes a new emissions estimation methodology for aircraft emissions in support of community-scale assessments of air quality around airports and presents an illustration of its application at the Los Angeles International Airport during the LAX 2011/2012 Air Quality Source Apportionment Study.
交通基础设施(包括道路交通、港口和机场)对国家经济至关重要。随着经济的增长,飞机活动预计将在全球范围内增长。在美国,与机场有关的排放虽然总体上很小,但对空气污染和相关的不良健康影响并非微不足道。然而,目前缺乏工具,可以很容易地应用于研究近源污染和探索改善空气质量和暴露的好处。筛选级别的空气质素模型是一种有用的工具,可用于研究机场运作对城市空气质素的影响。筛选级建模需要空间分辨的飞机发射。为了创建空间分辨的飞机排放,我们开发了一种自下而上的排放估算方法,该方法包括来自航空环境设计工具(AEDT)的全球记录清单数据集的数据。这种方法的最初实施是在洛杉矶国际机场(LAX)。本文描述了一种新的飞机排放估算方法,以支持机场周围社区规模的空气质量评估,并在洛杉矶国际机场2011/2012年空气质量源分摊研究期间展示了该方法在洛杉矶国际机场的应用实例。
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引用次数: 1
Evaluation of the NO2 burden within a joint street canyon and tunnel portal micro environment 街道峡谷与隧道入口联合微环境NO2负荷评价
IF 0.7 4区 环境科学与生态学 Q4 ENVIRONMENTAL SCIENCES Pub Date : 2019-08-22 DOI: 10.1504/IJEP.2019.10023398
U. Uhrner, R. Reifeltshammer, P. Sturm
Substantial breaches in NO2 limits in the vicinity of a tunnel portal and street canyon micro environment provided the motivation for this paper. The impact of portal and surface road emissions was assessed and mitigation scenarios computed, in order to aid the authorities responsible. Emphasis was placed on detailed emission processing. A unique data set from nine NO2 monitors located near the portal and within the street canyon was used to evaluate the model approach using a Lagrangian particle model. Good agreement with measurements was obtained using simple NOx/NO2 conversion approaches. The NOx/NO2 concentration pattern is dominated by surface road emissions. A kerbside area of ~30 m in the driving direction is clearly dominated by the portal emissions indicating effective diffusion at the portal. Major uncertainties are related to the interaction of flow and turbulent mixing from ambient atmospheric conditions and traffic, particularly at low wind speed conditions.
隧道入口附近NO2限制的大量突破和街道峡谷微环境为本文提供了动力。评估了门户和地面道路排放的影响,并计算了缓解方案,以协助主管当局。重点放在详细的排放处理上。利用位于入口附近和街道峡谷内的9个二氧化氮监测仪的独特数据集,使用拉格朗日粒子模型来评估模型方法。使用简单的NOx/NO2转换方法与测量结果吻合良好。NOx/NO2浓度格局以路面排放为主。车辆行驶方向约30 m的路边区域明显受到门洞辐射的支配,表明门洞处的有效扩散。主要的不确定性与来自环境大气条件和交通的流动和湍流混合的相互作用有关,特别是在低风速条件下。
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引用次数: 0
Emission projections and limit values of air pollution concentration - a case study using the EMEP4PL model 排放预测及空气污染浓度极限值-使用EMEP4PL模式的个案研究
IF 0.7 4区 环境科学与生态学 Q4 ENVIRONMENTAL SCIENCES Pub Date : 2019-08-22 DOI: 10.1504/IJEP.2019.10023404
M. Werner, M. Kryza, K. Wałaszek
In this study, we applied the EMEP/MSC-W model at a high spatial resolution of 4 km × 4 km over Poland (EMEP4PL), and ran the model for the whole of the years 2015 and 2030. For the second simulation we used GAINS PRIMES emission projection and kept the meteorology from 2015. Although the model results are satisfactory and comparable to the results in other European countries, the number of days with exceedances of the limit value is highly underestimated in comparison to observations for 2015. It shows that the model is limited in its simulation of very high particulate matter concentrations in the winter season. Therefore, we applied a bias correction for the year 2030 based on the observations and model results for the year 2015. Bias corrected simulation shows that at 60 stations (out of 104), the PM10 daily limit value will be exceeded at least 35 times in 2030.
在这项研究中,我们在波兰上空应用了4公里×4公里的高空间分辨率的EMEP/MS-W模型(EMEP4PL),并在2015年和2030年运行了该模型。在第二次模拟中,我们使用了GAINSPRIMES排放预测,并保留了2015年的气象数据。尽管模型结果令人满意,并可与其他欧洲国家的结果相比较,但与2015年的观测结果相比,超过限值的天数被严重低估。这表明,该模型在模拟冬季非常高的颗粒物浓度方面是有限的。因此,我们根据2015年的观测结果和模型结果,对2030年进行了偏差校正。偏差校正模拟显示,在104个站点中的60个站点,2030年PM10日限值将至少超过35次。
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引用次数: 2
Modelling the air quality for assessing the health benefits of urban regeneration: a case of Tallinn city Centre, Estonia 建立空气质量模型以评估城市再生对健康的益处:以爱沙尼亚塔林市中心为例
IF 0.7 4区 环境科学与生态学 Q4 ENVIRONMENTAL SCIENCES Pub Date : 2019-08-22 DOI: 10.1504/IJEP.2019.10023410
M. Kaasik, Mihkel Pindus, Tanel Tamm, H. Orru
Concentrations of nitrogen dioxide and particulate matter were modelled to assess the health benefits of an urban regeneration scenario for the central part of Tallinn, where the traffic on two of the main streets will be reduced to create a more friendly space for active commuters. To model the air quality the stationary Gaussian plume model AEROPOL was used with a 25 m grid resolution. The model was validated against a stationary air quality monitoring station in the domain. The health benefits of the scenarios were calculated based on the changes in air pollution exposures for residents and daily visitors, using methods of health impact assessment. This research predicts that each year the reduction of exhaust (indicated by NO2) and road dust (indicated by PM10) exposure in the city centre would prevent up to 0.29 premature deaths (−27%) among the general population, 0.57 deaths (−3.6%) among daily visitors, 0.18 deaths (−21.2%) among pedestrians, and 0.03 deaths (−24.7%) among people public transport users.
对二氧化氮和颗粒物的浓度进行了建模,以评估塔林市中心城市再生方案的健康效益,其中两条主要街道的交通量将减少,为活跃的通勤者创造一个更友好的空间。为了模拟空气质量,使用了25米网格分辨率的静止高斯羽流模型AEROPOL。该模型与该领域的一个固定空气质量监测站进行了验证。这些情景的健康效益是根据居民和日常访客的空气污染暴露变化,使用健康影响评估方法计算的。这项研究预测,每年减少市中心的废气(以NO2表示)和道路灰尘(以PM10表示)暴露将防止普通人群中多达0.29人过早死亡(−27%),日常游客中多达0.57人死亡(−3.6%),行人中多达0.18人死亡(–21.2%),公共交通使用者中多达0.03人死亡(-24.7%)。
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引用次数: 1
Air exchange in urban canyons with variable building width: a numerical LES approach 可变建筑宽度的城市峡谷中的空气交换:数值LES方法
IF 0.7 4区 环境科学与生态学 Q4 ENVIRONMENTAL SCIENCES Pub Date : 2019-08-22 DOI: 10.1504/IJEP.2019.101836
M. Garau, M. G. Badas, Simon Ferrari, A. Seoni, G. Querzoli
The aim of this work is to gain further insight into the role played by the building aspect ratio (ARB, i.e., the ratio of the building width, WB, to the building height, H) and its influence on street canyon flow. We carried out a series of large eddy simulations with arrays of obstacles with different widths, ranging from 0.5 to 2.0, and two canyon aspect ratios (ARC, i.e., the ratio of the canyon width, W, to H) ARC = 0.5 and ARC = 1.0. Experimental data was obtained in a water channel for the corresponding configuration and used to validate numerical simulations. Results were found strongly dependent on the building aspect ratios, with two distinct behaviours identified with respect to the canyon aspect ratio. The residence time decreases with decreasing ARB, irrespective of the canyon aspect ratio, suggesting that ARB and ARC can be optimised to guarantee optimal street canyon ventilation in urban planning.
这项工作的目的是进一步了解建筑纵横比(ARB,即建筑宽度WB与建筑高度H的比值)所起的作用及其对街道峡谷流量的影响。我们用不同宽度(从0.5到2.0)的障碍物阵列和两个峡谷纵横比(ARC,即峡谷宽度W与H的比率)ARC=0.5和ARC=1.0进行了一系列大涡模拟。在水道中获得了相应配置的实验数据,并用于验证数值模拟。结果强烈依赖于建筑纵横比,峡谷纵横比有两种不同的行为。无论峡谷纵横比如何,居住时间都会随着ARB的减少而减少,这表明ARB和ARC可以进行优化,以确保城市规划中街道峡谷的最佳通风。
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引用次数: 4
Spatial representativeness evaluation of air quality monitoring sites by point-centred variography 点中心变差法评价空气质量监测点的空间代表性
IF 0.7 4区 环境科学与生态学 Q4 ENVIRONMENTAL SCIENCES Pub Date : 2019-08-22 DOI: 10.1504/IJEP.2019.10023409
O. Kracht, M. Gerboles
We propose a geostatistical technique based on point-centred semi-variograms that can be used to derive valuable information about the spatial representativeness of air quality monitoring sites. Whereas classical geostatistics describes the spatial correlation structure of a concentration field in terms of the variogram, point-centred variography is based on the average of squared concentration differences observed in pairs formed from a particular central point and the set of all other points in the domain. It thereby places a monitoring station in the context of the local or regional air quality pattern. We demonstrate how a mathematical inversion of the point-centred variogram can provide estimates of the extent of the representativeness area of a monitoring site. The application of this approach is tested on a set of modelling data from the city of Antwerp, which was used for the FAIRMODE/AQUILA intercomparison exercise of methods for the assessment of spatial representativeness.
我们提出了一种基于点中心半变方差的地质统计技术,该技术可用于获得有关空气质量监测点空间代表性的有价值信息。经典地质统计学根据变异函数描述浓度场的空间相关结构,而以点为中心的变异函数是基于从特定中心点和域中所有其他点的集合形成的成对观察到的浓度差的平方的平均值。因此,它将监测站置于当地或区域空气质量模式的背景下。我们展示了以点为中心的变差函数的数学反演如何提供监测站点的代表性区域范围的估计。该方法的应用在安特卫普市的一组建模数据上进行了测试,该数据用于FAIRMODE/AQUILA空间代表性评估方法的相互比较。
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引用次数: 2
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International Journal of Environment and Pollution
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