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2019 IEEE Research and Applications of Photonics in Defense Conference (RAPID)最新文献

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Light-Induced Assembly and Reconfiguration of Chiral Nanostructures 手性纳米结构的光诱导组装与重构
Pub Date : 2019-08-01 DOI: 10.1109/RAPID.2019.8864373
Jiyoung Kim, Jihyeon Yeom, Heather A. Calcaterra, Gongpu Zhao, Peijun Zhang, Jiyoun Munn, N. Kotov
Matured syntheses of inorganic nanocolloids today have allowed production of diverse asymmertic nanoparticles (NP) and even more complex assemblies, introducing a variety of nanomaterials with unique properties. Chirality is one of most intriguing symmetry groups in field of material science due to the optical rotatory power of chiral substances. Strong optical activity of inorganic nanoparticles (NPs) afford photosynthetic routes to chiral superstructures using circularly polarized photons (1). Although plasmonic NPs are promising candidates for such synthetic routes due to the strong rotatory power of highly delocalized plasmonic states (2), realization of light- driven synthesis of chiral nanostructures has been more challenging for plasmonic NPs than for the semiconductor due to the short lifetime of the plasmonic states. The process also can be difficult to recognize, and therefore requires unconventional approaches for the quantification of chiral products. Here, we demonstrate that illumination of Au precursors in the presence of citric acid with right- (left-) handed circularly polarized light (CPL) induces the formation of chiral Au nanostructures. Despite seemingly irregular shape of the particles, the resulted colloids showed distinctive mirror-imaged opposite circular dichroism (CD) bands according to the handedness of illuminated CPL. Circular dichroic response and geometric chirality from these seemingly achiral structures were successfully demonstrated and quantified by implementing three-dimensional (3D) electron tomography (e-tomo) into computational model. The mechanism of the light-driven assembly of chiral nanostructures is based on the asymmetric displacement of NPs in dynamic assemblies by plasmonic fields fol-lowed by particle-to-particle attachment. The ability of Au nanostructures to retain the polarization information of incident photons can be applicable to light absorbing materials, thus to create a variety of chiral nanomaterials. Similar examination of seemingly irregular NP through suggested chirality measure can also elucidate previously puzzling optical response from unclear geometric asymmetry of nanomaterials.
如今,无机纳米胶体的成熟合成已经允许生产各种不对称纳米颗粒(NP)甚至更复杂的组件,引入了各种具有独特性能的纳米材料。由于手性物质具有旋光能力,手性是材料科学领域中最引人注目的对称群之一。无机纳米粒子(NPs)的强光学活性为利用圆偏振光子进行手性超结构的光合作用提供了途径(1)。尽管由于高度离域等离子体态的强旋转能力,等离子体纳米粒子是这种合成途径的有希望的候选物(2),但由于等离子体纳米粒子的寿命较短,实现光驱动合成手性纳米结构对等离子体纳米粒子来说比半导体更具挑战性。这个过程也很难识别,因此需要非常规的方法来量化手性产物。在这里,我们证明了在柠檬酸存在下,用右手(左手)圆偏振光(CPL)照射金前驱体可诱导手性金纳米结构的形成。尽管颗粒形状看似不规则,但所得到的胶体根据光照cpld的手性显示出独特的镜像相反的圆二色性(CD)带。通过将三维电子断层扫描(e-tomo)应用于计算模型,成功地证明了这些看似非手性结构的圆二色性响应和几何手性。光驱动手性纳米结构组装的机制是基于等离子体场在动态组装中NPs的不对称位移,然后是粒子间的附着。金纳米结构保留入射光子偏振信息的能力可应用于光吸收材料,从而制造出多种手性纳米材料。通过建议的手性测量对看似不规则的NP进行类似的检查,也可以解释以前令人困惑的纳米材料几何不对称的光学响应。
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引用次数: 0
Nonlinear Metasurfaces for Optical Applications 光学应用中的非线性超表面
Pub Date : 2019-08-01 DOI: 10.1109/RAPID.2019.8864424
A. Urbas
Metasurfaces have seen dramatic progress in broad band and large area systems recently and advances toward real applications are accelerating. While linear properties of metasurfaces are increasingly entering the engineering space, applications of nonlinear metasurface properties are emerging. Detecting optical signals in the mid and long wave infrared, and the generation, detection and conversion of single photons for quantum information applications are significant to a range of Air Force technologies and drive the research to increase performance and functionality. We explore how nonlinear properties of metasurfaces can be engineered for quantum information applications. We show that nonlinear multipolar interference allows both a non-reciprocal and unidirectional nonlinear generation from nanoelements, with the direction of nonlinear generation preserved with respect to a fixed laboratory coordinate system when reversing the direction of the fundamental field. This arises due to the existence of common (electric or magnetic) pathways inducing the electric and magnetic Mie resonances via a nonlinear interaction, such that switching the phase of one (electric or magnetic) of the vectors of the fundamental field can change simultaneously the phase of all (electric and magnetic) nonlinearly generated multipoles. These effects arise due to the nonlinear response of the component materials and we are actively pursuing novel materials systems and growth procedures to produce structures with controlled response. In order to develop such systems, precise control of structural dimensions at nanometric length scales is needed as well as plasmonic materials which are more resilient to nonlinear excitation intensities. A focus of our work is to explore novel materials systems that combine the functionality needed for nonlinear plasmonic metasurfaces and dynamic optical systems. This system is a useful example of where the engineering of materials response through structure to achieve desired optical properties can enable new potential technologies.
最近,超表面在宽带和大面积系统中取得了巨大的进步,并且在实际应用方面的进展正在加速。在超表面线性特性越来越多地进入工程领域的同时,非线性超表面特性的应用也在不断涌现。探测中波和长波红外光信号,以及用于量子信息应用的单光子的产生、探测和转换对空军的一系列技术具有重要意义,并推动了性能和功能的研究。我们探讨了如何将元表面的非线性特性用于量子信息应用。我们表明,非线性多极干涉允许纳米元件产生非互反和单向非线性,当基本场方向反转时,非线性产生的方向相对于固定的实验室坐标系保持不变。这是由于通过非线性相互作用诱导电和磁米氏共振的共同(电或磁)途径的存在而产生的,因此切换基本场矢量的一个(电或磁)的相位可以同时改变所有(电和磁)非线性产生的多极的相位。这些效应是由于组件材料的非线性响应而产生的,我们正在积极寻求新的材料系统和生长程序来生产具有可控响应的结构。为了开发这样的系统,需要在纳米尺度上精确控制结构尺寸,以及对非线性激发强度更有弹性的等离子体材料。我们的工作重点是探索结合非线性等离子体超表面和动态光学系统所需功能的新型材料系统。该系统是一个有用的例子,其中通过结构响应的材料工程可以实现所需的光学特性,从而实现新的潜在技术。
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引用次数: 0
Effects of Spatial Confinement on Nonlinear Light Emission from Plasmonic Nanostructures 空间约束对等离子体纳米结构非线性光发射的影响
Pub Date : 2019-08-01 DOI: 10.1109/RAPID.2019.8864429
R. Lemasters, H. Harutyunyan
Photoluminescence measurements from spatially confined resonant gap-mode plasmons in a metal-dielectric-metal geometry is performed. The PL signal is nonlinear and broadband in character, and the nonlinear power dependence is seen to deviate from spatially random systems such as rough metal films.
在金属-介电-金属几何结构中进行了空间受限共振隙模等离子体的光致发光测量。PL信号具有非线性和宽带特性,并且非线性功率依赖关系偏离了空间随机系统,如粗糙金属薄膜。
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引用次数: 0
Circularly Polarized Light Reflectance of and Wing Interference Patterns from Insects 昆虫的圆偏振光反射率及翅膀干涉图样
Pub Date : 2019-08-01 DOI: 10.1109/RAPID.2019.8864260
Laura E. Bagge, D. Goldstein, Nicholas I. Rummelt, M. Wehling
Certain insect body and wing surfaces interact with light in unique ways to reflect circularly polarized light or to produce colorful interference patterns. Our study characterizes these optical signatures with the goal of testing whether insects can perceive these optical signatures (i.e. have matched filters).
某些昆虫的身体和翅膀表面以独特的方式与光相互作用,反射圆偏振光或产生彩色干涉图案。我们的研究表征了这些光学特征,目的是测试昆虫是否可以感知这些光学特征(即具有匹配的过滤器)。
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引用次数: 0
High Power All-Fiber Amplifiers at Air Force Research Laboratory (AFRL) 美国空军研究实验室(AFRL)高功率全光纤放大器
Pub Date : 2019-08-01 DOI: 10.1109/rapid.2019.8864407
A. Flores, B. Anderson, N. Naderi, R. Holten, T. Ehrenreich, K. Rowland, I. Dajani
We present an overview of fiber amplifier power-scaling and beam-combining at AFRL. Nonlinear mitigation and power-scaling results of kW amplifiers is discussed. Here nonlinear suppression is attained through phase modulation and laser gain competition. Subsequently, five kW amplifiers were coherently combined into one 5kW beam.
本文对AFRL中光纤放大器的功率缩放和波束合并进行了综述。讨论了千瓦放大器的非线性抑制和功率缩放结果。通过相位调制和激光增益竞争实现非线性抑制。随后,5个kW的放大器被相干地组合成一个5kW的光束。
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引用次数: 1
Charge Injection in Organic Transistors and its Impact on the Validity of the Extracted Device Parameters 有机晶体管中的电荷注入及其对提取器件参数有效性的影响
Pub Date : 2019-08-01 DOI: 10.1109/RAPID.2019.8864270
O. Jurchescu
Organic semiconductors have sparked interest given their ease of processing, chemical diversity and tunable optoelectronic properties, which make them viable candidates for incorporation in low-cost, large-area flexible electronics. Nevertheless, transition to market place was not possible because the performance of organic devices has not reached the necessary benchmarks. Inefficient injection of charges from device electrodes into the semiconductor layer represents a significant hurdle in the pursuit of the promised potential of organic semiconductors. In this presentation I will discuss the origin and characterization of contact resistance in organic field-effect transistors (OFETs) and the impact on device performance and accuracy in extraction of charge carrier mobility. I will then present a strategy for reducing contact resistance in small molecule and polymeric OFETs, which consists of developing high work function domains at the surface of the injecting electrodes to promote channels of enhanced injection.1 By using this methodology, we demonstrated high-mobility transistors with near ideal current-voltage characteristics, contact resistances of 200 Ωcm, and device charge carrier mobilities of 20 cm2/Vs, independent of the applied gate voltage. I will further discuss fabrication of all-printed OFETs on conventional paper. For such devices, contacts were deposited using aerosol spray and patterned with a digitally printed mask from an office laser printer, at ambient temperature and pressure, while the organic semiconductor was deposited using an office laser printer.2 The method was successfully adopted for manufacturing different types of OFETs that showed an excellent tolerance to extreme bending, confirming its potential for emerging printed electronics applications.
有机半导体由于其易于加工、化学多样性和可调谐的光电特性而引起了人们的兴趣,这使它们成为低成本、大面积柔性电子产品的可行候选产品。然而,向市场过渡是不可能的,因为有机设备的性能尚未达到必要的基准。从器件电极向半导体层注入电荷的效率低下是追求有机半导体潜力的一个重大障碍。在本报告中,我将讨论有机场效应晶体管(ofet)中接触电阻的来源和表征,以及对器件性能和电荷载流子迁移率提取精度的影响。然后,我将提出一种在小分子和聚合物ofet中降低接触电阻的策略,该策略包括在注入电极表面开发高功函数域以促进增强注入通道通过使用这种方法,我们展示了具有接近理想电流电压特性的高迁移率晶体管,接触电阻为200 Ωcm,器件电荷载流子迁移率为20 cm2/Vs,与所施加的栅极电压无关。我将进一步讨论在传统纸张上制造全印刷的ofet。对于这类器件,在室温和环境压力下,使用气溶胶喷雾沉积触点,并使用办公室激光打印机的数字印刷掩模进行图案打印,而有机半导体则使用办公室激光打印机沉积该方法已成功用于制造不同类型的ofet,这些ofet对极端弯曲具有优异的耐受性,证实了其在新兴印刷电子应用中的潜力。
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引用次数: 0
Cavity-Resonator-Integrated Grating Couplers 腔-谐振腔-集成光栅耦合器
Pub Date : 2019-08-01 DOI: 10.1109/RAPID.2019.8864278
S. Ura, J. Inoue, K. Kintaka
Integration of a waveguide resonator can reduce an aperture of a grating coupler to enable its utilization in a channel waveguide. Resultantly obtained coupling characteristics such as selectivity or controllability are attractive for various applications including a compact WDM light source and micro-optic beam steering.
波导谐振器的集成可以减小光栅耦合器的孔径,使其能够在通道波导中使用。由此获得的耦合特性,如选择性或可控性,对包括紧凑型波分复用光源和微光束转向在内的各种应用具有吸引力。
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引用次数: 0
“Hybrid DAC” Approach to Increasing Dynamic Range and Signal to Noise in IRSP Systems 提高IRSP系统动态范围和信噪比的“混合DAC”方法
Pub Date : 2019-08-01 DOI: 10.1109/RAPID.2019.8864344
G. Ejzak, Miguel Hernandez, A. Landwehr, F. Kiamilev
We propose and show preliminary test results on a system to improve dynamic range and signal to noise ratio (SNR) in an infrared (IR) light-emitting diode (LED) display system by splitting the digital-to-analog conversion between the close-support electronics (CSE) and the read-in integrated-circuit (RIIC).
我们提出并展示了一个系统的初步测试结果,该系统通过在近支持电子(CSE)和读取集成电路(RIIC)之间分离数模转换来提高红外(IR)发光二极管(LED)显示系统的动态范围和信噪比(SNR)。
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引用次数: 0
Unique Photophysical Properties of Infrared Absorbing Polymers 红外吸收聚合物独特的光物理性质
Pub Date : 2019-08-01 DOI: 10.1109/RAPID.2019.8864395
M. Sfeir, Abagail K. Williams, Dana B. Sulas, N. Eedugurala, J. Azoulay
A nascent challenge for organic semiconductors is their application in infrared optoelectronics. However, infrared absorption is linked to the formation of strong electronic correlations and open-shell character. We use ultrafast spectroscopy to identify and explain the unusual photophysics of these materials.
有机半导体的一个新挑战是它们在红外光电子学中的应用。然而,红外吸收与形成强电子相关和开壳性质有关。我们使用超快光谱学来识别和解释这些材料的不寻常的光物理性质。
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引用次数: 0
Bioinspired/Chemically Enhanced Biosensor for Detection of Gaseous Isopropyl Alcohol 用于检测气态异丙醇的生物启发/化学增强生物传感器
Pub Date : 2019-08-01 DOI: 10.1109/RAPID.2019.8864317
Cody Walnoha, M. Brothers, Taneha Littlejohn, A. Islam, B. Maruyama, Jennifer A. Martin, Claude C. Grigsby, R. Naik, Steve S. Kim
Inhalation of IPA impairs cognition and depresses the nervous system. Current gas-phase sensors are unable to selectively detect isopropyl alcohol from other volatile organic compounds. We present the development of bioinspired sensors using nanomaterials to provide real-time monitoring and differentiate IPA from background compounds.
吸入IPA会损害认知能力,抑制神经系统。目前的气相传感器无法从其他挥发性有机化合物中选择性地检测异丙醇。我们提出了使用纳米材料的生物启发传感器的发展,以提供实时监测和区分IPA与背景化合物。
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引用次数: 0
期刊
2019 IEEE Research and Applications of Photonics in Defense Conference (RAPID)
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