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Advances in Ultrafast Condensed Phase Physics III最新文献

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Recombination dynamics in high energy (>3.5 eV) GaNAlN quantum dots: influence of lateral confinement, electric field and the dark-level trapping 高能(>3.5 eV) GaNAlN量子点的复合动力学:侧向约束、电场和暗能级俘获的影响
Pub Date : 2022-06-03 DOI: 10.1117/12.2621544
Maryna Hrytsaienko, M. Gallart, M. Ziegler, O. Crégut, P. Gilliot, S. Tamariz, R. Butté, N. Grandjean, B. Hönerlage
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引用次数: 0
Ultrafast light-induced strain and symmetry breaking in ferroic materials 铁材料的超快光致应变和对称破缺
Pub Date : 2022-06-03 DOI: 10.1117/12.2621510
R. Gu, G. Vaudel, V. Juvé, S. Fusil, V. Garcia, D. Sando, Mads Weber, C. Paillard, Vitalyi E. Goussev, H. Bouyanfif, B. Dkhil, C. Laulhé, P. Ruello
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引用次数: 0
DFT modelling of fused silica electronic structure under strong laser-induced excitation 激光强激发下熔融石英电子结构的DFT建模
Pub Date : 2022-06-03 DOI: 10.1117/12.2620774
A. Tsaturyan, E. Silaeva, R. Stoian, J. Colombier
Fused silica is an indispensable material in emergent photonic applications due to its unique optical, mechanical, and thermal properties, especially when it is nano-structured by an ultrashort laser pulse. The precision of the laser-induced modifications relies heavily on the control of the electron excitations and transient optical properties during the laser pulse. In this work we explore the fused silica band gap at high densities of excited electrons, using Density Functional Theory (DFT). Fused silica is a glass consisting of silica (SiO2) in amorphous form. It includes various structural variations since the topological arrangement of the SiO4 tetrahedra is not unique. We model fused silica as a molecule consisting of six SiO4 tetrahedra. Fused silica geometry parameters (bond lengths and angles) and electronic structure reported experimentally are well reproduced with a reasonable computational demand. Figure 1 shows the gap between the highest occupied molecular orbital (HOMO) and lowest unoccupied molecular orbital (LUMO) for molecular structures with different number of SiO4 tetrahedra. The HOMO-LUMO gap in this case represents the optical gap of fused silica measured experimentally.
熔融二氧化硅由于其独特的光学、机械和热性能,特别是在超短激光脉冲的纳米结构下,是新兴光子应用中不可缺少的材料。激光诱导修饰的精度很大程度上取决于对激光脉冲中电子激发和瞬态光学特性的控制。在这项工作中,我们利用密度泛函理论(DFT)探索了高密度激发电子下熔融二氧化硅带隙。熔融二氧化硅是由无定形的二氧化硅(SiO2)组成的玻璃。由于SiO4四面体的拓扑排列不是唯一的,因此它包括各种结构变化。我们将熔融二氧化硅建模为由六个SiO4四面体组成的分子。实验报道的熔融石英几何参数(键长和键角)和电子结构在合理的计算需求下得到了很好的再现。图1显示了不同数量SiO4四面体分子结构的最高已占据分子轨道(HOMO)和最低未占据分子轨道(LUMO)之间的间隙。在这种情况下,HOMO-LUMO间隙代表了实验测量的熔融二氧化硅的光学间隙。
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引用次数: 0
Ultrafast photoisomerization studied by time-resolved photoelectron spectroscopy 时间分辨光电子能谱法研究超快光异构化
Pub Date : 2022-06-03 DOI: 10.1117/12.2627142
C. Granados, E. Titov, J. Hummert, E. Ikonnikov, S. Haacke, R. Mitrić, O. Kornilov
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引用次数: 0
High harmonic generation in strongly correlated materials 强相关材料中的高谐波产生
Pub Date : 2022-06-03 DOI: 10.1117/12.2631085
Koichiro Tanaka
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引用次数: 0
Ultrafast laser generation of overcritical, nanoplasmas inside dielectrics 电介质内超临界纳米等离子体的超快激光产生
Pub Date : 2022-05-30 DOI: 10.1117/12.2621444
Mostafa E. Hassan, K. Ardaneh, R. Meyer, R. Giust, Xie Chen, B. Morel, I. Ouadghiri-Idrissi, L. Furfaro, L. Froehly, A. Couairon, G. Bonnaud, F. Courvoisier
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引用次数: 0
LaB6 nanotip as an ultrafast electron source LaB6纳米尖端作为超快电子源
Pub Date : 2022-05-30 DOI: 10.1117/12.2621526
O. Bhorade, I. Blum, J. Houard, B. Deconihout, A. Vella
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引用次数: 0
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Advances in Ultrafast Condensed Phase Physics III
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