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Multi-band chirped mirrors for enhanced dispersion management 用于增强频散管理的多波段啁啾反射镜
Pub Date : 2024-08-07 DOI: 10.1016/j.optlastec.2024.111525
Shih-Hsuan Chia, Yan-Cheng Li, Chi-Kuang Sun, Franz X. Kärtner
Effective dispersion management for broadband and highly dispersive optical systems becomes increasingly vital in ultrafast applications. While chirped mirrors provide a compact solution, their attainable dispersion is often limited by the operational bandwidth. This study introduces innovative multi-band chirped mirror designs that enable the management of group delay differences both within and between bands, further optimizing group delay dispersion across specific spectral regions. Here, we highlight the critical role of transmission group delay within multilayer coatings for broadband dispersion management, shifting the traditional interpretation which relies on the wavelength-dependent penetration of these coatings. We have thus developed a dual-band chirped mirror pair achieving group delay dispersion values of −100 fs in the 0.6–0.8 µm range and −260 fs in the 1.7–2.2 µm range, with the bands separated by more than an octave. Remarkably, this design outperformed a state-of-the-art ultrabroadband mirror pair by three and four times of group delay dispersion in the respective bands. We have also designed and implemented a specialized dual-band mirror pair for nonlinear light microscopy—a prime example of ultrafast applications—and successfully achieved transform-limited pulses for targeted fluorophore excitations. This research emphasizes the transformative potential of strategic group delay distribution, heralding a breakthrough in dispersive optical operations across specific wavelength ranges.
在超快应用中,对宽带和高色散光学系统进行有效的色散管理变得越来越重要。虽然啁啾镜提供了一种紧凑型解决方案,但其可实现的色散往往受到工作带宽的限制。本研究介绍了创新的多波段啁啾镜设计,能够管理波段内和波段间的群延迟差异,进一步优化特定光谱区域的群延迟色散。在这里,我们强调了多层涂层内的传输群延迟在宽带色散管理中的关键作用,改变了依赖于这些涂层的波长穿透性的传统解释。因此,我们开发了一种双波段啁啾镜对,在 0.6-0.8 µm 波段实现了 -100 fs 的群延迟色散值,在 1.7-2.2 µm 波段实现了 -260 fs 的群延迟色散值,两个波段之间的间隔超过一个倍频程。值得注意的是,这种设计在各自波段的群延迟色散上分别比最先进的超宽带镜对高出三倍和四倍。我们还设计并实现了用于非线性光显微镜的专用双波段镜对--这是超快应用的一个典型例子,并成功实现了用于目标荧光团激发的变换限制脉冲。这项研究强调了战略性群延迟分布的变革潜力,预示着特定波长范围内色散光学操作的突破。
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引用次数: 0
Generation of extremely strong accelerating electric field by focusing radially polarized THz pulses with a paraboloid ring 利用抛物面环聚焦径向偏振太赫兹脉冲,产生极强的加速电场
Pub Date : 2024-08-06 DOI: 10.1016/j.optlastec.2024.111554
László Pálfalvi, Zerihun T. Godana, György Tóth, János Hebling
Efficient acceleration of electrically charged particles by focused electromagnetic pulses requires a strong accelerating electric field as well as a sufficiently large interaction region. Single-cycle terahertz pulses are promising candidates for such applications due to their advantageous wavelength and available peak electric field at the level. We propose and characterize a focusing optics for a possible electron vacuum accelerator. This consists of a reflaxicon for beam shaping and a ring-like segment of an on-axis parabolic mirror for tight focusing of the radially polarized THz pulse in order to reach a strong accelerating electric field. The electric field distribution in the focal region was determined by the Stratton–Chu vector diffraction method. Semi-analytical and purely analytical formulae were also derived, simplifying the computation procedure. By focusing radially polarized single-cycle terahertz pulses with pulse energy, calculations predict accelerating electric field component in the order of , well suitable for particle acceleration.
利用聚焦电磁脉冲有效加速带电粒子需要强大的加速电场和足够大的相互作用区域。单周期太赫兹脉冲因其有利的波长和电平峰值电场而成为此类应用的理想候选者。我们为可能的电子真空加速器提出了一种聚焦光学器件,并对其进行了鉴定。它由一个用于光束整形的反射镜和一个轴上抛物面镜的环形部分组成,用于紧密聚焦径向偏振太赫兹脉冲,以获得强大的加速电场。焦点区域的电场分布是通过 Stratton-Chu 矢量衍射法确定的。同时还得出了半解析和纯解析公式,简化了计算过程。通过聚焦具有脉冲能量的径向极化单周期太赫兹脉冲,计算得出的加速电场分量为 ,非常适合粒子加速。
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引用次数: 0
Nonlinear optical response and application of indirect narrow-bandgap SbTe nanosheets 间接窄带隙碲化镉纳米片的非线性光学响应与应用
Pub Date : 2024-08-06 DOI: 10.1016/j.optlastec.2024.111563
Enlin Cai, Linhong Hao, Shanming Li, Min Chen, Shuaiyi Zhang, Xinxing Liu, Yin Hang
The nonlinear optical properties of antimony telluride (SbTe) crystal with indirect narrow bandgap are investigated, which exhibits superior performance for nonlinear laser modulation in the infrared band. The nonlinear optical coefficients of SbTe nanosheets are determined to be −3.3 cm/GW, −2.3 cm/GW, −1.9 cm/GW and the modulation depths are 5.5 %, 2.0 %, 1.5 % at 400 nm, 800 nm, 1064 nm, respectively. Based on the SbTe-SA, a Yb:GdScO laser centered at 1064 nm is achieved with 633 mW maximum output power, 56 fs pulse width and 104 MHz repetition rate. The damage threshold of the SbTe nanosheets is calculated to be exceed 338 GW/cm, revealing the great potential in high-power laser modulation. This investigation marks the inaugural theoretical and experimental analysis of SbTe’s optical properties and its application in laser modulation, laying the groundwork for future research into indirect narrow-bandgap materials in laser technology.
研究了具有间接窄带隙的碲化镉锑(SbTe)晶体的非线性光学特性,它在红外波段的非线性激光调制中表现出卓越的性能。在 400 nm、800 nm 和 1064 nm 波段,SbTe 纳米片的非线性光学系数分别为-3.3 cm/GW、-2.3 cm/GW、-1.9 cm/GW,调制深度分别为 5.5 %、2.0 %、1.5 %。在 SbTe-SA 的基础上,实现了以 1064 nm 为中心的 Yb:GdScO 激光器,其最大输出功率为 633 mW,脉冲宽度为 56 fs,重复频率为 104 MHz。根据计算,SbTe 纳米片的损伤阈值超过 338 GW/cm,揭示了高功率激光调制的巨大潜力。这项研究首次从理论和实验上分析了 SbTe 的光学特性及其在激光调制中的应用,为今后研究激光技术中的间接窄带隙材料奠定了基础。
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引用次数: 0
A nonlinear model of flexoelectric liquid crystal diffraction gratings 柔电液晶衍射光栅的非线性模型
Pub Date : 2024-08-06 DOI: 10.1016/j.optlastec.2024.111502
Qihao Han, Steve J. Elston, Waqas Kamal, Linpei Xue, Stephen M. Morris
This paper presents a nonlinear model for flexoelectric liquid crystal (LC) diffraction gratings and compares the results from simulations with those obtained from experiments, providing a more accurate description of the behaviour of the flexoelectric LC grating than that offered by the linear models that have been considered previously. The nonlinear model that is constructed considers both dielectric and flexoelectric coupling and, with the aid of numerical simulations, enables the visualization of the behaviour of the LC director in response to flexoelectric, dielectric, and elastic effects. From the numerical simulations, both in-plane and out-of-plane tilt angles are obtained which are then used to simulate the optical wave propagation and diffraction characteristics for light passing through the LC flexoelectric grating. To compare the results from simulations with experiments, we develop an LC mixture that is capable of forming a flexoelectric LC diffraction grating at room temperature. This mixture allows for real-time manipulation of the periodic splay-bend structure by adjusting the amplitude of the DC electric field, enabling control of the diffraction angle and intensity of light into the different diffraction orders. The consistency observed between our simulation results and experimental data underscores the reliability and accuracy of our proposed models.
本文提出了柔电液晶(LC)衍射光栅的非线性模型,并将模拟结果与实验结果进行了比较,从而对柔电液晶(LC)光栅的行为做出了比以往线性模型更精确的描述。所构建的非线性模型考虑了介电和挠电耦合,并借助数值模拟,使 LC 导向在挠电、介电和弹性效应下的行为可视化。通过数值模拟,可以得到平面内和平面外的倾斜角,然后利用这些倾斜角模拟光波传播和通过 LC 柔电光栅的衍射特性。为了将模拟结果与实验结果进行比较,我们开发了一种能够在室温下形成挠性 LC 衍射光栅的 LC 混合物。这种混合物可以通过调节直流电场的振幅来实时控制周期性的弯曲结构,从而控制进入不同衍射阶的光的衍射角和强度。我们的模拟结果与实验数据之间的一致性强调了我们提出的模型的可靠性和准确性。
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引用次数: 0
Analysis of plasmonic nanoparticles effects on the performance of perovskite solar cells through surface recombination and short-circuiting behaviors 通过表面重组和短路行为分析等离子纳米粒子对过氧化物太阳能电池性能的影响
Pub Date : 2024-08-05 DOI: 10.1016/j.optlastec.2024.111512
Mohamed M. Gad, Yasser M. El Batawy, Ezzeldin A. Soliman, Mai O. Sallam
Plasmonic photovoltaics integrate nanoparticles into the active layer to enhance power absorption. However a gap exists between simulated and experimental IV characteristics. Fabrication studies have attributed the issues to fabrication resolution, and recombination with no detailed step-by-step characterization. To address this issue, the paper presents a comprehensive optical and electrical study of a new plasmonic crescent nanoparticle (CNP). These particles serve as a near-field confinement source to enhance the efficiency of perovskite TiO-MAPbI-Spiro solar cells. The proposed design demonstrates that an optimized structure with polarization-dependent multiple modes can offer broad-spectrum absorption across both the visible and near-infrared spectra, resulting in a 15% improvement in the total absorption. The notably high stability of absorption with respect to parameter variation is a remarkable key factor. Employing Charge Transport (CHARGE) solver, the electrical characterization of the proposed plasmonic device is performed in a step-by-step procedure using three different models to characterize the sources of efficiency degradation The ohmic contact reduces quantum efficiency by 11%. Moreover, when surface recombination is considered, the degradation increases significantly to 54%, which matches the experimental studies in the literature. The paper also suggests incorporating a passivation layer which demonstrates its impact in enhancing the quantum efficiency from 18.2% to 22.2%.
等离子体光伏技术将纳米粒子集成到有源层中,以增强功率吸收。然而,模拟和实验 IV 特性之间存在差距。制造研究将问题归咎于制造分辨率和重组,但没有详细的分步表征。为解决这一问题,本文对一种新型等离子新月纳米粒子(CNP)进行了全面的光学和电学研究。这些粒子可用作近场约束源,以提高包晶TiO-MAPbI-Spiro太阳能电池的效率。所提出的设计表明,具有偏振相关多模式的优化结构可在可见光和近红外光谱范围内提供广谱吸收,从而使总吸收率提高 15%。与参数变化相关的高吸收稳定性是一个显著的关键因素。利用电荷传输(CHARGE)求解器,采用三种不同的模型对所提出的等离子器件进行了逐步的电学表征,以确定效率降低的原因。此外,当考虑到表面重组时,衰减显著增加到 54%,这与文献中的实验研究相吻合。论文还建议加入钝化层,这证明了钝化层在将量子效率从 18.2% 提高到 22.2% 方面的影响。
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引用次数: 0
Fabrication and characterization of self-lubricating anti-wear 316L stainless steel/h-BN composite coatings on Q235 substrate via laser cladding 通过激光熔覆在 Q235 基材上制作自润滑抗磨损 316L 不锈钢/h-BN 复合涂层并确定其特性
Pub Date : 2024-08-05 DOI: 10.1016/j.optlastec.2024.111564
Yun Chen, Yuliang Xu, Tao Li, Juan Du, Lingyu Guo, Kaixiong Hu
This paper presents the fabrication and characterization of self-lubricating, anti-wear 316L stainless steel composite coatings on a Q235 substrate using 316L stainless steel powders and nanoscale hexagonal boron nitride (h-BN) ceramic particles via coaxial powder feeding laser cladding. The influence of process parameters on cladding quality and geometry, and the impact of h-BN contents (2 wt% and 5 wt%) on the microstructure and mechanical properties of the coatings were studied. Optimal process parameters for 316L/5wt%BN coatings were identified: a powder feeding rate of 3–4 rpm, a laser power of 2200–2400 W, a scanning speed of 4–5 mm/s, and an overlapping rate of 40 %. Microstructural analysis showed a smooth surface without cracks or pores. X-ray diffraction revealed intermetallic compounds such as CrB, CrN, FeN, BN, and γ-(Fe, Ni). The inclusion of h-BN nanoparticles enhanced grain refinement, significantly increasing microhardness. Coatings with 5 wt% h-BN achieved an average microhardness of 438.8 HV10, 2.5 times higher than the substrate and the 316L stainless steel. Additionally, h-BN reduced friction coefficients, leading to substantial wear reduction. The 316L/5 wt% h-BN sample experienced only 4.2 mg of wear, 45.16 % of the substrate’s wear. These findings highlight the beneficial effects of h-BN nanoparticles on 316L stainless steel coatings, enhancing wear resistance, hardness, and overall performance.
本文介绍了利用 316L 不锈钢粉末和纳米级六方氮化硼(h-BN)陶瓷颗粒,通过同轴粉末进给激光熔覆技术,在 Q235 基材上制作自润滑抗磨损 316L 不锈钢复合涂层并对其进行表征。研究了工艺参数对熔覆质量和几何形状的影响,以及 h-BN 含量(2 wt% 和 5 wt%)对涂层微观结构和机械性能的影响。确定了 316L/5wt%BN 涂层的最佳工艺参数:粉末进给速度为 3-4 rpm,激光功率为 2200-2400 W,扫描速度为 4-5 mm/s,重叠率为 40%。微观结构分析表明,涂层表面光滑,无裂纹或气孔。X 射线衍射显示出金属间化合物,如 CrB、CrN、FeN、BN 和 γ-(Fe、Ni)。h-BN 纳米粒子的加入增强了晶粒细化,显著提高了显微硬度。含有 5 wt% h-BN 的涂层的平均显微硬度达到了 438.8 HV10,是基体和 316L 不锈钢的 2.5 倍。此外,h-BN 还降低了摩擦系数,从而大幅减少了磨损。316L/5 wt% h-BN 样品的磨损量仅为 4.2 毫克,是基体磨损量的 45.16%。这些发现凸显了 h-BN 纳米粒子对 316L 不锈钢涂层的有利影响,可提高耐磨性、硬度和整体性能。
{"title":"Fabrication and characterization of self-lubricating anti-wear 316L stainless steel/h-BN composite coatings on Q235 substrate via laser cladding","authors":"Yun Chen, Yuliang Xu, Tao Li, Juan Du, Lingyu Guo, Kaixiong Hu","doi":"10.1016/j.optlastec.2024.111564","DOIUrl":"https://doi.org/10.1016/j.optlastec.2024.111564","url":null,"abstract":"This paper presents the fabrication and characterization of self-lubricating, anti-wear 316L stainless steel composite coatings on a Q235 substrate using 316L stainless steel powders and nanoscale hexagonal boron nitride (h-BN) ceramic particles via coaxial powder feeding laser cladding. The influence of process parameters on cladding quality and geometry, and the impact of h-BN contents (2 wt% and 5 wt%) on the microstructure and mechanical properties of the coatings were studied. Optimal process parameters for 316L/5wt%BN coatings were identified: a powder feeding rate of 3–4 rpm, a laser power of 2200–2400 W, a scanning speed of 4–5 mm/s, and an overlapping rate of 40 %. Microstructural analysis showed a smooth surface without cracks or pores. X-ray diffraction revealed intermetallic compounds such as CrB, CrN, FeN, BN, and γ-(Fe, Ni). The inclusion of h-BN nanoparticles enhanced grain refinement, significantly increasing microhardness. Coatings with 5 wt% h-BN achieved an average microhardness of 438.8 HV10, 2.5 times higher than the substrate and the 316L stainless steel. Additionally, h-BN reduced friction coefficients, leading to substantial wear reduction. The 316L/5 wt% h-BN sample experienced only 4.2 mg of wear, 45.16 % of the substrate’s wear. These findings highlight the beneficial effects of h-BN nanoparticles on 316L stainless steel coatings, enhancing wear resistance, hardness, and overall performance.","PeriodicalId":19597,"journal":{"name":"Optics & Laser Technology","volume":"3 1","pages":""},"PeriodicalIF":0.0,"publicationDate":"2024-08-05","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141933933","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Effect of overlap pattern on the residual stress, surface morphology and fatigue properties of Ti-6Al-4V alloy by multiple laser shock peening 重叠模式对多重激光冲击强化 Ti-6Al-4V 合金的残余应力、表面形貌和疲劳性能的影响
Pub Date : 2024-08-05 DOI: 10.1016/j.optlastec.2024.111486
Xuekun Luo, Ziheng Xu, Kai Tian, Yiming Wang, Xin Wang, Kun Wang, Yang Yu, Chang Ye, Ning Dang
In this study, the effects of the laser shock peening (LSP) pattern on the fatigue properties of Ti-6Al-4V alloy were investigated. The residual stress distribution and surface morphology generated by LSP were analyzed using both experiments and numerical simulations. The results show that by optimizing the LSP patterns and overlap ratios, deep compressive residual stresses and beneficial surface morphology can be obtained, resulting in a significant improvement of the four-point bending fatigue performance. Specifically, LSP without optimization improves the fatigue life by a factor of 1.68 when the stress level is 550 MPa and the stress ratio is 0.1, while LSP with optimized parameters improves the fatigue life by a factor of 29.67. It has been demonstrated that the optimization of LSP patterns and overlap ratios plays an important role in enhancing the surface integrity and, thus, the fatigue performance of the Ti-6Al-4V alloy.
本研究探讨了激光冲击强化(LSP)模式对 Ti-6Al-4V 合金疲劳性能的影响。通过实验和数值模拟分析了 LSP 产生的残余应力分布和表面形态。结果表明,通过优化 LSP 模式和重叠率,可以获得深压残余应力和有益的表面形态,从而显著改善四点弯曲疲劳性能。具体来说,当应力水平为 550 兆帕、应力比为 0.1 时,未优化的 LSP 可将疲劳寿命提高 1.68 倍,而优化参数后的 LSP 可将疲劳寿命提高 29.67 倍。结果表明,优化 LSP 模式和重叠率对提高 Ti-6Al-4V 合金的表面完整性和疲劳性能具有重要作用。
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引用次数: 0
Flexible blind quantum computation with unnecessarily universal quantum servers 利用不必要的通用量子服务器实现灵活的盲量子计算
Pub Date : 2024-08-05 DOI: 10.1016/j.optlastec.2024.111548
Xingjia Xie, Qin Li, Xiaoqing Tan, Limin Gao, Yan Hong
Blind quantum computation (BQC) allows clients with limited quantum capabilities to delegate their tasks to powerful quantum servers and still keep their inputs, algorithms, and outputs private. However, in the noisy intermediate-scale quantum (NISQ) era, quantum computers as servers only control limited number of qubits and are not powerful enough. In addition, each of current BQC models is usually suitable for only one type of users. Therefore, this paper offers a flexible BQC ( for short) model for two types of users with different quantum capabilities where any one of two types of users can complete BQC tasks with the help of the other type of users and quantum servers. To be more specific, we propose two protocols by using the given model. In the first protocol, one user Alice only with the ability to prepare single-qubit states can realize BQC tasks by cooperating with another user Bob who is just capable of performing single-qubit measurements and a quantum server Charlie. Similarly in the second one, Bob can realize BQC tasks by cooperating with Alice and Charlie. In both protocols, the server Charlie only requires a quantum register of small size and performing CZ gates and thus it is unnecessary to be universal and may be less difficult to realize in the short run. Furthermore, both proposed protocols are verifiable, namely that the user can detect whether the server is honest. Finally, examples of the proposed protocols for implementing Deutsch’s algorithms are simulated through Qiskit framework to show their feasibility and correctness.
盲量子计算(BQC)允许量子能力有限的客户将其任务委托给强大的量子服务器,并仍然保持其输入、算法和输出的私密性。然而,在噪声中量子(NISQ)时代,作为服务器的量子计算机只能控制有限数量的量子比特,功能不够强大。此外,目前的每种 BQC 模型通常只适用于一类用户。因此,本文为具有不同量子能力的两类用户提供了一种灵活的 BQC(简称)模型,两类用户中的任何一类都可以在另一类用户和量子服务器的帮助下完成 BQC 任务。更具体地说,我们利用给定的模型提出了两个协议。在第一种协议中,一个只有单量子比特态准备能力的用户 Alice 可以通过与另一个只有单量子比特测量能力的用户 Bob 和一个量子服务器 Charlie 合作来实现 BQC 任务。同样,在第二种协议中,鲍勃可以通过与爱丽丝和查理合作实现 BQC 任务。在这两个协议中,服务器查理只需要一个小尺寸的量子寄存器和执行 CZ 门,因此不需要通用性,在短期内实现的难度也较低。此外,这两个协议都是可验证的,即用户可以检测服务器是否诚实。最后,我们通过 Qiskit 框架模拟了实现 Deutsch 算法的拟议协议示例,以展示其可行性和正确性。
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引用次数: 0
Rapid surface patterning to strengthen adhesive bonding of carbon fiber reinforced polymer by spatial shaping femtosecond laser 利用空间塑形飞秒激光快速制作表面图案,加强碳纤维增强聚合物的粘合力
Pub Date : 2024-08-05 DOI: 10.1016/j.optlastec.2024.111562
Yanping Yuan, Xiaoran Guo, Huiyu He, Kaihu Zhang, Weina Han
Carbon fiber reinforced polymer (CFRP) have become gradually important in the aerospace industry due to their outstanding strength-to-weight ratio. However, traditional mechanical surface treatment methods are challenging to apply to CFRP because of their anisotropic and nonhomogeneous properties. Femtosecond laser offers unique advantages for surface treatment, as it allows processing with very low thermal load due to the extremely short interaction time. This study investigates the effect of different surface structures resulting from surface treatment using a femtosecond laser on adhesive properties of CFRP. The experimental results show that: 1) beam shaping can be realized by using the plano-convex cylindrical mirror, which improves the quality of laser processing and greatly improves processing efficiency. It only takes 20 s to complete the laser processing of a 1 cm*1 cm area, which increases the work efficiency by 49 times. 2) pre-bonding surface treatment significantly enhances the tensile shear strength of the single lap joint, and the shear strength of samples with low spatial frequency LIPSS (LSFL) (14.57 ± 1.58 MPa) is 2.96 times higher than that of the untreated sample (US) (4.92 ± 1.34 MPa). 3) LSFL structure exhibits the best results, because the surface of CFRP with LSFL exhibits a relatively higher surface polarity and surface energy. This study provides an efficient, high-precision, and low-damage surface treatment method for preparing CFRP for adhesive bonding, which may promote the application of femtosecond laser technology in difficult-to-process composite materials and provide new methods and technical support for its application in aerospace, vehicle manufacturing, and other fields.
碳纤维增强聚合物(CFRP)因其出色的强度重量比,已逐渐成为航空航天工业的重要材料。然而,由于碳纤维增强聚合物的各向异性和非均质特性,传统的机械表面处理方法很难应用于碳纤维增强聚合物。飞秒激光在表面处理方面具有独特的优势,因为它的作用时间极短,可以在极低的热负荷下进行处理。本研究探讨了使用飞秒激光进行表面处理所产生的不同表面结构对 CFRP 粘合性能的影响。实验结果表明1) 使用平凸圆柱镜可以实现光束整形,从而提高激光加工质量,大大提高加工效率。完成 1 cm*1 cm 面积的激光加工仅需 20 秒,工作效率提高了 49 倍。2) 预粘接表面处理显著提高了单搭接接头的拉伸剪切强度,低空间频率 LIPSS(LSFL)样品的剪切强度(14.57 ± 1.58 MPa)是未处理样品(US)(4.92 ± 1.34 MPa)的 2.96 倍。3) LSFL 结构的效果最好,因为带有 LSFL 的 CFRP 表面具有相对较高的表面极性和表面能。本研究为 CFRP 的粘接制备提供了一种高效、高精度、低损伤的表面处理方法,可促进飞秒激光技术在难加工复合材料中的应用,为其在航空航天、车辆制造等领域的应用提供新的方法和技术支持。
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引用次数: 0
Laser irradiation-induced surface-enhanced Raman scattering of Sn@SnO composite films 激光辐照诱导的 Sn@SnO 复合薄膜表面增强拉曼散射
Pub Date : 2024-08-05 DOI: 10.1016/j.optlastec.2024.111560
Xingxing Du, Jiawei Wang, Ruijin Hong, Chunxian Tao, Qi Wang, Hui Lin, Zhaoxia Han, Dawei Zhang
In this work, Sn@SnO composite films were obtained by Nd:YAG fiber pulsed laser ablation at room temperature. The effects of laser ablation on the microstructure, optical properties, and Raman scattering properties of the films were investigated. Tunable Localized Surface Plasmon resonance(LSPR)of Sn nanoparticles was realized in the wavelength range of 380–450 nm by varying the scanning rate to modulate the degree of oxidation of Sn nanoparticles. Surface enhanced Raman scattering (SERS) was also observed in the composite structure, which was demonstrated excellent stability and SERS sensitivity with the detectable concentration of methylene blue (MB) as low as 10 M and an enhancement factor of 1.75 × 10 as well as a good uniformity. Finally, the electric field distribution of the samples before and after the laser treatment is simulated by the finite difference in time domain (FDTD) method, and the results are consistent with those of experimental ones.
本研究采用 Nd:YAG 光纤脉冲激光烧蚀法在室温下获得了 Sn@SnO 复合薄膜。研究了激光烧蚀对薄膜微观结构、光学特性和拉曼散射特性的影响。通过改变扫描速率来调节纳米锡粒子的氧化程度,实现了纳米锡粒子在 380-450 纳米波长范围内的可调局部表面等离子体共振(LSPR)。在复合结构中还观察到了表面增强拉曼散射(SERS),其稳定性和 SERS 灵敏度均表现优异,亚甲基蓝(MB)的可检测浓度低至 10 M,增强因子为 1.75 × 10,且均匀性良好。最后,利用时域有限差分(FDTD)方法模拟了样品在激光处理前后的电场分布,结果与实验结果一致。
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引用次数: 0
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Optics & Laser Technology
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