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Assessing SO2, NO2 and O3 in rural areas of the North West Province 西北省农村地区SO2、NO2和O3的评估
Q3 Environmental Science Pub Date : 2021-06-01 DOI: 10.17159/caj/2021/31/1.9087
Morongoa Morongoa Ngoasheng, J. Beukes, P. V. van Zyl, J. Swartz, Victor Loate, Portia Krisjan, Sandile Mpambani, M. Kulmala, V. Vakkari, L. Laakso
Air quality monitoring has been lacking in the rural and western North West Province. Here ambient sulphur dioxide (SO2), nitrogen dioxide (NO2) and ozone (O3) concentrations, monitored with passive samplers at 10 sites, are presented. Widespread SO2 and NO2 problems weren’t observed. However, regular O3 standard limit exceedances are likely across the province. Increased SO2 and NO2 concentrations in the colder and drier months were evident. Inversion layer trapping of low-level emissions during the colder months and open biomass burning in the drier months increased ground level pollutant concentrations. Wet deposition of SO2 and NO2, and enhanced SO2 conversion to particulate sulphate, result in lower wet season concentrations. O3 concentrations were lower from May to July and higher from August to March. Three phenomena contributed to this. Firstly, shorter daylight hours (less photochemistry) and secondly, lower biogenic volatile organic compound (O3 precursors) concentrations during the colder months. Thirdly, the late winter/early spring open biomass burning peak lead to elevated carbon monoxide (CO) concentration (also an O3 precursor). Spatial patterns indicated higher SO2 concentrations in the west, due mainly to industrial emissions. The NO2 spatial map indicated two areas of higher concentration, i.e. Bapong in the east due mainly to industrial emissions, and Taung with its higher population density. The O3 spatial map was almost the inverse of NO2. The lower O3 and higher NO2 around Taung showed that O3 is titrated there. Additionally, the results indicate that non-point source emissions of NO2 are high enough to results in exceedances of the O3 standard limit. Overlay back trajectory maps showed that sites in the east are more frequently impacted by pollution transported from the Mpumalanga Highveld, Vaal Triangle and the Johannesburg-Pretoria megacity if compared to the west. Conversely, cleaner air masses impact the west more than sites in the east.
西北省西部和农村地区的空气质量一直缺乏监测。本文介绍了在10个地点用被动采样器监测的环境二氧化硫(SO2)、二氧化氮(NO2)和臭氧(O3)浓度。没有观察到广泛的SO2和NO2问题。然而,全省范围内可能出现常规O3标准超标现象。在寒冷和干燥的月份,SO2和NO2浓度明显增加。在较冷的月份,低水平排放的逆温层捕获和在较干燥的月份开放式生物质燃烧增加了地面污染物浓度。SO2和NO2的湿沉积,以及SO2向颗粒硫酸盐的转化增强,导致雨季浓度降低。O3浓度在5月至7月较低,在8月至3月较高。有三种现象促成了这一现象。首先,白天时间更短(光化学更少),其次,在寒冷的月份,生物挥发性有机化合物(O3前体)浓度更低。第三,冬末春初开放的生物质燃烧峰值导致一氧化碳(CO)浓度升高(也是O3的前体)。空间格局表明,主要由于工业排放,西部的二氧化硫浓度较高。NO2空间图显示了两个浓度较高的地区,即东部的巴蓬,主要是由于工业排放,以及人口密度较高的头。O3的空间图几乎与NO2相反。Taung周围较低的O3和较高的NO2表明O3在那里被滴定。此外,结果表明,NO2的非点源排放量高到足以导致O3标准限值的超标。叠加轨迹图显示,与西部相比,东部地区更频繁地受到普马兰加高地、瓦尔三角和约翰内斯堡-比勒陀利亚特大城市污染的影响。相反,较清洁的气团对西部地区的影响大于东部地区。
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引用次数: 1
Commentary: The Ghana Urban Air Quality Project (GHAir): Bridging air pollution data gaps in Ghana 评论:加纳城市空气质量项目(GHAir):弥合加纳空气污染数据差距
Q3 Environmental Science Pub Date : 2021-05-31 DOI: 10.17159/caj/2021/31/1.11172
C. Sewor, Akua A. Obeng, A. Amegah
Air pollution has been recognized as a pressing sustainability concern seeing that it is directly mentioned in two SDG targets: SDG 3.9 (substantial reduction of health impacts from hazardous substances) and SDG 11.6 (reduction of adverse impacts of cities on people) (Rafaj et al., 2018). Air pollution, both ambient and indoor, is known to contribute significantly to the global burden of disease, contributing to a majority of non-communicable disease-related deaths in low to middle-income countries in Africa and Asia (WHO, 2016). In 2018, air pollution was attributed to 28,000 deaths in Ghana (Odonkor and Mahami, 2020).
空气污染已被认为是一个紧迫的可持续性问题,因为可持续发展目标的两个具体目标直接提到了空气污染:可持续发展目标3.9(大幅减少有害物质对健康的影响)和可持续发展目标11.6(减少城市对人们的不利影响)(Rafaj等人,2018年)。众所周知,环境和室内空气污染严重加重了全球疾病负担,导致非洲和亚洲中低收入国家大多数与非传染性疾病相关的死亡(世卫组织,2016年)。2018年,加纳的空气污染导致2.8万人死亡(Odonkor和Mahami, 2020年)。
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引用次数: 7
Commentary: Opportunities for the application of low-cost sensors in epidemiological studies to advance evidence of air pollution impacts on human health 评论:在流行病学研究中应用低成本传感器的机会,以推进空气污染对人类健康影响的证据
Q3 Environmental Science Pub Date : 2021-05-27 DOI: 10.17159/caj/2021/31/1.11219
B. Wernecke, C. Wright
Introduction Every year, air pollution is associated with more than 7 million deaths globally (Forouzanfar et al., 2016). It is one of the top environmental health risks in lowand middle-income countries (LMICs) (Joubert et al., 2020). Ambient and household air pollution (HAP) threaten human health and well-being, particularly for vulnerable groups such as infants and children, women, people with pre-existing diseases and the elderly (Forouzanfar et al., 2016).
引言每年,全球有700多万人死于空气污染(Forouzanfar等人,2016)。它是中低收入国家的首要环境健康风险之一(Joubert等人,2020)。环境和家庭空气污染(HAP)威胁着人类的健康和福祉,尤其是对婴儿和儿童、妇女、已有疾病的人和老年人等弱势群体(Forouzanfar等人,2016)。
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引用次数: 3
Intra-urban variability of PM2.5 in a dense, low-income settlement on the South African Highveld 南非高原区一个密集的低收入定居点PM2.5的城市内变异性
Q3 Environmental Science Pub Date : 2021-04-29 DOI: 10.17159/CAJ/2020/31/1.9413
Simon D. Moletsane, Farina Lindeque, B. Language, N. Nkosi, J. A. Adesina, R. Burger, G. Mkhatshwa, S. Piketh
High concentrations of the ambient particulate matter remains a concern on the South African Highveld, particularly in densely populated low-income settlements. These areas have several local emission sources that contribute to poor air quality and are often located close to industrial and other urban areas. The local sources vary in magnitude, space, and time. In South Africa, little has been done to assess the impacts of spatiotemporal variability on the credibility of using isolated ambient observations for regulatory purposes. This study aims to evaluate the intra-urban variability of ambient PM2.5 concentrations in a dense, low-income community. Ambient fine particulate matter (PM2.5) in distinct microenvironments of KwaZamokuhle were simultaneously measured at 4 sites between March and June 2018. These measurements were collected using one permanent ambient monitoring station (AMS) and a temporary network of three E-BAM monitors (Site 2, Site 3, and Site 4). The daily PM2.5 concentrations at AMS, Site 2, Site 3, and Site 4 varied from 10 to 86 µg.m-3, 10 to 103 µg.m-3, 11 to 101 µg.m-3, and 9 to 113 µg.m-3, respectively. Extreme PM2.5 concentrations which exceeded the 24h PM2.5 NAAQS of 40 µg.m-3 were seen during the cold period (May and June); meanwhile, the warm period (March and April) recorded relatively lower PM2.5 episodes across different sections of KwaZamokuhle. During May-June, the highest diurnal concentrations of hourly averaged ambient PM2.5 were recorded at Site 4, in a downward sequence, followed by Site 3, Site 2, and AMS. Furthermore, the results showed that across KwaZamokuhle, Site 4 has the highest proportion of households using solid fuels for domestic purposes (cooking and heating) (55%) and the number of informal dwellings (117 households). Therefore, the study highlights the complexity of quantifying ambient air quality in an area where several local emission sources vary in space and time. Attempts to use monitoring data from a single station to assess ambient air quality, quantify human exposure, or evaluate the potential impacts of mitigation strategies in dense, low-income settlements should be done with care.
环境微粒物质的高浓度仍然是南非高原的一个令人关切的问题,特别是在人口密集的低收入住区。这些地区有几个地方排放源,造成空气质量差,而且往往靠近工业区和其他城市地区。局部震源在大小、空间和时间上各不相同。在南非,几乎没有评估时空变异性对将孤立的环境观测用于监管目的的可信度的影响。本研究旨在评估一个人口密集的低收入社区环境PM2.5浓度的城市内变异性。2018年3月至6月,对夸扎木喀勒不同微环境中4个站点的环境细颗粒物(PM2.5)进行了同步测量。这些测量数据是通过一个永久性环境监测站(AMS)和一个由三个E-BAM监测站(Site 2、Site 3和Site 4)组成的临时网络收集的。AMS、Site 2、Site 3和Site 4的PM2.5日浓度在10至86微克之间变化。M-3, 10 ~ 103µg。M-3, 11 ~ 101µg。M-3, 9至113µg。分别m3。极端PM2.5浓度超过24小时PM2.5 NAAQS 40µg。冬季(5、6月)出现m-3;与此同时,温暖期(3月和4月)夸扎木勒不同地区的PM2.5浓度相对较低。5 - 6月,站点4的逐时平均PM2.5日浓度最高,依次为站点3、站点2和AMS。此外,结果显示,在整个KwaZamokuhle, Site 4使用固体燃料用于家庭目的(烹饪和取暖)的家庭比例最高(55%),非正式住宅数量最多(117户)。因此,该研究强调了在几个局部排放源在空间和时间上变化的地区量化环境空气质量的复杂性。在试图利用单一站点的监测数据评估环境空气质量、量化人类暴露或评估密集低收入住区缓解战略的潜在影响时,应谨慎行事。
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引用次数: 5
Ambient air quality data reported at Sasol Secunda monitoring stations during COVID-19 lockdown – Mpumalanga, South Africa 新冠肺炎封锁期间Sasol Secunda监测站报告的环境空气质量数据——南非普马兰加
Q3 Environmental Science Pub Date : 2021-03-23 DOI: 10.17159/CAJ/2021/31/1.8954
A. Venter, S. D. Vos
Various local and international research has been published on the effects of COVID-19 lockdown on ambient air quality. In most cases, a reduction in ambient NOx and PM concentrations have been observed with varying changes in ambient SO2 levels. Secunda, located in the Highveld Priority Area in Mpumalanga, South Africa is known for its large industrial facilities utilising coal as primary feedstock. The towns of Secunda and eMbalenhle provide the majority of the workforce to Sasol and has therefore been the focus of this study. The ambient air quality in the Secunda region was assessed due to the changes in human behaviour during lockdown, familiarity with the Sasol facility and the strategic locations of ambient air quality stations.Results show a clear decrease in ambient CO, NO2 and PM concentrations, especially during the first two weeks of lockdown. Only subtle changes were observed for ambient H2S and SO2 pollutant concentrations at the ambient monitoring stations. An increasing trend in all ambient species was observed towards the end and post lockdown, in contrast to declining ambient temperatures with the onset of winter. This is also contrary to the reduction in emissions from the factory that conducted annual maintenance in the month following lockdown (phase shutdown). This article concludes that human behaviour has a material local ambient impact on CO, NO2 and PM pollutant species, while H2S concentration profiles are more directly related to the industrial complex’s levels of activity. Ambient SO2 trends did not show a similar correlation with the facility’s activities (as H2S), but a stronger correlation was observed with the diverse local and regional sources in close proximity to Secunda and eMbalenhle. The influence of better dispersion especially on a local scale, brought about by more effective emission heights, is considered material. Moreover, meteorological factors, on local air quality, has been shown to be a material contributor to observed ambient air quality levels in the study domain
关于新冠肺炎封锁对环境空气质量的影响,国内外发表了多项研究。在大多数情况下,随着环境二氧化硫水平的不同变化,已观察到环境氮氧化物和PM浓度的减少。Secunda位于南非普马兰加省的高原区,以其以煤为主要原料的大型工业设施而闻名。塞孔达镇和恩巴伦勒镇为沙索尔提供了大部分劳动力,因此是本研究的重点。由于封锁期间人类行为的变化、对沙索尔设施的熟悉以及环境空气质量监测站的战略位置,对塞孔达地区的环境空气质量进行了评估。结果显示,环境CO、NO2和PM浓度明显下降,尤其是在封城的前两周。环境监测站的环境H2S和SO2污染物浓度变化不大。在封城结束和封城结束后,所有环境物种的温度都呈上升趋势,而随着冬季的到来,环境温度则呈下降趋势。这也与在封锁(阶段性停工)后一个月进行年度维护的工厂的排放量减少背道而驰。本文的结论是,人类行为对CO、NO2和PM污染物种类有重大的局部环境影响,而H2S浓度曲线与工业园区的活动水平更直接相关。环境SO2趋势与设施活动(如H2S)没有类似的相关性,但与Secunda和eMbalenhle附近的各种本地和区域来源有更强的相关性。更有效的发射高度所带来的更好的色散特别是在局部尺度上的影响被认为是物质的。此外,关于当地空气质量的气象因素已被证明是研究领域观测到的环境空气质量水平的一个重要因素
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引用次数: 2
Modeling tropospheric ozone and particulate matter in Tunis, Tunisia using generalized additive model 突尼斯使用广义加性模式模拟对流层臭氧和颗粒物
Q3 Environmental Science Pub Date : 2021-01-01 DOI: 10.17159/caj/2021/31/2.8880
Zouhour Hammouda, Leila Hedhili Zaier, N. Blond
The main purpose of this paper is to analyze the sensitivity of tropospheric ozone and particulate matter concentrations to changes in local scale meteorology with the aid of meteorological variables (wind speed, wind direction, relative humidity, solar radiation and temperature) and intensity of traffic using hourly concentration of NOX, which are measured in three different locations in Tunis, (i.e. Gazela, Mannouba and Bab Aliwa). In order to quantify the impact of meteorological conditions and precursor concentrations on air pollution, a general model was developed where the logarithm of the hourly concentrations of O3 and PM10 were modeled as a sum of non-linear functions using the framework of Generalized Additive Models (GAMs). Partial effects of each predictor are presented. We obtain a good fit with R² = 85% for the response variable O3 at Bab Aliwa station. Results show the aggregate impact of meteorological variables in the models explained 29% of the variance in PM10 and 41% in O3. This indicates that local meteorological condition is an active driver of air quality in Tunis. The time variables (hour of the day, day of the week and month) also have an effect. This is especially true for the time variable “month” that contributes significantly to the description of the study area.
本文的主要目的是利用突尼斯Gazela、Mannouba和Bab Aliwa三个不同地点(即Gazela、Mannouba和Bab Aliwa)的逐时NOX浓度,借助气象变量(风速、风向、相对湿度、太阳辐射和温度)和交通强度,分析对流层臭氧和颗粒物浓度对当地气象变化的敏感性。为了量化气象条件和前体浓度对空气污染的影响,开发了一个通用模型,其中使用广义可加模型(GAMs)框架将每小时O3和PM10浓度的对数建模为非线性函数的总和。给出了每个预测器的部分效应。我们对Bab Aliwa站的响应变量O3进行了R²= 85%的拟合。结果表明,各模式中气象变量的综合影响解释了PM10和O3变化的29%和41%。这表明当地的气象条件是突尼斯空气质量的一个积极驱动因素。时间变量(一天中的几小时、一周中的几号和一个月中的几号)也有影响。对于对研究区域的描述有重要贡献的时间变量“月”来说尤其如此。
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引用次数: 1
Quantifying potential particulate matter intake dose in a low-income community in South Africa 量化南非一个低收入社区的潜在颗粒物摄入剂量
Q3 Environmental Science Pub Date : 2021-01-01 DOI: 10.17159/caj/2021/31/2.9426
B. Wernecke, R. Burger, B. Language, C. Wright, S. Piketh
Understanding how exposure to particulate matter impacts human health is complex. Personal exposure is a function of the pollution concentrations measured at any given place and time. The health impacts of this exposure are, amongst other factors, determined by how high pollutant concentrations are and what enters the body. This study considered data gathered in the winter of 2013 in a low-income community on the Mpumalanga Highveld, South Africa, which is a geographical area known for its high air pollution levels. Time-activity data collected by GPS monitors worn by individuals in the community were used to understand in which microenvironments people spend most of their time. Eight days’ worth of ambient, indoor and personal particulate matter measurements were paired with individual GPS positioning data for one study participant. We identified pollutant concentrations where the person spent time and how much particulate matter was potentially inhaled in specific micro-environments. Participants spent time in five main micro-environments: (highest rank first) inside a house, directly outside a house, on a dirt road, on a tar road, and on an open field. Exposure to particulate matter concentrations in these micro-environments exceeded the National Ambient Air Quality Standards. Highest exposure was measured inside the dwelling and directly outside the dwelling. When comparing directly- and indirectly derived time-weighted potential intake doses, directly derived intake doses were higher and more likely to represent particulate matter concentrations inhaled by the participant. This study suggests that people living in communities on the Mpumalanga Highveld are exposed to unacceptably high air pollution levels in places in which they spend most of their time. Direct exposure and intake dose assessments are an essential element of environmental health studies to supplement data collected by stationary monitors.
了解接触颗粒物如何影响人体健康是很复杂的。个人接触是在任何给定地点和时间测量的污染浓度的函数。除其他因素外,这种接触对健康的影响取决于污染物浓度的高低和进入人体的污染物。这项研究考虑了2013年冬天在南非普马兰加高原一个低收入社区收集的数据,这是一个以高空气污染水平而闻名的地理区域。由社区中个人佩戴的GPS监测器收集的时间-活动数据被用来了解人们在哪些微环境中度过了大部分时间。研究人员将一名研究参与者8天的环境、室内和个人颗粒物测量数据与个人GPS定位数据配对。我们确定了这个人待过的地方的污染物浓度,以及在特定的微环境中可能吸入多少颗粒物。参与者在五个主要的微环境中度过时间:(最高排名第一)在房子里,直接在房子外面,在土路上,在柏油路上,在开阔的田野上。暴露在这些微环境中的颗粒物浓度超过了国家环境空气质量标准。在住宅内和直接在住宅外测量最高暴露量。当比较直接和间接得出的时间加权潜在摄入剂量时,直接得出的摄入剂量更高,更可能代表参与者吸入的颗粒物浓度。这项研究表明,生活在普马兰加高原社区的人们在他们大部分时间居住的地方暴露在令人无法接受的高空气污染水平下。直接接触和摄入剂量评估是环境健康研究的一个重要组成部分,以补充固定监测仪收集的数据。
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引用次数: 0
Air Pollution and Its Impacts on Health in Africa - insights from the State of Global Air 2020 空气污染及其对非洲健康的影响——来自2020年全球空气状况的见解
Q3 Environmental Science Pub Date : 2020-12-07 DOI: 10.17159/caj/2020/30/2.9270
Joanna L Keel, Katherine D. Walker, Pallavi Pant
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引用次数: 7
A summary of the paper “Natural archives of long-range transported contamination at the remote lake Letšeng-la Letsie, Maloti Mountains, Lesotho” 论文摘要“莱索托马洛蒂山脉偏远湖泊Letšeng la Letsie的长期运输污染自然档案”
Q3 Environmental Science Pub Date : 2020-12-07 DOI: 10.17159/caj/2020/30/2.9273
N. Rose, A. Milner, J. Fitchett, Kristy E. Langerman, Handong Yang, S. Turner, A. Jourdan, James Shilland, C. Martins, A. C. Souza, C. Curtis
Lake sediments and wetland peats provide valuable archives of changes in anthropogenic inputs into natural ecosystems. Sediments of remote mountain lakes are particularly useful because contaminants in these settings are solely derived from atmospheric deposition. This study presents the first historical record of contamination for Lesotho, a hydrologically important region in southern Africa, exporting about 35% of the water used in the Gauteng/Mpumalanga urban-industrial complex in South Africa.
湖泊沉积物和湿地泥炭提供了人类对自然生态系统投入变化的宝贵档案。偏远山区湖泊的沉积物特别有用,因为这些环境中的污染物完全来自大气沉积。这项研究首次展示了莱索托污染的历史记录,莱索托是非洲南部一个重要的水文地区,南非豪登省/普马兰加省城市-工业综合体用水的35%用于出口。
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引用次数: 0
Low-cost sensors, an interesting alternative for air quality monitoring in Africa. 低成本传感器,是非洲空气质量监测的一种有趣的替代方案。
Q3 Environmental Science Pub Date : 2020-12-07 DOI: 10.17159/caj/2020/30/2.9223
F. Rahal
In Algeria, the lack of continuous measurement of air pollution is a real problem that hinders studies, strategies and decisionmaking to fight against this phenomenon. Indeed, the pollution measurement networks installed by the public authorities in the main urban centers of the country (Rahal et al., 2014) are no longer operational. This situation in Algeria is just one example among many in developing countries where the monitoring of air quality is in a deplorable state (Kumar et al., 2019), because this monitoring is a costly policy, which requires sufficient and sustainable financial means. Furthermore, the technical skills to maintain and operate the instrumentation of measuring equipment are scarce.
在阿尔及利亚,缺乏对空气污染的持续测量是一个真正的问题,阻碍了对抗这一现象的研究、战略和决策。事实上,公共当局在该国主要城市中心安装的污染测量网络(Rahal等人,2014)已不再运行。阿尔及利亚的这种情况只是发展中国家空气质量监测状况不佳的一个例子(Kumar et al.,2019),因为这种监测是一项代价高昂的政策,需要足够和可持续的财政手段。此外,维护和操作测量设备仪器的技术技能也很匮乏。
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引用次数: 1
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Clean Air Journal
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