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Possibility of Discovering the Super-Heavy Elements Z=119 and 120 发现超重元素 Z=119 和 120 的可能性
IF 1.6 4区 物理与天体物理 Q2 PHYSICS, MULTIDISCIPLINARY Pub Date : 2024-08-29 DOI: 10.1007/s13538-024-01551-6
H. C. Manjunatha, N. Sowmya, P. S. Damodara Gupta, N. Manjunatha, T. Nandi

We reveal that inclusion of fission barrier, nuclear level densities, neutron and fission decay widths in a better way in the advanced statistical method and dinuclear system model can lead to reproduce well the measured production cross sections of the cold and hot fusion reactions in the range (Z=102-118). In addition, we show that the optimal beam energies, where the production cross section reaches its maximum, can also be effectively determined using quasielastic barrier distribution curves. This theoretical approach helps us to verify the cause of low production cross section measured for the super-heavy element (SHE) (^{278})Nh with the reaction (^{70})Zn + (^{209})Bi and null results from the reaction (^{86})Kr+(^{208})Pb used for synthesizing the SHE Z=118. Furthermore, the same has been employed to explore the reason for the failure of many trials in synthesizing the SHEs for (Z=119) and 120. ER cross sections at the optimal energies for a few heavy-ion reactions in synthesizing the SHE (Z=119) and 120 are seen to be measurable. Thus, the synthesis of the SHEs for (Z=)119 and 120 is on the cards.

我们发现,将裂变势垒、核级密度、中子和裂变衰变宽度以更好的方式纳入先进的统计方法和二核系统模型,可以很好地再现在 (Z=102-118) 范围内测量到的冷核聚变和热核聚变反应的产生截面。此外,我们还表明,利用准弹性势垒分布曲线也可以有效地确定产生截面达到最大值的最佳束流能量。这种理论方法帮助我们验证了通过反应 (^{70})Zn + (^{209})Bi 测得的超重元素(SHE)(^{278})Nh 的生产截面较低的原因,以及用于合成 SHE Z=118 的反应 (^{86})Kr+(^{208})Pb 的无效结果。此外,同样的方法也被用来探索在合成 Z=119 和 120 的 SHE 时多次试验失败的原因。在合成 SHE (Z=119)和 120 的过程中,可以看到一些重离子反应在最佳能量下的 ER 截面是可以测量的。因此,合成 (Z=)119 和 120 的 SHE 是有可能的。
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引用次数: 0
Anisotropic Fractional Brownian Field Synthesis via Curvelet Transform 通过曲线小波变换合成各向异性的分数布朗场
IF 1.6 4区 物理与天体物理 Q2 PHYSICS, MULTIDISCIPLINARY Pub Date : 2024-08-29 DOI: 10.1007/s13538-024-01580-1
M. V. C. Henriques, F. E. A. Leite

The proposed model employs curvelet-based techniques to generate anisotropic Fractional Brownian Fields, simulating systems with orientation-dependent self-similar properties. Curvelets are a mathematical tool that allows for an efficient representation of data with edges and other anisotropic singularities, being essential for capturing the directional complexity in the self-similar properties of the modeled systems. The synthesis procedure involves generating coefficients in curvelet space with a zero-mean Gaussian distribution. This approach is tailored to depict the stochastic behavior of natural systems, particularly in scenarios where angular distributions of correlations are critical. The main contribution of this paper is presenting a novel method for generating 2-D anisotropic Fractional Brownian Fields (AFBFs) using the Curvelet Transform, demonstrating the Curvelet Transform’s efficiency in modeling anisotropic properties. Potential applications include modeling heterogeneous geological structures, anisotropic materials, and complex disordered media.

所提出的模型采用了基于小曲线的技术来生成各向异性的分数布朗场,模拟具有方向依赖性自相似特性的系统。小曲线是一种数学工具,可以有效地表示具有边缘和其他各向异性奇异点的数据,对于捕捉模型系统自相似特性中的方向复杂性至关重要。合成过程包括在曲线空间生成零均值高斯分布的系数。这种方法专门用于描述自然系统的随机行为,尤其是在相关性的角度分布至关重要的情况下。本文的主要贡献在于提出了一种利用曲线小波变换生成二维各向异性分数布朗场(AFBF)的新方法,展示了曲线小波变换在模拟各向异性特性方面的效率。其潜在应用包括异质地质结构、各向异性材料和复杂无序介质建模。
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引用次数: 0
An Investigation on Structural, Optical, Thermal, and Dielectric Analysis of L-Lysine Iodide Semiorganic Nonlinear Optical Single Crystal for Opto-electronic Application 用于光电应用的 L-赖氨酸碘化物半有机非线性光学单晶的结构、光学、热学和介电分析研究
IF 1.6 4区 物理与天体物理 Q2 PHYSICS, MULTIDISCIPLINARY Pub Date : 2024-08-28 DOI: 10.1007/s13538-024-01588-7
P. Revathi, T. Balakrishnan, J. Thirupathy

A single crystal of L-lysine iodide (LLI) was created by utilizing a room-temperature slow evaporation approach. The monoclinic of the crystal lattice system was confirmed by estimating the lattice parameters of the synthesized single crystals using single crystal X-ray diffraction analysis. The crystalline structure and planar indexing were confirmed by powder XRD. In order to confirm that the produced LLI crystals included functional groups, the FT-IR spectra were analyzed. Spectra of visible, near-infrared, and ultraviolet light (ranging from 200 to 1100 nm) were analyzed and the cutoff wavelength of 268 nm. Vickers microhardness tester was used to find out how strong the formed crystal was mechanically stable. From 50 Hz to 3 MHz, the dielectric response of the manufactured crystal was studied at different temperatures. Thermogravimetric analysis used to look at the thermal characteristics. Human pathogens were the primary focus of antimicrobial research. Using scanning electron microscopy (SEM), the surface characteristics of the generated crystal were examined. The produced LLI crystal was recommended for use in opto-electronic and biological applications.

通过室温慢速蒸发方法制备出了 L-赖氨酸碘化物(LLI)单晶体。通过使用单晶 X 射线衍射分析估算合成单晶的晶格参数,确认了该晶体的单斜晶格体系。粉末 XRD 证实了晶体结构和平面分度。为了确认所制得的 LLI 晶体包含官能团,对其进行了傅立叶变换红外光谱分析。分析了可见光、近红外线和紫外线(波长范围从 200 纳米到 1100 纳米)的光谱,截止波长为 268 纳米。使用维氏硬度计来测定所形成晶体的机械稳定性。从 50 Hz 到 3 MHz,在不同温度下研究了所制造晶体的介电响应。热重分析用于研究热特性。人类病原体是抗菌研究的主要重点。使用扫描电子显微镜(SEM)检查了生成晶体的表面特征。建议将生成的 LLI 晶体用于光电子和生物应用领域。
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引用次数: 0
Giant Dielectric Permittivity and Electronic Structure in Hydrogenated (La/Mn) Merge Codoped TiO2 Ceramics 氢化(La/Mn)并合掺杂二氧化钛陶瓷中的巨介电常数和电子结构
IF 1.6 4区 物理与天体物理 Q2 PHYSICS, MULTIDISCIPLINARY Pub Date : 2024-08-27 DOI: 10.1007/s13538-024-01582-z
A. A. Dakhel

Titanium oxide (TiO2) nanoparticles (NPs) codoped with (La/Mn) ions were synthesized by a hydrothermal decomposition technique. The prepared codoped NPs were hydrogenated at 400 °C and systematically studied by X‐ray diffraction (XRD), optical diffuse reflection spectroscopy (DRS), and electrical insulating measurements. The codoped solid solution (SS) NPs were prepared to be built of core/shell-like electronic nanostructures that having giant permittivity (GP) of order 104, which is extremely higher than that of undoped TiO2. The electronic nature of the built structures was described according to the foundation of the doping mechanisms. Thus, the codoping was employed in the present work to fabricate coalesce dielectric crystalline medium of GP. Two Mn-dopant concentrations were used in the present investigation for comparison. Thus, the objective of creation of GP properties was successfully achieved. Moreover, the results of the electrical measurements were analyzed according to the available models: the correlated barrier hopping (CBH) model, the polarons-hopping conduction model, and Jonsher’s AC power law.

通过水热分解技术合成了掺杂(La/Mn)离子的氧化钛(TiO2)纳米粒子(NPs)。制备的掺杂 NPs 在 400 °C 下氢化,并通过 X 射线衍射 (XRD)、光学漫反射光谱 (DRS) 和电绝缘测量进行了系统研究。制备出的掺杂固溶体(SS)纳米粒子由核/壳状电子纳米结构组成,其巨导率(GP)为 104,远高于未掺杂的二氧化钛。根据掺杂机制的基础,对所构建结构的电子性质进行了描述。因此,本研究采用了共掺杂的方法来制造具有 GP 的凝聚介电晶体介质。本研究中使用了两种锰掺杂浓度进行比较。因此,成功实现了创造 GP 特性的目标。此外,电学测量结果根据现有模型进行了分析:相关势垒跳变(CBH)模型、极子跳变传导模型和 Jonsher 交流幂律。
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引用次数: 0
An Emerging Strategy in Sequential Synthesis of Catalyst and Carbon Nanotube Foams by Employing a Chemical Vapor Deposition Procedure: Structural Evaluation and Growth Mechanism 采用化学气相沉积程序依次合成催化剂和碳纳米管泡沫的新策略:结构评估与生长机理
IF 1.6 4区 物理与天体物理 Q2 PHYSICS, MULTIDISCIPLINARY Pub Date : 2024-08-27 DOI: 10.1007/s13538-024-01583-y
J. Logeswari, T. Kamatchi, P. Kumaresan

In an effort to further expand the simplification of the bulk production of carbon nanotube (CNT) foams, herein, a new approach based on one-step synthesis procedure is developed, where the production of the catalyst is followed by CNT foam growth in a chemical vapor deposition (CVD) furnace during acetylene decomposition over three various mole ratios of Fe: Mo: MgO: PEG (polyethylene glycol) sol-gel viscous precursor catalyst (viz., 1: 0.5: 13: 4.8, 1: 1: 13: 5, and 1: 1: 50: 17.3) under Ar/H2 atmosphere at various reaction conditions. The growth of multi-walled CNT foams was directly carried out, i.e., without preceding any reduction and oxidation phases over viscous gels. The various parameters such as molar ratio, reaction temperature, and acetylene flow rate were optimized individually for the production of ultra-lightweight foamed CNTs. The CNT foams grown from the optimized reaction conditions were discussed by using various physicochemical characterization studies, such as XRD, FT-Raman, SEM, TEM, FE-SEM with EDX, N2 sorption isotherms, and thermal analysis. The issues regarding the growth mechanism of high specific surface area CNT foams are taken in the present approach. Such a mechanism has been proposed for the carbo-thermal reduction of acetylene over the optimized viscous catalyst precursors gel at 800 °C in a CVD furnace.

为了进一步简化碳纳米管(CNT)泡沫的批量生产,本文开发了一种基于一步合成程序的新方法,即在乙炔分解过程中,在三种不同摩尔比的铁:钼:氧化镁的化学气相沉积(CVD)炉中,先生产催化剂,然后生长 CNT 泡沫:PEG(聚乙二醇)溶胶凝胶粘性前驱体催化剂(即 1:0.5:13:4.8、1:1:13:5 和 1:1:50:17.3),在 Ar/H2 气氛下,在不同的反应条件下进行乙炔分解。多壁碳纳米管泡沫的生长是直接进行的,即在粘性凝胶上不经过任何还原和氧化阶段。对摩尔比、反应温度和乙炔流速等各种参数进行了单独优化,以生产超轻泡沫 CNT。通过各种物理化学表征研究,如 XRD、FT-Raman、SEM、TEM、带 EDX 的 FE-SEM、N2 吸附等温线和热分析,讨论了在优化反应条件下生长的 CNT 泡沫。本研究还探讨了高比表面积 CNT 泡沫的生长机制问题。在 800 °C 的 CVD 炉中,经过优化的粘性催化剂前驱体凝胶对乙炔进行羧基热还原时,提出了这种机制。
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引用次数: 0
Quantum Field Theoretical Study of Correlated Quantum Ising Model with Next-Nearest-Neighbour Interaction 具有近邻相互作用的相关量子伊辛模型的量子场理论研究
IF 1.6 4区 物理与天体物理 Q2 PHYSICS, MULTIDISCIPLINARY Pub Date : 2024-08-23 DOI: 10.1007/s13538-024-01584-x
Ranjith R. Kumar, Sujit Sarkar

We present the results of quantum Ising and longer range quantum Ising model for strongly correlated emergent Hamiltonian. We show explicitly that the ordered ferromagnetic (FM) phase to the disorder quantum paramagnet (dqpI) quantum phase transition occurs only in the strongly correlated regime for the quantum Ising model otherwise only dqpI phase appears for a non-interacting and attractive regime. We show that short-range FM coupling and longer range coupling are competing with each other and also the effect of strong correlation in this competition. We also show the most interesting feature that the transverse field opposes the FM coupling of quantum Ising model but it favours the longer range coupling. We find the evidence of another disorder quantum paramagnetic (dqpII) phase due to the relevance of longer-range coupling. We also present the existence of another quantum phase the transition from dqpII phase to the FM phase. We also observe three different kinds of coexistence phases depending on the correlated regime. The fixed point analysis of the three sets of RG equations is carried out.

我们介绍了强相关新兴哈密顿的量子伊辛模型和长程量子伊辛模型的研究结果。我们明确显示,量子伊辛模型的有序铁磁(FM)相到无序量子准磁体(dqpI)的量子相变只发生在强相关体系中,否则在非相互作用和吸引力体系中只会出现 dqpI 相。我们展示了短程调频耦合和长程耦合之间的竞争,以及强相关性在这种竞争中的影响。我们还显示了一个最有趣的特征,即横向场与量子伊辛模型的调频耦合相反,但却有利于长程耦合。由于长程耦合的相关性,我们发现了另一种无序量子顺磁(dqpII)相的证据。我们还发现了从 dqpII 相过渡到调频相的另一种量子相。我们还观察到三种不同的共存相,这取决于相关制度。我们对三组 RG 方程进行了定点分析。
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引用次数: 0
The One-Dimensional Gyroidal Superconductor Photonic Crystals Based Cutoff Frequency Tunability for THz Applications 太赫兹应用中基于截止频率可调性的一维陀螺超导体光子晶体
IF 1.6 4区 物理与天体物理 Q2 PHYSICS, MULTIDISCIPLINARY Pub Date : 2024-08-22 DOI: 10.1007/s13538-024-01577-w
Ahmed Mehaney, Ahmed M. El-Sherbeeny, Arafa H. Aly, Chittaranjan Nayak, Bhuvneshwer Suthar, Wail Al Zoubi, Mostafa R. Abukhadra, Hussein A. Elsayed

For possible uses in the THz frequency range, we investigated the one-dimensional gyroidal superconductor photonic crystals in the current work. In this regard, each unit cell is designed from gyroidal Bi2Sr2CaCu2O8 (BSCCO) and SrTiO3 layers. Here, BSCCO is embedded in a hosting dielectric medium of SrTiO3 to design the gyroidal layer. The transfer matrix approach and the two-fluid model are both used in the computational analysis of the suggested structure. Studying the optical properties and investigating how several factors, including filling fraction, operating temperature, and layer thicknesses, affect the PC's performance. The results showed the emergence of the cutoff frequency at 5.35 THz. In this regard, the value of the cutoff frequency can be tuned based on the filling fraction, operating temperature, and refractive index of the hosting medium, making the structure promising for optical communication applications.

为了在太赫兹频率范围内实现可能的应用,我们在目前的工作中研究了一维陀螺超导体光子晶体。在这方面,每个单元格都是由陀螺状的 Bi2Sr2CaCu2O8(BSCCO)层和 SrTiO3 层设计而成。在这里,BSCCO 被嵌入到 SrTiO3 的宿主介质中以设计陀螺层。在对建议结构进行计算分析时,采用了传递矩阵方法和双流体模型。研究光学特性,并探讨填充分数、工作温度和层厚度等因素如何影响 PC 的性能。结果显示,截止频率出现在 5.35 THz。因此,截止频率值可根据填充分数、工作温度和寄存介质的折射率进行调整,从而使该结构在光通信应用中大有可为。
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引用次数: 0
Decoherence Channels Effects on Thermal Quantum Correlations Within a Two-Dimensional Graphene System 退相干通道对二维石墨烯系统内热量子相关性的影响
IF 1.6 4区 物理与天体物理 Q2 PHYSICS, MULTIDISCIPLINARY Pub Date : 2024-08-22 DOI: 10.1007/s13538-024-01585-w
Zakaria Bouafia, Mourad Benzahra, Mostafa Mansour

Two-dimensional graphene systems present considerable advantages for quantum information processing. Electrons within graphene possess not just spin but also additional attributes associated with their specific positions within the lattice and valley index. This study investigates how decoherence channels impact thermal quantum correlations within individual electrons in a two-dimensional graphene system, considering the electron pseudospin and valley index degrees of freedom. Using quantum metrics such as uncertainty-induced non-locality (UIN) and local quantum Fisher information (LQFI), this research evaluates skew-information and non-classical correlations among these extra degrees of freedom of electrons within the graphene system. The dynamics of the intra-particle quantum correlations in graphene’s thermal state is analyzed with respect to factors such as scattering strength, the band structure of graphene, and wavenumber operators. The findings suggest that adjusting the parameters of the graphene system holds promise for enhancing LQFI and UIN, thereby mitigating the adverse effects of increasing equilibrium temperature. Moreover, the study examines how intra-particle thermal quantum correlations evolve under various decoherence channels, including phase damping (PD), phase flip (PF), and amplitude damping (AD). It is observed that under AD and PD channels, both metrics display similar evolution, diminishing as the decoherence parameter increases, with LQFI demonstrating greater resilience compared to UIN. However, distinct behavior is observed when graphene’s thermal state undergoes the PF channel, where both metrics display symmetrical behaviors around the decoherence parameter of (p=0.5).

二维石墨烯系统在量子信息处理方面具有相当大的优势。石墨烯中的电子不仅具有自旋,还具有与其在晶格中的特定位置和谷指数相关的附加属性。考虑到电子的伪自旋和谷指数自由度,本研究探讨了退相干通道如何影响二维石墨烯系统中单个电子内部的热量子相关性。这项研究利用不确定性诱导的非位置性(UIN)和局部量子费雪信息(LQFI)等量子度量,评估了石墨烯系统内电子的这些额外自由度之间的偏斜信息和非经典相关性。研究分析了石墨烯热状态下粒子内量子相关性的动态变化与散射强度、石墨烯的带状结构和波长算子等因素的关系。研究结果表明,调整石墨烯系统的参数有望增强 LQFI 和 UIN,从而减轻平衡温度升高带来的不利影响。此外,研究还考察了粒子内热量子相关性在各种退相干通道下的演变过程,包括相位阻尼(PD)、相位翻转(PF)和振幅阻尼(AD)。研究发现,在 AD 和 PD 信道下,两个指标都显示出相似的演化,随着退相干参数的增加而减弱,与 UIN 相比,LQFI 显示出更强的恢复能力。然而,当石墨烯的热状态经历 PF 通道时,观察到了截然不同的行为,两个指标在去相干参数 (p=0.5)附近显示出对称的行为。
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引用次数: 0
Investigation of Hot Press and Cold Press Effects on Structural, Electrical and Magnetic Properties of Pyrene Added Bulk MgB2 研究热压和冷压对添加了芘的块状 MgB2 的结构、电学和磁学特性的影响
IF 1.6 4区 物理与天体物理 Q2 PHYSICS, MULTIDISCIPLINARY Pub Date : 2024-08-21 DOI: 10.1007/s13538-024-01586-9
O. Erdem

In this paper, the effects of hot pressing and cold pressing on the superconducting properties of pyrene (C16H10) added bulk MgB2 were compared. For this aim, the polycrystalline disk-shaped MgB2 samples with addition of 4 wt % C16H10 powder were fabricated by a pellet/closed tube method at 850 °C, after hot pressing at 200 °C and cold pressing. The XRD and SEM results showed that although a-lattice parameters reduce for both C16H10 added samples, the average crystallite size increases after cold pressing because of the accumulation and inhomogeneous distribution of C in the MgB2 structure while it reduces for the C16H10 added hot pressed sample. The resistivity measurements showed that the increment of electron scattering is higher for the C16H10 added cold pressed sample than that of the C16H10 added hot pressed one which shows relatively better grain connectivity, and the Tc values of the samples are not appreciably affected by the pressing conditions. From the magnetisation measurements the in-field Jc values at 10 K and 5.5 T were obtained as 8.41 × 103 A/cm2, 1.62 × 104 A/cm2, 6.90 × 103 A/cm2 and the Hirr values while Jc = 100 A/cm2 at 20 K were obtained as 5.99 T, 6.55 T and 6.19 T for the pure sample and the C16H10 added hot and cold pressed samples, respectively. The higher Jc and Hirr values obtained for the C16H10 added hot pressed sample is because of the homogenous C substitution into MgB2 grains, as compatible with its lower Δρ value, and thus increased flux pinning ability.

本文比较了热压和冷压对添加芘(C16H10)的块状 MgB2 超导特性的影响。为此,在 850 ℃ 下采用球团/闭管法制备了添加了 4 wt % C16H10 粉末的多晶盘状 MgB2 样品,然后在 200 ℃ 下进行热压和冷压。XRD 和 SEM 结果表明,虽然两种添加了 C16H10 的样品的 a-晶格参数都降低了,但由于 C 在 MgB2 结构中的积累和不均匀分布,冷压后平均晶粒尺寸增大了,而添加了 C16H10 的热压样品的平均晶粒尺寸减小了。电阻率测量结果表明,添加了 C16H10 的冷压样品的电子散射增量比添加了 C16H10 的热压样品的电子散射增量要高,这表明其晶粒连通性相对较好。根据磁化测量结果,纯样品和添加了 C16H10 的热压和冷压样品在 10 K 和 5.5 T 时的场内 Jc 值分别为 8.41 × 103 A/cm2, 1.62 × 104 A/cm2, 6.90 × 103 A/cm2 ,而在 20 K 时 Jc = 100 A/cm2 的 Hirr 值分别为 5.99 T, 6.55 T 和 6.19 T。添加了 C16H10 的热压样品的 Jc 值和 Hirr 值较高,这是因为 MgB2 晶粒中的 C 被均匀取代,这与其较低的Δρ 值相符,从而提高了磁通钉扎能力。
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引用次数: 0
Thermoluminescence Spectra of Rare-Earth Doped Calcium Fluoride 掺杂稀土的氟化钙的热致发光光谱
IF 1.6 4区 物理与天体物理 Q2 PHYSICS, MULTIDISCIPLINARY Pub Date : 2024-08-17 DOI: 10.1007/s13538-024-01575-y
V. S. M. de Barros, M. E. Yamato, P. L. Guzzo, V. K. Asfora, C. N. P. Oliveira, H. J. Khoury

This study investigates the thermoluminescence (TL) emission spectra of various doped CaF2 materials after exposure to ionizing radiation. The understanding of the TL spectra of these single-doped materials, systematically produced under the same sintering conditions, contributes to the interpretation of complex TL spectra observed in naturally occurring fluorite crystals. The production of Ce3+, Tm3+, Tb3+, Dy3+, Er3+, Pr3+, Nd3+, and Yb3+ doped calcium fluoride was carried out using the combustion synthesis method. The emission spectrum lines could be ascribed to the RE transitions that occur when a trapped hole center recombines with a RE2+. Emissions range from the ultra-violet to the near-infrared. This study aids in tailoring new materials for specific applications and the matching of emitted light to specific filters and instrumentation used for detection.

本研究调查了各种掺杂 CaF2 材料暴露于电离辐射后的热致发光 (TL) 发射光谱。了解这些在相同烧结条件下系统生产的单一掺杂材料的 TL 光谱,有助于解释在天然萤石晶体中观察到的复杂 TL 光谱。采用燃烧合成法生产了掺杂 Ce3+、Tm3+、Tb3+、Dy3+、Er3+、Pr3+、Nd3+ 和 Yb3+ 的氟化钙。发射光谱线可归因于被困空穴中心与 RE2+ 重新结合时发生的 RE 转变。发射范围从紫外线到近红外。这项研究有助于为特定应用定制新材料,并将发射光与特定滤光片和用于检测的仪器相匹配。
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引用次数: 0
期刊
Brazilian Journal of Physics
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