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Spin freezing induced giant exchange bias in a doped Hund's metal 掺杂亨氏金属中自旋冻结诱导的巨型交换偏置
Pub Date : 2024-09-06 DOI: arxiv-2409.04149
S. J. Li, D. Zhao, J. Li, B. L. Kang, M. Shan, Y. B. Zhou, X. Y. Li, T. Wu, X. H. Chen
Exchange bias (EB) is a fundamental phenomenon in widespread informationtechnologies. However, a comprehensive understanding of its microscopic originremains a great challenge. One key issue in the debate is the role offrustration and disorder in the EB mechanism, which motivates the explorationof the EB effect in spin glass (SG) systems. Here,in the SG state of Cr-dopedHund's metal CsFe2As2, we discover a giant EB effect with a maximum bias fieldof ~ 2 Tesla, which is almost two orders of magnitude larger than that oftraditional alloy SGs. Our results indicate that the giant EB effect shouldoriginate from the exchange interactions at the natural boundaries between thetunable ferromagnetic-like (FM) regions around Cr dopants and the SG matrix,via which the FM spins are strongly pinned by the frozen spins in the SGmatrix. In addition, the temperature-dependent and cooling-field-dependent EBbehaviors could be interpreted well by the SG model with frustrated FM/SGboundaries, which provides an intuitive and explicit understanding of theimpact of glassy parameters on the EB effect. All these results suggest thatthe correlated metals are promising directions for exploring the EB effect inthe SG state.
交换偏差(EB)是广泛应用的信息技术中的一种基本现象。然而,全面了解其微观起源仍然是一个巨大的挑战。争论中的一个关键问题是自旋玻璃(SG)体系中的无序和混乱在 EB 机制中的作用,这促使人们探索自旋玻璃体系中的 EB 效应。在这里,我们在掺杂铬的亨德金属 CsFe2As2 的自旋玻璃态中发现了巨大的 EB 效应,其最大偏置场约为 2 特斯拉,几乎比传统合金自旋玻璃大两个数量级。我们的研究结果表明,巨型 EB 效应源于铬掺杂物周围的可调谐类铁磁性(FM)区域与 SG 矩阵之间自然边界的交换相互作用,通过这种相互作用,FM 自旋被 SG 矩阵中的冻结自旋强烈钉住。此外,具有受挫调频/SG 边界的 SG 模型可以很好地解释随温度变化和随冷却场变化的 EB 行为,从而直观而清晰地了解玻璃参数对 EB 效应的影响。所有这些结果表明,相关金属是探索 SG 状态下 EB 效应的有前途的方向。
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引用次数: 0
Pairing tendencies in the doped Kitaev-Heisenberg model 掺杂基塔耶夫-海森堡模型中的配对趋势
Pub Date : 2024-09-06 DOI: arxiv-2409.04389
Pontus Laurell, Bradraj Pandey, Gábor B. Halász, Satoshi Okamoto, Gonzalo Alvarez, Elbio Dagotto
We study the impact of hole-doping on the Kitaev-Heisenberg model on thehoneycomb lattice. We investigate the pairing tendencies and correlationfunctions in the framework of a $t-J-K$ model using density matrixrenormalization group calculations on three-leg cylinders. In the case of thepure Kitaev model, which realizes a quantum spin-liquid phase at half-filling,we find that binding of two holes only occurs at low values of the hopping,where the holes are slow. We have theoretically verified that pair formationoccurs in the limit of immobile holes, where the pure Kitaev model remainsexactly solvable. When we instead fix the hopping at an intermediate, morerealistic, value, and vary the Heisenberg and Kitaev interaction strengths, wefind pairing tendencies only in the N'eel phase. This is in contrast to priormean-field calculations, highlighting the importance of accounting for thekinetic energy of dopants in generalized Kitaev models. Interestingly, we alsofind signatures of pair-density wave formation over the studied range of modelparameters, namely a periodic modulation of the charge density as well as thespin-spin and pair-pair correlations in real space. Moreover, we present acomparative study of the different correlations as a function of doping. Wefinally discuss the potential for experimentally observing the studied physicsin quantum materials and heterostructures.
我们研究了在蜂巢晶格上掺入空穴对基塔耶夫-海森堡模型的影响。我们在$t-J-K$模型的框架内,利用三脚圆柱体上的密度矩阵归一化群计算,研究了配对趋势和相关函数。在实现半填充量子自旋液相的纯基塔耶夫模型中,我们发现两个空穴的结合只发生在空穴速度较慢的低跳变值上。我们已经从理论上验证了在空穴不动的极限下会发生成对现象,在这种情况下,纯基塔耶夫模型仍然是精确可解的。相反,当我们把跳跃固定在一个中间的、现实的值,并改变海森堡和基塔耶夫的相互作用强度时,我们发现只有在N(鳗鱼)阶段才有配对倾向。这与先前的均场计算结果截然不同,突出了在广义基塔耶夫模型中考虑掺杂剂动能的重要性。有趣的是,在所研究的模型参数范围内,我们还发现了配对密度波形成的特征,即电荷密度的周期性调制以及实空间的自旋-自旋和配对-配对相关性。此外,我们还介绍了不同相关性作为掺杂函数的比较研究。最后,我们讨论了在量子材料和异质结构中实验观察所研究的物理学的潜力。
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引用次数: 0
Superconductivity, topological crystalline insulator and the absence of valence-skipping in AgSnSe$_2$ AgSnSe$_2$ 中的超导性、拓扑晶体绝缘体和不存在价跳现象
Pub Date : 2024-09-06 DOI: arxiv-2409.04096
Shubham Patel, A Taraphder
The recent suggestion of valence-skipping phenomenon driving a two-gapsuperconductivity in $Ag$-doped SnSe, by Kataria, textit{et al.} [Phys. Rev. B107, 174517 (2023)], has brought to the fore a long-standing issue once again.The absence of crystallographically inequivalent Sn cites corroborated byelectronic properties of AgSnSe$_2$, calculated using first-principles densityfunctional theory, however, does not appear to provide a strong support infavor of valence-skipping in this system. Interestingly, the signature ofavoided band-crossings (with the inclusion of SOC) and non-zero textit{mirror}Chern number ($n_{mathcal{M}}$) confirm a non-trivial topology. The presenceof mirror symmetry-protected surface states along the mirror planes indicatesthat AgSnSe$_2$ could be a potential candidate for topological crystallineinsulators (TCIs). Moreover, our calculation of electron-phonon coupling andanisotropic superconducting properties of AgSnSe$_2$, using Migdal-Eliashbergtheory, gives a single-gap superconductivity with critical temperature $T_capprox 7$K, consistent with the experimental value of $5$K. The interplay oftopology and superconductivity in this three-dimensional material appears quiteintriguing and it may provide new insights into the exploration ofsuperconductivity and topology.
最近,Kataria、textit{et al.}等人提出的价跃现象驱动了掺杂$Ag$的SnSe中的双间隙超导现象[Phys Rev B107, 174517 (2023)],再次把一个长期存在的问题推到了风口浪尖。[然而,利用第一原理密度函数理论计算的 AgSnSe$_2$ 的电子特性所证实的晶体学上不等价的锡引物的缺失,似乎并没有为该体系中的价跳现象提供有力的支持。有趣的是,避免带交叉的特征(包含 SOC)和非零 textit{mirror}Chern 数($n_{mathcal{M}}$)证实了非三维拓扑结构。沿镜面存在的镜面对称保护表面态表明,AgSnSe$_2$ 可能是拓扑晶体绝缘体(TCIs)的潜在候选材料。此外,我们利用 Migdal-Eliashberg 理论计算了 AgSnSe$_2$ 的电子-声子耦合和各向异性超导特性,得到了临界温度为 $T_capprox 7$K 的单隙超导,与实验值 5$K 一致。这种三维材料中拓扑学与超导性的相互作用似乎相当引人入胜,它可能为超导性与拓扑学的探索提供新的见解。
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引用次数: 0
Local Limit Disorder Characteristics of Superconducting Radio Frequency Cavities 超导射频腔的局部极限无序特性
Pub Date : 2024-09-06 DOI: arxiv-2409.04203
Anastasiya Lebedeva, Matúš Hladký, Marcel Polák, František Herman
Nowadays superconducting radio frequency (SRF) cavities represent fundamentaltools used for (Standard Model) particle acceleration, (beyond Standard Model)particle probing and long-lifetime photon preservation. We study the SRFfrequency shift in the vicinity of the critical temperature $T_c$ and thequality factor mainly at low temperatures within the Dynes superconductormodel. We scrutinize and use the local limit response to the externalelectromagnetic field. Our approach allows for a finer analysis of the peculiarbehavior of the resonant frequency shift immensely close to $T_c$, observed inrecent experiments. In the ideal dirty limit, we analytically elaborate on thewidth and depth of the resulting dip. Studying the sign of the slope of theresonant frequency shift at $T_c$ in the moderately clean regime reveals therole of the pair-breaking and pair-conserving disorder. Next, to find therelevance of our description, we compare and also fit our results with therecent experimental data from the N-doped Nb sample presented in[arXiv:2307.07905v1]. Our analysis remarkably complies with the experimentalfindings, especially concerning the dip width. We offer straightforward,homogeneous-disorder-based interpretation within the moderately clean regime.Assuming the same regime at low temperatures, we address details of thehigh-quality plateaus. Summing all up, this work presents (and studies thelimits of) the simple effective description of the complex problemcorresponding to the electromagnetic response in the superconductors combininghomogeneous conventional pairing and two different kinds of disorderscattering.
如今,超导射频(SRF)空腔是用于(标准模型)粒子加速、(超越标准模型)粒子探测和长寿命光子保存的基本工具。我们研究了临界温度 $T_c$ 附近的 SRF 频率偏移,以及戴尼斯超导模型中主要在低温下的品质因数。我们仔细研究并使用了对外部电磁场的局部极限响应。我们的方法可以更精细地分析在最近的实验中观察到的共振频率在非常接近 $T_c$ 时的奇特偏移行为。在理想的脏极限下,我们通过分析阐述了所产生的倾角的宽度和深度。在中等清洁度条件下,研究在 $T_c$ 时共振频率偏移斜率的符号,可以揭示成对断裂和成对守恒无序的作用。接下来,为了找到我们描述的相关性,我们将我们的结果与[arXiv:2307.07905v1]中掺杂 N 的铌样品的最新实验数据进行了比较和拟合。我们的分析结果与实验结果非常吻合,尤其是在倾角宽度方面。假定低温下存在相同的机制,我们将讨论高质量高原的细节。总之,这项工作提出了(并研究了)对复杂问题的简单有效描述,这些复杂问题与超导体中结合了同质常规配对和两种不同的无序散射的电磁响应有关。
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引用次数: 0
Emergence of Superconductivity at 20 K in Th$_3$P$_4$-type In$_{3-x}$S$_4$ Synthesized by Diamond Anvil Cell with Boron-doped Diamond Electrodes 使用掺硼金刚石电极的金刚石砧电池合成的 Th$_3$P$_4$ 型 In$_{3-x}$S$_4$ 在 20 K 时出现超导电性
Pub Date : 2024-09-05 DOI: arxiv-2409.03409
Ryo Matsumoto, Kazuki Yamane, Terumasa Tadano, Kensei Terashima, Toru Shinmei, Tetsuo Irifune, Yoshihiko Takano
The exploration of superconductors in metastable phases by manipulatingcrystal structures through high-pressure techniques has attracted significantinterest in materials science to achieve a high critical temperature ($T_c$).In this study, we report an emergence of novel superconductivity in ametastable phase of Th$_3$P$_4$-type cubic In$_{3-x}$S$_4$ with remarkably high$T_c$ at 20 K under 45 GPa by using an originally designed diamond anvil cellequipped with boron-doped diamond electrodes, which can perform a high-pressuresynthesis and an in-situ electrical transport measurement simultaneously.In-situ structural analysis indicates that the In$_{3-x}$S$_4$ appearspartially above 40 GPa without heating. The high-pressure annealing treatmentinduces complete transformation to the Th$_3$P$_4$-type structure, and thedefected concentration of x in In$_{3-x}$S$_4$ decreases with increasingannealing temperature. The $T_c$ in In$_{3-x}$S$_4$ is maximized at x = 0 andapproaches 20 K. Electronic band calculations show that the high density ofstates composed of sulfur and indium bands are located at the conduction bandbottom near Fermi energy. The record high $T_c$ in In$_{3-x}$S$_4$ amongsuperconducting sulfides accelerates the further exploration of high $T_c$materials within the Th$_3$P$_4$-type cubic family by using flexibility incrystal structure.
通过高压技术操纵晶体结构来探索瞬变相超导体以达到高临界温度($T_c$)的研究引起了材料科学领域的极大兴趣。在这项研究中,我们报告了在 Th$_{3-x}$S$_4$ 型立方 In$_{3-x}$S$_4$ 的瞬变相中出现的新型超导电性,这种超导电性在 20 K、45 GPa 条件下具有显著的高 T_c$。原位结构分析表明,在不加热的情况下,In$_{3-x}$S$_4$ 部分出现在 40 GPa 以上。高压退火处理使其完全转变为 Th$_3$P$_4$ 型结构,并且随着退火温度的升高,In$_{3-x}$S$_4$ 中 x 的缺陷浓度降低。电子能带计算表明,硫带和铟带组成的高密度态位于费米能附近的导带底部。超导硫化物 In$_{3-x}$S$_4$ 中创纪录的高 T_c$ 值加速了人们利用晶体结构的灵活性进一步探索 Th$_3$P$_4$ 型立方体家族中的高 T_c$ 材料。
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引用次数: 0
Multidimensional Terahertz Probes of Quantum Materials 量子材料的多维太赫兹探针
Pub Date : 2024-09-05 DOI: arxiv-2409.03719
Albert Liu
Multidimensional spectroscopy has a long history originating from nuclearmagnetic resonance, and has now found widespread application at infrared andoptical frequencies as well. However, the energy scales of traditionalmultidimensional probes have been ill-suited for studying quantum materials.Recent technological advancements have now enabled extension of thesemultidimensional techniques to the terahertz frequency range, in whichcollective excitations of quantum materials are typically found. ThisPerspective introduces the technique of two-dimensional terahertz spectroscopy(2DTS) and the unique physics of quantum materials revealed by 2DTS spectra,accompanied by a selection of the rapidly expanding experimental andtheoretical literature. While 2DTS has so far been primarily applied to quantummaterials at equilibrium, we provide an outlook for its application towardsunderstanding their dynamical non-equilibrium states and beyond.
多维光谱学由来已久,起源于核磁共振,目前在红外和光学频率上也有广泛应用。然而,传统多维探针的能级并不适合研究量子材料。最近的技术进步使多维技术扩展到了太赫兹频率范围,而量子材料的集合激发通常就出现在太赫兹频率范围。本展望介绍了二维太赫兹光谱(2DTS)技术以及 2DTS 光谱所揭示的量子材料的独特物理特性,并选取了一些迅速扩展的实验和理论文献。虽然迄今为止二维太赫兹光谱主要应用于平衡态量子材料,但我们展望了它在理解非平衡态及其他动态态方面的应用。
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引用次数: 0
Competition between the modification of intrinsic superconducting properties and the pinning landscape under external pressure in CaKFe$_4$As$_4$ single crystals CaKFe$_4$As$_4$ 单晶内在超导特性的改变与外压作用下的引脚分布之间的竞争
Pub Date : 2024-09-05 DOI: arxiv-2409.03809
Shuyuan Huyan, Nestor Haberkorn, Mingyu Xu, Paul C. Canfield, Sergey L. Bud'ko
Measurements of low field magnetization, trapped flux magnetization and 5 Kflux creep in single crystal of CaKFe$_4$As$_4$ under pressure up to 7.5 GPa ina diamond pressure cell are presented. The observed evolution of thetemperature dependence of the self-field critical current and slowing down ofthe base temperature flux creep rate are explained within the two sources ofpinning hypothesis involving presence of CaKFe$_4$As$_4$ intergrowths suggestedin the literature. Above the half collapsed tetragonal structural transitionunder pressure, where superconductivity is non-bulk or absent, criticallydiminished or no diamagnetism and flux trapped magnetization were observed.
本文介绍了在金刚石压力池中对 CaKFe$_4$As$_4$ 单晶体在高达 7.5 GPa 压力下的低场磁化、困磁和 5 Kflux 蠕变的测量结果。观察到的自场临界电流温度依赖性的演变和基温磁通蠕变速率的减慢,可以用文献中提出的涉及 CaKFe$_4$As$_4$ 间生长的两个旋流源假说来解释。在压力下的半塌陷四方结构转变以上,超导性为非大量存在或不存在,观察到二磁性和磁通陷磁化严重减弱或不存在。
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引用次数: 0
Anisotropic Spin Stripe Domains in Bilayer La$_3$Ni$_2$O$_7$ 双层 La$_3$Ni$_2$O$_7$ 中的各向异性自旋条纹域
Pub Date : 2024-09-05 DOI: arxiv-2409.03210
N. K Gupta, R. Gong, Y. Wu, M. Kang, C. T. Parzyck, B. Z. Gregory, N. Costa, R. Sutarto, S. Sarker, A. Singer, D. G. Schlom, K. M. Shen, D. G. Hawthorn
The discovery of superconductivity in La$_3$Ni$_2$O$_7$ under pressure hasmotivated the investigation of a parent spin density wave (SDW) state whichcould provide the underlying pairing interaction. Here, we employ resonant softx-ray scattering and polarimetry on thin films of bilayer La$_3$Ni$_2$O$_7$ todetermine that the magnetic structure of the SDW forms unidirectional diagonalspin stripes with moments lying within the NiO$_2$ plane and perpendicular to$mathbf{Q}_{SDW}$, but without the strong charge disproportionation typicallyassociated with other nickelates. These stripes form anisotropic domains withshorter correlation lengths perpendicular versus parallel to$mathbf{Q}_{SDW}$, revealing nanoscale rotational and translational symmetrybreaking analogous to the cuprate and Fe-based superconductors, with Bloch-likeantiferromagnetic domain walls separating orthogonal domains.
La$_3$Ni$_2$O$_7$ 在压力下的超导电性的发现激发了对母体自旋密度波 (SDW) 状态的研究,这种状态可能提供了基本的配对相互作用。在这里,我们在双层 La$_3$Ni$_2$O$_7$ 薄膜上使用了共振软X射线散射和极坐标测量法,以确定 SDW 的磁性结构形成了单向对角自旋条纹,其力矩位于 NiO$_2$ 平面内并垂直于 $mathbf{Q}_{SDW}$,但没有其他镍酸盐典型的强电荷比例失调。这些条纹形成了各向异性的畴,其垂直于$mathbf{Q}_{SDW}$的相关长度比平行于$mathbf{Q}_{SDW}$的相关长度短,揭示了类似于铜氧化物和铁基超导体的纳米级旋转和平移对称性破坏,布洛赫类反铁磁畴壁将正交的畴分隔开来。
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引用次数: 0
Stabilization of Ambient Pressure Rocksalt Crystal Structure and High Critical Field Superconductivity in ReC via Mo and W Substitution 通过钼和钨替代稳定 ReC 中的常压岩石盐晶体结构和高临界场超导性
Pub Date : 2024-09-05 DOI: arxiv-2409.03592
P. K. Meena, S. Jangid, R. K. Kushwaha, P. Manna, S. Sharma, P. Mishra, R. P. Singh
Transition-metal-based carbides (TMCs), renowned for their exceptionalhardness, mechanical strength, and thermal properties, have recently emerged aspromising candidates for topological superconductivity. In this study, wesynthesized ReC in the NaCl structure at ambient pressure by substituting Mo orW at the Re-site. We investigated the superconducting properties ofRe$_{1-x}$T$_{x}$C (where T = Mo, W) for $x = 0.5$ using magnetization,resistivity and specific heat measurements. These compounds display type-II,fully gapped, weakly coupled superconductivity with high critical fields,establishing them as new members of superconducting ultra-hard materials atambient pressure and paving the way for superconducting device applicationsunder extreme conditions.
过渡金属基碳化物(TMC)以其优异的硬度、机械强度和热性能而闻名,最近已成为拓扑超导性的理想候选材料。在这项研究中,我们通过在 Re-site 处取代 Mo 或 W,在常压下在 NaCl 结构中合成了 ReC。我们利用磁化、电阻率和比热测量方法研究了 Re$_{1-x}$T$_{x}$C(其中 T = Mo、W)在 $x = 0.5$ 时的超导特性。这些化合物显示出具有高临界场的 II 型、全间隙、弱耦合超导性,使它们成为常压超导超硬材料的新成员,并为极端条件下的超导设备应用铺平了道路。
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引用次数: 0
Single photon detection up to 2 um in pair of parallel microstrips based on NbRe ultrathin films 基于 NbRe 超薄薄膜的一对平行微带的单光子探测能力可达 2 um
Pub Date : 2024-09-04 DOI: arxiv-2409.02619
C. Cirillo, M. Ejrnaes, P. Ercolano, C. Bruscino, A. Cassinese, D. Salvoni, C. Attanasio, G. P. Pepe, L. Parlato
Superconducting Microstrip Single Photon Detectors (SMSPDs) are increasinglyattracting the interest of the scientific community as a new platform for largearea detectors with unprecedented advantaged in terms of fabrication. However,while their operativity at the telecommunication wavelength was achieved,working beyond 1.55 um is challenging. Here, we experimentally demonstratesingle-photon operation of NbRe microstrips at wavelengths of 1.55 and 2 um.The devices are structured as pairs of parallel microstrips with widths rangingfrom 1.4 to 2.2 um and lengths from 5 to 10 um. This innovative design mayassure large sensitive areas, without affecting the kinetic inductance, namelythe time performance of the detectors. The results are discussed in theframework of the hot-spot two-temperature model.
超导微带单光子探测器(SMSPD)作为大面积探测器的新平台,在制造方面具有前所未有的优势,正日益吸引科学界的兴趣。然而,虽然其在电信波长上的工作能力已经实现,但要在 1.55 um 以上的波长上工作仍具有挑战性。在这里,我们通过实验演示了掺钕铼微带在 1.55 和 2 微米波长下的单光子工作原理。该器件的结构是一对平行微带,宽度为 1.4 至 2.2 微米,长度为 5 至 10 微米。这种创新设计可以保证大的敏感区域,而不影响动感,即探测器的时间性能。研究结果将在热点双温模型框架内进行讨论。
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引用次数: 0
期刊
arXiv - PHYS - Superconductivity
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