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Nodeless superconductivity and topological nodal states in molybdenum carbide 碳化钼中的无结点超导性和拓扑结点态
Pub Date : 2024-09-04 DOI: arxiv-2409.02380
Tian Shang, Yuting Wang, Bochen Yu, Keqi Xia, Darek J. Gawryluk, Yang Xu, Qingfeng Zhan, Jianzhou Zhao, Toni Shiroka
The orthorhombic molybdenum carbide superconductor with $T_c$ = 3.2 K wasinvestigated by muon-spin rotation and relaxation ($mu$SR) measurements and byfirst-principle calculations. The low-temperature superfluid density,determined by transverse-field $mu$SR, suggests a fully-gapped superconductingstate in Mo$_2$C, with a zero-temperature gap $Delta_0$ = 0.44 meV and amagnetic penetration depth $lambda_0$ = 291 nm. The time-reversal symmetry ispreserved in the superconducting state, as confirmed by the absence of anadditional muon-spin relaxation in the zero-field $mu$SR spectra.Band-structure calculations indicate that the density of states at the Fermilevel is dominated by the Mo $4d$-orbitals, which are marginally hybridizedwith the C $2p$-orbitals over a wide energy range. The symmetry analysisconfirms that, in the absence of spin-orbit coupling (SOC), Mo$_2$C hoststwofold-degenerate nodal surfaces and fourfold-degenerate nodal lines. Whenconsidering SOC, the fourfold-degenerate nodal lines cross the Fermi level andcontribute to the electronic properties. Our results suggest that, similarly toother phases of carbides, also the orthorhombic transition-metal carbides hosttopological nodal states and may be potential candidates for future studies oftopological superconductivity.
通过μ介子自旋旋转和弛豫($mu$SR)测量以及第一性原理计算,研究了T_c$ = 3.2 K的正交碳化钼超导体。通过横向场$mu$SR测定的低温超流体密度表明,Mo$_2$C中存在一个全隙缝超导态,其零温间隙为$Delta_0$ = 0.44 meV,非磁性穿透深度为$lambda_0$ = 291 nm。带状结构计算表明,费米级的态密度由 Mo 4d 元轨道主导,而 Mo 4d 元轨道在很宽的能量范围内与 C 2p 元轨道有微弱的杂化。对称性分析证实,在没有自旋轨道耦合(SOC)的情况下,Mo$_2$C 存在两重退化的结面和四重退化的结线。当考虑到自旋轨道耦合时,四重退化的结点线穿过费米级并对电子特性做出贡献。我们的研究结果表明,与碳化物的其他相类似,正交过渡金属碳化物也蕴藏着拓扑结点态,可能成为未来拓扑超导研究的潜在候选对象。
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引用次数: 0
Josephson diode effect in one-dimensional quantum wires connected to superconductors with mixed singlet-triplet pairing 与单三态混合配对超导体相连的一维量子线中的约瑟夫森二极管效应
Pub Date : 2024-09-04 DOI: arxiv-2409.02794
Abhiram Soori
The Josephson diode effect (JDE), characterized by asymmetric criticalcurrents in a Josephson junction, has drawn considerable attention in the fieldof condensed matter physics. We investigate the conditions under which JDE canmanifest in a one-dimensional Josephson junction composed of aspin-orbit-coupled quantum wire with an applied Zeeman field, connected betweentwo superconductors. Our study reveals that while spin-orbit coupling (SOC) anda Zeeman field in the quantum wire are not sufficient to induce JDE when thesuperconductors are purely singlet, the introduction of triplet pairing in thesuperconductors leads to the emergence of JDE. This finding highlights thepotential of JDE as a probe for triplet superconductivity. We furtherdemonstrate that even in absence of SOC in the quantum wire, JDE can arise whenthe directions of the triplet pairing and the Zeeman field are non-collinear,provided the superconductors exhibit mixed singlet-triplet pairing.Additionally, we identify specific conditions under which JDE is absent,namely, when the pairing is purely triplet and the directions of the SOC andthe triplet pairing are perpendicular. Our findings indicate that JDE is alwaysaccompanied by the anomalous Josephson effect. The diode effect coefficient isfound to oscillate with variations in the chemical potential of the quantumwire, driven by Fabry-P'erot interference effects. Our results suggest thatquantum wires in Josephson junctions could serve as effective platforms forprobing triplet superconductivity through the observation of JDE.
约瑟夫森二极管效应(JDE)以约瑟夫森结中的不对称临界电流为特征,在凝聚态物理领域引起了广泛关注。我们研究了约瑟夫森二极管效应在一维约瑟夫森结中产生的条件,该结由带有外加泽曼场的自旋轨道耦合量子线组成,连接在两个超导体之间。我们的研究发现,虽然量子线中的自旋轨道耦合(SOC)和泽曼场在超导体为纯单线时不足以诱发 JDE,但在超导体中引入三重配对会导致 JDE 的出现。这一发现凸显了 JDE 作为三重超导探针的潜力。我们进一步证明,即使量子线中不存在SOC,只要超导体表现出单线-三线混合配对,当三线配对和泽曼场的方向不共线时,也会出现JDE。我们的研究结果表明,JDE 总是伴随着反常约瑟夫森效应。在法布里-波特干涉效应的驱动下,二极管效应系数会随着量子线化学势的变化而摆动。我们的研究结果表明,约瑟夫森结中的量子线可以作为通过观察 JDE 来探测三重超导性的有效平台。
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引用次数: 0
Ephemeral Superconductivity Atop the False Vacuum 假真空之上的短暂超导现象
Pub Date : 2024-09-04 DOI: arxiv-2409.02992
Gal Shavit, Stevan Nadj-Perge, Gil Refael
A many body system in the vicinity of a first-order phase transition may gettrapped in a local minimum of the free energy landscape. These so-calledfalse-vacuum states may survive for exceedingly long times if the barrier fortheir decay is high enough. The rich phase diagram obtained in graphenemultilayer devices presents a unique opportunity to explore transientsuperconductivity on top of a correlated false vacuum. Specifically, weconsider superconductors which are terminated by an apparent first-order phasetransition to a correlated phase with different symmetry. We propose thatquenching across this transition leads to a non-equilibrium ephemeralsuperconductor, readily detectable using straightforward transportmeasurements. Besides enabling a simple detection scheme, the transientsuperconductor also generically enhances the false vacuum lifetime, potentiallyby orders of magnitude. In several scenarios, the complimentary effect takesplace as well: superconductivity is temporarily emboldened in the false vacuum,albeit ultimately decaying. We demonstrate the applicability of these claimsfor two different instances of superconductivity terminated by a first ordertransition in rhombohedral graphene. The obtained decay timescales positionthis class of materials as a promising playground to unambiguously realize andmeasure non-equilibrium superconductivity.
在一阶相变附近的多体系统可能会被困在自由能谱的局部最小值中。如果其衰变的势垒足够高,这些所谓的假真空态可能会存活很长时间。在石墨烯多层器件中获得的丰富相图为探索相关假真空之上的瞬态超导性提供了一个独特的机会。具体来说,我们考虑的超导体是由一个明显的一阶相位转变到一个具有不同对称性的相关相位所终止的。我们提出,跨越这一转变的淬火会导致一种非平衡的短暂超导体,而这种超导体很容易通过直接的传输测量进行探测。瞬态超导体除了能实现简单的探测方案外,还能普遍增强假真空寿命,可能达到几个数量级。在几种情况下,还出现了互补效应:超导性在假真空中暂时增强,尽管最终会衰减。我们在斜方体石墨烯中通过一阶转变终止超导的两个不同实例中证明了这些说法的适用性。所获得的衰变时间尺度将这一类材料定位为明确实现和测量非平衡超导性的理想场所。
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引用次数: 0
Accelerated Lanthanide Intercalation into Graphite Catalyzed by Na 在 Na 催化下加速镧系元素与石墨的互钙化
Pub Date : 2024-09-03 DOI: arxiv-2409.01624
Akira Iyo, Hiroshi Fujihisa, Yoshito Gotoh, Shigeyuki Ishida, Hiroshi Eisaki, Hiraku Ogino, Kenji Kawashima
Lanthanides ($Ln$) are notoriously difficult to intercalate into graphite. Weinvestigated the possibility of using Na to catalyze the formation of$Ln$-intercalated graphite and successfully synthesized $Ln$C$_6$ ($Ln$ = Sm,Eu, and Yb) significantly rapidly in high yields. The synthesis processinvolves the formation of the reaction intermediate NaC$_x$, through the mixingof Na and C, which subsequently reacts with $Ln$ upon heating to form$Ln$C$_6$. Well-sintered $Ln$C$_6$ pellets with low residual Na concentrations($Ln$:Na = 98:2) were fabricated by the two-step method. The pellets enabledthe evaluation of $Ln$C$_6$ by powder X-ray diffraction and electricalresistivity measurements. This study highlights the versatility of theNa-catalyzed method and lays the foundation for the rapid mass production of$Ln$C$_6$, with potential applications in superconducting and rechargeablebattery materials.
众所周知,镧系元素($Ln$)很难插层到石墨中。我们研究了使用 Na 催化形成$Ln$插层石墨的可能性,并成功地以高产率快速合成了$Ln$C$$_6$($Ln$ = Sm、Eu 和 Yb)。合成过程包括通过 Na 和 C 的混合形成反应中间体 NaC$_x$,然后在加热过程中与 $Ln$ 反应形成 $Ln$C$_6$。通过两步法制造出了烧结良好的低残留 Na 浓度($Ln$:Na = 98:2)$Ln$C$_6$颗粒。通过粉末 X 射线衍射和电电阻率测量,可以对这些颗粒进行 $Ln$C$_6$ 评估。这项研究凸显了 Na 催化方法的多功能性,并为 Ln$C$_6$ 的快速量产奠定了基础,有望应用于超导材料和可充电电池材料。
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引用次数: 0
Analysis of Thermal Grooving Effects on Vortex Penetration in Vapor-Diffused Nb3Sn 蒸汽扩散 Nb3Sn 中涡流穿透的热开槽效应分析
Pub Date : 2024-09-03 DOI: arxiv-2409.01569
Eric M. Lechner, Olga Trofimova, Jonathan W. Angle, Madison C. DiGuilio, Uttar Pudasaini
While Nb3Sn theoretically offers better superconducting RF cavity performance(Q0 and Eacc) to Nb at any given temperature, peak RF magnetic fieldsconsistently fall short of the 400 mT prediction. The relatively roughtopography of vapor-diffused Nb3Sn is widely conjectured to be one of thefactors that limit the attainable performance of Nb3Sn-coated Nb cavitiesprepared via Sn vapor diffusion. Here we investigate the effect of coatingduration on the topography of vapor-diffused Nb3Sn on Nb and calculate theassociated magnetic field enhancement and superheating field suppressionfactors using atomic force microscopy topographies. It is shown that thethermally grooved grain boundaries are major defects which may contribute to asubstantial decrease in the achievable accelerating field. The severity ofthese grooves increases with total coating duration due to the deepening ofthermal grooves during the coating process.
虽然在任何给定温度下,Nb3Sn 理论上都比 Nb 具有更好的超导射频腔性能(Q0 和 Eacc),但峰值射频磁场始终低于 400 mT 的预测值。人们普遍认为,气相扩散 Nb3Sn 相对粗糙的形貌是限制通过锡气相扩散制备的 Nb3Sn 涂层铌空腔性能的因素之一。在这里,我们研究了镀层持续时间对铌上气相扩散 Nb3Sn 形貌的影响,并利用原子力显微镜形貌计算了相关的磁场增强和过热场抑制因子。结果表明,热沟槽晶界是主要缺陷,可能导致可实现的加速磁场大幅降低。由于在镀膜过程中热沟槽加深,这些沟槽的严重程度随着总镀膜时间的延长而增加。
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引用次数: 0
Pairing transitions in a Binary Bose Gas 二元玻色气体中的配对转换
Pub Date : 2024-09-03 DOI: arxiv-2409.01565
Zesheng Shen, Lan Yin
The stable Bardeen-Schrieffer-Cooper (BCS) pairing state of a bosonic systemhas long been sought theoretically and experimentally. Here we study the BCSstate of a binary Bose gas with $s$-wave intra-species repulsions and aninter-species attraction in the mean-field-stable region. We find that abovethe Bose-Einstein-Condensation (BEC) transtion temperature, there is a phasetranstion from the normal state to the BCS state due to inter-species pairing.When the temperature decreases, another phase transtion from the BCS state tothe mixture state with both atomic BEC and inter-species pairs occurs. As thetemperature is further lowered, the mixuture state is taken over by the BECstate. The phase diagram of this system is presented and experimentalimplications are discussed.
长期以来,人们一直在理论和实验上寻找玻色系统的稳定巴丁-施里弗-库珀(BCS)配对态。在这里,我们研究了在均值场稳定区具有s$波种内排斥和种间吸引的双玻色气体的BCS态。我们发现,在玻色-爱因斯坦凝聚(BEC)跃迁温度之上,由于种间配对,会出现从正常态到 BCS 态的相跃迁。随着温度的进一步降低,混合态被 BEC 态所取代。本文展示了这一系统的相图,并讨论了其实验意义。
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引用次数: 0
Field-free superconducting diode effect in layered superconductor FeSe 层状超导体 FeSe 中的无场超导二极管效应
Pub Date : 2024-09-03 DOI: arxiv-2409.01715
Utane NagataDep. Electronic Science and Engineering, Kyoto Univ, Motomi AokiDep. Electronic Science and Engineering, Kyoto UnivCSRN-Kyoto, Akito DaidoGraduate School of Science, Kyoto Univ, Shigeru KasaharaOkayama Univ, Yuichi KasaharaGraduate School of Science, Kyoto Univ, Ryo OhshimaDep. Electronic Science and Engineering, Kyoto UnivCSRN-Kyoto, Yuichiro AndoDep. Electronic Science and Engineering, Kyoto UnivCSRN-Kyoto, Youichi YanaseCSRN-KyotoGraduate School of Science, Kyoto Univ, Yuji MatsudaGraduate School of Science, Kyoto Univ, Masashi ShiraishiDep. Electronic Science and Engineering, Kyoto UnivCSRN-Kyoto
The superconducting diode effect (SDE), where zero-resistance states appearnonreciprocally during current injection, is receiving tremendous interest inboth fundamental and applied physics because the SDE is a novel manifestationof symmetry breaking and enables the creation of a novel diode without energyloss. In particular, magnetic-field-free SDEs have been extensivelyinvestigated because of their potential to serve as building blocks forsuperconducting circuit technology. In this letter, we report the field-freeSDE in a layered superconductor, FeSe. Its underlying physics is clarified bysystematic controlled experiments to be an interplay of a large thermoelectricresponse and geometrical asymmetry in FeSe. Our findings can pave a new avenuefor the construction of novel material and device platforms utilizing SDEs.
超导二极管效应(SDE)是指零电阻状态在电流注入过程中不递减地出现,它在基础物理学和应用物理学领域都受到了极大的关注,因为超导二极管效应是对称性破缺的一种新表现形式,它能够在不损失能量的情况下制造出新型二极管。特别是无磁场 SDE,由于其作为超导电路技术构件的潜力而受到广泛研究。在这封信中,我们报告了层状超导体 FeSe 中的无磁场 SDE。我们通过系统控制实验阐明了其基本物理原理,即 FeSe 中的大热电响应和几何不对称的相互作用。我们的发现为利用 SDE 构建新型材料和器件平台铺平了新的道路。
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引用次数: 0
Impurity States in Altermagnetic Superconductors 异磁超导体中的杂质状态
Pub Date : 2024-09-02 DOI: arxiv-2409.01008
Andrea Maiani, Rubén Seoane Souto
Altermagnetic superconductors hold the potential for novel phenomena,including topological states, finite-momentum superconductivity, as well aspromising applications in spintronics. However, an experimental demonstrationof the coexistence of these two effects is still lacking. In this work, wepropose potential impurities as a way to probe the distinctive properties ofaltermagnetic superconductors. These impurities induce spin-polarized subgapstates that extend along the crystal axes, inheriting the magneticcharacteristics of the bulk. When the impurities respect the bulk symmetries,they generate spin-degenerate doublets; otherwise, the degeneracy is lifted. Anexternal magnetic field aligned with the N'eel vector can tune the energies ofthe spin components of the subgap states. These components show differentspatial extensions that can be measured via local probes, like scanningtunneling microscopy. For certain parameters, the impurity state can induce alocal sign change on the order parameter, so-called $pi$-transition. Lastly,we investigate the interaction between impurities, revealing aposition-dependent effective coupling that facilitates the engineering ofspin-dependent tunneling. This tunable coupling introduces a new approach forin-situ control of devices critical for quantum information processing andtopological superconductivity.
异磁超导体有可能产生新的现象,包括拓扑态、有限动量超导,以及在自旋电子学中的应用。然而,目前还缺乏对这两种效应共存的实验证明。在这项工作中,我们提出用潜在的杂质来探测顺磁超导体的独特性质。这些杂质会诱发沿晶轴延伸的自旋极化亚间隙态,从而继承了体质的磁性特征。当杂质尊重体对称性时,它们会产生自旋退化的双态;反之,退化会被解除。与N(鳗鱼)矢量对齐的外部磁场可以调节亚隙态自旋分量的能量。这些分量显示出不同的空间延伸,可以通过局部探针测量,如扫描隧道显微镜。对于某些参数,杂质态可以引起阶次参数的局部符号变化,即所谓的 $pi$ 转变。最后,我们研究了杂质之间的相互作用,揭示了依赖于位置的有效耦合,这种耦合促进了依赖于自旋的隧道工程。这种可调耦合为量子信息处理和拓扑超导关键器件的原位控制引入了一种新方法。
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引用次数: 0
Universal degradation of high-temperature superconductors due to impurity scattering: predicting the performance loss in fusion magnets 杂质散射导致的高温超导体普遍退化:预测聚变磁体的性能损失
Pub Date : 2024-09-02 DOI: arxiv-2409.01376
M. Eisterer, A. Bodenseher, R. Unterrainer
Predicting the change of performance of superconductors under neutronradiation is indispensable for designing compact fusion devices. The favorableenhancement of the critical current caused by flux pinning is separated fromthe degrading effect of increased scattering of the charge carriers to derive adegradation function from the expected change of the superfluid density(reducing to Homes law in the dirty limit) and the observed increase in fluxcreep. The degradation turned out to be a universal function of disorder, notdepending on the particular tape nor the particle radiation: thermal and/orfast neutrons, as well as 1.2 MeV protons. The universal behavior enables theanalysis of changes in flux pinning corrected by the adverse enhancement ofscattering. A more reliable prediction of the performance change of coatedconductors in a fusion reactor based on proxies for neutrons is anticipated.
预测超导体在中子辐照下的性能变化对于设计紧凑型核聚变装置是必不可少的。从超流体密度的预期变化(在脏极限下降至霍姆斯定律)和观察到的通量衰减的增加中,分离出了由通量钉扎引起的临界电流的有利增强效应和电荷载流子散射增加的衰减效应,从而推导出衰减函数。结果表明,降解是一种普遍的无序函数,既不取决于特定的磁带,也不取决于粒子辐射:热中子和/或快中子,以及 1.2 MeV 质子。这种普遍行为使我们能够分析由散射的不利增强所修正的磁通量针脚变化。预计在聚变反应堆中,基于中子的代用指标对涂层导体性能变化的预测将更加可靠。
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引用次数: 0
Directly visualizing nematic superconductivity driven by the pair density wave in NbSe$_2$ 直接可视化 NbSe$_2$ 中由对密度波驱动的向列超导性
Pub Date : 2024-09-01 DOI: arxiv-2409.00660
Lu Cao, Yucheng Xue, Yingbo Wang, Fu-Chun Zhang, Jian Kang, Hong-Jun Gao, Jinhai Mao, Yuhang Jiang
Pair density wave (PDW) is a distinct superconducting state characterized bya periodic modulation of its order parameter in real space. Its intricateinterplay with the charge density wave (CDW) state is a continuing topic ofinterest in condensed matter physics. While PDW states have been discovered incuprates and other unconventional superconductors, the understanding of diversePDWs and their interactions with different types of CDWs remains limited. Here,utilizing scanning tunneling microscopy, we unveil the subtle correlationsbetween PDW ground states and two distinct CDW phases -- namely,anion-centered-CDW (AC-CDW) and hollow-centered-CDW (HC-CDW) -- in 2H-NbSe$_2$.In both CDW regions, we observe coexisting PDWs with a commensurate structurethat aligns with the underlying CDW phase. The superconducting gap size,$Delta(r)$, related to the pairing order parameter is in phase with the chargedensity in both CDW regions. Meanwhile, the coherence peak height, $H(r)$,qualitatively reflecting the electron-pair density, exhibits a phase differenceof approximately $2pi/3$ relative to the CDW. The three-fold rotationalsymmetry is preserved in the HC-CDW region but is spontaneously broken in theAC-CDW region due to the PDW state, leading to the emergence of nematicsuperconductivity.
对密度波(PDW)是一种独特的超导态,其特征是其阶参数在实空间的周期性调制。它与电荷密度波(CDW)态之间错综复杂的相互作用是凝聚态物理学中一个持续关注的话题。虽然人们已经发现了超导体和其他非常规超导体中的 PDW 状态,但对各种 PDW 及其与不同类型 CDW 的相互作用的了解仍然有限。在这里,我们利用扫描隧道显微镜揭示了 2H-NbSe$_2$ 中的 PDW 基态与两种不同的 CDW 相(即阴离子中心 CDW(AC-CDW)和空心 CDW(HC-CDW))之间的微妙关联。与配对阶次参数相关的超导间隙大小($Delta(r)$)与两个 CDW 区域的带电强度相一致。同时,定性反映电子对密度的相干峰高$H(r)$相对于CDW表现出大约2美元的相位差。三倍旋转对称性在HC-CDW区得以保留,但在AC-CDW区由于PDW态而自发被打破,从而导致了线性超导的出现。
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引用次数: 0
期刊
arXiv - PHYS - Superconductivity
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