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Spin-Hall effect in topological materials: evaluating the proper spin current in systems with arbitrary degeneracies 拓扑材料中的自旋-霍尔效应:评估任意变性系统中的适当自旋电流
Pub Date : 2024-11-21 DOI: 10.1038/s44306-024-00057-w
Hongyang Ma, James H. Cullen, Serajum Monir, Rajib Rahman, Dimitrie Culcer
The spin-Hall effect underpins some of the most active topics in modern physics, including spin torques and the inverse spin-Hall effect, yet it lacks a proper theoretical description. This makes it difficult to differentiate the SHE from other mechanisms, as well as differentiate band structure and disorder contributions. Here, by exploiting recent analytical breakthroughs in the understanding of the intrinsic spin-Hall effect, we devise a density functional theory method for evaluating the conserved (proper) spin current in a generic system. Spin non-conservation makes the conventional spin current physically meaningless, while the conserved spin current has been challenging to evaluate since it involves the position operator between Bloch bands. The novel method we introduce here can handle band structures with arbitrary degeneracies and incorporates all matrix elements of the position operator, including the notoriously challenging diagonal elements, which are associated with Fermi surface, group velocity, and dipolar effects but often diverge if not treated correctly. We apply this method to the most important classes of spin-Hall materials: topological insulators, 2D quantum spin-Hall insulators, non-collinear antiferromagnets, and strongly spin-orbit coupled metals. We demonstrate that the torque dipole systematically suppresses contributions to the conventional spin current such that, the proper spin current is generally smaller in magnitude and often has a different sign. Remarkably, its energy-dependence is relatively flat and featureless, and its magnitude is comparable in all classes of materials studied. These findings will guide the experiment in characterizing charge-to-spin interconversion in spintronic and orbitronic devices. We also discuss briefly a potential generalization of the method to calculate extrinsic spin currents generated by disorder scattering.
自旋-霍尔效应是现代物理学中一些最活跃课题的基础,包括自旋力矩和反自旋-霍尔效应,但它缺乏适当的理论描述。这使得我们很难区分自旋霍尔效应和其他机制,也很难区分带状结构和无序贡献。在此,我们利用最近在理解本征自旋-霍尔效应方面取得的分析突破,设计了一种密度泛函理论方法,用于评估通用系统中的守恒(适当)自旋电流。自旋不守恒使得传统的自旋电流在物理上失去意义,而守恒自旋电流由于涉及布洛赫带之间的位置算子,其评估一直具有挑战性。我们在此介绍的新方法可以处理具有任意退变性的带状结构,并包含位置算子的所有矩阵元素,包括臭名昭著的对角元素,这些元素与费米面、群速度和偶极效应有关,但如果处理不当,往往会发散。我们将这种方法应用于最重要的自旋霍尔材料类别:拓扑绝缘体、二维量子自旋霍尔绝缘体、非共轭反铁磁体和强自旋轨道耦合金属。我们证明,转矩偶极子系统性地抑制了对传统自旋电流的贡献,因此适当的自旋电流通常较小,而且经常具有不同的符号。值得注意的是,其能量依赖性相对平缓且无特征,其大小在所研究的各类材料中都相当。这些发现将指导自旋电子和轨道电子器件中的电荷-自旋相互转换实验。我们还简要讨论了计算无序散射产生的外在自旋电流的方法的潜在推广。
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引用次数: 0
Recent progress on controlling spin-orbit torques by materials design 通过材料设计控制自旋轨道力矩的最新进展
Pub Date : 2024-11-21 DOI: 10.1038/s44306-024-00054-z
Guiping Ji, Yuejie Zhang, Yahong Chai, Tianxiang Nan
Spin-orbit torques (SOTs) provide an energy-efficient approach for the electrical manipulation of magnetization, pivotal for next-generation information storage and processing devices. SOTs can be generated via various mechanisms, such as spin Hall effect, Rashba-Edelstein effect, orbital Hall effect, magnons, and spin swapping. SOTs-based devices hold potential advantages over spin-transfer torque (STT) devices, including low power consumption, enhanced durability, and a broader selection of applicable materials for both SOT generation and excitation. Despite the discovery of numerous materials capable of generating significant SOTs, achieving efficient and deterministic field-free switching of perpendicular magnetization remains a critical challenge, which is essential for the practical deployment of SOT in high-density magnetic memories. This review highlights recent progress in controlling SOTs through innovative materials design, encompassing strategies such as strain engineering of the spin Hall angle, interfacial engineering of the spin transmissivity and topological surface states, and symmetry engineering to achieve deterministic field-free switching of perpendicular magnetization. By exploring these effective methods for manipulating SOTs, this review aims to lay the groundwork for the development of optimized spintronics devices and applications.
自旋轨道力矩(SOT)为磁化的电操纵提供了一种节能方法,对下一代信息存储和处理设备至关重要。自旋轨道力矩可通过各种机制产生,如自旋霍尔效应、拉什巴-爱德斯坦效应、轨道霍尔效应、磁子和自旋交换。与自旋转移力矩(STT)器件相比,基于 SOT 的器件具有潜在的优势,包括功耗低、耐用性强,以及 SOT 生成和激发的适用材料选择范围更广。尽管发现了许多能够产生显著自旋转移力矩的材料,但实现垂直磁化的高效和确定性无磁场切换仍然是一个严峻的挑战,这对于在高密度磁存储器中实际部署自旋转移力矩至关重要。本综述重点介绍通过创新材料设计控制 SOT 的最新进展,包括自旋霍尔角的应变工程、自旋透射率和拓扑表面态的界面工程以及对称性工程等策略,以实现垂直磁化的确定性无磁场切换。本综述旨在通过探讨这些操纵 SOT 的有效方法,为开发优化的自旋电子器件和应用奠定基础。
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引用次数: 0
Enhanced performance and functionality in spintronic sensors 增强自旋电子传感器的性能和功能
Pub Date : 2024-11-06 DOI: 10.1038/s44306-024-00058-9
Diana C. Leitao, Floris J. F. van Riel, Mahmoud Rasly, Pedro D. R. Araujo, Maria Salvador, Elvira Paz, Bert Koopmans
Spintronic sensors are uniquely positioned to deliver the next generation of high-performance magnetic field measurement tools with re-configurable key features. In this perspective article, we focus on giant and tunnel magnetoresistance sensors that exploit changes in the electrical resistance of thin films in response to an external magnetic field. We discuss strategies to address ongoing open challenges to improve operation limits. The goal is to meet current technological needs and thus expand the scope of existing applications. We also propose innovative approaches to design sensors with adaptable characteristics and embedded multifunctionality, aiming to create opportunities for future magnetic sensing applications. These solutions leverage the versatility of spintronic sensors, from the thin-film multilayers that form their building blocks, to device fabrication methods and potential integration with other technologies. The outlook of novel applications spans multiple areas, including electric vehicles, robotics, remote detection, or biomedicine.
自旋电子传感器在提供具有可重新配置关键特性的下一代高性能磁场测量工具方面具有得天独厚的优势。在这篇视角文章中,我们将重点讨论巨磁阻和隧道磁阻传感器,这些传感器利用薄膜电阻的变化对外部磁场做出响应。我们讨论了应对当前挑战的策略,以改善操作极限。我们的目标是满足当前的技术需求,从而扩大现有的应用范围。我们还提出了设计具有适应性特征和嵌入式多功能传感器的创新方法,旨在为未来的磁感应应用创造机会。这些解决方案充分利用了自旋电子传感器的多功能性,从构成其构件的多层薄膜,到设备制造方法以及与其他技术的潜在集成。新型应用前景涵盖多个领域,包括电动汽车、机器人、远程检测或生物医学。
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引用次数: 0
Connecting physics to systems with modular spin-circuits 用模块化自旋电路将物理学与系统联系起来
Pub Date : 2024-11-06 DOI: 10.1038/s44306-024-00059-8
Kemal Selcuk, Saleh Bunaiyan, Nihal Sanjay Singh, Shehrin Sayed, Samiran Ganguly, Giovanni Finocchio, Supriyo Datta, Kerem Y. Camsari
An emerging paradigm in modern electronics is that of CMOS+ $${mathsf{X}}$$ requiring the integration of standard CMOS technology with novel materials and technologies denoted by $${mathsf{X}}$$ . In this context, a crucial challenge is to develop accurate circuit models for $${mathsf{X}}$$ that are compatible with standard models for CMOS-based circuits and systems. In this perspective, we present physics-based, experimentally benchmarked modular circuit models that can be used to evaluate a class of CMOS+ $${mathsf{X}}$$ systems, where $${mathsf{X}}$$ denotes magnetic and spintronic materials and phenomena. This class of materials is particularly challenging because they go beyond conventional charge-based phenomena and involve the spin degree of freedom which involves non-trivial quantum effects. Starting from density matrices—the central quantity in quantum transport—using well-defined approximations, it is possible to obtain spin-circuits that generalize ordinary circuit theory to 4-component currents and voltages (1 for charge and 3 for spin). With step-by-step examples that progressively become more complex, we illustrate how the spin-circuit approach can be used to start from the physics of magnetism and spintronics to enable accurate system-level evaluations. We believe the core approach can be extended to include other quantum degrees of freedom like valley and pseudospins starting from corresponding density matrices.
现代电子学的一个新兴范式是 CMOS+ $${mathsf{X}}$,要求将标准 CMOS 技术与新型材料和技术(以 $${mathsf{X}}$ 表示)相集成。 在这种情况下,一个关键的挑战是为 $${mathsf{X}}$ 开发与基于 CMOS 电路和系统的标准模型兼容的精确电路模型。从这个角度出发,我们提出了基于物理学、以实验为基准的模块化电路模型,可用于评估一类 CMOS+ $${mathsf{X}}$ 系统,其中 $${mathsf{X}}$ 表示磁性和自旋电子材料及现象。这一类材料特别具有挑战性,因为它们超越了传统的电荷现象,涉及自旋自由度,而自旋自由度涉及非三维量子效应。从密度矩阵--量子传输中的核心量--开始,利用定义明确的近似值,可以获得自旋电路,将普通电路理论推广到 4 分量电流和电压(1 分量电荷,3 分量自旋)。通过逐步变得更加复杂的实例,我们说明了如何利用自旋电路方法从磁学和自旋电子学的物理学出发,实现精确的系统级评估。我们相信,这种核心方法可以扩展到其他量子自由度,如从相应的密度矩阵出发的谷和伪自旋。
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引用次数: 0
The mysterious magnetic ground state of Ba14MnBi11 is likely self-doped and altermagnetic Ba14MnBi11 的神秘磁基态可能是自掺杂和变磁性的
Pub Date : 2024-10-26 DOI: 10.1038/s44306-024-00056-x
Po-Hao Chang, Igor I. Mazin
Magnetism in the Zintl compound Ba14MnBi11 is rather poorly understood. Experimental claims are largely inconsistent with ab initio calculations, much beyond typical errors of the latter. We revisit this old problem, assuming that the root of the problem may be in nonstoichiometry of existing samples. Our key finding is that the magnetic ground state is indeed very susceptible to charge doping (band filling). Calculations for stoichiometric Ba14MnBi11 give a rather stable ferromagnetic metallic state, in agreement with previous publications. However, by adding exactly one electron per Mn, the system becomes semiconducting as expected, and becomes weakly antiferromagnetic (AF). On the other hand, upon small amount of hole doping, the system transitions to a special type of AF state known as altermagnetism. Furthermore, hole and electron doping-induced phase transitions result from different underlying mechanisms, influencing different exchange pathways. We propose that the inconsistency between experiment and theory is not a failure of the latter, but results from a nontrivial ramification of nonstoichiometry. The possibility of doping-stabilized altermagnetism is exciting.
人们对 Zintl 化合物 Ba14MnBi11 的磁性了解甚少。实验结果在很大程度上与 ab initio 计算结果不一致,远远超出了后者的典型误差。我们重新审视了这个老问题,假设问题的根源可能在于现有样品的非化学计量。我们的主要发现是,磁基态确实非常容易受到电荷掺杂(带填充)的影响。通过计算化学计量 Ba14MnBi11,可以得到相当稳定的铁磁金属态,这与之前发表的文章一致。然而,当每锰恰好加入一个电子时,该体系就会如预期的那样成为半导体,并变成弱反铁磁性(AF)。另一方面,当掺入少量空穴时,体系会过渡到一种特殊的反铁磁性(AF)状态,即所谓的 "变磁"(altermagnetism)。此外,空穴掺杂和电子掺杂诱导的相变产生于不同的基本机制,影响着不同的交换途径。我们提出,实验与理论之间的不一致并不是理论的失败,而是由于非化学计量学的非微不足道的衍生物造成的。掺杂稳定变磁性的可能性令人兴奋。
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引用次数: 0
Communicating with magnons 与磁石交流
Pub Date : 2024-10-14 DOI: 10.1038/s44306-024-00060-1
Qiming Shao
Increasing the bandwidth of existing optical fiber networks is vital as society’s appetite for information grows. This Editorial presents a spintronics-based solution in the context of recent research findings.
随着社会对信息的需求日益增长,提高现有光纤网络的带宽至关重要。本社论结合最新研究成果,介绍一种基于自旋电子学的解决方案。
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引用次数: 0
Absence of magnetic order in RuO2: insights from μSR spectroscopy and neutron diffraction RuO2 中的磁序缺失:μSR 光谱和中子衍射的启示
Pub Date : 2024-10-05 DOI: 10.1038/s44306-024-00055-y
Philipp Keßler, Laura Garcia-Gassull, Andreas Suter, Thomas Prokscha, Zaher Salman, Dmitry Khalyavin, Pascal Manuel, Fabio Orlandi, Igor I. Mazin, Roser Valentí, Simon Moser
Altermagnets are a novel class of magnetic materials, where magnetic order is staggered both in coordinate and momentum space. The metallic rutile oxide RuO2, long believed to be a textbook Pauli paramagnet, recently emerged as a putative workhorse altermagnet when resonant X-ray and neutron scattering studies reported nonzero magnetic moments and long-range collinear order. While some experiments seem consistent with altermagnetism, magnetic order in RuO2 remains controversial. We show that RuO2 is nonmagnetic, both in bulk and thin film. Muon spectroscopy complemented by density-functional theory finds at most 1.14 × 10−4 μB/Ru in bulk and at most 7.5 × 10−4 μB/Ru in 11 nm epitaxial films, at our spectrometers’ detection limit, and dramatically smaller than previously reported neutron results that were used to rationalize altermagnetic behavior. Our own neutron diffraction measurements on RuO2 single crystals identify multiple scattering as the source for the false signal in earlier studies.
变磁体是一类新型磁性材料,其磁序在坐标空间和动量空间都是交错的。金属金红石氧化物 RuO2 长期以来一直被认为是教科书式的保利旁磁体,最近,当共振 X 射线和中子散射研究报告了非零磁矩和长程共线阶时,它被认为是一种潜在的工作母体变磁体。虽然一些实验似乎与变磁性相一致,但 RuO2 中的磁序仍然存在争议。我们的研究表明,RuO2 在块体和薄膜中都是非磁性的。μ介子光谱法辅以密度函数理论发现,在块体中最多为 1.14 × 10-4 μB/Ru,而在 11 纳米的外延薄膜中最多为 7.5 × 10-4 μB/Ru,达到了我们光谱仪的检测极限,而且大大小于之前报道的用于合理解释变磁性的中子结果。我们自己对 RuO2 单晶体进行的中子衍射测量发现,多重散射是早期研究中出现错误信号的原因。
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引用次数: 0
Recent progress in spin-orbit torque magnetic random-access memory 自旋轨道力矩磁随机存取存储器的最新进展
Pub Date : 2024-10-01 DOI: 10.1038/s44306-024-00044-1
V. D. Nguyen, S. Rao, K. Wostyn, S. Couet
Spin-orbit torque magnetic random-access memory (SOT-MRAM) offers promise for fast operation and high endurance but faces challenges such as low switching current, reliable field free switching, and back-end of line manufacturing processes. We review recent advancements in perpendicular SOT-MRAM devices, emphasizing on material developments to enhance charge-spin conversion efficiency and large-scale device integration strategies. We also discuss the remaining challenges in achieving a single device with low switching current, reliable field free switching to unlock the full potential of SOT-MRAM technology.
自旋轨道力矩磁性随机存取存储器(SOT-MRAM)有望实现快速运行和高耐用性,但也面临着低开关电流、可靠的无场开关和生产线后端制造工艺等挑战。我们回顾了垂直 SOT-MRAM 器件的最新进展,重点介绍了提高电荷-自旋转换效率的材料开发和大规模器件集成战略。我们还讨论了在实现具有低开关电流和可靠的无场开关的单一器件方面仍然存在的挑战,以充分释放 SOT-MRAM 技术的潜力。
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引用次数: 0
Mott materials: unsuccessful metals with a bright future 莫特材料:前途光明的不成功金属
Pub Date : 2024-10-01 DOI: 10.1038/s44306-024-00047-y
Alessandra Milloch, Michele Fabrizio, Claudio Giannetti
Achieving the full understanding and control of the insulator-to-metal transition in Mott materials is key for the next generation of electronics devices, with applications ranging from ultrafast transistors, volatile and non-volatile memories and artificial neurons for neuromorphic computing. In this work, we will review the state-of-the-art knowledge of the Mott transition, with specific focus on materials of relevance for actual devices, such as vanadium and other transition metal oxides and chalcogenides. We will emphasize the current attempts in controlling the Mott switching dynamics via the application of external voltage and electromagnetic pulses and we will discuss how the recent advances in time- and space-resolved techniques are boosting the comprehension of the firing process. The nature of the voltage/light-induced Mott switching is inherently different from what is attainable by the slower variation of thermodynamic parameters, thus offering promising routes to achieving the reversible and ultrafast control of conductivity and magnetism in Mott nanodevices.
全面了解和控制莫特材料中从绝缘体到金属的转变是下一代电子器件的关键,其应用范围包括超快晶体管、易失和非易失存储器以及用于神经形态计算的人工神经元。在这项工作中,我们将回顾莫特转变的最新知识,特别关注与实际设备相关的材料,如钒和其他过渡金属氧化物和瑀。我们将强调目前通过施加外部电压和电磁脉冲来控制莫特转换动态的尝试,并将讨论时间和空间分辨技术的最新进展如何促进对点火过程的理解。电压/光诱导莫特开关的性质本质上不同于热力学参数的缓慢变化,因此为在莫特纳米器件中实现导电性和磁性的可逆和超快控制提供了前景广阔的途径。
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引用次数: 0
Hybrid magnon-phonon crystals 混合镁-声子晶体
Pub Date : 2024-09-04 DOI: 10.1038/s44306-024-00052-1
Liyang Liao, Jiacheng Liu, Jorge Puebla, Qiming Shao, Yoshichika Otani
Magnons and phonons are engineered in artificial lattices with tunable modes and band dispersions. Recent advance in magnon-phonon coupling shined a light on combining magnonic and phononic crystals as hybrid magnon-phonon crystals, benefit from the tunable magnon-phonon coupling, the time-reversal symmetry breaking of magnons, and the long lifetime of phonons. This perspective summarizes lattice-based mutual control of magnons and phonons, and proposes the opportunities provided by the hybrid magnon-phonon crystals.
人工晶格中的磁子和声子具有可调的模式和频带色散。最近在磁子-声子耦合方面取得的进展,使人们看到了将磁子晶体和声子晶体结合为混合磁子-声子晶体的曙光,这得益于可调谐的磁子-声子耦合、磁子的时间逆对称破缺和声子的长寿命。这一观点总结了基于晶格的磁子和声子相互控制,并提出了混合磁子-声子晶体提供的机遇。
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引用次数: 0
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npj Spintronics
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