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Analysis of Status Fourteen Hours after All Power Loss at the Fukushima Daiichi Nuclear Power Plant Unit 1 福岛第一核电站1号机组全部断电14小时后的状况分析
Q4 Engineering Pub Date : 2021-01-01 DOI: 10.3327/taesj.j21.006
Tsuyoshi Matsuoka
The author independently conducted a detailed analysis of plant conditions, based on a new meltdown process, during the 14 hours after all power loss at the Fukushima Daiichi Nuclear Power Plant Unit 1. After 3 : 30 PM on March 11, 2011, all power loss caused reactor core cooling function loss and the vaporization of water in the reactor vessel ( RPV ) , and the RPV was filled with high-temperature hydrogen gas generated by decay heat and Zr - H 2 O reactions. The reactor core melted and the periph-eral stainless-steel structures and nuclear vessel walls were heated by the radiation energy of decay heat. Then, the shrouds and other components near the reactor core started melting and the wall temperature of the RPV was raised. Along with the wall temperature rising to nearly 650 ℃ , the aluminum insulation near the wall started melting ( aluminum melting point, about 650 ℃) . The heat from the collapsed insulation caused the superheated state of the containment pressure and temperature of 0.84 MPa and 400 ℃ , respectively, around 3 AM from the saturated state of 0.6 MPa around 1 AM on March 12. After that, the containment vessel was depressurized gradually and kept under stable cooling 14 hours after all power loss, for the time from 4 to 6 AM. By the first water injection to the reac tor core at 4 AM, radioactivity release increased slightly and the containment pressure was stable. However, the situation changed significantly after continuous water injection to the reactor core start ed at around 6 AM. The water injection into the high-temperature reactor core generated film boiling ( poor heat transfer ) and good reactor core cooling was no longer available; thus, increased heating by the Zr - H 2 O reactions started. The results of the author’s analysis showed good consistency with the measured reactor pressure, containment pressure, containment temperature and radioactivity near the main gate. Although decay heat cannot be decreased intentionally, the occurrence of the Zr - H 2 O reactions can be inhibited. It is proposed that the best way to mitigate the effects of a meltdown is to stop water injection to the core after detecting the initiation of film boiling or inferring that the fuel rods are not covered with water.
作者在福岛第一核电站1号机组全部断电后的14小时内,根据一个新的熔毁过程,独立地对电站状况进行了详细的分析。2011年3月11日下午3时30分以后,全部功率损失导致堆芯冷却功能丧失,反应堆容器(RPV)内的水蒸发,RPV内充满衰变热和Zr - h2o反应产生的高温氢气。反应堆堆芯熔化,外围不锈钢结构和核容器壁被衰变热的辐射能加热。然后,堆芯附近的罩壳和其他部件开始熔化,RPV的壁温升高。随着壁面温度上升到接近650℃时,靠近壁面的保温铝开始熔化(铝的熔点,约650℃)。3月12日凌晨1点左右,隔热层坍塌产生的热量使安全壳压力和温度从0.6 MPa的饱和状态分别在凌晨3点左右达到0.84 MPa和400℃的过热状态。在此之后,安全壳逐渐减压,并在所有断电后的14小时内保持稳定冷却,时间为上午4点至6点。上午4点第一次向堆芯注水时,放射性释放略有增加,安全壳压力稳定。然而,在早上6点左右开始向反应堆堆芯持续注水后,情况发生了显著变化。高温堆芯注水产生的膜沸腾(传热差)和良好的堆芯冷却不再有效;因此,Zr - h2o反应开始升温。作者的分析结果与主闸口附近测量到的反应堆压力、安全壳压力、安全壳温度和放射性具有良好的一致性。虽然不能有意地降低衰变热,但可以抑制Zr - h2o反应的发生。建议减轻熔毁影响的最佳方法是在检测到膜沸腾的开始或推断燃料棒没有被水覆盖后停止向堆芯注水。
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引用次数: 0
Development of Element Assignment Program Based on Feature Quantity Extraction Method from Emission Spectra of Glow-Discharged Atomic Vapor Source Obtained with Czerny–Turner Spectrometer 基于特征量提取方法的发光原子蒸汽源发射光谱元素分配程序的开发
Q4 Engineering Pub Date : 2021-01-01 DOI: 10.3327/taesj.j20.012
D. Ishikawa, N. Oku, S. Hasegawa
To analyze the radioactive wastes produced by the accident at the Fukushima Daiichi Nuclear Power Plant, we have been developing a laser absorption and emission spectroscopic system for sample screening. By the sputtering technique, neutral atomic vapor can be produced from a solid sample even if the chemical forms of the samples are complex. This system utilizes a DC glow-discharged hollow cathode atomic source that does not require an extensive chemical pretreatment. Although it is possible to perform emission spectroscopy for multi-element simultaneous analysis to clarify the ele-ments of samples with this system, it takes much time to assign complex peaks of the samples. A program was developed for the rapid assignment of the emission spectra. We utilized a Czerny – Turner spectrometer, which has a low resolution power. The program written in Python could assign the large emission peaks because of the ease of signal discrimination.
为了分析福岛第一核电站事故产生的放射性废物,我们一直在开发用于样品筛选的激光吸收和发射光谱系统。通过溅射技术,即使样品的化学形态很复杂,也可以从固体样品中产生中性原子蒸汽。该系统采用直流辉光放电空心阴极原子源,不需要广泛的化学预处理。虽然利用该系统可以进行多元素同时分析的发射光谱,以澄清样品中的元素,但需要花费大量时间来分配样品的复杂峰。开发了一个快速分配发射光谱的程序。我们使用了低分辨率的切尔尼-特纳光谱仪。由于易于识别信号,用Python编写的程序可以分配较大的发射峰。
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引用次数: 0
Practical Method of Risk-Informed Decision Making in Nuclear Power Plant Operation and Its Safety Effect 核电厂运行风险知情决策的实用方法及其安全效果
Q4 Engineering Pub Date : 2021-01-01 DOI: 10.3327/TAESJ.J19.029
Yutaka Shikami
Before the Fukushima-Daiichi Accident, Japanese nuclear power plants ( NPPs ) were utilized with a capacity factor of around 70 % , 20 % lower than the US capacity factor of around 90 % , which is a consequence of Japanese NPPs being operated with a shorter fuel cycle and longer outage period. One reason for this situation is that Japanese decision making is strongly focused on equipment reli-ability. In a typical pressurized-water reactor, however, core damage frequency ( CDF ) during refueling outage is higher than that during operation, that is, a short fuel cycle could possibly increase the total CDF of NPPs. In this paper, a decision-making rule using an index representing CDF par power generation is firstly proposed. Secondly, using this rule, a decision process is simulated to optimize the fuel cycle and refueling outage period while showing the effects on CDF reduction in each plant. Thirdly, by applying this decision process to all Japanese NPPs, the total CDF reduction in Japan is indicated. This simulation shows that the change of decision-making rule will bring about an 18 % CDF reduction or 16 % increase in power generation in total in Japan. At the same time, each NPP gains strong incentive to improve its own safety because this new rule permits a higher capacity factor operation only for the NPPs that are safer than the average.
在福岛第一核电站事故发生之前,日本核电站的容量系数约为70%,比美国的容量系数约为90%低20%,这是日本核电站燃料循环较短、停运时间较长的结果。造成这种情况的一个原因是,日本的决策非常注重设备的可靠性。然而,在典型的压水堆中,换料停堆期间堆芯损坏频率(CDF)高于运行期间,即短的燃料循环可能会增加核电厂的总CDF。本文首先提出了一种用指标表示CDF平价发电量的决策规则。其次,利用该规则,模拟了优化燃料循环和停运周期的决策过程,并展示了对各电厂减少碳排放的影响。第三,通过将这一决策过程应用于所有日本核电站,可以指出日本的清洁发展基金减少总额。模拟结果表明,决策规则的改变将使日本减少18%的CDF或增加16%的总发电量。同时,每个核电站都有强烈的动力来提高自身的安全性,因为新规则只允许比平均安全水平更高的核电站运行容量系数。
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引用次数: 0
Development of evaluation method for diffusion and filtration behavior of colloid in compacted bentonites using dendrimers 用树状大分子评价膨润土中胶体的扩散和过滤行为
Q4 Engineering Pub Date : 2021-01-01 DOI: 10.3327/TAESJ.J20.001
T. Endo, Y. Tachi, T. Ishidera, M. Terashima
2021 ) A new method of evaluating colloid diffusion and filtration in compacted bentonites using den drimers was developed. Polyamidoamine ( PAMAM ) dendrimers with sizes of 5.7 and 7.2 nm were chosen as diffusion probes owing to their high monodispersity and well-defined molecular structure. The diffusion and filtration behaviors were investigated by a through-diffusion experiment in benton ite compacted to 0.8 Mg / m 3 and saturated with 0.005–0.5 mol / L NaCl. The breakthrough curves were observed under all conditions, demonstrating that dendrimers could diffuse through the pore network in compacted bentonite. The effective diffusivity ( D e ) and filtration ratio ( R f ) of dendrimers were de-termined from the breakthrough curves and the depth profiles in compacted bentonite, respectively. The D e values of the negatively charged dendrimers increased when porewater salinity increased and dendrimer size decreased owing to the anion exclusion effect on negatively charged clay surfaces. The R f values increased when porewater salinity decreased and dendrimer size increased, demonstrating that significant fractions of dendrimers were filtered by the narrow pores in the complex pore net -works. The results of this study confirm the validity of the evaluation method using dendrimers and the importance of the need for further investigation under various conditions to understand the fac tors controlling colloid diffusion and filtration and their relationships with the microstructure in com pacted bentonite.
2021)开发了一种利用孔洞驱动剂评价膨润土中胶体扩散和过滤的新方法。选用尺寸为5.7 nm和7.2 nm的聚胺胺(PAMAM)树状大分子作为扩散探针,因为其具有较高的单分散性和清晰的分子结构。通过透扩散实验,研究了膨润土在压实至0.8 Mg / m 3、0.005 ~ 0.5 mol / L NaCl饱和条件下的扩散和过滤行为。在所有条件下观察到的突破曲线表明,树状大分子可以在压实的膨润土中通过孔隙网络扩散。树状大分子的有效扩散系数(D e)和过滤比(R f)分别由压实膨润土的穿透曲线和深度剖面确定。带负电荷的树状大分子的D e值随着孔隙水矿化度的增加而增加,并且由于带负电荷的粘土表面的阴离子排斥作用,树状大分子的尺寸减小。随着孔隙水矿化度的降低和枝状大分子尺寸的增大,R - f值增大,表明在复杂的孔隙网络中,相当一部分枝状大分子被狭窄的孔隙过滤了。本研究的结果证实了树状大分子评价方法的有效性,以及在不同条件下进一步研究控制胶体扩散和过滤的因素及其与膨润土微观结构的关系的重要性。
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引用次数: 0
New approach for describing reactor and containment pressure change after loss of core cooling at Fukushima meltdown accident 描述福岛堆芯冷却失效后反应堆和安全壳压力变化的新方法
Q4 Engineering Pub Date : 2021-01-01 DOI: 10.3327/taesj.j20.033
Tsuyoshi Matsuoka
The purpose of this comment is to clarify the whole history of reactor and containment pressure change during the Fukushima meltdown accident. It is based on a new approach for film boiling, which is sustained after the Zr – H 2 O reaction. As the reaction rate is proportional to the reactor or containment vessel pressure under film boiling, it increases rapidly and stops abruptly while sustaining film boiling. The containment vessel pressure change consists of three phases, namely, pressurization, holding a high pressure and depressurization. The containment vessel is pressurized with H 2 gas and steam produced by the Zr – H 2 O reaction and depressurized by heat removal by heatsinks such as the containment vessel wall and inner concrete after the reaction stops. The high pressure between these pressure changes is sustained by balancing the amount of H 2 gas produced by the reaction and that of gas leaking from the gap of the top hat of the containment vessel. The amount of core decay heat is large, but the change of this is negligible. Thus, pressurization is calculated from the amounts of H 2 gas and steam produced by the Zr – H 2 O reaction. The amount removed by the heatsink balances with that produced by the reaction during the high-pressure phase. Depressurization occurs after the reac tion is over, so the reaction heat rate can be calculated from the heat removal rate of the heatsink, which is equal to the condensation rate during depressurization. The rate of gas leakage can be calcu lated from the reaction rate. It is very important that the reaction rate was slow owing to the insuffi cient steam supply, as the melted core in the Fukushima accident was covered with H 2 gas and steam at a pressure of 0.8 MPa or lower. This is different from the rate ( at approximately 7 MPa ) in the Three Mile Island accident, as the specific volume of steam at 0.8 MPa is ten times larger than that at 7 MPa. The calculation results based on this assumption show that almost all the Zr in each core of Units 1, 2 and 3 reacted with water. The location of a small penetration hole produced by the contact of the high-temperature H 2 gas with the suppression chamber wall, is estimated in Unit 2.
这个评论的目的是澄清整个历史的反应堆和安全壳压力变化在福岛事故。它是基于一种新的膜沸腾方法,这种方法是在Zr - h2o反应后持续的。在膜沸腾状态下,反应速率与反应器或容器压力成正比,在维持膜沸腾状态下,反应速率迅速增加,并突然停止。安全壳压力变化包括增压、保高压和降压三个阶段。安全壳由Zr - h2o反应产生的h2气体和蒸汽加压,反应停止后由诸如安全壳壁和内部混凝土等散热器散热减压。这些压力变化之间的高压是通过平衡反应产生的h2气体的量和从安全壳顶帽间隙泄漏的气体的量来维持的。堆芯衰变热的量很大,但其变化可以忽略不计。因此,压力是由Zr - h2o反应产生的h2气体和蒸汽的量来计算的。由散热器去除的量与高压阶段反应产生的量相平衡。减压是在反应结束后发生的,所以反应的热速率可以通过散热器的排热速率来计算,它等于减压过程中的冷凝速率。气体泄漏率可由反应速率计算出来。很重要的一点是,由于蒸汽供应不足,反应速度较慢,因为福岛事故中熔化的堆芯被压力为0.8 MPa或更低的h2气体和蒸汽覆盖。这与三里岛事故中的速率(约7兆帕)不同,因为0.8兆帕时的蒸汽比容是7兆帕时的十倍。基于这一假设的计算结果表明,1、2、3号机组各堆芯中Zr几乎全部与水发生反应。在单元2中估计了高温h2气体与抑制室壁接触产生的小穿透孔的位置。
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引用次数: 0
Study on solubility of cesium iodide and cesium molybdate in water at around room temperature 室温下碘化铯和钼酸铯在水中溶解度的研究
Q4 Engineering Pub Date : 2021-01-01 DOI: 10.3327/taesj.j20.037
Jumpei Imoto, K. Nakajima, M. Osaka
Some of the Cs inside the Fukushima Daiichi Nuclear Power Station would be deposited in chemical forms such as CsI and Cs 2 MoO 4 . Since Cs compounds are generally water-soluble, it is pre-dicted that the migration of Cs through the aqueous phase occurs in the long term. Knowledge of the solubility in water is required as basic data for such migration behavior evaluation. Therefore, this study was conducted to investigate the dissolution properties of CsI and Cs 2 MoO 4 in water at 20 ℉ and 25 ℉ . The solubilities of CsI at 25 ℉ calculated using thermodynamic data and the Pitzer ion interaction model were in good agreement with the literature value. It was found that the literature value of CsI at around room temperature is highly reliable. The experimental value of CsI at 20 ℃ obtained by the OECD test guideline 105 flask method ( test guideline ) was also in good agreement with the literature value. The measured solubility of Cs 2 MoO 4 was 256.8 ± 12.7 ( g / 100 g H 2 O ) at 20 ℃ using the test guideline. This measured solubility of Cs 2 MoO 4 was found to be comparable to those of other alkaline molybdates and considered to be more reliable than the literature value.
福岛第一核电站(Fukushima Daiichi Nuclear Power Station)内部的一些铯将以CsI和c2mo_4等化学形式沉积。由于Cs化合物通常是水溶性的,因此可以预测Cs在水相中的迁移是长期发生的。了解在水中的溶解度是评价这种迁移行为的基础数据。因此,本文研究了CsI和c2moo4在20℉和25℉水中的溶解特性。利用热力学数据和Pitzer离子相互作用模型计算的25℉时CsI的溶解度与文献值吻合较好。研究发现,常温前后CsI的文献值具有较高的可靠性。采用OECD试验指南105烧瓶法(试验指南)得到的20℃下CsI的实验值也与文献值吻合较好。在20℃条件下,c2moo4的溶解度为256.8±12.7 (g / 100 g h2o)。c2moo4的溶解度与其他碱性钼酸盐的溶解度相当,比文献值更可靠。
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引用次数: 0
Method of Applying Graded Approach in Corrective Action Program and Its Safety Effects 分级法应用于纠正措施方案的方法及其安全效果
Q4 Engineering Pub Date : 2021-01-01 DOI: 10.3327/TAESJ.J19.025
Yutaka Shikami
increase. the significant risk issues. First the gap between the significance used in traditional Japanese CAP and risk-informed significance is clarified in this paper. Second, a CAP process model with two conditions of potential safety issues depending on whether the cause is removed or not is prepared. This model can explain how the CAP works to suppress the recurrence of safety issues. Third, using this model, the trend that the CDF is increased by the safety issues is parametrically simulated. Simulation results show that the CAP using risk-informed significance can reduce the CDF increase by 40 % over 20 years. For the NPPs that have long been using an inappropriate significance scale, the application of risk-informed significance in CAP is one of the most effective actions for sup pressing future CDF.
增加。重大风险问题。首先,本文澄清了日本传统CAP中使用的意义与风险知情意义之间的差距。其次,根据原因是否被消除,准备了具有潜在安全问题两种条件的CAP过程模型。该模型可以解释CAP如何抑制安全问题的再次发生。第三,利用该模型,参数化模拟了CDF随安全问题增加的趋势。模拟结果表明,采用风险知情显著性的CAP可以使CDF在20年内减少40%的增长。对于长期以来一直使用不适当的显著性量表的核电站来说,在CAP中应用风险知情显著性是支持未来CDF的最有效措施之一。
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引用次数: 0
Public Attitudes towards Local Agreement over the Restart of Nuclear Power Plants: A Questionnaire Survey on the Case of Hamaoka 公众对重启核电站地方协议的态度:以滨冈县为例的问卷调查
Q4 Engineering Pub Date : 2021-01-01 DOI: 10.3327/taesj.j20.006
Tomoyuki Tatsumi, T. Nakazawa
Not just whether nuclear power stations should be restarted, but how local agreement over the restart should be achieved has been controversial issues in Japan since the Fukushima Nuclear Di-saster. In this paper, public attitudes towards local agreement in the case of Hamaoka Nuclear Power Plants are explored with a postal questionnaire survey in Shizuoka prefecture. Through descriptive statistics and factor analysis, the study shows that extending the “local” scale and judgement by ordi-nary citizens is given more support than the conventional local agreement process. Factor analysis reveals three factors behind respondents’ attitudes towards local agreement: “conventional decision-makers”, “narrow localism” and “national interests”. The analysis of the factor scores reveals that attitudes towards local agreement differ depending on attitudes towards the restart of the plant and the prefectural referendum, as well as generation, while no significant difference is found among gen ders and residential areas excluding the second factor. By clarifying the public attitudes towards how local agreement should be made, this study makes a significant step toward the design of a socially more agreeable local agreement.
自福岛核灾难以来,不仅是核电站是否应该重启,而且应该如何就重启达成地方协议,一直是日本有争议的问题。本文以静冈县为研究对象,以邮政问卷调查的方式,探讨公众对滨冈核电站地方协议的态度。通过描述性统计和因子分析,研究表明,扩大“地方”尺度和普通公民的判断比传统的地方协议过程更受支持。因子分析揭示了受访者对地方协议态度背后的三个因素:“传统决策者”、“狭隘的地方主义”和“国家利益”。对因素得分的分析显示,对地方协议的态度取决于对核电站重启和县公投的态度,以及世代,而在性别和住宅区之间没有发现显著差异,排除第二个因素。通过澄清公众对如何制定地方协议的态度,本研究朝着设计社会上更容易接受的地方协议迈出了重要的一步。
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引用次数: 1
Validation of Photoneutron Energy Distributions in Shielding Calculation of the Medical Linac Room 医用直线室屏蔽计算中光子-中子能量分布的验证
Q4 Engineering Pub Date : 2021-01-01 DOI: 10.3327/taesj.j20.016
K. Kosako
It is necessary to consider the effect of photoneutrons produced by photonuclear reactions in the shielding calculation of a medical linac room with incident electron energies greater than 10 MeV. For photonuclear reaction files, the validation of photoneutron energy distributions has not been reported. We compared the evaluated data of photoneutron energy distributions in LA150 and JENDL / PD-2016.1 with the experimental data for 11 nuclides taken from the EXFOR database. For dominant shielding materials of linac, we validated the tendency of energy distributions by comparing the experimental data of neighborhood nuclides. Consequently, we found problems in the evaluations of the photoneutron energy distributions of the photonuclear reaction files.
在入射电子能量大于10兆电子伏特的医用直线室的屏蔽计算中,必须考虑光子核反应产生的光子中子的影响。对于光子核反应文件,光子中子能量分布的验证尚未见报道。我们将LA150和JENDL / PD-2016.1中光子中子能量分布的评估数据与EXFOR数据库中11种核素的实验数据进行了比较。对于直线加速器的优势屏蔽材料,我们通过比较邻域核素的实验数据验证了能量分布的趋势。因此,我们发现在评估光子核反应文件的光子中子能量分布时存在问题。
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引用次数: 0
Mass Discrimination Effect in Isotope Ratio Measurement of Barium by Triple-Quadrupole Inductively Coupled Plasma-Mass Spectrometry: Estimation of Mass Bias Coefficient for Isotopic Analysis of Radioactive Cesium Nuclides 三重四极电感耦合等离子体质谱法测量钡同位素比值的质量分辨效应:放射性铯核素同位素分析的质量偏倚系数估算
Q4 Engineering Pub Date : 2020-01-01 DOI: 10.3327/taesj.j19.030
Hiroki Shibahara, Mami Yuki, Yuki Ohishi, Yasutaka Takeuchi, Z. Yoshida
The mass discrimination effect in the isotope analyses of barium isotopes with natural abundance, from Ba-130 to Ba-138, was investigated by triple-quadrupole inductively coupled plasmamass spectrometry (ICP-QQQ). The mass bias coefficients for Ba isotopes, denoted by ε(Ba), were determined from the slope of a linear relationship between the atomic mass differences and the ratios of ion count rates for a given isotope pair experimentally determined and calculated from natural abundances. The effect of the addition of a collision-reaction cell (CRC) gas such as helium, hydrogen, nitrous oxide, or carbon dioxide on ε(Ba) was examined. Large ε(Ba) values were observed in the case of Heor H2-CRC gas, and the values were from +0.8 to +1.7% per atomic mass unit. On the other hand, ε(Ba) observed with CRC gasses containing N2O or CO2 was relatively small and below +0.3% per atomic mass unit. In addition, the dependence of the energy discrimination potential (ED) applied between the CRC and the second quadrupole mass separator of ICP-QQQ on ε(Ba) was investigated. Finally, the analytical mass bias coefficient of the radioactive cesium nuclides Cs, Cs, and Cs, ε(Cs), was discussed for ε(Ba) in the same mass range as that of Ba isotopes.
采用三重四极电感耦合等离子体质谱法(ICP-QQQ)研究了天然丰度为Ba-130 ~ Ba-138的钡同位素同位素分析中的质量分辨效应。Ba同位素的质量偏差系数用ε(Ba)表示,由实验测定和自然丰度计算的给定同位素对的原子质量差与离子计数率比值之间的线性关系的斜率确定。研究了碰撞反应电池(CRC)气体(如氦、氢、氧化亚氮或二氧化碳)的加入对ε(Ba)的影响。Heor H2-CRC气体的ε(Ba)值较大,为+0.8 ~ +1.7% /原子质量单位。另一方面,在含有N2O或CO2的CRC气体中观测到的ε(Ba)相对较小,每原子质量单位低于+0.3%。此外,还研究了ICP-QQQ的CRC与第二四极质量分离器之间的能量鉴别势(ED)对ε(Ba)的依赖关系。最后,讨论了铯放射性核素Cs、Cs和Cs、ε(Cs)在与Ba同位素相同质量范围内的分析质量偏差系数。
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引用次数: 1
期刊
Transactions of the Atomic Energy Society of Japan
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