Pub Date : 2025-12-12DOI: 10.1134/S0021364025608292
M. Yu. Azarkin, M. R. Kirakosyan
In this study, the effect of γ-radiation from typical commercial medical sources based on X-ray tubes and linear accelerators on the electrostatic properties of radiosensitizing gold nanoparticles located in a tissue-like medium has been evaluated numerically using a Monte Carlo simulation in the Geant4 software package. It has been shown that for realistic radiation doses, a significant fraction of gold nanoparticles of up to ~10‒1 can, at least temporarily, change their surface charge sufficiently to convert anionic gold nanoparticles into cationic ones, which can lead to cytotoxic effects.
{"title":"Effect of Ionizing Radiation on the Electrostatic Properties of Gold Nanoparticles","authors":"M. Yu. Azarkin, M. R. Kirakosyan","doi":"10.1134/S0021364025608292","DOIUrl":"10.1134/S0021364025608292","url":null,"abstract":"<p>In this study, the effect of γ-radiation from typical commercial medical sources based on X-ray tubes and linear accelerators on the electrostatic properties of radiosensitizing gold nanoparticles located in a tissue-like medium has been evaluated numerically using a Monte Carlo simulation in the Geant4 software package. It has been shown that for realistic radiation doses, a significant fraction of gold nanoparticles of up to ~10<sup>‒1</sup> can, at least temporarily, change their surface charge sufficiently to convert anionic gold nanoparticles into cationic ones, which can lead to cytotoxic effects.</p>","PeriodicalId":604,"journal":{"name":"JETP Letters","volume":"122 9","pages":"562 - 567"},"PeriodicalIF":1.3,"publicationDate":"2025-12-12","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145730019","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2025-12-04DOI: 10.1134/S0021364025608528
L. L. Losev, V. S. Pazyuk
A physical mechanism of the generation of an ultraviolet resonant dispersive wave in a hollow waveguide is proposed based on a nonlinear phase modulation process with equal group velocities of an optical infrared soliton and an ultraviolet radiation pulse. An analytical expression for the wavelength of the resonant dispersive wave is obtained. Experiments confirming the proposed mechanism are conducted.
{"title":"Features of the Generation of a UV Resonant Dispersive Wave in a Hollow Waveguide","authors":"L. L. Losev, V. S. Pazyuk","doi":"10.1134/S0021364025608528","DOIUrl":"10.1134/S0021364025608528","url":null,"abstract":"<p>A physical mechanism of the generation of an ultraviolet resonant dispersive wave in a hollow waveguide is proposed based on a nonlinear phase modulation process with equal group velocities of an optical infrared soliton and an ultraviolet radiation pulse. An analytical expression for the wavelength of the resonant dispersive wave is obtained. Experiments confirming the proposed mechanism are conducted.</p>","PeriodicalId":604,"journal":{"name":"JETP Letters","volume":"122 8","pages":"486 - 490"},"PeriodicalIF":1.3,"publicationDate":"2025-12-04","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145665981","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2025-12-04DOI: 10.1134/S0021364025607900
A. V. Bogatskaya, Yu. S. Gulina, A. E. Rupasov, E. A. Volkova, A. M. Popov, S. I. Kudryashov
The laser writing of microstructures in the bulk of fused silica exposed to tightly focused laser pulses has been analyzed in detail. The self-consistent simulation of a single laser pulse exposure and the formation of electron–hole plasma together with the experimental data has made it possible to verify the mechanism of plasma self-organization and relate it to the mechanisms of defect accumulation in dense plasma regions under multipulse exposure. The dependence of the parameters of the induced microstructures on the wavelength, duration, energy, and exposure of the laser pulse has been investigated. The role of plasma-electron-induced defocusing effects, as well as the contribution of radiation self-focusing, has been analyzed. The heating of the material by the end of the laser pulse has been estimated.
{"title":"Direct Laser Writing of Subwavelength Microstructures in the Bulk of Fused Silica by Tightly Focused Laser Pulses (Brief Review)","authors":"A. V. Bogatskaya, Yu. S. Gulina, A. E. Rupasov, E. A. Volkova, A. M. Popov, S. I. Kudryashov","doi":"10.1134/S0021364025607900","DOIUrl":"10.1134/S0021364025607900","url":null,"abstract":"<p>The laser writing of microstructures in the bulk of fused silica exposed to tightly focused laser pulses has been analyzed in detail. The self-consistent simulation of a single laser pulse exposure and the formation of electron–hole plasma together with the experimental data has made it possible to verify the mechanism of plasma self-organization and relate it to the mechanisms of defect accumulation in dense plasma regions under multipulse exposure. The dependence of the parameters of the induced microstructures on the wavelength, duration, energy, and exposure of the laser pulse has been investigated. The role of plasma-electron-induced defocusing effects, as well as the contribution of radiation self-focusing, has been analyzed. The heating of the material by the end of the laser pulse has been estimated.</p>","PeriodicalId":604,"journal":{"name":"JETP Letters","volume":"122 8","pages":"507 - 516"},"PeriodicalIF":1.3,"publicationDate":"2025-12-04","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://link.springer.com/content/pdf/10.1134/S0021364025607900.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145665982","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2025-12-04DOI: 10.1134/S002136402560853X
D. A. Myzin, P. V. Borisyuk, K. L. Gubskii, N. V. Didenko, F. A. Korneev, A. P. Kuznetsov, Yu. Yu. Lebedinskii, Zh. M. Nauryzbaev, S. V. Popruzhenko, E. V. Tkalya, E. V. Chubunova, V. A. Shilov
The results of an experiment on the two-photon excitation of exciton states in krypton cryocrystals by the fifth harmonic of 209-nm laser radiation have been presented. It has been shown that the two-photon excitation mechanism allows reaching a density of 1016 cm−3 of free excitons with an excitation energy of ~8.4 eV at a focal radiation intensity of ( approx {{10}^{{11}}}{kern 1pt} ) W/cm2. The observed broad photoluminescence line arising from the relaxation of excited exciton states covers the (3{text{/}}{{2}^{ + }}(8.4{kern 1pt} ;{text{eV}}) to 5{text{/}}{{2}^{ + }}(0.0)) low-energy nuclear isomeric transition in 229Th. Analytical estimates showing that two-photon laser generation of exciton states in noble gas crystals can be used as a new method for the excitation of the nuclear isomeric state of thorium at a pump intensity of ~1011 W/cm2 have been provided.
{"title":"Two-Photon Mechanism of the Excitation of Exciton States in Noble Gas Cryocrystals","authors":"D. A. Myzin, P. V. Borisyuk, K. L. Gubskii, N. V. Didenko, F. A. Korneev, A. P. Kuznetsov, Yu. Yu. Lebedinskii, Zh. M. Nauryzbaev, S. V. Popruzhenko, E. V. Tkalya, E. V. Chubunova, V. A. Shilov","doi":"10.1134/S002136402560853X","DOIUrl":"10.1134/S002136402560853X","url":null,"abstract":"<p>The results of an experiment on the two-photon excitation of exciton states in krypton cryocrystals by the fifth harmonic of 209-nm laser radiation have been presented. It has been shown that the two-photon excitation mechanism allows reaching a density of 10<sup>16</sup> cm<sup>−3</sup> of free excitons with an excitation energy of ~8.4 eV at a focal radiation intensity of <span>( approx {{10}^{{11}}}{kern 1pt} )</span> W/cm<sup>2</sup>. The observed broad photoluminescence line arising from the relaxation of excited exciton states covers the <span>(3{text{/}}{{2}^{ + }}(8.4{kern 1pt} ;{text{eV}}) to 5{text{/}}{{2}^{ + }}(0.0))</span> low-energy nuclear isomeric transition in <sup>229</sup>Th. Analytical estimates showing that two-photon laser generation of exciton states in noble gas crystals can be used as a new method for the excitation of the nuclear isomeric state of thorium at a pump intensity of ~10<sup>11</sup> W/cm<sup>2</sup> have been provided.</p>","PeriodicalId":604,"journal":{"name":"JETP Letters","volume":"122 8","pages":"480 - 485"},"PeriodicalIF":1.3,"publicationDate":"2025-12-04","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145665953","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2025-12-04DOI: 10.1134/S0021364025608322
A. S. Fedorov, V. V. Demidov, M. V. Logunov
Ferrites with the garnet structure containing rare-earth ions have very diverse magnetic properties, in particular due to different Landé g-factors of rare-earth ions and to the splitting of their energy levels under the effect of crystal fields and/or the spin–orbit coupling. Thulium iron garnet Tm3Fe5O12 has a low gyromagnetic ratio. It has been shown in this work that the effective gyromagnetic ratio in such materials can be significantly increased (by a factor of 3–5) by diluting iron with gallium ions. In this case, the gyromagnetic ratio depends on both the content of gallium ions and their distribution between the octahedral and tetrahedral sublattices of the iron garnet. The possibility of achieving a high gyromagnetic ratio in ferrimagnets, which have no magnetic and angular momentum compensation points, has been experimentally discovered and theoretically confirmed for the first time. The gyromagnetic ratio is a key parameter determining the speed of processes in a magnetic spin system, and the results obtained in this work are important for a significant increase in the operation speed of spintronic devices based on ferrimagnetic materials.
{"title":"High Gyromagnetic Ratio in Thulium Iron Garnets","authors":"A. S. Fedorov, V. V. Demidov, M. V. Logunov","doi":"10.1134/S0021364025608322","DOIUrl":"10.1134/S0021364025608322","url":null,"abstract":"<p>Ferrites with the garnet structure containing rare-earth ions have very diverse magnetic properties, in particular due to different Landé <i>g</i>-factors of rare-earth ions and to the splitting of their energy levels under the effect of crystal fields and/or the spin–orbit coupling. Thulium iron garnet Tm<sub>3</sub>Fe<sub>5</sub>O<sub>12</sub> has a low gyromagnetic ratio. It has been shown in this work that the effective gyromagnetic ratio in such materials can be significantly increased (by a factor of 3–5) by diluting iron with gallium ions. In this case, the gyromagnetic ratio depends on both the content of gallium ions and their distribution between the octahedral and tetrahedral sublattices of the iron garnet. The possibility of achieving a high gyromagnetic ratio in ferrimagnets, which have no magnetic and angular momentum compensation points, has been experimentally discovered and theoretically confirmed for the first time. The gyromagnetic ratio is a key parameter determining the speed of processes in a magnetic spin system, and the results obtained in this work are important for a significant increase in the operation speed of spintronic devices based on ferrimagnetic materials.</p>","PeriodicalId":604,"journal":{"name":"JETP Letters","volume":"122 8","pages":"528 - 533"},"PeriodicalIF":1.3,"publicationDate":"2025-12-04","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145665950","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2025-12-04DOI: 10.1134/S0021364025608620
A. S. Belov, A. N. Zelenskii, K. A. Ivshin, M. V. Kulikov, V. A. Lebedev, A. N. Solov’ev, E. M. Syresin, Yu. N. Filatov, V. V. Fimushkin
Sources of polarized protons and deuterons with a storage cell for polarized atoms in a charge-exchange plasma ionizer are considered. A new approach is based on the transverse injection of an atomic beam into a T-shaped storage ionizer cell. This scheme has a number of advantages over sources with the longitudinal injection of the atomic beam into the storage cell, which will help eliminate the limitations inherent in a source with longitudinal injection and significantly reduce the emittance of the polarized ion beam. This should increase the intensity and polarization of the proton and deuteron beams from the source, which is required for obtaining the design luminosity and polarization at the Nuclotron based ion collider facility (NICA, Joint Institute for Nuclear Research).
{"title":"Polarized Ion Sources with a Storage Cell in a Charge-Exchange Plasma Ionizer","authors":"A. S. Belov, A. N. Zelenskii, K. A. Ivshin, M. V. Kulikov, V. A. Lebedev, A. N. Solov’ev, E. M. Syresin, Yu. N. Filatov, V. V. Fimushkin","doi":"10.1134/S0021364025608620","DOIUrl":"10.1134/S0021364025608620","url":null,"abstract":"<p>Sources of polarized protons and deuterons with a storage cell for polarized atoms in a charge-exchange plasma ionizer are considered. A new approach is based on the transverse injection of an atomic beam into a T-shaped storage ionizer cell. This scheme has a number of advantages over sources with the longitudinal injection of the atomic beam into the storage cell, which will help eliminate the limitations inherent in a source with longitudinal injection and significantly reduce the emittance of the polarized ion beam. This should increase the intensity and polarization of the proton and deuteron beams from the source, which is required for obtaining the design luminosity and polarization at the Nuclotron based ion collider facility (NICA, Joint Institute for Nuclear Research).</p>","PeriodicalId":604,"journal":{"name":"JETP Letters","volume":"122 8","pages":"465 - 471"},"PeriodicalIF":1.3,"publicationDate":"2025-12-04","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145665954","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2025-12-04DOI: 10.1134/S0021364025608012
M. V. Dolgopolov, A. S. Chipura
A new physical phenomenon—the dominance of the isotopic mass effect over the strain contribution in cubic crystals, which is manifested in a negative shift of a phonon mode—has been discovered. The universality of the relation ω ~ μ–1/2 for symmetric lattices has been experimentally proven on the example of 3C-SiC. The contrast with a positive shift in anisotropic 4H/6H-SiC proves the key role of crystal symmetry in the competitive separation of the mass effect and strain contributions.
{"title":"Negative Isotopic Shift of the LO Phonon in 3C-SiC: A Universal Mechanism of Mass Effect Dominance in Cubic Crystals","authors":"M. V. Dolgopolov, A. S. Chipura","doi":"10.1134/S0021364025608012","DOIUrl":"10.1134/S0021364025608012","url":null,"abstract":"<p>A new physical phenomenon—the dominance of the isotopic mass effect over the strain contribution in cubic crystals, which is manifested in <i>a negative</i> shift of a phonon mode—has been discovered. The universality of the relation ω ~ μ<sup>–1/2</sup> for symmetric lattices has been experimentally proven on the example of 3C-SiC. The contrast with <i>a positive</i> shift in anisotropic 4H/6H-SiC proves the key role of crystal symmetry in the competitive separation of the mass effect and strain contributions.</p>","PeriodicalId":604,"journal":{"name":"JETP Letters","volume":"122 8","pages":"500 - 506"},"PeriodicalIF":1.3,"publicationDate":"2025-12-04","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://link.springer.com/content/pdf/10.1134/S0021364025608012.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145665952","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2025-12-04DOI: 10.1134/S0021364025608231
E. D. Tsyplakov, Yu. N. Filatov, A. M. Kondratenko, M. A. Kondratenko, S. V. Vinogradov, A. V. Butenko, V. P. Ladygin, V. A. Lebedev, E. M. Syresin, E. A. Butenko
The possibility of conducting experiments with polarized protons at the Nuclotron of the NICA accelerator complex at JINR (Dubna) is under discussion. To preserve polarization during beam acceleration a partial siberian snake is supposed to be used based on dynamic superconducting solenoids developed at JINR. Design options for a solenoid snake in the Nuclotron, both with and without compensation of betatron coupling, have been proposed. Spin orientation control for experiments with an extracted proton beam in a continuous momentum range is achieved with a spin rotator based on longitudinal and transverse magnetic fields, located in the beam transport channel to the external target. At discrete energies, occurring approximately in 0.5 GeV steps, which correspond to integer spin resonances, the polarization direction at internal and external targets can be changed without a spin rotator, applying spin navigators based on weak magnetic fields, located inside the Nuclotron.
{"title":"Preservation and Control of Proton Polarization Direction for Spin Experiments at the Nuclotron/JINR","authors":"E. D. Tsyplakov, Yu. N. Filatov, A. M. Kondratenko, M. A. Kondratenko, S. V. Vinogradov, A. V. Butenko, V. P. Ladygin, V. A. Lebedev, E. M. Syresin, E. A. Butenko","doi":"10.1134/S0021364025608231","DOIUrl":"10.1134/S0021364025608231","url":null,"abstract":"<p>The possibility of conducting experiments with polarized protons at the Nuclotron of the NICA accelerator complex at JINR (Dubna) is under discussion. To preserve polarization during beam acceleration a partial siberian snake is supposed to be used based on dynamic superconducting solenoids developed at JINR. Design options for a solenoid snake in the Nuclotron, both with and without compensation of betatron coupling, have been proposed. Spin orientation control for experiments with an extracted proton beam in a continuous momentum range is achieved with a spin rotator based on longitudinal and transverse magnetic fields, located in the beam transport channel to the external target. At discrete energies, occurring approximately in 0.5 GeV steps, which correspond to integer spin resonances, the polarization direction at internal and external targets can be changed without a spin rotator, applying spin navigators based on weak magnetic fields, located inside the Nuclotron.</p>","PeriodicalId":604,"journal":{"name":"JETP Letters","volume":"122 8","pages":"472 - 479"},"PeriodicalIF":1.3,"publicationDate":"2025-12-04","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://link.springer.com/content/pdf/10.1134/S0021364025608231.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145665980","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2025-12-04DOI: 10.1134/S0021364025607584
V. S. Zakharov, S. V. Zakharov, T. V. Shmeleva
A theoretical model of the experimentally observed collimation of soft radiation from a capillary discharge with hollow electrodes without the use of collimating optics has been proposed. The effect of focusing and channeling of hard radiation with a small difference of the refractive index of the discharge plasma from the vacuum value is possible with its multiple refractions on density disturbances caused by the generation of small-scale waves due to two-stream plasma instabilities. The numerical solution of the eikonal equation shows the possibility of such focusing in a periodic plasma structure. The conditions for focusing of hard radiation in a turbulent plasma structure for almost paraxial rays have been obtained by averaging the equations over an ensemble of stochastic wave disturbances, and the effect of focusing and channeling of the inner part of the beam, similar to that observed in a capillary discharge has been numerically demonstrated. The quasiperiodic structure of rays during channeling with alternating antinodes and nodes has been shown. Due to the fundamental nature of the processes under consideration, it can be expected that the phenomenon of focusing and channeling of X rays by density waves should be observed not only in capillary discharges, but also in jets from accretion disks around stars and black holes, which has been qualitatively demonstrated by comparing the numerical tracing results with astronomical observations by the Chandra X-ray Observatory.
{"title":"Effect of X-Ray Focusing in a Turbulent Plasma Structure with Fast Particle Fluxes","authors":"V. S. Zakharov, S. V. Zakharov, T. V. Shmeleva","doi":"10.1134/S0021364025607584","DOIUrl":"10.1134/S0021364025607584","url":null,"abstract":"<p>A theoretical model of the experimentally observed collimation of soft radiation from a capillary discharge with hollow electrodes without the use of collimating optics has been proposed. The effect of focusing and channeling of hard radiation with a small difference of the refractive index of the discharge plasma from the vacuum value is possible with its multiple refractions on density disturbances caused by the generation of small-scale waves due to two-stream plasma instabilities. The numerical solution of the eikonal equation shows the possibility of such focusing in a periodic plasma structure. The conditions for focusing of hard radiation in a turbulent plasma structure for almost paraxial rays have been obtained by averaging the equations over an ensemble of stochastic wave disturbances, and the effect of focusing and channeling of the inner part of the beam, similar to that observed in a capillary discharge has been numerically demonstrated. The quasiperiodic structure of rays during channeling with alternating antinodes and nodes has been shown. Due to the fundamental nature of the processes under consideration, it can be expected that the phenomenon of focusing and channeling of X rays by density waves should be observed not only in capillary discharges, but also in jets from accretion disks around stars and black holes, which has been qualitatively demonstrated by comparing the numerical tracing results with astronomical observations by the Chandra X-ray Observatory.</p>","PeriodicalId":604,"journal":{"name":"JETP Letters","volume":"122 8","pages":"491 - 499"},"PeriodicalIF":1.3,"publicationDate":"2025-12-04","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://link.springer.com/content/pdf/10.1134/S0021364025607584.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145665977","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2025-11-24DOI: 10.1134/S0021364025609613
E. I. Nikulin, A. I. Chernov, D. A. Svintsov
We study the interplay of electron–phonon and electron–impurity scattering in graphene and its manifestations in thermopower S. Electron scattering by acoustic phonons dominating in clean samples results in energy-independent carrier diffusivity, which translates into zero value of S. Inclusion of charged impurities plays a twofold role. At low impurity densities, the diffusivity becomes energy-dependent, which elevates S. In largely disordered samples, the carrier density becomes inhomogeneous, which results in self-averaging of thermopower. The latter effect is tackled here with effective medium theory, and predicts a slow drop in (S) with increasing the impurity density. The competition of these effects results in thermopower maximization at an optimal density of impurities ({{n}_{{{text{imp}}}}}). The latter is estimated as (2 times {{10}^{{11}}}) cm–2 at room temperature, which corresponds to the highest-quality chemical vapor deposited graphene.
我们研究了石墨烯中电子-声子和电子-杂质散射的相互作用及其在热电s中的表现。在干净样品中,声子主导的电子散射导致能量无关的载流子扩散率,这转化为s的零值。在低杂质密度下,扩散系数变得依赖于能量,从而提高了s。在大量无序的样品中,载流子密度变得不均匀,导致热功率自平均。本文用有效介质理论解决了后一种效应,并预测(S)随杂质密度的增加而缓慢下降。这些影响的竞争导致在最佳杂质密度下热功率最大化({{n}_{{{text{imp}}}}})。后者在室温下估计为(2 times {{10}^{{11}}}) cm-2,这对应于最高质量的化学气相沉积石墨烯。
{"title":"Maximization of Thermopower in Optimally-Disordered Graphene","authors":"E. I. Nikulin, A. I. Chernov, D. A. Svintsov","doi":"10.1134/S0021364025609613","DOIUrl":"10.1134/S0021364025609613","url":null,"abstract":"<p>We study the interplay of electron–phonon and electron–impurity scattering in graphene and its manifestations in thermopower <i>S</i>. Electron scattering by acoustic phonons dominating in clean samples results in energy-independent carrier diffusivity, which translates into zero value of <i>S</i>. Inclusion of charged impurities plays a twofold role. At low impurity densities, the diffusivity becomes energy-dependent, which elevates <i>S</i>. In largely disordered samples, the carrier density becomes inhomogeneous, which results in self-averaging of thermopower. The latter effect is tackled here with effective medium theory, and predicts a slow drop in <span>(S)</span> with increasing the impurity density. The competition of these effects results in thermopower maximization at an optimal density of impurities <span>({{n}_{{{text{imp}}}}})</span>. The latter is estimated as <span>(2 times {{10}^{{11}}})</span> cm<sup>–2</sup> at room temperature, which corresponds to the highest-quality chemical vapor deposited graphene.</p>","PeriodicalId":604,"journal":{"name":"JETP Letters","volume":"122 11","pages":"757 - 763"},"PeriodicalIF":1.3,"publicationDate":"2025-11-24","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"146016111","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}