Pub Date : 2024-04-01DOI: 10.1134/s0030400x23100223
E. Yu. Shamparov, A. L. Bugrimov, S. V. Rode, I. N. Jagrina
Abstract
The infrared transmission and reflection spectra of a series of samples of bismuth films of different thicknesses on identical single-crystal silicon substrates were measured. Transmission and reflection oscillations caused by interference on the film thickness are investigated. Properties of Si-plates are estimated. Refractive index and absorption index of bismuth are calculated.
{"title":"Ir Transparency of Thin Bismuth Films","authors":"E. Yu. Shamparov, A. L. Bugrimov, S. V. Rode, I. N. Jagrina","doi":"10.1134/s0030400x23100223","DOIUrl":"https://doi.org/10.1134/s0030400x23100223","url":null,"abstract":"<h3 data-test=\"abstract-sub-heading\">Abstract</h3><p>The infrared transmission and reflection spectra of a series of samples of bismuth films of different thicknesses on identical single-crystal silicon substrates were measured. Transmission and reflection oscillations caused by interference on the film thickness are investigated. Properties of Si-plates are estimated. Refractive index and absorption index of bismuth are calculated.</p>","PeriodicalId":723,"journal":{"name":"Optics and Spectroscopy","volume":null,"pages":null},"PeriodicalIF":0.6,"publicationDate":"2024-04-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"140562040","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2024-04-01DOI: 10.1134/s0030400x23100144
A. G. Mirochnik, E. V. Fedorenko, A. Yu. Beloliptsev
Abstract
The processes of the formation of J-aggregates during the dissolution 2,2-difluoro-4,6-di(4'-methylphenyl)-1,3,2-dioxaborine crystals (1) and their subsequent dissociation have been studied by absorption and luminescence spectroscopy and quantum-chemical modeling. It is shown that two luminescent centers are observed in the solution 1: monomeric luminescence and luminescence of J-aggregates (dual luminescence). Evolution of absorption, excitation and luminescence spectra is observed over time, indicating a slow dissociation of J-aggregates.
{"title":"Luminescence of Boron Difluoride Ditoluoylmethanate. Formation of J-Aggregates","authors":"A. G. Mirochnik, E. V. Fedorenko, A. Yu. Beloliptsev","doi":"10.1134/s0030400x23100144","DOIUrl":"https://doi.org/10.1134/s0030400x23100144","url":null,"abstract":"<h3 data-test=\"abstract-sub-heading\">Abstract</h3><p>The processes of the formation of J-aggregates during the dissolution 2,2-difluoro-4,6-di(4'-methylphenyl)-1,3,2-dioxaborine crystals (<b>1</b>) and their subsequent dissociation have been studied by absorption and luminescence spectroscopy and quantum-chemical modeling. It is shown that two luminescent centers are observed in the solution <b>1</b>: monomeric luminescence and luminescence of J-aggregates (dual luminescence). Evolution of absorption, excitation and luminescence spectra is observed over time, indicating a slow dissociation of J-aggregates.</p>","PeriodicalId":723,"journal":{"name":"Optics and Spectroscopy","volume":null,"pages":null},"PeriodicalIF":0.6,"publicationDate":"2024-04-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"140561792","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2024-04-01DOI: 10.1134/s0030400x23100120
N. N. Kuzmin, K. N. Boldyrev, V. V. Maltsev
Abstract
The paper presents a flux crystal growth technique, studies of the structural peculiarities and the optical absorption spectra of double orthoborate TbCr3(BO3)4 with a huntite structure. The intensities of the phonon modes were used to determine the ratios of the rhombohedral and monoclinic polytypes for this compound, depending on the growth conditions. The broadband absorption spectra of the Tb3+ ions in TbCr3(BO3)4 single crystals were studied in the temperature range from room temperature to 3.0 K. From them, the energies of the crystal-field levels of the Tb3+ ion were determined. The temperature dependence of the absorption spectra of the Er3+ probe ion in TbCr3(BO3)4:Er(1%) shows that there are two phase transitions and agrees with their previously proposed interpretation: at 8.8 K, the chromium subsystem antiferromagnetically orders, and at 5 K, a reorientation of chromium magnetic moments occurs.
摘要 本文介绍了一种通量晶体生长技术、对具有亨廷石结构的双正硼酸盐 TbCr3(BO3)4 的结构特征和光学吸收光谱的研究。利用声子模式的强度确定了该化合物的斜方多面体和单斜多面体的比例,具体取决于生长条件。研究了 TbCr3(BO3)4 单晶中 Tb3+ 离子在室温至 3.0 K 温度范围内的宽带吸收光谱。TbCr3(BO3)4:Er(1%)中 Er3+ 探针离子吸收光谱的温度依赖性表明存在两个相变,这与他们之前提出的解释一致:在 8.8 K 时,铬子系统反铁磁有序,而在 5 K 时,铬磁矩发生重新定向。
{"title":"Spectroscopic Investigation of Structural and Magnetic Properties of TbCr3(BO3)4","authors":"N. N. Kuzmin, K. N. Boldyrev, V. V. Maltsev","doi":"10.1134/s0030400x23100120","DOIUrl":"https://doi.org/10.1134/s0030400x23100120","url":null,"abstract":"<h3 data-test=\"abstract-sub-heading\">Abstract</h3><p>The paper presents a flux crystal growth technique, studies of the structural peculiarities and the optical absorption spectra of double orthoborate TbCr<sub>3</sub>(BO<sub>3</sub>)<sub>4</sub> with a huntite structure. The intensities of the phonon modes were used to determine the ratios of the rhombohedral and monoclinic polytypes for this compound, depending on the growth conditions. The broadband absorption spectra of the Tb<sup>3+</sup> ions in TbCr<sub>3</sub>(BO<sub>3</sub>)<sub>4</sub> single crystals were studied in the temperature range from room temperature to 3.0 K. From them, the energies of the crystal-field levels of the Tb<sup>3+</sup> ion were determined. The temperature dependence of the absorption spectra of the Er<sup>3+</sup> probe ion in TbCr<sub>3</sub>(BO<sub>3</sub>)<sub>4</sub>:Er(1%) shows that there are two phase transitions and agrees with their previously proposed interpretation: at 8.8 K, the chromium subsystem antiferromagnetically orders, and at 5 K, a reorientation of chromium magnetic moments occurs.</p>","PeriodicalId":723,"journal":{"name":"Optics and Spectroscopy","volume":null,"pages":null},"PeriodicalIF":0.6,"publicationDate":"2024-04-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"140561802","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2024-04-01DOI: 10.1134/s0030400x2310017x
S. S. Pakhomy, O. V. Zlobina, I. O. Bugaeva, G. N. Maslyakova, A. N. Ivanov, A. O. Moskvina
Abstract
We studied the effect of long-term constant light exposure on the severity and reversibility of morphological changes in the liver of laboratory rats. Modeling of light exposure was carried out by means of 24 h exposure to artificial light (in the daytime—300 lk, at night—500 lk). During the study we found that morphological changes in the liver were represented by damage to the parenchyma and circulatory disorders, the degree of which increased with increasing duration of exposure. After providing natural light in the laboratory, gradual recovery of the morphological structure of the organ was observed, which indicates the reversibility of the changes detected.
{"title":"Influence of the Duration of Circadian Rhythm Dis-Turbance by Light Exposure on the Morphology of the Liver of Laboratory Rats","authors":"S. S. Pakhomy, O. V. Zlobina, I. O. Bugaeva, G. N. Maslyakova, A. N. Ivanov, A. O. Moskvina","doi":"10.1134/s0030400x2310017x","DOIUrl":"https://doi.org/10.1134/s0030400x2310017x","url":null,"abstract":"<h3 data-test=\"abstract-sub-heading\">Abstract</h3><p>We studied the effect of long-term constant light exposure on the severity and reversibility of morphological changes in the liver of laboratory rats. Modeling of light exposure was carried out by means of 24 h exposure to artificial light (in the daytime—300 lk, at night—500 lk). During the study we found that morphological changes in the liver were represented by damage to the parenchyma and circulatory disorders, the degree of which increased with increasing duration of exposure. After providing natural light in the laboratory, gradual recovery of the morphological structure of the organ was observed, which indicates the reversibility of the changes detected.</p>","PeriodicalId":723,"journal":{"name":"Optics and Spectroscopy","volume":null,"pages":null},"PeriodicalIF":0.6,"publicationDate":"2024-04-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"140882864","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2024-04-01DOI: 10.1134/s0030400x23070160
V. B. Sovkov, Jizhou Wu, Jie Ma
Abstract
In order to model the spectroscopic and scattering properties of a quantum system, we propose and explore a new absorbing complex-type optical potential based on a combination of cosine functions. This function provides a high degree of smoothness to joint with a physical real-type potential. The capabilities of this function are investigated in terms of its effect on otherwise freely evolving quantum dynamics. We use our open-source programs to implement the Fourier Grid method with the Optimizer package (in Matlab), freely available at https://sourceforge.net/projects/optimizer-sovkov/.
{"title":"Cosine-Type Absorbing Optical Potential for the Modeling of Quantum Dynamics with the Fourier Grid and Optimizer Packages","authors":"V. B. Sovkov, Jizhou Wu, Jie Ma","doi":"10.1134/s0030400x23070160","DOIUrl":"https://doi.org/10.1134/s0030400x23070160","url":null,"abstract":"<h3 data-test=\"abstract-sub-heading\">Abstract</h3><p>In order to model the spectroscopic and scattering properties of a quantum system, we propose and explore a new absorbing complex-type optical potential based on a combination of cosine functions. This function provides a high degree of smoothness to joint with a physical real-type potential. The capabilities of this function are investigated in terms of its effect on otherwise freely evolving quantum dynamics. We use our open-source programs to implement the Fourier Grid method with the Optimizer package (in Matlab), freely available at https://sourceforge.net/projects/optimizer-sovkov/.</p>","PeriodicalId":723,"journal":{"name":"Optics and Spectroscopy","volume":null,"pages":null},"PeriodicalIF":0.6,"publicationDate":"2024-04-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"140882952","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2024-04-01DOI: 10.1134/s0030400x23100193
M. N. Popova
Abstract
A brief review of studies of crystals containing metal ions with unfilled f- or d-shells, made in the Institute of Spectroscopy of the Russian Academy of Sciences by high-resolution Fourier spectroscopy, is given. The main directions of study include hyperfine structure in spectra, isotopic effects, the role of random deformations, phase transition spectroscopy, low-dimensional magnets, coupled electron–phonon excitations.
摘要 简要回顾了俄罗斯科学院光谱学研究所利用高分辨率傅立叶光谱学对含有未填充 f 或 d 壳金属离子的晶体进行的研究。研究的主要方向包括光谱中的超细结构、同位素效应、随机变形的作用、相变光谱学、低维磁体、电子-声子耦合激发。
{"title":"High-Resolution Spectroscopy of Crystals Containing Transition Metal Ions (Review)","authors":"M. N. Popova","doi":"10.1134/s0030400x23100193","DOIUrl":"https://doi.org/10.1134/s0030400x23100193","url":null,"abstract":"<h3 data-test=\"abstract-sub-heading\">Abstract</h3><p>A brief review of studies of crystals containing metal ions with unfilled <i>f</i>- or <i>d</i>-shells, made in the Institute of Spectroscopy of the Russian Academy of Sciences by high-resolution Fourier spectroscopy, is given. The main directions of study include hyperfine structure in spectra, isotopic effects, the role of random deformations, phase transition spectroscopy, low-dimensional magnets, coupled electron–phonon excitations.</p>","PeriodicalId":723,"journal":{"name":"Optics and Spectroscopy","volume":null,"pages":null},"PeriodicalIF":0.6,"publicationDate":"2024-04-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"140889691","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2024-04-01DOI: 10.1134/s0030400x23100089
Yu. S. Gulina
Abstract
An experimental study of nonlinear absorption process of ultrashort laser pulses in bulk of natural diamond has been carried out. The results of experimental studies on measuring nonlinear transmission of 1 mm thick plane-parallel plate made of diamond irradiated with focused by micro lens (NA = 0.55 with focal length f ' = 5 mm) 0.3 and 10 ps laser pulses with 1030 nm wavelength are presented. It is shown that in this sample the main attenuation mechanism of ultrashort laser pulses with 1030 nm wavelength at intensities not exceeding 10 TW/cm2 is two-photon absorption at color centers, the absorption coefficient β2 = 4.1 ± 0.3 cm/TW is determined.
{"title":"Measurement of Two-Photon Absorption Coefficient of 1030 nm Ultrashort Laser Pulses on Natural Diamond Color Centers","authors":"Yu. S. Gulina","doi":"10.1134/s0030400x23100089","DOIUrl":"https://doi.org/10.1134/s0030400x23100089","url":null,"abstract":"<h3 data-test=\"abstract-sub-heading\">Abstract</h3><p>An experimental study of nonlinear absorption process of ultrashort laser pulses in bulk of natural diamond has been carried out. The results of experimental studies on measuring nonlinear transmission of 1 mm thick plane-parallel plate made of diamond irradiated with focused by micro lens (<i>NA</i> = 0.55 with focal length <i>f</i> ' = 5 mm) 0.3 and 10 ps laser pulses with 1030 nm wavelength are presented. It is shown that in this sample the main attenuation mechanism of ultrashort laser pulses with 1030 nm wavelength at intensities not exceeding 10 TW/cm<sup>2</sup> is two-photon absorption at color centers, the absorption coefficient β<sub>2</sub> = 4.1 ± 0.3 cm/TW is determined.</p>","PeriodicalId":723,"journal":{"name":"Optics and Spectroscopy","volume":null,"pages":null},"PeriodicalIF":0.6,"publicationDate":"2024-04-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"140561801","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2024-04-01DOI: 10.1134/s0030400x23100053
K. V. Ezdakova (Voronina), A. V. Rudakova, I. V. Krauklis, Ya. V. Shergin, A. A. Tsyganenko
Abstract
The effect of adsorption of acid gases CO2, SO2, and SO3 on the electron accepting ability of cations on the surface of calcium oxide was studied by low-temperature IR spectroscopy of adsorbed CO. It is shown that the formation of carbonate, sulfite and sulfate anions in the surface layer leads to the appearance of Lewis acid sites, the strength of which, estimated by the shift in the vibration frequency of CO molecules associated with them, increases in the appropriate order, approaching that for calcium-containing zeolites. The results of the calculation of cluster models by the DFT method confirm the observed trends in the variation of the vibrational frequency and the absorption coefficient of CO molecules bound through both the carbon and oxygen atoms, and also demonstrate the dependence of the ability of a cation for CO linkage isomerism on its local environment.
摘要 通过对吸附的 CO 进行低温红外光谱分析,研究了酸性气体 CO2、SO2 和 SO3 的吸附对氧化钙表面阳离子电子接受能力的影响。结果表明,表层中碳酸盐、亚硫酸盐和硫酸盐阴离子的形成会导致路易斯酸位点的出现,根据与之相关的 CO 分子振动频率的移动来估算,路易斯酸位点的强度会按适当的顺序增加,接近含钙沸石的路易斯酸位点。用 DFT 方法计算簇模型的结果证实了观察到的通过碳原子和氧原子结合的 CO 分子的振动频率和吸收系数的变化趋势,还证明了阳离子的 CO 链接异构能力取决于其局部环境。
{"title":"The Influence of the Local Environment on the Electron Accepting Ability of the Cation: Induced Lewis Acidity","authors":"K. V. Ezdakova (Voronina), A. V. Rudakova, I. V. Krauklis, Ya. V. Shergin, A. A. Tsyganenko","doi":"10.1134/s0030400x23100053","DOIUrl":"https://doi.org/10.1134/s0030400x23100053","url":null,"abstract":"<h3 data-test=\"abstract-sub-heading\">Abstract</h3><p>The effect of adsorption of acid gases CO<sub>2</sub>, SO<sub>2</sub>, and SO<sub>3</sub> on the electron accepting ability of cations on the surface of calcium oxide was studied by low-temperature IR spectroscopy of adsorbed CO. It is shown that the formation of carbonate, sulfite and sulfate anions in the surface layer leads to the appearance of Lewis acid sites, the strength of which, estimated by the shift in the vibration frequency of CO molecules associated with them, increases in the appropriate order, approaching that for calcium-containing zeolites. The results of the calculation of cluster models by the DFT method confirm the observed trends in the variation of the vibrational frequency and the absorption coefficient of CO molecules bound through both the carbon and oxygen atoms, and also demonstrate the dependence of the ability of a cation for CO linkage isomerism on its local environment.</p>","PeriodicalId":723,"journal":{"name":"Optics and Spectroscopy","volume":null,"pages":null},"PeriodicalIF":0.6,"publicationDate":"2024-04-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"140561883","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2024-04-01DOI: 10.1134/s0030400x23100107
K. R. Karimullin, A. I. Arzhanov, N. V. Surovtsev, A. V. Naumov
Abstract
The temperature-dependent luminescence spectra were analyzed to determine the parameters of the electron–phonon interaction (Huang–Rhys factor and the average phonon energy) for nanocomposites with colloidal CdSe/CdS/ZnS quantum dots (deposited on the surface of a glass substrate and embedded in a thin polymer film of polyisobutylene, and in a frozen colloidal solution in toluene). The measured values of the parameters are analyzed in comparison with model calculations and data obtained using the low-frequency Raman spectroscopy. It is found that in the case of a vitrified colloidal solution of quantum dots in toluene, the matrix effect leads to a noticeable change in the parameters of the electron–phonon interaction.
{"title":"Electron–Phonon Interaction in Composites with Colloidal Quantum Dots: A Study by Luminescence Spectroscopy and Raman Scattering","authors":"K. R. Karimullin, A. I. Arzhanov, N. V. Surovtsev, A. V. Naumov","doi":"10.1134/s0030400x23100107","DOIUrl":"https://doi.org/10.1134/s0030400x23100107","url":null,"abstract":"<h3 data-test=\"abstract-sub-heading\">Abstract</h3><p>The temperature-dependent luminescence spectra were analyzed to determine the parameters of the electron–phonon interaction (Huang–Rhys factor and the average phonon energy) for nanocomposites with colloidal CdSe/CdS/ZnS quantum dots (deposited on the surface of a glass substrate and embedded in a thin polymer film of polyisobutylene, and in a frozen colloidal solution in toluene). The measured values of the parameters are analyzed in comparison with model calculations and data obtained using the low-frequency Raman spectroscopy. It is found that in the case of a vitrified colloidal solution of quantum dots in toluene, the matrix effect leads to a noticeable change in the parameters of the electron–phonon interaction.</p>","PeriodicalId":723,"journal":{"name":"Optics and Spectroscopy","volume":null,"pages":null},"PeriodicalIF":0.6,"publicationDate":"2024-04-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"140882861","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2024-04-01DOI: 10.1134/s0030400x23070159
E. A. Smirnova, N. A. Lozing, M. G. Gladush, A. V. Naumov
Abstract
The current paper demonstrates theoretical analysis of two types of spectral curves for several configurations of system of two-level light emitters, considering the influence of local field and close environment inside a transparent medium. Probe field absorption spectra and resonant fluorescence spectra are calculated under excitation of a strong monochromatic cw laser. The sensitivity of absorption and emission optical spectroscopy method is compared for revealing the effects of the medium on individual emitters and their ensembles. Spectral curves were calculated for model emitters considering local field influence of a transparent dielectric medium and local electron-phonon interactions, which determined the response of the emitters to an external laser field and effective relaxation mechanisms. The calculation formalism is based on a semiclassical approach, while the relaxation processes associated with the phonon contribution are introduced phenomenologically with references to other studies.
{"title":"The Effects of Local Environment on a Probe Signal Absorption and Resonance Fluorescence for Quantum Emitters in Transparent Media","authors":"E. A. Smirnova, N. A. Lozing, M. G. Gladush, A. V. Naumov","doi":"10.1134/s0030400x23070159","DOIUrl":"https://doi.org/10.1134/s0030400x23070159","url":null,"abstract":"<h3 data-test=\"abstract-sub-heading\">Abstract</h3><p>The current paper demonstrates theoretical analysis of two types of spectral curves for several configurations of system of two-level light emitters, considering the influence of local field and close environment inside a transparent medium. Probe field absorption spectra and resonant fluorescence spectra are calculated under excitation of a strong monochromatic cw laser. The sensitivity of absorption and emission optical spectroscopy method is compared for revealing the effects of the medium on individual emitters and their ensembles. Spectral curves were calculated for model emitters considering local field influence of a transparent dielectric medium and local electron-phonon interactions, which determined the response of the emitters to an external laser field and effective relaxation mechanisms. The calculation formalism is based on a semiclassical approach, while the relaxation processes associated with the phonon contribution are introduced phenomenologically with references to other studies.</p>","PeriodicalId":723,"journal":{"name":"Optics and Spectroscopy","volume":null,"pages":null},"PeriodicalIF":0.6,"publicationDate":"2024-04-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"140883058","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}