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Parametric Down-Conversion of Near-IR Laser Radiation into the Mid-IR Range Using Nonlinear LiGaSe2 and LiGaS2 Crystals with Antireflection Microstructures 具有增反射微结构的非线性LiGaS2和LiGaS2晶体将近红外激光辐射参数下转换为中红外
IF 1.1 4区 物理与天体物理 Q3 PHYSICS, MULTIDISCIPLINARY Pub Date : 2025-09-04 DOI: 10.3103/S1541308X25600308
S. N. Smetanin, P. D. Kharitonova, A. G. Papashvili, L. I. Isaenko, A. F. Kurus, A. P. Yelisseyev, A. A. Goloshumova, A. A. Bushunov, A. A. Teslenko, V. A. Lazarev, M. K. Tarabrin

The LiGaSe2 and LiGaS2 crystals with antireflection microstructures are comparatively tested as frequency down-converters into the mid-infrared range (4874 nm) in a two-stage optical parametric oscillator with a single cavity under intracavity pumping with a Nd:YLF laser with a wavelength of 1047 nm and a pulse duration of 25 ns. The first stage of optical parametric oscillation in the KTiOAsO4 crystal produces two-micron radiation with wavelengths of 1724 and 2668 nm at a pulse energy of up to 2 mJ. In the second stage of conversion, the LiGaS2 crystal with antireflection microstructures compared to LiGaSe2 with antireflection microstructures proves to be more efficient despite the lower effective nonlinearity coefficient, which can be explained by the higher optical quality of the crystal. The energy of the radiation pulse with a wavelength of 4874 nm reaches the level of 100 nJ.

利用波长为1047 nm、脉冲持续时间为25 ns的Nd:YLF激光器,在单腔双级光学参量振荡器中,对具有抗反射微结构的LiGaSe2和LiGaS2晶体进行了中红外(4874 nm)降频测试。KTiOAsO4晶体的光学参量振荡的第一阶段产生波长为1724和2668 nm的两微米辐射,脉冲能量高达2 mJ。在转换的第二阶段,与具有增透微结构的LiGaS2晶体相比,具有增透微结构的LiGaS2晶体的效率更高,尽管有效非线性系数更低,这可以解释为晶体的光学质量更高。波长为4874 nm的辐射脉冲能量达到100 nJ的水平。
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引用次数: 0
Partially Diffusive Structural Mechanism of the Transitions between Ices III and V III型和V型冰过渡的部分扩散结构机制
IF 1.1 4区 物理与天体物理 Q3 PHYSICS, MULTIDISCIPLINARY Pub Date : 2025-07-20 DOI: 10.3103/S1541308X2570013X
E. A. Zheligovskaya

It is shown that the structures of ices III and V can be divided into nearly identical chiral layers. In achiral ice V, the right-handed enantiomorphic layers alternate with the left-handed ones. Chiral ice III consists of only right-handed or only left-handed layers. A structural mechanism preserving these layers is proposed for the transitions between ices III and V. This mechanism is partially diffusive. The possibility for the proposed structural mechanism to provide the experimentally observed high transition rate is discussed. Small structural units of crystal ices are shown to change regularly with increasing pressure in the sequence III, V, and VI. Such small structures formed by water molecules can be present in liquid near the crystallization curve.

结果表明,冰III和冰V的结构可以划分为几乎相同的手性层。在非手性冰V中,右手对纯层与左手对纯层交替存在。手性冰III只由右手或左手层组成。在冰III和冰v之间的过渡中,提出了一种保留这些层的结构机制,这种机制部分是扩散的。讨论了所提出的结构机制提供实验观察到的高跃迁速率的可能性。晶体冰的小结构单元在III、V和VI序列中随着压力的增加而有规律地变化。这种由水分子形成的小结构可以出现在结晶曲线附近的液体中。
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引用次数: 0
Paradox of Radiant Power and the Issue of Localized Currents 辐射功率悖论与局域电流问题
IF 1.1 4区 物理与天体物理 Q3 PHYSICS, MULTIDISCIPLINARY Pub Date : 2025-07-20 DOI: 10.3103/S1541308X25600047
Yu. A. Akimov

Two fundamental questions of modern theoretical physics—the paradox of radiant power and the issue of localized currents—are discussed in the paper. The radiant power paradox is the dilemma of whether electrodynamic systems radiate power outward or not. Mathematical analysis of the microscopic Maxwell equations describing excitation and propagation of electromagnetic fields shows that the total radiant power should be zero, whereas many classical problems considering localized currents argue the opposite. The paradox is resolved by proving limited applicability of localized-current models to calculations of energy and momentum characteristics of electromagnetic fields. The nonzero value of the total radiant power for these currents turns out to be the localized current approximation error, while the true radiant power value is always zero for physically consistent excitation currents. On the basis of analysis of physically consistent currents, an improved model of localized currents is proposed that enables physically consistent description of electromagnetic fields from the viewpoint of their energy and momentum characteristics but at the expense of causality violation in the external current-free region.

本文讨论了现代理论物理学的两个基本问题——辐射功率悖论和定域电流问题。辐射功率悖论是电动力系统是否向外辐射功率的困境。对描述电磁场激发和传播的微观麦克斯韦方程组的数学分析表明,总辐射功率应为零,而许多考虑局域电流的经典问题则相反。通过证明局域电流模型在电磁场能量和动量特性计算中的有限适用性,解决了这一悖论。这些电流的总辐射功率的非零值是局部电流近似误差,而物理一致励磁电流的真实辐射功率值始终为零。在分析物理一致电流的基础上,提出了一种改进的局域电流模型,该模型能够从能量和动量特征的角度对电磁场进行物理一致的描述,但代价是在外无电流区域违反因果关系。
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引用次数: 0
Random Pinning Models: Phase Transitions in Aqueous Solutions of Colloidal Particles 随机钉钉模型:胶体颗粒水溶液中的相变
IF 1.1 4区 物理与天体物理 Q3 PHYSICS, MULTIDISCIPLINARY Pub Date : 2025-07-20 DOI: 10.3103/S1541308X25700116
E. N. Tsiok, S. A. Bobkov, E. E. Tareyeva, Yu. D. Fomin, V. N. Ryzhov

Self-assembly of colloidal particles may occur, for example, both under the action of external fields and due to the presence of pinning centers in a real experimental system. Of particular interest is the formation of condensed phases from an aqueous solution of colloidal particles on a substrate in an external rotating magnetic field. Substrate defects (for example, the substrate roughness) are of great importance in an experiment. These defects can act as pinning centers, to which colloidal particles are strongly attracted; this may lead to a change in the melting scenario. Changing the field rotation angle, one can obtain different colloidal structures. At small rotation angles, the system behaves like a two-dimensional system with a purely repulsive soft-disk potential, whereas at large angles it is similar to a generalized Lennard-Jones (LJ) system with an (nm)-potential. When the field rotates in the plane of the system, its phase diagram qualitatively resembles that of a classical model system with a LJ pair potential. The results of the computer simulation of a two-dimensional system with a LJ potential in the presence of Gauss pinning are discussed in the context of its influence on the phase diagram and melting scenario. It is shown that random pinning with a Gauss potential leads to an increase in the hexatic phase range; formation of dense clusters near pinning centers, which reduce the average effective density of the system; and a change in the melting scenario.

胶体粒子的自组装可能发生,例如,在外场的作用下,由于在实际的实验系统中存在钉住中心。特别令人感兴趣的是,在外部旋转磁场中,胶体颗粒的水溶液在衬底上形成凝聚相。衬底缺陷(例如,衬底粗糙度)在实验中是非常重要的。这些缺陷可以作为钉住中心,胶体粒子被强烈吸引到那里;这可能导致融化情景的变化。改变磁场旋转角度,可以得到不同的胶体结构。在较小的旋转角度下,系统表现得像一个具有纯排斥软盘势的二维系统,而在较大的旋转角度下,它类似于一个具有(nm)势的广义Lennard-Jones (LJ)系统。当场在系统平面上旋转时,其相图定性地类似于具有LJ对势的经典模型系统的相图。本文讨论了具有LJ势的二维体系在高斯钉钉作用下的计算机模拟结果,并讨论了其对相图和熔化情况的影响。结果表明,高斯势随机钉住导致六相范围增大;在钉钉中心附近形成密集的团簇,降低了体系的平均有效密度;以及融化情况的改变。
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引用次数: 0
Optimization of the Characteristics of Fiber-Optic Fabry–Perot Interferometer Mirrors in Measurement Systems Using Broadband Radiation 宽带辐射测量系统中光纤法布里-珀罗干涉仪反射镜特性的优化
IF 1.1 4区 物理与天体物理 Q3 PHYSICS, MULTIDISCIPLINARY Pub Date : 2025-07-20 DOI: 10.3103/S1541308X25700165
I. G. Likhachev

The fiber-optic Fabry–Perot interferometer (FPI) has been analyzed to determine its reflection and transmission coefficients providing the maximum useful signal in a high-precision scheme for measuring the FPI length. It is shown that the traditionally applied criterion, which is aimed at achieving the maximum visibility of the interference pattern, is not applicable in this scheme. An adequate criterion is proposed, and an analysis based on it is presented. The optimal characteristics of the FPI mirrors are calculated taking into account the diffraction effects. The result of the study is a set of simple analytical relations necessary for designing mirrors in the form of thin films deposited on the fiber end face. In particular, the possibility of implementing a desired mirror on the fiber end in the form of a single-layer dielectric film is investigated and its characteristics are obtained.

对光纤法布里-珀罗干涉仪(FPI)进行了分析,确定了其反射系数和透射系数,为高精度测量FPI长度提供了最大有用信号。结果表明,传统的干涉图可见性准则在该方案中不适用。提出了一个适当的判据,并在此基础上进行了分析。在考虑衍射效应的情况下,计算了FPI反射镜的最佳特性。研究的结果是一组简单的分析关系,这是设计以薄膜形式沉积在光纤端面的反射镜所必需的。特别地,研究了在光纤端以单层介质膜的形式实现所需反射镜的可能性,并获得了其特性。
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引用次数: 0
Investigation of the Influence of pH and Temperature of an Aqueous Solution on the Stability of the Gold Nanoparticles–Lysozyme Protein System by Optical Methods 光学方法研究水溶液pH和温度对金纳米颗粒-溶菌酶蛋白体系稳定性的影响
IF 1.1 4区 物理与天体物理 Q3 PHYSICS, MULTIDISCIPLINARY Pub Date : 2025-07-20 DOI: 10.3103/S1541308X25700141
E. A. Molkova, T. A. Matveeva, I. V. Baimler, R. M. Sarimov, S. V. Gudkov, A. S. Dorokhov, A. Yu. Izmailov

Gold nanoparticles are widely used in spectroscopy for detecting/studying substances in biological media. Such particles in biological objects inevitably interact with proteins, which obviously affects the functions and properties of the nanomaterial. The influence of external conditions on the interaction of nanoparticles with proteins in the aqueous phase has still remained little studied. In this paper we investigate the influence of temperature and pH of the medium on the interaction of lysozyme protein with gold nanoparticles in aqueous solutions. It is found that the temperature of the medium affects the size of aggregates of gold nanoparticles with protein at pH 7.5 of the aqueous solutions. It is found that lysozyme prevents protein aggregation at acidic pH values; with an increase in temperature, gold particles with a lysozyme protein crown retain their size. The results of this study gain a deeper insight into the processes of interaction between enzymes and gold nanoparticles with a change in the solvent properties.

金纳米颗粒被广泛应用于光谱检测/研究生物介质中的物质。这些粒子在生物物体中不可避免地与蛋白质相互作用,这明显影响了纳米材料的功能和性能。外界条件对纳米颗粒与水相蛋白质相互作用的影响研究仍然很少。本文研究了温度和pH对溶菌酶蛋白与金纳米颗粒在水溶液中相互作用的影响。研究发现,在pH为7.5的水溶液中,介质温度对金纳米粒子与蛋白质聚集体的大小有影响。发现溶菌酶在酸性pH值下阻止蛋白质聚集;随着温度的升高,具有溶菌酶蛋白冠的金颗粒保持其大小。本研究的结果对酶与金纳米颗粒的相互作用过程以及溶剂性质的变化有了更深入的了解。
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引用次数: 0
Short-Period Background Internal Waves in the Kara Sea in the Water Area near Cape Zhelaniya 热拉尼亚角附近海域喀拉海短周期背景内波
IF 1.1 4区 物理与天体物理 Q3 PHYSICS, MULTIDISCIPLINARY Pub Date : 2025-07-20 DOI: 10.3103/S1541308X25700207
Yu. V. Nazarenko, D. D. Sidorov, A. V. Zimin, E. I. Svergun, V. G. Petnikov, I. O. Kopyshov, I. E. Kozlov

The results from field measurements of hydrological characteristics of the Kara Sea water during the expedition on the research vessel Professor Molchanov in the summer of 2024 are reported. Vertical oscillations of temperature at fixed depths (vertical liquid oscillations) caused by short-period background internal waves are detected in the thermocline using extended “yo-yo” CTD profiling synchronous with an independently operating buoy-mounted thermistor chain. Their considerable effect on the vertical temperature distribution is shown. Energy spectra of the above-mentioned oscillations are obtained. It is demonstrated that the region under consideration near Novaya Zemlya can be regarded as a region where background internal waves quite often occur. The statistical characteristics of the fields of these waves are compared to those of similar wave fields on the Atlantic shelf and near the Kamchatka shore.

报告了2024年夏天莫尔查诺夫教授号科考船对喀拉海水水文特征的实地测量结果。利用扩展的“悠悠”CTD剖面与独立运行的浮标热敏电阻链同步,在温跃层中探测到由短周期背景内波引起的固定深度温度垂直振荡(垂直液体振荡)。它们对垂直温度分布有相当大的影响。得到了上述振荡的能谱。结果表明,所考虑的靠近新地岛的区域可以看作是一个经常发生背景内波的区域。将这些波场的统计特征与大西洋陆架和堪察加海岸附近的类似波场进行了比较。
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引用次数: 0
Investigation of ZnWO4 Crystals Doped with Tm3+ and Li+ Ions at Different Concentrations 掺杂不同浓度Tm3+和Li+离子的ZnWO4晶体的研究
IF 1.1 4区 物理与天体物理 Q3 PHYSICS, MULTIDISCIPLINARY Pub Date : 2025-07-20 DOI: 10.3103/S1541308X25700177
Yu. I. Zimina, K. A. Subbotin, A. I. Titov, P. A. Volkov, Ya. S. Didenko, D. A. Lis, S. K. Pavlov, E. V. Zharikov

A series of Tm,Li:ZnWO4 single crystals with different combinations of thulium and lithium concentrations is grown by the Czochralski method. Actual concentrations of both dopants are measured using inductively coupled plasma mass spectrometry. Segregation coefficients of thulium and lithium in the crystals are calculated by the initial point method. It is shown that introduction of lithium into the crystal composition increases the segregation coefficient of thulium between the crystal and the melt by at least a factor of 2, from 0.2 to 0.4. At the same time, the segregation coefficient of lithium monotonically decreases from 0.18 to 0.08 with its increasing concentration. Thus, to produce a sample with considerable and equimolar Tm and Li concentrations in the crystal, the nominal concentration of lithium is required to be very high, severalfold higher than that of thulium. Polarized optical absorption spectra of the crystals are measured at room temperature for all possible combinations of orientations of the strength vectors of the test beam’s electric and magnetic fields with respect to the optical indicatrix axes of the crystals. It is shown that at the electric field orientation E || Nm the shape of the absorption spectra appreciably depends on the magnetic field orientation as well. The influence of the lithium presence/absence in the crystal on the shape of the absorption spectra is determined. Absorption cross sections of thulium in the given crystal are refined and found to be considerably larger than previously published. Mechanical strength characteristics, microhardness and fracture toughness, are measured for the series of Tm,Li:ZnWO4 crystals using the indentation method. It is shown that these characteristics are noticeably deteriorated when Tm3+ ions are introduced into the crystal without simultaneously introducing the charge compensator—Li+ ions—because there arise zinc vacancies that loosen the crystal structure. Additional introduction of lithium in equimolar amounts results in that the strength characteristics of the crystals are not only restored but even exceed those of undoped ZnWO4, since this simultaneous doping does not lead to formation of zinc vacancies. Thus, conditions are revealed that allow fabrication of heavily thulium-doped crystals with maximum possible mechanical strength characteristics of ZnWO4.

采用Czochralski法生长了一系列具有不同铥和锂浓度组合的Tm,Li:ZnWO4单晶。使用电感耦合等离子体质谱法测量两种掺杂剂的实际浓度。用初始点法计算了晶体中铥和锂的偏析系数。结果表明,在晶体组成中引入锂使铥在晶体和熔体之间的偏析系数增加了至少2倍,从0.2增加到0.4。同时,随着锂离子浓度的增加,锂离子的偏析系数从0.18单调降低到0.08。因此,为了在晶体中产生具有相当大的等摩尔Tm和Li浓度的样品,锂的标称浓度需要非常高,比铥的浓度高几倍。在室温下测量了晶体的偏振光学吸收光谱,测量了测试光束的电场和磁场的强度矢量相对于晶体的光学指示轴的所有可能的方向组合。结果表明,在电场取向E || Nm处,吸收光谱的形状也明显依赖于磁场取向。确定了晶体中锂的存在/不存在对吸收光谱形状的影响。在给定晶体中,铥的吸收截面被细化,发现比以前发表的要大得多。采用压痕法测定了Tm,Li:ZnWO4系列晶体的机械强度特性、显微硬度和断裂韧性。结果表明,在没有同时引入电荷补偿器(li +)的情况下,当Tm3+离子引入晶体时,这些特性明显恶化,因为存在锌空位,使晶体结构松动。额外引入等摩尔量的锂,不仅恢复了晶体的强度特性,甚至超过了未掺杂的ZnWO4,因为这种同时掺杂不会导致锌空位的形成。因此,揭示了允许制造具有最大可能的ZnWO4机械强度特性的重掺铥晶体的条件。
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引用次数: 0
Increase in the Relative Content of ortho-Н2О Molecules in Vapor above Boiling Water 沸水以上蒸汽中邻位羟基-Н2О分子相对含量的增加
IF 1.1 4区 物理与天体物理 Q3 PHYSICS, MULTIDISCIPLINARY Pub Date : 2025-07-20 DOI: 10.3103/S1541308X25700189
E. V. Stepanov, S. M. Pershin

The spin selectivity of the processes occurring in vapor above the surface of boiling water has been experimentally demonstrated. This selectivity leads to a significant increase in the fraction of ortho-H2O molecules in vapor. An increase in the relative content of ortho/para-isomers of water from the equilibrium value of 3 : 1 (determined by quantum statistics) to 5 : 1 was observed. The content of H2O spin isomers in vapor above the water surface was analyzed using a tunable diode laser. Spectral analysis of the ortho- and para-H2O content was performed using the absorption lines of these molecules belonging to the vibrational–rotational band 101-000 and having transition frequencies of 7355.557 and 7354.599 cm–1, respectively. When water is heated from room temperature (20°C) to the second boiling phase (~80°C), a ratio of ortho- and para-spin isomers of ~3 : 1 was observed, which is typical of normal conditions. During the second and third boiling phases (80–90°C), the ortho/para ratio increases to 5:1. A possible mechanism for increasing the fraction of ortho-H2O in the vapor formed during boiling may be associated with the depletion of the equilibrium mixture in the para-H2O isomer, due to its higher activity in condensation and formation of water microdrops, dimers, and trimers.

实验证明了在沸水表面以上的蒸汽中发生的过程的自旋选择性。这种选择性导致蒸汽中邻水分子的比例显著增加。观察到水的邻位/对位异构体的相对含量从平衡值3:1(由量子统计确定)增加到5:1。用可调谐二极管激光分析了水面以上蒸汽中水自旋异构体的含量。利用振动旋转带101-000、跃迁频率分别为7355.557和7354.599 cm-1的分子吸收谱线对邻位和对水分子含量进行了光谱分析。当水从室温(20°C)加热到第二沸腾相(~80°C)时,观察到邻旋和对旋异构体的比例为~ 3:1,这是典型的正常条件。在第二和第三沸腾阶段(80-90℃),邻位/对位比增加到5:1。在沸腾过程中形成的蒸汽中增加邻水分数的可能机制可能与对水异构体中平衡混合物的耗尽有关,因为它在冷凝和形成水微滴、二聚体和三聚体方面具有较高的活性。
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引用次数: 0
On Noise Power in High-Current Relativistic Electron Beams Formed by Explosive-Emission Cathodes 爆炸发射阴极形成的大电流相对论电子束中的噪声功率
IF 1.1 4区 物理与天体物理 Q3 PHYSICS, MULTIDISCIPLINARY Pub Date : 2025-07-20 DOI: 10.3103/S1541308X25700190
I. L. Bogdankevich, S. E. Andreev, O. T. Loza, K. V. Mal’chik

Numerical simulation is used to compare two methods for measuring power of wideband electromagnetic noise in experimental facilities with high-current relativistic electron beams formed by explosive-emission cathodes. The simulation shows that the difference in the experimental results by two orders of magnitude—several megawatts for pulses with a duration of few nanoseconds and tens of kilowatts for pulses with a duration of hundreds of nanoseconds—arises from the nature of the noise itself at different stages of the explosive-emission cathode operation rather than from difference of the measurement methods.

采用数值模拟的方法,比较了两种测量爆炸发射阴极形成的大电流相对论电子束宽带电磁噪声功率的方法。仿真结果表明,实验结果的两个数量级差异(持续时间为几纳秒的脉冲为几兆瓦,持续时间为数百纳秒的脉冲为几十千瓦)是由爆炸发射阴极操作不同阶段的噪声本身的性质引起的,而不是由测量方法的差异引起的。
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引用次数: 0
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Physics of Wave Phenomena
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