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Restructuring and integrity of molecular catalysts in electrochemical CO 2 reduction 电化学还原co2分子催化剂的结构调整与完整性研究
Natural sciences (Weinheim, Germany)
Pub Date : 2022-07-15 DOI: 10.1002/ntls.20210628
Conor L. Rooney, Yueshen Wu, David J. Gallagher, Hailiang Wang
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引用次数: 4
Topological monopole's gauge field‐induced anomalous Hall effect in artificial honeycomb lattice 人工蜂窝晶格中拓扑单极子规范场诱导的反常霍尔效应
Natural sciences (Weinheim, Germany)
Pub Date : 2022-07-12 DOI: 10.1002/ntls.20210083
Jiasen Guo, V. Dugaev, A. Ernst, G. Yumnam, Pousali Ghosh, D. Singh
Vortex magnetic structure in artificial honeycomb lattice provides a unique platform to explore emergent properties due to the additional Berry phase curvature imparted by chiral magnetization to circulating electrons via direct interaction. We argue that while the perpendicularly-aligned magnetic component leads to the quantized flux of monopole at the center of the Berry sphere, the in-plane vortex circulation of magnetization gives rise to unexpected non-trivial topological Berry phase due to the gauge field transformation. The unprecedented effect signifies the importance of vector potential in multiply-connected geometrical systems. Experimental confirmations to proposed hypotheses are obtained from Hall resistance measurements on permalloy honeycomb lattice. Investigation of the topological gauge transformation due to the in-plane chirality reveals anomalous quasi-oscillatory behavior in Hall resistance $R_{xy}$ as function of perpendicular field. The oscillatory nature of $R_{xy}$ is owed to the fluctuation in equilibrium current as a function of Fermi wave-vector $k_F$, envisaged under the proposed new formulation in this article. Our synergistic approach suggests that artificially tunable nanostructured material provides new vista to the exploration of topological phenomena of strong fundamental importance.
人工蜂窝晶格中的涡旋磁结构提供了一个独特的平台来探索由于手性磁化通过直接相互作用赋予循环电子额外的贝里相曲率而产生的涌现特性。我们认为，虽然垂直排列的磁分量导致Berry球中心单极子的量子化通量，但由于规范场变换，磁化的平面内涡旋循环会产生意想不到的非平凡拓扑Berry相。这一前所未有的效应表明了向量势在多连通几何系统中的重要性。通过对坡莫合金蜂窝晶格的霍尔电阻测量，实验证实了上述假设。研究了由于面内手性引起的拓扑规范变换，揭示了霍尔电阻R_{xy}$随垂直场的变化具有反常的准振荡行为。R_{xy}$的振荡性质是由于平衡电流作为费米波矢量k_F$的函数的波动，这是在本文提出的新公式中设想的。我们的协同方法表明，人工可调谐纳米结构材料为探索具有重要基础意义的拓扑现象提供了新的前景。
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引用次数: 1
Ultrafast phonon‐driven charge transfer in van der Waals heterostructures 范德华异质结构中声子驱动的超快电荷转移
Natural sciences (Weinheim, Germany)
Pub Date : 2022-07-07 DOI: 10.1002/ntls.20220014
Giuseppe Meneghini, S. Brem, E. Malic
Van der Waals heterostructures built by vertically stacked transition metal dichalcogenides (TMDs) exhibit a rich energy landscape including interlayer and intervalley excitons. Recent experiments demonstrated an ultrafast charge transfer in TMD heterostructures. However, the nature of the charge transfer process has remained elusive. Based on a microscopic and material-realistic exciton theory, we reveal that phonon-mediated scattering via strongly hybridized intervalley excitons governs the charge transfer process that occurs on a sub-100fs timescale. We track the time-, momentum-, and energy-resolved relaxation dynamics of optically excited excitons and determine the temperature- and stacking-dependent charge transfer time for different TMD bilayers. The provided insights present a major step in microscopic understanding of the technologically important charge transfer process in van der Waals heterostructures.
由垂直堆叠的过渡金属二硫族化合物(TMDs)构建的范德华异质结构具有丰富的能量景观，包括层间和谷间激子。最近的实验证明了TMD异质结构中的超快电荷转移。然而，电荷转移过程的性质仍然是难以捉摸的。基于微观和物质现实的激子理论，我们揭示了通过强杂化谷间激子的声子介导散射控制着发生在亚100fs时间尺度上的电荷转移过程。我们跟踪了光激发激子的时间、动量和能量分辨弛豫动力学，并确定了不同TMD双层中与温度和堆叠相关的电荷转移时间。所提供的见解在微观理解范德华异质结构中技术上重要的电荷转移过程方面迈出了重要的一步。
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引用次数: 10
Retroviral lineage analysis reveals dual contribution from ectodermal placodes and neural crest cells to avian olfactory sensory and GnRH neurons. 逆转录病毒谱系分析揭示了外胚层基板细胞和神经嵴细胞对鸟类嗅觉感觉和GnRH神经元的双重贡献。
Natural sciences (Weinheim, Germany)
Pub Date : 2022-07-01 DOI: 10.1002/ntls.20210037
Alison Koontz, Hugo A Urrutia, Marianne E Bronner

The origin of the neurons and glia in the olfactory system of vertebrates has been controversial, with different cell types attributed to being of ectodermal placode versus neural crest lineage, depending upon the species. Here, we use replication incompetent avian (RIA) retroviruses to perform prospective cell lineage analysis of either presumptive olfactory placode or neural crest cells during early development of the chick embryo. Surprisingly, the results reveal a dual contribution from both the olfactory placode and neural crest cells to sensory neurons in the nose and Gonadotropin Releasing Hormone (GnRH) neurons migrating to the olfactory bulb. We also confirm that olfactory ensheathing glia are solely derived from the neural crest. Finally, our results show that neural crest cells and olfactory placode cells contribute to p63 positive cells, likely to be basal stem cells of the olfactory epithelium. Taken together, these finding provide evidence for previously unknown contributions of neural crest cells to some cell types in the chick olfactory system and help resolve previous discrepancies in the literature.

脊椎动物嗅觉系统中神经元和神经胶质的起源一直存在争议，根据物种的不同，有不同的细胞类型被归因于外胚层基板和神经嵴谱系。在这里，我们使用复制不能力禽(RIA)逆转录病毒对鸡胚胎早期发育过程中推测的嗅觉基板细胞或神经嵴细胞进行前瞻性细胞谱系分析。令人惊讶的是，结果显示嗅觉基板和神经嵴细胞对鼻子的感觉神经元和促性腺激素释放激素(GnRH)神经元迁移到嗅球的双重贡献。我们也证实了嗅鞘胶质细胞完全来源于神经嵴。最后，我们的研究结果表明，神经嵴细胞和嗅觉基板细胞有助于p63阳性细胞，可能是嗅觉上皮的基底干细胞。综上所述，这些发现为以前未知的神经嵴细胞对鸡嗅觉系统中某些细胞类型的贡献提供了证据，并有助于解决先前文献中的差异。
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引用次数: 1
Front Cover: One‐pot synthesis of high‐capacity silicon anodes via on‐copper growth of a semiconducting, porous polymer 封面:通过在铜上生长半导体多孔聚合物，一锅合成高容量硅阳极
Natural sciences (Weinheim, Germany)
Pub Date : 2022-07-01 DOI: 10.1002/ntls.10060
Jieyang Huang, Andréa Martin, Anna Urbanski, Ranjit Kulkarni, P. Amsalem, Moritz Exner, Guiping Li, Johannes Müller, David Burmeister, Norbert Koch, T. Brezesinski, N. Pinna, P. Uhlmann, Michael J. Bojdys
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引用次数: 0
Diagnosing cancer from a drop of blood 从一滴血中诊断癌症
Natural sciences (Weinheim, Germany)
Pub Date : 2022-06-05 DOI: 10.1002/ntls.20220015
K. Pagel
This Research Highlight showcases the Research Paper entitled, Big cohort metabolomic profiling of serum for oral squamous cell carcinoma screening and diagnosis, https
本研究重点展示了题为《口腔鳞状细胞癌筛查和诊断的血清大队列代谢组学分析》的研究论文
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引用次数: 0
Gravity enables self‐assembly 重力使自组装成为可能
Natural sciences (Weinheim, Germany)
Pub Date : 2022-05-31 DOI: 10.1002/ntls.20220007
I. Grega, A. Shaikeea, H. Wadley, V. Deshpande
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引用次数: 1
Capture the missing: formation of (PbBi 3 ) − and {[AuPb 5 Bi 3 ] 2 } 4− via atom exchange 捕获缺失:通过原子交换形成(pbbi3)−和{[aupb5bi3] 2} 4−
Natural sciences (Weinheim, Germany)
Pub Date : 2022-05-25 DOI: 10.1002/ntls.202103302
Fuxing Pan, Lukas Guggolz, S. Dehnen
{"title":"Capture the missing: formation of (PbBi\u0000 <sub>3</sub>\u0000 )\u0000 <sup>−</sup>\u0000 and {[AuPb\u0000 <sub>5</sub>\u0000 Bi\u0000 <sub>3</sub>\u0000 ]\u0000 <sub>2</sub>\u0000 }\u0000 <sup>4−</sup>\u0000 via atom exchange","authors":"Fuxing Pan, Lukas Guggolz, S. Dehnen","doi":"10.1002/ntls.202103302","DOIUrl":"https://doi.org/10.1002/ntls.202103302","url":null,"abstract":"","PeriodicalId":74244,"journal":{"name":"Natural sciences (Weinheim, Germany)","volume":null,"pages":null},"PeriodicalIF":0.0,"publicationDate":"2022-05-25","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"83203030","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 1
Tuning protecto‐flexibility in nature: Case of the fish scale 调整保护-灵活性在自然界:鱼鳞的情况
Natural sciences (Weinheim, Germany)
Pub Date : 2022-03-11 DOI: 10.1002/ntls.20210097
S. Murcia, S. Ghods, Alexander Ossa, D. Arola
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引用次数: 3
Supramolecular p/n‐heterojunction of C 60 ‐functionalized bis(merocyanine) quadruple stack: A model system for charge carrier separation and recombination in organic solar cells c60功能化双(merocyanine)四层堆叠的超分子p/n异质结:有机太阳能电池中载流子分离和重组的模型系统
Natural sciences (Weinheim, Germany)
Pub Date : 2022-03-10 DOI: 10.1002/ntls.20210430
D. Bialas, F. Fennel, Niklas Noll, M. Holzapfel, A. Schmiedel, C. Lambert, F. Würthner
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引用次数: 0
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