Pub Date : 2026-01-20DOI: 10.1007/s11433-025-2797-y
Guangyao Huang, Jibang Fu, Xiaofeng Yi, Weichen Wang, Bo Ren, Zhaohua Yang, Shichuan Xue, Xinfang Zhang, Mingtang Deng
Majorana zero modes (MZMs), promising for topological quantum computation, are naturally hosted in vortices of two-dimensional topological superconductors (TSCs). However, precise control and braiding of these vortex-bound MZMs remain a significant challenge. This work proposes and numerically demonstrates a novel braiding scheme utilizing a programmable matrix of spintransfer torque (STT) devices (STT-matrix) integrated with a TSC layer. By selectively activating individual STT elements, their localized stray fields enable deterministic manipulation, including driving, braiding, and fusion, of superconducting vortices and their associated MZMs. We establish a comprehensive simulation framework combining finite element analysis for STT-induced vortex formation, time-dependent Ginzburg-Landau equations for vortex dynamics and time-dependent Bogoliubov-de Gennes equations for MZM evolution. Simulations confirm the STT-matrix’s capability for high-fidelity vortex manipulation and demonstrate MZM braiding dynamics. We quantify the impact of vortex acceleration and finite MZM coupling on braiding fidelity, showing that it can be optimized by adjusting STT spacing and vortex separation. Furthermore, we demonstrate controlled MZM fusion and measure the resultant energy splitting. This STT-matrix-based approach offers a highly versatile, scalable, and potentially practical platform for operating MZMs within TSC vortices, advancing the development of fault-tolerant topological quantum computation.
马约拉纳零模式(Majorana zero mode, MZMs)是一种很有希望用于拓扑量子计算的零模式,通常存在于二维拓扑超导体(tsc)的涡旋中。然而,精确控制和编织这些涡束缚的MZMs仍然是一个重大的挑战。这项工作提出并数值演示了一种新的编织方案,利用可编程的自旋传递扭矩(STT)器件矩阵(STT矩阵)集成了TSC层。通过选择性地激活单个STT元件,它们的局部杂散场可以实现超导涡旋及其相关MZMs的驱动、编织和融合等确定性操作。我们建立了一个综合的模拟框架,将stt诱导涡旋形成的有限元分析、涡旋动力学的时变Ginzburg-Landau方程和MZM演化的时变Bogoliubov-de Gennes方程相结合。仿真验证了stt -矩阵的高保真涡旋操纵能力,并演示了MZM编织动力学。我们量化了涡加速度和有限MZM耦合对编织保真度的影响,表明可以通过调整STT间距和涡距来优化编织保真度。此外,我们还演示了可控的MZM聚变,并测量了由此产生的能量分裂。这种基于stt矩阵的方法为在TSC涡旋中操作mzm提供了一个高度通用、可扩展和潜在实用的平台,促进了容错拓扑量子计算的发展。
{"title":"Scheme for braiding Majorana zero modes in vortices using STT-matrix","authors":"Guangyao Huang, Jibang Fu, Xiaofeng Yi, Weichen Wang, Bo Ren, Zhaohua Yang, Shichuan Xue, Xinfang Zhang, Mingtang Deng","doi":"10.1007/s11433-025-2797-y","DOIUrl":"10.1007/s11433-025-2797-y","url":null,"abstract":"<div><p>Majorana zero modes (MZMs), promising for topological quantum computation, are naturally hosted in vortices of two-dimensional topological superconductors (TSCs). However, precise control and braiding of these vortex-bound MZMs remain a significant challenge. This work proposes and numerically demonstrates a novel braiding scheme utilizing a programmable matrix of spintransfer torque (STT) devices (STT-matrix) integrated with a TSC layer. By selectively activating individual STT elements, their localized stray fields enable deterministic manipulation, including driving, braiding, and fusion, of superconducting vortices and their associated MZMs. We establish a comprehensive simulation framework combining finite element analysis for STT-induced vortex formation, time-dependent Ginzburg-Landau equations for vortex dynamics and time-dependent Bogoliubov-de Gennes equations for MZM evolution. Simulations confirm the STT-matrix’s capability for high-fidelity vortex manipulation and demonstrate MZM braiding dynamics. We quantify the impact of vortex acceleration and finite MZM coupling on braiding fidelity, showing that it can be optimized by adjusting STT spacing and vortex separation. Furthermore, we demonstrate controlled MZM fusion and measure the resultant energy splitting. This STT-matrix-based approach offers a highly versatile, scalable, and potentially practical platform for operating MZMs within TSC vortices, advancing the development of fault-tolerant topological quantum computation.</p></div>","PeriodicalId":774,"journal":{"name":"Science China Physics, Mechanics & Astronomy","volume":"69 4","pages":""},"PeriodicalIF":7.5,"publicationDate":"2026-01-20","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"146082532","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2026-01-19DOI: 10.1007/s11433-025-2854-8
Luting Xu, Lingzhen Guo
Chiral and nonreciprocal quantum devices are crucial for signal routing and processing in a quantum network. In this work, we study the chirality and nonreciprocity of a giant atom coupled to a one-dimensional waveguide. We clarify that the chiral emission of the giant atom is not directly related to the time-reversal symmetry breaking but to the mirror-symmetry breaking. We propose a passive scheme, by extending the legs of the giant atom, to realize the chiral emission without breaking time-reversal symmetry. We prove that the time-reversal symmetry breaking alone via nonuniform coupling phases is not sufficient for the nonreciprocal single-photon scattering of the giant atom. The nonreciprocity needs both the time-reversal symmetry breaking and the finite external dissipation of the giant atom. Our work clarifies the roles of symmetries in the chirality and nonreciprocity of giant-atom systems and paves the way for the design of on-chip functional devices with superconducting giant atoms.
{"title":"Chirality, nonreciprocity and symmetries for a giant atom","authors":"Luting Xu, Lingzhen Guo","doi":"10.1007/s11433-025-2854-8","DOIUrl":"10.1007/s11433-025-2854-8","url":null,"abstract":"<div><p>Chiral and nonreciprocal quantum devices are crucial for signal routing and processing in a quantum network. In this work, we study the chirality and nonreciprocity of a giant atom coupled to a one-dimensional waveguide. We clarify that the chiral emission of the giant atom is not directly related to the time-reversal symmetry breaking but to the mirror-symmetry breaking. We propose a passive scheme, by extending the legs of the giant atom, to realize the chiral emission without breaking time-reversal symmetry. We prove that the time-reversal symmetry breaking alone via nonuniform coupling phases is not sufficient for the nonreciprocal single-photon scattering of the giant atom. The nonreciprocity needs both the time-reversal symmetry breaking and the finite external dissipation of the giant atom. Our work clarifies the roles of symmetries in the chirality and nonreciprocity of giant-atom systems and paves the way for the design of on-chip functional devices with superconducting giant atoms.</p></div>","PeriodicalId":774,"journal":{"name":"Science China Physics, Mechanics & Astronomy","volume":"69 4","pages":""},"PeriodicalIF":7.5,"publicationDate":"2026-01-19","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"146082828","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2026-01-16DOI: 10.1007/s11433-025-2861-x
Yu-Han Cao, Kai-Yue Jiang, Hong-Yan Lu, Da Wang, Qiang-Hua Wang
Recently, the films of the Ruddlesden-Popper (RP) nickelate superconductors, in which the (La,Pr)3Ni2O7 system exhibits a remarkable transition temperature Tc exceeding 40 K, were synthesized at ambient pressure. We systematically investigate the band structures and electronic correlation effects to identify the key factors controlling superconductivity and pathways to enhance Tc. Based on density functional theory (DFT) calculations, we construct a bilayer two-orbital ((3d_{{3{z}^{2}}-{r}^{2}}) and (3d_{{{x}^{2}}-{y}^{2}})) tight-binding model for a series of in-plane compression mimicking the substrate effect. We find the band energy at the M point drops with the compression, leading to an increase in the density of states at the Fermi level, in stark contrast to the behavior of the bulk under pressure. We then apply the functional renormalization group (FRG) method to study the electronic correlation effect on the superconductivity. We find the s±-wave pairing symmetry remains robust in the films, the same as the bulk. But somewhat surprisingly, for the films, we find Tc can be enhanced by reducing the in-plane lattice constant, increasing the out-of-plane lattice constant, or further electron-doping. These findings are consistent with the itinerant picture of the superconductivity induced by spin-fluctuations and provide theoretical support for further boosting Tc in future experiments.
{"title":"Strain-engineered electronic structure and superconductivity in La3Ni2O7 thin films","authors":"Yu-Han Cao, Kai-Yue Jiang, Hong-Yan Lu, Da Wang, Qiang-Hua Wang","doi":"10.1007/s11433-025-2861-x","DOIUrl":"10.1007/s11433-025-2861-x","url":null,"abstract":"<div><p>Recently, the films of the Ruddlesden-Popper (RP) nickelate superconductors, in which the (La,Pr)<sub>3</sub>Ni<sub>2</sub>O<sub>7</sub> system exhibits a remarkable transition temperature <i>T</i><sub><i>c</i></sub> exceeding 40 K, were synthesized at ambient pressure. We systematically investigate the band structures and electronic correlation effects to identify the key factors controlling superconductivity and pathways to enhance <i>T</i><sub><i>c</i></sub>. Based on density functional theory (DFT) calculations, we construct a bilayer two-orbital (<span>(3d_{{3{z}^{2}}-{r}^{2}})</span> and <span>(3d_{{{x}^{2}}-{y}^{2}})</span>) tight-binding model for a series of in-plane compression mimicking the substrate effect. We find the band energy at the <i>M</i> point drops with the compression, leading to an increase in the density of states at the Fermi level, in stark contrast to the behavior of the bulk under pressure. We then apply the functional renormalization group (FRG) method to study the electronic correlation effect on the superconductivity. We find the <i>s</i><sub>±</sub>-wave pairing symmetry remains robust in the films, the same as the bulk. But somewhat surprisingly, for the films, we find <i>T</i><sub><i>c</i></sub> can be enhanced by reducing the in-plane lattice constant, increasing the out-of-plane lattice constant, or further electron-doping. These findings are consistent with the itinerant picture of the superconductivity induced by spin-fluctuations and provide theoretical support for further boosting <i>T</i><sub><i>c</i></sub> in future experiments.</p></div>","PeriodicalId":774,"journal":{"name":"Science China Physics, Mechanics & Astronomy","volume":"69 4","pages":""},"PeriodicalIF":7.5,"publicationDate":"2026-01-16","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"146082893","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
The growing usage of industrial dyes makes the sewage treatment a global issue, therefore low-cost, highly efficient catalysts are urgently demanded for wastewater purification. We present an ultrasonic-engineered catalytic technology, which can achieve an extremely high efficiency in azo dye degradation via a tiny dosage of 0.1 g L−1 (only one-fifth of the normally used dosage) Fe81Si9B10 amorphous powders (APs) with a low activation energy of 45.32 kJ mol−1 and a high reaction rate of 0.70291 min−1. The non-destructive ultrasonic vibration (UV) treatment with very short processing times (0.43–1.08 s) amplifies degradation efficiency by an astonishing 55-fold compared to untreated APs. Combined with high-energy X-ray diffraction and small-angle neutron scattering analyses, we reveal that the UV-induced structural reconstruction at both short- and medium-range order effectively lower reaction energy barriers while accelerating charge transfer kinetics. The high-energy ultrasonic attacks promote the exposure of massive fresh active sites, which enhance the Fe2+/Fe3+ redox circulation and thereby lead to the fast Fenton-like oxidation processes. By integrating ultrasonic physics with amorphous materials, this work develops an energy-efficient catalytic activation method, enabling sustainable water purification and innovative pollutant treatment strategies.
随着工业染料的使用日益增多,污水处理成为一个全球性问题,因此迫切需要低成本、高效的废水净化催化剂。本文提出了一种超声催化技术,通过0.1 g L−1(仅为常用用量的五分之一)的Fe81Si9B10非晶粉末(APs),以45.32 kJ mol−1的低活化能和0.70291 min−1的高反应速率,实现了偶氮染料的高效降解。与未经处理的APs相比,非破坏性超声振动(UV)处理的降解效率提高了55倍,处理时间非常短(0.43-1.08秒)。结合高能x射线衍射和小角中子散射分析,我们发现紫外诱导的中短程结构重构有效地降低了反应能垒,同时加速了电荷转移动力学。高能超声攻击促进了大量新鲜活性位点的暴露,增强了Fe2+/Fe3+的氧化还原循环,从而导致快速的Fenton-like氧化过程。通过将超声物理与非晶材料相结合,本研究开发了一种节能的催化活化方法,实现了可持续的水净化和创新的污染物处理策略。
{"title":"A highly efficient amorphous catalyst achieved by ultrasonic vibration","authors":"Jiayi Ruan, Wei Li, Chenchen Yuan, Luyao Li, Weihang Feng, Wei He, Tao Lu, Fujun Lan, Qiaoshi Zeng, Yujiao Lu, Zheng Wang, Xuelian Wu, Yubing Ke, Hua Yang, Jiang Ma, Ye Pan, Weihua Wang","doi":"10.1007/s11433-025-2845-y","DOIUrl":"10.1007/s11433-025-2845-y","url":null,"abstract":"<div><p>The growing usage of industrial dyes makes the sewage treatment a global issue, therefore low-cost, highly efficient catalysts are urgently demanded for wastewater purification. We present an ultrasonic-engineered catalytic technology, which can achieve an extremely high efficiency in azo dye degradation via a tiny dosage of 0.1 g L<sup>−1</sup> (only one-fifth of the normally used dosage) Fe<sub>81</sub>Si<sub>9</sub>B<sub>10</sub> amorphous powders (APs) with a low activation energy of 45.32 kJ mol<sup>−1</sup> and a high reaction rate of 0.70291 min<sup>−1</sup>. The non-destructive ultrasonic vibration (UV) treatment with very short processing times (0.43–1.08 s) amplifies degradation efficiency by an astonishing 55-fold compared to untreated APs. Combined with high-energy X-ray diffraction and small-angle neutron scattering analyses, we reveal that the UV-induced structural reconstruction at both short- and medium-range order effectively lower reaction energy barriers while accelerating charge transfer kinetics. The high-energy ultrasonic attacks promote the exposure of massive fresh active sites, which enhance the Fe<sup>2+</sup>/Fe<sup>3+</sup> redox circulation and thereby lead to the fast Fenton-like oxidation processes. By integrating ultrasonic physics with amorphous materials, this work develops an energy-efficient catalytic activation method, enabling sustainable water purification and innovative pollutant treatment strategies.</p></div>","PeriodicalId":774,"journal":{"name":"Science China Physics, Mechanics & Astronomy","volume":"69 3","pages":""},"PeriodicalIF":7.5,"publicationDate":"2026-01-15","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"146082332","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2026-01-15DOI: 10.1007/s11433-025-2777-1
Hengyu Gao, Shaodong Ding, Ziyang Liu, Jiefu Zhang, Bolun Li, Zhiwu An, Li Wang, Jing Jing, Tao Liu, Yubo Fan, Zhongtao Hu
Accurate targeting is critical for the effectiveness of transcranial focused ultrasound (tFUS) neuromodulation. While CT provides accurate skull acoustic properties, its ionizing radiation and poor soft tissue contrast limit clinical applicability. In contrast, MRI offers superior neuroanatomical visualization without radiation exposure but lacks skull property mapping. This study proposes a novel, fully CT-free simulation framework that integrates MRI-derived synthetic CT (sCT) with efficient modeling techniques for rapid and precise tFUS targeting. We trained a deep-learning model to generate sCT from T1-weighted MRI and integrated it with both full-wave (k-Wave) and accelerated simulation methods—hybrid angular spectrum (kW-ASM) and Rayleigh-Sommerfeld ASM (RS-ASM). Across five skull models, both full-wave and hybrid pipelines using sCT demonstrated sub-millimeter targeting deviation, focal shape consistency (FWHM ∼3.3–3.8 mm), and <0.2 normalized pressure error compared to CT-based gold standard. Notably, the kW-ASM and RS-ASM pipelines reduced simulation time from (∼3320 ±1270) to (187±27) and (345±85) s respectively, achieving ∼94% and ∼90% time savings. These results confirm that MRI-derived sCT combined with innovative rapid simulation techniques enables fast, accurate, and radiation-free tFUS planning, supporting its feasibility for scalable clinical applications.
{"title":"Rapid simulation framework integrating MRI-derived synthetic CT for precise transcranial focused ultrasound targeting","authors":"Hengyu Gao, Shaodong Ding, Ziyang Liu, Jiefu Zhang, Bolun Li, Zhiwu An, Li Wang, Jing Jing, Tao Liu, Yubo Fan, Zhongtao Hu","doi":"10.1007/s11433-025-2777-1","DOIUrl":"10.1007/s11433-025-2777-1","url":null,"abstract":"<div><p>Accurate targeting is critical for the effectiveness of transcranial focused ultrasound (tFUS) neuromodulation. While CT provides accurate skull acoustic properties, its ionizing radiation and poor soft tissue contrast limit clinical applicability. In contrast, MRI offers superior neuroanatomical visualization without radiation exposure but lacks skull property mapping. This study proposes a novel, fully CT-free simulation framework that integrates MRI-derived synthetic CT (sCT) with efficient modeling techniques for rapid and precise tFUS targeting. We trained a deep-learning model to generate sCT from T1-weighted MRI and integrated it with both full-wave (k-Wave) and accelerated simulation methods—hybrid angular spectrum (kW-ASM) and Rayleigh-Sommerfeld ASM (RS-ASM). Across five skull models, both full-wave and hybrid pipelines using sCT demonstrated sub-millimeter targeting deviation, focal shape consistency (FWHM ∼3.3–3.8 mm), and <0.2 normalized pressure error compared to CT-based gold standard. Notably, the kW-ASM and RS-ASM pipelines reduced simulation time from (∼3320 ±1270) to (187±27) and (345±85) s respectively, achieving ∼94% and ∼90% time savings. These results confirm that MRI-derived sCT combined with innovative rapid simulation techniques enables fast, accurate, and radiation-free tFUS planning, supporting its feasibility for scalable clinical applications.</p></div>","PeriodicalId":774,"journal":{"name":"Science China Physics, Mechanics & Astronomy","volume":"69 10","pages":""},"PeriodicalIF":7.5,"publicationDate":"2026-01-15","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"146045511","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2026-01-14DOI: 10.1007/s11433-025-2873-4
Jia-Jia Lu, Fan-Chi Zeng, Tian-Yu Zhao, Wen-Hao Qi, Ge Yan, Wen-Ming Zhang, Li Cheng
The performance sensitivity of quasi-zero-stiffness (QZS) isolators to load-position mismatches poses significant challenges and hinders their practical implementation. Herein, a translation-scaling coordinated transformation method is proposed for decoupled adjustment of the rated load and equilibrium position. By coordinating translation and scaling transformations of negative and positive stiffnesses, the rated load and equilibrium position can be independently tuned, thereby mitigating performance sensitivity under time-varying operating conditions. Based on this method, a load-position decoupled QZS isolator (LPD-QZS) is developed and systematically investigated. A liftable nested magnet-coil pair is employed to generate translatable and scalable negative stiffness, while an end-to-end magnet-coil pair combined with a membrane spring pair provides nonuniformly scalable positive stiffness. Analyses reveal and verify the tunable stiffness characteristics and the effectiveness of the translation-scaling coordinated transformation in achieving load-position decoupled adjustment, as well as the distinctive behavior arising from it. Finally, offline and online tests are conducted to evaluate the robustness of the LPD-QZS under varying rated loads and equilibrium positions. Sweep excitation tests indicate that the LPD-QZS exhibits excellent low-frequency vibration isolation performance, with a low isolation frequency starting from 3.3 Hz, in drastic contrast with the degraded performance without load-position decoupled adjustment under load-position mismatches. Significantly, through translation-scaling coordinated transformation, the LPD-QZS preserves its QZS characteristic across various applied loads and operating positions, highlighting its potential for practical engineering applications, particularly in multi-leg QZS platforms.
{"title":"Load-position decoupled quasi-zero stiffness vibration isolation via translation-scaling coordinated transformation","authors":"Jia-Jia Lu, Fan-Chi Zeng, Tian-Yu Zhao, Wen-Hao Qi, Ge Yan, Wen-Ming Zhang, Li Cheng","doi":"10.1007/s11433-025-2873-4","DOIUrl":"10.1007/s11433-025-2873-4","url":null,"abstract":"<div><p>The performance sensitivity of quasi-zero-stiffness (QZS) isolators to load-position mismatches poses significant challenges and hinders their practical implementation. Herein, a translation-scaling coordinated transformation method is proposed for decoupled adjustment of the rated load and equilibrium position. By coordinating translation and scaling transformations of negative and positive stiffnesses, the rated load and equilibrium position can be independently tuned, thereby mitigating performance sensitivity under time-varying operating conditions. Based on this method, a load-position decoupled QZS isolator (LPD-QZS) is developed and systematically investigated. A liftable nested magnet-coil pair is employed to generate translatable and scalable negative stiffness, while an end-to-end magnet-coil pair combined with a membrane spring pair provides nonuniformly scalable positive stiffness. Analyses reveal and verify the tunable stiffness characteristics and the effectiveness of the translation-scaling coordinated transformation in achieving load-position decoupled adjustment, as well as the distinctive behavior arising from it. Finally, offline and online tests are conducted to evaluate the robustness of the LPD-QZS under varying rated loads and equilibrium positions. Sweep excitation tests indicate that the LPD-QZS exhibits excellent low-frequency vibration isolation performance, with a low isolation frequency starting from 3.3 Hz, in drastic contrast with the degraded performance without load-position decoupled adjustment under load-position mismatches. Significantly, through translation-scaling coordinated transformation, the LPD-QZS preserves its QZS characteristic across various applied loads and operating positions, highlighting its potential for practical engineering applications, particularly in multi-leg QZS platforms.</p></div>","PeriodicalId":774,"journal":{"name":"Science China Physics, Mechanics & Astronomy","volume":"69 4","pages":""},"PeriodicalIF":7.5,"publicationDate":"2026-01-14","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"146027146","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
The discovery of superconductivity in pressurized Ruddlesden-Popper (RP) nickelates has provided new perspectives on the mechanism of high-temperature superconductivity. Up to now, most experiments concentrated on the lanthanum-related RP phase, so the discovery of new superconducting RP nickelates is highly desirable to reveal their generality. Here we report the observation of superconductivity in Pr4Ni3O10 single crystals above 10 GPa, achieving a maximum Tc of 39 K without saturation, significantly exceeding the value of 25–30 K of La4Ni3O10. Ultrasensitive magnetic susceptibility measurements under high pressure indicate bulk superconductivity with appreciable superconducting volume fractions. Unlike La4Ni3O10, the electronic structure of the high-pressure phase of Pr4Ni3O10 exhibits a dramatic metallization of the σ-bonding band consisting of three (d_{z^{2}}) orbitals and van Hove singularity of coupled bands of (d_{x^{2}-y^{2}}) orbitals near the Fermi level, similar to La3Ni2O7. These findings reveal some generic features of both crystal and electronic structures for high-temperature superconductivity in nickelates and multi-layer cuprates.
{"title":"Unveiling pressurized bulk superconductivity in a trilayer nickelate Pr4Ni3O10 single crystal","authors":"Cuiying Pei, Mingxin Zhang, Di Peng, Yang Shen, Shangxiong Huangfu, Shihao Zhu, Qi Wang, Juefei Wu, Junjie Wang, Zhenfang Xing, Lili Zhang, Hirokazu Kadobayashi, Saori I. Kawaguchi, Yulin Chen, Jinkui Zhao, Wenge Yang, Hongli Suo, Hanjie Guo, Qiaoshi Zeng, Guang-Ming Zhang, Yanpeng Qi","doi":"10.1007/s11433-025-2852-4","DOIUrl":"10.1007/s11433-025-2852-4","url":null,"abstract":"<div><p>The discovery of superconductivity in pressurized Ruddlesden-Popper (RP) nickelates has provided new perspectives on the mechanism of high-temperature superconductivity. Up to now, most experiments concentrated on the lanthanum-related RP phase, so the discovery of new superconducting RP nickelates is highly desirable to reveal their generality. Here we report the observation of superconductivity in Pr<sub>4</sub>Ni<sub>3</sub>O<sub>10</sub> single crystals above 10 GPa, achieving a maximum <i>T</i><sub>c</sub> of 39 K without saturation, significantly exceeding the value of 25–30 K of La<sub>4</sub>Ni<sub>3</sub>O<sub>10</sub>. Ultrasensitive magnetic susceptibility measurements under high pressure indicate bulk superconductivity with appreciable superconducting volume fractions. Unlike La<sub>4</sub>Ni<sub>3</sub>O<sub>10</sub>, the electronic structure of the high-pressure phase of Pr<sub>4</sub>Ni<sub>3</sub>O<sub>10</sub> exhibits a dramatic metallization of the σ-bonding band consisting of three <span>(d_{z^{2}})</span> orbitals and van Hove singularity of coupled bands of <span>(d_{x^{2}-y^{2}})</span> orbitals near the Fermi level, similar to La<sub>3</sub>Ni<sub>2</sub>O<sub>7</sub>. These findings reveal some generic features of both crystal and electronic structures for high-temperature superconductivity in nickelates and multi-layer cuprates.</p></div>","PeriodicalId":774,"journal":{"name":"Science China Physics, Mechanics & Astronomy","volume":"69 3","pages":""},"PeriodicalIF":7.5,"publicationDate":"2026-01-13","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"146026724","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2026-01-09DOI: 10.1007/s11433-025-2862-6
Jialin Chen, Chuanshu Xu, Qiaoyi Li, Wei Li
The recently discovered trilayer nickelate superconductor La4Ni3O10 under pressure has emerged as a promising platform for exploring unconventional superconductivity. However, the pairing mechanism remains a subject of active investigations. With large-scale density matrix renormalization group calculations on a realistic two-orbital trilayer Hubbard model, we elucidate the superconducting (SC) mechanism in this system. Our results reveal distinct magnetic correlations in the two different orbitals: while the (d_{{z}^{2}}) orbital exhibits both interlayer and cross-layer antiferromagnetic (AFM) correlations, the (d_{{x}^{2} - {y}^{2}}) orbital shows exclusively cross-layer AFM correlations, rendering a quasi-long-range SC order in the latter. We demonstrate that the Hund’s rule coupling is essential for forming the SC order, and discuss the effects of kinetic AFM correlation and Hubbard repulsive U. Our findings motivate a further simplification of the trilayer Hubbard to an effective bilayer mixed-dimensional Hubbard model, providing a unified framework for understanding interlayer SC in both trilayer and bilayer nickelates.
{"title":"Magnetically mediated cross-layer pairing in pressurized trilayer nickelate La4Ni3O10","authors":"Jialin Chen, Chuanshu Xu, Qiaoyi Li, Wei Li","doi":"10.1007/s11433-025-2862-6","DOIUrl":"10.1007/s11433-025-2862-6","url":null,"abstract":"<div><p>The recently discovered trilayer nickelate superconductor La<sub>4</sub>Ni<sub>3</sub>O<sub>10</sub> under pressure has emerged as a promising platform for exploring unconventional superconductivity. However, the pairing mechanism remains a subject of active investigations. With large-scale density matrix renormalization group calculations on a realistic two-orbital trilayer Hubbard model, we elucidate the superconducting (SC) mechanism in this system. Our results reveal distinct magnetic correlations in the two different orbitals: while the <span>(d_{{z}^{2}})</span> orbital exhibits both interlayer and cross-layer antiferromagnetic (AFM) correlations, the <span>(d_{{x}^{2} - {y}^{2}})</span> orbital shows exclusively cross-layer AFM correlations, rendering a quasi-long-range SC order in the latter. We demonstrate that the Hund’s rule coupling is essential for forming the SC order, and discuss the effects of kinetic AFM correlation and Hubbard repulsive <i>U</i>. Our findings motivate a further simplification of the trilayer Hubbard to an effective bilayer mixed-dimensional Hubbard model, providing a unified framework for understanding interlayer SC in both trilayer and bilayer nickelates.</p></div>","PeriodicalId":774,"journal":{"name":"Science China Physics, Mechanics & Astronomy","volume":"69 4","pages":""},"PeriodicalIF":7.5,"publicationDate":"2026-01-09","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"146026838","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
The discovery of Ni-based superconductors has brought new hope to the field of high-temperature superconductivity. Understanding the dimensional characteristics and anisotropy of nickelate superconductors has become a central focus in current research. However, the nature of the nickelate superconductivity, especially the transition between 2D and 3D superconductivity, remains debated. In this study, we investigated the magnetic field-dependent electrical transport behaviors of infinite-layer nickelates. The La0.8Sr0.2NiO2 films exhibit highly anisotropic superconductivity, which fits well with the 2D Tinkham model, indicating a purely 2D superconducting nature. In contrast, the Nd0.8Sr0.2NiO2 films show isotropic behavior with a mixed 2D + 3D superconducting characteristics. This “mixed 2D + 3D superconducting behavior” is typically associated with the complexity of the electronic band structure in the material. Through a systematic comparison of two model systems with distinct rare-earth orbital contributions, we propose a new perspective based on orbital selectivity. The observed difference likely originates from Nd0.8Sr0.2NiO2 incorporates the Nd (5d_{{z}^{2}}) orbital, adding a 3D component. Its interaction with the Ni (3d_{{x}^{2} - {y}^{2}}) orbital leads to orbital-selective pairing. Theoretical calculations provide key evidence that the Nd-based system exhibits greater isotropy and 3D character compared to the La-based system. Our study thus suggests that orbital selectivity serves as a critical mechanism governing the superconducting properties, and the distinction between rare-earth elements (such as La and Nd) ultimately influences the dimensional characteristics of superconductivity through this mechanism.
{"title":"Electrical transport and dimensionality control in infinite-layer nickelates","authors":"Yan Zhao, Minghui Xu, Lingyi Ao, Fanrong Lin, Xiangru Han, Hangbo Qi, Ke Zhang, Huaqian Leng, Yu Chen, Wenbo Yang, Xiaoqiang Wu, Yong Zhao, Haiyan Xiao, Bing Huang, Yanpeng Liu, Hongtao Yuan, Yanrong Li, Liang Qiao","doi":"10.1007/s11433-025-2843-8","DOIUrl":"10.1007/s11433-025-2843-8","url":null,"abstract":"<div><p>The discovery of Ni-based superconductors has brought new hope to the field of high-temperature superconductivity. Understanding the dimensional characteristics and anisotropy of nickelate superconductors has become a central focus in current research. However, the nature of the nickelate superconductivity, especially the transition between 2D and 3D superconductivity, remains debated. In this study, we investigated the magnetic field-dependent electrical transport behaviors of infinite-layer nickelates. The La<sub>0.8</sub>Sr<sub>0.2</sub>NiO<sub>2</sub> films exhibit highly anisotropic superconductivity, which fits well with the 2D Tinkham model, indicating a purely 2D superconducting nature. In contrast, the Nd<sub>0.8</sub>Sr<sub>0.2</sub>NiO<sub>2</sub> films show isotropic behavior with a mixed 2D + 3D superconducting characteristics. This “mixed 2D + 3D superconducting behavior” is typically associated with the complexity of the electronic band structure in the material. Through a systematic comparison of two model systems with distinct rare-earth orbital contributions, we propose a new perspective based on orbital selectivity. The observed difference likely originates from Nd<sub>0.8</sub>Sr<sub>0.2</sub>NiO<sub>2</sub> incorporates the Nd <span>(5d_{{z}^{2}})</span> orbital, adding a 3D component. Its interaction with the Ni <span>(3d_{{x}^{2} - {y}^{2}})</span> orbital leads to orbital-selective pairing. Theoretical calculations provide key evidence that the Nd-based system exhibits greater isotropy and 3D character compared to the La-based system. Our study thus suggests that orbital selectivity serves as a critical mechanism governing the superconducting properties, and the distinction between rare-earth elements (such as La and Nd) ultimately influences the dimensional characteristics of superconductivity through this mechanism.</p></div>","PeriodicalId":774,"journal":{"name":"Science China Physics, Mechanics & Astronomy","volume":"69 3","pages":""},"PeriodicalIF":7.5,"publicationDate":"2026-01-08","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"146027033","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}