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Droplet impact on a wettability-patterned woven mesh 水滴对润湿性图案编织网的影响
Pub Date : 2023-06-08 DOI: 10.1002/dro2.53
Sotiris Catsoulis, Uddalok Sen, Jens H. Walther, Constantine M. Megaridis

Droplet impact and breakup on meshes are relevant to a number of applications involving filters, textiles, and other spatially inhomogeneous media encountering gas-dispersed liquids. This study presents high-resolution simulation results of mm-size droplets striking wettability-patterned meshes with the goal of (a) replicating prior physical experiments, (b) identifying sensitivities to the initial conditions and wettability of the mesh wires, and (c) studying the fluid-field dynamics when droplets strike such meshes. The insights from the present model may help to advance understanding of droplet atomization on meshes, which depends on a number of parameters that are nontrivial to control in an experimental setting. The analysis is carried out by benchmarking the numerical methods used in a commercial software package for orthogonal droplet impact on a flat smooth surface, followed by a convergence analysis, and finally, simulation of specific experiments and case studies involving wettability-patterned mesh targets. We show that the wettability contrast between the hydrophilic and hydrophobic domains on the mesh as well as the contact angle hysteresis on each side play a critical role in determining whether liquid pinch-off occurs. The three-dimensional computational framework constructed in this work is a step toward predicting the postimpact behavior of droplets that strike woven meshes and other porous inhomogeneous media consisting of materials with different wetting properties.

液滴对网格的冲击和破裂与许多应用有关,包括过滤器、纺织品和其他遇到气体分散液体的空间不均匀介质。本研究提供了mm尺寸液滴撞击润湿性图案化网格的高分辨率模拟结果,目的是(a)复制先前的物理实验,(b)确定对初始条件和网格线润湿性的敏感性,以及(c)研究液滴撞击此类网格时的流场动力学。本模型的见解可能有助于加深对网格上液滴雾化的理解,这取决于在实验环境中难以控制的许多参数。该分析是通过对商业软件包中使用的数值方法进行基准测试来进行的,该软件包用于在平坦光滑表面上进行正交液滴冲击,然后进行收敛性分析,最后模拟涉及润湿性图案化网格目标的具体实验和案例研究。我们表明,网格上亲水和疏水区域之间的润湿性对比以及每一侧的接触角滞后在决定是否发生液体夹断方面起着关键作用。这项工作中构建的三维计算框架是预测液滴撞击编织网和其他由具有不同润湿特性的材料组成的多孔非均匀介质的后冲击行为的一步。
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引用次数: 4
Droplet orthogonal impact on nonuniform wettability surfaces 液滴对不均匀润湿性表面的正交影响
Pub Date : 2023-05-23 DOI: 10.1002/dro2.63
Shashwata Moitra, Mohamed Elsharkawy, Antonio Russo, Sreya Sarkar, Ranjan Ganguly, Pietro Asinari, Constantine M. Megaridis

The vast majority of prior studies on droplet impact have focused on collisions of liquid droplets with spatially homogeneous (i.e., uniform-wettability) surfaces. But in recent years, there has been growing interest on droplet impact on nonuniform wettability surfaces, which are more relevant in practice. This paper presents first an experimental study of axisymmetric droplet impact on wettability-patterned surfaces. The experiments feature millimeter-sized water droplets impacting centrally with We<100 $Welt 100$ on a flat surface that has a circular region of wettability θ1 ${theta }_{1}$ (Area 1) surrounded by a region of wettability θ2 ${theta }_{2}$ (Area 2), where θ1<θ2 ${theta }_{1}lt {theta }_{2}$ (i.e., outer domain is less wettable than the inner one). Depending upon the droplet momentum at impact, the experiments reveal the existence of three possible regimes of axisymmetric spreading, namely (I) interior (only within Area 1) spreading, (II) contact-line entrapment at the periphery of Area 1, and (III) exterior (extending into Area 2) spreading. We present an analysis based on energetic principles for θ1<θ2 ${theta }_{1}lt {theta }_{2}$, and further extend it for cases where

绝大多数先前关于液滴撞击的研究都集中在液滴与空间均匀(即均匀润湿性)表面的碰撞上。但近年来,人们对液滴对不均匀润湿性表面的影响越来越感兴趣,这在实践中更具相关性。本文首次对轴对称液滴对润湿性图案表面的冲击进行了实验研究。实验的特征是毫米大小的水滴以W e<;100$Welt 100$在平坦表面上,该平坦表面具有被润湿区域包围的圆形润湿区域θ1${θ}_{1}$(区域1)θ2${θ}_{2}$(区域2),其中θ1<;θ2${θ}_{1}lt{θ}_{2}$(即,外域的可润湿性低于内域)。根据撞击时的液滴动量,实验揭示了轴对称扩散的三种可能状态的存在,即(I)内部(仅在区域1内)扩散,(II)区域1外围的接触线截留,以及(III)外部(延伸到区域2)扩散。我们基于能量原理对θ1<;θ2${θ}_{1}lt{θ}_{2}$,并将其进一步扩展到θ1>;θ2${θ}_{1}gt{θ{2}$(即,外域比内域更易润湿)。实验观察结果与分析模型的缩放和预测一致,从而概述了预测更复杂润湿性模式的液滴冲击行为的策略。
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引用次数: 0
Hybrid electrodes effective for both electrowetting- and dielectrowetting-driven digital microfluidics 混合电极对电润湿和介电润湿驱动的数字微流体都有效
Pub Date : 2023-05-11 DOI: 10.1002/dro2.58
Hongyao Geng, Sung Kwon Cho

Electrowetting on dielectric (EWOD) and dielectrowetting (DEW) are two major principles to drive droplets in digital microfluidics. EWOD is effective to manipulate (create, transport, split, and merge) conductive droplets being currently used for many biological, chemical, and optical applications. DEW can also manipulate droplets but more efficiently with dielectric (nonconductive) fluids. A digital microfluidic platform efficiently operable by both EWOD and DEW would offer higher versatility in handling a wide range of fluids, regardless of their conductivities. In this regard, this article presents a new hybrid electrode design enabling EWOD and DEW to drive various kinds of droplet fluids on a single platform. In addition, a slippery liquid-infused surface (SLIPS) is integrated with the hybrid electrodes. The SLIPS is well known to resist biofouling and repel sticky fluids, which endows the hybrid electrodes with much wider application spectra. As a result, the present SLIPS-integrated hybrid electrodes facilitate actuating various kinds of fluids which would not be driven by conventional EWOD and/or DEW electrodes. This paper presents the successful transportation of not only conductive fluids including water, protein solution, glycerol, and honey but also nonconductive fluids including dodecane, silicone oil, and light and heavy crude oil, all driven by the SLIPS-integrated hybrid electrodes. The performance comparisons among solid, interdigitating, and hybrid electrodes are made by testing both conductive and nonconductive droplets.

电介质电润湿(EWOD)和介电润湿(DEW)是数字微流体中驱动液滴的两个主要原理。EWOD可以有效地操纵(创建、传输、分裂和合并)导电液滴,目前用于许多生物、化学和光学应用。DEW也可以操纵液滴,但使用介电(非导电)流体更有效。EWOD和DEW都能有效操作的数字微流体平台将在处理各种流体方面提供更高的通用性,无论其电导率如何。在这方面,本文提出了一种新的混合电极设计,使EWOD和DEW能够在单个平台上驱动各种液滴。此外,光滑的液体注入表面(SLIPS)与混合电极集成在一起。众所周知,SLIPS可以抵抗生物污垢和排斥粘性流体,这使混合电极具有更宽的应用范围。结果,本发明的SLIPS集成混合电极有助于致动各种流体,这些流体将不会由传统的EWOD和/或DEW电极驱动。本文介绍了SLIPS集成混合电极驱动的不仅包括水、蛋白质溶液、甘油和蜂蜜在内的导电流体,还包括十二烷、硅油以及轻质和重质原油在内的非导电流体的成功输送。通过测试导电液滴和非导电液滴,对固体电极、叉指电极和混合电极的性能进行了比较。
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引用次数: 4
Inside Front Cover, Volume 2, Number 2, April 2023 封面内侧,第2卷,第2期,2023年4月
Pub Date : 2023-04-18 DOI: 10.1002/dro2.62
Xiaolong Yang, Biao Qi, Yao Lu, Wang Zhang, Xiaolei Wang

Inside Front Cover: The cover image is based on the Research Article Bionic surface diode for droplet steering by Yang et al.

Ultraslippery patterned surfaces with significant droplet sliding anisotropy were created by coordinating the heterogeneous wettability of the back of dessert beetle, directional-dependent architecture of butterfly wing, and ultraslippery configuration of Nepenthes alata. The sliding anisotropy of the functional surface is threefold higher than that of natural butterfly wings, which enables the simultaneous handling of multiple droplets without mass loss. (DOI: 10.1002/dro2.46)

封面内侧:封面图像基于Yang等人的研究文章《用于液滴操纵的仿生表面二极管》。通过协调甜点甲虫背部的不均匀润湿性、蝴蝶翅膀的方向依赖性结构和有翼猪笼草的超唇形构形,创造了具有显著液滴滑动各向异性的超唇形图案表面。功能表面的滑动各向异性是天然蝴蝶翅膀的三倍,这使得能够在没有质量损失的情况下同时处理多个液滴。(DOI:10.1002/dro2.46)
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引用次数: 0
Front Cover, Volume 2, Number 2, April 2023 封面,第2卷,第2期,2023年4月
Pub Date : 2023-04-18 DOI: 10.1002/dro2.59
David Van Assche, Thomas Beneyton, Jean-Christophe Baret

Front Cover: The cover image is based on the Research Article Rectifying jet breakup by electric forcing by Van Assche et al.

Electric fields provide means to actuate droplet at high-throughput in microfluidics. Using a modulated AC-field, droplets are generated at high-throughput in a jetting regime with improved monodispersity. (DOI: 10.1002/dro2.45)

封面:封面图像基于Van Assche等人的研究文章《通过电强迫矫正射流破裂》。电场提供了在微流体中以高通量驱动液滴的方法。使用调制的AC场,在具有改进的单分散性的喷射状态下以高通量产生液滴。(DOI:10.1002/dro2.45)
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引用次数: 0
Back Cover, Volume 2, Number 2, April 2023 封底,第2卷,第2期,2023年4月
Pub Date : 2023-04-18 DOI: 10.1002/dro2.61
Youhua Jiang, Christian Machado, Kyoo-Chul K. Park

Back Cover: The cover image is based on the Review Article From capture to transport: A review of engineered surfaces for fog collection by Jiang et al.

This cover image demonstrates that the collection of fog from an incoming fog-laden wind includes the aerodynamics-governed fog-capturing process and interfacial-phenomena-determined liquid transport process. This review introduces and discusses the definition of fog collection, fog capture process, liquid transport process, the effects of surface characteristics on fog collection performance, and the optimization of a fog collector. (DOI: 10.1002/dro2.55)

封底:封面图片基于姜等人的评论文章《从捕捉到运输:收集雾的工程表面综述》。这张封面图片表明,从充满雾的风中收集雾包括空气动力学控制的雾捕捉过程和界面现象决定的液体运输过程。本文介绍并讨论了雾收集的定义、雾捕获过程、液体传输过程、表面特性对雾收集性能的影响以及雾收集器的优化。(DOI:10.1002/dro2.55)
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引用次数: 0
Inside Back Cover, Volume 2, Number 2, April 2023 内封底,第2卷,第2期,2023年4月
Pub Date : 2023-04-18 DOI: 10.1002/dro2.60
Yi Huang, Shuai Yin, Haiwang Li, Sihang Liu, Teck Neng Wong

Inside Back Cover: The cover image is based on the Research Article One-step fabrication of moon-shaped microrobots through in situ solidification of magnetic Janus droplets in microchannels by Huang et al.

A micro-robotic Janus particle with solid and liquid compartments has been fabricated in a one-step microfluidic process. The moon-shaped solid compartment is made up of UV-curable materials containing magnetic nanoparticles, which allows the particle to be steered by an external magnetic field, hence functioning as a micro-robot for various applications such as drug delivery and vortex generation. (DOI: 10.1002/dro2.56)

封底内部:封面图像基于Huang等人的研究文章《通过在微通道中原位固化磁性Janus液滴一步制造月球形状的微型机器人》。在一步微流体工艺中制造了具有固体和液体隔间的微型机器人Janus颗粒。月球形状的固体隔间由含有磁性纳米颗粒的紫外线固化材料组成,这使颗粒能够通过外部磁场进行操纵,因此可以作为微型机器人用于各种应用,如药物输送和涡流产生。(DOI:10.1002/dro2.56)
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引用次数: 0
One-step fabrication of moon-shaped microrobots through in situ solidification of magnetic Janus droplets in microchannels 通过微通道中磁性Janus液滴的原位固化一步制造月球形状的微型机器人
Pub Date : 2023-04-11 DOI: 10.1002/dro2.56
Yi Huang, Shuai Yin, Haiwang Li, Sihang Liu, Teck Neng Wong

Special-shaped microscale structures have shed light on new possibilities in key fields of chemistry, medicine, and energy. Asymmetrical microrobots with sensitive magnetic responses can be useful tools in controlled chemical reactions, drug delivery, and functional material synthesis. Microfluidic-based emulsion generation technology is adopted as a powerful platform for the fabrication of steerable microrobots with refined control. Specifically, Janus droplets are generated in microfluidic chips featuring a flow-focusing configuration. Asymmetrical morphologies of the Janus droplets are achieved by balancing the interfacial tensions, where the portion containing magnetic nanoparticles is solidified through the UV-initiated polymerization process right after the formation while the Janus structure is left intact. We succeed in controlling the morphology of the Janus droplet along with the moon-shaped robots hydrodynamically and applying them in flow control at the microscale under external magnetic fields, which are characterized and quantified by three-dimensional profile measurement and high-speed microparticle velocimetry measurement. Our proposed on-chip fabrication method using a microfluidic platform not only provides a method for fabricating magnetic robots but also enables tuning the complex morphologies and functionalities at the microscale, which could shed light on new possibilities in key fields of controlled chemistry reaction, medicine synthesis, and energy generation.

特殊形状的微尺度结构揭示了化学、医学和能源等关键领域的新可能性。具有灵敏磁响应的不对称微型机器人可以成为控制化学反应、药物输送和功能材料合成的有用工具。基于微流体的乳液生成技术被用作制造具有精细控制的可操纵微型机器人的强大平台。具体而言,Janus液滴是在具有流动聚焦配置的微流体芯片中产生的。Janus液滴的不对称形态是通过平衡界面张力来实现的,其中含有磁性纳米颗粒的部分在形成后立即通过UV引发的聚合过程固化,而Janus结构保持完整。我们成功地用流体动力学方法控制了Janus液滴和月形机器人的形态,并将其应用于外部磁场下的微尺度流动控制,通过三维轮廓测量和高速微粒测速测量对其进行了表征和量化。我们提出的使用微流体平台的芯片上制造方法不仅提供了一种制造磁性机器人的方法,而且能够在微尺度上调整复杂的形态和功能,这可以为受控化学反应、药物合成和能源产生等关键领域提供新的可能性。
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引用次数: 5
From capture to transport: A review of engineered surfaces for fog collection 从捕获到运输:雾收集工程表面综述
Pub Date : 2023-04-10 DOI: 10.1002/dro2.55
Youhua Jiang, Christian Machado, Kyoo-Chul K. Park

Collecting microscale water droplets suspended in the wind, that is, fog, using permeable surfaces is a promising solution to the worldwide problem of water scarcity and is of great interest to industries, such as mist elimination and recapturing water in cooling towers. In the past few decades, this topic has attracted a drastically increasing number of researchers across a wide range of subjects. However, many aspects remain unclear, such as the definition and process of fog collection, fog collection determined from the perspectives of both the fog capture process and the liquid transport process, and how surface characteristics affect fog collection performance. In this review, we introduce and discuss fog collection from the perspectives of aerodynamics-governed fog-capturing processes and interfacial-phenomena-determined liquid transport processes. Then, an emphasis is given to the design and engineering of permeable surfaces at different length scales to optimize the fog collection performance, including the dimension, morphology, and arrangement of wires at the millimetric scale, unidirectional spreading, and Laplace pressure gradient induced by asymmetric surface geometry and nano-/microstructures. At last, a brief outlook of future research directions is provided.

利用可渗透表面收集悬浮在风中的微小水滴,即雾,是解决全球缺水问题的一种很有前途的解决方案,对工业界来说也很有意义,例如消除薄雾和在冷却塔中回收水。在过去的几十年里,这个话题吸引了越来越多的研究人员,涉及广泛的学科。然而,许多方面仍不清楚,如雾收集的定义和过程,从雾捕获过程和液体传输过程的角度确定的雾收集,以及表面特性如何影响雾收集性能。在这篇综述中,我们从空气动力学控制的雾捕获过程和界面现象决定的液体传输过程的角度介绍和讨论了雾收集。然后,重点研究了不同长度尺度下可渗透表面的设计和工程,以优化雾收集性能,包括毫米尺度下金属丝的尺寸、形态和排列、单向扩展以及不对称表面几何形状和纳米/微观结构引起的拉普拉斯压力梯度。最后,对未来的研究方向进行了简要展望。
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引用次数: 12
Droplet interface in additive manufacturing: From process to application 增材制造中的液滴界面:从工艺到应用
Pub Date : 2023-04-10 DOI: 10.1002/dro2.57
Zhengnan Sun, Xu Zeng, Xu Deng, Xiaosheng Zhang, Yi Zhang

Additive manufacturing (AM), which is often referred to as three-dimensional printing, revolutionizes manufacturing by providing a high degree of design freedom and customization. Several AM methods entail precise control of droplet interfacial properties to ensure the high quality of the printed products. At the same time, the rapid growth of AM technology has made it possible to prepare novel surfaces with complex structures, further expanding the range of potential applications of droplet interface. To provide a unified framework to guide the continuous development of AM that involves droplet interface, this manuscript reviews related work in this field from two aspects—the droplet interface phenomenon in AM processes and the applications of droplet interface prepared by AM. Limitations of existing works are discussed, and potential future directions are suggested.

增材制造(AM),通常被称为三维打印,通过提供高度的设计自由度和定制,彻底改变了制造业。几种AM方法需要精确控制液滴界面性质,以确保印刷产品的高质量。同时,AM技术的快速发展使制备具有复杂结构的新型表面成为可能,进一步扩大了液滴界面的潜在应用范围。为了提供一个统一的框架来指导涉及液滴界面的AM的持续发展,本文从AM工艺中的液滴界面现象和AM制备的液滴接口的应用两个方面综述了该领域的相关工作。讨论了现有工作的局限性,并提出了潜在的未来方向。
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引用次数: 2
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