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Structural insights into soft matter materials via spin echo small angle neutron scattering and small angle neutron scattering 通过自旋回波小角中子散射和小角中子散射洞察软物质材料的结构
Pub Date : 2024-08-16 DOI: 10.1016/j.nucana.2024.100128
Tingting Wang

The recent advancements in neutron scattering technologies in China, with the development of China's first Spin-Echo Small-Angle Neutron Scattering (SESANS) spectrometer at China Mianyang Research Reactor (CMRR) and the integration of a Very Small Angle Neutron Scattering (VSANS) instrument at China Spallation Neutron Source (CSNS), have significantly bolstered the nation's scientific capabilities. This review aims to highlight the distinctive features and applications of SESANS and SANS, and to offer a valuable contribution by demonstrating how SESANS and SANS can be leveraged for the study of soft matters and solid-state materials, with a particular emphasis on the benefits of techniques such as chain labeling, contrast variation, and contrast matching. We also aim to illustrate what types of information can be gleaned from these methods. The review is structured to first introduce the general concepts of SANS and SESANS, followed by a discussion on the information these techniques can provide. Then the applications of these techniques, in combination with other techniques, on various material investigations will be demonstrated. The review concludes with a summary and future perspectives, aiming to inspire further interdisciplinary research and collaboration, and beneficial to a broader audience.

随着中国绵阳中子研究堆(CMRR)研制出中国第一台自旋回波小角中子散射(SESANS)光谱仪,以及中国溅射中子源(CSNS)集成了甚小角中子散射(VSANS)仪器,中国中子散射技术的最新进展极大地增强了国家的科学能力。本综述旨在强调 SESANS 和 SANS 的独特功能和应用,并通过展示如何利用 SESANS 和 SANS 研究软物质和固态材料,特别强调链标记、对比度变化和对比度匹配等技术的益处,从而做出有价值的贡献。我们还旨在说明从这些方法中可以收集到哪些类型的信息。综述的结构是首先介绍 SANS 和 SESANS 的一般概念,然后讨论这些技术可以提供的信息。然后将展示这些技术与其他技术相结合在各种材料研究中的应用。综述的最后是总结和未来展望,旨在激励进一步的跨学科研究与合作,并使更多读者受益。
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引用次数: 0
Gold nanoparticle effect on dose and DNA damage enhancement in the vicinity of gold nanoparticles 金纳米粒子对剂量和金纳米粒子附近 DNA 损伤增强的影响
Pub Date : 2024-08-13 DOI: 10.1016/j.nucana.2024.100126
Adil Bardane , Nabil Maalej , El Mahjoub Chakir , El Mehdi Al Ibrahmi

This study uses Monte Carlo simulations to examine the dose enhancement effect of gold nanoparticles (AuNPs) in radiation therapy and its effects on DNA damage. Using the GATE- 9.0 and Geant4-DNA packages, Monte Carlo simulations were used to simulate a mathematical phantom and determine the energy deposition in the vicinity of AuNP. The simulations were conducted for various photon beam energies (50, 100, 250, and 6000 keV) with and without the presence of different-size AuNPs (10, 30, 50 and 100 nm). The dose enhancement factor (DER) was evaluated using Geant4-DNA to examine the effects AuNP sizes and photon beam energies on DNA damage. A multi-scale Monte Carlo simulation was conducted to evaluate enhanced DNA damage owing to nanoparticles in the proximity of cancer cells. The Monte Carlo simulations indicated that AuNPs boost the dose delivery, resulting in enhanced energy deposition and subsequent DNA damage. The DER analysis revealed a significant increase in the dose deposition within DNA, leading to single or double-strand breaks. Geant4-DNA simulations revealed information on the dosage enhancement factor for various AuNP sizes and photon beam intensities, enabling a deeper comprehension of the underlying mechanics. The outcomes of this study emphasize the potential of AuNPs as effective radiosensitizers in radiation therapy and contribute to the growing body of research on the use of nanotechnology in enhancing cancer treatment outcomes. Further investigations and experimental validations are necessary to optimize the usage of AuNPs for improved radiation therapy.

本研究利用蒙特卡罗模拟来研究金纳米粒子(AuNPs)在放射治疗中的剂量增强效应及其对 DNA 损伤的影响。利用 GATE- 9.0 和 Geant4-DNA 软件包,蒙特卡罗模拟法模拟了一个数学模型,并确定了 AuNP 附近的能量沉积。模拟针对不同光子束能量(50、100、250 和 6000 keV)、不同尺寸 AuNPs(10、30、50 和 100 nm)的存在和不存在进行。使用 Geant4-DNA 评估了剂量增强因子 (DER),以研究 AuNP 尺寸和光子束能量对 DNA 损伤的影响。进行了多尺度蒙特卡洛模拟,以评估纳米粒子在癌细胞附近造成的 DNA 损伤增强。蒙特卡洛模拟结果表明,金纳米粒子提高了剂量传递,从而增强了能量沉积和随后的DNA损伤。DER 分析显示,DNA 内的剂量沉积明显增加,导致单链或双链断裂。Geant4-DNA 模拟揭示了不同 AuNP 尺寸和光子束强度下剂量增强因子的信息,从而加深了对基本力学的理解。这项研究的成果强调了 AuNPs 在放射治疗中作为有效放射增敏剂的潜力,并为越来越多的利用纳米技术提高癌症治疗效果的研究做出了贡献。要优化 AuNPs 的使用,提高放射治疗效果,还需要进一步的研究和实验验证。
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引用次数: 0
Fusion mechanism involved in the synthesis of superheavy element Z>118 using Mn projectiles 利用锰射弹合成超重元素 Z>118 所涉及的聚变机制
Pub Date : 2024-08-06 DOI: 10.1016/j.nucana.2024.100124
H.S. Anushree , N. Sowmya , H.C Manjunatha , S. Shubha
<div><div>We conducted an in-depth investigation of Mn-induced fusion reactions aimed at synthesizing superheavy elements with atomic numbers Z=119 to Z=123. Our analysis considers the total potential, which combines Coulomb and nuclear potentials. The nuclear potential was calculated using the Thomas–Fermi approach, a valuable method for modeling the behavior of nucleons in atomic nuclei. within the framework of advanced statistical model, the evaporation residue cross-sections were determined. At optimal energies, we have calculated capture, fusion, and evaporation residue cross-sections for the reactions of all the projectile–target combinations. All <span><math><msup><mrow></mrow><mrow><mn>53</mn><mo>−</mo><mn>55</mn></mrow></msup></math></span>Mn isotopes with larger half-lives were taken into consideration as projectiles. Fusion reactions between <span><math><msup><mrow></mrow><mrow><mn>53</mn><mo>−</mo><mn>55</mn></mrow></msup></math></span>Mn projectiles with <span><math><msup><mrow></mrow><mrow><mn>238</mn><mo>−</mo><mn>242</mn><mo>,</mo><mn>244</mn></mrow></msup></math></span>Pu, <span><math><msup><mrow></mrow><mrow><mn>241</mn><mo>−</mo><mn>243</mn></mrow></msup></math></span>Am, <span><math><msup><mrow></mrow><mrow><mn>242</mn><mo>−</mo><mn>248</mn><mo>,</mo><mn>250</mn></mrow></msup></math></span>Cm, <span><math><msup><mrow></mrow><mrow><mn>247</mn><mo>−</mo><mn>249</mn></mrow></msup></math></span>Bk, and <span><math><msup><mrow></mrow><mrow><mn>248</mn><mo>−</mo><mn>254</mn></mrow></msup></math></span>Cf. Detailed investigations were made and promising reactions viz. <span><math><mrow><msup><mrow></mrow><mrow><mn>241</mn></mrow></msup><mi>Pu</mi></mrow></math></span> (<span><math><mrow><msup><mrow></mrow><mrow><mn>55</mn></mrow></msup><mi>Mn</mi></mrow></math></span>, 3n)<sup>293</sup>119, <span><math><mrow><msup><mrow></mrow><mrow><mn>242</mn></mrow></msup><mi>Am</mi></mrow></math></span> (<span><math><mrow><msup><mrow></mrow><mrow><mn>55</mn></mrow></msup><mi>Mn</mi></mrow></math></span>, 3n)<sup>294</sup>120, <span><math><mrow><msup><mrow></mrow><mrow><mn>247</mn></mrow></msup><mi>Cm</mi></mrow></math></span> (<span><math><mrow><msup><mrow></mrow><mrow><mn>55</mn></mrow></msup><mi>Mn</mi></mrow></math></span>, 3n)<sup>299</sup>121, <span><math><mrow><msup><mrow></mrow><mrow><mn>248</mn></mrow></msup><mi>Bk</mi></mrow></math></span> (<span><math><mrow><msup><mrow></mrow><mrow><mn>55</mn></mrow></msup><mi>Mn</mi></mrow></math></span>, 3n)<sup>300</sup>122 and <span><math><mrow><msup><mrow></mrow><mrow><mn>251</mn></mrow></msup><mi>Cf</mi></mrow></math></span> (<span><math><mrow><msup><mrow></mrow><mrow><mn>53</mn></mrow></msup><mi>Mn</mi></mrow></math></span>, 3n)<sup>301</sup>123 with maximum <span><math><msub><mrow><mi>σ</mi></mrow><mrow><mi>E</mi><mi>R</mi></mrow></msub></math></span> are found to be 415.1 fb at 240 MeV, 115.4 fb at 244 MeV, 36.5 fb at 245 MeV, 13.6 fb at 249 MeV, 5.4 fb at 250 MeV for Z=119-123 respectively. Th
我们对旨在合成原子序数为 Z=119 至 Z=123 的超重元素的锰诱导聚变反应进行了深入研究。我们的分析考虑了库仑势和核势相结合的总势能。核势能是用托马斯-费米方法计算的,这是一种模拟原子核中核子行为的重要方法。在最佳能量下,我们计算了所有射弹-靶组合反应的俘获、聚变和蒸发残余截面。所有具有较大半衰期的 53-55Mn 同位素都被视为射弹。对 53-55Mn 射弹与 238-242、244Pu、241-243Am、242-248、250Cm、247-249Bk 和 248-254Cf 之间的聚变反应进行了详细的研究,发现有希望的反应包括241Pu (55Mn, 3n)293119, 242Am (55Mn, 3n)294120, 247Cm (55Mn, 3n)299121, 248Bk (55Mn, 3n)300122 和 251Cf (53Mn, 3n)301123 的最大 σER 为 415.1 fb,244 MeV 时为 115.4 fb,245 MeV 时为 36.5 fb,249 MeV 时为 13.6 fb,250 MeV 时为 5.4 fb。这些预测可能有助于未来的实验人员探索元素周期表中的第 8 行。
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All &lt;span&gt;&lt;math&gt;&lt;msup&gt;&lt;mrow&gt;&lt;/mrow&gt;&lt;mrow&gt;&lt;mn&gt;53&lt;/mn&gt;&lt;mo&gt;−&lt;/mo&gt;&lt;mn&gt;55&lt;/mn&gt;&lt;/mrow&gt;&lt;/msup&gt;&lt;/math&gt;&lt;/span&gt;Mn isotopes with larger half-lives were taken into consideration as projectiles. Fusion reactions between &lt;span&gt;&lt;math&gt;&lt;msup&gt;&lt;mrow&gt;&lt;/mrow&gt;&lt;mrow&gt;&lt;mn&gt;53&lt;/mn&gt;&lt;mo&gt;−&lt;/mo&gt;&lt;mn&gt;55&lt;/mn&gt;&lt;/mrow&gt;&lt;/msup&gt;&lt;/math&gt;&lt;/span&gt;Mn projectiles with &lt;span&gt;&lt;math&gt;&lt;msup&gt;&lt;mrow&gt;&lt;/mrow&gt;&lt;mrow&gt;&lt;mn&gt;238&lt;/mn&gt;&lt;mo&gt;−&lt;/mo&gt;&lt;mn&gt;242&lt;/mn&gt;&lt;mo&gt;,&lt;/mo&gt;&lt;mn&gt;244&lt;/mn&gt;&lt;/mrow&gt;&lt;/msup&gt;&lt;/math&gt;&lt;/span&gt;Pu, &lt;span&gt;&lt;math&gt;&lt;msup&gt;&lt;mrow&gt;&lt;/mrow&gt;&lt;mrow&gt;&lt;mn&gt;241&lt;/mn&gt;&lt;mo&gt;−&lt;/mo&gt;&lt;mn&gt;243&lt;/mn&gt;&lt;/mrow&gt;&lt;/msup&gt;&lt;/math&gt;&lt;/span&gt;Am, &lt;span&gt;&lt;math&gt;&lt;msup&gt;&lt;mrow&gt;&lt;/mrow&gt;&lt;mrow&gt;&lt;mn&gt;242&lt;/mn&gt;&lt;mo&gt;−&lt;/mo&gt;&lt;mn&gt;248&lt;/mn&gt;&lt;mo&gt;,&lt;/mo&gt;&lt;mn&gt;250&lt;/mn&gt;&lt;/mrow&gt;&lt;/msup&gt;&lt;/math&gt;&lt;/span&gt;Cm, &lt;span&gt;&lt;math&gt;&lt;msup&gt;&lt;mrow&gt;&lt;/mrow&gt;&lt;mrow&gt;&lt;mn&gt;247&lt;/mn&gt;&lt;mo&gt;−&lt;/mo&gt;&lt;mn&gt;249&lt;/mn&gt;&lt;/mrow&gt;&lt;/msup&gt;&lt;/math&gt;&lt;/span&gt;Bk, and &lt;span&gt;&lt;math&gt;&lt;msup&gt;&lt;mrow&gt;&lt;/mrow&gt;&lt;mrow&gt;&lt;mn&gt;248&lt;/mn&gt;&lt;mo&gt;−&lt;/mo&gt;&lt;mn&gt;254&lt;/mn&gt;&lt;/mrow&gt;&lt;/msup&gt;&lt;/math&gt;&lt;/span&gt;Cf. Detailed investigations were made and promising reactions viz. &lt;span&gt;&lt;math&gt;&lt;mrow&gt;&lt;msup&gt;&lt;mrow&gt;&lt;/mrow&gt;&lt;mrow&gt;&lt;mn&gt;241&lt;/mn&gt;&lt;/mrow&gt;&lt;/msup&gt;&lt;mi&gt;Pu&lt;/mi&gt;&lt;/mrow&gt;&lt;/math&gt;&lt;/span&gt; (&lt;span&gt;&lt;math&gt;&lt;mrow&gt;&lt;msup&gt;&lt;mrow&gt;&lt;/mrow&gt;&lt;mrow&gt;&lt;mn&gt;55&lt;/mn&gt;&lt;/mrow&gt;&lt;/msup&gt;&lt;mi&gt;Mn&lt;/mi&gt;&lt;/mrow&gt;&lt;/math&gt;&lt;/span&gt;, 3n)&lt;sup&gt;293&lt;/sup&gt;119, &lt;span&gt;&lt;math&gt;&lt;mrow&gt;&lt;msup&gt;&lt;mrow&gt;&lt;/mrow&gt;&lt;mrow&gt;&lt;mn&gt;242&lt;/mn&gt;&lt;/mrow&gt;&lt;/msup&gt;&lt;mi&gt;Am&lt;/mi&gt;&lt;/mrow&gt;&lt;/math&gt;&lt;/span&gt; (&lt;span&gt;&lt;math&gt;&lt;mrow&gt;&lt;msup&gt;&lt;mrow&gt;&lt;/mrow&gt;&lt;mrow&gt;&lt;mn&gt;55&lt;/mn&gt;&lt;/mrow&gt;&lt;/msup&gt;&lt;mi&gt;Mn&lt;/mi&gt;&lt;/mrow&gt;&lt;/math&gt;&lt;/span&gt;, 3n)&lt;sup&gt;294&lt;/sup&gt;120, &lt;span&gt;&lt;math&gt;&lt;mrow&gt;&lt;msup&gt;&lt;mrow&gt;&lt;/mrow&gt;&lt;mrow&gt;&lt;mn&gt;247&lt;/mn&gt;&lt;/mrow&gt;&lt;/msup&gt;&lt;mi&gt;Cm&lt;/mi&gt;&lt;/mrow&gt;&lt;/math&gt;&lt;/span&gt; (&lt;span&gt;&lt;math&gt;&lt;mrow&gt;&lt;msup&gt;&lt;mrow&gt;&lt;/mrow&gt;&lt;mrow&gt;&lt;mn&gt;55&lt;/mn&gt;&lt;/mrow&gt;&lt;/msup&gt;&lt;mi&gt;Mn&lt;/mi&gt;&lt;/mrow&gt;&lt;/math&gt;&lt;/span&gt;, 3n)&lt;sup&gt;299&lt;/sup&gt;121, &lt;span&gt;&lt;math&gt;&lt;mrow&gt;&lt;msup&gt;&lt;mrow&gt;&lt;/mrow&gt;&lt;mrow&gt;&lt;mn&gt;248&lt;/mn&gt;&lt;/mrow&gt;&lt;/msup&gt;&lt;mi&gt;Bk&lt;/mi&gt;&lt;/mrow&gt;&lt;/math&gt;&lt;/span&gt; (&lt;span&gt;&lt;math&gt;&lt;mrow&gt;&lt;msup&gt;&lt;mrow&gt;&lt;/mrow&gt;&lt;mrow&gt;&lt;mn&gt;55&lt;/mn&gt;&lt;/mrow&gt;&lt;/msup&gt;&lt;mi&gt;Mn&lt;/mi&gt;&lt;/mrow&gt;&lt;/math&gt;&lt;/span&gt;, 3n)&lt;sup&gt;300&lt;/sup&gt;122 and &lt;span&gt;&lt;math&gt;&lt;mrow&gt;&lt;msup&gt;&lt;mrow&gt;&lt;/mrow&gt;&lt;mrow&gt;&lt;mn&gt;251&lt;/mn&gt;&lt;/mrow&gt;&lt;/msup&gt;&lt;mi&gt;Cf&lt;/mi&gt;&lt;/mrow&gt;&lt;/math&gt;&lt;/span&gt; (&lt;span&gt;&lt;math&gt;&lt;mrow&gt;&lt;msup&gt;&lt;mrow&gt;&lt;/mrow&gt;&lt;mrow&gt;&lt;mn&gt;53&lt;/mn&gt;&lt;/mrow&gt;&lt;/msup&gt;&lt;mi&gt;Mn&lt;/mi&gt;&lt;/mrow&gt;&lt;/math&gt;&lt;/span&gt;, 3n)&lt;sup&gt;301&lt;/sup&gt;123 with maximum &lt;span&gt;&lt;math&gt;&lt;msub&gt;&lt;mrow&gt;&lt;mi&gt;σ&lt;/mi&gt;&lt;/mrow&gt;&lt;mrow&gt;&lt;mi&gt;E&lt;/mi&gt;&lt;mi&gt;R&lt;/mi&gt;&lt;/mrow&gt;&lt;/msub&gt;&lt;/math&gt;&lt;/span&gt; are found to be 415.1 fb at 240 MeV, 115.4 fb at 244 MeV, 36.5 fb at 245 MeV, 13.6 fb at 249 MeV, 5.4 fb at 250 MeV for Z=119-123 respectively. 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引用次数: 0
Evaluation of Potassium-40 and Uranium-238 activities and radiological risk in Missour, Morocco soils using gamma spectrometry 利用伽马能谱仪评估摩洛哥米苏尔土壤中钾-40 和铀-238 的放射性活度及辐射风险
Pub Date : 2024-08-05 DOI: 10.1016/j.nucana.2024.100125
Abdessamad Didi , Hamid Bounouira , Abir Adnane , Soumaia El Khamsi Chahd , Hamid Amsil , Abdelwahab Badague , Iliasse Aarab

The objective of this study is to assess natural activity in soil to estimate potential radiological risks for the population. Given that soil is inherently radioactive and can reach hazardous levels, it is crucial to determine the activities of radionuclides such as Potassium-40 and Uranium-238 descendants at different depths and geographical positions. For this work, gamma spectrometry method was employed to analyze soil samples collected at three different positions in the Missour region. Each position was sampled at five different depths, spaced 5 cm apart, resulting in a total of 15 samples. The activity of Potassium-40 and Uranium238 descendants in the soil was accurately assessed using Lvis software, enabling the estimation of radiological doses.

这项研究的目的是评估土壤中的天然放射性活度,以估计对人口的潜在辐射风险。鉴于土壤本身具有放射性,并可达到危险水平,因此确定不同深度和地理位置的放射性核素(如钾-40 和铀-238 后裔)的放射性活度至关重要。在这项工作中,采用了伽马能谱法分析在米苏尔地区三个不同位置采集的土壤样本。每个位置采集了五个不同深度的样本,样本间距为 5 厘米,共采集了 15 个样本。利用 Lvis 软件对土壤中钾-40 和铀-238 后裔的活度进行了准确评估,从而估算出辐射剂量。
{"title":"Evaluation of Potassium-40 and Uranium-238 activities and radiological risk in Missour, Morocco soils using gamma spectrometry","authors":"Abdessamad Didi ,&nbsp;Hamid Bounouira ,&nbsp;Abir Adnane ,&nbsp;Soumaia El Khamsi Chahd ,&nbsp;Hamid Amsil ,&nbsp;Abdelwahab Badague ,&nbsp;Iliasse Aarab","doi":"10.1016/j.nucana.2024.100125","DOIUrl":"10.1016/j.nucana.2024.100125","url":null,"abstract":"<div><p>The objective of this study is to assess natural activity in soil to estimate potential radiological risks for the population. Given that soil is inherently radioactive and can reach hazardous levels, it is crucial to determine the activities of radionuclides such as Potassium-40 and Uranium-238 descendants at different depths and geographical positions. For this work, gamma spectrometry method was employed to analyze soil samples collected at three different positions in the Missour region. Each position was sampled at five different depths, spaced 5 cm apart, resulting in a total of 15 samples. The activity of Potassium-40 and Uranium238 descendants in the soil was accurately assessed using Lvis software, enabling the estimation of radiological doses.</p></div>","PeriodicalId":100965,"journal":{"name":"Nuclear Analysis","volume":"3 3","pages":"Article 100125"},"PeriodicalIF":0.0,"publicationDate":"2024-08-05","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.sciencedirect.com/science/article/pii/S2773183924000259/pdfft?md5=b064fa8f6785305a19ec020d1f7ebcfe&pid=1-s2.0-S2773183924000259-main.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141964342","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Compound nucleus formation probability of heavy and superheavy nuclei synthesized using heavy ion fusion reactions 利用重离子聚变反应合成的重核和超重核的复合核形成概率
Pub Date : 2024-07-31 DOI: 10.1016/j.nucana.2024.100123
Reddi Rani L. , N. Sowmya , H.C. Manjunatha , M.M. Armstrong Arasu
The role of entrance channel parameters such as Z2/A, charge asymmetry αz, mass-asymmetry (ηA), charge product (Z1Z2), mean fissility χm, Coulomb interaction parameter and (NZ)/(N+Z) on compound nucleus formation of actinide nuclei using heavy ion fusion reactions were investigated. For the formation of compound nuclei, the considered atomic number range of the projectile varies between 5Z14 and the mass number lies between 10A34. Similarly, the studied target atomic number varies between 78Z92 and the mass number range is 197A238. Among these entrance channel parameters, PCN is more systematic for (NZ)(N+Z), Z2/A and αz. In addition to entrance channel parameters, the Ecm and EBass also play a significant role in the prediction of PCN. The proposed empirical formulae are applicable to the compound nuclei from Fr to Sg. These findings are significant for the PCN prediction from Fr to Sg.
研究了入口通道参数,如 Z2/A、电荷不对称性 αz、质量不对称性 (ηA)、电荷乘积 (Z1Z2)、平均裂变率 χm、库仑相互作用参数和 (N-Z)/(N+Z) 对利用重离子聚变反应形成锕系核的复合核的作用。为了形成复合核,考虑的射弹原子序数范围在 5≤Z≤14 之间,质量数在 10≤A≤34 之间。同样,研究的靶原子序数在 78≤Z≤92 之间变化,质量数范围为 197≤A≤238。在这些入口通道参数中,(N-Z)(N+Z)、Z2/A 和 αz 的 PCN 更有系统性。除入口通道参数外,Ecm 和 EBass 对 PCN 的预测也起着重要作用。所提出的经验公式适用于从 Fr 到 Sg 的化合物核。这些发现对于从 Fr 到 Sg 的 PCN 预测具有重要意义。
{"title":"Compound nucleus formation probability of heavy and superheavy nuclei synthesized using heavy ion fusion reactions","authors":"Reddi Rani L. ,&nbsp;N. Sowmya ,&nbsp;H.C. Manjunatha ,&nbsp;M.M. Armstrong Arasu","doi":"10.1016/j.nucana.2024.100123","DOIUrl":"10.1016/j.nucana.2024.100123","url":null,"abstract":"<div><div>The role of entrance channel parameters such as <span><math><mrow><msup><mrow><mi>Z</mi></mrow><mrow><mn>2</mn></mrow></msup><mo>/</mo><mi>A</mi></mrow></math></span>, charge asymmetry <span><math><msub><mrow><mi>α</mi></mrow><mrow><mi>z</mi></mrow></msub></math></span>, mass-asymmetry (<span><math><msub><mrow><mi>η</mi></mrow><mrow><mi>A</mi></mrow></msub></math></span>), charge product (<span><math><mrow><msub><mrow><mi>Z</mi></mrow><mrow><mn>1</mn></mrow></msub><msub><mrow><mi>Z</mi></mrow><mrow><mn>2</mn></mrow></msub></mrow></math></span>), mean fissility <span><math><msub><mrow><mi>χ</mi></mrow><mrow><mi>m</mi></mrow></msub></math></span>, Coulomb interaction parameter and <span><math><mrow><mrow><mo>(</mo><mi>N</mi><mo>−</mo><mi>Z</mi><mo>)</mo></mrow><mo>/</mo><mrow><mo>(</mo><mi>N</mi><mo>+</mo><mi>Z</mi><mo>)</mo></mrow></mrow></math></span> on compound nucleus formation of actinide nuclei using heavy ion fusion reactions were investigated. For the formation of compound nuclei, the considered atomic number range of the projectile varies between <span><math><mrow><mn>5</mn><mo>≤</mo><mi>Z</mi><mo>≤</mo><mn>14</mn></mrow></math></span> and the mass number lies between <span><math><mrow><mn>10</mn><mo>≤</mo><mi>A</mi><mo>≤</mo><mn>34</mn></mrow></math></span>. Similarly, the studied target atomic number varies between <span><math><mrow><mn>78</mn><mo>≤</mo><mi>Z</mi><mo>≤</mo><mn>92</mn></mrow></math></span> and the mass number range is <span><math><mrow><mn>197</mn><mo>≤</mo><mi>A</mi><mo>≤</mo><mn>238</mn></mrow></math></span>. Among these entrance channel parameters, <span><math><msub><mrow><mi>P</mi></mrow><mrow><mi>C</mi><mi>N</mi></mrow></msub></math></span> is more systematic for <span><math><mfrac><mrow><mrow><mo>(</mo><mi>N</mi><mo>−</mo><mi>Z</mi><mo>)</mo></mrow></mrow><mrow><mrow><mo>(</mo><mi>N</mi><mo>+</mo><mi>Z</mi><mo>)</mo></mrow></mrow></mfrac></math></span>, <span><math><mrow><msup><mrow><mi>Z</mi></mrow><mrow><mn>2</mn></mrow></msup><mo>/</mo><mi>A</mi></mrow></math></span> and <span><math><msub><mrow><mi>α</mi></mrow><mrow><mi>z</mi></mrow></msub></math></span>. In addition to entrance channel parameters, the <span><math><msub><mrow><mi>E</mi></mrow><mrow><mi>c</mi><mi>m</mi></mrow></msub></math></span> and <span><math><msub><mrow><mi>E</mi></mrow><mrow><mi>B</mi><mi>a</mi><mi>s</mi><mi>s</mi></mrow></msub></math></span> also play a significant role in the prediction of <span><math><msub><mrow><mi>P</mi></mrow><mrow><mi>C</mi><mi>N</mi></mrow></msub></math></span>. The proposed empirical formulae are applicable to the compound nuclei from Fr to Sg. These findings are significant for the <span><math><msub><mrow><mi>P</mi></mrow><mrow><mi>C</mi><mi>N</mi></mrow></msub></math></span> prediction from Fr to Sg.</div></div>","PeriodicalId":100965,"journal":{"name":"Nuclear Analysis","volume":"3 4","pages":"Article 100123"},"PeriodicalIF":0.0,"publicationDate":"2024-07-31","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142358342","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Feasibility of producing 225Ac via thermal neutron irradiation of 226Ra: A systematic theoretical study 通过热中子辐照 226Ra 生产 225Ac 的可行性:系统理论研究
Pub Date : 2024-07-20 DOI: 10.1016/j.nucana.2024.100122
Long Qiu , Jinsong Zhang , Tu Lan , Jiali Liao , Yuanyou Yang , Feize Li , Ning Liu

With a suitable half-life and abundant radiolabeling strategy, 225Ac has become one of the most promising radionuclides in the area of targeted alpha therapy. However, limited radionuclide supply is threatening the development of 225Ac related endoradiotherapy dramatically. As the parent nuclide of 225Ac, 229Th can be produced via 226Ra(3n, 2β)229Th reaction in a nuclear reactor. However, related practice has not been conducted in large scale, since the nuclear reaction pathway for producing 229Th is complicated. In this work, the feasibility of producing 225Ac/229Th in a reactor was confirmed by systematic theoretical calculations, and a procedure that combines irradiation with separation process was proposed. The results show that 176 MBq of 229Th can be produced by irradiating 1.0 g of 226Ra with a neutron flux density of 1 × 1015 n cm−2 s−1 for 90 days. This will generate 150 MBq of 225Ac monthly from a radionuclide generator, which is sufficient for the single treatment cycle of 200 patients each year considering the radioactivity loss in radiochemical separation, transfer and radiolabeling process. In addition, this irradiation process will also produce 37.8 GBq 227Ac for the preparation of 227Ac-227Th-223Ra generator. In general, the production of 225Ac by neutron irradiation of 226Ra in reactor is practicable and holds potential to alleviate the shortage of current supply of 225Ac.

225Ac 具有合适的半衰期和丰富的放射性标记策略,已成为α靶向治疗领域最有前途的放射性核素之一。然而,有限的放射性核素供应正极大地威胁着与 225Ac 相关的放射治疗的发展。作为 225Ac 的母核素,229Th 可在核反应堆中通过 226Ra(3n,2β)229Th 反应生成。然而,由于产生 229Th 的核反应途径复杂,相关实践尚未大规模开展。在这项工作中,通过系统的理论计算证实了在反应堆中生产 225Ac/229Th 的可行性,并提出了一种将辐照与分离过程相结合的程序。结果表明,用 1 × 1015 n cm-2 s-1 的中子通量密度对 1.0 克 226Ra 进行辐照 90 天,可产生 176 MBq 的 229Th。考虑到放射化学分离、转移和放射性标记过程中的放射性损失,这足以满足每年 200 名患者一个治疗周期的需要。此外,这一辐照过程还将产生 37.8 GBq 227Ac 用于制备 227Ac-227Th-223Ra 发生器。总之,在反应堆中用中子辐照 226Ra 生产 225Ac 是切实可行的,并有可能缓解目前 225Ac 供应短缺的问题。
{"title":"Feasibility of producing 225Ac via thermal neutron irradiation of 226Ra: A systematic theoretical study","authors":"Long Qiu ,&nbsp;Jinsong Zhang ,&nbsp;Tu Lan ,&nbsp;Jiali Liao ,&nbsp;Yuanyou Yang ,&nbsp;Feize Li ,&nbsp;Ning Liu","doi":"10.1016/j.nucana.2024.100122","DOIUrl":"10.1016/j.nucana.2024.100122","url":null,"abstract":"<div><p>With a suitable half-life and abundant radiolabeling strategy, <sup>225</sup>Ac has become one of the most promising radionuclides in the area of targeted alpha therapy. However, limited radionuclide supply is threatening the development of <sup>225</sup>Ac related endoradiotherapy dramatically. As the parent nuclide of <sup>225</sup>Ac, <sup>229</sup>Th can be produced via <sup>226</sup>Ra(3n, 2β)<sup>229</sup>Th reaction in a nuclear reactor. However, related practice has not been conducted in large scale, since the nuclear reaction pathway for producing <sup>229</sup>Th is complicated. In this work, the feasibility of producing <sup>225</sup>Ac/<sup>229</sup>Th in a reactor was confirmed by systematic theoretical calculations, and a procedure that combines irradiation with separation process was proposed. The results show that 176 MBq of <sup>229</sup>Th can be produced by irradiating 1.0 g of <sup>226</sup>Ra with a neutron flux density of 1 × 10<sup>15</sup> n cm<sup>−2</sup> s<sup>−1</sup> for 90 days. This will generate 150 MBq of <sup>225</sup>Ac monthly from a radionuclide generator, which is sufficient for the single treatment cycle of 200 patients each year considering the radioactivity loss in radiochemical separation, transfer and radiolabeling process. In addition, this irradiation process will also produce 37.8 GBq <sup>227</sup>Ac for the preparation of <sup>227</sup>Ac-<sup>227</sup>Th-<sup>223</sup>Ra generator. In general, the production of <sup>225</sup>Ac by neutron irradiation of <sup>226</sup>Ra in reactor is practicable and holds potential to alleviate the shortage of current supply of <sup>225</sup>Ac.</p></div>","PeriodicalId":100965,"journal":{"name":"Nuclear Analysis","volume":"3 3","pages":"Article 100122"},"PeriodicalIF":0.0,"publicationDate":"2024-07-20","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.sciencedirect.com/science/article/pii/S2773183924000223/pdfft?md5=459ab0fb9ccb924e8ab5a6fed4199880&pid=1-s2.0-S2773183924000223-main.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141839148","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Radiological impact of hydrocarbon waste release on drinking water of ughievwen and udu communities, delta state Nigeria 碳氢化合物废物排放对尼日利亚三角洲州 Ughievwen 和 Udu 社区饮用水的辐射影响
Pub Date : 2024-07-16 DOI: 10.1016/j.nucana.2024.100121
Oghenevovwero Emmanuel Esi

Well water quality has been characterized with constant and continuous changes via the interaction of rock, soil and natural nano-filters which terminates at the aquiferous layer for clean well-water collection. The continuous exploration and production of crude oil has resulted significant increase of unwanted elements such as naturally occurring radionuclides in the water-bed which necessitates this study. The study determines the radionuclides based health impact or hazards associated with drinking water from crude oil exploration/production release in Ughievwen and Udu communities of Delta State, Nigeria. Sixty well water samples (three samples from each community) were collected and analyzed using sodium iodide (Nal (Tl)) detector. The obtained mean values of 238U, 232Th and 40K are 6.91 ± 1.62BqL−1, 4.39 ± 1.47 BqL−1 and 24.54 ± 1.59 BqL−1 respectively. The 238U, 232Th and 40K results showed that the measured values are higher than the world standard (UNSCEAR; WHO) and the control values The mean values of total annual effective dose of different age groups are: 11.08 mSvy−1, 2.54 mSvy−1, 1.93 mSvy−1, 2.52 mSvy−1, 7.03 mSvy−1 and 1.12 mSvy−1 respectively. While the mean committed effective dose of adult is 55.94 mSvy−1. The total annual effective dose, committed effective dose, cancer risks and hereditary effects are all lower than recommended limit (WHO; ICRP; USEPA) and reported scientific values except 11.08 mSvy−1 and 7.03 mSvy−1 that are higher than limit. It is evident from obtained results that the drinking water may not be radiologically safe for use by the public, which necessitates routine monitoring and caution to circumvent increase in radiation and the radiological of the studied communities’ drinking water. This is to avoid long term radiological risk arising from accumulation of such release in the studied communities.

井水水质的特点是通过岩石、土壤和天然纳米过滤器的相互作用不断发生持续变化,最终在含水层收集清洁的井水。原油的不断勘探和生产导致水床中的有害元素(如天然放射性核素)显著增加,因此有必要进行这项研究。本研究确定了尼日利亚三角洲州 Ughievwen 和 Udu 社区原油勘探/生产释放的饮用水中放射性核素对健康的影响或危害。研究人员收集了 60 份井水样本(每个社区 3 份),并使用碘化钠(Nal (Tl))检测器进行了分析。获得的 238U、232Th 和 40K 平均值分别为 6.91 ± 1.62BqL-1 、 4.39 ± 1.47 BqL-1 和 24.54 ± 1.59 BqL-1。238U、232Th 和 40K 的测量结果表明,测量值高于世界标准值(UNSCEAR;WHO)和对照值:11.08 mSvy-1、2.54 mSvy-1、1.93 mSvy-1、2.52 mSvy-1、7.03 mSvy-1 和 1.12 mSvy-1。成人的平均承诺有效剂量为 55.94 mSvy-1。除 11.08 mSvy-1 和 7.03 mSvy-1 高于推荐限值外,其余的年总有效剂量、承诺有效剂量、癌症风险和遗传影响均低于推荐限值(世界卫生组织、国际癌症研究委员会、美国环保局)和报告的科学值。从获得的结果可以看出,公众使用的饮用水在辐射方面可能并不安全,因此有必要进行例行监测并采取谨慎措施,以避免辐射的增加和所研究社区饮用水的辐射性。这样做是为了避免在所研究的社区中因这种释放的累积而产生长期的辐射风险。
{"title":"Radiological impact of hydrocarbon waste release on drinking water of ughievwen and udu communities, delta state Nigeria","authors":"Oghenevovwero Emmanuel Esi","doi":"10.1016/j.nucana.2024.100121","DOIUrl":"10.1016/j.nucana.2024.100121","url":null,"abstract":"<div><p>Well water quality has been characterized with constant and continuous changes via the interaction of rock, soil and natural nano-filters which terminates at the aquiferous layer for clean well-water collection. The continuous exploration and production of crude oil has resulted significant increase of unwanted elements such as naturally occurring radionuclides in the water-bed which necessitates this study. The study determines the radionuclides based health impact or hazards associated with drinking water from crude oil exploration/production release in Ughievwen and Udu communities of Delta State, Nigeria. Sixty well water samples (three samples from each community) were collected and analyzed using sodium iodide (Nal (Tl)) detector. The obtained mean values of <sup>238</sup>U, <sup>232</sup>Th and <sup>40</sup>K are 6.91 <span><math><mrow><mo>±</mo></mrow></math></span> 1.62BqL<sup>−1</sup>, 4.39 <span><math><mrow><mo>±</mo></mrow></math></span> 1.47 BqL<sup>−1</sup> and 24.54 <span><math><mrow><mo>±</mo></mrow></math></span> 1.59 BqL<sup>−1</sup> respectively. The <sup>238</sup>U, <sup>232</sup>Th and <sup>40</sup>K results showed that the measured values are higher than the world standard (UNSCEAR; WHO) and the control values The mean values of total annual effective dose of different age groups are: 11.08 mSvy<sup>−1</sup>, 2.54 mSvy<sup>−1</sup>, 1.93 mSvy<sup>−1</sup>, 2.52 mSvy<sup>−1</sup>, 7.03 mSvy<sup>−1</sup> and 1.12 mSvy<sup>−1</sup> respectively. While the mean committed effective dose of adult is 55.94 mSvy<sup>−1</sup>. The total annual effective dose, committed effective dose, cancer risks and hereditary effects are all lower than recommended limit (WHO; ICRP; USEPA) and reported scientific values except 11.08 mSvy<sup>−1</sup> and 7.03 mSvy<sup>−1</sup> that are higher than limit. It is evident from obtained results that the drinking water may not be radiologically safe for use by the public, which necessitates routine monitoring and caution to circumvent increase in radiation and the radiological of the studied communities’ drinking water. This is to avoid long term radiological risk arising from accumulation of such release in the studied communities.</p></div>","PeriodicalId":100965,"journal":{"name":"Nuclear Analysis","volume":"3 3","pages":"Article 100121"},"PeriodicalIF":0.0,"publicationDate":"2024-07-16","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.sciencedirect.com/science/article/pii/S2773183924000211/pdfft?md5=869ab386a09f2b2eca91c3c05f0eb686&pid=1-s2.0-S2773183924000211-main.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141850667","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Temperature distribution in the PGAA system: Collimator, shutter, and filter in TRIGA Mark II reactor PGAA 系统中的温度分布:TRIGA Mark II 反应器中的准直器、快门和过滤器
Pub Date : 2024-07-09 DOI: 10.1016/j.nucana.2024.100120
Jamila Yousfi , Abdessamad Didi , Hamane Lemziouka , Lamiae Mrharrab , Hamid Amsil , Otman Jai , Hamid Bounouira , Khalid Larakil

This article examines the impact of temperature on the steel collimator cap and the primary beam shutter. These components will be used to implement the Prompt Gamma Activation Analysis (PGAA) technique in the Moroccan TRIGA Mark-II research reactor. The steel collimator plug is essential for forming the neutron beam, while the main role of the shutter is to stop the beam when the channel is inactive. This study analyzes the effect of temperature on the collimator and shutter system, particularly focusing on the variation in maximum temperature over a month of operation with 8-h cycles per day, the behavior of temperature over 24 h, the total heat flux as a function of the length of the experimental device, the temperature distribution in mild steel (E235) and 304L stainless steel materials, and the total displacement and strain gradient as a function of temperature. All calculations were performed using COMSOL Multiphysics simulation software, based on the finite element method.

本文研究了温度对钢制准直器盖和主光束快门的影响。这些部件将用于在摩洛哥 TRIGA Mark-II 研究反应堆中实施即时伽马活化分析(PGAA)技术。钢制准直器塞对于中子束的形成至关重要,而快门的主要作用是在通道处于非活动状态时阻止中子束。本研究分析了温度对准直器和快门系统的影响,尤其侧重于每天 8 小时周期运行一个月内最高温度的变化、24 小时内的温度行为、总热通量与实验装置长度的函数关系、低碳钢(E235)和 304L 不锈钢材料的温度分布以及总位移和应变梯度与温度的函数关系。所有计算均使用基于有限元法的 COMSOL Multiphysics 仿真软件进行。
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引用次数: 0
Exploring the impact of anode material on X-ray photon fluence and characteristics: A Monte Carlo simulation study 探索阳极材料对 X 射线光子通量和特性的影响:蒙特卡罗模拟研究
Pub Date : 2024-06-01 DOI: 10.1016/j.nucana.2024.100112
Hassan Ouhadda , Mustapha Zerfaoui , Karim Bahhous , Yassine Oulhouq , Abdessamad Didi , Abdeslem Rrhioua , Dikra Bakari

This study investigates the critical significance of anode material selection in defining the energy spectrum and properties of X-ray photons in medical physics applications. Using the GATE platform and Monte Carlo simulations, a direct relationship between anode material atomic number and photon fluence is demonstrated. As the atomic number increases from Z = 29 (Copper) to Z = 74 (Tungsten), photon fluence rises by 62 %, indicating a substantial impact on X-ray production. Furthermore, the X-ray spectrum is affected by this material-driven changes, revealing a noticeable shift towards higher energy values: the mean energy of the continuous spectrum rises from 46.97 keV for Copper to 49.0 keV for Tungsten. The thermal properties of the material affect the temperature increase at the focal point. Rhodium and Molybdenum have a higher temperature rise than Copper (Cu) and Tungsten (W), because Cu and W have a greater thermal diffusion compared to other materials. These findings underscore the significance of anode material choice in optimizing X-ray systems which may enhance diagnostic accuracy and efficiency in diverse applications.

本研究探讨了阳极材料的选择在确定医学物理应用中 X 射线光子的能谱和特性方面的重要意义。利用 GATE 平台和蒙特卡罗模拟,证明了阳极材料原子序数与光子通量之间的直接关系。当原子序数从 Z = 29(铜)增加到 Z = 74(钨)时,光子通量增加了 62%,表明这对 X 射线的产生有重大影响。此外,X 射线光谱也受到这种材料驱动变化的影响,显示出向高能量值的明显转变:连续光谱的平均能量从铜的 46.97 keV 上升到钨的 49.0 keV。材料的热特性会影响焦点处的温度升高。铑和钼的温升比铜(Cu)和钨(W)高,因为与其他材料相比,铜和钨的热扩散能力更强。这些发现强调了选择阳极材料对优化 X 射线系统的重要意义,可提高各种应用中的诊断准确性和效率。
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引用次数: 0
Simulating the impact of electron beam energy deposition on lead target temperature 模拟电子束能量沉积对铅靶温度的影响
Pub Date : 2024-06-01 DOI: 10.1016/j.nucana.2024.100113
Walid Oueslati

This study delves into the thermal dynamics induced by an electron beam sourced from the CIRCE III accelerator, focusing on a lead target previously employed at the National Centre for Nuclear Science and Technology (CNSTN) in Tunisia for neutron and photon production. Leveraging FLUKA software, we simulate the intricate interplay between electrons and the target surface, analyzing variations in deposited energy across different target thicknesses. Beyond elucidating the electron-target interaction, our investigation extends to predicting crucial parameters such as the maximum operational threshold and surface temperature distribution of the target. To achieve this, a computational model harnessing the finite volume method is employed, offering insights into the thermal response dynamics and paving the way for optimized operational protocols and target design refinements. Through this comprehensive analysis, we aim to advance the understanding of thermal phenomena in electron-target interactions, thereby bolstering the efficiency and safety of particle accelerator operations in diverse scientific applications.

本研究深入探讨了来自 CIRCE III 加速器的电子束所引起的热动力学,重点是突尼斯国家核科学技术中心(CNSTN)以前用于中子和光子生产的铅靶。利用 FLUKA 软件,我们模拟了电子与靶表面之间错综复杂的相互作用,分析了不同靶厚度下沉积能量的变化。除了阐明电子与靶的相互作用外,我们的研究还扩展到预测靶的最大运行阈值和表面温度分布等关键参数。为此,我们采用了一个利用有限体积法的计算模型,以深入了解热响应动力学,为优化操作规程和改进靶设计铺平道路。通过这项综合分析,我们旨在推进对电子-靶相互作用中热现象的理解,从而提高粒子加速器在各种科学应用中的运行效率和安全性。
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引用次数: 0
期刊
Nuclear Analysis
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