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Temperature distribution in the PGAA system: Collimator, shutter, and filter in TRIGA Mark II reactor PGAA 系统中的温度分布:TRIGA Mark II 反应器中的准直器、快门和过滤器
Pub Date : 2024-07-09 DOI: 10.1016/j.nucana.2024.100120
Jamila Yousfi , Abdessamad Didi , Hamane Lemziouka , Lamiae Mrharrab , Hamid Amsil , Otman Jai , Hamid Bounouira , Khalid Larakil

This article examines the impact of temperature on the steel collimator cap and the primary beam shutter. These components will be used to implement the Prompt Gamma Activation Analysis (PGAA) technique in the Moroccan TRIGA Mark-II research reactor. The steel collimator plug is essential for forming the neutron beam, while the main role of the shutter is to stop the beam when the channel is inactive. This study analyzes the effect of temperature on the collimator and shutter system, particularly focusing on the variation in maximum temperature over a month of operation with 8-h cycles per day, the behavior of temperature over 24 h, the total heat flux as a function of the length of the experimental device, the temperature distribution in mild steel (E235) and 304L stainless steel materials, and the total displacement and strain gradient as a function of temperature. All calculations were performed using COMSOL Multiphysics simulation software, based on the finite element method.

本文研究了温度对钢制准直器盖和主光束快门的影响。这些部件将用于在摩洛哥 TRIGA Mark-II 研究反应堆中实施即时伽马活化分析(PGAA)技术。钢制准直器塞对于中子束的形成至关重要,而快门的主要作用是在通道处于非活动状态时阻止中子束。本研究分析了温度对准直器和快门系统的影响,尤其侧重于每天 8 小时周期运行一个月内最高温度的变化、24 小时内的温度行为、总热通量与实验装置长度的函数关系、低碳钢(E235)和 304L 不锈钢材料的温度分布以及总位移和应变梯度与温度的函数关系。所有计算均使用基于有限元法的 COMSOL Multiphysics 仿真软件进行。
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引用次数: 0
Exploring the impact of anode material on X-ray photon fluence and characteristics: A Monte Carlo simulation study 探索阳极材料对 X 射线光子通量和特性的影响:蒙特卡罗模拟研究
Pub Date : 2024-06-01 DOI: 10.1016/j.nucana.2024.100112
Hassan Ouhadda , Mustapha Zerfaoui , Karim Bahhous , Yassine Oulhouq , Abdessamad Didi , Abdeslem Rrhioua , Dikra Bakari

This study investigates the critical significance of anode material selection in defining the energy spectrum and properties of X-ray photons in medical physics applications. Using the GATE platform and Monte Carlo simulations, a direct relationship between anode material atomic number and photon fluence is demonstrated. As the atomic number increases from Z = 29 (Copper) to Z = 74 (Tungsten), photon fluence rises by 62 %, indicating a substantial impact on X-ray production. Furthermore, the X-ray spectrum is affected by this material-driven changes, revealing a noticeable shift towards higher energy values: the mean energy of the continuous spectrum rises from 46.97 keV for Copper to 49.0 keV for Tungsten. The thermal properties of the material affect the temperature increase at the focal point. Rhodium and Molybdenum have a higher temperature rise than Copper (Cu) and Tungsten (W), because Cu and W have a greater thermal diffusion compared to other materials. These findings underscore the significance of anode material choice in optimizing X-ray systems which may enhance diagnostic accuracy and efficiency in diverse applications.

本研究探讨了阳极材料的选择在确定医学物理应用中 X 射线光子的能谱和特性方面的重要意义。利用 GATE 平台和蒙特卡罗模拟,证明了阳极材料原子序数与光子通量之间的直接关系。当原子序数从 Z = 29(铜)增加到 Z = 74(钨)时,光子通量增加了 62%,表明这对 X 射线的产生有重大影响。此外,X 射线光谱也受到这种材料驱动变化的影响,显示出向高能量值的明显转变:连续光谱的平均能量从铜的 46.97 keV 上升到钨的 49.0 keV。材料的热特性会影响焦点处的温度升高。铑和钼的温升比铜(Cu)和钨(W)高,因为与其他材料相比,铜和钨的热扩散能力更强。这些发现强调了选择阳极材料对优化 X 射线系统的重要意义,可提高各种应用中的诊断准确性和效率。
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引用次数: 0
Simulating the impact of electron beam energy deposition on lead target temperature 模拟电子束能量沉积对铅靶温度的影响
Pub Date : 2024-06-01 DOI: 10.1016/j.nucana.2024.100113
Walid Oueslati

This study delves into the thermal dynamics induced by an electron beam sourced from the CIRCE III accelerator, focusing on a lead target previously employed at the National Centre for Nuclear Science and Technology (CNSTN) in Tunisia for neutron and photon production. Leveraging FLUKA software, we simulate the intricate interplay between electrons and the target surface, analyzing variations in deposited energy across different target thicknesses. Beyond elucidating the electron-target interaction, our investigation extends to predicting crucial parameters such as the maximum operational threshold and surface temperature distribution of the target. To achieve this, a computational model harnessing the finite volume method is employed, offering insights into the thermal response dynamics and paving the way for optimized operational protocols and target design refinements. Through this comprehensive analysis, we aim to advance the understanding of thermal phenomena in electron-target interactions, thereby bolstering the efficiency and safety of particle accelerator operations in diverse scientific applications.

本研究深入探讨了来自 CIRCE III 加速器的电子束所引起的热动力学,重点是突尼斯国家核科学技术中心(CNSTN)以前用于中子和光子生产的铅靶。利用 FLUKA 软件,我们模拟了电子与靶表面之间错综复杂的相互作用,分析了不同靶厚度下沉积能量的变化。除了阐明电子与靶的相互作用外,我们的研究还扩展到预测靶的最大运行阈值和表面温度分布等关键参数。为此,我们采用了一个利用有限体积法的计算模型,以深入了解热响应动力学,为优化操作规程和改进靶设计铺平道路。通过这项综合分析,我们旨在推进对电子-靶相互作用中热现象的理解,从而提高粒子加速器在各种科学应用中的运行效率和安全性。
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引用次数: 0
Temperature feedback reactivity analysis for LEU-Fuelled SLOWPOKE-2 research reactor using DRAGON5 and DONJON5 codes 使用 DRAGON5 和 DONJON5 代码对 LEU-Fuelled SLOWPOKE-2 研究反应堆进行温度反馈反应性分析
Pub Date : 2024-04-29 DOI: 10.1016/j.nucana.2024.100111
Otman Jaï , Otmane El Hajjaji , Abdessamad Didi

The purpose of this study is to provide a new deterministic model for the SLOWPOKE-2 nuclear research reactor at École Polytechnique de Montréal (EPM) with LEU (Low Enriched Uranium) core. Using the latest release of the code system DRAGON5 and DONJON5 and the cross-section data library ENDFB.VII rel.1 evaluation, the developed model is applied to simulate the neutronic behavior of the SLOWPOKE-2 research reactor. We studied the separate temperature effects of the main components of the core (i.e., fuel, coolant/moderator, beryllium reflector, and water reflector). The contribution of different physical phenomena to the RTC was assessed. The temperature reactivity feedback calculated using the deterministic approach based on the DRAGON5 and DONJON5 code system using the ENDF/B-VII.1 evaluated nuclear data library produced in the WIMD-D4 format is in good agreement. Therefore, this work proves the capability of DRAGON5 and DONJON5 codes, normally used for power reactors, to reliably simulate a low-power research reactor.

本研究的目的是为蒙特利尔理工学院(EPM)采用 LEU(低浓铀)堆芯的 SLOWPOKE-2 核研究反应堆提供一个新的确定性模型。利用最新发布的 DRAGON5 和 DONJON5 代码系统以及截面数据图书馆 ENDFB.VII rel.1 评估,所开发的模型被用于模拟 SLOWPOKE-2 研究反应堆的中子行为。我们研究了堆芯主要部件(即燃料、冷却剂/慢化剂、铍反射器和水反射器)的单独温度效应。我们评估了不同物理现象对 RTC 的贡献。使用基于 DRAGON5 和 DONJON5 代码系统的确定性方法,利用 WIMD-D4 格式制作的ENDF/B-VII.1 评估核数据图书馆计算出的温度反应性反馈非常一致。因此,这项工作证明了通常用于动力反应堆的 DRAGON5 和 DONJON5 代码能够可靠地模拟低功率研究反应堆。
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引用次数: 0
Strategic analysis for advancing Morocco's nuclear infrastructure using PESTELE framework 利用 PESTELE 框架推进摩洛哥核基础设施的战略分析
Pub Date : 2024-04-05 DOI: 10.1016/j.nucana.2024.100110
Hafsa Housni , Naila Amrous , Najima Daoudi , Mohamed Jaouad Malzi

Morocco's exploration of nuclear energy aligns with both climate goals and national energy ambitions, offering a promising low-carbon alternative to conventional fossil fuels. Despite the nation's significant strides in renewable energy, nuclear power remains understudied, revealing a critical literature gap. This research underscores the global imperative to transition to net-zero emissions and the pivotal role nuclear energy plays in addressing climate change. Within the context of Morocco's 2030 plan, which prioritizes renewable energy, nuclear energy stands as an underexplored aspect, lacking comprehensive research. To bridge this gap, the study employs a PESTLE analysis to examine the political, economic, societal, technological, legal, and environmental factors influencing Morocco's nuclear energy landscape. The integration of insights from various sources, including press releases, reports, and scientific publications, ensures a holistic and well-informed perspective on Morocco's nuclear industry. The paper concludes by providing an overview of nuclear energy use on different scales, accompanied by a detailed discussion of the PESTLE analysis outcomes. This approach seeks to contribute valuable insights for informed decision-making and strategic planning in the realm of nuclear energy development.

摩洛哥对核能的探索符合气候目标和国家能源雄心,为传统化石燃料提供了一种前景广阔的低碳替代能源。尽管摩洛哥在可再生能源方面取得了长足进步,但对核能的研究仍然不足,这暴露出了一个重要的文献空白。这项研究强调了全球向净零排放过渡的必要性,以及核能在应对气候变化方面发挥的关键作用。摩洛哥的 2030 年计划将可再生能源列为优先事项,在这一背景下,核能是一个未被充分探索的方面,缺乏全面的研究。为了弥补这一不足,本研究采用了 PESTLE 分析法,以考察影响摩洛哥核能格局的政治、经济、社会、技术、法律和环境因素。通过整合各种来源(包括新闻稿、报告和科学出版物)的见解,确保对摩洛哥核工业有一个全面和充分了解的视角。本文最后概述了不同规模的核能利用情况,并对 PESTLE 分析结果进行了详细讨论。这种方法旨在为核能发展领域的知情决策和战略规划提供有价值的见解。
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引用次数: 0
Adsorption of molybdenum (VI) from wastewater using a metal-organic framework material 利用金属有机框架材料吸附废水中的钼 (VI)
Pub Date : 2024-03-01 DOI: 10.1016/j.nucana.2024.100101
Rui Zhang, Wanjun Mu

With the aim of removing 99Mo from radioactive wastewater, a metal-organic framework Zr-MOF and its functionalized derivatives (Zr-MOF-SO4 and Zr-MOF-C2O4) were prepared as adsorbents, and characterized by SEM, XPS and FI-IR. The results showed the –SO4 and –C2O4 groups were successfully loaded onto the surface of the original Zr-MOF; the obtained Zr-MOF-SO4 and Zr-MOF-C2O4 presented different morphologies as small pellets. Both exhibit high adsorption efficiency and fast adsorption rates due to their abundant –SO4 and –C2O4 surface groups, that provide many adsorption sites for Mo(VI). The maximum adsorption capacities for Mo(VI) of Zr-MOF-SO4 and Zr-MOF-C2O4 are 192.5 mg g−1 and 432.3 mg g−1, respectively, which is an improvement over other similar adsorbents. In addition, thermodynamic studies indicate a spontaneous exothermic mechanism for the adsorption process. These results demonstrate that anchoring of the functionalized groups is a good way to improve Mo(VI) adsorption capacity of MOF materials.

以去除放射性废水中的 99Mo 为目的,制备了金属有机框架 Zr-MOF 及其功能化衍生物(Zr-MOF-SO4 和 Zr-MOF-C2O4)作为吸附剂,并通过扫描电镜、XPS 和 FI-IR 对其进行了表征。结果表明,-SO4 和 -C2O4 基团成功地负载到了原始 Zr-MOF 的表面;得到的 Zr-MOF-SO4 和 Zr-MOF-C2O4 呈现出不同的小颗粒形态。二者都表现出较高的吸附效率和较快的吸附速率,这是因为它们表面有大量的 -SO4 和 -C2O4 基团,为 Mo(VI) 提供了许多吸附位点。Zr-MOF-SO4 和 Zr-MOF-C2O4 对 Mo(VI) 的最大吸附容量分别为 192.5 mg g-1 和 432.3 mg g-1,比其他同类吸附剂有所提高。此外,热力学研究表明吸附过程存在自发放热机制。这些结果表明,锚定功能化基团是提高 MOF 材料 Mo(VI) 吸附能力的一种好方法。
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引用次数: 0
Determination of 58Fe/54Fe isotope ratios in Chang’E-5 lunar regolith by instrumental neutron activation analysis 利用仪器中子活化分析测定嫦娥五号月球碎屑中的 58Fe/54Fe 同位素比率
Pub Date : 2024-03-01 DOI: 10.1016/j.nucana.2024.100102
Yonggang Yao, Caijin Xiao, Liang Zhao, Yuqing Li, Tianfu Li, Bing Guo, Dongfeng Chen

Traditionally, the determination of isotope ratios is analyzed by mass spectrometry (MS) method, which is usually destructive to sample (i.e., sample dissolution). Furthermore, the 58Fe abundance (0.282%) is generally rather low relative to other Fe isotopes, therefore, 58Fe/54Fe results is not reported in the routine measurement for MS methods. Given the importance of investigating a possible genetic relationship between the stable isotope composition of the Moon and the Earth, here, we firstly report the isotope ratios of 58Fe/54Fe in the Chang’E-5 (CE-5) scooped bulk lunar sample. In this work, the 58Fe/54Fe ratios were analyzed by instrumental neutron activation analysis (INAA) which is essentially distinguished and a potentially complementary advantage for MS in the determination of stable isotope ratios. These data obtained for the CE-5 lunar sample were also compared with those of terrestrial sample GBW07105.

传统上,同位素比值的测定是通过质谱法(MS)进行分析的,而质谱法通常对样品具有破坏性(即样品溶解)。此外,58Fe 丰度(0.282%)相对于其他铁同位素而言通常较低,因此在质谱法的常规测量中没有报告 58Fe/54Fe 的结果。鉴于研究月球与地球稳定同位素组成之间可能存在的遗传关系的重要性,我们在此首次报告了嫦娥五号(CE-5)舀取的块状月球样品中 58Fe/54Fe 的同位素比值。在这项工作中,58Fe/54Fe的比值是通过仪器中子活化分析(INAA)进行分析的,INAA与MS在测定稳定同位素比值方面有着本质的区别和潜在的互补优势。CE-5 月球样品获得的这些数据还与地面样品 GBW07105 的数据进行了比较。
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引用次数: 0
The blackening of organotin catalyzed silicone adhesive via low dose rate gamma irradiation 通过低剂量率伽马辐照使有机锡催化的硅胶粘合剂变黑
Pub Date : 2023-12-28 DOI: 10.1016/j.nucana.2023.100100
Bo Liu, Lei Yu, Yinyong Ao, Pucheng Wang, Wei Huang

Low dose rate gamma irradiation blackening effect of organotin catalyzed silicone adhesive is presented. When the total dose accumulated to 350 kGy at low dose rate (0.03 Gy/s), there is a significant blackening of the color changing from transparent to black by the increasing of dose, which is simultaneously deepened by the decreasing of dose rate. That is, low dose rate and accumulated dose both affect the final color of silicone adhesive. The structure changes of silicone adhesive before and after blackening are characterized by UV–vis, FTIR, and SPME-GC-MS, and the mechanism of blackening is deduced to be related to the content of SnO.

介绍了有机锡催化硅酮胶的低剂量率伽马辐照黑化效应。在低剂量率(0.03 Gy/s)条件下,当总剂量累积到 350 kGy 时,随着剂量的增加,硅胶的颜色由透明变为黑色,同时随着剂量率的降低,颜色加深。也就是说,低剂量率和累积剂量都会影响硅酮胶的最终颜色。通过紫外-可见光、傅立叶变换红外光谱和 SPME-GC-MS 对硅胶变黑前后的结构变化进行了表征,并推断出变黑的机理与氧化锡的含量有关。
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引用次数: 0
Design of emergency solar energy system adjacent the nuclear power plant to prevent nuclear accidents and increase safety 设计核电站附近的应急太阳能系统,以防止核事故并提高安全性
Pub Date : 2023-12-20 DOI: 10.1016/j.nucana.2023.100092
M. Chabook, S. Tashakor

Providing sufficient energy in emergency situations in nuclear power plants is of great importance due to their crucial role in improving power plant safety and eliminating disasters.

Solar power is capable of providing a secure energy source which could be used for emergency power loads. The main goal of this study is application of solar energy for providing emergency loads of the Tehran research reactor. A 100 kW solar power plant connected to the grid and 400 kWh battery pack which is capable of providing 50 kw loads for 8 h is designed. As the first priority, the plant charges the battery pack and discharges excess energy to the power grid. Therefore, the proposed scheme, in addition to increasing safety, also has economic benefits. Design procedure of the power plant was carried out using PVsyst which is international well known software for designing solar power plants and results were investigated. Economic evaluation of the project is carried out using RETSCREEN software and different schemes are evaluated. Due to the critical nature of the power loads and their sensitivity, application of this scheme for providing emergency energy loads of the Tehran research reactor is suggested. Considering the expansion of nuclear safety and the protection of the environment and humanity, we request the respected editors and reviewers of the journal to have positive opinions about the publication of the article.

太阳能能够提供安全的能源,可用于应急电力负荷。本研究的主要目标是应用太阳能为德黑兰研究反应堆提供应急负荷。设计了一个与电网相连的 100 千瓦太阳能发电站和 400 千瓦时电池组,可在 8 小时内提供 50 千瓦负荷。作为首要任务,发电站为电池组充电,并将多余的能量释放到电网。因此,建议的方案除了提高安全性外,还具有经济效益。发电厂的设计程序是利用国际知名的太阳能发电厂设计软件 PVsyst 进行的,并对结果进行了调查。使用 RETSCREEN 软件对项目进行了经济评估,并对不同的方案进行了评估。由于电力负荷的关键性质及其敏感性,建议将该方案用于为德黑兰研究反应堆提供紧急能源负荷。考虑到核安全的扩展以及对环境和人类的保护,我们请求尊敬的期刊编辑和审稿人对文章的发表提出积极的意见。
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引用次数: 0
The lifetime distribution of finite fission chain group around the prompt criticality 迅速临界周围有限裂变链组的寿命分布
Pub Date : 2023-12-04 DOI: 10.1016/j.nucana.2023.100091
Hui Gao, Qilin Xie, Xiaoqiang Fan

In order to describe the behavior of finite fission chains in a fission system initiated by a δ neutron source, we present the conception of the finite fission chains group (FFCG). The group is the collectivity of the fission chains initiated by plenty of neutrons at the same time. Based on the result of the solving generating function, we deduced the lifetime distribution formula of FFCG based on the point kinetics model. Finally, the formula is validated by the experiment with a single pulse neutron source in CFBR-Ⅱ.

为了描述由δ中子源引发的裂变系统中有限裂变链的行为,我们提出了有限裂变链组(FFCG)的概念。该组是由大量中子同时引发的裂变链的集合体。根据求解生成函数的结果,我们推导出了基于点动力学模型的 FFCG 寿命分布公式。最后,该公式通过 CFBR-Ⅱ 中的单脉冲中子源实验得到了验证。
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引用次数: 0
期刊
Nuclear Analysis
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