首页 > 最新文献

Progress in Nuclear Energy最新文献

英文 中文
Fuzzy adaptive sliding mode control of U-tube steam generator water level based on a nonlinear dynamic model 基于非线性动态模型的u型管蒸汽发生器水位模糊自适应滑模控制
IF 3.2 3区 工程技术 Q1 NUCLEAR SCIENCE & TECHNOLOGY Pub Date : 2026-03-01 Epub Date: 2026-01-06 DOI: 10.1016/j.pnucene.2025.106235
Ze Zhu , Xiaojie Guo , Zhiwu Ke , Kelong Zhang , Pengfei Wang
The false water level caused by the so-called “swell and shrink”, and the measurement errors, are the two major challenges in the water level control of U-tube steam generators (UTSGs). This paper proposes a fuzzy adaptive sliding mode controller (FASMC), which effectively mitigates the adverse impacts of false water levels, thus improving the water level control performance. Firstly, an ideal SMC (ISMC) was designed based on a detailed nonlinear UTSG model. Then, to reduce the adverse impacts of measurement errors, a water level estimator was constructed based on the backstepping and Lyapunov's second method, and an adaptive SMC (ASMC) was designed. Finally, the fuzzy algorithm was used to calibrate the hyperparameters in the ASMC online. The simulation results show that the established ISMC, ASMC, and FASMC outperform the PID controller under different operating conditions, with the integrated absolute errors (IAEs) of water level reduced by at least 5.68 %. And the FASMC has the best performance, with the IAE reduced by up to 74.8 %. This demonstrates the effectiveness and superiors of the proposed FASMC, which can provide a valuable reference for mitigating the adverse impacts of false water level in engineering practices and improving the UTSG water level control performance.
所谓“胀缩”引起的假水位和测量误差是u型管蒸汽发生器水位控制面临的两大挑战。本文提出了一种模糊自适应滑模控制器(FASMC),有效地减轻了假水位的不利影响,从而提高了水位控制性能。首先,基于详细的非线性UTSG模型,设计了理想SMC (ISMC)。然后,为了减小测量误差的不利影响,基于反推法和Lyapunov第二方法构造了水位估计器,并设计了自适应SMC (ASMC)。最后,利用模糊算法对ASMC超参数进行在线标定。仿真结果表明,所建立的ISMC、ASMC和FASMC在不同工况下均优于PID控制器,水位的综合绝对误差(iae)至少降低了5.68%。其中FASMC的性能最好,IAE降低了74.8%。验证了该方法的有效性和优越性,可为工程实践中减轻假水位的不利影响,提高UTSG水位控制性能提供有价值的参考。
{"title":"Fuzzy adaptive sliding mode control of U-tube steam generator water level based on a nonlinear dynamic model","authors":"Ze Zhu ,&nbsp;Xiaojie Guo ,&nbsp;Zhiwu Ke ,&nbsp;Kelong Zhang ,&nbsp;Pengfei Wang","doi":"10.1016/j.pnucene.2025.106235","DOIUrl":"10.1016/j.pnucene.2025.106235","url":null,"abstract":"<div><div>The false water level caused by the so-called “swell and shrink”, and the measurement errors, are the two major challenges in the water level control of U-tube steam generators (UTSGs). This paper proposes a fuzzy adaptive sliding mode controller (FASMC), which effectively mitigates the adverse impacts of false water levels, thus improving the water level control performance. Firstly, an ideal SMC (ISMC) was designed based on a detailed nonlinear UTSG model. Then, to reduce the adverse impacts of measurement errors, a water level estimator was constructed based on the backstepping and Lyapunov's second method, and an adaptive SMC (ASMC) was designed. Finally, the fuzzy algorithm was used to calibrate the hyperparameters in the ASMC online. The simulation results show that the established ISMC, ASMC, and FASMC outperform the PID controller under different operating conditions, with the integrated absolute errors (IAEs) of water level reduced by at least 5.68 %. And the FASMC has the best performance, with the IAE reduced by up to 74.8 %. This demonstrates the effectiveness and superiors of the proposed FASMC, which can provide a valuable reference for mitigating the adverse impacts of false water level in engineering practices and improving the UTSG water level control performance.</div></div>","PeriodicalId":20617,"journal":{"name":"Progress in Nuclear Energy","volume":"193 ","pages":"Article 106235"},"PeriodicalIF":3.2,"publicationDate":"2026-03-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145927142","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
The α-radiolysis behavior and mechanism of tri-isoamyl phosphate (TiAP): New insights from 4He2+ beam irradiation experiments and theoretical calculations 磷酸三异戊酯(TiAP) α-辐射分解行为和机理:来自4He2+辐照实验和理论计算的新见解
IF 3.2 3区 工程技术 Q1 NUCLEAR SCIENCE & TECHNOLOGY Pub Date : 2026-03-01 Epub Date: 2026-01-06 DOI: 10.1016/j.pnucene.2025.106233
Shilong Shi , Yaoshuang Wan , Guofeng Qu , Runyu Zhang , Jiajian Song , Xuanhao Huang , Jijun Yang , Zhihui Li , Tu Lan , Songdong Ding , Yuanyou Yang , Jiali Liao , Wen Feng , Jing Peng , Ning Liu
Understanding the α-radiolysis of extractants is crucial for their applications in nuclear fuel reprocessing. However, current methodologies face challenges in conducting α-irradiation experiments and elucidating the underlying mechanisms. Herein, a 4–7 MeV 4He2+ beam provided by a CS-30 cyclotron was employed as a fast, convenient, and versatile α-irradiation source to simulate actual radiative scenarios in nuclear fuel reprocessing, which was firstly employed to investigate the α-radiolysis of tri-iso-amyl phosphate (TiAP) in alkane diluent, an alternative extractant in Plutonium Uranium Recovery by Extraction. The dominant radiolysis products of TiAP including hydrogen, methane and di-iso-amyl phosphate (DiAP) were qualitatively and quantitatively determined by GC and HR-MS. Ehrenfest dynamic simulations and DFT calculations revealed the ionization of TiAP induced by electronic stopping is the dominant process in its α-radiolysis process, as confirmed by experimental results. The C‒O bond cleavage in TiAP, leading to the formation of DiAP, is attributed to the decomposition of TiAP+ and TiAP∗, as well as reactions between TiAP and ·OH or secondary electrons. Finally, the radiolysis mechanism of TiAP in alkane diluent was proposed based on the analysis of radiolytic products and multi-time-scale theoretical calculations. This study paves the way for advancing research on the α-radiolysis of extractants for spent fuel reprocessing.
了解萃取剂的α-辐射分解对其在核燃料后处理中的应用至关重要。然而,目前的方法在进行α-辐照实验和阐明潜在机制方面面临挑战。本文采用CS-30回旋加速器提供的4-7 MeV 4He2+束流作为快速、方便、通用的α-辐照源,模拟了核燃料后处理过程中的实际辐射情景,并首次应用该辐照源研究了三异戊基磷酸(TiAP)在提取法回收钚铀的替代萃取剂烷烃稀释剂中的α-辐射分解。采用气相色谱(GC)和质谱(HR-MS)对TiAP的主要辐射分解产物氢、甲烷和磷酸二异戊酯(DiAP)进行了定性和定量分析。Ehrenfest动力学模拟和DFT计算表明,TiAP α-辐射分解过程中电子停止引起的电离是主要过程,实验结果也证实了这一点。TiAP中C-O键的断裂导致了DiAP的形成,这归因于TiAP+和TiAP *的分解,以及TiAP与·OH或二次电子之间的反应。最后,通过辐射分解产物分析和多时间尺度理论计算,提出了TiAP在烷烃稀释剂中的辐射分解机理。本研究为推进乏燃料后处理萃取剂α-辐射分解的研究奠定了基础。
{"title":"The α-radiolysis behavior and mechanism of tri-isoamyl phosphate (TiAP): New insights from 4He2+ beam irradiation experiments and theoretical calculations","authors":"Shilong Shi ,&nbsp;Yaoshuang Wan ,&nbsp;Guofeng Qu ,&nbsp;Runyu Zhang ,&nbsp;Jiajian Song ,&nbsp;Xuanhao Huang ,&nbsp;Jijun Yang ,&nbsp;Zhihui Li ,&nbsp;Tu Lan ,&nbsp;Songdong Ding ,&nbsp;Yuanyou Yang ,&nbsp;Jiali Liao ,&nbsp;Wen Feng ,&nbsp;Jing Peng ,&nbsp;Ning Liu","doi":"10.1016/j.pnucene.2025.106233","DOIUrl":"10.1016/j.pnucene.2025.106233","url":null,"abstract":"<div><div>Understanding the α-radiolysis of extractants is crucial for their applications in nuclear fuel reprocessing. However, current methodologies face challenges in conducting α-irradiation experiments and elucidating the underlying mechanisms. Herein<strong>,</strong> a 4–7 MeV <sup>4</sup>He<sup>2+</sup> beam provided by a CS-30 cyclotron was employed as a fast, convenient, and versatile α-irradiation source to simulate actual radiative scenarios in nuclear fuel reprocessing, which was firstly employed to investigate the α-radiolysis of tri-iso-amyl phosphate (TiAP) in alkane diluent, an alternative extractant in Plutonium Uranium Recovery by Extraction. The dominant radiolysis products of TiAP including hydrogen, methane and di-iso-amyl phosphate (DiAP) were qualitatively and quantitatively determined by GC and HR-MS. Ehrenfest dynamic simulations and DFT calculations revealed the ionization of TiAP induced by electronic stopping is the dominant process in its α-radiolysis process, as confirmed by experimental results. The C‒O bond cleavage in TiAP, leading to the formation of DiAP, is attributed to the decomposition of TiAP<sup>+</sup> and TiAP∗, as well as reactions between TiAP and ·OH or secondary electrons. Finally, the radiolysis mechanism of TiAP in alkane diluent was proposed based on the analysis of radiolytic products and multi-time-scale theoretical calculations. This study paves the way for advancing research on the α-radiolysis of extractants for spent fuel reprocessing.</div></div>","PeriodicalId":20617,"journal":{"name":"Progress in Nuclear Energy","volume":"193 ","pages":"Article 106233"},"PeriodicalIF":3.2,"publicationDate":"2026-03-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145927139","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
A study on the long-term variation of signal current in rhodium self-powered neutron detectors under in-core burnup conditions 在堆芯内燃耗条件下铑自供电中子探测器信号电流长期变化的研究
IF 3.2 3区 工程技术 Q1 NUCLEAR SCIENCE & TECHNOLOGY Pub Date : 2026-03-01 Epub Date: 2026-01-03 DOI: 10.1016/j.pnucene.2025.106232
Zhi-qi Guo , Wen-hua Yang , Jing-yi Han , Shuo Zhang , Chun-hui Zhang , Zhan Li , Ding-jun Zhu , Jian-xiong Shao
As a key instrument for measuring neutron flux within a reactor core, the signal current of a Self-Powered Neutron Detector (SPND) is subject to change due to continuous material burnup. Accurately accounting for the long-term evolution of SPND signals is essential for reliable power monitoring and safe reactor operation. This study focuses on the Rhodium Self-Powered Neutron Detector (Rh-SPND) and, within the context of a typical Pressurized Water Reactor (PWR), develops a predictive model for signal current variation using a Back Propagation Neural Network (BPNN). The model incorporates changes in emitter material composition due to burnup and utilizes a layered approach to calculate the radial distribution of burnup. Key parameters such as beta electron generation rate, escape probability, gamma photon generation, and gamma-induced electron escape rate are all taken into account. Results show that over a 10-year period at a neutron flux of 1 × 1014 n/(cm2·s), the smaller the radius of the rhodium wire, the greater the variation in detector sensitivity. Specifically, a 0.1 mm wire radius results in a 51.3 % sensitivity reduction, while a 1 mm wire radius yields a 25.2 % reduction. The proposed model enables accurate sensitivity compensation for Rh-SPNDs over time, thereby minimizing neutron flux measurement errors and enhancing reactor safety and stability.
作为测量堆芯内中子通量的关键仪器,自供电中子探测器(SPND)的信号电流由于材料的持续燃烧而发生变化。准确计算SPND信号的长期演变对可靠的电力监测和反应堆的安全运行至关重要。本研究的重点是铑自供电中子探测器(Rh-SPND),并在典型的压水堆(PWR)的背景下,使用反向传播神经网络(BPNN)开发了信号电流变化的预测模型。该模型包含了由于燃耗引起的发射器材料组成的变化,并利用分层方法计算燃耗的径向分布。关键参数,如β电子产生率,逃逸概率,γ光子产生,和γ诱导电子逃逸率都考虑在内。结果表明,在中子通量为1 × 1014 n/(cm2·s)的10年周期内,铑丝半径越小,探测器灵敏度变化越大。具体来说,0.1 mm的线材半径会导致51.3%的灵敏度降低,而1 mm的线材半径会导致25.2%的灵敏度降低。所提出的模型能够对rh - spnd进行精确的灵敏度补偿,从而最大限度地减少中子通量测量误差,提高反应堆的安全性和稳定性。
{"title":"A study on the long-term variation of signal current in rhodium self-powered neutron detectors under in-core burnup conditions","authors":"Zhi-qi Guo ,&nbsp;Wen-hua Yang ,&nbsp;Jing-yi Han ,&nbsp;Shuo Zhang ,&nbsp;Chun-hui Zhang ,&nbsp;Zhan Li ,&nbsp;Ding-jun Zhu ,&nbsp;Jian-xiong Shao","doi":"10.1016/j.pnucene.2025.106232","DOIUrl":"10.1016/j.pnucene.2025.106232","url":null,"abstract":"<div><div>As a key instrument for measuring neutron flux within a reactor core, the signal current of a Self-Powered Neutron Detector (SPND) is subject to change due to continuous material burnup. Accurately accounting for the long-term evolution of SPND signals is essential for reliable power monitoring and safe reactor operation. This study focuses on the Rhodium Self-Powered Neutron Detector (Rh-SPND) and, within the context of a typical Pressurized Water Reactor (PWR), develops a predictive model for signal current variation using a Back Propagation Neural Network (BPNN). The model incorporates changes in emitter material composition due to burnup and utilizes a layered approach to calculate the radial distribution of burnup. Key parameters such as beta electron generation rate, escape probability, gamma photon generation, and gamma-induced electron escape rate are all taken into account. Results show that over a 10-year period at a neutron flux of 1 × 10<sup>14</sup> n/(cm<sup>2</sup>·s), the smaller the radius of the rhodium wire, the greater the variation in detector sensitivity. Specifically, a 0.1 mm wire radius results in a 51.3 % sensitivity reduction, while a 1 mm wire radius yields a 25.2 % reduction. The proposed model enables accurate sensitivity compensation for Rh-SPNDs over time, thereby minimizing neutron flux measurement errors and enhancing reactor safety and stability.</div></div>","PeriodicalId":20617,"journal":{"name":"Progress in Nuclear Energy","volume":"193 ","pages":"Article 106232"},"PeriodicalIF":3.2,"publicationDate":"2026-03-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145927080","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Innovative design and safety evaluation of the decay heat removal system for the China fast reactor 中国快堆消热系统的创新设计与安全性评价
IF 3.2 3区 工程技术 Q1 NUCLEAR SCIENCE & TECHNOLOGY Pub Date : 2026-03-01 Epub Date: 2026-01-10 DOI: 10.1016/j.pnucene.2026.106238
Zhiwen Dai , Donghui Zhang , Yuting Yang , Zhiwei Zhou , Chao Lin , Xiuli Xue , Xintai Yu , Dalin Zhang , Xiyong Chen , Shangang Cao , Songping Wang , Chengwen Xing , Shuiwen Jiang
Pool-type sodium-cooled fast reactors (SFR) have become one of the main selections of Generation-IV reactors due to large thermal inertia and inherent safety, which solve the future shortage of natural uranium and the disposal challenges of spent nuclear fuel (SNF). The decay heat removal system (DHRS) is one of the most important safety systems and must be highly reliable. This study illustrates the design and innovations of the DHRS on the China Fast Reactor. A thermal-hydraulic analysis was conducted using the system program (named ERAC) under station blackout (SBO) conditions, and key parameters of the natural circulation process were evaluated. China's fast reactor design is innovative in many respects, and its novel DHRS design ensures the reactor's safety during emergencies. The analysis results show that the DHRS system operates effectively and that the calculations align with the design goals. Under natural circulation, the peak temperature reached approximately 592 °C at 1000 s. As natural circulation progressed, the core outlet temperature gradually decreased; by 5000 s, the average core fuel outlet temperature was 574 °C. The design of the core throttling component meets the requirements and can provide sufficient natural circulation. This study could provide a valuable reference for the design of SFRs.
池式钠冷快堆(SFR)由于热惯量大、固有安全性好,已成为第四代反应堆的主要选择之一,解决了未来天然铀短缺和乏核燃料(SNF)处理的难题。衰变排热系统(DHRS)是最重要的安全系统之一,必须具有高可靠性。本研究说明了中国快堆的DHRS的设计和创新。利用系统程序(ERAC)进行了电站停电条件下的热液分析,并对自然循环过程的关键参数进行了评价。中国的快堆设计在许多方面具有创新性,其新颖的DHRS设计确保了反应堆在紧急情况下的安全性。分析结果表明,该系统运行有效,计算结果符合设计目标。在自然循环条件下,1000 s温度峰值约为592℃。随着自然循环的进行,岩心出口温度逐渐降低;到5000s时,堆芯燃料出口平均温度为574℃。核心节流元件的设计满足要求,并能提供充分的自然循环。本研究可为SFRs的设计提供有价值的参考。
{"title":"Innovative design and safety evaluation of the decay heat removal system for the China fast reactor","authors":"Zhiwen Dai ,&nbsp;Donghui Zhang ,&nbsp;Yuting Yang ,&nbsp;Zhiwei Zhou ,&nbsp;Chao Lin ,&nbsp;Xiuli Xue ,&nbsp;Xintai Yu ,&nbsp;Dalin Zhang ,&nbsp;Xiyong Chen ,&nbsp;Shangang Cao ,&nbsp;Songping Wang ,&nbsp;Chengwen Xing ,&nbsp;Shuiwen Jiang","doi":"10.1016/j.pnucene.2026.106238","DOIUrl":"10.1016/j.pnucene.2026.106238","url":null,"abstract":"<div><div>Pool-type sodium-cooled fast reactors (SFR) have become one of the main selections of Generation-IV reactors due to large thermal inertia and inherent safety, which solve the future shortage of natural uranium and the disposal challenges of spent nuclear fuel (SNF). The decay heat removal system (DHRS) is one of the most important safety systems and must be highly reliable. This study illustrates the design and innovations of the DHRS on the China Fast Reactor. A thermal-hydraulic analysis was conducted using the system program (named ERAC) under station blackout (SBO) conditions, and key parameters of the natural circulation process were evaluated. China's fast reactor design is innovative in many respects, and its novel DHRS design ensures the reactor's safety during emergencies. The analysis results show that the DHRS system operates effectively and that the calculations align with the design goals. Under natural circulation, the peak temperature reached approximately 592 °C at 1000 s. As natural circulation progressed, the core outlet temperature gradually decreased; by 5000 s, the average core fuel outlet temperature was 574 °C. The design of the core throttling component meets the requirements and can provide sufficient natural circulation. This study could provide a valuable reference for the design of SFRs.</div></div>","PeriodicalId":20617,"journal":{"name":"Progress in Nuclear Energy","volume":"193 ","pages":"Article 106238"},"PeriodicalIF":3.2,"publicationDate":"2026-03-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145927223","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Study on mixed convection heat transfer characteristics of liquid lead-bismuth eutectic 液态铅铋共晶混合对流换热特性研究
IF 3.2 3区 工程技术 Q1 NUCLEAR SCIENCE & TECHNOLOGY Pub Date : 2026-03-01 Epub Date: 2025-12-30 DOI: 10.1016/j.pnucene.2025.106205
Jieming Hou , Bo Kuang , Shirui Li , Wenjun Hu
This study experimentally investigated the mixed convective heat transfer characteristics of liquid lead-bismuth eutectic (LBE) under buoyancy-aided flow condition. Over 30 steady-state tests were conducted on the Multi-Application LBE Thermal-Hydraulic test facility (MATH). By independently varying heating power, tube diameter and loop resistance, the combined influence of forced and natural convection was systematically explored. Dimensionless parameters (Gr, Re, Nu) reveal that buoyancy effects remain negligible when GrRe2 < 0.01, with Nu close to the existing forced convection correlation. As buoyancy increases, heat transfer decreases, and the flow enters the mixed-convection regime. An empirical correlation for the mixed-convective heat transfer of lead-bismuth eutectic with buoyancy correction was proposed based on theoretical derivation and experimental data. Deviations between predicted and experimental data remain within ±10 %. The results improve the accuracy of thermal-hydraulic simulations for LBE-cooled fast reactors under natural-circulation accident scenarios and provide a validated benchmark for further studies at higher heat fluxes and different flow orientations.
实验研究了浮力辅助流动条件下液态铅铋共晶(LBE)混合对流换热特性。在多用途LBE热液试验装置(MATH)上进行了30多次稳态试验。通过单独改变加热功率、管径和回路阻力,系统探索了强迫对流和自然对流的综合影响。无因次参数(Gr, Re, Nu)表明,当GrRe2 <; 0.01时,浮力的影响可以忽略不计,Nu接近现有的强迫对流相关。随着浮力的增加,换热减少,气流进入混合对流状态。基于理论推导和实验数据,提出了铅铋共晶混合对流换热的浮力修正经验关系式。预测数据与实验数据之间的偏差保持在±10%以内。研究结果提高了lbe冷却快堆在自然循环事故情景下的热工模拟精度,并为进一步研究高热流通量和不同流动方向下的热工模拟提供了验证基准。
{"title":"Study on mixed convection heat transfer characteristics of liquid lead-bismuth eutectic","authors":"Jieming Hou ,&nbsp;Bo Kuang ,&nbsp;Shirui Li ,&nbsp;Wenjun Hu","doi":"10.1016/j.pnucene.2025.106205","DOIUrl":"10.1016/j.pnucene.2025.106205","url":null,"abstract":"<div><div>This study experimentally investigated the mixed convective heat transfer characteristics of liquid lead-bismuth eutectic (LBE) under buoyancy-aided flow condition. Over 30 steady-state tests were conducted on the Multi-Application LBE Thermal-Hydraulic test facility (MATH). By independently varying heating power, tube diameter and loop resistance, the combined influence of forced and natural convection was systematically explored. Dimensionless parameters (<em>Gr</em>, Re, <em>Nu</em>) reveal that buoyancy effects remain negligible when <span><math><mrow><mfrac><mtext>Gr</mtext><msup><mtext>Re</mtext><mn>2</mn></msup></mfrac></mrow></math></span> &lt; 0.01, with <em>Nu</em> close to the existing forced convection correlation. As buoyancy increases, heat transfer decreases, and the flow enters the mixed-convection regime. An empirical correlation for the mixed-convective heat transfer of lead-bismuth eutectic with buoyancy correction was proposed based on theoretical derivation and experimental data. Deviations between predicted and experimental data remain within ±10 %. The results improve the accuracy of thermal-hydraulic simulations for LBE-cooled fast reactors under natural-circulation accident scenarios and provide a validated benchmark for further studies at higher heat fluxes and different flow orientations.</div></div>","PeriodicalId":20617,"journal":{"name":"Progress in Nuclear Energy","volume":"193 ","pages":"Article 106205"},"PeriodicalIF":3.2,"publicationDate":"2026-03-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145884671","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Heterogeneity: A multi-robot radioactive source search technique 异质性:一种多机器人放射源搜索技术
IF 3.2 3区 工程技术 Q1 NUCLEAR SCIENCE & TECHNOLOGY Pub Date : 2026-03-01 Epub Date: 2026-01-01 DOI: 10.1016/j.pnucene.2025.106223
Jianwen Huo , Mingrun Ling , Junling Wang , Ying Zhou
In this study, we develop a search technique involving heterogeneous robots to achieve a rapid and accurate search for a lost radioactive source by effectively utilizing radiation data. The system includes robots with different levels of radiation resistance. Two fixed robots with lower radiation resistance are positioned at the edge of the environment to collect low-value radiation data and apply a maximum likelihood estimation algorithm based on the natural gradient (NG-MLE) for localization. Concurrently, a mobile robot with high radiation resistance enters the warning area to collect high-value radiation data, and the localization of the radioactive source is performed based on particle filtering and prior information obtained from the fixed robots. The movement of the mobile robot is directed by a decision-making algorithm based on Fisher information distance (FID). Simulation results show that the proposed algorithm achieves higher localization accuracy and requires fewer radiation detections.
在本研究中,我们开发了一种涉及异构机器人的搜索技术,通过有效利用辐射数据来实现对丢失放射源的快速准确搜索。该系统包括具有不同抗辐射水平的机器人。在环境边缘放置两个辐射阻力较低的固定机器人,收集低值辐射数据,并应用基于自然梯度的最大似然估计算法(NG-MLE)进行定位。同时,高抗辐射移动机器人进入预警区域采集高值辐射数据,基于粒子滤波和固定机器人获得的先验信息对放射源进行定位。移动机器人的运动由基于Fisher信息距离(FID)的决策算法指导。仿真结果表明,该算法具有较高的定位精度和较少的辐射检测。
{"title":"Heterogeneity: A multi-robot radioactive source search technique","authors":"Jianwen Huo ,&nbsp;Mingrun Ling ,&nbsp;Junling Wang ,&nbsp;Ying Zhou","doi":"10.1016/j.pnucene.2025.106223","DOIUrl":"10.1016/j.pnucene.2025.106223","url":null,"abstract":"<div><div>In this study, we develop a search technique involving heterogeneous robots to achieve a rapid and accurate search for a lost radioactive source by effectively utilizing radiation data. The system includes robots with different levels of radiation resistance. Two fixed robots with lower radiation resistance are positioned at the edge of the environment to collect low-value radiation data and apply a maximum likelihood estimation algorithm based on the natural gradient (NG-MLE) for localization. Concurrently, a mobile robot with high radiation resistance enters the warning area to collect high-value radiation data, and the localization of the radioactive source is performed based on particle filtering and prior information obtained from the fixed robots. The movement of the mobile robot is directed by a decision-making algorithm based on Fisher information distance (FID). Simulation results show that the proposed algorithm achieves higher localization accuracy and requires fewer radiation detections.</div></div>","PeriodicalId":20617,"journal":{"name":"Progress in Nuclear Energy","volume":"193 ","pages":"Article 106223"},"PeriodicalIF":3.2,"publicationDate":"2026-03-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145884609","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Void fraction migration in developing bubbly flow through sudden cross-section contraction and expansion in square channels 方形通道中突然横截面收缩和膨胀的气泡流动中空隙率的迁移
IF 3.2 3区 工程技术 Q1 NUCLEAR SCIENCE & TECHNOLOGY Pub Date : 2026-03-01 Epub Date: 2026-01-09 DOI: 10.1016/j.pnucene.2025.106214
Ayodeji A. Ala , Lorlornyo Abusah , Shouxu Qiao , Bin Ye , Sichao Tan
Precise prediction of the flow pattern and proper estimation of the void fraction distribution are needed to design and optimize multiphase reactors and bubble columns. This research presents the cross-sectional and averaged void fraction distributions of adiabatic air-water mixtures across square-to-square channel cross-section expansion and contraction, with gas superficial velocity (jg) ranging from 0.003 m/s to 0.0054 m/s and water superficial velocity (jl) from 0.08 m/s to 0.36 m/s. A high-speed imaging system captures the bubble information, while key liquid phase flow features are extracted using the particle image velocimetry technique. Changing jg and jl have different effects on the bubble size distributions. In addition to the slowing flow after the expansion plane, the higher void fraction near the walls before the expansion influences the void fraction distribution in the expansion area. Void fraction distribution in channels with contraction displays a wall and core peaking profile. Conversely, a reduction in the contraction ratio in the channel increases the wall-peaking void fraction compared to the core. The decreasing averaged void fraction across the contraction transitions from linear to polynomial as the contraction in the channel increases. A code was developed to estimate the void fraction distribution before the contraction plane in a square channel, and the output was compared with available data.
在多相反应器和气泡塔的设计和优化中,需要精确的流态预测和合理的空隙率分布估计。研究结果表明,在气表速度(jg)为0.003 ~ 0.0054 m/s,水表速度(jl)为0.08 ~ 0.36 m/s的条件下,绝热空气-水混合物的横截面和平均空隙率分布。高速成像系统捕获气泡信息,同时利用粒子图像测速技术提取关键的液相流动特征。改变jg和jl对气泡尺寸分布有不同的影响。除了膨胀面后流动变缓外,膨胀前壁面附近较高的空隙率影响了膨胀区的空隙率分布。孔隙率在收缩通道中的分布表现为壁面和岩心峰值。相反,与岩心相比,通道中收缩比的减小增加了壁面峰值空隙率。随着通道收缩的增加,收缩过程中减少的平均空隙率从线性转变为多项式。开发了估算方形通道收缩面前空隙率分布的程序,并将输出结果与现有数据进行了比较。
{"title":"Void fraction migration in developing bubbly flow through sudden cross-section contraction and expansion in square channels","authors":"Ayodeji A. Ala ,&nbsp;Lorlornyo Abusah ,&nbsp;Shouxu Qiao ,&nbsp;Bin Ye ,&nbsp;Sichao Tan","doi":"10.1016/j.pnucene.2025.106214","DOIUrl":"10.1016/j.pnucene.2025.106214","url":null,"abstract":"<div><div>Precise prediction of the flow pattern and proper estimation of the void fraction distribution are needed to design and optimize multiphase reactors and bubble columns. This research presents the cross-sectional and averaged void fraction distributions of adiabatic air-water mixtures across square-to-square channel cross-section expansion and contraction, with gas superficial velocity (<em>j</em><sub><em>g</em></sub>) ranging from 0.003 m/s to 0.0054 m/s and water superficial velocity (<em>j</em><sub><em>l</em></sub>) from 0.08 m/s to 0.36 m/s. A high-speed imaging system captures the bubble information, while key liquid phase flow features are extracted using the particle image velocimetry technique. Changing <em>j</em><sub><em>g</em></sub> and <em>j</em><sub><em>l</em></sub> have different effects on the bubble size distributions. In addition to the slowing flow after the expansion plane, the higher void fraction near the walls before the expansion influences the void fraction distribution in the expansion area. Void fraction distribution in channels with contraction displays a wall and core peaking profile. Conversely, a reduction in the contraction ratio in the channel increases the wall-peaking void fraction compared to the core. The decreasing averaged void fraction across the contraction transitions from linear to polynomial as the contraction in the channel increases. A code was developed to estimate the void fraction distribution before the contraction plane in a square channel, and the output was compared with available data.</div></div>","PeriodicalId":20617,"journal":{"name":"Progress in Nuclear Energy","volume":"193 ","pages":"Article 106214"},"PeriodicalIF":3.2,"publicationDate":"2026-03-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145927140","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Data assimilation-based momentum source parameter calibration in subchannel code CUNLUN 基于数据同化的子信道动量源参数标定
IF 3.2 3区 工程技术 Q1 NUCLEAR SCIENCE & TECHNOLOGY Pub Date : 2026-03-01 Epub Date: 2026-01-06 DOI: 10.1016/j.pnucene.2026.106236
Hongwei Jiang , Xian Zhang , Guangliang Chen , Zhaofei Tian , Jinchao Li , Hao Qian , Xinli Yin , Hang Wang
To enhance the accuracy of 3D flow simulations in fuel assembly subchannels, a data assimilation framework (DA-DRM) is proposed by integrating the Ensemble Kalman Filter (EnKF) into the fine-mesh subchannel thermal-hydraulic code CUNLUN. In this framework, DA-DRM serves as the overall data assimilation scheme, while the EnKF functions as the core algorithm to iteratively update model parameters and state variables. This approach dynamically calibrates key momentum source parameters and updates the state variables based on the covariance of simulation–observation residuals, while maintaining physical consistency.As a result, both local adaptability and global consistency of flow predictions are improved.The method is validated against the MATiS-H international thermal-hydraulic benchmark. Multiple observation configurations are designed to systematically assess the impact of sensor placement on optimization performance. Results show that the EnKF-based DA-DRM framework significantly improves the spatial agreement of both axial and lateral velocities across representative cross-sections. In regions with steep velocity gradients downstream of the mixing spacer grid (region Z=0.5Dh), the root mean square error (RMSE) of velocity predictions is reduced from 0.127 to 0.039, corresponding to a 69.6 % reduction.Further convergence analysis reveals that well-designed observation layouts not only enhance prediction accuracy but also accelerate and stabilize the data assimilation process. Simplified configurations yield faster convergence, while more complex setups offer improved robustness. Overall, the proposed framework provides an effective and generalizable strategy for calibrating subchannel models and improving the fidelity of thermal-hydraulic simulations in complex reactor components.
为了提高燃油组件子通道内三维流动模拟的精度,将集成卡尔曼滤波器(Ensemble Kalman Filter, EnKF)集成到细网格子通道热工代码CUNLUN中,提出了一种数据同化框架(DA-DRM)。在该框架中,DA-DRM作为整体数据同化方案,EnKF作为核心算法迭代更新模型参数和状态变量。该方法在保持物理一致性的前提下,根据仿真-观测残差的协方差动态标定关键动量源参数并更新状态变量。从而提高了流量预测的局部适应性和全局一致性。通过MATiS-H国际热工基准测试,验证了该方法的有效性。设计了多个观测配置,以系统地评估传感器放置对优化性能的影响。结果表明,基于enkf的DA-DRM框架显著提高了代表性截面上轴向和横向速度的空间一致性。在混合间隔网格下游速度梯度较大的区域(Z=0.5Dh区域),速度预测的均方根误差(RMSE)从0.127降低到0.039,降低了69.6%。进一步的收敛性分析表明,设计良好的观测布局不仅可以提高预测精度,而且可以加速和稳定数据同化过程。简化的配置产生更快的收敛,而更复杂的设置提供更好的鲁棒性。总的来说,所提出的框架为校准子通道模型和提高复杂反应堆部件热工仿真的保真度提供了一种有效和通用的策略。
{"title":"Data assimilation-based momentum source parameter calibration in subchannel code CUNLUN","authors":"Hongwei Jiang ,&nbsp;Xian Zhang ,&nbsp;Guangliang Chen ,&nbsp;Zhaofei Tian ,&nbsp;Jinchao Li ,&nbsp;Hao Qian ,&nbsp;Xinli Yin ,&nbsp;Hang Wang","doi":"10.1016/j.pnucene.2026.106236","DOIUrl":"10.1016/j.pnucene.2026.106236","url":null,"abstract":"<div><div>To enhance the accuracy of 3D flow simulations in fuel assembly subchannels, a data assimilation framework (DA-DRM) is proposed by integrating the Ensemble Kalman Filter (EnKF) into the fine-mesh subchannel thermal-hydraulic code CUNLUN. In this framework, DA-DRM serves as the overall data assimilation scheme, while the EnKF functions as the core algorithm to iteratively update model parameters and state variables. This approach dynamically calibrates key momentum source parameters and updates the state variables based on the covariance of simulation–observation residuals, while maintaining physical consistency.As a result, both local adaptability and global consistency of flow predictions are improved.The method is validated against the MATiS-H international thermal-hydraulic benchmark. Multiple observation configurations are designed to systematically assess the impact of sensor placement on optimization performance. Results show that the EnKF-based DA-DRM framework significantly improves the spatial agreement of both axial and lateral velocities across representative cross-sections. In regions with steep velocity gradients downstream of the mixing spacer grid (region <span><math><mrow><mi>Z</mi><mo>=</mo><mn>0.5</mn><msub><mi>D</mi><mi>h</mi></msub></mrow></math></span>), the root mean square error (RMSE) of velocity predictions is reduced from 0.127 to 0.039, corresponding to a 69.6 % reduction.Further convergence analysis reveals that well-designed observation layouts not only enhance prediction accuracy but also accelerate and stabilize the data assimilation process. Simplified configurations yield faster convergence, while more complex setups offer improved robustness. Overall, the proposed framework provides an effective and generalizable strategy for calibrating subchannel models and improving the fidelity of thermal-hydraulic simulations in complex reactor components.</div></div>","PeriodicalId":20617,"journal":{"name":"Progress in Nuclear Energy","volume":"193 ","pages":"Article 106236"},"PeriodicalIF":3.2,"publicationDate":"2026-03-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145927138","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Experimental investigation of turbulent flow in a rod bundle with flow blockage 流阻棒束湍流的实验研究
IF 3.2 3区 工程技术 Q1 NUCLEAR SCIENCE & TECHNOLOGY Pub Date : 2026-03-01 Epub Date: 2025-12-31 DOI: 10.1016/j.pnucene.2025.106215
Denggao Chen, Jingliang Bi, Yanping Huang, Dewen Yuan, Yuanfeng Zan, Jianjun Xu
{"title":"Experimental investigation of turbulent flow in a rod bundle with flow blockage","authors":"Denggao Chen,&nbsp;Jingliang Bi,&nbsp;Yanping Huang,&nbsp;Dewen Yuan,&nbsp;Yuanfeng Zan,&nbsp;Jianjun Xu","doi":"10.1016/j.pnucene.2025.106215","DOIUrl":"10.1016/j.pnucene.2025.106215","url":null,"abstract":"","PeriodicalId":20617,"journal":{"name":"Progress in Nuclear Energy","volume":"193 ","pages":"Article 106215"},"PeriodicalIF":3.2,"publicationDate":"2026-03-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145884668","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
A critical review of spent nuclear fuel drying 乏核燃料干燥技术综述
IF 3.2 3区 工程技术 Q1 NUCLEAR SCIENCE & TECHNOLOGY Pub Date : 2026-03-01 Epub Date: 2025-12-22 DOI: 10.1016/j.pnucene.2025.106196
Ji Hwan Lim
This review critically examines advanced methodologies for drying spent nuclear fuel (SNF), emphasizing the optimization of vacuum drying strategies and the role of forced helium drying (FHD). SNF drying is vital for safe storage and prevents issues like moisture-induced corrosion and hydrogen radiolysis. Traditional vacuum drying remains a staple, yet challenges like ice formation and ineffective moisture removal in damaged fuel necessitate innovations like FHD, which ensures thorough moisture elimination through active gas circulation. Empirical studies and enhanced simulations have refined understanding, showing automation and real-time moisture sensors could streamline drying, improve safety, and reduce time. Also, developments in hydride reorientation in zirconium cladding due to high temperatures during drying highlight the need for precise thermal management to prevent cladding embrittlement. Recent research emphasizes tailored drying criteria for diverse fuel types, focusing on damage-prone fuel requiring extended, heat-assisted drying strategies or supportive agents like hydrogen getters to mitigate gas build-up risks. Monitoring technologies are advancing to include dew point sensors and acoustic devices for real-time drying assessment. Thus, while vacuum methods are robust, an international collaborative effort is essential to standardize best practices for complex scenarios involving high-burnup and damaged SNF, ensuring fuel integrity and regulatory compliance across the nuclear industry.
本文综述了干燥乏核燃料(SNF)的先进方法,强调了真空干燥策略的优化和强制氦干燥(FHD)的作用。SNF干燥对于安全储存至关重要,可以防止湿气腐蚀和氢辐射分解等问题。传统的真空干燥仍然是主要的,但挑战,如冰的形成和无效的水分去除损坏的燃料需要创新,如FHD,确保通过主动气体循环彻底消除水分。经验研究和增强的模拟加深了人们的理解,表明自动化和实时湿度传感器可以简化干燥,提高安全性并缩短时间。此外,由于干燥过程中的高温,锆包层中氢化物重定向的发展突出了精确热管理以防止包层脆化的必要性。最近的研究强调了针对不同燃料类型量身定制的干燥标准,重点是需要扩展的热辅助干燥策略或氢吸收剂等辅助剂来减轻气体积聚风险的易损坏燃料。监测技术正在发展,包括露点传感器和用于实时干燥评估的声学设备。因此,尽管真空方法是强大的,但对于涉及高燃耗和SNF损坏的复杂场景的最佳实践标准化,确保整个核工业的燃料完整性和法规遵从性,国际合作的努力是必不可少的。
{"title":"A critical review of spent nuclear fuel drying","authors":"Ji Hwan Lim","doi":"10.1016/j.pnucene.2025.106196","DOIUrl":"10.1016/j.pnucene.2025.106196","url":null,"abstract":"<div><div>This review critically examines advanced methodologies for drying spent nuclear fuel (SNF), emphasizing the optimization of vacuum drying strategies and the role of forced helium drying (FHD). SNF drying is vital for safe storage and prevents issues like moisture-induced corrosion and hydrogen radiolysis. Traditional vacuum drying remains a staple, yet challenges like ice formation and ineffective moisture removal in damaged fuel necessitate innovations like FHD, which ensures thorough moisture elimination through active gas circulation. Empirical studies and enhanced simulations have refined understanding, showing automation and real-time moisture sensors could streamline drying, improve safety, and reduce time. Also, developments in hydride reorientation in zirconium cladding due to high temperatures during drying highlight the need for precise thermal management to prevent cladding embrittlement. Recent research emphasizes tailored drying criteria for diverse fuel types, focusing on damage-prone fuel requiring extended, heat-assisted drying strategies or supportive agents like hydrogen getters to mitigate gas build-up risks. Monitoring technologies are advancing to include dew point sensors and acoustic devices for real-time drying assessment. Thus, while vacuum methods are robust, an international collaborative effort is essential to standardize best practices for complex scenarios involving high-burnup and damaged SNF, ensuring fuel integrity and regulatory compliance across the nuclear industry.</div></div>","PeriodicalId":20617,"journal":{"name":"Progress in Nuclear Energy","volume":"193 ","pages":"Article 106196"},"PeriodicalIF":3.2,"publicationDate":"2026-03-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145841096","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
期刊
Progress in Nuclear Energy
全部 Acc. Chem. Res. ACS Applied Bio Materials ACS Appl. Electron. Mater. ACS Appl. Energy Mater. ACS Appl. Mater. Interfaces ACS Appl. Nano Mater. ACS Appl. Polym. Mater. ACS BIOMATER-SCI ENG ACS Catal. ACS Cent. Sci. ACS Chem. Biol. ACS Chemical Health & Safety ACS Chem. Neurosci. ACS Comb. Sci. ACS Earth Space Chem. ACS Energy Lett. ACS Infect. Dis. ACS Macro Lett. ACS Mater. Lett. ACS Med. Chem. Lett. ACS Nano ACS Omega ACS Photonics ACS Sens. ACS Sustainable Chem. Eng. ACS Synth. Biol. Anal. Chem. BIOCHEMISTRY-US Bioconjugate Chem. BIOMACROMOLECULES Chem. Res. Toxicol. Chem. Rev. Chem. Mater. CRYST GROWTH DES ENERG FUEL Environ. Sci. Technol. Environ. Sci. Technol. Lett. Eur. J. Inorg. Chem. IND ENG CHEM RES Inorg. Chem. J. Agric. Food. Chem. J. Chem. Eng. Data J. Chem. Educ. J. Chem. Inf. Model. J. Chem. Theory Comput. J. Med. Chem. J. Nat. Prod. J PROTEOME RES J. Am. Chem. Soc. LANGMUIR MACROMOLECULES Mol. Pharmaceutics Nano Lett. Org. Lett. ORG PROCESS RES DEV ORGANOMETALLICS J. Org. Chem. J. Phys. Chem. J. Phys. Chem. A J. Phys. Chem. B J. Phys. Chem. C J. Phys. Chem. Lett. Analyst Anal. Methods Biomater. Sci. Catal. Sci. Technol. Chem. Commun. Chem. Soc. Rev. CHEM EDUC RES PRACT CRYSTENGCOMM Dalton Trans. Energy Environ. Sci. ENVIRON SCI-NANO ENVIRON SCI-PROC IMP ENVIRON SCI-WAT RES Faraday Discuss. Food Funct. Green Chem. Inorg. Chem. Front. Integr. Biol. J. Anal. At. Spectrom. J. Mater. Chem. A J. Mater. Chem. B J. Mater. Chem. C Lab Chip Mater. Chem. Front. Mater. Horiz. MEDCHEMCOMM Metallomics Mol. Biosyst. Mol. Syst. Des. Eng. Nanoscale Nanoscale Horiz. Nat. Prod. Rep. New J. Chem. Org. Biomol. Chem. Org. Chem. Front. PHOTOCH PHOTOBIO SCI PCCP Polym. Chem.
×
引用
GB/T 7714-2015
复制
MLA
复制
APA
复制
导出至
BibTeX EndNote RefMan NoteFirst NoteExpress
×
0
微信
客服QQ
Book学术公众号 扫码关注我们
反馈
×
意见反馈
请填写您的意见或建议
请填写您的手机或邮箱
×
提示
您的信息不完整,为了账户安全,请先补充。
现在去补充
×
提示
您因"违规操作"
具体请查看互助需知
我知道了
×
提示
现在去查看 取消
×
提示
确定
Book学术官方微信
Book学术文献互助
Book学术文献互助群
群 号:604180095
Book学术
文献互助 智能选刊 最新文献 互助须知 联系我们:info@booksci.cn
Book学术提供免费学术资源搜索服务,方便国内外学者检索中英文文献。致力于提供最便捷和优质的服务体验。
Copyright © 2023 Book学术 All rights reserved.
ghs 京公网安备 11010802042870号 京ICP备2023020795号-1