首页 > 最新文献

Science and Technology of Nuclear Installations最新文献

英文 中文
Multiple Assessments on the Gamma-Ray Protection Properties of Niobium-Doped Borotellurite Glasses: A Wide Range Investigation Using Monte Carlo Simulations 掺铌硼碲化物玻璃伽马射线防护性能的多重评估:蒙特卡罗模拟的宽范围研究
IF 1.1 4区 工程技术 Q3 Energy Pub Date : 2022-03-18 DOI: 10.1155/2022/5890896
H. Tekin, Fatema T. Ali, G. Almisned, G. Susoy, S. Issa, A. Ene, W. Elshami, H. Zakaly
In this study, the monotonic effect of Ta2O5 and ZrO2 in some selected borotellurite glasses was investigated in terms of their impact on gamma-ray-shielding competencies. Accordingly, three niobium-reinforced borotellurite glasses (S1 : 75TeO2 + 15B2O3 + 10Nb2O5, S2 : 75TeO2 + 15B2O3 + 9Nb2O5 + 1Ta2O5, and S3 : 75TeO2 + 15B2O3 + 8Nb2O5 + 1Ta2O5 + 1ZrO2) were modelled in the general-purpose MCNPX Monte Carlo code. They have been defined as an attenuator sample between the point isotropic gamma-ray source and the detector in terms of determining their attenuation coefficients. To verify the MC results, attenuation coefficients were then compared with the Phy-X/PSD program data. Our findings clearly demonstrate that although some behavioral changes occurred in the shielding qualities, modest improvements occurred in the attenuation properties depending on the modifier variation and its magnitude. However, the replacement of 2% moles of Nb2O5 with 1% mole of Ta2O5 and 1% mole of ZrO2 provided significant improvements in both glass density and attenuation properties against gamma rays. Finally, the HVL values of the S3 sample were compared with some glass- and concrete-shielding materials and the S3 sample was reported for its outstanding properties. As a consequence of this investigation, it can be concluded that the indicated type of additive to be added to borotellurite glasses will provide some advantages, particularly when used in radiation fields, by increasing the shielding qualities moderately.
在本研究中,研究了Ta2O5和ZrO2在一些选定的硼碲化物玻璃中对伽马射线屏蔽能力的影响。因此,三种铌增强的碲化硼玻璃(S1 : 75TeO2 + 15B2O3 + 10Nb2O5,S2 : 75TeO2 + 15B2O3 + 9Nb2O5 + 1Ta2O5和S3 : 75TeO2 + 15B2O3 + 8Nb2O5 + 1Ta2O5 + 1ZrO2)在通用MCNPX蒙特卡罗程序中建模。就确定其衰减系数而言,它们被定义为点各向同性伽马射线源和探测器之间的衰减器样本。为了验证MC结果,然后将衰减系数与Phy-X/PSD程序数据进行比较。我们的研究结果清楚地表明,尽管屏蔽质量发生了一些行为变化,但根据改性剂的变化及其幅度,衰减性能略有改善。然而,用1%摩尔的Ta2O5和1%摩尔的ZrO2代替2%摩尔的Nb2O5在玻璃密度和对伽马射线的衰减性能方面提供了显著的改进。最后,将S3样品的HVL值与一些玻璃和混凝土屏蔽材料进行了比较,并报道了S3样品的优异性能。作为这项研究的结果,可以得出结论,要添加到碲化硼玻璃中的指定类型的添加剂将提供一些优势,特别是当在辐射场中使用时,通过适度地提高屏蔽质量。
{"title":"Multiple Assessments on the Gamma-Ray Protection Properties of Niobium-Doped Borotellurite Glasses: A Wide Range Investigation Using Monte Carlo Simulations","authors":"H. Tekin, Fatema T. Ali, G. Almisned, G. Susoy, S. Issa, A. Ene, W. Elshami, H. Zakaly","doi":"10.1155/2022/5890896","DOIUrl":"https://doi.org/10.1155/2022/5890896","url":null,"abstract":"In this study, the monotonic effect of Ta2O5 and ZrO2 in some selected borotellurite glasses was investigated in terms of their impact on gamma-ray-shielding competencies. Accordingly, three niobium-reinforced borotellurite glasses (S1 : 75TeO2 + 15B2O3 + 10Nb2O5, S2 : 75TeO2 + 15B2O3 + 9Nb2O5 + 1Ta2O5, and S3 : 75TeO2 + 15B2O3 + 8Nb2O5 + 1Ta2O5 + 1ZrO2) were modelled in the general-purpose MCNPX Monte Carlo code. They have been defined as an attenuator sample between the point isotropic gamma-ray source and the detector in terms of determining their attenuation coefficients. To verify the MC results, attenuation coefficients were then compared with the Phy-X/PSD program data. Our findings clearly demonstrate that although some behavioral changes occurred in the shielding qualities, modest improvements occurred in the attenuation properties depending on the modifier variation and its magnitude. However, the replacement of 2% moles of Nb2O5 with 1% mole of Ta2O5 and 1% mole of ZrO2 provided significant improvements in both glass density and attenuation properties against gamma rays. Finally, the HVL values of the S3 sample were compared with some glass- and concrete-shielding materials and the S3 sample was reported for its outstanding properties. As a consequence of this investigation, it can be concluded that the indicated type of additive to be added to borotellurite glasses will provide some advantages, particularly when used in radiation fields, by increasing the shielding qualities moderately.","PeriodicalId":21629,"journal":{"name":"Science and Technology of Nuclear Installations","volume":null,"pages":null},"PeriodicalIF":1.1,"publicationDate":"2022-03-18","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"44100267","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 5
Experimental Research for CHF Sensitivity of Heat Flux Distribution under IVR Conditions IVR条件下热流分布对CHF敏感性的实验研究
IF 1.1 4区 工程技术 Q3 Energy Pub Date : 2022-03-16 DOI: 10.1155/2022/3522470
Shilei Han, Pengfei Liu, B. Kuang, Yanhua Yang
In-vessel retention (IVR) through external reactor vessel cooling (ERVC) is one of the most effective severe accident mitigation measures in the nuclear power plants. The most influential issues on the IVR strategy are in-vessel core melt evolution, the heat fluxes imposed on the lower head, and the external cooling of reactor pressurized vessel (RPV). In the molten pool research, there are mainly two different molten pool configurations: two layers and three layers. Based on the different distributions of heat flux in molten pool configurations, a new problem was raised: whether the in-vessel heat flux distribution will affect the CHF on the outer wall of RPV and further affect the effectiveness of IVR measures? A full-height external reactor vessel cooling and natural circulating facility was conducted to study the CHF sensitivity of different heat flux distributions. The experimental results show that the characteristics of natural circulation are similar and the CHF of the RPV lower head external surface is not obviously affected under the different heat flux distributions. The varying heat flux distribution during severe accident process will not threaten significantly the success of IVR strategy.
通过反应堆容器外部冷却进行容器内滞留(IVR)是核电站中最有效的严重事故缓解措施之一。IVR策略中最具影响力的问题是容器内堆芯熔体的演变、施加在下封头上的热通量以及反应堆压力容器(RPV)的外部冷却。在熔池研究中,主要有两种不同的熔池结构:两层和三层。基于熔池结构中热通量的不同分布,提出了一个新的问题:容器内热通量的分布是否会影响RPV外壁上的CHF,并进一步影响IVR措施的有效性?采用全高堆外冷却和自然循环装置研究了不同热通量分布对CHF的敏感性。实验结果表明,在不同的热通量分布下,RPV下封头外表面的自然循环特性相似,CHF不受明显影响。严重事故过程中热通量分布的变化不会对IVR策略的成功产生重大威胁。
{"title":"Experimental Research for CHF Sensitivity of Heat Flux Distribution under IVR Conditions","authors":"Shilei Han, Pengfei Liu, B. Kuang, Yanhua Yang","doi":"10.1155/2022/3522470","DOIUrl":"https://doi.org/10.1155/2022/3522470","url":null,"abstract":"In-vessel retention (IVR) through external reactor vessel cooling (ERVC) is one of the most effective severe accident mitigation measures in the nuclear power plants. The most influential issues on the IVR strategy are in-vessel core melt evolution, the heat fluxes imposed on the lower head, and the external cooling of reactor pressurized vessel (RPV). In the molten pool research, there are mainly two different molten pool configurations: two layers and three layers. Based on the different distributions of heat flux in molten pool configurations, a new problem was raised: whether the in-vessel heat flux distribution will affect the CHF on the outer wall of RPV and further affect the effectiveness of IVR measures? A full-height external reactor vessel cooling and natural circulating facility was conducted to study the CHF sensitivity of different heat flux distributions. The experimental results show that the characteristics of natural circulation are similar and the CHF of the RPV lower head external surface is not obviously affected under the different heat flux distributions. The varying heat flux distribution during severe accident process will not threaten significantly the success of IVR strategy.","PeriodicalId":21629,"journal":{"name":"Science and Technology of Nuclear Installations","volume":null,"pages":null},"PeriodicalIF":1.1,"publicationDate":"2022-03-16","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"41295859","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 2
Verification of the Efficacy of Passive Autocatalytic Recombiners in a Typical Pressurized Water Reactor under a Station Blackout Condition 电站停电条件下典型压水反应堆中非能动自催化复合器的有效性验证
IF 1.1 4区 工程技术 Q3 Energy Pub Date : 2022-03-12 DOI: 10.1155/2022/7129092
Dae-Hwa Hong, D. Cho, Jinwoo Kim, A. Diab, Cigdem Cildag
The presence of a stable stratified gas cloud inside the containment near or at the flammability limit may lead to deflagration or even detonation which may challenge the containment and cause a radioactive material release into the environment. To mitigate this risk, a number of approaches have been proposed, for example, containment inerting or venting and use of passive autocatalytic recombiners or igniters. However, for these measures to be effective, a thorough analysis of the hydrogen dispersion and associated phenomena is indispensable during the design phase as well as the mitigation phase during a severe accident. In this work, a MAAP analysis is performed to assess the hydrogen risk in a typical pressurized water reactor (PWR) containment. An extended station blackout (SBO) was chosen as an initiating event given its high contribution to the core damage frequency. RCS depressurization and external injection are mitigation techniques implemented consecutively to extend the coping capability of the plant for the extended SBO scenario. A sensitivity study is performed to select the combination of timing and flow rate that generate the most severe case for the “in-vessel phase of hydrogen generation.” Subsequently, a number of passive autocatalytic recombiners (PARs) were implemented to mitigate the hydrogen risk during the first three days of the accident. The Shapiro diagram is used to assess the flammability condition of the containment atmosphere based on MAAP analysis. The results show that the gas mixture composition is acceptable in the majority of the containment compartments and only marginally acceptable in the cavity. Even under the conservative conditions of the accident, the simulation results confirmed the sufficiency of recombiners alone without igniters in the low hydrogen concentration zones, while for compartments close to the sources, additional mitigation may be needed.
安全壳内接近或处于可燃极限的稳定分层气体云可能导致爆燃甚至爆炸,这可能会挑战安全壳并导致放射性物质释放到环境中。为了减轻这种风险,已经提出了许多方法,例如,安全壳惰性化或排气以及使用被动自催化复合器或点火器。然而,为了使这些措施有效,在设计阶段以及严重事故期间的缓解阶段,对氢气扩散和相关现象进行彻底分析是必不可少的。在这项工作中,进行了MAAP分析,以评估典型压水堆(PWR)安全壳中的氢气风险。考虑到延长电站停电(SBO)对堆芯损坏频率的贡献很大,因此选择其作为启动事件。RCS降压和外部注入是连续实施的缓解技术,以扩展核电站在扩展SBO场景下的应对能力。进行了敏感性研究,以选择产生“容器内制氢阶段”最严重情况的时间和流速组合。随后,在事故发生的前三天,实施了一些非能动自催化复合器(PAR),以降低氢气风险。夏皮罗图用于基于MAAP分析评估安全壳大气的可燃性条件。结果表明,气体混合物成分在大多数安全壳隔间中是可接受的,而在空腔中只是勉强可接受的。即使在事故的保守条件下,模拟结果也证实了在低氢浓度区单独使用复合器而不使用点火器的充分性,而对于靠近源的隔间,可能需要额外的缓解措施。
{"title":"Verification of the Efficacy of Passive Autocatalytic Recombiners in a Typical Pressurized Water Reactor under a Station Blackout Condition","authors":"Dae-Hwa Hong, D. Cho, Jinwoo Kim, A. Diab, Cigdem Cildag","doi":"10.1155/2022/7129092","DOIUrl":"https://doi.org/10.1155/2022/7129092","url":null,"abstract":"The presence of a stable stratified gas cloud inside the containment near or at the flammability limit may lead to deflagration or even detonation which may challenge the containment and cause a radioactive material release into the environment. To mitigate this risk, a number of approaches have been proposed, for example, containment inerting or venting and use of passive autocatalytic recombiners or igniters. However, for these measures to be effective, a thorough analysis of the hydrogen dispersion and associated phenomena is indispensable during the design phase as well as the mitigation phase during a severe accident. In this work, a MAAP analysis is performed to assess the hydrogen risk in a typical pressurized water reactor (PWR) containment. An extended station blackout (SBO) was chosen as an initiating event given its high contribution to the core damage frequency. RCS depressurization and external injection are mitigation techniques implemented consecutively to extend the coping capability of the plant for the extended SBO scenario. A sensitivity study is performed to select the combination of timing and flow rate that generate the most severe case for the “in-vessel phase of hydrogen generation.” Subsequently, a number of passive autocatalytic recombiners (PARs) were implemented to mitigate the hydrogen risk during the first three days of the accident. The Shapiro diagram is used to assess the flammability condition of the containment atmosphere based on MAAP analysis. The results show that the gas mixture composition is acceptable in the majority of the containment compartments and only marginally acceptable in the cavity. Even under the conservative conditions of the accident, the simulation results confirmed the sufficiency of recombiners alone without igniters in the low hydrogen concentration zones, while for compartments close to the sources, additional mitigation may be needed.","PeriodicalId":21629,"journal":{"name":"Science and Technology of Nuclear Installations","volume":null,"pages":null},"PeriodicalIF":1.1,"publicationDate":"2022-03-12","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"42403020","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Research on Channel Modeling and Communication Coverage of Wireless Sensor Networks in Barrier Area of Nuclear Power Plants 核电站屏障区无线传感器网络信道建模与通信覆盖研究
IF 1.1 4区 工程技术 Q3 Energy Pub Date : 2022-03-07 DOI: 10.1155/2022/5223755
Zhiguang Deng, Qian Wu, Xin Lv, Bi-Wei Zhu, M. Xiang, Xue-Mei Wang, Jia-Liang Zhu
In view of the multimetal barrier environment of nuclear power plant, by considering the factors such as transmission power, transmission position, and multipath interference, based on the simulation of metal pipes and equipment, this paper carries out the barrier area channel modeling in logarithmic fading mode and makes quantitative analysis on the channel transmission, path loss, channel power characteristics, and so on under the metal barrier environment. Based on the channel modeling, this paper optimizes the coverage of the network in the obstacle area by using the improved teaching and learning group intelligent algorithm. The simulation results show that the improved teaching and learning algorithm can optimize the network coverage of the obstacle area well, and under the four obstacle modules, 14 nodes can cover the whole area by more than 99%. This provides a solution to the problem of network coverage in the practical application of wireless sensor networks.
针对核电站多金属屏障环境,在对金属管道和设备进行仿真的基础上,考虑传输功率、传输位置、多径干扰等因素,进行对数衰落模式下的屏障区域信道建模,定量分析了金属屏障环境下的信道传输、路径损耗、信道功率特性等。在信道建模的基础上,采用改进的教与学群智能算法对网络在障碍物区域的覆盖进行优化。仿真结果表明,改进的教与学算法可以很好地优化网络对障碍物区域的覆盖,在4个障碍物模块下,14个节点对整个区域的覆盖达到99%以上。这为无线传感器网络实际应用中的网络覆盖问题提供了一种解决方案。
{"title":"Research on Channel Modeling and Communication Coverage of Wireless Sensor Networks in Barrier Area of Nuclear Power Plants","authors":"Zhiguang Deng, Qian Wu, Xin Lv, Bi-Wei Zhu, M. Xiang, Xue-Mei Wang, Jia-Liang Zhu","doi":"10.1155/2022/5223755","DOIUrl":"https://doi.org/10.1155/2022/5223755","url":null,"abstract":"In view of the multimetal barrier environment of nuclear power plant, by considering the factors such as transmission power, transmission position, and multipath interference, based on the simulation of metal pipes and equipment, this paper carries out the barrier area channel modeling in logarithmic fading mode and makes quantitative analysis on the channel transmission, path loss, channel power characteristics, and so on under the metal barrier environment. Based on the channel modeling, this paper optimizes the coverage of the network in the obstacle area by using the improved teaching and learning group intelligent algorithm. The simulation results show that the improved teaching and learning algorithm can optimize the network coverage of the obstacle area well, and under the four obstacle modules, 14 nodes can cover the whole area by more than 99%. This provides a solution to the problem of network coverage in the practical application of wireless sensor networks.","PeriodicalId":21629,"journal":{"name":"Science and Technology of Nuclear Installations","volume":null,"pages":null},"PeriodicalIF":1.1,"publicationDate":"2022-03-07","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"47236389","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Interaction of Mechanical Heterogeneity and Residual Stress on Mechanical Field at Crack Tips in DMWJs DMWJs裂纹尖端力学场中力学不均匀性与残余应力的相互作用
IF 1.1 4区 工程技术 Q3 Energy Pub Date : 2022-02-26 DOI: 10.1155/2022/7462200
Yubiao Zhang, H. Xue, Shun Zhang, Shuai Wang, Yuman Sun, Yonggang Zhang, Yongjie Yang
The interaction between the mechanical heterogeneity and the residual stress in dissimilar metal welded joints (DMWJs) leads to a complex mechanical field of crack tips, which strongly affects stress corrosion cracking (SCC) behaviors. A dual-field coupling model was established by using the user-defined field (USDFLD) and the predefined stress field method based on the elastoplastic finite element method in this study. Thus, the mechanical heterogeneity and the residual stress of the DMWJ are realized. The influence of the interaction between the mechanical heterogeneity and the residual stress on the mechanical field of crack tips at different locations was investigated. The results show that the mechanical heterogeneity causes the stress and strain distribution on both sides of the crack tip asymmetry. And the residual stress affects the magnitude of the stress and strain around the crack tip. The variation trend of the stress and strain along the crack propagation with crack length is basically the same as that of the residual stress. However, the stress and strain distributions are slightly lagging behind the residual stress distribution due to the redistribution of the residual stress caused by the crack propagation. In addition, the stress and strain range of cracks at different positions with crack length are also different.
异种金属焊接接头的力学非均质性与残余应力的相互作用导致裂纹尖端形成复杂的力学场,对应力腐蚀开裂(SCC)行为产生强烈影响。本研究基于弹塑性有限元法,采用自定义场(USDFLD)和预定义应力场方法建立了双场耦合模型。从而实现了DMWJ的力学非均质性和残余应力。研究了不同位置裂纹尖端的力学非均质性和残余应力相互作用对裂纹尖端力学场的影响。结果表明:力学非均质性导致裂纹尖端两侧应力应变分布不对称;残余应力影响裂纹尖端周围的应力和应变大小。应力和应变随裂纹扩展的变化趋势与残余应力的变化趋势基本一致。然而,由于裂纹扩展引起残余应力的重新分布,应力应变分布略落后于残余应力分布。此外,随着裂纹长度的变化,不同位置裂纹的应力应变范围也不同。
{"title":"Interaction of Mechanical Heterogeneity and Residual Stress on Mechanical Field at Crack Tips in DMWJs","authors":"Yubiao Zhang, H. Xue, Shun Zhang, Shuai Wang, Yuman Sun, Yonggang Zhang, Yongjie Yang","doi":"10.1155/2022/7462200","DOIUrl":"https://doi.org/10.1155/2022/7462200","url":null,"abstract":"The interaction between the mechanical heterogeneity and the residual stress in dissimilar metal welded joints (DMWJs) leads to a complex mechanical field of crack tips, which strongly affects stress corrosion cracking (SCC) behaviors. A dual-field coupling model was established by using the user-defined field (USDFLD) and the predefined stress field method based on the elastoplastic finite element method in this study. Thus, the mechanical heterogeneity and the residual stress of the DMWJ are realized. The influence of the interaction between the mechanical heterogeneity and the residual stress on the mechanical field of crack tips at different locations was investigated. The results show that the mechanical heterogeneity causes the stress and strain distribution on both sides of the crack tip asymmetry. And the residual stress affects the magnitude of the stress and strain around the crack tip. The variation trend of the stress and strain along the crack propagation with crack length is basically the same as that of the residual stress. However, the stress and strain distributions are slightly lagging behind the residual stress distribution due to the redistribution of the residual stress caused by the crack propagation. In addition, the stress and strain range of cracks at different positions with crack length are also different.","PeriodicalId":21629,"journal":{"name":"Science and Technology of Nuclear Installations","volume":null,"pages":null},"PeriodicalIF":1.1,"publicationDate":"2022-02-26","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"42490934","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 2
Rapid Determination of Gross Alpha/Beta Activity in Water Based on Reverse Osmosis Membrane Enrichment Pretreatment 基于反渗透膜富集预处理的水中总α / β活性快速测定
IF 1.1 4区 工程技术 Q3 Energy Pub Date : 2022-02-15 DOI: 10.1155/2022/2868792
Ruiqi Zhang, Jianye Wang, Nanjing Zhao, Xuyun Huang
Radioactivity of gross alpha/beta is an index of water quality detection, which can reflect the radioactivity intensity of water. However, the traditional detection method of these parameters, thick source method, has problems of cumbersome and time consumption in sample preparation and cannot realize the rapid detection on-site. Based on this, this paper studies the enrichment method based on reverse osmosis membrane to accurately and quickly determine the gross α and gross β in water by using the reverse osmosis membrane as the carrier and enriching the radionuclides in water to the high-pressure side of the reverse osmosis membrane to replace the sample preparation process in traditional thick source method, so as to shorten the sample processing time in the detection process and avoid the cumbersome sample preparation process. The reverse osmosis membrane enrichment method for the determination of gross in 241Am and 40KCl standard solutions was used to study gross alpha/beta radioactivity, and the results showed that the average recoveries of radioactivity of gross alpha/beta were 95.0% and 93.6%, respectively. At the same time, the results of the thick source method and the reverse osmosis membrane method on the gross alpha/beta of actual water samples in 5 different regions were compared. It showed that the thick source method and the reverse osmosis membrane method had a good consistency in the detection results of total α and total β radioactivity, and the reverse osmosis membrane method had better stability than the thick source method. The average relative standard deviations (RSD) of the gross alpha and gross beta activity obtained by the thick source method are 11.9% and 7.3%, respectively, while RSD of the gross alpha and gross beta radioactivity obtained by the reverse osmosis membrane method were 6.9% and 4.7%, respectively. The preparation time of single sample was reduced by 75.7%, and the overall detection cycle time was reduced by 68.1%.
总α / β放射性是水质检测的一项指标,能反映水体的放射性强度。但传统的粗源法检测这些参数存在制样繁琐、耗时等问题,无法实现现场快速检测。基于此,本文研究了基于反渗透膜的富集方法,以反渗透膜为载体,将水中的放射性核素富集到反渗透膜的高压侧,以替代传统厚源法的制样过程,准确、快速地测定水中的总α和总β。从而缩短检测过程中的样品处理时间,避免繁琐的样品制备过程。采用反渗透膜富集法测定gross在241Am和40KCl标准溶液中的α / β放射性,结果表明,gross α / β的平均放射性回收率分别为95.0%和93.6%。同时,比较了厚源法和反渗透膜法对5个不同地区实际水样的总α / β值的影响。结果表明,厚源法和反渗透膜法对总α和总β放射性的检测结果具有较好的一致性,且反渗透膜法比厚源法具有更好的稳定性。厚源法得到的总α和总β活性的平均相对标准偏差(RSD)分别为11.9%和7.3%,而反渗透膜法得到的总α和总β放射性的平均相对标准偏差(RSD)分别为6.9%和4.7%。单样品制备时间缩短75.7%,总检测周期缩短68.1%。
{"title":"Rapid Determination of Gross Alpha/Beta Activity in Water Based on Reverse Osmosis Membrane Enrichment Pretreatment","authors":"Ruiqi Zhang, Jianye Wang, Nanjing Zhao, Xuyun Huang","doi":"10.1155/2022/2868792","DOIUrl":"https://doi.org/10.1155/2022/2868792","url":null,"abstract":"Radioactivity of gross alpha/beta is an index of water quality detection, which can reflect the radioactivity intensity of water. However, the traditional detection method of these parameters, thick source method, has problems of cumbersome and time consumption in sample preparation and cannot realize the rapid detection on-site. Based on this, this paper studies the enrichment method based on reverse osmosis membrane to accurately and quickly determine the gross <i>α</i> and gross <i>β</i> in water by using the reverse osmosis membrane as the carrier and enriching the radionuclides in water to the high-pressure side of the reverse osmosis membrane to replace the sample preparation process in traditional thick source method, so as to shorten the sample processing time in the detection process and avoid the cumbersome sample preparation process. The reverse osmosis membrane enrichment method for the determination of gross in <sup>241</sup>Am and <sup>40</sup>KCl standard solutions was used to study gross alpha/beta radioactivity, and the results showed that the average recoveries of radioactivity of gross alpha/beta were 95.0% and 93.6%, respectively. At the same time, the results of the thick source method and the reverse osmosis membrane method on the gross alpha/beta of actual water samples in 5 different regions were compared. It showed that the thick source method and the reverse osmosis membrane method had a good consistency in the detection results of total <i>α</i> and total <i>β</i> radioactivity, and the reverse osmosis membrane method had better stability than the thick source method. The average relative standard deviations (RSD) of the gross alpha and gross beta activity obtained by the thick source method are 11.9% and 7.3%, respectively, while RSD of the gross alpha and gross beta radioactivity obtained by the reverse osmosis membrane method were 6.9% and 4.7%, respectively. The preparation time of single sample was reduced by 75.7%, and the overall detection cycle time was reduced by 68.1%.","PeriodicalId":21629,"journal":{"name":"Science and Technology of Nuclear Installations","volume":null,"pages":null},"PeriodicalIF":1.1,"publicationDate":"2022-02-15","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"138513441","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Study on Missing Data Filling Algorithm of Nuclear Power Plant Operation Parameters 核电站运行参数缺失数据填充算法研究
IF 1.1 4区 工程技术 Q3 Energy Pub Date : 2022-02-04 DOI: 10.1155/2022/4172622
Tianshu Wang, Ren Yu, Qiao Peng
By analyzing the recorded operation data of a nuclear power plant (NPP), its results can serve the fault detection or operation experience feedback. Data missing exists in the recorded operation data. It may lower the data quality and affect the accuracy of the analysis results. In order to improve the data quality, two parts of researches are carried on. Firstly, to locate the missing data accurately the detecting algorithm for missing data of the NPP operation parameters based on wavelet analysis. Different judging basis is proposed for discrete and continuous missing respectively. Then, the filling method based on the hot deck algorithm are studied. As the dynamic properties of the parameters are closely related to the operating state of NPP, the similarity of the operation parameter vectors are formed to express the similarity of the operating states, so as to fulfill the requirements of the hot deck algorithm. To improve the accuracy of the measuring results, taken the differences between the characteristics of the analog parameters and the switch parameters into consideration, the similarity measurements using Mahalanobis distance for the analog parameter vectors and the matching measure for the switch parameter vectors are studied respectively. Finally, the operation data is taken to build the experiment data set for the algorithm verification. The results shows that the designed algorithm performs much better than the mean interpolation method and LSTM.
通过对核电站运行记录数据的分析,其结果可以为故障检测或运行经验反馈服务。记录的操作数据中存在丢失的数据。它可能会降低数据质量并影响分析结果的准确性。为了提高数据质量,本文进行了两部分研究:一是基于小波分析的核电站运行参数缺失数据检测算法,以准确定位缺失数据。分别对离散缺失和连续缺失提出了不同的判断依据。然后,研究了基于热甲板算法的填充方法。由于参数的动态特性与核电厂的运行状态密切相关,因此形成运行参数向量的相似性来表达运行状态的相似性,以满足热甲板算法的要求。为了提高测量结果的准确性,考虑到模拟参数和开关参数特性之间的差异,分别研究了模拟参数向量的马氏距离和开关参数向量的匹配测度的相似性测量。最后,利用运算数据建立实验数据集,对算法进行验证。结果表明,所设计的算法比均值插值法和LSTM算法性能要好得多。
{"title":"Study on Missing Data Filling Algorithm of Nuclear Power Plant Operation Parameters","authors":"Tianshu Wang, Ren Yu, Qiao Peng","doi":"10.1155/2022/4172622","DOIUrl":"https://doi.org/10.1155/2022/4172622","url":null,"abstract":"By analyzing the recorded operation data of a nuclear power plant (NPP), its results can serve the fault detection or operation experience feedback. Data missing exists in the recorded operation data. It may lower the data quality and affect the accuracy of the analysis results. In order to improve the data quality, two parts of researches are carried on. Firstly, to locate the missing data accurately the detecting algorithm for missing data of the NPP operation parameters based on wavelet analysis. Different judging basis is proposed for discrete and continuous missing respectively. Then, the filling method based on the hot deck algorithm are studied. As the dynamic properties of the parameters are closely related to the operating state of NPP, the similarity of the operation parameter vectors are formed to express the similarity of the operating states, so as to fulfill the requirements of the hot deck algorithm. To improve the accuracy of the measuring results, taken the differences between the characteristics of the analog parameters and the switch parameters into consideration, the similarity measurements using Mahalanobis distance for the analog parameter vectors and the matching measure for the switch parameter vectors are studied respectively. Finally, the operation data is taken to build the experiment data set for the algorithm verification. The results shows that the designed algorithm performs much better than the mean interpolation method and LSTM.","PeriodicalId":21629,"journal":{"name":"Science and Technology of Nuclear Installations","volume":null,"pages":null},"PeriodicalIF":1.1,"publicationDate":"2022-02-04","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"47647916","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Thermomechanical Analysis of a Reactor Pressure Vessel under Pressurized Thermal Shock Caused by Inadvertent Actuation of the Safety Injection System 反应堆压力容器在安全注射系统误动引起的加压热冲击下的热力学分析
IF 1.1 4区 工程技术 Q3 Energy Pub Date : 2022-02-02 DOI: 10.1155/2022/5886583
M. Annor-Nyarko, Hong Xia, A. Ayodeji
The damage induced pressurized thermal shock (PTS) may pose to a reactor pressure vessel (RPV) is a critical safety requirement assessed as part of the ageing management programme of pressurized water reactors (PWRs). A number of researches have studied PTS initiated mainly by postulated accidents such as loss of coolant accidents (LOCAs). However, investigations on PTS-induced threat on RPV caused by inadvertent actuation of the safety injection, a frequent anticipated transient, have not been thoroughly studied. In this paper, a simplified multistep analysis method is applied to study the thermomechanical status of a two-loop PWR under PTS loads caused by inadvertent actuation of the safety injection system. A direct-coupling thermomechanical analysis is performed using a three-dimensional (3D) RPV finite element model. A 3D finite element submodel (consisting of the highiest stress concentration area in the RPV) and an assumed crack are then used to perform fracture mechanics analysis. Subsequently, the critical integrity parameter-stress intensity factor (SIF) is estimated based on FRANC3D-M-integral method coupled in the multistep simulation. The material fracture toughness of the vessel is computed based on the master curve method with experimental fracture toughness data. The results obtained from the direct coupling stress analysis in comparison with sequential coupling approach demonstrate the effectiveness of the proposed multistep method. Also, comparing SIF results obtained with that calculated based on the conventional virtual crack-closure technique (VCCT) and extended finite element method (XFEM) show good agreement. This study provides a useful basis for future studies on anticipated transient-induced crack propagation and remaining service life prediction of ageing reactor pressure vessels.
压力热冲击对反应堆压力容器造成的损伤是压水堆老化管理方案中一个重要的安全要求。许多对PTS的研究主要是由假设的事故如冷却剂损失事故(LOCAs)发起的。然而,由于安全注入的意外驱动(一种常见的预期瞬态)而引起的pts对RPV的威胁尚未得到充分研究。本文采用一种简化的多步分析方法,研究了安全喷射系统误动引起的PTS载荷下双环压水堆的热力状态。采用三维(3D) RPV有限元模型进行了直接耦合热力学分析。然后使用三维有限元子模型(由RPV中最高应力集中区组成)和假设裂纹进行断裂力学分析。在此基础上,基于franc3d - m积分法在多步模拟中耦合估计了临界完整性参数-应力强度因子(SIF)。利用实验断裂韧性数据,采用主曲线法计算容器材料断裂韧性。将直接耦合应力分析结果与顺序耦合方法进行了比较,验证了多步骤方法的有效性。将所得的SIF结果与基于传统虚拟裂纹闭合技术(VCCT)和扩展有限元法(XFEM)的计算结果进行了比较,结果吻合较好。该研究为今后对老化反应堆压力容器瞬态裂纹扩展的预测和剩余使用寿命的预测提供了有益的基础。
{"title":"Thermomechanical Analysis of a Reactor Pressure Vessel under Pressurized Thermal Shock Caused by Inadvertent Actuation of the Safety Injection System","authors":"M. Annor-Nyarko, Hong Xia, A. Ayodeji","doi":"10.1155/2022/5886583","DOIUrl":"https://doi.org/10.1155/2022/5886583","url":null,"abstract":"The damage induced pressurized thermal shock (PTS) may pose to a reactor pressure vessel (RPV) is a critical safety requirement assessed as part of the ageing management programme of pressurized water reactors (PWRs). A number of researches have studied PTS initiated mainly by postulated accidents such as loss of coolant accidents (LOCAs). However, investigations on PTS-induced threat on RPV caused by inadvertent actuation of the safety injection, a frequent anticipated transient, have not been thoroughly studied. In this paper, a simplified multistep analysis method is applied to study the thermomechanical status of a two-loop PWR under PTS loads caused by inadvertent actuation of the safety injection system. A direct-coupling thermomechanical analysis is performed using a three-dimensional (3D) RPV finite element model. A 3D finite element submodel (consisting of the highiest stress concentration area in the RPV) and an assumed crack are then used to perform fracture mechanics analysis. Subsequently, the critical integrity parameter-stress intensity factor (SIF) is estimated based on FRANC3D-M-integral method coupled in the multistep simulation. The material fracture toughness of the vessel is computed based on the master curve method with experimental fracture toughness data. The results obtained from the direct coupling stress analysis in comparison with sequential coupling approach demonstrate the effectiveness of the proposed multistep method. Also, comparing SIF results obtained with that calculated based on the conventional virtual crack-closure technique (VCCT) and extended finite element method (XFEM) show good agreement. This study provides a useful basis for future studies on anticipated transient-induced crack propagation and remaining service life prediction of ageing reactor pressure vessels.","PeriodicalId":21629,"journal":{"name":"Science and Technology of Nuclear Installations","volume":null,"pages":null},"PeriodicalIF":1.1,"publicationDate":"2022-02-02","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"46884654","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 3
Analysis of Heat Release Processes inside Storage Facilities Containing Irradiated Nuclear Graphite 辐照核石墨贮存设施内部放热过程分析
IF 1.1 4区 工程技术 Q3 Energy Pub Date : 2022-01-30 DOI: 10.1155/2022/2957310
A. Pavliuk, Evgeniy V. Bespala, S. Kotlyarevskiy, I. Novoselov, V. N. Kotov
The article is dedicated to the safety assessment of mixed storage of irradiated graphite and other types of radioactive waste accumulated during the operation of uranium-graphite reactors. The analysis of heat release processes inside storages containing irradiated nuclear graphite, representing a potential hazard due to the possible heating and, accordingly, the release of long-lived radionuclides during oxidation was carried out. The following factors were considered as the main factors that can lead to an increase in the temperature inside the storage facility: corrosion of metallic radioactive waste, the presence of fuel fragments, and also the random exposure of irradiated graphite to local sources of thermal energy (spark, etc.). It was noted in the work that the combined or separate influence of some factors can lead to an increase in the temperature of the onset of the initiation of Wigner energy release in graphite radwaste (Tin ≈ 90–100°C for the “Worst-case” graphite). The model of heat generation in the storage was developed based on the analysis of the features of graphite radioactive waste storage and Wigner energy release. The layered location of different types of waste (graphite and aluminum) and the local character of the distribution of heat sources were adopted in this model. The greatest heating is achieved if graphite radioactive waste is located near the concrete walls of the storage facility, as well as in direct contact with irradiated aluminum radioactive waste, which was shown in this paper.
本文致力于对铀-石墨反应堆运行过程中积累的辐照石墨和其他类型放射性废物的混合储存进行安全评估。对含有辐照核石墨的仓库内的热释放过程进行了分析,这代表了由于可能的加热而产生的潜在危险,因此,在氧化过程中释放了长寿命放射性核素。以下因素被认为是可能导致储存设施内温度升高的主要因素:金属放射性废物的腐蚀、燃料碎片的存在、,以及辐照石墨随机暴露于局部热能源(火花等)。工作中注意到,一些因素的组合或单独影响会导致石墨放射性废物中Wigner能量释放起始温度的升高(Tin ≈ 90–100°C(对于“最坏情况”的石墨)。在分析石墨放射性废物贮存和Wigner能量释放特征的基础上,建立了贮存过程中的热量产生模型。该模型采用了不同类型废物(石墨和铝)的分层位置和热源分布的局部特征。如本文所示,如果石墨放射性废物位于储存设施的混凝土墙附近,并与辐照过的铝放射性废物直接接触,则可实现最大的加热。
{"title":"Analysis of Heat Release Processes inside Storage Facilities Containing Irradiated Nuclear Graphite","authors":"A. Pavliuk, Evgeniy V. Bespala, S. Kotlyarevskiy, I. Novoselov, V. N. Kotov","doi":"10.1155/2022/2957310","DOIUrl":"https://doi.org/10.1155/2022/2957310","url":null,"abstract":"The article is dedicated to the safety assessment of mixed storage of irradiated graphite and other types of radioactive waste accumulated during the operation of uranium-graphite reactors. The analysis of heat release processes inside storages containing irradiated nuclear graphite, representing a potential hazard due to the possible heating and, accordingly, the release of long-lived radionuclides during oxidation was carried out. The following factors were considered as the main factors that can lead to an increase in the temperature inside the storage facility: corrosion of metallic radioactive waste, the presence of fuel fragments, and also the random exposure of irradiated graphite to local sources of thermal energy (spark, etc.). It was noted in the work that the combined or separate influence of some factors can lead to an increase in the temperature of the onset of the initiation of Wigner energy release in graphite radwaste (Tin ≈ 90–100°C for the “Worst-case” graphite). The model of heat generation in the storage was developed based on the analysis of the features of graphite radioactive waste storage and Wigner energy release. The layered location of different types of waste (graphite and aluminum) and the local character of the distribution of heat sources were adopted in this model. The greatest heating is achieved if graphite radioactive waste is located near the concrete walls of the storage facility, as well as in direct contact with irradiated aluminum radioactive waste, which was shown in this paper.","PeriodicalId":21629,"journal":{"name":"Science and Technology of Nuclear Installations","volume":null,"pages":null},"PeriodicalIF":1.1,"publicationDate":"2022-01-30","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"46561240","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Innovative Design of Compact Heavy-Load Independent Transfer Device for Nuclear Engineering System 核工程系统紧凑型重载独立转移装置的创新设计
IF 1.1 4区 工程技术 Q3 Energy Pub Date : 2022-01-30 DOI: 10.1155/2022/5256808
Hao Wan, Songfeng Weng, Hua Du, Dailin Dong, Bingyan Wang, Tianda Yu
The transportation of heavy equipment in nuclear engineering has always been the focus of engineers, especially those transfer devices with the characteristics of small geometric size and heavy load. According to this kind of compact heavy-load transfer device and its engineering tasks, the core problems caused by excessive vertical and horizontal forces in the design process were analyzed. By introducing the theory of inventive problem solving (TRIZ) design method, these problems were creatively solved by the contradiction theory and substance-field model in TRIZ, and an innovative design scheme of the compact heavy load-independent transfer device was obtained. Through the analysis of the design scheme and the stability and rapidity of its hydraulic system, some key parameters were determined. The power of the transfer device was all from the hydraulic system, and it can carry up to 300 t weight of reactor equipment, while its geometric size was only 1600 × 400 × 500 mm. It was of great significance to improve the efficiency of the nuclear engineering system.
核工程中重型设备的运输一直是工程师们关注的焦点,尤其是那些具有几何尺寸小、载荷大等特点的转运装置。根据这种紧凑型重载传递装置及其工程任务,分析了设计过程中竖向和水平力过大引起的核心问题。通过引入创造性问题解决理论(TRIZ)设计方法,利用TRIZ中的矛盾理论和物质场模型创造性地解决了这些问题,得到了紧凑型重载独立转移装置的创新设计方案。通过对其液压系统的设计方案和稳定性、快速性的分析,确定了一些关键参数。传送装置的动力全部来自液压系统,它最多可携带300 t反应堆设备的重量,而其几何尺寸只有1600 × 400 × 500 这对提高核工程系统的效率具有重要意义。
{"title":"Innovative Design of Compact Heavy-Load Independent Transfer Device for Nuclear Engineering System","authors":"Hao Wan, Songfeng Weng, Hua Du, Dailin Dong, Bingyan Wang, Tianda Yu","doi":"10.1155/2022/5256808","DOIUrl":"https://doi.org/10.1155/2022/5256808","url":null,"abstract":"The transportation of heavy equipment in nuclear engineering has always been the focus of engineers, especially those transfer devices with the characteristics of small geometric size and heavy load. According to this kind of compact heavy-load transfer device and its engineering tasks, the core problems caused by excessive vertical and horizontal forces in the design process were analyzed. By introducing the theory of inventive problem solving (TRIZ) design method, these problems were creatively solved by the contradiction theory and substance-field model in TRIZ, and an innovative design scheme of the compact heavy load-independent transfer device was obtained. Through the analysis of the design scheme and the stability and rapidity of its hydraulic system, some key parameters were determined. The power of the transfer device was all from the hydraulic system, and it can carry up to 300 t weight of reactor equipment, while its geometric size was only 1600 × 400 × 500 mm. It was of great significance to improve the efficiency of the nuclear engineering system.","PeriodicalId":21629,"journal":{"name":"Science and Technology of Nuclear Installations","volume":null,"pages":null},"PeriodicalIF":1.1,"publicationDate":"2022-01-30","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"47122539","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 1
期刊
Science and Technology of Nuclear Installations
全部 Acc. Chem. Res. ACS Applied Bio Materials ACS Appl. Electron. Mater. ACS Appl. Energy Mater. ACS Appl. Mater. Interfaces ACS Appl. Nano Mater. ACS Appl. Polym. Mater. ACS BIOMATER-SCI ENG ACS Catal. ACS Cent. Sci. ACS Chem. Biol. ACS Chemical Health & Safety ACS Chem. Neurosci. ACS Comb. Sci. ACS Earth Space Chem. ACS Energy Lett. ACS Infect. Dis. ACS Macro Lett. ACS Mater. Lett. ACS Med. Chem. Lett. ACS Nano ACS Omega ACS Photonics ACS Sens. ACS Sustainable Chem. Eng. ACS Synth. Biol. Anal. Chem. BIOCHEMISTRY-US Bioconjugate Chem. BIOMACROMOLECULES Chem. Res. Toxicol. Chem. Rev. Chem. Mater. CRYST GROWTH DES ENERG FUEL Environ. Sci. Technol. Environ. Sci. Technol. Lett. Eur. J. Inorg. Chem. IND ENG CHEM RES Inorg. Chem. J. Agric. Food. Chem. J. Chem. Eng. Data J. Chem. Educ. J. Chem. Inf. Model. J. Chem. Theory Comput. J. Med. Chem. J. Nat. Prod. J PROTEOME RES J. Am. Chem. Soc. LANGMUIR MACROMOLECULES Mol. Pharmaceutics Nano Lett. Org. Lett. ORG PROCESS RES DEV ORGANOMETALLICS J. Org. Chem. J. Phys. Chem. J. Phys. Chem. A J. Phys. Chem. B J. Phys. Chem. C J. Phys. Chem. Lett. Analyst Anal. Methods Biomater. Sci. Catal. Sci. Technol. Chem. Commun. Chem. Soc. Rev. CHEM EDUC RES PRACT CRYSTENGCOMM Dalton Trans. Energy Environ. Sci. ENVIRON SCI-NANO ENVIRON SCI-PROC IMP ENVIRON SCI-WAT RES Faraday Discuss. Food Funct. Green Chem. Inorg. Chem. Front. Integr. Biol. J. Anal. At. Spectrom. J. Mater. Chem. A J. Mater. Chem. B J. Mater. Chem. C Lab Chip Mater. Chem. Front. Mater. Horiz. MEDCHEMCOMM Metallomics Mol. Biosyst. Mol. Syst. Des. Eng. Nanoscale Nanoscale Horiz. Nat. Prod. Rep. New J. Chem. Org. Biomol. Chem. Org. Chem. Front. PHOTOCH PHOTOBIO SCI PCCP Polym. Chem.
×
引用
GB/T 7714-2015
复制
MLA
复制
APA
复制
导出至
BibTeX EndNote RefMan NoteFirst NoteExpress
×
0
微信
客服QQ
Book学术公众号 扫码关注我们
反馈
×
意见反馈
请填写您的意见或建议
请填写您的手机或邮箱
×
提示
您的信息不完整,为了账户安全,请先补充。
现在去补充
×
提示
您因"违规操作"
具体请查看互助需知
我知道了
×
提示
现在去查看 取消
×
提示
确定
Book学术官方微信
Book学术文献互助
Book学术文献互助群
群 号:481959085
Book学术
文献互助 智能选刊 最新文献 互助须知 联系我们:info@booksci.cn
Book学术提供免费学术资源搜索服务,方便国内外学者检索中英文文献。致力于提供最便捷和优质的服务体验。
Copyright © 2023 Book学术 All rights reserved.
ghs 京公网安备 11010802042870号 京ICP备2023020795号-1