Pub Date : 2023-12-15DOI: 10.1007/s11430-023-1187-8
Meng Li, Xin Li, Stephen P. Hesselbo, Mingjie Li, Wenjin Liu, Wei Wu, Jienan Pan, Ruizhen Gao
Lake-level changes can significantly affect paleoenvironmental evolution, resource occurrence, terrestrial carbon budget, and biodiversity in continental basins. Climate is one of the most critical factors controlling lake-level changes. Paleoclimate of the Early Jurassic has been evidenced by oscillating icehouses to (super) greenhouses with interrupted intermittent extreme climatic events (hyperthermal and cooling), e.g., the Toarcian oceanic anoxic event (~183 Ma) and the late Pliensbachian cooling event (~185 Ma). Lake-level evolution and hydrologic cycling on Earth’s surface during the Early Jurassic icehouses-to-(super)greenhouses are thus far poorly understood due to a lack of continuous high-resolution nonmarine evidence. Here we present a super-long nonmarine lake level record for this pivotal interval from the early Pliensbachian to Toarcian by sedimentary noise modeling, and construct a 16.7-Myr-long astronomical time scale (174.2 Ma to 190.9 Ma) based on cyclostratigraphy analysis of rock color datasets (CIE b*) of the Qaidam Basin. Our results document lake-level oscillations on a 5-to 10-million-year (Myr) scale which shows a pronounced correlation with long-term climate variation and extreme climatic events, and 1- to 2.5-Myr-scale lake-level changes that are prominently paced by the 2.4-Myr long-eccentricity forcing and the 1.2-Myr obliquity forcing. At the Pliensbachian Stage, the 1.2-Myr-scale lake-level changes are in phase with the coeval sea-level variations. Orbitally forced growth and decay of the ephemeral or permanent ice sheets in polar regions are interpreted to control the synchronous ups-and-downs of continental lake level and global sea level. However, during the Toarcian ice-free greenhouses to (super)greenhouses, the 1.2-Myr-scale lake-level variations show an anti-phase relationship with global sea level, indicating a ‘seesaw’ interaction between continental reservoirs (lakes and groundwater) and global oceans. The 2.4-Myr long-eccentricity cycles mainly regulate variations of lake level and sea level by controlling the growth and decay of small-scale continental ice sheets, which is especially notable during the Pliensbachian Stage. These findings indicate a remarkable transition of hydrological cycling pattern during the Pliensbachian-Toarcian icehouses to (super)greenhouses, which provides new perspectives and evidence for investigating the hypothesis of global sea-level changes (e.g., glacio-eustasy and aquifer-eustasy) and long-period astronomical forcing in nonmarine stratigraphy.
{"title":"Orbital pacing and secular evolution of lake-level changes reconstructed by sedimentary noise modeling during the Early Jurassic icehouses-(super)greenhouses","authors":"Meng Li, Xin Li, Stephen P. Hesselbo, Mingjie Li, Wenjin Liu, Wei Wu, Jienan Pan, Ruizhen Gao","doi":"10.1007/s11430-023-1187-8","DOIUrl":"https://doi.org/10.1007/s11430-023-1187-8","url":null,"abstract":"<p>Lake-level changes can significantly affect paleoenvironmental evolution, resource occurrence, terrestrial carbon budget, and biodiversity in continental basins. Climate is one of the most critical factors controlling lake-level changes. Paleoclimate of the Early Jurassic has been evidenced by oscillating icehouses to (super) greenhouses with interrupted intermittent extreme climatic events (hyperthermal and cooling), e.g., the Toarcian oceanic anoxic event (~183 Ma) and the late Pliensbachian cooling event (~185 Ma). Lake-level evolution and hydrologic cycling on Earth’s surface during the Early Jurassic icehouses-to-(super)greenhouses are thus far poorly understood due to a lack of continuous high-resolution nonmarine evidence. Here we present a super-long nonmarine lake level record for this pivotal interval from the early Pliensbachian to Toarcian by sedimentary noise modeling, and construct a 16.7-Myr-long astronomical time scale (174.2 Ma to 190.9 Ma) based on cyclostratigraphy analysis of rock color datasets (CIE b*) of the Qaidam Basin. Our results document lake-level oscillations on a 5-to 10-million-year (Myr) scale which shows a pronounced correlation with long-term climate variation and extreme climatic events, and 1- to 2.5-Myr-scale lake-level changes that are prominently paced by the 2.4-Myr long-eccentricity forcing and the 1.2-Myr obliquity forcing. At the Pliensbachian Stage, the 1.2-Myr-scale lake-level changes are in phase with the coeval sea-level variations. Orbitally forced growth and decay of the ephemeral or permanent ice sheets in polar regions are interpreted to control the synchronous ups-and-downs of continental lake level and global sea level. However, during the Toarcian ice-free greenhouses to (super)greenhouses, the 1.2-Myr-scale lake-level variations show an anti-phase relationship with global sea level, indicating a ‘seesaw’ interaction between continental reservoirs (lakes and groundwater) and global oceans. The 2.4-Myr long-eccentricity cycles mainly regulate variations of lake level and sea level by controlling the growth and decay of small-scale continental ice sheets, which is especially notable during the Pliensbachian Stage. These findings indicate a remarkable transition of hydrological cycling pattern during the Pliensbachian-Toarcian icehouses to (super)greenhouses, which provides new perspectives and evidence for investigating the hypothesis of global sea-level changes (e.g., glacio-eustasy and aquifer-eustasy) and long-period astronomical forcing in nonmarine stratigraphy.</p>","PeriodicalId":21651,"journal":{"name":"Science China Earth Sciences","volume":"19 1","pages":""},"PeriodicalIF":5.7,"publicationDate":"2023-12-15","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"138744834","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"地球科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2023-12-15DOI: 10.1007/s11430-023-1229-7
Zhongrui Wang, Haohao Sun, Lili Lei, Zhe-Min Tan, Yi Zhang
Despite a specific data assimilation method, data assimilation (DA) in general can be decomposed into components of the prior information, observation forward operator that is given by the observation type, observation error covariances, and background error covariances. In a classic Lorenz model, the influences of the DA components on the initial conditions (ICs) and subsequent forecasts are systematically investigated, which could provide a theoretical basis for the design of DA for different scales of interests. The forecast errors undergo three typical stages: a slow growth stage from 0 h to 5 d, a fast growth stage from 5 d to around 15 d with significantly different error growth rates for ensemble and deterministic forecasts, and a saturation stage after 15 d. Assimilation strategies that provide more accurate ICs can improve the predictability. Cycling assimilation is superior to offline assimilation, and a flow-dependent background error covariance matrix (Pf) provides better analyses than a static background error covariance matrix (B) for instantaneous observations and frequent time-averaged observations; but the opposite is true for infrequent time-averaged observations, since cycling simulation cannot construct informative priors when the model lacks predictive skills and the flow-dependent Pf cannot effectively extract information from low-informative observations as the static B. Instantaneous observations contain more information than time-averaged observations, thus the former is preferred, especially for infrequent observing systems. Moreover, ensemble forecasts have advantages over deterministic forecasts, and the advantages are enlarged with less informative observations and lower predictive-skill model priors.
尽管有特定的数据同化方法,但数据同化(DA)一般可分解为先验信息、观测类型给出的观测前向算子、观测误差协方差和背景误差协方差等组成部分。在经典的洛伦兹模型中,系统地研究了先验信息成分对初始条件(IC)和后续预测的影响,这为设计不同规模的先验信息提供了理论依据。预报误差经历了三个典型阶段:从 0 h 到 5 d 的缓慢增长阶段;从 5 d 到 15 d 左右的快速增长阶段(集合预报和确定性预报的误差增长率明显不同);以及 15 d 后的饱和阶段。循环同化优于离线同化,对于瞬时观测数据和频繁的时间平均观测数据,与流量相关的背景误差协方差矩阵(Pf)比静态背景误差协方差矩阵(B)能提供更好的分析;但对于不频繁的时间平均观测数据,情况则恰恰相反,因为当模式缺乏预测能力时,循环模拟无法构建信息丰富的先验,而与流量相关的 Pf 无法像静态 B 那样有效地从信息量低的观测数据中提取信息。瞬时观测数据比时间平均观测数据包含更多的信息,因此前者更受欢迎,特别是对于不频繁的观测系统。此外,集合预报比确定性预报更有优势,而且在观测信息量较少和模型预报技能较低的情况下,集合预报的优势会进一步扩大。
{"title":"The importance of data assimilation components for initial conditions and subsequent error growth","authors":"Zhongrui Wang, Haohao Sun, Lili Lei, Zhe-Min Tan, Yi Zhang","doi":"10.1007/s11430-023-1229-7","DOIUrl":"https://doi.org/10.1007/s11430-023-1229-7","url":null,"abstract":"<p>Despite a specific data assimilation method, data assimilation (DA) in general can be decomposed into components of the prior information, observation forward operator that is given by the observation type, observation error covariances, and background error covariances. In a classic Lorenz model, the influences of the DA components on the initial conditions (ICs) and subsequent forecasts are systematically investigated, which could provide a theoretical basis for the design of DA for different scales of interests. The forecast errors undergo three typical stages: a slow growth stage from 0 h to 5 d, a fast growth stage from 5 d to around 15 d with significantly different error growth rates for ensemble and deterministic forecasts, and a saturation stage after 15 d. Assimilation strategies that provide more accurate ICs can improve the predictability. Cycling assimilation is superior to offline assimilation, and a flow-dependent background error covariance matrix (<b>P</b><sup><i>f</i></sup>) provides better analyses than a static background error covariance matrix (<b>B</b>) for instantaneous observations and frequent time-averaged observations; but the opposite is true for infrequent time-averaged observations, since cycling simulation cannot construct informative priors when the model lacks predictive skills and the flow-dependent <b>P</b><sup><i>f</i></sup> cannot effectively extract information from low-informative observations as the static <b>B</b>. Instantaneous observations contain more information than time-averaged observations, thus the former is preferred, especially for infrequent observing systems. Moreover, ensemble forecasts have advantages over deterministic forecasts, and the advantages are enlarged with less informative observations and lower predictive-skill model priors.</p>","PeriodicalId":21651,"journal":{"name":"Science China Earth Sciences","volume":"44 1","pages":""},"PeriodicalIF":5.7,"publicationDate":"2023-12-15","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"138744548","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"地球科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2023-12-15DOI: 10.1007/s11430-022-1183-4
Dijun Guo, Jianzhong Liu, James W. Head, Fuqin Zhang, Zongcheng Ling, Shengbo Chen, Jianping Chen, Xiaozhong Ding, Jinzhu Ji, Ziyuan Ouyang
A geologic time scale is a chronological system that separates the geological strata of a planetary body into different units in temporal sequence and shows its progressive evolution. The time scale of the Moon was established a half-century ago during the telescopic-early Apollo exploration era, using data with limited spatial coverage and resolution. The past decades have seen a wide array of studies, which have significantly extended our understanding of global lunar geologic evolution. Based on a comprehensive review of lunar evolution with respect to the dynamical changes, we propose two major updates to the current lunar time scale paradigm to include the evolution of both endogenic and exogenic dynamic forces now known to have influenced early lunar history. Firstly, based on the temporal interplay of exogenic and endogenic processes in altering the Moon, we defined three Eon/Eonothem-level units to represent three dynamical evolutionary phases. Secondly, the pre-Nectarian System is redefined and divided as the magma ocean-era Magma-oceanian System and the following Aitkenian System beginning with the South Pole-Aitken basin. The ejecta of this basin, Das Formation, was deposited on the primordial lunar crust as the oldest stratum produced from exogenic processes. The updated lunar time scale, facilitated by the post-Apollo exploration and research advances, provides an integrated framework to depict the evolution of the Moon and has important implications for the geologic study of other terrestrial planets.
地质时间尺度是一种年代学系统,它将行星体的地质层按时间顺序分成不同的单元,并显示其逐渐演变的过程。月球的时间尺度是半个世纪前在望远镜-早期阿波罗探测时代利用有限的空间覆盖和分辨率数据建立的。在过去的几十年里,我们开展了大量的研究,极大地扩展了我们对全球月球地质演变的认识。在全面回顾月球演化动态变化的基础上,我们对目前的月球时间尺度范式提出了两大更新建议,以纳入目前已知的影响早期月球历史的内源和外源动力的演化。首先,根据改变月球的外源和内源过程在时间上的相互作用,我们定义了三个Eon/Eonothem级单元,分别代表三个动力学演化阶段。其次,重新定义了前内行星系统,并将其划分为岩浆洋时代的岩浆洋系统和从南极-艾特肯盆地开始的艾特肯系统。该盆地的喷出物 Das Formation 沉积在原始月壳上,是外生过程产生的最古老地层。阿波罗之后的探索和研究进展促进了月球时间尺度的更新,为描述月球的演变提供了一个综合框架,并对其他陆地行星的地质研究产生了重要影响。
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Pub Date : 2023-12-14DOI: 10.1007/s11430-022-1191-8
<h3>Abstract</h3> <p>Establishing a quantitative relationship between modern pollen and vegetation remains a pivotal but intricate pursuit within the field of Quaternary palynology. The <em>R</em>-value, a well-established and traditional metric characterized by its simplicity and direct applicability, serves to calibrate the nonlinear disparities between surface pollen and modern vegetation. This study entails the construction of a comprehensive pollen R-value dataset for China derived from <em>R</em>-values published between 1987 and 2021. The dataset, compiled after rigorous screening, calibration, and standardization processes, encompasses 898 modern pollen sampling sites and 2115 pollen R-value data entries, encapsulating 152 pollen taxa spanning 65 families and 113 genera. Synthesizing the extracted <em>R</em>-values yielded the following insights: (1) A macrospatial analysis validates previously established knowledge at a site-specific scale. Evidently, pollen <em>R</em>-value variations across China are statistically significant. Approximately two-thirds of pollen taxa exhibit underrepresentation (e.g., Taxodiaceae, <em>Corylus</em>, <em>Nitraria</em>, <em>Tamarix</em>, Cyperaceae, Poaceae, and Fabaceae), while the remaining one-third display overrepresentation (e.g., <em>Pinus</em>, <em>Picea</em>, <em>Betula</em>, <em>Ephedra</em>, Chenopodiaceae, and <em>Artemisia</em>). The degree of underrepresentation surpasses that of over-representation, and the representation patterns of <em>Castanea</em>, <em>Quercus</em>, Polygonaceae, and Asteraceae are contingent upon vegetation types. (2) Pollen <em>R</em>-values follow distinct spatial distribution patterns within China. In the woody vegetation region of eastern China, <em>R</em>-values progressively decline from north to south, correlating with rising temperatures and precipitation. Conversely, in herbaceous vegetation regions of northern and western China, <em>R</em>-values decrease from east to west and from northeast to southwest, corresponding to increased aridity. Nevertheless, pollen <em>R</em>-values manifest variation contingent on pollen taxa, vegetation types, and climatic regions, even differing for the same taxa across varying vegetation types and climatic conditions. This highlights the intricate nature of pollen <em>R</em>-values and their interpretation of pollen-vegetation relationships. (3) Pollen <em>R</em>-values and relative pollen production estimates exhibit resemblances and a modest positive correlation. However, adjudicating between them as representatives of vegetation requires nuanced consideration, as both metrics convey pollen representation within vegetation, demonstrating the multifaceted relationships they share with modern vegetation. Further recommendations suggest that when assessing pollen representation in modern vegetation, fossil pollen content should be weighted using either the median or log-transformed <em>R</em>-value. This approach underscores the
摘要 建立现代花粉与植被之间的定量关系仍然是第四纪古生物学领域的一项关键而又复杂的工作。R值是一个成熟的传统指标,其特点是简单、直接适用,可用于校准地表花粉与现代植被之间的非线性差异。本研究通过 1987 年至 2021 年间发表的 R 值,为中国建立了一个全面的花粉 R 值数据集。该数据集经过严格的筛选、校准和标准化流程编制而成,包含 898 个现代花粉采样点和 2115 个花粉 R 值数据条目,涵盖 152 个花粉类群,涵盖 65 科 113 属。综合提取的 R 值得出以下结论:(1) 宏观空间分析在特定地点尺度上验证了先前建立的知识。显然,中国各地的花粉 R 值差异在统计学上是显著的。约三分之二的花粉类群表现出代表性不足(如杉木科、榛属、稔属、柽柳属、香蒲科、禾本科和豆科),而其余三分之一的类群则表现出代表性过高(如松属、杉属、桦属、麻黄属、藜属和蒿属)。代表性不足的程度超过了代表性过剩的程度,蓖麻科、柞树科、蓼科和菊科的代表性模式取决于植被类型。(2)花粉 R 值在中国境内有明显的空间分布格局。在中国东部木本植被区,R 值由北向南逐渐下降,这与气温和降水量的上升有关。相反,在中国北部和西部的草本植被区,R 值从东到西和从东北到西南逐渐降低,这与干旱加剧有关。尽管如此,花粉 R 值仍因花粉类群、植被类型和气候区域的不同而存在差异,甚至同一类群在不同植被类型和气候条件下也存在差异。这凸显了花粉 R 值及其对花粉植被关系解释的复杂性。(3) 花粉 R 值与相对花粉产量估计值有相似之处,并呈适度的正相关。然而,将它们作为植被的代表进行判定需要细微的考虑,因为这两个指标都表达了植被中的花粉代表性,显示了它们与现代植被的多方面关系。进一步的建议表明,在评估现代植被中的花粉代表性时,应使用中位数或对数变换的 R 值对化石花粉含量进行加权。这种方法强调了全面考虑不同空间尺度和植被类型中的差异和趋同的必要性,尤其是在不同地区的相同花粉类群中观察到的差异。
{"title":"Regional features of pollen R-values in China","authors":"","doi":"10.1007/s11430-022-1191-8","DOIUrl":"https://doi.org/10.1007/s11430-022-1191-8","url":null,"abstract":"<h3>Abstract</h3> <p>Establishing a quantitative relationship between modern pollen and vegetation remains a pivotal but intricate pursuit within the field of Quaternary palynology. The <em>R</em>-value, a well-established and traditional metric characterized by its simplicity and direct applicability, serves to calibrate the nonlinear disparities between surface pollen and modern vegetation. This study entails the construction of a comprehensive pollen R-value dataset for China derived from <em>R</em>-values published between 1987 and 2021. The dataset, compiled after rigorous screening, calibration, and standardization processes, encompasses 898 modern pollen sampling sites and 2115 pollen R-value data entries, encapsulating 152 pollen taxa spanning 65 families and 113 genera. Synthesizing the extracted <em>R</em>-values yielded the following insights: (1) A macrospatial analysis validates previously established knowledge at a site-specific scale. Evidently, pollen <em>R</em>-value variations across China are statistically significant. Approximately two-thirds of pollen taxa exhibit underrepresentation (e.g., Taxodiaceae, <em>Corylus</em>, <em>Nitraria</em>, <em>Tamarix</em>, Cyperaceae, Poaceae, and Fabaceae), while the remaining one-third display overrepresentation (e.g., <em>Pinus</em>, <em>Picea</em>, <em>Betula</em>, <em>Ephedra</em>, Chenopodiaceae, and <em>Artemisia</em>). The degree of underrepresentation surpasses that of over-representation, and the representation patterns of <em>Castanea</em>, <em>Quercus</em>, Polygonaceae, and Asteraceae are contingent upon vegetation types. (2) Pollen <em>R</em>-values follow distinct spatial distribution patterns within China. In the woody vegetation region of eastern China, <em>R</em>-values progressively decline from north to south, correlating with rising temperatures and precipitation. Conversely, in herbaceous vegetation regions of northern and western China, <em>R</em>-values decrease from east to west and from northeast to southwest, corresponding to increased aridity. Nevertheless, pollen <em>R</em>-values manifest variation contingent on pollen taxa, vegetation types, and climatic regions, even differing for the same taxa across varying vegetation types and climatic conditions. This highlights the intricate nature of pollen <em>R</em>-values and their interpretation of pollen-vegetation relationships. (3) Pollen <em>R</em>-values and relative pollen production estimates exhibit resemblances and a modest positive correlation. However, adjudicating between them as representatives of vegetation requires nuanced consideration, as both metrics convey pollen representation within vegetation, demonstrating the multifaceted relationships they share with modern vegetation. Further recommendations suggest that when assessing pollen representation in modern vegetation, fossil pollen content should be weighted using either the median or log-transformed <em>R</em>-value. This approach underscores the","PeriodicalId":21651,"journal":{"name":"Science China Earth Sciences","volume":"4 1","pages":""},"PeriodicalIF":5.7,"publicationDate":"2023-12-14","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"138681017","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"地球科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2023-12-14DOI: 10.1007/s11430-022-1164-2
Deng Liu, Jinpeng Cao, Shanshan Yang, Yating Yin, Pengcong Wang, Dominic Papineau, Hongmei Wang, Xuan Qiu, Genming Luo, Zongmin Zhu, Fengping Wang
The origin of sedimentary dolomite has become a long-standing problem in the Earth Sciences. Some carbonate minerals like ankerite have the same crystal structure as dolomite, hence their genesis may provide clues to help solving the dolomite problem. The purpose of this study was to probe whether microbial activity can be involved in the formation of ankerite. Bio-carbonation experiments associated with microbial iron reduction were performed in batch systems with various concentrations of Ca2+(0–20 mmol/L), with a marine iron-reducing bacterium Shewanella piezotolerans WP3 as the reaction mediator, and with lactate and ferrihydrite as the respective electron donor and acceptor. Our biomineralization data showed that Ca-amendments expedited microbially-mediated ferrihydrite reduction by enhancing the adhesion between WP3 cells and ferrihydrite particles. After bioreduction, siderite occurred as the principal secondary mineral in the Ca-free systems. Instead, Ca-Fe carbonates were formed when Ca2+ ions were present. The CaCO3 content of microbially-induced Ca-Fe carbonates was positively correlated with the initial Ca2+ concentration. The Ca-Fe carbonate phase produced in the 20 mmol/L Ca-amended biosystems had a chemical formula of Ca0.8Fe1.2(CO3)2, which is close to the theoretical composition of ankerite. This ankerite-like phase was nanometric in size and spherical, Ca-Fe disordered, and structurally defective. Our simulated diagenesis experiments further demonstrated that the resulting ankerite-like phase could be converted into ordered ankerite under hydrothermal conditions. We introduced the term “proto-ankerite” to define the Ca-Fe phases that possess near-ankerite stoichiometry but disordered cation arrangement. On the basis of the present study, we proposed herein that microbial activity is an important contributor to the genesis of sedimentary ankerite by providing the metastable Ca-Fe carbonate precursors.
{"title":"Microbially-mediated formation of Ca-Fe carbonates during dissimilatory ferrihydrite reduction: Implications for the origin of sedimentary ankerite","authors":"Deng Liu, Jinpeng Cao, Shanshan Yang, Yating Yin, Pengcong Wang, Dominic Papineau, Hongmei Wang, Xuan Qiu, Genming Luo, Zongmin Zhu, Fengping Wang","doi":"10.1007/s11430-022-1164-2","DOIUrl":"https://doi.org/10.1007/s11430-022-1164-2","url":null,"abstract":"<p>The origin of sedimentary dolomite has become a long-standing problem in the Earth Sciences. Some carbonate minerals like ankerite have the same crystal structure as dolomite, hence their genesis may provide clues to help solving the dolomite problem. The purpose of this study was to probe whether microbial activity can be involved in the formation of ankerite. Bio-carbonation experiments associated with microbial iron reduction were performed in batch systems with various concentrations of Ca<sup>2+</sup>(0–20 mmol/L), with a marine iron-reducing bacterium <i>Shewanella piezotolerans</i> WP3 as the reaction mediator, and with lactate and ferrihydrite as the respective electron donor and acceptor. Our biomineralization data showed that Ca-amendments expedited microbially-mediated ferrihydrite reduction by enhancing the adhesion between WP3 cells and ferrihydrite particles. After bioreduction, siderite occurred as the principal secondary mineral in the Ca-free systems. Instead, Ca-Fe carbonates were formed when Ca<sup>2+</sup> ions were present. The CaCO<sub>3</sub> content of microbially-induced Ca-Fe carbonates was positively correlated with the initial Ca<sup>2+</sup> concentration. The Ca-Fe carbonate phase produced in the 20 mmol/L Ca-amended biosystems had a chemical formula of Ca<sub>0.8</sub>Fe<sub>1.2</sub>(CO<sub>3</sub>)<sub>2</sub>, which is close to the theoretical composition of ankerite. This ankerite-like phase was nanometric in size and spherical, Ca-Fe disordered, and structurally defective. Our simulated diagenesis experiments further demonstrated that the resulting ankerite-like phase could be converted into ordered ankerite under hydrothermal conditions. We introduced the term “proto-ankerite” to define the Ca-Fe phases that possess near-ankerite stoichiometry but disordered cation arrangement. On the basis of the present study, we proposed herein that microbial activity is an important contributor to the genesis of sedimentary ankerite by providing the metastable Ca-Fe carbonate precursors.</p>","PeriodicalId":21651,"journal":{"name":"Science China Earth Sciences","volume":"4 1","pages":""},"PeriodicalIF":5.7,"publicationDate":"2023-12-14","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"138681235","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"地球科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2023-12-14DOI: 10.1007/s11430-023-1189-y
Rong Chai, Jianghai Yang, Yuansheng Du, Chengshan Wang
The Late Triassic witnessed significant collisional orogenic events in the Qinling orogenic belt, accompanied by magma underplating and tectonic deformation. These processes potentially resulted in substantial crustal thickening and uplift of the Qinling orogen. However, due to the absence of igneous rock records from this period in the eastern section of the Qinling orogen, the changes in crustal thickness during this orogenic process have not been thoroughly investigated. A series of foreland basins emerged during the Early Mesozoic to the south of the East Qinling orogenic belt. These basins have preserved clastic sedimentary rocks derived from the uplift and erosion of the orogenic belt. These sedimentary records serve as crucial records to reconstruct the evolutionary history of the Qinling orogen. To further clarify the collisional orogenic process of the Qinling orogenic belt, this study conducted in situ volcanic lithic fragment geochemistry, detrital zircon U-Pb chronology and trace element composition analysis on the sandstones of the Lower Jurassic Tongzhuyuan Formation in the Zigui Basin. The results suggest that the sandstones, which exhibit a significant abundance of volcanic lithic fragments, has a characteristic detrital zircon age group of 250–200 Ma, indicating a major provenance from the Triassic volcanic rocks. Combined with regional correlation and paleocurrent analysis, the detrital zircon U-Pb age data show that the source area of volcanic rocks should be in the Qinling orogenic belt to the north of the basin. This interpretation is further supported by the Triassic granitic rocks exposed in the western part of the orogenic belt, representing the magmatism during the Triassic collisional orogenesis in the Qinling orogen. Based on the co-varying relationships between present-day crust thickness with the chemical compositions of granite rocks and zircons, the La/Yb ratio of volcanic lithic fragments in the Tongzhuyuan Formation and the Eu/Eu ratio of detrital zircons with Triassic ages indicate that the Qinling orogen experienced crustal thickening during the Late Triassic, reaching its maximum thickness of 60–70 km at ca. 220–210 Ma. This crustal thickening in the eastern Qinling orogen is temporally consistent with that in the western orogen as recorded by the Triassic granitic rocks and may be related to large-scale crustal shortening and magmatism during the collisional orogeny.
{"title":"Provenance of the Lower Jurassic pyroclastic sediments in the Zigui Basin: Implication for crustal thickening in the eastern Qinling orogenic belt","authors":"Rong Chai, Jianghai Yang, Yuansheng Du, Chengshan Wang","doi":"10.1007/s11430-023-1189-y","DOIUrl":"https://doi.org/10.1007/s11430-023-1189-y","url":null,"abstract":"<p>The Late Triassic witnessed significant collisional orogenic events in the Qinling orogenic belt, accompanied by magma underplating and tectonic deformation. These processes potentially resulted in substantial crustal thickening and uplift of the Qinling orogen. However, due to the absence of igneous rock records from this period in the eastern section of the Qinling orogen, the changes in crustal thickness during this orogenic process have not been thoroughly investigated. A series of foreland basins emerged during the Early Mesozoic to the south of the East Qinling orogenic belt. These basins have preserved clastic sedimentary rocks derived from the uplift and erosion of the orogenic belt. These sedimentary records serve as crucial records to reconstruct the evolutionary history of the Qinling orogen. To further clarify the collisional orogenic process of the Qinling orogenic belt, this study conducted in situ volcanic lithic fragment geochemistry, detrital zircon U-Pb chronology and trace element composition analysis on the sandstones of the Lower Jurassic Tongzhuyuan Formation in the Zigui Basin. The results suggest that the sandstones, which exhibit a significant abundance of volcanic lithic fragments, has a characteristic detrital zircon age group of 250–200 Ma, indicating a major provenance from the Triassic volcanic rocks. Combined with regional correlation and paleocurrent analysis, the detrital zircon U-Pb age data show that the source area of volcanic rocks should be in the Qinling orogenic belt to the north of the basin. This interpretation is further supported by the Triassic granitic rocks exposed in the western part of the orogenic belt, representing the magmatism during the Triassic collisional orogenesis in the Qinling orogen. Based on the co-varying relationships between present-day crust thickness with the chemical compositions of granite rocks and zircons, the La/Yb ratio of volcanic lithic fragments in the Tongzhuyuan Formation and the Eu/Eu ratio of detrital zircons with Triassic ages indicate that the Qinling orogen experienced crustal thickening during the Late Triassic, reaching its maximum thickness of 60–70 km at ca. 220–210 Ma. This crustal thickening in the eastern Qinling orogen is temporally consistent with that in the western orogen as recorded by the Triassic granitic rocks and may be related to large-scale crustal shortening and magmatism during the collisional orogeny.</p>","PeriodicalId":21651,"journal":{"name":"Science China Earth Sciences","volume":"27 1","pages":""},"PeriodicalIF":5.7,"publicationDate":"2023-12-14","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"138744774","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"地球科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2023-12-14DOI: 10.1007/s11430-023-1237-6
Bao Yang, M. He
{"title":"Global warming strengthens the association between ENSO and the Asian-Australian summer monsoon","authors":"Bao Yang, M. He","doi":"10.1007/s11430-023-1237-6","DOIUrl":"https://doi.org/10.1007/s11430-023-1237-6","url":null,"abstract":"","PeriodicalId":21651,"journal":{"name":"Science China Earth Sciences","volume":"9 2","pages":""},"PeriodicalIF":5.7,"publicationDate":"2023-12-14","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"138971380","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"地球科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2023-12-13DOI: 10.1007/s11430-022-1224-1
Fangzhong Shi, Xiuchen Wu, Xiaoyan Li, Philippe Ciais, Hongyan Liu, Chao Yue, Yuting Yang, Shulei Zhang, Shushi Peng, Yi Yin, Benjamin Poulter, Deliang Chen
The recurrent extreme El Niño events are commonly linked to reduced vegetation growth and the land carbon sink over many but discrete regions of the Northern Hemisphere (NH). However, we reported here a pervasive and continuous vegetation greening and no weakened land carbon sink in the maturation phase of the 2015/2016 El Niño event over the NH (mainly in the extra-tropics), based on multiple evidences from remote sensing observations, global ecosystem model simulations and atmospheric CO2 inversions. We discovered a significant compensation effect of the enhanced vegetation growth in spring on subsequent summer/autumn vegetation growth that sustained vegetation greening and led to a slight increase in the land carbon sink over the spring and summer of 2015 (average increases of 23.34% and 0.63% in net ecosystem exchange from two independent datasets relative to a 5-years average before the El Niño event, respectively) and spring of 2016 (6.82%), especially in the extra-tropics of the NH, where the water supply during the pre-growing-season (November of the previous year to March of the current year) had a positive anomaly. This seasonal compensation effect was much stronger than that in 1997 and 1998 and significantly alleviated the adverse impacts of the 2015/2016 El Niño event on vegetation growth during its maturation phase. The legacy effect of water supply during the pre-growing-season on subsequent vegetation growth lasted up to approximately six months. Our findings highlight the role of seasonal compensation effects on mediating the land carbon sink in response to episodic extreme El Niño events.
{"title":"Seasonal compensation implied no weakening of the land carbon sink in the Northern Hemisphere under the 2015/2016 El Niño","authors":"Fangzhong Shi, Xiuchen Wu, Xiaoyan Li, Philippe Ciais, Hongyan Liu, Chao Yue, Yuting Yang, Shulei Zhang, Shushi Peng, Yi Yin, Benjamin Poulter, Deliang Chen","doi":"10.1007/s11430-022-1224-1","DOIUrl":"https://doi.org/10.1007/s11430-022-1224-1","url":null,"abstract":"<p>The recurrent extreme El Niño events are commonly linked to reduced vegetation growth and the land carbon sink over many but discrete regions of the Northern Hemisphere (NH). However, we reported here a pervasive and continuous vegetation greening and no weakened land carbon sink in the maturation phase of the 2015/2016 El Niño event over the NH (mainly in the extra-tropics), based on multiple evidences from remote sensing observations, global ecosystem model simulations and atmospheric CO<sub>2</sub> inversions. We discovered a significant compensation effect of the enhanced vegetation growth in spring on subsequent summer/autumn vegetation growth that sustained vegetation greening and led to a slight increase in the land carbon sink over the spring and summer of 2015 (average increases of 23.34% and 0.63% in net ecosystem exchange from two independent datasets relative to a 5-years average before the El Niño event, respectively) and spring of 2016 (6.82%), especially in the extra-tropics of the NH, where the water supply during the pre-growing-season (November of the previous year to March of the current year) had a positive anomaly. This seasonal compensation effect was much stronger than that in 1997 and 1998 and significantly alleviated the adverse impacts of the 2015/2016 El Niño event on vegetation growth during its maturation phase. The legacy effect of water supply during the pre-growing-season on subsequent vegetation growth lasted up to approximately six months. Our findings highlight the role of seasonal compensation effects on mediating the land carbon sink in response to episodic extreme El Niño events.</p>","PeriodicalId":21651,"journal":{"name":"Science China Earth Sciences","volume":"29 1","pages":""},"PeriodicalIF":5.7,"publicationDate":"2023-12-13","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"138681007","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"地球科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2023-12-13DOI: 10.1007/s11430-023-1210-5
YongFei Zheng
<p>Plate tectonics theory, established in the 1960s, has been successful in explaining many geological phenomena, processes and events that occurred in the Phanerozoic. However, the theory has often struggled to provide a coherent framework in interpreting geological records in continental interior and Precambrian period. In dealing with the relationship between plate tectonics and continental geology, continental interior tectonics was often separated from continental margin tectonics in the inheritance and development of their structure and composition. This separation led to the illusion that the plate tectonics theory is not applicable to Precambrian geology, particularly in explaining the fundamental geological characteristics of Archean cratons. Although this illusion does not mean that the Archean continental crust did not originate from a regime of plate tectonics, it led to the development of alternative tectonic models, often involving vertical movements under a regime of stagnant lid tectonics, including not only endogenous processes such as gravitational sagduction, mantle plumes and heat pipes but also exogenous processes such as bolide impacts. These vertical processes were not unique to the Archean but persisted into the Phanerozoic. They result from mantle poloidal convection at different depths, not specific to any particular period. Upgrading the plate tectonics theory from the traditional kinematic model in the 20th century to a holistic kinematic-dynamic model in the 21st century and systematically examining the vertical transport of matter and energy at plate margins, it is evident that plate tectonics can explain the common geological characteristics of Archean cratons, such as lithological associations, structural patterns and metamorphic evolution. By deciphering the structure and composition of convergent plate margins as well as their dynamics, the formation and evolution of continental crust since the Archean can be divided into ancient plate tectonics in the Precambrian and modern plate tectonics in the Phanerozoic. In addition, there are the following three characteristic features in the Archean: (1) convective mantle temperatures were 200–300°C higher than in the Phanerozoic, (2) newly formed basaltic oceanic crust was as thick as 30–40 km, and (3) the asthenosphere had a composition similar to the primitive mantle rather than the depleted mantle at present. On this basis, the upgraded plate tectonics theory can successfully explain the major geological phenomena of Archean cratons. This approach provides a new perspective on and deep insights into the evolution of early Earth and the origin of continental crust. In detail, Archean tonalite-trondhjemite-granodiorite (TTG) rocks would result from partial melting of the over-thick basaltic oceanic crust at convergent plate margins. The structural patterns of gneissic domes and greenstone keels would result from the buoyancy-driven emplacement of TTG magmas and its inte
{"title":"Plate tectonics in the Archean: Observations versus interpretations","authors":"YongFei Zheng","doi":"10.1007/s11430-023-1210-5","DOIUrl":"https://doi.org/10.1007/s11430-023-1210-5","url":null,"abstract":"<p>Plate tectonics theory, established in the 1960s, has been successful in explaining many geological phenomena, processes and events that occurred in the Phanerozoic. However, the theory has often struggled to provide a coherent framework in interpreting geological records in continental interior and Precambrian period. In dealing with the relationship between plate tectonics and continental geology, continental interior tectonics was often separated from continental margin tectonics in the inheritance and development of their structure and composition. This separation led to the illusion that the plate tectonics theory is not applicable to Precambrian geology, particularly in explaining the fundamental geological characteristics of Archean cratons. Although this illusion does not mean that the Archean continental crust did not originate from a regime of plate tectonics, it led to the development of alternative tectonic models, often involving vertical movements under a regime of stagnant lid tectonics, including not only endogenous processes such as gravitational sagduction, mantle plumes and heat pipes but also exogenous processes such as bolide impacts. These vertical processes were not unique to the Archean but persisted into the Phanerozoic. They result from mantle poloidal convection at different depths, not specific to any particular period. Upgrading the plate tectonics theory from the traditional kinematic model in the 20th century to a holistic kinematic-dynamic model in the 21st century and systematically examining the vertical transport of matter and energy at plate margins, it is evident that plate tectonics can explain the common geological characteristics of Archean cratons, such as lithological associations, structural patterns and metamorphic evolution. By deciphering the structure and composition of convergent plate margins as well as their dynamics, the formation and evolution of continental crust since the Archean can be divided into ancient plate tectonics in the Precambrian and modern plate tectonics in the Phanerozoic. In addition, there are the following three characteristic features in the Archean: (1) convective mantle temperatures were 200–300°C higher than in the Phanerozoic, (2) newly formed basaltic oceanic crust was as thick as 30–40 km, and (3) the asthenosphere had a composition similar to the primitive mantle rather than the depleted mantle at present. On this basis, the upgraded plate tectonics theory can successfully explain the major geological phenomena of Archean cratons. This approach provides a new perspective on and deep insights into the evolution of early Earth and the origin of continental crust. In detail, Archean tonalite-trondhjemite-granodiorite (TTG) rocks would result from partial melting of the over-thick basaltic oceanic crust at convergent plate margins. The structural patterns of gneissic domes and greenstone keels would result from the buoyancy-driven emplacement of TTG magmas and its inte","PeriodicalId":21651,"journal":{"name":"Science China Earth Sciences","volume":"87 1","pages":""},"PeriodicalIF":5.7,"publicationDate":"2023-12-13","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"138693263","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"地球科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2023-12-13DOI: 10.1007/s11430-022-1171-3
Abstract
Rheology of rocks controls the deformation of the Earth at various space-time scales, which is crucial to understand the tectonic evolution of continental lithosphere. Researches of rock rheology are mainly conducted via high-pressure and high-temperature rheological experiments and multi-scale observations and measurements of naturally deformed rocks. At present, a large amount of data from such kinds of studies have been accumulated. This paper first provides an up-to-date comprehensive review of the rheological mechanisms, fabric types and seismic properties of the main rock-forming minerals at different depths of continental lithosphere, including olivine, orthopyroxene, clinopyroxene, amphibole, plagioclase, quartz and mica. Then, progress in high-pressure and high-temperature experiments and natural deformation observations is introduced, mainly regarding the rheological strength and behavior, seismic velocity and anisotropy of lithospheric mantle peridotite, eclogite, mafic granulite, amphibolite and felsic rocks. Finally, by taking the Tibetan Plateau as an example, the application of rock rheology for quantitative interpretation of seismic anisotropy data is discussed. The combination of mineral deformation fabrics and seismic anisotropy is expected to make an important breakthrough in understanding the rheological properties and structure of continental lithosphere.
{"title":"Rheology of continental lithosphere and seismic anisotropy","authors":"","doi":"10.1007/s11430-022-1171-3","DOIUrl":"https://doi.org/10.1007/s11430-022-1171-3","url":null,"abstract":"<h3>Abstract</h3> <p>Rheology of rocks controls the deformation of the Earth at various space-time scales, which is crucial to understand the tectonic evolution of continental lithosphere. Researches of rock rheology are mainly conducted via high-pressure and high-temperature rheological experiments and multi-scale observations and measurements of naturally deformed rocks. At present, a large amount of data from such kinds of studies have been accumulated. This paper first provides an up-to-date comprehensive review of the rheological mechanisms, fabric types and seismic properties of the main rock-forming minerals at different depths of continental lithosphere, including olivine, orthopyroxene, clinopyroxene, amphibole, plagioclase, quartz and mica. Then, progress in high-pressure and high-temperature experiments and natural deformation observations is introduced, mainly regarding the rheological strength and behavior, seismic velocity and anisotropy of lithospheric mantle peridotite, eclogite, mafic granulite, amphibolite and felsic rocks. Finally, by taking the Tibetan Plateau as an example, the application of rock rheology for quantitative interpretation of seismic anisotropy data is discussed. The combination of mineral deformation fabrics and seismic anisotropy is expected to make an important breakthrough in understanding the rheological properties and structure of continental lithosphere.</p>","PeriodicalId":21651,"journal":{"name":"Science China Earth Sciences","volume":"83 1","pages":""},"PeriodicalIF":5.7,"publicationDate":"2023-12-13","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"138681514","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"地球科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}