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Low-Dimensional Magnetism in Namibite Cu(BiO)2VO4OH 纳米石 Cu(BiO)2VO4OH 中的低维磁性
IF 1.1 4区 物理与天体物理 Q3 PHYSICS, MULTIDISCIPLINARY Pub Date : 2023-12-10 DOI: 10.1134/s1063776123100114
L. V. Shvanskaya, T. D. Bushneva, A. G. Ivanova, Z. V. Pchelkina, T. M. Vasil’chikova, O. S. Volokova, A. N. Vasil’ev

Abstract

A synthetic analog of rare secondary mineral namibite Cu(BiO)2VO4OH has been obtained by the hydrothermal method. The crystal structure of this compound contains isolated uniform chains of vertex-connected copper–oxygen octahedra. Magnetic susceptibility (χ) and magnetization (M) measurements have not indicated the long-range order in the temperature interval 2–300 K. Specific heat (Cp) measurements suggest the formation of a spin-liquid state at low temperatures. X-band electron paramagnetic resonance data recorded at low temperatures have demonstrated only a signal from impurities. First-principles calculations have estimated the exchange interaction in the chains as J = 555 K, whereas exchange interactions between the chains turn out to be one to two orders of magnitude smaller. Thus, namibite represents a rare example of an unordered half-integer spin chain.

摘要 通过水热法获得了稀有次生矿物纳米比石的合成类似物 Cu(BiO)2VO4OH。该化合物的晶体结构包含孤立的顶点连接的铜氧八面体均匀链。磁感应强度(χ)和磁化率(M)测量结果表明,在 2-300 K 的温度区间内不存在长程有序性。在低温下记录的 X 波段电子顺磁共振数据显示,只有杂质信号。第一原理计算估计链中的交换相互作用为 J = 555 K,而链之间的交换相互作用则小一到两个数量级。因此,namibite 是无序半整数自旋链的罕见实例。
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引用次数: 0
Propagation of a Laser-Induced Magnetostatic Wave Packet in a Pseudo Spin Valve in the Presence of Spin Pumping 存在自旋泵浦时激光诱导的磁静电波包在伪自旋阀中的传播
IF 1.1 4区 物理与天体物理 Q3 PHYSICS, MULTIDISCIPLINARY Pub Date : 2023-12-10 DOI: 10.1134/s1063776123100035
A. E. Fedianin, N. E. Khokhlov, A. M. Kalashnikova

Abstract

Spin pumping and angular momentum transfer, i.e., the emission of a spin current by a precessing magnetization and the reverse process of absorption, play an important role in coherent magnetic dynamics processes in multilayered structures. For ferromagnetic layers separated by a nonmagnetic interlayer these effects give rise to a dynamic coupling between the layers that is dissipative in nature and affects the damping of coherent magnetization precession. We have used micromagnetic simulations to analyze the influence of such a dynamic coupling on the propagation of a laser-induced surface magnetostatic wave (MSW) packet in a pseudo spin valve structure consisting of two ferromagnetic metallic layers separated by a nonmagnetic metallic interlayer. We have considered the MSW generation due to laser-induced heating, which leads to dynamic changes in magnetization and magnetic anisotropy, and added the dynamic coupling effect to the equations for our micromagnetic simulations. As a result, we have revealed that under certain conditions such a coupling leads to a decrease in the spatial damping of the wave packet that corresponds to the acoustic MSW mode forming in the structure considered.

摘要自旋抽运和角动量传递,即自旋电流通过预处理磁化的发射和反向吸收过程,在多层结构的相干磁动力学过程中发挥着重要作用。对于被非磁性夹层隔开的铁磁层,这些效应会引起层间的动态耦合,这种耦合具有耗散性质,会影响相干磁化前冲的阻尼。我们利用微磁模拟分析了这种动态耦合对激光诱导的表面磁静电波(MSW)包在伪自旋阀结构中传播的影响,该结构由两个被非磁性金属夹层隔开的铁磁性金属层组成。我们考虑了激光诱导加热导致磁化和磁各向异性动态变化而产生的 MSW,并在微磁模拟方程中加入了动态耦合效应。结果表明,在某些条件下,这种耦合会导致波包空间阻尼的减小,这与在所考虑的结构中形成的声 MSW 模式相对应。
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引用次数: 0
Specific Features of g ≈ 4.3 EPR Line Behavior in Magnetic Nanogranular Composites 磁性纳米粒状复合材料中 g ≈ 4.3 EPR 线行为的具体特征
IF 1.1 4区 物理与天体物理 Q3 PHYSICS, MULTIDISCIPLINARY Pub Date : 2023-12-10 DOI: 10.1134/s1063776123100023
A. B. Drovosekov, N. M. Kreines, D. A. Ziganurov, A. V. Sitnikov, S. N. Nikolaev, V. V. Rylkov

Abstract

Films of metal-insulator nanogranular composites MxD100 – x with different composition and percentage of metal and dielectric phases (M = Fe, Co, CoFeB; D = Al2O3, SiO2, LiNbO3; x ≈ 15–70 at %) are investigated by magnetic resonance in a wide range of frequencies (f = 7–37 GHz) and temperatures (T = 4.2–360 K). In addition to the usual ferromagnetic resonance signal from an array of nanogranules, the experimental spectra contain an additional absorption peak, which we associate with the electron paramagnetic resonance (EPR) of Fe and Co ions dispersed in the insulating space between the granules. In contrast to the traditional EPR of Fe and Co ions in weakly doped non-magnetic matrices, the observed peak demonstrates a number of unusual properties, which we explain by the presence of magnetic interactions between ions and granules.

摘要 通过磁共振研究了金属-绝缘体纳米粒状复合材料 MxD100 - x 薄膜,其金属和介电相(M = Fe、Co、CoFeB;D = Al2O3、SiO2、LiNbO3;x ≈ 15-70 at %)的组成和比例各不相同,频率(f = 7-37 GHz)和温度(T = 4.2-360 K)范围很广。除了来自纳米颗粒阵列的常规铁磁共振信号外,实验光谱还包含一个额外的吸收峰,我们将其与分散在颗粒之间绝缘空间的铁离子和钴离子的电子顺磁共振(EPR)联系起来。与传统的铁离子和钴离子在弱掺杂的非磁性基质中的电子顺磁共振不同,观察到的峰值显示出许多不寻常的特性,我们将其解释为离子和颗粒之间存在磁性相互作用。
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引用次数: 0
Influence of Impurities on Adhesion at the TiAl/Al2O3 Interface 杂质对TiAl/Al2O3界面附着力的影响
IF 1.1 4区 物理与天体物理 Q3 PHYSICS, MULTIDISCIPLINARY Pub Date : 2023-10-26 DOI: 10.1134/S1063776123090030
A. V. Bakulin, A. S. Kulkov, S. E. Kulkova

The influence of substitutional impurities on adhesion at the TiAl/Al2O3 interface with an oxygen termination has been studied by the projector augmented-wave method within the density functional theory. It has been shown that transition metals and a number of s,p-elements substituting for the interfacial titanium atom reduce adhesion, whereas Group VB and VIB elements enhance chemical bonding at the interface. The local densities of states, charge density distribution, overlap populations for interfacial atom bonding, and other electronic characteristics have been calculated that make it possible to reveal key factors influencing adhesion at the alloy–oxide interface. A correlation has been found between the influence of impurities on bonding energy at the inner and outer interfaces. A comparison of obtained data with those for the interface with Ti-enriched Ti3Al alloy shows that the interface loses strength with decreasing Ti content in the alloy.

用密度泛函理论中的投影增广波方法研究了取代杂质对氧终止TiAl/Al_2O_3界面粘附性的影响。已经表明,过渡金属和许多取代界面钛原子的s,p元素降低了粘附性,而VB族和VIB族元素增强了界面处的化学键合。已经计算了局部态密度、电荷密度分布、界面原子键的重叠布居和其他电子特性,这些特性使得揭示影响合金-氧化物界面粘附的关键因素成为可能。杂质对内外界面结合能的影响之间存在相关性。将获得的数据与富Ti Ti3Al合金界面的数据进行比较表明,界面强度随着合金中Ti含量的降低而降低。
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引用次数: 0
Periodic Variations of the Radon Concentration Measured by the Large Volume Detector at the Gran Sasso Underground Laboratory Gran Sasso地下实验室大体积探测器测量氡浓度的周期变化
IF 1.1 4区 物理与天体物理 Q3 PHYSICS, MULTIDISCIPLINARY Pub Date : 2023-10-26 DOI: 10.1134/S106377612309008X
N. Yu. Agafonova, E. A. Dobrynina, N. A. Filimonova, I. R. Shakiryanova

Time series of gamma-ray photons from natural radioactivity measured with the Large Volume Detector (LVD) at the Gran Sasso underground laboratory (Laboratori Nazionali del Gran Sasso, Italy) have been analyzed. The instrument is used to detect neutrinos from gravitational collapses of stellar cores in the Galaxy. The background of the experiment is due to neutrons and gamma-ray photons from the decays of daughter nuclei of uranium and thorium. An analysis of periodic variations of the number of gamma-ray photons caused by the radon concentration in the underground laboratory has shown the presence of diurnal, weekly, monthly, and annual modulations. Data collected from 2004 to 2021, including a period of low activity in the hall of the Gran Sasso laboratory during the COVID-19 pandemic, have been reported.

分析了在格兰萨索地下实验室(意大利格兰萨索国家实验室)用大体积探测器(LVD)测量的天然放射性伽马射线光子的时间序列。该仪器用于探测银河系恒星核心引力坍缩产生的中微子。实验的背景是铀和钍的子核衰变产生的中子和伽马射线光子。对地下实验室中氡浓度引起的伽马射线光子数量周期性变化的分析表明,存在昼夜、每周、每月和每年的调制。报告了2004年至2021年收集的数据,包括新冠肺炎大流行期间格兰萨索实验室大厅的低活动期。
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引用次数: 0
Verification of T Invariance in the Total Interaction Cross Section of Neutrons with Unpolarized Nuclei Using the Polarization–Asymmetry Theorem 用极化-不对称定理验证中子与非极化核全相互作用截面中的T不变性
IF 1.1 4区 物理与天体物理 Q3 PHYSICS, MULTIDISCIPLINARY Pub Date : 2023-10-26 DOI: 10.1134/S1063776123090066
V. R. Skoy

To date, the violation of T invariance (TI) has been experimentally established for the decays [J. H. Christenson et al., Phys. Rev. Lett. 13, 138 (1964)] and oscillations [A. Angelopoulos et al., Phys. Lett. B 444, 43 (1998)] of neutral kaons. Phenomenologically, TI violation in the system of neutral kaons is associated with the difference of the Kobayashi–Maskawa phase from zero (or from π) in the standard model of the electroweak interaction. For nucleon–nucleus interactions, this phase turns out to be very small [P. Herszeg, in Symmetries and Fundamental Interactions in Nuclei, World Scientific, Singapore (1995), p. 89)]. Estimates of the nucleon–nucleon matrix element corresponding to TI violation in various models are given in [V. Gudkov, in Fundamental Physics with Pulsed Neutron Beams, World Scientific, Singapore (2001), p. 117]. All these estimates are small and have a large spread. Therefore, the verification of TI in nuclear processes actually means a search for other mechanisms for its violation. Below is a description of the experimental methods for TI verification in the total interaction cross sections of low-energy resonance neutrons with unpolarized nuclei with the use of the polarization–asymmetry (PA) theorem.

到目前为止,已经通过实验确定了中性kaon的衰变[J.H.Christenson等人,Phys.Rev.Lett.13138(1964)]和振荡[A.A.Angelopoulos等人,Phys.Lett.B4444,43(1998)]对T不变性(TI)的破坏。在现象学上,中性kaons系统中的TI破坏与电弱相互作用标准模型中Kobayashi–Maskawa相与零(或π)的差异有关。对于核子-核相互作用,这一阶段被证明是非常小的[P.Herszeg,《核的对称性和基本相互作用》,世界科学,新加坡(1995),第89页]。[V.Gudkov,《脉冲中子束基础物理》,世界科技,新加坡(2001),第117页]中给出了各种模型中与TI违反相对应的核子-核子矩阵元素的估计。所有这些估计都很小,而且分布很大。因此,核查核进程中的TI实际上意味着寻找违反TI的其他机制。以下是使用极化-不对称性(PA)定理在低能共振中子与非极化核的总相互作用截面中验证TI的实验方法的描述。
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引用次数: 0
Coherent Backscattering Peak for Radiation with Low Spatial Coherence 低空间相干辐射的相干后向散射峰
IF 1.1 4区 物理与天体物理 Q3 PHYSICS, MULTIDISCIPLINARY Pub Date : 2023-10-26 DOI: 10.1134/S1063776123090108
V. L. Kuzmin, A. Yu. Valkov, Yu. A. Zhavoronkov

The theory is developed and numerical simulation is performed for the coherent backscattering effect in a strongly inhomogeneous random medium with a finite spatial coherence length. It is shown using the Monte Carlo method that the limitation imposed on the number of scattering events corresponds to lowering of incident radiation coherence and leads to angular broadening of the backscattering peak, extending the possibility of using coherent backscattering in biomedical applications. Based on the diagrammatic technique, the modeling of coherent backscattering is developed for the first time beyond the frames of the ladder approximation.

建立了具有有限空间相干长度的强非均匀随机介质中相干后向散射效应的理论,并对其进行了数值模拟。使用蒙特卡罗方法表明,对散射事件数量的限制对应于入射辐射相干性的降低,并导致后向散射峰值的角度加宽,从而扩展了在生物医学应用中使用相干后向散射的可能性。基于图解技术,首次在梯形近似的框架之外建立了相干后向散射的模型。
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引用次数: 0
Single Electron Capture in Collisions of Fast Ions with Molecular Hydrogen in the Impact Parameter Representation 冲击参数表示中快离子与分子氢碰撞中的单电子捕获
IF 1.1 4区 物理与天体物理 Q3 PHYSICS, MULTIDISCIPLINARY Pub Date : 2023-10-26 DOI: 10.1134/S1063776123090042
F. F. Goryaev

A theoretical method for evaluating the single-electron capture (SEC) cross sections in collisions of fast ions with a ground-state H2 molecule is presented. The scattering problem for ion-molecule collisions is formulated in the impact parameter representation using the relation between the quantum-mechanical amplitude and quasi-classical impact parameter one. The capture amplitudes and corresponding probabilities of capture to (nlm) states of an incident ion are derived within the framework of the Brinkman–Kramers approximation. The general expressions for the SEC probability amplitudes to n-states, summed over l and m quantum numbers, are deduced, from which the corresponding SEC probabilities can be then calculated using a procedure of multichannel normalization. The dependence of the differential cross sections, integrated over projectile impact parameters, on the molecular orientation for charge exchange in H+ + H2 collisions is considered and compared with measurements and other calculations. Total SEC cross sections, integrated over the molecular orientations and summed over n-states for several bare and dressed ions, are calculated and compared with available experimental data and results of calculations by means of other theoretical methods.

提出了一种计算快离子与基态H2分子碰撞时单电子捕获截面的理论方法。利用量子力学振幅与准经典碰撞参数之间的关系,在碰撞参数表示中公式化了离子-分子碰撞的散射问题。在Brinkman–Kramers近似的框架内导出了入射离子的捕获振幅和捕获到(nlm)态的相应概率。推导了在l和m个量子数上求和的n态SEC概率幅度的一般表达式,然后可以使用多通道归一化程序计算相应的SEC概率。考虑了H++H2碰撞中电荷交换的分子取向与微分横截面的相关性,并与测量和其他计算进行了比较。计算了几个裸离子和修饰离子在分子取向上积分和在n态上求和的总SEC截面,并通过其他理论方法与可用的实验数据和计算结果进行了比较。
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引用次数: 0
On Estimation Methods of Depolarization Losses for Ultracold Neutrons in Magnetic Traps 磁阱中超冷中子去极化损耗的估算方法
IF 1.1 4区 物理与天体物理 Q3 PHYSICS, MULTIDISCIPLINARY Pub Date : 2023-10-26 DOI: 10.1134/S1063776123090054
G. N. Klyushnikov, A. P. Serebrov

The problem of finding the depolarization losses of neutrons is investigated in connection with the need to determine the systematic error for experiments with magnetic storage of ultracold neutrons in traps. In this paper, we consider three methods to estimate the neutrons depolarization probability: classical, quantum mechanical and approximate one. They are used to estimate the depolarization probability of ultracold neutrons in two magnetic traps: the trap developed in Los Alamos National Laboratory (LANL) and the one designed in the neutron physics laboratory of “NRC Kurchatov Institute”—PNPI. It is shown that all three methods are successfully used to estimate depolarization. This is of particular importance to compare of theoretical predictions with the results of measurement in experiments to determine the neutron lifetime.

研究了寻找中子去极化损失的问题,同时需要确定超冷中子在陷阱中磁存储实验的系统误差。本文考虑了三种估计中子去极化概率的方法:经典方法、量子力学方法和近似方法。它们被用来估计超冷中子在两个磁阱中的去极化概率:洛斯阿拉莫斯国家实验室(LANL)开发的阱和“NRC库尔恰托夫研究所”中子物理实验室设计的阱——PNPI。结果表明,这三种方法都能成功地用于估计去极化。这对于将理论预测与实验中的测量结果进行比较以确定中子寿命具有特别重要的意义。
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引用次数: 0
Jahn–Teller Ordering Dynamics in the Paraelectric BiMn7O12 Phase: 57Fe Probe Mössbauer Diagnostics 准电BiMn7O12相中的Jahn–Teller有序动力学:57Fe探针Mössbauer诊断
IF 1.1 4区 物理与天体物理 Q3 PHYSICS, MULTIDISCIPLINARY Pub Date : 2023-10-26 DOI: 10.1134/S1063776123090145
A. V. Sobolev, V. I. Nitsenko, A. A. Belik, I. S. Glazkova, M. S. Kondratyeva, I. A. Presniakov

The electrical hyperfine interactions of the 57Fe probe nuclei stabilized in the structure of the BiMn7O12 manganite are studied by Mössbauer spectroscopy. Mössbauer spectra are measured in the para-electric temperature range, which includes the structural phase transitions I2/mIm(bar {3}) (T1 ≈ 600 K) and Im ↔ I2/m (T2 ≈ 450 K). The calculation of the parameters of the electric field gradient tensor with allowance for the dipole contributions of Bi3+ cations in the range of the first phase transition allowed us to confirm a random orientation of the dipole moments pBi in the cubic phase of the manganite (Im(bar {3})). Based on an analysis of the Mössbauer spectra recorded at T2 < T < T1, we considered various scenarios for the manifestation of the dynamic Jahn–Teller effect, which leads to the “melting” of the orbital order in the manganese sublattice, in terms of a two-level relaxation model.

用穆斯堡尔谱研究了BiMn7O12亚锰酸盐结构中稳定的57Fe探针核的超精细电相互作用。穆斯堡尔谱是在准电温度范围内测量的,其中包括结构相变I2/M↔ Im(bar{3})(T1≈600 K)和Im↔ I2/m(T2≈450 K)。考虑到Bi3+阳离子在第一相变范围内的偶极贡献,计算电场梯度张量的参数使我们能够确认锰酸盐立方相中偶极矩pBi的随机取向(Im(bar{3}))。基于对在T2<;T<;T1,我们考虑了动态Jahn–Teller效应表现的各种场景,该效应导致锰亚晶格中轨道序的“熔化”,根据两能级弛豫模型。
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引用次数: 0
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