Pub Date : 2024-01-12DOI: 10.1134/S1063776123110122
D. P. Agapov, I. V. Belovolov, S. A. Magnitskii, D. N. Frolovtsev, A. S. Chirkin
The possibility of obtaining an object image using a fiber-optic endoscope based on ghost imaging principle is demonstrated experimentally. The endoscope consists of a multimode fiber and includes a radiation source with thermal statistics, which is formed by means of random modulation of He–Ne laser radiation with the help of a phase spatial light modulator. It is shown that after the passage through the fiber, the field preserves the pseudo-thermal statistics. Radiation obtained in this way is used for ghost imaging in transmitted as well as scattered light.
{"title":"Ghost Imaging in a Fiber-Optic Endoscope Based on Light Scattering","authors":"D. P. Agapov, I. V. Belovolov, S. A. Magnitskii, D. N. Frolovtsev, A. S. Chirkin","doi":"10.1134/S1063776123110122","DOIUrl":"10.1134/S1063776123110122","url":null,"abstract":"<p>The possibility of obtaining an object image using a fiber-optic endoscope based on ghost imaging principle is demonstrated experimentally. The endoscope consists of a multimode fiber and includes a radiation source with thermal statistics, which is formed by means of random modulation of He–Ne laser radiation with the help of a phase spatial light modulator. It is shown that after the passage through the fiber, the field preserves the pseudo-thermal statistics. Radiation obtained in this way is used for ghost imaging in transmitted as well as scattered light.</p>","PeriodicalId":629,"journal":{"name":"Journal of Experimental and Theoretical Physics","volume":"137 5","pages":"622 - 629"},"PeriodicalIF":1.0,"publicationDate":"2024-01-12","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"139462229","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2024-01-12DOI: 10.1134/S1063776123110079
A. Ya. Maltsev
We consider the Lifshitz topological transitions and the corresponding changes in the galvano-magnetic properties of a metal from the point of view of the general classification of open electron trajectories arising on Fermi surfaces of arbitrary complexity in the presence of magnetic field. The construction of such a classification is the content of the Novikov problem and is based on the division of non-closed electron trajectories into topologically regular and chaotic trajectories. The description of stable topologically regular trajectories gives a basis for a complete classification of non-closed trajectories on arbitrary Fermi surfaces and is connected with special topological structures on these surfaces. Using this description, we describe here the distinctive features of possible changes in the picture of electron trajectories during the Lifshitz transitions, as well as changes in the conductivity behavior in the presence of a strong magnetic field. As it turns out, the use of such an approach makes it possible to describe not only the changes associated with stable electron trajectories, but also the most general changes of the conductivity diagram in strong magnetic fields.
{"title":"Lifshitz Transitions and Angular Conductivity Diagrams in Metals with Complex Fermi Surfaces","authors":"A. Ya. Maltsev","doi":"10.1134/S1063776123110079","DOIUrl":"10.1134/S1063776123110079","url":null,"abstract":"<p>We consider the Lifshitz topological transitions and the corresponding changes in the galvano-magnetic properties of a metal from the point of view of the general classification of open electron trajectories arising on Fermi surfaces of arbitrary complexity in the presence of magnetic field. The construction of such a classification is the content of the Novikov problem and is based on the division of non-closed electron trajectories into topologically regular and chaotic trajectories. The description of stable topologically regular trajectories gives a basis for a complete classification of non-closed trajectories on arbitrary Fermi surfaces and is connected with special topological structures on these surfaces. Using this description, we describe here the distinctive features of possible changes in the picture of electron trajectories during the Lifshitz transitions, as well as changes in the conductivity behavior in the presence of a strong magnetic field. As it turns out, the use of such an approach makes it possible to describe not only the changes associated with stable electron trajectories, but also the most general changes of the conductivity diagram in strong magnetic fields.</p>","PeriodicalId":629,"journal":{"name":"Journal of Experimental and Theoretical Physics","volume":"137 5","pages":"706 - 724"},"PeriodicalIF":1.0,"publicationDate":"2024-01-12","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"139465276","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2024-01-12DOI: 10.1134/S1063776123110110
A. D. Sukhov, A. G. Petrov
We consider fluid flow with a free boundary, which is defined as a function of height from coordinate x with two asymptotes at positive and negative infinities (hydraulic jump). The Boussinesq approximation is used to describe the phenomenon, and an additional force is introduced. The force is chosen to depend only on the height of the surface. The problem is solved analytically without using numerical schemes. This technique is used to determine the jump surface and the acting force depending on the wave propagation coordinate.
摘要 我们考虑了具有自由边界的流体流动,自由边界被定义为坐标 x 高度的函数,在正无穷大和负无穷大处有两个渐近线(水力跃迁)。我们采用布森斯克近似来描述这一现象,并引入了一个附加力。该力只取决于表面的高度。该问题采用分析方法求解,不使用数值方案。该技术用于确定跃迁面以及取决于波传播坐标的作用力。
{"title":"Hydraulic Jump for Planar and Axisymmetric Flow of a Fluid Layer","authors":"A. D. Sukhov, A. G. Petrov","doi":"10.1134/S1063776123110110","DOIUrl":"10.1134/S1063776123110110","url":null,"abstract":"<p>We consider fluid flow with a free boundary, which is defined as a function of height from coordinate <i>x</i> with two asymptotes at positive and negative infinities (hydraulic jump). The Boussinesq approximation is used to describe the phenomenon, and an additional force is introduced. The force is chosen to depend only on the height of the surface. The problem is solved analytically without using numerical schemes. This technique is used to determine the jump surface and the acting force depending on the wave propagation coordinate.</p>","PeriodicalId":629,"journal":{"name":"Journal of Experimental and Theoretical Physics","volume":"137 5","pages":"725 - 731"},"PeriodicalIF":1.0,"publicationDate":"2024-01-12","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"139465349","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2023-12-10DOI: 10.1134/S1063776123100138
V. V. Val’kov
The effective the two-band Hamiltonian is obtained for iridium oxides with account for strong electron correlations (SEC) and the spin–orbit interaction. The intraatomic electron correlations in iridium ions induce the formation of Hubbard fermions (HF) filling the states in the valence band. Another consequence of SEC is associated with the emergence of the antiferromagnetic (AFM) exchange interaction between HF in accordance with the Anderson mechanism. As a result, a long-range antiferromagnetic order is established in the system, and in the conditions of band overlapping, the intersite Coulomb interaction induces a phase transition to the excitonic insulator (EI) state with a long-range AFM order. The system of integral self-consistent equations, the solution to which determines the excitonic order parameter components Δi,j(k), sublattice magnetization M, Hubbard fermion concentration nd, and chemical potential μ, is obtained using the atomic representation, the method of two-time temperature Green’s functions, and the Zwanzig–Mori projection technique. The symmetry classification of AFM EI phases is performed, and it is shown that in the nearest neighbor approximation, state Δi,j(k) with the s-type symmetry corresponds to the ground state, while the phases with the d- and p-symmetries are metastable.
摘要 在考虑强电子关联(SEC)和自旋轨道相互作用的情况下,得到了铱氧化物的有效两带哈密顿。铱离子中的原子内电子相关诱导形成了填充价带状态的哈伯德费米子(HF)。根据安德森机制,SEC 的另一个结果与 HF 之间出现的反铁磁(AFM)交换相互作用有关。因此,在系统中建立了长程反铁磁阶,在能带重叠的条件下,场内库仑相互作用诱导了向具有长程 AFM 阶的激子绝缘体(EI)态的相变。利用原子表示法、双时间温度格林函数法和 Zwanzig-Mori 投影技术,得到了积分自洽方程组,该方程组的解决定了激子阶参数分量 Δi、j(k)、亚晶格磁化 M、哈伯德费米子浓度 nd 和化学势 μ。对 AFM EI 相进行了对称性分类,结果表明,在近邻近似中,具有 s 型对称性的态Δi, j(k)对应于基态,而具有 d 型和 p 型对称性的相则是可转移的。
{"title":"Antiferromagnetic Excitonic Insulator","authors":"V. V. Val’kov","doi":"10.1134/S1063776123100138","DOIUrl":"10.1134/S1063776123100138","url":null,"abstract":"<p>The effective the two-band Hamiltonian is obtained for iridium oxides with account for strong electron correlations (SEC) and the spin–orbit interaction. The intraatomic electron correlations in iridium ions induce the formation of Hubbard fermions (HF) filling the states in the valence band. Another consequence of SEC is associated with the emergence of the antiferromagnetic (AFM) exchange interaction between HF in accordance with the Anderson mechanism. As a result, a long-range antiferromagnetic order is established in the system, and in the conditions of band overlapping, the intersite Coulomb interaction induces a phase transition to the excitonic insulator (EI) state with a long-range AFM order. The system of integral self-consistent equations, the solution to which determines the excitonic order parameter components Δ<sub><i>i</i>,</sub> <sub><i>j</i></sub>(<i>k</i>), sublattice magnetization <i>M</i>, Hubbard fermion concentration <i>n</i><sub><i>d</i></sub>, and chemical potential μ, is obtained using the atomic representation, the method of two-time temperature Green’s functions, and the Zwanzig–Mori projection technique. The symmetry classification of AFM EI phases is performed, and it is shown that in the nearest neighbor approximation, state Δ<sub><i>i</i>,</sub> <sub><i>j</i></sub>(<i>k</i>) with the <i>s</i>-type symmetry corresponds to the ground state, while the phases with the <i>d</i>- and <i>p</i>-symmetries are metastable.</p>","PeriodicalId":629,"journal":{"name":"Journal of Experimental and Theoretical Physics","volume":"137 :","pages":"474 - 485"},"PeriodicalIF":0.8,"publicationDate":"2023-12-10","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"138569798","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2023-12-10DOI: 10.1134/S1063776123100060
M. A. Morozova, O. V. Matveev, D. V. Romanenko, S. A. Nikitov
The influence of double (electrical and magnetic) nonlinearity on the Bragg resonances of the hybrid electromagnetic-spin waves in a multiferroic crystal has been theoretically and experimentally revealed. The multiferroic crystal consists of an yttrium iron garnet layer with a periodic system of grooves on the surface and a ferroelectric strontium–barium titanate layer. A dispersion relation for the hybrid waves is obtained, and the mechanism of formation of main and hybrid band gaps, namely, suppression bands, is revealed. It is shown that taking into account the magnetic nonlinearity leads to frequency rearrangement of both band gaps and taking into account the electrical nonlinearity leads to frequency rearrangement of only the hybrid band gap. In the general case, the effects of the electrical and magnetic nonlinearities on the hybrid band gap can be compensated.
{"title":"Bragg Resonances in a Multiferroic Double-Nonlinearity Crystal","authors":"M. A. Morozova, O. V. Matveev, D. V. Romanenko, S. A. Nikitov","doi":"10.1134/S1063776123100060","DOIUrl":"10.1134/S1063776123100060","url":null,"abstract":"<p>The influence of double (electrical and magnetic) nonlinearity on the Bragg resonances of the hybrid electromagnetic-spin waves in a multiferroic crystal has been theoretically and experimentally revealed. The multiferroic crystal consists of an yttrium iron garnet layer with a periodic system of grooves on the surface and a ferroelectric strontium–barium titanate layer. A dispersion relation for the hybrid waves is obtained, and the mechanism of formation of main and hybrid band gaps, namely, suppression bands, is revealed. It is shown that taking into account the magnetic nonlinearity leads to frequency rearrangement of both band gaps and taking into account the electrical nonlinearity leads to frequency rearrangement of only the hybrid band gap. In the general case, the effects of the electrical and magnetic nonlinearities on the hybrid band gap can be compensated.</p>","PeriodicalId":629,"journal":{"name":"Journal of Experimental and Theoretical Physics","volume":"137 :","pages":"432 - 441"},"PeriodicalIF":0.8,"publicationDate":"2023-12-10","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"138562143","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2023-12-10DOI: 10.1134/S1063776123100126
V. V. Ustinov, I. A. Yasyulevich
We construct a nonlinear theory of electric resistance of chiral helimagnets, in which the shape changes and the magnetization spiral starts rotating during the passage of electric current due to the spin transfer torque effect. It is shown that the rotation of the spin spiral under the action of the passing current, the electric resistance of the helimagnet is always lower than the resistance of a helimagnet in which the spin spiral is stationary. It is found that the current–voltage characteristic of the helimagnet in the presence of the spin transfer torque from the conduction electron system to the system of localized electrons can be essentially nonlinear. The possibility of the spin electric bistability effect in helimagnets is predicted for the situation when the spin contribution to electric resistance of a helimagnet can take two different values for the same value of the current passing through it. The possibility of realization of states with a negative differential resistance in helimagnets is demonstrated.
{"title":"Spin Transfer Torque and Nonlinear Quantum Electron Transport in Chiral Helimagnets","authors":"V. V. Ustinov, I. A. Yasyulevich","doi":"10.1134/S1063776123100126","DOIUrl":"10.1134/S1063776123100126","url":null,"abstract":"<p>We construct a nonlinear theory of electric resistance of chiral helimagnets, in which the shape changes and the magnetization spiral starts rotating during the passage of electric current due to the spin transfer torque effect. It is shown that the rotation of the spin spiral under the action of the passing current, the electric resistance of the helimagnet is always lower than the resistance of a helimagnet in which the spin spiral is stationary. It is found that the current–voltage characteristic of the helimagnet in the presence of the spin transfer torque from the conduction electron system to the system of localized electrons can be essentially nonlinear. The possibility of the spin electric bistability effect in helimagnets is predicted for the situation when the spin contribution to electric resistance of a helimagnet can take two different values for the same value of the current passing through it. The possibility of realization of states with a negative differential resistance in helimagnets is demonstrated.</p>","PeriodicalId":629,"journal":{"name":"Journal of Experimental and Theoretical Physics","volume":"137 :","pages":"422 - 431"},"PeriodicalIF":0.8,"publicationDate":"2023-12-10","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"138561882","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2023-12-10DOI: 10.1134/S1063776123100187
M. A. Kuznetsov, A. A. Fraerman
It is shown that the energy of a ferromagnetic film deposited onto a paramagnetic or superconducting substrate acquires a contribution in the form of the Dzyaloshinskii–Moriya interaction. This contribution appears as a result of the magnetostatic interaction of the magnetization of the ferromagnetic film with the magnetization induced by it in a paramagnet or by the supercurrent in the superconductor and leads to the removal of the chiral degeneracy, nonreciprocity of spin waves, and the formation of chiral states such as magnetic skyrmions. Our estimates indicate the possibility of experimental observation of predicted effects.
{"title":"Magnetostatic Mechanism of Chiral Symmetry Breaking in Multilayer Magnetic Structures","authors":"M. A. Kuznetsov, A. A. Fraerman","doi":"10.1134/S1063776123100187","DOIUrl":"10.1134/S1063776123100187","url":null,"abstract":"<p>It is shown that the energy of a ferromagnetic film deposited onto a paramagnetic or superconducting substrate acquires a contribution in the form of the Dzyaloshinskii–Moriya interaction. This contribution appears as a result of the magnetostatic interaction of the magnetization of the ferromagnetic film with the magnetization induced by it in a paramagnet or by the supercurrent in the superconductor and leads to the removal of the chiral degeneracy, nonreciprocity of spin waves, and the formation of chiral states such as magnetic skyrmions. Our estimates indicate the possibility of experimental observation of predicted effects.</p>","PeriodicalId":629,"journal":{"name":"Journal of Experimental and Theoretical Physics","volume":"137 :","pages":"442 - 452"},"PeriodicalIF":0.8,"publicationDate":"2023-12-10","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"139329164","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2023-12-10DOI: 10.1134/S1063776123100011
K. N. Boldyrev, M. Diab, I. A. Gudim, M. N. Popova
The high-resolution optical absorption spectra of NdFe3(BO3)4 single crystals have been recorded at temperatures from 4 to 40 K in the IR range of f–f transitions in a Nd3+ ion. Light linearly polarized at different angles to the C2 axes in the basal plane has been passed along the trigonal C3 axis. Below the temperature of magnetic moment ordering into a collinear antiferromagnetic structure (TN ≈ 30 K), dichroism, that is, the absorption versus polarization dependence, arises. The temperature and angular dependences of dichroism indicate that the magnetic moments of iron are directed along the C2 axes up to about 17 K, the number of domains with variously directed C2 axes being different. The mechanism of linear dichroism has been discussed. Below 17 K, a smooth transition to the helicoidal magnetic phase has been observed, with the collinear phase coexisting with the helicoidal one. Data presented in this article contradict the earlier concept of magnetic moments fluctuating in the low-temperature phase near the C2 axis within the ±10° interval.
{"title":"Optical Linear Dichroism in the ab-Plane of NdFe3(BO3)4 Ferroborate","authors":"K. N. Boldyrev, M. Diab, I. A. Gudim, M. N. Popova","doi":"10.1134/S1063776123100011","DOIUrl":"10.1134/S1063776123100011","url":null,"abstract":"<p>The high-resolution optical absorption spectra of NdFe<sub>3</sub>(BO<sub>3</sub>)<sub>4</sub> single crystals have been recorded at temperatures from 4 to 40 K in the IR range of <i>f</i>–<i>f</i> transitions in a Nd<sup>3+</sup> ion. Light linearly polarized at different angles to the <i>C</i><sub>2</sub> axes in the basal plane has been passed along the trigonal <i>C</i><sub>3</sub> axis. Below the temperature of magnetic moment ordering into a collinear antiferromagnetic structure (<i>T</i><sub>N</sub> ≈ 30 K), dichroism, that is, the absorption versus polarization dependence, arises. The temperature and angular dependences of dichroism indicate that the magnetic moments of iron are directed along the <i>C</i><sub>2</sub> axes up to about 17 K, the number of domains with variously directed <i>C</i><sub>2</sub> axes being different. The mechanism of linear dichroism has been discussed. Below 17 K, a smooth transition to the helicoidal magnetic phase has been observed, with the collinear phase coexisting with the helicoidal one. Data presented in this article contradict the earlier concept of magnetic moments fluctuating in the low-temperature phase near the <i>C</i><sub>2</sub> axis within the ±10° interval.</p>","PeriodicalId":629,"journal":{"name":"Journal of Experimental and Theoretical Physics","volume":"137 :","pages":"486 - 491"},"PeriodicalIF":0.8,"publicationDate":"2023-12-10","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"138569413","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2023-12-10DOI: 10.1134/S1063776123100096
D. V. Popov, R. G. Batulin, M. A. Cherosov, I. V. Yatsyk, T. I. Chupakhina, Yu. A. Deeva, I. I. Fazlizhanov, R. M. Eremina, T. Maiti
A double perovskite Sr2CrNbO6 powder compound was studied by using X-ray diffraction, AC and DC magnetization, and ESR measurements. Two transitions in antiferromagnetically ordered regimes were observed through magnetization measurements at T = 5 and 2 K and were confirmed by the linear dependence of the magnetization on the applied magnetic field at these temperatures, approximations of the temperature dependence of the ESR linewidth, and AC magnetization. The zero field cooling curve was approximated by Bonner–Fisher law for quasi one dimensional chain with the exchange integral J/kB = 1 K between chromium spins. An approximation of linear part of magnetic susceptibility temperature dependence was performed using Curie–Weiss law. To describe the obtained effective moment μeff = 3.577μB, the presence Cr3+ and Cr4+ ions is estimated at a respective ratio about 0.8 : 0.2.
{"title":"Magnetic Properties of the Double Perovskite Sr2CrNbO6","authors":"D. V. Popov, R. G. Batulin, M. A. Cherosov, I. V. Yatsyk, T. I. Chupakhina, Yu. A. Deeva, I. I. Fazlizhanov, R. M. Eremina, T. Maiti","doi":"10.1134/S1063776123100096","DOIUrl":"10.1134/S1063776123100096","url":null,"abstract":"<p>A double perovskite Sr<sub>2</sub>CrNbO<sub>6</sub> powder compound was studied by using X-ray diffraction, AC and DC magnetization, and ESR measurements. Two transitions in antiferromagnetically ordered regimes were observed through magnetization measurements at <i>T</i> = 5 and 2 K and were confirmed by the linear dependence of the magnetization on the applied magnetic field at these temperatures, approximations of the temperature dependence of the ESR linewidth, and AC magnetization. The zero field cooling curve was approximated by Bonner–Fisher law for quasi one dimensional chain with the exchange integral <i>J</i>/<i>k</i><sub>B</sub> = 1 K between chromium spins. An approximation of linear part of magnetic susceptibility temperature dependence was performed using Curie–Weiss law. To describe the obtained effective moment μ<sub>eff</sub> = 3.577μ<sub>B</sub>, the presence Cr<sup>3+</sup> and Cr<sup>4+</sup> ions is estimated at a respective ratio about 0.8 : 0.2.</p>","PeriodicalId":629,"journal":{"name":"Journal of Experimental and Theoretical Physics","volume":"137 :","pages":"555 - 561"},"PeriodicalIF":0.8,"publicationDate":"2023-12-10","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"138569540","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2023-12-10DOI: 10.1134/S1063776123100175
Yu. S. Gokhfeld, N. V. Kazak, N. A. Bel’skaya, M. S. Molokeev, I. A. Gudim, O. A. Kondratiev, E. V. Eremin, Yu. V. Knyazev, D. A. Velikanov, S. G. Ovchinnikov
Cu2FeBO5 ludwigite single crystals have been grown from a solution–melt by spontaneous crystallization. Using the X-ray diffraction method, the crystal structure has been resolved in detail. Cations in sites M2, M3, and M4 have turned out to be structurally disordered. It has been found that oxygen atoms are disordered in one of five nonequivalent sites (O4). As can be seen from Mössbauer spectroscopy data, Fe3+ ions occupy four nonequivalent sites with different distortions of coordination octahedra. In the temperature range 40 K ≤ T ≤ 300 K, the spectra represent a superposition of quadrupole doublets. Static susceptibility measurements have revealed two magnetic features at T1 = 35 K and T2 = 20 K and spin-glass effects. Specific heat measurements in the interval 4–300 K have not discovered magnetic-transition-related anomalies.
摘要 通过自发结晶,从溶液熔体中生长出了 Cu2FeBO5 绿泥石单晶。利用 X 射线衍射方法详细解析了晶体结构。结果表明,位于 M2、M3 和 M4 位点的阳离子在结构上是无序的。研究还发现,氧原子在五个非等价位点(O4)中的一个位点处于无序状态。从莫斯鲍尔光谱数据可以看出,Fe3+ 离子占据了四个非等价位点,配位八面体的畸变程度各不相同。在 40 K ≤ T ≤ 300 K 的温度范围内,光谱代表了四极双重的叠加。静态磁感应强度测量显示了在 T1 = 35 K 和 T2 = 20 K 时的两个磁性特征以及自旋玻璃效应。4-300 K区间的比热测量没有发现与磁转变有关的异常现象。
{"title":"Structural Disorder, Specific Heat, and Magnetic Transitions in Cu2FeBO5","authors":"Yu. S. Gokhfeld, N. V. Kazak, N. A. Bel’skaya, M. S. Molokeev, I. A. Gudim, O. A. Kondratiev, E. V. Eremin, Yu. V. Knyazev, D. A. Velikanov, S. G. Ovchinnikov","doi":"10.1134/S1063776123100175","DOIUrl":"10.1134/S1063776123100175","url":null,"abstract":"<p>Cu<sub>2</sub>FeBO<sub>5</sub> ludwigite single crystals have been grown from a solution–melt by spontaneous crystallization. Using the X-ray diffraction method, the crystal structure has been resolved in detail. Cations in sites M2, M3, and M4 have turned out to be structurally disordered. It has been found that oxygen atoms are disordered in one of five nonequivalent sites (O4). As can be seen from Mössbauer spectroscopy data, Fe<sup>3+</sup> ions occupy four nonequivalent sites with different distortions of coordination octahedra. In the temperature range 40 K ≤ <i>T</i> ≤ 300 K, the spectra represent a superposition of quadrupole doublets. Static susceptibility measurements have revealed two magnetic features at <i>T</i><sub>1</sub> = 35 K and <i>T</i><sub>2</sub> = 20 K and spin-glass effects. Specific heat measurements in the interval 4–300 K have not discovered magnetic-transition-related anomalies.</p>","PeriodicalId":629,"journal":{"name":"Journal of Experimental and Theoretical Physics","volume":"137 :","pages":"494 - 505"},"PeriodicalIF":0.8,"publicationDate":"2023-12-10","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"138569539","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}