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Fundamentals governing membrane engineering 膜工程基本原理
IF 24.1 Pub Date : 2026-02-23 DOI: 10.1038/s44221-026-00603-2
The design of separation membranes depends on accurately interpreting transport processes, making this a timely moment to reassess the models and simulations used in such studies and to consider more optimal approaches.
分离膜的设计依赖于对传输过程的准确解释,这是重新评估此类研究中使用的模型和模拟并考虑更优化方法的及时时机。
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引用次数: 0
A systematic review of Indigenous peoples’ participation in dominant systems of water governance 对土著人民参与主要水管理系统的系统审查
IF 24.1 Pub Date : 2026-02-18 DOI: 10.1038/s44221-025-00580-y
Laila Kasuri, Sam Watkins, Alexandra M. Collins
Indigenous peoples’ rights and responsibilities to water are routinely undermined by dominant or colonial water governance systems. Although the importance of engaging Indigenous peoples in water governance is recognized, few studies have assessed the extent or nature of their participation. Here we present a systematic review of peer-reviewed literature on Indigenous participation in dominant water governance, analysing 226 journal articles and 183 case studies. Case studies span 15 countries, with the majority (77%) from Western settler-colonial countries. Forms of participation differ across regions, and some decision-making scales are better studied than others. Few participatory processes give consideration to Indigenous values and knowledge, and even fewer evaluate Indigenous participation, making it difficult to determine whether such participation was meaningful. Participation in international water governance processes is evident but remains underexamined in the literature. Crucially, Indigenous peoples are influencing and reshaping dominant water governance at all levels. Participation is widely recognized as essential for effective water governance, with growing interest in the meaningful inclusion of Indigenous peoples in decision-making. A global systematic review reveals key trends and gaps: research is concentrated in settler-colonial contexts and local scales, while reporting on procedural quality and consideration of Indigenous knowledge and values remains limited.
土著人民对水的权利和责任经常受到主导或殖民水治理系统的破坏。虽然认识到土著人民参与水治理的重要性,但很少有研究评估他们参与的程度或性质。在这里,我们对同行评议的土著参与主导水治理的文献进行了系统回顾,分析了226篇期刊文章和183个案例研究。案例研究横跨15个国家,其中大多数(77%)来自西方移民-殖民国家。参与的形式因地区而异,一些决策尺度比其他决策尺度得到了更好的研究。很少有参与性进程考虑到土著的价值和知识,评价土著参与的进程就更少了,因此很难确定这种参与是否有意义。参与国际水治理进程是显而易见的,但在文献中仍未得到充分审查。至关重要的是,土著人民正在影响和重塑各级占主导地位的水治理。人们普遍认为,参与是有效的水治理的必要条件,人们越来越关心土著人民有意义地参与决策。全球系统审查揭示了主要趋势和差距:研究集中在定居者-殖民地背景和地方规模,而关于程序质量和考虑土著知识和价值观的报告仍然有限。
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引用次数: 0
A multiscale perspective for understanding transport mechanisms in desalination and ion-selective membranes 从多尺度角度理解脱盐和离子选择膜的传输机制
IF 24.1 Pub Date : 2026-02-17 DOI: 10.1038/s44221-026-00585-1
Hanqing Fan, Makenna Parkinson, Kumar Varoon Agrawal, Mihail Barboiu, Lydéric Bocquet, Bezawit A. Getachew, Qilin Li, Ying Li, Shihong Lin, Chong Liu, Aleksandr Noy, Boya Radha, Dietmar Schwahn, Anthony Szymczyk, Menachem Elimelech
Membranes with nanometre- and subnanometre-scale pores play a vital role in aqueous separations across applications ranging from desalination and wastewater reuse to resource recovery and green hydrogen production. Despite their widespread use, the molecular-level mechanisms that govern water and solute transport in these membranes remain inadequately understood. In this Perspective, we examine advances in membrane and nanochannel transport across macroscopic, microscopic and molecular scales to establish a unified mechanistic framework. We begin by analysing current macroscopic models, highlighting their simplifying assumptions and inherent limitations. We then explore insights from nano- and ångström-scale fluidic studies, revealing unconventional transport phenomena that are not captured by classical continuum theories. Next, we describe how molecular simulations offer atomistic resolution of transport processes, providing mechanistic insight into how water and ions traverse the dynamic, heterogeneous porous networks of real-world, state-of-the-art polymer membranes. Finally, we discuss how to integrate these molecular, microscopic and macroscopic scales to advance theoretical understanding and inform the rational design of next-generation membranes. We conclude by identifying key knowledge gaps and outlining emerging opportunities to bridge scales through advanced characterization techniques and multiscale modelling. This Perspective explores the multiscale transport mechanisms of water and solutes in desalination and ion selective membranes, offering mechanistic insights to guide the design of next-generation membranes and nanoporous systems for applications in water purification, separations, and energy technologies.
具有纳米级和亚纳米级孔隙的膜在水分离中发挥着至关重要的作用,从海水淡化、废水回用到资源回收和绿色制氢。尽管它们被广泛使用,但控制这些膜中水和溶质运输的分子水平机制仍然没有得到充分的了解。从这个角度来看,我们研究了膜和纳米通道运输在宏观、微观和分子尺度上的进展,以建立统一的机制框架。我们首先分析当前的宏观模型,强调其简化的假设和固有的局限性。然后,我们探索纳米和ångström-scale流体研究的见解,揭示了经典连续介质理论未捕获的非常规传输现象。接下来,我们描述了分子模拟如何提供传输过程的原子分辨率,为水和离子如何穿越现实世界中最先进的聚合物膜的动态,非均质多孔网络提供了机制见解。最后,我们讨论了如何整合这些分子,微观和宏观尺度,以推进理论认识和指导下一代膜的合理设计。最后,我们确定了关键的知识差距,并概述了通过先进的表征技术和多尺度建模来弥合规模的新机会。本展望探讨了海水淡化和离子选择膜中水和溶质的多尺度传输机制,为指导下一代膜和纳米孔系统的设计提供了机制见解,用于水净化、分离和能源技术。
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引用次数: 0
Distilling hydrological and land-surface model parameters from physio-geographical properties using text-generating AI 使用文本生成人工智能从自然地理属性中提取水文和陆地表面模型参数
IF 24.1 Pub Date : 2026-02-13 DOI: 10.1038/s44221-026-00583-3
Moritz Feigl, Mathew Herrnegger, Karsten Schulz
Estimating parameters for distributed hydrological and land-surface models is challenging, particularly in regions with limited observational data. One possible approach uses transfer functions that relate catchment attributes to model parameters, but these functions have so far been largely specified by hand, limiting flexibility and their practical use. Here we show that variational autoencoders can be used as text-generating models to automatically derive interpretable parameter transfer functions. This approach reformulates equation discovery as an optimization problem in a continuous latent space, improving both efficiency and transparency. We evaluate the method in a prediction-in-ungauged-basins setting using the mesoscale Hydrological Model across 162 German basins. The resulting transfer functions lead to improved runoff predictions compared with established regionalization methods and regional long short-term memory networks. In addition, the learned functions are robust across catchments, scalable to large spatial domains and maintain physical interpretability. These results demonstrate a pathway towards more transparent and transferable parameter estimation for large-scale process-based environmental models. Estimating parameters for distributed hydrological models is challenging, especially in regions with limited data. Here the authors employ variational autoencoders to generate optimal parameter transfer functions, enhancing runoff predictions in ungauged basins and advancing the interpretability and scalability of environmental modelling.
估计分布式水文和陆地表面模型的参数具有挑战性,特别是在观测数据有限的地区。一种可能的方法是使用将集水区属性与模型参数关联起来的传递函数,但这些函数迄今为止主要是手工指定的,限制了灵活性和实际应用。在这里,我们展示了变分自编码器可以作为文本生成模型来自动导出可解释的参数传递函数。这种方法将方程发现重新表述为连续潜在空间中的优化问题,提高了效率和透明度。我们利用162个德国流域的中尺度水文模型评估了该方法在未测量流域的预测设置。与已建立的区划方法和区域长短期记忆网络相比,所得到的传递函数导致径流预测的改进。此外,学习到的函数在集水区具有鲁棒性,可扩展到大空间域并保持物理可解释性。这些结果为大规模基于过程的环境模型的更透明和可转移的参数估计提供了一条途径。估计分布式水文模型的参数是具有挑战性的,特别是在数据有限的地区。在这里,作者使用变分自编码器来生成最佳参数传递函数,增强了未测量流域的径流预测,并提高了环境建模的可解释性和可扩展性。
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引用次数: 0
Deep learning can facilitate physically interpretable geoscientific modelling 深度学习可以促进物理上可解释的地球科学建模
IF 24.1 Pub Date : 2026-02-13 DOI: 10.1038/s44221-026-00589-x
Hoshin V. Gupta
Modern deep learning can be used not only to improve predictions, but also to uncover interpretable equations that connect observable properties to the parameters of physically based geoscientific models.
现代深度学习不仅可以用来改进预测,还可以用来发现可解释的方程,这些方程将可观察到的属性与基于物理的地球科学模型的参数联系起来。
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引用次数: 0
Antibiotic membranes with broad-spectrum antibacterial properties for efficient molecular separations 具有广谱抗菌特性的抗生素膜,用于高效的分子分离
IF 24.1 Pub Date : 2026-02-13 DOI: 10.1038/s44221-025-00581-x
Yuxin Yuan, Miaomiao Jia, Hai Liu, Da Chen, Wanbin Li
Membrane separation provides an efficient alternative to alleviate water scarcity. However, it remains challenging to mitigate membrane fouling, especially biofouling, and surpass performance trade-off limitation. Here we report an antibiotic membrane with broad-spectrum antibacterial properties for highly permeable and selective water purification. Using the antibiotic kanamycin and trimesoyl chloride as monomers, a polyamide-polyester membrane was constructed through interfacial polymerization. This membrane exhibits competitive separation performance, with a high water permeance of 47.9 l m−2 h−1 bar−1, solute rejection of 99.6% and solute–solute selectivity of ~10,000, outperforming most existing membranes. Moreover, this membrane can effectively inactivate Gram-negative/positive, single/multiple-resistant and disinfectant-resistant bacteria at high concentrations of 3 × 107 colony-forming units per millilitre, showing mortality ratios of 93.6–99.9%. In addition, this membrane maintains long-term antibacterial durability during crossflow filtration for at least 170 h. These concepts and findings offer an alternative route to the design of high-performance and antifouling membranes for water treatment. This study reports an ultrathin kanamycin-based composite membrane that overcomes permeability–selectivity trade-offs while delivering strong fouling resistance and broad-spectrum antibacterial activity for water purification.
膜分离为缓解水资源短缺提供了一种有效的替代方法。然而,如何减轻膜污染,特别是生物污染,并超越性能权衡限制仍然是一个挑战。在这里,我们报道了一种具有广谱抗菌特性的抗生素膜,用于高渗透和选择性水净化。以抗生素卡那霉素和三甲酰氯为单体,通过界面聚合法制备了聚酰胺-聚酯膜。该膜具有良好的分离性能,具有47.9 l m−2 h−1 bar−1的高透水性,99.6%的溶质截留率和~10,000的溶质-溶质选择性,优于大多数现有膜。该膜对革兰氏阴性/阳性、单耐/多重耐药和消毒剂耐药菌均有良好的灭活作用,浓度为3 × 107菌落形成单位/毫升,死亡率为93.6 ~ 99.9%。此外,该膜在横流过滤期间保持至少170小时的长期抗菌耐久性。这些概念和发现为设计用于水处理的高性能防污膜提供了另一种途径。本研究报道了一种超薄卡那霉素复合膜,该膜克服了渗透性和选择性的权衡,同时具有强大的抗污性和广谱抗菌活性,用于水净化。
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引用次数: 0
A quantitative metric for industrial water use sustainability for environmental, social and governance reporting 环境、社会和治理报告中工业用水可持续性的定量度量
IF 24.1 Pub Date : 2026-02-10 DOI: 10.1038/s44221-025-00575-9
Yoora Cho, Jay Hyuk Rhee, Yong Sik Ok, William A. Mitch
Despite rapid growth in corporate environmental, social and governance reporting, water use sustainability reporting remains inadequate. Current reporting combines qualitative evaluations of investment pledges to improve sustainability with limited quantitative metrics. Unfortunately, these semi-quantitative metrics differ substantially across reporting entities, and their algorithms may not be publicly available. Their non-uniform and opaque nature raises the potential for greenwashing and hinders identifying cost-effective investments to improve sustainability. To address this deficiency, we propose a transparent and quantitative ‘water sustainability index’ (WSI) as a novel metric. The WSI considers the volume and source water type for watershed withdrawals, the volume and quality of wastewater discharges, the volume of water consumed, and the extent to which facilities reuse water. Weighting factors adjust for operations in stressed watersheds while being tuned to encourage the adoption of sustainable facility improvements. WSI’s quantitative and transparent nature helps corporations identify cost-effective investments to improve water sustainability. Quantifying water sustainability relies on limited and non-uniform metrics that risk greenwashing and hinder effective investment decisions. To address this, the proposed water sustainability index (WSI) offers a transparent, quantitative framework that accounts for water withdrawals, discharges, consumption, reuse and watershed stress to guide cost-effective sustainability improvements.
尽管企业环境、社会和治理报告迅速增长,但水资源利用可持续性报告仍然不足。目前的报告将改善可持续性的投资承诺的定性评估与有限的定量指标结合起来。不幸的是,这些半定量指标在报告实体之间存在很大差异,而且它们的算法可能无法公开获得。它们的不统一和不透明的性质增加了洗绿的可能性,并阻碍了确定具有成本效益的投资以提高可持续性。为了解决这一不足,我们提出了一个透明和定量的“水可持续性指数”(WSI)作为一个新的度量标准。WSI考虑了流域取水的量和水源类型、废水排放的量和质量、消耗的水量以及设施回用水的程度。加权系数根据压力大的流域的作业进行调整,同时进行调整以鼓励采用可持续的设施改进。WSI的量化和透明性质帮助企业确定具有成本效益的投资,以提高水的可持续性。量化水的可持续性依赖于有限和不统一的指标,这些指标有可能“漂绿”并阻碍有效的投资决策。为了解决这个问题,拟议的水可持续性指数(WSI)提供了一个透明的定量框架,该框架考虑了取水、排放、消耗、再利用和流域压力,以指导经济有效的可持续性改进。
{"title":"A quantitative metric for industrial water use sustainability for environmental, social and governance reporting","authors":"Yoora Cho, Jay Hyuk Rhee, Yong Sik Ok, William A. Mitch","doi":"10.1038/s44221-025-00575-9","DOIUrl":"10.1038/s44221-025-00575-9","url":null,"abstract":"Despite rapid growth in corporate environmental, social and governance reporting, water use sustainability reporting remains inadequate. Current reporting combines qualitative evaluations of investment pledges to improve sustainability with limited quantitative metrics. Unfortunately, these semi-quantitative metrics differ substantially across reporting entities, and their algorithms may not be publicly available. Their non-uniform and opaque nature raises the potential for greenwashing and hinders identifying cost-effective investments to improve sustainability. To address this deficiency, we propose a transparent and quantitative ‘water sustainability index’ (WSI) as a novel metric. The WSI considers the volume and source water type for watershed withdrawals, the volume and quality of wastewater discharges, the volume of water consumed, and the extent to which facilities reuse water. Weighting factors adjust for operations in stressed watersheds while being tuned to encourage the adoption of sustainable facility improvements. WSI’s quantitative and transparent nature helps corporations identify cost-effective investments to improve water sustainability. Quantifying water sustainability relies on limited and non-uniform metrics that risk greenwashing and hinder effective investment decisions. To address this, the proposed water sustainability index (WSI) offers a transparent, quantitative framework that accounts for water withdrawals, discharges, consumption, reuse and watershed stress to guide cost-effective sustainability improvements.","PeriodicalId":74252,"journal":{"name":"Nature water","volume":"4 2","pages":"138-146"},"PeriodicalIF":24.1,"publicationDate":"2026-02-10","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"147269055","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Hierarchically semi-interpenetrating polymer nanofilms for high-performance seawater desalination 用于高性能海水淡化的分层半互穿聚合物纳米膜
IF 24.1 Pub Date : 2026-02-04 DOI: 10.1038/s44221-025-00577-7
Yu Chen, Jia Xu, Kaiyuan Song, Ziying Li, Baiyang Chen, Qijing Huang, Li Yu, Yue Su, Ruijiao Dong
Thin-film composite polyamide membranes remain the benchmark for water desalination and purification. However, conventional polyamide membranes are greatly limited by the trade-off between water permeance and ion permselectivity, but also susceptible to chlorine degradation and membrane fouling. Here we addressed these issues by molecularly creating hierarchically structured polymer nanofilms featuring polyamide/polyethylene glycol (PEG) semi-interpenetrating polymer networks (semi-IPN) and interconnected hydrated micropores via macromolecule-regulated interfacial polymerization. This strategy enables controlled synthesis of nanofilms with semi-IPN architectures and tunable subnanometre-scale micropores, spanning reverse osmosis to nanofiltration. The resultant semi-IPN networks synergistically enhance water permeance and ion permselectivity to overcome the intrinsic permeability–selectivity trade-off, but also further provide superior resistance to chlorine, biofouling and mineral scaling and long-term operational stability in seawater desalination, outperforming commercial polyamide membranes. This work offers a robust platform for creating hierarchically ordered polymer networks for high-performance seawater desalination to solve the global water crisis. A macromolecule-regulated interfacial polymerization strategy enables control over polymer network architectures and micropore sizes, leading to membranes breaking the intrinsic permeability–selectivity trade-off with resistance to chlorine and membrane biofouling.
薄膜复合聚酰胺膜仍然是海水淡化和净化的基准。然而,传统的聚酰胺膜受到水透性和离子透性之间权衡的极大限制,而且容易受到氯降解和膜污染的影响。在这里,我们通过分子创建具有聚酰胺/聚乙二醇(PEG)半互穿聚合物网络(半ipn)和通过大分子调节的界面聚合相互连接的水合微孔的分层结构聚合物纳米膜来解决这些问题。这种策略可以控制合成具有半ipn结构和可调亚纳米级微孔的纳米膜,从反渗透到纳滤。由此产生的半ipn网络协同提高了水渗透性和离子选择性,克服了固有的渗透性和选择性之间的权衡,而且还进一步提供了优越的抗氯、生物污垢和矿物结垢性,以及在海水淡化中的长期运行稳定性,优于商用聚酰胺膜。这项工作为创建用于高性能海水淡化的分层有序聚合物网络提供了一个强大的平台,以解决全球水危机。大分子调节的界面聚合策略可以控制聚合物网络结构和微孔大小,从而使膜打破固有的渗透性-选择性权衡,抵抗氯和膜生物污染。
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引用次数: 0
Transformative adaptation needed to break cycles of inequitable urban flood management 变革适应需要打破不公平的城市洪水管理循环
IF 24.1 Pub Date : 2026-02-04 DOI: 10.1038/s44221-025-00569-7
Rebecca L. Hale, Krista Capps, Elizabeth M. Cook, Rachel Scarlett
Urban water hazards, including floods, water scarcity and water contamination, are increasing due to climate change. Risks associated with urban flooding are shaped by past decisions, institutional forms of oppression, their legacies, and the interactions of these legacies with ongoing climate change. When legacies of oppression and the contemporary social landscape are not considered, technocratic adaptation measures perpetuate inequitable infrastructure investment and risk. Here we review the inequitable distribution of urban flood risks within and among cities, discussing the forces driving these inequities and why many adaptation measures to address flooding exacerbate environmental injustices. Transformative approaches for equitable adaptation include systemic changes to planning, governance, and adaptive management and funding, with an explicit focus on social justice to address the underlying causes of urban flood risks. Climate adaptation provides the opportunity not only to increase urban resilience to climate change, but also to address historic injustices. Urban water hazards like flooding and contamination are worsening due to climate change, and their risks are deeply influenced by historical oppression and inequitable infrastructure decisions. This Perspective examines how urban flood risk is inequitably distributed and argues that climate adaptation should prioritize systemic, justice-focused reforms to address both resilience and historic social injustices.
由于气候变化,城市水害,包括洪水、缺水和水污染,正在增加。与城市洪水相关的风险是由过去的决策、压迫的制度形式、其遗留问题以及这些遗留问题与当前气候变化的相互作用所决定的。如果不考虑压迫的遗留问题和当代社会景观,技术官僚的适应措施将使不公平的基础设施投资和风险永久化。本文回顾了城市洪水风险在城市内部和城市之间的不公平分布,讨论了导致这些不公平的力量,以及为什么许多应对洪水的适应措施加剧了环境不公正。公平适应的变革性方法包括对规划、治理、适应性管理和资金进行系统性改革,明确关注社会正义,以解决城市洪水风险的根本原因。气候适应不仅为提高城市应对气候变化的能力提供了机会,也为解决历史上的不公正现象提供了机会。由于气候变化,洪水和污染等城市水害正在恶化,其风险深受历史压迫和不公平的基础设施决策的影响。本《展望》探讨了城市洪水风险是如何不公平分配的,并认为气候适应应优先考虑系统性、以正义为重点的改革,以解决复原力和历史上的社会不公正问题。
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引用次数: 0
Estimating methane emissions from global sewer networks 估算全球下水道网络的甲烷排放量
IF 24.1 Pub Date : 2026-02-02 DOI: 10.1038/s44221-025-00574-w
Keshab Sharma, Jiuling Li, Tao Liu, John Willis, Yiwen Liu, Zhiyu Zhang, Zhiguo Yuan
Conclusive evidence has emerged showing substantial methane (CH4) emissions from sewer systems, contradictory to the ‘zero emission’ assumption made by the Intergovernmental Panel on Climate Change. However, the global magnitude of sewer CH4 emissions remains unknown. By ingeniously integrating mechanistic and knowledge-supported data-driven modelling, we have derived from the relatively small datasets available a simple set of robust and interpretable equations to estimate CH4 emissions from sewer networks based on readily available information such as sewer geometry, the design and actual dry weather flows, and wastewater temperature. With this tool, we estimate that, globally, sewers emit 1.18–1.95 Tg CH4 yr−1 (95% confidence interval), adding 15.7–37.6% to the currently estimated carbon footprint of wastewater management and 1.7–3.3% to the currently estimated global methane emissions by the waste sector. Our developed tool can reliably and efficiently estimate sewer methane emissions, supporting water authorities globally to establish emissions inventories and pursue carbon-neutral wastewater management. Sewer systems have long been assumed to be negligible sources of methane, yet emerging evidence suggests that they represent a previously overlooked contributor to greenhouse gas emissions. This study shows that global sewer networks emit ~1.2–2.0 Tg CH4 yr−1, substantially increasing wastewater-sector methane emissions and challenging the IPCC zero-emission assumption.
确凿的证据表明,下水道系统排放了大量甲烷(CH4),这与政府间气候变化专门委员会(ipcc)提出的“零排放”假设相矛盾。然而,下水道甲烷排放的全球规模仍然未知。通过巧妙地整合机制和知识支持的数据驱动模型,我们从相对较小的可用数据集中推导出一套简单可靠且可解释的方程,以根据下水道几何形状、设计和实际干燥天气流量以及废水温度等现成信息估算下水道网络的甲烷排放量。通过该工具,我们估计,全球下水道排放1.18-1.95 Tg CH4 yr - 1(95%置信区间),使目前估计的废水管理碳足迹增加15.7-37.6%,使目前估计的全球废物部门甲烷排放量增加1.7-3.3%。我们开发的工具可以可靠有效地估算下水道甲烷排放量,支持全球水务部门建立排放清单,实现碳中和废水管理。长期以来,人们一直认为下水道系统是可以忽略不计的甲烷来源,但新出现的证据表明,它们是以前被忽视的温室气体排放源。该研究表明,全球下水道网络每年排放约1.2-2.0 Tg CH4 - 1,大大增加了废水部门的甲烷排放量,挑战了IPCC的零排放假设。
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引用次数: 0
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