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Improvement of the determination of radioactivity concentrations of short-lived radioisotopes with the time-dependent leakage model of VVER-type nuclear reactor 利用 VVER 型核反应堆随时间变化的泄漏模型改进短寿命放射性同位素放射性浓度的测定方法
IF 1.9 3区 工程技术 Q1 NUCLEAR SCIENCE & TECHNOLOGY Pub Date : 2024-09-23 DOI: 10.1016/j.anucene.2024.110929
The leak-free operation is a fundamental necessity for the entire duration of each nuclear reactor cycle. While the physical and chemical processes resulting from fuel failures typically do not avert the safe operation of the reactor, they can have direct operational and economic consequences. The state of leak-free operation in the reactor core is monitored on-line by gamma spectra measurements of the primary coolant. Estimating the burnup and leakage parameters of defective fuel elements is achieved through calculations employing relevant leakage models. This paper presents a novel approach to assessing the time-dependent sample delay time, which is used to calculate the time-dependent radioactivity concentrations of the fission products in the primary coolant from their number of nuclei calculated by the time-dependent leakage model. The performance of three models with different basic assumptions was individually and collectively investigated. The new sample delay time model allows a more accurate estimation of the time-dependent radioactivity concentration, especially of the short-lived 137Xe, 138Xe, 138Cs, and 134I isotopes in the primary coolant.
在每个核反应堆循环的整个过程中,无泄漏运行是一项基本要求。虽然燃料故障导致的物理和化学过程通常不会影响反应堆的安全运行,但会对运行和经济造成直接影响。反应堆堆芯的无泄漏运行状态是通过一次冷却剂的伽马能谱测量进行在线监测的。通过采用相关泄漏模型进行计算,可以估算出缺陷燃料元件的燃耗和泄漏参数。本文提出了一种评估随时间变化的样品延迟时间的新方法,该方法用于根据随时间变化的泄漏模型计算出的核子数量,计算初级冷却剂中裂变产物随时间变化的放射性浓度。我们对三种具有不同基本假设的模型的性能进行了单独和集体研究。新的样品延迟时间模型可以更准确地估计随时间变化的放射性浓度,特别是初级冷却剂中寿命较短的 137Xe、138Xe、138Cs 和 134I 同位素的浓度。
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引用次数: 0
Nuclide number density prediction in the lattice physics calculation based on Dynamic mode decomposition 基于动态模式分解的晶格物理计算中的核素数量密度预测
IF 1.9 3区 工程技术 Q1 NUCLEAR SCIENCE & TECHNOLOGY Pub Date : 2024-09-20 DOI: 10.1016/j.anucene.2024.110924

Burnup analysis in nuclear reactors requires iterative computation of neutron transport and fuel depletion, which is computationally intensive, particularly for large-scale scenarios. This study introduces an innovative approach leveraging the Dynamic Mode Decomposition (DMD) algorithm to predict the temporal evolution of nuclide densities. By identifying and utilizing the DMD modes and eigenvalues from snapshots of nuclide density, this method aims to alleviate the computational demands of the coupled transport and burnup calculations. Firstly, the methodology selects the key reactivity-contributing nuclides to evaluate the correlation between the complexity of the reduced-order model and the precision of predictions. Subsequently, an optimized reduced-order model is employed for forecasting nuclide densities in a pin-cell. In most cases, DMD predicts more accurately than traditional quadratic extrapolation methods. Moreover, the DMD algorithm demonstrates commendable accuracy in predicting the nuclide density distribution within a PWR fuel assembly, suggesting its promising potential for reactor burnup analysis applications.

核反应堆的燃耗分析需要对中子传输和燃料耗竭进行迭代计算,计算量很大,尤其是在大规模情况下。本研究引入了一种创新方法,利用动态模式分解(DMD)算法来预测核素密度的时间演化。通过识别和利用核素密度快照中的 DMD 模式和特征值,该方法旨在减轻耦合输运和燃耗计算的计算需求。首先,该方法选择关键的反应性贡献核素,以评估降阶模型的复杂性与预测精度之间的相关性。随后,采用优化的降阶模型预测针胞中的核素密度。在大多数情况下,DMD 比传统的二次外推法预测得更准确。此外,DMD 算法在预测压水堆燃料组件内核素密度分布方面表现出了令人称道的准确性,表明其在反应堆燃烧分析应用方面具有广阔的发展前景。
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引用次数: 0
Excitation functions for fast neutron induced reactions on Al, Zr, In and Au 铝、锆、铟和金上快中子诱导反应的激发函数
IF 1.9 3区 工程技术 Q1 NUCLEAR SCIENCE & TECHNOLOGY Pub Date : 2024-09-20 DOI: 10.1016/j.anucene.2024.110925

Cross sections of the 27Al(n,α)24Na, 96Zr(n,2n)95Zr, 115In(n,p)115gCd, 115In(n, 2n)114mIn and 197Au(n,2n)196/196m2Au reactions induced by D-T neutrons are presented with the activation method and off-line γ-ray spectrometry technique. Uncertainty propagation and correlation of the cross sections were estimated using covariance analysis. It shows that, our results are consistent with most of the previous literature data of EXFOR library. Experimental values, including previous literature data, are compared with evaluated nuclear data of the CENDL-3.2, BROND-3.1, ENDF/B-VIII.0, IRDFF-II, JENDL-5 and JEFF-3.3 libraries. Besides, these excitation functions were theoretically calculated by using the TALYS-2.0 code up to the neutron energy of 20 MeV. It shows that significant discrepancies were found between experiment data and those of calculated results and evaluated data.

利用活化法和离线 γ 射线光谱技术介绍了 D-T 中子诱导的 27Al(n,α)24Na、96Zr(n,2n)95Zr、115In(n,p)115gCd、115In(n, 2n)114mIn 和 197Au(n,2n)196/196m2Au 反应的横截面。利用协方差分析估算了截面的不确定性传播和相关性。结果表明,我们的研究结果与 EXFOR 库中大部分以前的文献数据是一致的。实验值(包括以前的文献数据)与 CENDL-3.2、BROND-3.1、ENDF/B-VIII.0、IRDFF-II、JENDL-5 和 JEFF-3.3 库的评估核数据进行了比较。此外,还使用 TALYS-2.0 代码对这些激发函数进行了理论计算,最大中子能量为 20 MeV。结果表明,实验数据与计算结果和评估数据之间存在明显差异。
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引用次数: 0
Phase-field simulation of recrystallization and calculation of the effective thermal conductivity of polycrystalline UO2 多晶二氧化铀再结晶的相场模拟和有效热导率计算
IF 1.9 3区 工程技术 Q1 NUCLEAR SCIENCE & TECHNOLOGY Pub Date : 2024-09-19 DOI: 10.1016/j.anucene.2024.110918

During the operational lifespan of uranium dioxide (UO2) fuel, the emergence of a specific process termed recrystallization may transpire. The influence of recrystallization on the thermal conductivity of the fuel holds paramount significance, bearing direct implications for both safety and economic considerations. In the current investigation, a phase-field model incorporating an explicit nucleation model for recrystallized grains was formulated to study the formation and growth of recrystallized grains within polycrystalline UO2. The simulations conducted in this study revealed that the kinetics of recrystallization adhered to the empirical equation, and the observed variation in grain size during recrystallization exhibited concordance with experimental data. To elucidate the variation in thermal conductivity during recrystallization, a thermal conductivity model based on the microstructure generated through phase-field simulations was employed. The relationship between grain boundary (GB) thermal resistance and phase-field simulation parameters has been determined through empirical formulas. The simulated values of thermal conductivity during recrystallization demonstrated a commendable agreement with empirical functions. By comparing the computational results of thermal conductivity with or without recrystallization, it is proven that recrystallization is beneficial to the effective thermal conductivity because the increase in thermal conductivity due to the elimination of defects by recrystallization exceeds the decrease in thermal conductivity due to the introduction of large area GBs.

在二氧化铀(UO2)燃料的运行寿命期间,可能会出现一种称为再结晶的特殊过程。再结晶对燃料热导率的影响至关重要,对安全和经济因素都有直接影响。在当前的研究中,制定了一个相场模型,其中包含一个明确的再结晶晶粒成核模型,用于研究多晶二氧化铀中再结晶晶粒的形成和生长。模拟结果表明,再结晶动力学符合经验方程,观察到的再结晶过程中晶粒大小的变化与实验数据一致。为阐明再结晶过程中热导率的变化,采用了基于相场模拟产生的微观结构的热导率模型。通过经验公式确定了晶界(GB)热阻与相场模拟参数之间的关系。再结晶过程中的热导率模拟值与经验函数的一致性值得称赞。通过比较有无再结晶的热导率计算结果,证明了再结晶有利于提高有效热导率,因为再结晶消除缺陷所带来的热导率提高超过了引入大面积晶界所带来的热导率降低。
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引用次数: 0
Steady-state analysis of Xi’an Pulse Reactor based on the multi-physics coupling method 基于多物理场耦合方法的西安脉冲反应堆稳态分析
IF 1.9 3区 工程技术 Q1 NUCLEAR SCIENCE & TECHNOLOGY Pub Date : 2024-09-18 DOI: 10.1016/j.anucene.2024.110922

A multi-physics coupling system has been developed in this work based on the MOOSE framework for the steady-state analysis of XAPR (Xi’an Pulse Reactor). It consists of three physical models including neutronics, thermo-mechanics model of fuel element and fluid flow model. These models have been coupled by Picard iteration through the MultiApp and Transfer system based on MOOSE framework. The core state parameters of XAPR under steady-state operation condition are analyzed and the 3-dimensional space-dependent power density, fuel element temperature as well as the coolant temperature are provided by the multi-physics model. The multi-physics model successfully reproduced the experimental results of the monitored fuel element temperature in XAPR under different power level, and the deviation was less than 20 K. Future work would be to study the dynamics behavior of XAPR to further validate the multi-physics model and simulate other advanced micro reactors.

本研究基于 MOOSE 框架开发了一个多物理场耦合系统,用于 XAPR(西安脉冲反应堆)的稳态分析。该系统由三个物理模型组成,包括中子学模型、燃料元件热力学模型和流体流动模型。这些模型通过基于 MOOSE 框架的多应用和传输系统进行 Picard 迭代耦合。多物理场模型分析了稳态运行条件下 XAPR 的核心状态参数,并提供了三维空间功率密度、燃料元件温度和冷却剂温度。多物理场模型成功再现了不同功率水平下 XAPR 中燃料元件温度监测的实验结果,偏差小于 20 K。未来的工作将是研究 XAPR 的动力学行为,以进一步验证多物理场模型,并模拟其他先进的微型反应堆。
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引用次数: 0
Applicability domain and gaps of SNF decay heat validation data – A similarity-based approach 核燃料衰变热验证数据的适用领域和差距--基于相似性的方法
IF 1.9 3区 工程技术 Q1 NUCLEAR SCIENCE & TECHNOLOGY Pub Date : 2024-09-18 DOI: 10.1016/j.anucene.2024.110905

Decay heat measurements on spent nuclear fuel (SNF) provide a basis for code validation. Their applicability domain (AD) and gaps, which are the focus of this study, are not commonly discussed in the literature. The analyzed validation data are based on measurements at the Clab facility and on calculations using the Polaris and ORIGEN codes of the SCALE code system. Bias-predicting machine learning (ML) models are applied: random forest and weighted k-nearest neighbors. The models weigh the similarity between the cases, expressed using correlations. The learning curves are studied by examining the prediction error versus the sample size and the similarity coefficient. The obtained error reduction at higher similarity coefficients supports the argument that the similarity or correlation is informative. However, a marginal error reduction is expected from increasing the validation data size from its current status. Following this, a validation AD is proposed as a range of SNF characteristics within which the validation data and the ML models are observed and tested. Within the AD, different levels of error, i.e., safety margins and conservatism, were evaluated. Beyond the AD, validation gaps exist. Examination of light-water reactor SNF applications indicates that the validation coverage is absent in both MOX fuel and short cooling, diminishes rapidly at higher burnup for low-enrichment fuel, and extends with burnup for high-enrichment cases. Additional measurements are justified to reduce conservatism or achieve validation coverage in applications. A case study of typical UO2 and MOX SNF applications is analyzed. It is shown that a few tens of optimally selected measurements from both SNF types are necessary to complete validation coverage in numerous applications.

乏核燃料(SNF)的衰变热测量为代码验证提供了基础。其适用领域(AD)和差距是本研究的重点,在文献中并未得到普遍讨论。分析的验证数据基于 Clab 设施的测量结果以及 SCALE 代码系统中 Polaris 和 ORIGEN 代码的计算结果。应用了偏差预测机器学习(ML)模型:随机森林和加权 k 近邻。这些模型使用相关性来权衡案例之间的相似性。通过检测预测误差与样本量和相似性系数的关系,研究了学习曲线。相似性系数越高,误差越小,这支持了相似性或相关性具有信息量的论点。不过,从目前的情况来看,增加验证数据的规模预计会使误差略有减少。在此基础上,提出了一个验证 AD,作为观测和测试验证数据和 ML 模型的 SNF 特征范围。在 AD 范围内,对不同程度的误差(即安全边际和保守性)进行了评估。在 AD 之外,还存在验证差距。对轻水堆 SNF 应用的研究表明,在 MOX 燃料和短时冷却中都不存在验证范围,对于低浓缩燃料,在较高燃耗时验证范围迅速缩小,而对于高浓缩情况,验证范围则随着燃耗的增加而扩大。为减少保守性或在应用中实现验证覆盖,有必要进行额外的测量。对典型的二氧化铀和混合氧化物 SNF 应用案例进行了分析。结果表明,要完成众多应用中的验证范围,需要对两种 SNF 类型进行几十次优化选择的测量。
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引用次数: 0
Coupled analysis of oxidation corrosion and heat transfer in lead-cooled fast reactors 铅冷快堆氧化腐蚀和传热耦合分析
IF 1.9 3区 工程技术 Q1 NUCLEAR SCIENCE & TECHNOLOGY Pub Date : 2024-09-16 DOI: 10.1016/j.anucene.2024.110919

The coupled code LETHAC-Oxide is developed for analysis of thermal–hydraulic and safety characteristics in lead-cooled fast reactors, considering the impact of oxidation corrosion during prolonged operation. Based on experimental data from CORRIDA, Tsu-2M, and SM-1 facility, the oxidation model is well verified. The reactor concepts LESMOR and BREST-OD-300 are modeled, and the results show that the oxide layer significantly influences heat transfer, particularly at higher temperatures. A comparison between LESMOR and BREST-OD-300 demonstrates that a 95 °C difference in average system temperature will cause 14 times increase in oxide layer thickness and 7 times decrease in steam generator heat exchange capability. Conclusively, LESMOR forms a protective oxide film after a refueling cycle, offering structural material protection without major heat transfer impact. In contrast, BREST-OD-300 shows a substantial increase in cladding temperature and decrease in heat transfer capacity. This result underscores the necessity of oxygen control technology to mitigate risks associated with oxidation corrosion, providing valuable insights for optimal reactor performance and safety.

考虑到长期运行期间氧化腐蚀的影响,开发了耦合代码 LETHAC-Oxide,用于分析铅冷快堆的热-水力和安全特性。根据 CORRIDA、Tsu-2M 和 SM-1 设施的实验数据,氧化模型得到了很好的验证。对反应堆概念 LESMOR 和 BREST-OD-300 进行了建模,结果表明氧化层对传热有显著影响,尤其是在较高温度下。LESMOR 和 BREST-OD-300 的比较表明,系统平均温度相差 95 ℃ 会导致氧化层厚度增加 14 倍,蒸汽发生器的热交换能力降低 7 倍。最终,LESMOR 在一个加油周期后会形成一层氧化保护膜,为结构材料提供保护,而不会对传热产生重大影响。相比之下,BREST-OD-300 的包层温度大幅上升,传热能力下降。这一结果凸显了氧气控制技术对降低氧化腐蚀相关风险的必要性,为优化反应堆性能和安全提供了宝贵的见解。
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引用次数: 0
A study on the optimization through the evaluation of radiation exposure by scenarios during steam generator dismantling 通过评估蒸汽发生器拆除过程中的辐照情况进行优化的研究
IF 1.9 3区 工程技术 Q1 NUCLEAR SCIENCE & TECHNOLOGY Pub Date : 2024-09-15 DOI: 10.1016/j.anucene.2024.110901

Steam generator (SG) replacements in South Korea began with the Kori No. 1 unit in 1998 due to performance degradation. Currently, 20 steam generators have been replaced in total. While additional decommissioning of dozens of steam generator will be required soon due to life-expiration of several nuclear power plants, there has been no actual dismantling performance of steam generators yet, and the replaced decommissioned steam generators are currently stored in intermediate storage facilities. To minimize waste volume and facilitate site reuse, it’s necessary to proactively dismantle steam generators. These components are less radioactively contaminated and easier to dismantle compared to primary equipment like reactors. Additionally, securing related dismantling technology is essential for managing future replacements or equipment that has been stored. Establishing a process scenario about where and how the steam generator will be safely dismantled is important. It is necessary to analyze the advantages and disadvantages of each scenario to study the timing, location, and method of dismantling, and to develop an optimal process scenario through analysis of worker radiation exposure and dismantling costs. For this purpose, simulations were conducted on the radiation dose to workers according to the timing and method of dismantling, using 3D dismantling simulation software developed by Cyclife Digital Solutions, a subsidiary of French EDF, and the results were reviewed by mathematically modeling and analyzing the radiation doses exposed to workers over the years using an exponential decay model.

由于性能下降,韩国从 1998 年开始更换 Kori 1 号机组的蒸汽发生器(SG)。目前,总共更换了 20 台蒸汽发生器。虽然由于几座核电站的寿命到期,很快还需要退役几十台蒸汽发生器,但蒸汽发生器还没有实际的拆除性能,更换下来的退役蒸汽发生器目前存放在中间储存设施中。为了最大限度地减少废物量并促进现场再利用,有必要主动拆除蒸汽发生器。与反应堆等主要设备相比,这些部件受到的放射性污染较少,也更容易拆除。此外,确保相关的拆卸技术对于管理未来的替换设备或已储存的设备至关重要。就蒸汽发生器的安全拆除地点和方式制定一个流程方案非常重要。有必要对每种方案的优缺点进行分析,以研究拆除的时间、地点和方法,并通过对工人辐射暴露和拆除成本的分析来制定最佳工艺方案。为此,使用法国电力公司子公司 Cyclife Digital Solutions 开发的三维拆卸模拟软件,根据拆卸时间和方法对工人受到的辐射剂量进行了模拟,并使用指数衰减模型对多年来工人受到的辐射剂量进行了数学建模和分析,对结果进行了审查。
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引用次数: 0
Experimental study on CHF enhancement of different oxidized surfaces of low carbon steel in nanofluid 低碳钢不同氧化表面在纳米流体中增强 CHF 的实验研究
IF 1.9 3区 工程技术 Q1 NUCLEAR SCIENCE & TECHNOLOGY Pub Date : 2024-09-15 DOI: 10.1016/j.anucene.2024.110923

Considerable research has been undertaken to explore the use of nanofluids for augmenting the critical heat flux in the in-vessel retention (IVR) strategy deployed in reactors, demonstrating significant improvements in CHF. However, it is important to consider the potential bias in previous studies on surface CHF due to the oxidation of low carbon steel, which is commonly used in reactor vessels, in both air and water under real-life conditions. This study represents the initial investigation into the oxidation behavior of low carbon steel in an air environment, followed by subsequent boiling in water. The results indicate that when the mild steel surface is pre-oxidized in air, the CHF value in deionized water decreases. However, this effect is not readily apparent in nanofluids. Consequently, it suggests that CHF under real operational conditions could be lower than anticipated. Additionally, nanofluids significantly increase the CHF of surface, however, the enhancement of CHF for oxidized surfaces in water is not as pronounced, a point which has never been mentioned by researchers. The mechanisms of surface oxidation and nanofluid-induced CHF enhancement are explained. Consequently, this paper provides important reference value for studying the application of nanofluids in IVR accidents.

人们已经开展了大量研究,探索如何在反应堆采用的舱内滞留(IVR)策略中使用纳米流体来增加临界热通量,结果表明纳米流体的临界热通量(CHF)得到了显著改善。然而,重要的是要考虑到由于反应器容器中常用的低碳钢在空气和水中的实际条件下会发生氧化,因此以往关于表面 CHF 的研究可能存在偏差。本研究是对低碳钢在空气环境中氧化行为以及随后在水中沸腾行为的初步调查。结果表明,当低碳钢表面在空气中发生预氧化时,其在去离子水中的 CHF 值会降低。然而,这种效应在纳米流体中并不明显。因此,这表明实际操作条件下的 CHF 值可能低于预期值。此外,纳米流体可显著提高表面的 CHF 值,但在水中氧化表面的 CHF 值的提高并不明显,这一点从未被研究人员提及。本文解释了表面氧化和纳米流体诱导 CHF 增强的机理。因此,本文为研究纳米流体在 IVR 事故中的应用提供了重要的参考价值。
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引用次数: 0
Research on core thermal hydraulic parameters prediction based on the improved GAN method and combined ANN model 基于改进的 GAN 方法和组合 ANN 模型的岩心热工水力参数预测研究
IF 1.9 3区 工程技术 Q1 NUCLEAR SCIENCE & TECHNOLOGY Pub Date : 2024-09-14 DOI: 10.1016/j.anucene.2024.110913

This research presents advanced methods of data processing as tools applicable in nuclear engineering. Three methods-autoencoder, random forest and multilayer perceptron were considered for the testing. The multi-layer perceptron (MLP) method preserved best the structure of the data. A better generative adversarial network (GAN) based on the Wasserstein distance was implemented for data generation, which overcomes the issues of gradient vanishing and mode collapse prevailing in common GANs. While examining the generated data, advanced statistical and machine learning techniques were applied to minutely compare the generated and original data. Data forecasting applied a combined model of MLP, convolutional neural network (CNN), and recurrent neural networks (RNN). With limited-memory broyden-fletcher-goldfarb-shanno (LBFGS) optimization algorithm being combined with bayesian optimization, there was significant improved prediction of core thermal hydraulic parameters. Meanwhile, this research provides important techniques to deal with challenges of nuclear engineering data which further impacts the field of nuclear engineering.

这项研究提出了先进的数据处理方法,作为适用于核工程的工具。测试中考虑了三种方法--自动编码器、随机森林和多层感知器。多层感知器(MLP)方法最好地保留了数据的结构。在生成数据时,采用了一种基于 Wasserstein 距离的更好的生成式对抗网络(GAN),它克服了普通 GAN 中普遍存在的梯度消失和模式崩溃问题。在检查生成的数据时,应用了先进的统计和机器学习技术,对生成的数据和原始数据进行了细致的比较。数据预测应用了 MLP、卷积神经网络(CNN)和递归神经网络(RNN)的组合模型。通过将有限记忆布洛伊登-弗莱彻-金法布-山诺(LBFGS)优化算法与贝叶斯优化相结合,岩芯热工水力参数的预测得到了显著改善。同时,这项研究为应对核工程数据挑战提供了重要技术,进一步影响了核工程领域。
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引用次数: 0
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