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An organic quantum battery 有机量子电池
Pub Date : 2020-12-11 DOI: 10.21203/rs.3.rs-123919/v1
J. Quach, K. McGhee, L. Ganzer, D. Rouse, B. Lovett, Erik Gauger, Jonathan Keeling, G. Cerullo, David G Lidzey, T. Virgili
Quantum batteries harness the unique properties of quantum mechanics to enhance energy storage compared to conventional batteries. In particular, they are predicted to undergo superextensive charging, where batteries with larger capacity actually take less time to charge. Up until now however, they have not been experimentally demonstrated, due to the challenges in quantum coherent control. Here we implement an array of two-level systems coupled to a photonic mode to realise a Dicke quantum battery. Our quantum battery is constructed with a microcavity formed by two dielectric mirrors enclosing a thin film of a fluorescent molecular dye in a polymer matrix. We use ultrafast optical spectroscopy to time resolve the charging dynamics of the quantum battery at femtosecond resolution. We experimentally demonstrate superextensive increases in both charging power and storage capacity, in agreement with our theoretical modelling. We find that decoherence plays an important role in stabilising energy storage, analogous to the role that dissipation plays in photosynthesis. This experimental proof-of-concept is a major milestone towards the practical application of quantum batteries in quantum and conventional devices. Our work opens new opportunities for harnessing collective effects in light-matter coupling for nanoscale energy capture, storage, and transport technologies, including the enhancement of solar cell efficiencies.
与传统电池相比,量子电池利用量子力学的独特特性来增强能量存储。特别是,电池容量越大,充电时间就会越短,因此预计会出现“超长充电”现象。然而,到目前为止,由于量子相干控制方面的挑战,它们还没有得到实验证明。在这里,我们实现了一组耦合到光子模式的两能级系统来实现Dicke量子电池。我们的量子电池是由两个介电镜在聚合物基质中包裹一层荧光分子染料薄膜形成的微腔构成的。我们利用超快光谱学在飞秒分辨率下对量子电池的充电动力学进行时间解析。我们通过实验证明了充电功率和存储容量的大幅增加,与我们的理论模型一致。我们发现退相干在稳定能量储存中起着重要作用,类似于耗散在光合作用中的作用。这一实验概念验证是量子电池在量子和传统设备中实际应用的一个重要里程碑。我们的工作为利用光物质耦合中的集体效应用于纳米级能量捕获、存储和传输技术,包括提高太阳能电池效率,开辟了新的机会。
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引用次数: 3
Ultrabright Multiplexed Energy-Time-Entangled Photon Generation from Lithium Niobate on Insulator Chip 铌酸锂在绝缘体芯片上产生超亮多路能量-时间纠缠光子
Pub Date : 2020-12-11 DOI: 10.1103/PhysRevApplied.15.064059
Guang-Tai Xue, Y. Niu, Xiaoyue Liu, Jiachen Duan, Wenjun Chen, Ying Pan, Kunpeng Jia, Xiaohan Wang, Hua-Ying Liu, Yong Zhang, P. Xu, G. Zhao, Xinlun Cai, Y. Gong, Xiaopeng Hu, Zhenda Xie, Shi-ning Zhu
High-flux entangled photon source is the key resource for quantum optical study and application. Here it is realized in a lithium niobate on isolator (LNOI) chip, with 2.79*10^11 Hz/mW photon pair rate and 1.53*10^9 Hz/nm/mW spectral brightness. These data are boosted by over two orders of magnitude compared to existing technologies. A 130-nm broad bandwidth is engineered for 8-channel multiplexed energy-time entanglement. Harnessed by high-extinction frequency correlation and Franson interferences up to 99.17% visibility, such energy-time entanglement multiplexing further enhances high-flux data rate, and warrants broad applications in quantum information processing on a chip.
高通量纠缠光子源是量子光学研究和应用的关键资源。本文在铌酸锂隔离器(LNOI)芯片上实现了光子对速率为2.79*10^11 Hz/mW,光谱亮度为1.53*10^9 Hz/nm/mW。与现有技术相比,这些数据提升了两个数量级以上。130纳米宽带宽设计用于8通道复用能量时间纠缠。利用高消光频率相关和高达99.17%可见性的Franson干扰,这种能量-时间纠缠复用进一步提高了高通量数据速率,在芯片上的量子信息处理中具有广泛的应用前景。
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引用次数: 29
Learning from Physics Experiments with Quantum Computers: Applications in Muon Spectroscopy 从量子计算机的物理实验中学习:在μ介子光谱中的应用
Pub Date : 2020-12-11 DOI: 10.1103/PRXQuantum.2.020349
Sam McArdle
Computational physics is an important tool for analysing, verifying, and -- at times -- replacing physical experiments. Nevertheless, simulating quantum systems and analysing quantum data has so far resisted an efficient classical treatment in full generality. While programmable quantum systems have been developed to address this challenge, the resources required for classically intractable problems still lie beyond our reach. In this work, we consider a new target for quantum simulation algorithms; analysing the data arising from physics experiments -- specifically, muon spectroscopy experiments. These experiments can be used to probe the quantum interactions present in condensed matter systems. However, fully analysing their results can require classical computational resources scaling exponentially with the simulated system size, which can limit our understanding of the studied system. We show that this task may be a natural fit for the coming generations of quantum computers. We use classical emulations of our quantum algorithm on systems of up to 29 qubits to analyse real experimental data, and to estimate both the near-term and error corrected resources required for our proposal. We find that our algorithm exhibits good noise resilience, stemming from our desire to extract global parameters from a fitted curve, rather than targeting any individual data point. In some respects, our resource estimates go further than some prior work in quantum simulation, by estimating the resources required to solve a complete task, rather than just to run a given circuit. Taking the overhead of observable measurement and calculating multiple datapoints into account, we find that significant challenges still remain if our algorithm is to become practical for analysing muon spectroscopy data.
计算物理是分析、验证和(有时)替代物理实验的重要工具。然而,到目前为止,模拟量子系统和分析量子数据还没有得到有效的经典处理。虽然可编程量子系统已经被开发出来应对这一挑战,但解决经典棘手问题所需的资源仍然超出了我们的能力范围。在这项工作中,我们考虑了量子模拟算法的新目标;分析物理实验产生的数据,特别是介子光谱实验。这些实验可以用来探测存在于凝聚态系统中的量子相互作用。然而,充分分析他们的结果可能需要经典的计算资源与模拟系统的大小成指数比例,这可能会限制我们对所研究系统的理解。我们表明,这项任务可能是未来几代量子计算机的自然选择。我们在多达29个量子比特的系统上使用我们的量子算法的经典模拟来分析真实的实验数据,并估计我们的提议所需的近期和纠错资源。我们发现我们的算法表现出良好的噪声弹性,源于我们希望从拟合曲线中提取全局参数,而不是针对任何单个数据点。在某些方面,我们的资源估计比量子模拟中的一些先前工作走得更远,通过估计解决完整任务所需的资源,而不仅仅是运行给定的电路。考虑到观测测量和计算多个数据点的开销,我们发现如果我们的算法要成为分析μ子光谱数据的实用方法,仍然存在重大挑战。
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引用次数: 2
Quantum battery of interacting spins with environmental noise 自旋与环境噪声相互作用的量子电池
Pub Date : 2020-12-11 DOI: 10.1103/PHYSREVA.103.033715
Fang Zhao, F. Dou, Qing Zhao
A quantum battery is a temporary energy-storage system. We constructed the quantum battery model of an N-spin chain with nearest-neighbor hopping interaction and investigated the charging process of the quantum battery. We obtained the maximum energy in the quantum battery charged by a coherent cavity driving field or a thermal heat bath. We confirmed that for a finite-length spin chain, thermal charging results in a nonzero ergotropy, contradicting a previous result: that an incoherent heat source cannot charge a single-spin quantum battery. The nearest-neighbor hopping interaction induces energy band splitting, which enhances the energy storage and the ergotropy of the quantum battery. We found a critical point in the energy and ergotropy resulting from the ground-state quantum phase transition, after which the energy significantly enhance. Finally, we also found that disorder increased the energy of the quantum battery.
量子电池是一种临时的能量存储系统。我们建立了具有最近邻跳变相互作用的n -自旋链量子电池模型,并研究了量子电池的充电过程。我们获得了在相干腔驱动场或热浴中充电的量子电池的最大能量。我们证实,对于有限长度的自旋链,热充电导致非零自恋,这与之前的结果相矛盾:非相干热源不能给单自旋量子电池充电。最近邻跳变相互作用引起能带分裂,增强了量子电池的能量储存和自恋性。在基态量子相变引起的能量和自恋性中发现了一个临界点,在此之后能量显著增强。最后,我们还发现无序增加了量子电池的能量。
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引用次数: 14
Absolute Determination of the Single-Photon Optomechanical Coupling Rate via a Hopf Bifurcation 基于Hopf分岔的单光子光力学耦合速率的绝对确定
Pub Date : 2020-12-10 DOI: 10.1103/PHYSREVAPPLIED.15.034012
P. Piergentili, Wenlin Li, R. Natali, D. Vitali, G. Di Giuseppe
We establish a method for the determination of the single-photon optomechanical coupling rate, which characterizes the radiation pressure interaction in an optomechanical system. The estimation of the rate with which a mechanical oscillator, initially in a thermal state, undergoes a Hopf bifurcation, and reaches a limit cycle, allows us to determine the single-photon optomechanical coupling rate in a simple and consistent way. Most importantly, and in contrast to other methods, our method does not rely on knowledge of the system's bath temperature and on a calibration of the signal. We provide the theoretical framework, and experimentally validate this method, providing a procedure for the full characterization of an optomechanical system, which could be extended outside cavity optomechanics, whenever a resonator is driven into a limit cycle by the appropriate interaction with another degree of freedom.
建立了表征光机械系统中辐射压力相互作用的单光子光机械耦合率的测定方法。从热态到Hopf分岔并达到极限环的速率估计,使我们能够以一种简单而一致的方式确定单光子光机耦合速率。最重要的是,与其他方法相比,我们的方法不依赖于系统浴液温度的知识和信号的校准。我们提供了理论框架,并通过实验验证了该方法,为光力学系统的完整表征提供了一个过程,该过程可以扩展到腔光力学之外,每当谐振器通过与另一个自由度的适当相互作用被驱动到极限环时。
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引用次数: 9
Optimal Manipulation Of Correlations And Temperature In Quantum Thermodynamics 量子热力学中相关和温度的最佳操作
Pub Date : 2020-12-08 DOI: 10.13097/archive-ouverte/unige:145933
F. Clivaz
This thesis is devoted to studying two tasks: refrigeration and the creation of correlations. In the refrigeration part, two different paradigms of cooling, namely coherent and incoherent, are defined. The connection that these paradigms have with other existing refrigeration techniques such as heat bath algorithmic cooling (HBAC), the resource theoretic approach to quantum thermodynamics, and autonomous cooling is then made. Each paradigm is then investigated on its own. This in particular allows for the derivation of a general and attainable bound. The bound is striking in its simplicity: it depends on a single parameter of the environment/machine used to cool the system of interest. The creation of correlations part is devoted to the quantitative study of how much correlations can be created for a given amount of energy. After having precisely formulated the problem of interest, we solve it for arbitrary finite dimensional bipartite systems for vanishing background temperatures. For non-vanishing background temperature the symmetry of the problem breaks down, making it much harder to tackle. When both systems are copies of each other, enough symmetry is restored to formulate an upper bound valid for all (finite) dimensional systems and prove its attainability for dimension 3 and 4. We furthermore conjecture, as well as show evidence for, the bound to be attainable in any dimension.
本论文致力于研究两个任务:冷藏和相关性的创建。在制冷部分,定义了两种不同的冷却范式,即相干和非相干。然后,将这些范例与其他现有的制冷技术(如热浴算法冷却(HBAC))、量子热力学的资源理论方法和自主冷却)联系起来。然后对每个范例进行单独的研究。这特别允许推导一个一般的和可实现的界。这个界限非常简单:它取决于用于冷却感兴趣系统的环境/机器的单个参数。关联的创建部分致力于定量研究给定能量可以创建多少关联。在精确地表述了感兴趣的问题之后,我们求解了任意有限维二部系统的背景温度消失问题。对于不消失的背景温度,问题的对称性被打破,使其更难处理。当两个系统是彼此的副本时,恢复足够的对称性来制定一个对所有(有限)维系统有效的上界,并证明其在维3和维4上的可达性。我们进一步推测,并证明了在任何维度上都可以达到的界限。
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引用次数: 1
Variational quantum simulations of stochastic differential equations 随机微分方程的变分量子模拟
Pub Date : 2020-12-08 DOI: 10.1103/PhysRevA.103.052425
K. Kubo, Yuya O. Nakagawa, Suguru Endo, S. Nagayama
Stochastic differential equations (SDE), which models uncertain phenomena as the time evolution of random variables, are exploited in various fields of natural and social sciences such as finance. Since SDEs rarely admit analytical solutions and must usually be solved numerically with huge classical-computational resources in practical applications, there is strong motivation to use quantum computation to accelerate the calculation. Here, we propose a quantum-classical hybrid algorithm that solves SDEs based on variational quantum simulation (VQS). We first approximate the target SDE by a trinomial tree structure with discretization and then formulate it as the time-evolution of a quantum state embedding the probability distributions of the SDE variables. We embed the probability distribution directly in the amplitudes of the quantum state while the previous studies did the square-root of the probability distribution in the amplitudes. Our embedding enables us to construct simple quantum circuits that simulate the time-evolution of the state for general SDEs. We also develop a scheme to compute the expectation values of the SDE variables and discuss whether our scheme can achieve quantum speed-up for the expectation-value evaluations of the SDE variables. Finally, we numerically validate our algorithm by simulating several types of stochastic processes. Our proposal provides a new direction for simulating SDEs on quantum computers.
随机微分方程(SDE)将不确定现象建模为随机变量的时间演化,在金融等自然科学和社会科学的各个领域都得到了应用。由于SDEs很少允许解析解,并且在实际应用中通常必须使用大量的经典计算资源进行数值求解,因此使用量子计算来加速计算具有强烈的动机。在此,我们提出一种基于变分量子模拟(VQS)的量子经典混合算法来求解SDEs。我们首先用离散化的三叉树结构近似目标SDE,然后将其表述为嵌入SDE变量概率分布的量子态的时间演化。我们将概率分布直接嵌入到量子态的幅值中,而以前的研究是在幅值中嵌入概率分布的平方根。我们的嵌入使我们能够构建简单的量子电路来模拟一般sde状态的时间演化。我们还开发了一种计算SDE变量期望值的方案,并讨论了该方案是否可以实现SDE变量期望值计算的量子加速。最后,我们通过模拟几种类型的随机过程来数值验证我们的算法。我们的研究为在量子计算机上模拟SDEs提供了一个新的方向。
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引用次数: 26
Phase sensitivity approaching the quantum Cramér-Rao bound in a modified SU(1,1) interferometer 改进SU(1,1)干涉仪中接近量子cram<s:1> - rao界的相位灵敏度
Pub Date : 2020-12-08 DOI: 10.1103/PHYSREVA.103.032617
Jian-Dong Zhang, Chenglong You, Chuang Li, Shuai Wang
SU(1,1) interferometers, based on the usage of nonlinear elements, are superior to passive interferometers in phase sensitivity. However, the SU(1,1) interferometer cannot make full use of photons carrying phase information as the second nonlinear element annihilates some of the photons inside. Here, we focus on improving phase sensitivity and propose a new protocol based on a modified SU(1,1) interferometer, where the second nonlinear element is replaced by a beam splitter. We utilize two coherent states as inputs and implement balanced homodyne measurement at the output. Our analysis suggests that the protocol we propose can achieve sub-shot-noise-limited phase sensitivity and is robust against photon loss and background noise. Our work is important for practical quantum metrology using SU(1,1) interferometers.
基于非线性元件的SU(1,1)干涉仪在相位灵敏度上优于无源干涉仪。然而,SU(1,1)干涉仪不能充分利用携带相位信息的光子,因为第二非线性元件会湮灭其中的一些光子。在此,我们着重于提高相位灵敏度,并提出了一种基于改进SU(1,1)干涉仪的新协议,其中第二非线性元件由分束器取代。我们利用两个相干态作为输入,并在输出处实现平衡同差测量。我们的分析表明,我们提出的协议可以实现亚短噪声限制的相位灵敏度,并且对光子损失和背景噪声具有鲁棒性。本文的工作对实际使用SU(1,1)干涉仪进行量子计量具有重要意义。
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引用次数: 6
Reachability in Controlled Markovian Quantum Systems: An Operator-Theoretic Approach 受控马尔可夫量子系统的可达性:一种算子论方法
Pub Date : 2020-12-07 DOI: 10.14459/2020md1559809
F. V. Ende
In quantum systems theory one of the fundamental problems boils down to: Given an initial state, which final states can be reached by the dynamic system in question? Formulated in the framework of bilinear control systems, the evolution shall be governed by an inevitable Hamiltonian drift term, finitely many control Hamiltonians allowing for (at least) piecewise constant control amplitudes, plus a (possibly bang-bang switchable) noise term in Kossakowski-Lindblad form. Now assuming switchable coupling of finite-dimensional systems to a thermal bath of arbitrary temperature, the core problem of reachability boils down to studying points in the standard simplex amenable to two types of controls that can be used interleaved: Permutations within the simplex, and contractions by a dissipative one-parameter semigroup. We illustrate how the solutions of the core problem pertain to the reachable set of the original controlled Markovian quantum system. This allows us to show that for global as well as local switchable coupling to a temperature-zero bath one can generate every quantum state from every initial state up to arbitrary precision. Moreover we present an inclusion for non-zero temperatures as a consequence of our results on d-majorization. Then we consider infinite-dimensional open quantum-dynamical systems following a unital Kossakowski-Lindblad master equation extended by controls. Here the drift Hamiltonian can be arbitrary, the finitely many control Hamiltonians are bounded, and the switchable noise term is generated by a single compact normal operator. Via new majorization results of ours, we show that such bilinear quantum control systems allow to approximately reach any target state majorized by the initial one, as up to now only has been known in finite-dimensional analogues.
在量子系统理论中,一个基本问题可以归结为:给定一个初始状态,所讨论的动态系统可以达到哪些最终状态?在双线性控制系统的框架中,演化应由一个不可避免的哈密顿漂移项,有限个控制哈密顿量允许(至少)分段恒定的控制幅度,加上一个(可能是bang-bang可切换的)Kossakowski-Lindblad形式的噪声项来控制。现在,假设有限维系统与任意温度的热浴的可切换耦合,可达性的核心问题归结为研究标准单纯形中的点,这些点适用于两种可交错使用的控制:单纯形内的置换和耗散单参数半群的收缩。我们说明了核心问题的解如何与原始受控马尔可夫量子系统的可达集有关。这使我们能够证明,对于全局和局部可切换耦合到零温度浴,可以从每个初始状态生成任意精度的每个量子态。此外,我们提出了一个包含非零温度作为我们的结果在d-多数化。然后,我们考虑无限维开放量子动力系统遵循由控制扩展的一元Kossakowski-Lindblad主方程。其中,漂移哈密顿量可以是任意的,有限个控制哈密顿量是有界的,可切换噪声项由单个紧正规算子产生。通过我们的新多数化结果,我们表明这种双线性量子控制系统允许近似达到任何被初始状态多数化的目标状态,因为到目前为止只在有限维类似物中已知。
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引用次数: 5
Operational Significance of the Quantum Resource Theory of Buscemi Nonlocality Buscemi非定域量子资源理论的运算意义
Pub Date : 2020-12-07 DOI: 10.1103/PRXQUANTUM.2.020301
Patryk Lipka-Bartosik, Andrés F. Ducuara, T. Purves, Paul Skrzypczyk
Although entanglement is necessary for observing nonlocality in a Bell experiment, there are entangled states which can never be used to demonstrate nonlocal correlations. In a seminal paper [PRL 108, 200401 (2012)] F. Buscemi extended the standard Bell experiment by allowing Alice and Bob to be asked quantum, instead of classical, questions. This gives rise to a broader notion of nonlocality, one which can be observed for every entangled state. In this work we study a resource theory of this type of nonlocality referred to as Buscemi nonlocality. We propose a geometric quantifier measuring the ability of a given state and local measurements to produce Buscemi nonlocal correlations and establish its operational significance. In particular, we show that any distributed measurement which can demonstrate Buscemi nonlocal correlations provides strictly better performance than any distributed measurement which does not use entanglement in the task of distributed state discrimination. We also show that the maximal amount of Buscemi nonlocality that can be generated using a given state is precisely equal to its entanglement content. Finally, we prove a quantitative relationship between: Buscemi nonlocality, the ability to perform nonclassical teleportation, and entanglement. Using this relationship we propose new discrimination tasks for which nonclassical teleportation and entanglement lead to an advantage over their classical counterparts.
虽然在贝尔实验中,纠缠态对于观察非局域性是必要的,但是纠缠态永远不能用于证明非局域相关。在一篇开创性的论文[PRL 108, 200401(2012)]中,F. Buscemi扩展了标准贝尔实验,允许Alice和Bob被问量子问题,而不是经典问题。这产生了一个更广泛的非定域性概念,它可以在每个纠缠态中被观察到。在这项工作中,我们研究了这种类型的非定域性资源理论,称为Buscemi非定域性。我们提出了一个几何量词来测量给定状态和局部测量产生Buscemi非局部相关的能力,并建立了它的操作意义。特别是,我们证明了任何能够证明Buscemi非局部相关的分布式测量在分布式状态判别任务中比任何不使用纠缠的分布式测量提供了严格更好的性能。我们还证明了使用给定状态可以产生的Buscemi非定域性的最大数量恰好等于它的纠缠内容。最后,我们证明了Buscemi非定域性、执行非经典隐形传态的能力和纠缠之间的定量关系。利用这种关系,我们提出了新的判别任务,其中非经典隐形传态和纠缠导致优于经典对应任务的优势。
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引用次数: 7
期刊
arXiv: Quantum Physics
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