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Sub-nanosecond coherent optical manipulation of a single aromatic molecule at cryogenic temperature 在低温条件下对单个芳香族分子进行亚纳秒级相干光操纵
Q2 QUANTUM SCIENCE & TECHNOLOGY Pub Date : 2023-12-01 DOI: 10.1116/5.0180689
Q. Deplano, P. Tamarat, B. Lounis, Jean-Baptiste Trebbia
Single molecules trapped in the solid state at liquid helium temperatures are promising quantum emitters for the development of quantum technologies owing to their remarkable photostability and their lifetime-limited optical coherence time of the order of 10 ns. The coherent preparation of their electronic state requires resonant excitation with a Rabi period much shorter than their optical coherence time. Sculpting the optical excitation with sharp edges and a high on–off intensity ratio (∼3 × 105) from a single-frequency laser beam, we demonstrate sub-nanosecond drive of a single dibenzanthanthrene molecule embedded in a naphthalene matrix at 3.2 K, over more than 17 Rabi periods. With pulses tailored for a half-Rabi period, the electronic excited state is prepared with fidelity as high as 0.97. Using single-molecule Ramsey spectroscopy, we prove up to 5 K that the optical coherence lifetime remains at its fundamental upper limit set by twice the excited-state lifetime, making single molecules suitable for quantum bit manipulations under standard cryogen-free cooling technologies.
在液氦温度下被困在固态中的单分子具有优异的光稳定性和10 ns量级的光学相干时间,是发展量子技术的有前途的量子发射体。其电子态的相干制备需要比光学相干时间短得多的拉比周期共振激发。利用单频激光束雕刻出具有锐利边缘和高开关强度比(~ 3 × 105)的光激发,我们演示了在3.2 K下嵌入萘基质中的单个二苯并蒽分子在超过17个拉比周期内的亚纳秒驱动。利用半拉比周期的脉冲,制备出的电子激发态保真度高达0.97。利用单分子拉姆齐光谱,我们证明了在5k下,光相干寿命保持在其基本上限,是激发态寿命的两倍,使得单分子适合在标准无冷冷却技术下进行量子比特操作。
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引用次数: 0
Single-photon-based clock analysis and recovery in quantum key distribution 量子密钥分发中基于单光子的时钟分析和恢复
Q2 QUANTUM SCIENCE & TECHNOLOGY Pub Date : 2023-11-23 DOI: 10.1116/5.0167549
M. Zahidy, D. Ribezzo, R. Muller, J. Riebesehl, A. Zavatta, M. Galili, L. Oxenløwe, Davide Bacco
Quantum key distribution is one of the first quantum technologies ready for the market. Current quantum telecommunication systems usually utilize a service channel for synchronizing the transmitter (Alice) and the receiver (Bob). However, the possibility of removing this service channel and exploiting a clock recovery method are intriguing for future implementation, both in fiber and free-space links. In this paper, we investigate criteria to recover the clock in a quantum communication scenario and experimentally demonstrated the possibility of using a quantum-based clock recovery system in a time-bin quantum key distribution protocol. The performance of the clock recovery technique, in terms of quantum bit error rate and secret key rate, is equivalent to using the service channel for clock sharing.
量子密钥分发是最早进入市场的量子技术之一。当前的量子通信系统通常利用服务通道来同步发送器(Alice)和接收器(Bob)。然而,无论是在光纤链路还是自由空间链路中,移除服务信道并利用时钟恢复方法的可能性对未来的实施都很有吸引力。在本文中,我们研究了在量子通信场景中恢复时钟的标准,并通过实验证明了在分时量子密钥分发协议中使用基于量子的时钟恢复系统的可能性。就量子比特错误率和秘钥率而言,时钟恢复技术的性能等同于使用服务信道进行时钟共享。
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引用次数: 0
Estimation of the number of single-photon emitters for multiple fluorophores with the same spectral signature 具有相同光谱特征的多个荧光团的单光子发射体数量的估计
Q2 QUANTUM SCIENCE & TECHNOLOGY Pub Date : 2023-11-14 DOI: 10.1116/5.0162501
Wenchao Li, Shuo Li, Timothy C. Brown, Qiang Sun, Xuezhi Wang, Vladislav V. Yakovlev, Allison Kealy, Bill Moran, Andrew D. Greentree
Fluorescence microscopy is of vital importance for understanding biological function. However, most fluorescence experiments are only qualitative inasmuch as the absolute number of fluorescent particles can often not be determined. Additionally, conventional approaches to measuring fluorescence intensity cannot distinguish between two or more fluorophores that are excited and emit in the same spectral window, as only the total intensity in a spectral window can be obtained. Here we show that, by using photon number resolving experiments, we are able to determine the number of emitters and their probability of emission for a number of different species, all with the same measured spectral signature. We illustrate our ideas by showing the determination of the number of emitters per species and the probability of photon collection from that species, for one, two and three otherwise unresolvable fluorophores. The convolution binomial model is presented to represent the counted photons emitted by multiple species. Then, the expectation-maximization (EM) algorithm is used to match the measured photon counts to the expected convolution binomial distribution function. In applying the EM algorithm, to leverage the problem of being trapped in a sub-optimal solution, the moment method is introduced to yield an initial guess for the EM algorithm. Additionally, the associated Cramér–Rao lower bound is derived and compared with the simulation results.
荧光显微镜对了解生物功能具有重要意义。然而,大多数荧光实验只是定性的,因为荧光粒子的绝对数量往往不能确定。此外,传统的测量荧光强度的方法不能区分两个或多个在同一光谱窗口中被激发和发射的荧光团,因为只能获得光谱窗口中的总强度。在这里,我们表明,通过使用光子数解析实验,我们能够确定许多不同物种的发射器数量及其发射概率,所有这些物种都具有相同的测量光谱特征。我们通过显示每个物种的发射器数量和从该物种收集光子的概率来说明我们的想法,对于一个,两个和三个其他无法分辨的荧光团。提出了一种卷积二项模型来表示多物种发射的光子计数。然后,利用期望最大化(EM)算法将测量到的光子数与期望卷积二项分布函数匹配。在应用EM算法时,为了解决陷入次优解的问题,引入矩量法对EM算法进行初始猜测。此外,还推导了相应的cram r - rao下界,并与仿真结果进行了比较。
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引用次数: 0
Atomic diffraction from single-photon transitions in gravity and Standard-Model extensions 引力中单光子跃迁的原子衍射和标准模型的扩展
Q2 QUANTUM SCIENCE & TECHNOLOGY Pub Date : 2023-11-14 DOI: 10.1116/5.0174258
Alexander Bott, Fabio Di Pumpo, Enno Giese
Single-photon transitions are one of the key technologies for designing and operating very-long-baseline atom interferometers tailored for terrestrial gravitational-wave and dark-matter detection. Since such setups aim at the detection of relativistic and beyond-Standard-Model physics, the analysis of interferometric phases as well as of atomic diffraction must be performed to this precision and including these effects. In contrast, most treatments focused on idealized diffraction so far. Here, we study single-photon transitions, both magnetically induced and direct ones, in gravity and Standard-Model extensions modeling dark matter as well as Einstein-equivalence-principle violations. We take into account relativistic effects like the coupling of internal to center-of-mass degrees of freedom, induced by the mass defect, as well as the gravitational redshift of the diffracting light pulse. To this end, we also include chirping of the light pulse required by terrestrial setups, as well as its associated modified momentum transfer for single-photon transitions.
单光子跃迁是设计和运行用于地面引力波和暗物质探测的超长基线原子干涉仪的关键技术之一。由于这些装置的目的是检测相对论和超标准模型物理,干涉相位和原子衍射的分析必须达到这个精度,并包括这些效应。相比之下,迄今为止,大多数处理都集中在理想衍射上。在这里,我们研究了单光子跃迁,包括磁诱导和直接跃迁,在引力和标准模型扩展中模拟暗物质以及爱因斯坦等效原理的违反。我们考虑了由质量缺陷引起的内部和质心自由度的耦合等相对论性效应,以及衍射光脉冲的引力红移。为此,我们还包括地面装置所需的光脉冲啁啾,以及其相关的单光子跃迁修正动量转移。
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引用次数: 2
Efficient numerical description of the dynamics of interacting multispecies quantum gases 相互作用的多种量子气体动力学的有效数值描述
Q2 QUANTUM SCIENCE & TECHNOLOGY Pub Date : 2023-11-07 DOI: 10.1116/5.0163850
Annie Pichery, Matthias Meister, Baptist Piest, Jonas Böhm, Ernst Maria Rasel, Eric Charron, Naceur Gaaloul
We present a highly efficient method for the numerical solution of coupled Gross–Pitaevskii equations describing the evolution dynamics of a multi-species mixture of Bose–Einstein condensates in time-dependent potentials. This method, based on a moving and expanding reference frame, compares favorably to a more standard but much more computationally expensive solution based on a frozen frame. It allows an accurate description of the long-time behavior of interacting, multi-species quantum mixtures including the challenging problem of long free expansions relevant to microgravity and space experiments. We demonstrate a successful comparison to experimental measurements of a binary Rb–K mixture recently performed with the payload of a sounding rocket experiment.
我们提出了一种高效的方法来数值求解描述多组分玻色-爱因斯坦凝聚体在时变势下的演化动力学的Gross-Pitaevskii方程。这种基于移动和扩展参考系的方法优于基于固定参考系的更标准但计算成本更高的解决方案。它可以精确描述相互作用的长时间行为,多物种量子混合物,包括与微重力和空间实验相关的长时间自由膨胀的挑战性问题。我们演示了最近用探空火箭实验的有效载荷进行的二元Rb-K混合物的实验测量的成功比较。
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引用次数: 2
ℓ 00 ℓ entanglement and the twisted quantum eraser 和扭曲量子擦除器
Q2 QUANTUM SCIENCE & TECHNOLOGY Pub Date : 2023-11-07 DOI: 10.1116/5.0167938
Dylan Danese, Sabine Wollmann, Saroch Leedumrongwatthanakun, Will McCutcheon, Manuel Erhard, William N. Plick, Mehul Malik
We demonstrate the generation of unbalanced two-photon entanglement in the Laguerre–Gaussian (LG) transverse-spatial degree-of-freedom, where one photon carries a fundamental (Gauss) mode and the other a higher-order LG mode with a non-zero azimuthal (ℓ) or radial (p) component. Taking a cue from the N00N state nomenclature, we call these types of states ℓ00ℓ-entangled. They are generated by shifting one photon in the LG mode space and combining it with a second (initially uncorrelated) photon at a beamsplitter, followed by coincidence detection. In order to verify two-photon coherence, we demonstrate a two-photon “twisted” quantum eraser, where Hong–Ou–Mandel interference is recovered between two distinguishable photons by projecting them into a rotated LG superposition basis. Using an entanglement witness, we find that our generated states have fidelities of 95.31% and 89.80% to their respective ideal maximally entangled states. In addition to being of fundamental interest, this type of entanglement will likely have a significant impact on tickling the average quantum physicist's funny bone.
我们展示了在拉盖尔-高斯(LG)横空间自由度中产生的不平衡双光子纠缠,其中一个光子携带基本(高斯)模式,另一个光子携带具有非零方位(r)或径向(p)分量的高阶LG模式。从N00N态的命名法中得到提示,我们称这些态为l00l00纠缠态。它们是通过移动LG模式空间中的一个光子,并在分束器中将其与第二个(最初不相关的)光子结合,然后进行巧合检测而产生的。为了验证双光子相干性,我们展示了一个双光子“扭曲”量子擦除器,其中Hong-Ou-Mandel干涉通过将两个可区分的光子投射到旋转的LG叠加基中来恢复。使用纠缠见证,我们发现我们生成的状态对各自的理想最大纠缠态的保真度分别为95.31%和89.80%。除了具有基本的兴趣之外,这种类型的纠缠可能会对普通量子物理学家的笑料产生重大影响。
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引用次数: 0
Emulating an atomic gyroscope with multiple accelerometers 模拟具有多个加速度计的原子陀螺仪
Q2 QUANTUM SCIENCE & TECHNOLOGY Pub Date : 2023-11-03 DOI: 10.1116/5.0166281
Nathan Shettell, Rainer Dumke
The main advantage of an atomic accelerometer when compared to a classical accelerometer is negligible bias drift, allowing for stable long-term measurements, which opens the potential application in navigation. This negligible drift arises from the fact that the measurements can be traced back to natural constants, and the system is intrinsically stable due to the simple design. In this manuscript, we extend this property of long-term stability to gyroscopic measurements by considering an array of atomic accelerometers, and comparing the performance to atomic gyroscopes, which are technologically more prone to bias drifts. We demonstrate that an array consisting of four three-axis atomic accelerometers can outperform state-of-the-art atomic gyroscopes with respect to long-term stability.
与传统加速度计相比,原子加速度计的主要优点是可以忽略偏置漂移,允许稳定的长期测量,这为导航打开了潜在的应用。这种可忽略的漂移源于这样一个事实,即测量可以追溯到自然常数,并且由于简单的设计,系统本质上是稳定的。在本文中,我们通过考虑一系列原子加速度计,将这种长期稳定性的特性扩展到陀螺仪测量,并将其性能与原子陀螺仪进行比较,原子陀螺仪在技术上更容易发生偏置漂移。我们证明了由四个三轴原子加速度计组成的阵列在长期稳定性方面优于最先进的原子陀螺仪。
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引用次数: 0
Detecting intermediate-mass black hole binaries with atom interferometer observatories: Using the resonant mode for the merger phase 用原子干涉仪观测中质量黑洞双星:利用合并相位的共振模式
Q2 QUANTUM SCIENCE & TECHNOLOGY Pub Date : 2023-11-01 DOI: 10.1116/5.0162505
Alejandro Torres-Orjuela
Atom interferometry detectors like AION, ZAIGA, and AEDGE will be able to detect gravitational waves (GWs) at dHz covering the band between large space-based laser interferometers LISA/TianQin/Taiji and ground-based facilities LIGO/Virgo/KAGRA. They will detect the late inspiral and merger of GW sources containing intermediate-mass black holes (IMBHs) in the mass range 102−105 M⊙. We study how accurately the parameters of an IMBH binary can be measured using AION's power spectral density. Furthermore, we propose a detection scheme where the early inspiral of the binary is detected using the regular broadband mode while the merger is detected using the resonant mode. We find that using such a detection scheme, the signal-to-noise ratio of the detection and the detection accuracy of the parameters can be enhanced compared to the full detection of the signal using the broadband mode. We, further, assess the impact of the necessary detection gap while switching from broadband to resonant mode studying the case of a short (30 s) and a long (600 s) gap. We find that the improvement in the detection accuracy for both gaps is around 40% for the total mass and the spin of the heavier black hole. For the short gap, the accuracy always improves ranging between 2% and 31% for the other parameters. For the long gap, there is a decrease in the detection accuracy for the luminosity distance, the inclination, and the initial phase but only by 1%–6% while for the remaining parameters, we have improved accuracies of around 2%–20%.
像AION、ZAIGA和AEDGE这样的原子干涉测量探测器将能够探测到覆盖在大型天基激光干涉仪LISA/TianQin/Taiji和地面设施LIGO/Virgo/KAGRA之间的dHz波段的引力波。他们将探测到含有质量范围在102 ~ 105 M⊙的中质量黑洞(IMBHs)的GW源的后期激发和合并。我们研究了利用AION的功率谱密度测量IMBH双星参数的准确性。此外,我们还提出了一种检测方案,其中使用常规宽带模式检测双星的早期启发,而使用谐振模式检测合并。我们发现,与使用宽带模式对信号进行全检测相比,使用这种检测方案可以提高检测的信噪比和参数的检测精度。我们进一步评估了从宽带模式切换到谐振模式时必要的检测间隙的影响,研究了短(30秒)和长(600秒)间隙的情况。我们发现,对于总质量和较重黑洞的自旋,两个间隙的探测精度都提高了40%左右。对于短间隙,其他参数的精度提高幅度在2% ~ 31%之间。对于较长的间隙,光度距离、倾角和初始相位的检测精度下降了1% ~ 6%,其余参数的检测精度提高了2% ~ 20%左右。
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引用次数: 0
Status of the GINGER project GINGER项目的状态
Q2 QUANTUM SCIENCE & TECHNOLOGY Pub Date : 2023-10-26 DOI: 10.1116/5.0167940
Carlo Altucci, Francesco Bajardi, Andrea Basti, Nicolò Beverini, Giorgio Carelli, Salvatore Capozziello, Simone Castellano, Donatella Ciampini, Fabrizio Davì, Francesco dell'Isola, Gaetano De Luca, Roberto Devoti, Giuseppe Di Somma, Angela D. V. Di Virgilio, Francesco Fuso, Ivan Giorgio, Aladino Govoni, Enrico Maccioni, Paolo Marsili, Antonello Ortolan, Alberto Porzio, Matteo Luca Ruggiero, Raffaele Velotta
Large frame ring laser gyroscopes, based on the Sagnac effect, are top sensitivity instrumentation to measure angular velocity with respect to the fixed stars. GINGER (Gyroscopes IN GEneral Relativity) project foresees the construction of an array of three large dimension ring laser gyroscopes, rigidly connected to the Earth. GINGER has the potentiality to measure general relativity effects and Lorentz Violation in the gravity sector, once a sensitivity of 10−9, or better, of the Earth rotation rate is obtained. Being attached to the Earth crust, the array will also provide useful data for geophysical investigation. For this purpose, it is at present under construction as part of the multi-components observatory called Underground Geophysics at Gran Sasso (UGSS). Sensitivity is the key point to determine the relevance of this instrument for fundamental science. The most recent progress in the sensitivity measurement, obtained on a ring laser prototype called GINGERINO, indicates that GINGER should reach the level of 1 part in 1011 of the Earth rotation rate.
基于Sagnac效应的大框架环形激光陀螺仪是测量恒星角速度的高灵敏度仪器。GINGER(广义相对论中的陀螺仪)项目预计将建造一个由三维环形激光陀螺仪组成的阵列,与地球紧密相连。一旦获得10−9或更高的地球自转速率灵敏度,GINGER就有可能测量引力部门的广义相对论效应和洛伦兹破坏。由于与地壳相连,该阵列还将为地球物理调查提供有用的数据。为此目的,它目前正在建设中,作为Gran Sasso地下地球物理(UGSS)多组件天文台的一部分。灵敏度是决定该仪器是否适用于基础科学的关键。在名为GINGERINO的环形激光样机上获得的灵敏度测量的最新进展表明,GINGER应该达到地球自转速度的1 / 1011的水平。
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引用次数: 0
Accelerating quantum optimal control of multi-qubit systems with symmetry-based Hamiltonian transformations 基于对称哈密顿变换的多量子位系统加速量子最优控制
Q2 QUANTUM SCIENCE & TECHNOLOGY Pub Date : 2023-10-03 DOI: 10.1116/5.0162455
Xian Wang, Mahmut Sait Okyay, Anshuman Kumar, Bryan M. Wong
We present a novel, computationally efficient approach to accelerate quantum optimal control calculations of large multi-qubit systems used in a variety of quantum computing applications. By leveraging the intrinsic symmetry of finite groups, the Hilbert space can be decomposed and the Hamiltonians block diagonalized to enable extremely fast quantum optimal control calculations. Our approach reduces the Hamiltonian size of an n-qubit system from 2n×2n to O(n×n) or O((2n/n)×(2n/n)) under Sn or Dn symmetry, respectively. Most importantly, this approach reduces the computational runtime of qubit optimal control calculations by orders of magnitude while maintaining the same accuracy as the conventional method. As prospective applications, we show that (1) symmetry-protected subspaces can be potential platforms for quantum error suppression and simulation of other quantum Hamiltonians and (2) Lie–Trotter–Suzuki decomposition approaches can generalize our method to a general variety of multi-qubit systems.
我们提出了一种新的,计算效率高的方法来加速各种量子计算应用中使用的大型多量子位系统的量子最优控制计算。利用有限群的固有对称性,可以对希尔伯特空间进行分解,并将哈密顿量块对角化,从而实现极快的量子最优控制计算。我们的方法将n-量子比特系统的哈密顿大小分别从2n×2n降低到O(n×n)或O((2n/n)×(2n/n)),在Sn或Dn对称下。最重要的是,该方法在保持与传统方法相同精度的同时,将量子比特最优控制计算的计算运行时间减少了几个数量级。作为潜在的应用,我们表明(1)对称保护子空间可以成为量子误差抑制和模拟其他量子哈密顿量的潜在平台;(2)Lie-Trotter-Suzuki分解方法可以将我们的方法推广到各种各样的多量子位系统。
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引用次数: 1
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AVS quantum science
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