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The process of molecular plating and the characteristics of the produced thin films – What we have learned in 60 years and what is still unknown 分子电镀的工艺和薄膜的特性——60年来我们学到了什么,还有什么是未知的
Pub Date : 2023-01-01 DOI: 10.1051/epjconf/202328503001
E. Artes, C. Düllmann, Carl-Christian Meyer, D. Renisch
Molecular plating is a well-established and widely used method for producing thin films of various elements, which are used in variety of nuclear physics applications. Sixty years have passed since the method was established, and some insights into the chemical process underlying the method and the composition of the thin films have been gained. A brief overview of what has been learned about molecular plating since its introduction and the methods applied in the characterization of molecular plated thin films is given here. Through various spectroscopic and microscopic methods, the process of molecular plating and the chemical composition are gradually being elucidated, albeit we still do not understand all aspects.
分子电镀是一种成熟而广泛使用的制备各种元素薄膜的方法,用于各种核物理应用。自该方法建立以来,已经过去了60年,人们对该方法的化学过程和薄膜的组成有了一些了解。本文简要介绍了分子镀技术自问世以来所取得的进展,以及分子镀薄膜的表征方法。通过各种光谱学和显微学的方法,分子电镀的过程和化学成分正在逐渐被阐明,尽管我们仍然不了解所有的方面。
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引用次数: 2
Neutrons propagation in Lead: A feasibility study for experiments in the RSV TAPIRO fast research reactor 中子在铅中的传播:RSV TAPIRO快堆实验的可行性研究
Pub Date : 2023-01-01 DOI: 10.1051/epjconf/202328408006
V. Fabrizio, N. Burgio, D. Castelluccio, L. Falconi, G. Grasso, F. Lodi, A. Mengoni, V. Peluso, R. Pergreffi, Alfonso Santagata, M. Sarotto
The increasing worldwide interest in Lead-cooled Fast Reactors (LFRs) substantiates the need to validate the analytical codes and methods used to support their design. For neutronic analyses, this is chiefly reflected in assessing the impact of nuclear data uncertainties on the integral and local parameters resulting from such analyses. The aim of refining nuclear data moves continuous efforts for more accurate measurements, be them differential or integral, for which adequate facilities are required. The availability at the ENEA's Casaccia research center of a fast source reactor – RSV TAPIRO – provides a unique opportunity to perform new integral experiments in support of fast reactors, including LFRs, owing to the well-characterized neutron spectrum of the thermal column. A series of experiments has been envisaged, dealing with the use of Lead in a reactor. The experiments concern the propagation of neutrons through blocks of materials representing relevant elements of a reactor core, and ranging from pure Lead to mixtures reproducing portions of the reflector and shield in LFRs. The paper is focused on the feasibility study of some of these experiments in which Lead and mixture blocks are inserted in the so-called thermal column of the RSV TAPIRO reactor and irradiated by the neutron flux emerging from the Copper reflector surrounding the reactor core.
世界范围内对铅冷快堆(LFRs)日益增长的兴趣证实了验证用于支持其设计的分析规范和方法的必要性。对于中子分析,这主要体现在评估核数据不确定性对这些分析产生的积分和局部参数的影响。为了完善核数据,需要不断努力进行更精确的测量,无论是微分测量还是积分测量,为此需要适当的设施。ENEA Casaccia研究中心的快源反应堆RSV TAPIRO提供了一个独特的机会来进行新的集成实验,以支持包括LFRs在内的快堆,由于热柱的中子谱特征良好。已经设想了一系列关于铅在反应堆中的使用的实验。实验涉及中子通过代表反应堆堆芯相关元素的材料块的传播,范围从纯铅到复制lfr中反射器和屏蔽部分的混合物。本文重点研究了将铅和混合块插入RSV TAPIRO反应堆的所谓热柱中,并由反应堆堆芯周围铜反射器产生的中子通量照射的一些实验的可行性。
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引用次数: 0
Magnetic and non-magnetic AGB mixing for s-processing 用于s加工的磁性和非磁性AGB混合
Pub Date : 2023-01-01 DOI: 10.1051/epjconf/202327501005
M. Busso
I outline a few features of recent models for the formation of the neutron source 13C(α,n)16O in low mass stars (1 ≲ M/M⊙ ≲ 3, LMS ) ascendingfor the second time the Red Giant Branch, generally called Asymptotic Giant Branch, or AGB stars. I also briefly outline the nucleosynthesis results obtained trough them. The mentioned models consider the physical structure below the frequent downward extensions of the convective envelope into the He-intershell (the so-called third dredge-up or TDU episodes). There, the conditions are such that the occurrence of further mixing is strongly facilitated, due to the minimal temperature gradient. A way to induce proton mixing from the envelope (certainly not the only one) arises whenever the ambient magnetic fields expected for LMS promote the buoyancy of strongly magnetized flux tubes. I review some characteristics of the ensuing mixing episodes, mentioning how different hydrodynamical processes might yield similar effects, thus encouraging stellar physicists to verify in more detail this possibility.
我概述了中子源13C(α,n)16O在低质量恒星(1 > M/M⊙> 3,LMS)第二次上升的红巨星分支(通常称为渐近巨星分支,或AGB恒星中形成的最新模型的一些特征。我还简要概述了通过它们获得的核合成结果。上述模型考虑了对流包络层频繁向下延伸进入He-intershell(所谓的第三次挖掘或TDU事件)以下的物理结构。在这种情况下,由于温度梯度最小,进一步混合的发生非常容易。每当LMS所期望的环境磁场促进强磁化磁通管的浮力时,就会出现一种从包络层诱导质子混合的方法(当然不是唯一的方法)。我回顾了随后的混合事件的一些特征,提到不同的流体动力过程如何产生相似的效果,从而鼓励恒星物理学家更详细地验证这种可能性。
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引用次数: 0
Generation of thermal scattering laws with the CINEL code 用CINEL代码生成热散射定律
Pub Date : 2023-01-01 DOI: 10.1051/epjconf/202328417002
G. Noguere, S. Xu, L. Desgrange, J. Boucher, E. Bourasseau, G. Carlot, A. Filhol, J. Ollivier, T. Hansen, V. Nassif, I. Ouente Orench, C. Colin, L. Laversenne, J. Zanotti, Q. Berrod
The thermal scattering laws (TSL) take into account the crystalline structure and atomic motions of isotopes bound in materials. This paper presents the CINEL code, which was developed to generate temperature-dependent TSL for solid, liquid and free gas materials of interest for nuclear reactors. CINEL is able to calculate TSL from the phonon density of states (PDOS) of materials under the Gaussian-Incoherent approximations. The PDOS can be obtained by using theoretical approaches (e.g., ab initio density functional theory and molecular dynamics) or experimental results. In this work, the PDOS presented in the ENDF/BVIII.0 and NJOY-NCrystal libraries were used for numerical validation purposes. The CINEL results are in good agreement with those reported in these databases, even in the specific cases of TSL with the newly mixed elastic format. The coding flexibility offered by Python using the JupyterLab interface allowed to investigate limits of physical models reported in the literature, such as a four-site model for UO2, anharmonic behaviors of oxygen atoms bound in a Fm3m structure, texture in Zry4 samples and jump corrections in a roto-translational diffusion model for liquid water. The use of graphic processing units (GPU) is a necessity to perform calculations in a few minutes. The performances of the CINEL code is illustrated with the results obtained on actinide oxides having a Fm3m structure (UO2, ThO2, NpO2 and PuO2), low enriched fuel (UMo), cladding (Zry4) and moderators (H2O with a specific emphasis on ice).
热散射定律(TSL)考虑了材料中结合的同位素的晶体结构和原子运动。本文介绍了CINEL代码,该代码用于为核反应堆中感兴趣的固体、液体和自由气体材料生成温度相关的TSL。CINEL能够在高斯-非相干近似下从材料的声子态密度(PDOS)计算出TSL。PDOS可以通过理论方法(例如从头算密度泛函理论和分子动力学)或实验结果获得。在这项工作中,PDOS在ENDF/BVIII中提出。0和NJOY-NCrystal库用于数值验证目的。CINEL结果与这些数据库中报告的结果一致,即使在具有新混合弹性格式的TSL的特定情况下也是如此。Python使用JupyterLab接口提供的编码灵活性允许研究文献中报道的物理模型的局限性,例如UO2的四位点模型,Fm3m结构中氧原子的非调和行为,Zry4样品中的织体以及液态水的旋转-平移扩散模型中的跳跃修正。图形处理单元(GPU)的使用是在几分钟内执行计算的必要条件。CINEL代码的性能用具有Fm3m结构的锕系氧化物(UO2, ThO2, NpO2和PuO2),低富集燃料(UMo),包层(Zry4)和减速剂(H2O,特别强调冰)的结果来说明。
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引用次数: 1
Prediction of prompt neutron spectra of the photon induced reactions on 238U and 232Th targets at incident energies from 4 to 22 MeV 4 ~ 22mev入射能量下238U和232Th靶上光子诱导反应的提示中子谱预测
Pub Date : 2023-01-01 DOI: 10.1051/epjconf/202328404024
A. Tudora, D. Filipescu, I. Gheorghe
The processing of experimental data for the photon induced reactions on 238U and 232Th investigated by quasi-monochromatic γ-ray beams (produced in Laser Compton scattering at the NewSUBARU facility) needs the prediction of prompt neutron spectra. They are obtained using reliable models and systematics, i.e. the most employed and well validated approach of the most probable fragmentation with input parameters provided by a recent systematic and fission chance probabilities based on nuclear reaction calculations performed with the EMPIRE code.
准单色γ射线束(在NewSUBARU激光康普顿散射中产生)对238U和232Th的光子诱导反应实验数据的处理需要提示中子谱的预测。它们是使用可靠的模型和系统学获得的,即最常用和最有效的最可能破碎的方法,输入参数由最近的系统和裂变机会概率提供,该方法基于使用EMPIRE代码进行的核反应计算。
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引用次数: 0
The Münster cluster-jet target for the future P̅ANDA experiment 为未来的P - ANDA实验准备的m<s:1> nster簇射目标
Pub Date : 2023-01-01 DOI: 10.1051/epjconf/202328502002
S. Vestrick, P. Brand, D. Bonaventura, Hanna Eick, C. Mannweiler, A. Khoukaz
For high precision storage ring experiments as the future P̅ANDA experiment, very sophisticated internal targets have to be used. For this purpose, a state-of-the-art cluster-jet target was developed at the University Münster. Basically, hydrogen is cooled to cryogenic temperatures and pressed through a specially shaped Laval nozzle to form a cluster-jet expanding into vacuum. Due to the stability and large mass of the clusters, a practically undisturbed flight path in vacuum of above 5 m is possible, leading to manifold possible applications, including the interaction with a storage ring beam at a distance of 2.25 m as desired for the P̅ANDA experiment. With a first prototype target, the “proof-of-principle” was delivered, and after first improvements the world record in target thickness in such large distance to the nozzle was measured. Based on this work, the final P̅ANDA cluster-jet target was developed and built up, and is presented in this article.
对于高精度的存储环实验,如未来的P ~ ANDA实验,必须使用非常复杂的内部靶。为此目的,大学 nster开发了一种最先进的集束喷射靶。基本上,氢气被冷却到低温,并通过一个特殊形状的拉瓦尔喷嘴被压制,形成一个膨胀到真空的簇状射流。由于团簇的稳定性和大质量,在5米以上的真空中几乎不受干扰的飞行路径是可能的,导致多种可能的应用,包括与P ' ANDA实验所需的2.25米距离的存储环束相互作用。有了第一个原型靶,“原理证明”就交付了,经过首次改进,在距离喷嘴如此之大的距离上测量了靶厚度的世界纪录。在此基础上,研制并建立了最终的p_anda集束喷射靶,并在本文中进行了介绍。
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引用次数: 0
Gyrotron anode voltage control in EAST ECRH system EAST ECRH系统回旋管阳极电压控制
Pub Date : 2023-01-01 DOI: 10.1051/epjconf/202327704007
Weiye Xu, Handong Xu, Jian Zhang, Fei Guo, Haozhang Sun
Four diode-type gyrotrons are used in the EAST ECRH system now. The anode is one of the main components of the gyrotron. We can control the output power of the gyrotron by changing the anode voltage. An anode voltage control system for ASIPP anode power supplies was developed based on the ethernet CompactDAQ chassis NI-cDAQ-9185. The anode voltage can be controlled up to 30 kV, and the maximum current is 100 mA. The maximum modulation frequency is 5 kHz at a 50% duty cycle.
目前在EAST ECRH系统中使用了四个二极管型回旋管。阳极是回旋管的主要组成部分之一。通过改变阳极电压,可以控制回旋管的输出功率。基于以太网CompactDAQ机箱NI-cDAQ-9185,开发了一种用于ASIPP阳极电源的阳极电压控制系统。阳极电压可控制至30kv,最大电流为100ma。最大调制频率为5khz,占空比为50%。
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引用次数: 0
Hadron production from heavy ion collisions 重离子碰撞产生强子
Pub Date : 2023-01-01 DOI: 10.1051/epjconf/202327606001
C. Ko
A brief review of some topics in hadron production from heavy ion collisions is given. They include charged pion ratio as a probe of nuclear symmetry energy, in-medium effects on pion production, en- hanced Λc/D0 ratio, Λ local polarization, and X(3872) production.
本文对重离子碰撞产生强子的一些问题作了简要评述。它们包括作为核对称能探测的带电介子比、介子产生的介质效应、增强的Λc/D0比、Λ局部极化和X(3872)产生。
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引用次数: 0
Design of Stray Radiation Sensor for ITER ECE Diagnostic ITER ECE诊断用杂散辐射传感器设计
Pub Date : 2023-01-01 DOI: 10.1051/epjconf/202327703010
S. Danani, Sheetal Punia, R.A.V. Kumar, H. Pandya, Vinay Kumar
The Electron Cyclotron Emission (ECE) diagnostic has a primary role in the measurement of electron temperature profile and electron temperature fluctuations in ITER. This diagnostic shall be exposed to significant power due to unabsorbed Electron Cyclotron Heating (ECH) power in the plasma. The expected stray power loads could be a few tens of watts, and therefore, the protection of millimetre wave components is one of the design challenges of ITER ECE diagnostic. This protection system includes sensors, a band stop notch filter, and a shutter to stop the RF stray radiation from being incident on the sensitive components. The sensors will be positioned along the ECE transmission line, and shall be used for real-time power monitoring of the stray radiation. Here, we describe a novel design of a sensor for monitoring the stray radiation power. This sensor is a Schottky Diode rectenna, known for high-power and high-speed millimetre wave detection capability. It consists of a 2x2 microstrip patch antenna array, a matching circuit, a diode, and a low pass filter. The antenna array is designed analytically and optimized in CST Microwave Studio, for wide reception angle, high gain, and low side lobe levels. Furthermore, the rectifying circuit is optimized using Agilent Advanced Design System (ADS) software to get better rectification and impedance matching of the signal, thereby improving its detection sensitivity. The ADS simulation results show that the detection sensitivity is about 1000V/W for input power of -30 dBm at 170 GHz, thereby achieving the required performance of the sensor.
电子回旋发射(ECE)诊断在ITER中电子温度分布和电子温度波动的测量中起着主要作用。由于等离子体中未吸收的电子回旋加热(ECH)功率,该诊断应暴露在显著的功率下。预期的杂散功率负载可能是几十瓦,因此,毫米波组件的保护是ITER ECE诊断的设计挑战之一。该保护系统包括传感器、带阻陷波滤波器和快门,以阻止射频杂散辐射入射到敏感元件上。传感器将沿ECE传输线放置,用于对杂散辐射进行实时功率监测。本文介绍了一种新型的杂散辐射功率传感器的设计。该传感器是肖特基二极管整流天线,以高功率和高速毫米波检测能力而闻名。它由一个2x2微带贴片天线阵列、一个匹配电路、一个二极管和一个低通滤波器组成。该天线阵列在CST Microwave Studio中进行了分析和优化设计,具有宽接收角度,高增益和低旁瓣电平。利用安捷伦先进设计系统(Agilent Advanced Design System, ADS)软件对整流电路进行优化,使信号得到更好的整流和阻抗匹配,从而提高其检测灵敏度。ADS仿真结果表明,在170 GHz频率下,当输入功率为-30 dBm时,检测灵敏度约为1000V/W,从而达到了传感器所要求的性能。
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引用次数: 0
Activation cross-sections for short-lived reaction products on hafnium isotopes induced by 1 – 20 MeV neutrons 1 - 20mev中子诱导的铪同位素短寿命反应产物的活化截面
Pub Date : 2023-01-01 DOI: 10.1051/epjconf/202328401038
V. Semkova, A. Demerdjiev, A. Moens, N. Otuka, A. Plompen, D. Tonev
Results of new activation cross-section measurements for production of 178m1Hf (T1/2 = 4.0 s) and 179m1Hf (T1/2 = 18.67 s) are presented for the following reactions: 178Hf(n,n´)178m1Hf, 179Hf(n,2n)178m1Hf, 180Hf(n,3n)178m1Hf, 179Hf(n,n´)179m1Hf, and 180Hf(n,2n)179m1Hf. The irradiations were carried out at the 7-MV Van de Graaff accelerator at EC-JRC, Geel. Neutrons in the 1-3 MeV energy range were produced via the 3H(p,n)3He reaction. Deuteron beam and a deuterium gas target were used to produce 5 and 6 MeV neutrons. For the production of quasi-monoenergetic neutrons between 16 and 19.5 MeV the 3H(d,n)4He reactions was employed. Both samples with natural composition and isotopic enrichment were employed to differentiate reactions leading to the same product. An automated pneumatic system was used for the sample irradiation, transport and radioactivity measurements. The radioactivity of the samples was determined by standard gamma-spectrometry using HPGe detector. The results obtained in the present work are compared with the data from other authors and TENDL-2017 evaluation.
给出了178Hf(n,n´)178m1Hf、179Hf(n,2n)178m1Hf、180Hf(n,3n)178m1Hf、179Hf(n,n´)179m1Hf、180Hf(n, n´)179m1Hf和180Hf(n,2n)179m1Hf的新活化截面测量结果(T1/2 = 4.0 s)和179m1Hf (T1/2 = 18.67 s)。辐照是在Geel EC-JRC的7 mv Van de Graaff加速器上进行的。通过3H(p,n)3He反应产生1-3 MeV能量范围内的中子。氘核束和氘气体靶被用来产生5和6兆电子伏特的中子。对于16 ~ 19.5 MeV的准单能中子,采用3H(d,n)4He反应。这两种样品都具有天然组成和同位素富集,被用来区分导致相同产物的反应。采用自动化气动系统对样品进行辐照、输送和放射性测量。样品的放射性用HPGe探测器用标准伽马能谱法测定。将所得结果与其他作者的数据和TENDL-2017评估进行了比较。
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引用次数: 0
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