首页 > 最新文献

Environmental Pollutants and Bioavailability最新文献

英文 中文
Interaction of Perfluorooctanoic Acid with terrestrial plants: Uptake, transfer and phytotoxicity aspects 全氟辛酸与陆生植物的相互作用:吸收、转移和植物毒性方面
IF 3.3 4区 环境科学与生态学 Q2 BIOCHEMISTRY & MOLECULAR BIOLOGY Pub Date : 2022-11-06 DOI: 10.1080/26395940.2022.2142672
Hongyuan Li, Yujing Wang, Wenchao Du, Hua He, Shaogui Yang
ABSTRACT Soil contamination with perfluorooctanoic acid (PFOA) is a global concern. PFOA in soil can enter plants, affect plant growth and threaten food safety. Therefore, understanding the plant utilization and phytotoxicity of PFOA is conducive to assessing the environmental risk of soil contaminated with PFOA. This review analyzed recent studies about the uptake and effects of PFOA on terrestrial plants from the aspects of absorption, transport, distribution, phytotoxicity, and the underlying mechanism. Based on current research, PFOA was predominantly taken by plant roots and showed adverse effects on plants by affecting the antioxidant system and metabolic process. Research in field or higher terrestrial plants is still very scarce. Given the importance of exploring the potential remediation methods for PFOA, more research with comprehensive consideration of soil and environmental factors should be carried out to tell its specific mechanisms of plant utilization and toxicity action.
全氟辛酸(PFOA)土壤污染是一个全球关注的问题。土壤中的PFOA可以进入植物体内,影响植物生长,威胁食品安全。因此,了解PFOA的植物利用和植物毒性有利于评估PFOA污染土壤的环境风险。本文从PFOA对陆生植物的吸收、运输、分布、植物毒性及其作用机制等方面综述了近年来有关研究进展。根据目前的研究,PFOA主要通过植物根系吸收,并通过影响植物的抗氧化系统和代谢过程对植物产生不良影响。对田间或高等陆生植物的研究仍然很少。鉴于探索PFOA潜在的修复方法的重要性,需要开展更多综合考虑土壤和环境因素的研究,以了解其对植物利用和毒性作用的具体机制。
{"title":"Interaction of Perfluorooctanoic Acid with terrestrial plants: Uptake, transfer and phytotoxicity aspects","authors":"Hongyuan Li, Yujing Wang, Wenchao Du, Hua He, Shaogui Yang","doi":"10.1080/26395940.2022.2142672","DOIUrl":"https://doi.org/10.1080/26395940.2022.2142672","url":null,"abstract":"ABSTRACT Soil contamination with perfluorooctanoic acid (PFOA) is a global concern. PFOA in soil can enter plants, affect plant growth and threaten food safety. Therefore, understanding the plant utilization and phytotoxicity of PFOA is conducive to assessing the environmental risk of soil contaminated with PFOA. This review analyzed recent studies about the uptake and effects of PFOA on terrestrial plants from the aspects of absorption, transport, distribution, phytotoxicity, and the underlying mechanism. Based on current research, PFOA was predominantly taken by plant roots and showed adverse effects on plants by affecting the antioxidant system and metabolic process. Research in field or higher terrestrial plants is still very scarce. Given the importance of exploring the potential remediation methods for PFOA, more research with comprehensive consideration of soil and environmental factors should be carried out to tell its specific mechanisms of plant utilization and toxicity action.","PeriodicalId":11785,"journal":{"name":"Environmental Pollutants and Bioavailability","volume":"24 1","pages":"518 - 526"},"PeriodicalIF":3.3,"publicationDate":"2022-11-06","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"73487961","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 1
Approaches for treating domestic wastewater with food waste and recovery of potential resources 食物垃圾处理生活污水的方法及潜在资源的回收
IF 3.3 4区 环境科学与生态学 Q2 BIOCHEMISTRY & MOLECULAR BIOLOGY Pub Date : 2022-10-21 DOI: 10.1080/26395940.2022.2137061
A. Giwa, Mingqiang Sheng, Xiaoqian Zhang, Yuanyuan Wu, Huang Bo, A. Memon, Shuqin Bai, N. Ali, Jean Maurice Ndungutse, Wang Kaijun
ABSTRACT Continuous population growth associated with sanitation, food waste (FW), and domestic wastewater (DWW) is becoming critical globally. Crucial efforts and appropriate measures to utilize the FW and DWW for resources are needed. This paper reviews the conventional treatment techniques, challenges, and associated merits for treating FW and DWW. In the context of this review, DWW is often referred to as blackwater (BW)/feces. Due to the rationale for resource amplification, the review proposed that both mixtures (FW and DWW) be stored in a sub-surface storage tank for several months or years. They are further biodegraded in a bioprocess to generate energy with stabilized digestates. The effluent’s peculiar features are low organic acids with a low pH4 value, offering a stabilized and sanitized effluent. The second proposed route was to integrate anaerobic digestion, composting, and pyrolysis. Anaerobic digestion will offer bioenergy and digestates. Composting will cater to compost production and avert digestate drying and heating costs during pyrolysis. The pyrolysis of the digestates will generate biochar and bioenergy materials, while improved bioprocess performance is attained with the simultaneous biochar utilization in the bioprocess. The integrated technological routes can valorize DWW and FW for maximum resource recovery and sustainable development in a real-world context. The concept can be applied to an existing facility to create a cleaner and more efficient DWW with FW recycling. However, a comprehensive techno-economic analysis must be conducted.
与卫生、食物垃圾(FW)和生活污水(DWW)相关的人口持续增长在全球变得越来越重要。需要作出重大努力并采取适当措施,利用FW和DWW获取资源。本文综述了水冷水和水冷水的常规处理技术、面临的挑战以及相关优点。在本综述中,DWW通常被称为黑水(BW)/粪便。由于资源放大的理由,该审查建议将两种混合物(FW和DWW)都储存在地下储罐中数月或数年。它们在生物过程中进一步生物降解,以稳定的消化物产生能量。出水的特点是有机酸含量低,ph值低,出水稳定、消毒。第二条建议的路线是整合厌氧消化,堆肥和热解。厌氧消化将提供生物能源和消化物。堆肥将迎合堆肥生产,避免在热解过程中消化干燥和加热成本。沼液热解生成生物炭和生物能源材料,同时生物炭在生物过程中得到利用,提高了生物工艺性能。综合技术路线可以使DWW和FW在现实环境中实现最大的资源回收和可持续发展。这一概念可以应用于现有设施,以创造一个更清洁和更有效的DWW与FW回收。但是,必须进行全面的技术经济分析。
{"title":"Approaches for treating domestic wastewater with food waste and recovery of potential resources","authors":"A. Giwa, Mingqiang Sheng, Xiaoqian Zhang, Yuanyuan Wu, Huang Bo, A. Memon, Shuqin Bai, N. Ali, Jean Maurice Ndungutse, Wang Kaijun","doi":"10.1080/26395940.2022.2137061","DOIUrl":"https://doi.org/10.1080/26395940.2022.2137061","url":null,"abstract":"ABSTRACT Continuous population growth associated with sanitation, food waste (FW), and domestic wastewater (DWW) is becoming critical globally. Crucial efforts and appropriate measures to utilize the FW and DWW for resources are needed. This paper reviews the conventional treatment techniques, challenges, and associated merits for treating FW and DWW. In the context of this review, DWW is often referred to as blackwater (BW)/feces. Due to the rationale for resource amplification, the review proposed that both mixtures (FW and DWW) be stored in a sub-surface storage tank for several months or years. They are further biodegraded in a bioprocess to generate energy with stabilized digestates. The effluent’s peculiar features are low organic acids with a low pH4 value, offering a stabilized and sanitized effluent. The second proposed route was to integrate anaerobic digestion, composting, and pyrolysis. Anaerobic digestion will offer bioenergy and digestates. Composting will cater to compost production and avert digestate drying and heating costs during pyrolysis. The pyrolysis of the digestates will generate biochar and bioenergy materials, while improved bioprocess performance is attained with the simultaneous biochar utilization in the bioprocess. The integrated technological routes can valorize DWW and FW for maximum resource recovery and sustainable development in a real-world context. The concept can be applied to an existing facility to create a cleaner and more efficient DWW with FW recycling. However, a comprehensive techno-economic analysis must be conducted.","PeriodicalId":11785,"journal":{"name":"Environmental Pollutants and Bioavailability","volume":"104 1","pages":"501 - 517"},"PeriodicalIF":3.3,"publicationDate":"2022-10-21","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"79228807","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 3
Reviving of embedded MOFs in electrospun nanofibers by solvent swelling for arsenate removal in water 溶剂溶胀法去除水中砷酸盐对电纺丝纳米纤维中嵌入mof的回收
IF 3.3 4区 环境科学与生态学 Q2 BIOCHEMISTRY & MOLECULAR BIOLOGY Pub Date : 2022-10-19 DOI: 10.1080/26395940.2022.2136111
Qi Guo, Yuan Li, Xiaoyan Wei, Yi-Wen Shen, Xuelei Duan, Kai-Qiang He, Ke-gang Zhang, Chunmei Yuan
ABSTRACT Nanoparticles coated with electrospun fibers cannot fully exert their inherent properties. Therefore, it is critical to develop a method to enhance the intrinsic performances of the composite fibers. In this work, UiO-66/PAN composite nanofiber membranes with good physicochemical properties were prepared by electrospinning, and a swelling method was developed to improve its performances. The adsorption performance for arsenate was improved by 19.9% or 49% after swelling by nitrobenzene or pyridine solvent, respectively. The swelling process did not change the morphologies and structures of the fibers. The pyridine solvent as the swelling agent improved the adsorption performance of the nanofiber membrane by about 45% in 1 hour. There was no detectable leached Zr in the remaining solution, indicating that the composite membrane was stable during the course. This work provides a new strategy for functional promotion of electrospun nanofiber membrane and will be helpful for environmentally friendly applications of nanocomposites in water remediation.
电纺纤维包覆纳米粒子不能充分发挥其固有性能。因此,开发一种提高复合纤维内在性能的方法是至关重要的。本文采用静电纺丝法制备了具有良好理化性能的UiO-66/PAN复合纳米纤维膜,并开发了溶胀法来改善其性能。硝基苯和吡啶溶剂溶胀后对砷酸盐的吸附性能分别提高19.9%和49%。肿胀过程没有改变纤维的形态和结构。以吡啶溶剂为溶胀剂,在1 h内使纳米纤维膜的吸附性能提高约45%。剩余溶液中没有检测到浸出的Zr,表明复合膜在过程中是稳定的。本研究为电纺丝纳米纤维膜的功能提升提供了新的策略,有助于纳米复合材料在环境友好型水修复中的应用。
{"title":"Reviving of embedded MOFs in electrospun nanofibers by solvent swelling for arsenate removal in water","authors":"Qi Guo, Yuan Li, Xiaoyan Wei, Yi-Wen Shen, Xuelei Duan, Kai-Qiang He, Ke-gang Zhang, Chunmei Yuan","doi":"10.1080/26395940.2022.2136111","DOIUrl":"https://doi.org/10.1080/26395940.2022.2136111","url":null,"abstract":"ABSTRACT Nanoparticles coated with electrospun fibers cannot fully exert their inherent properties. Therefore, it is critical to develop a method to enhance the intrinsic performances of the composite fibers. In this work, UiO-66/PAN composite nanofiber membranes with good physicochemical properties were prepared by electrospinning, and a swelling method was developed to improve its performances. The adsorption performance for arsenate was improved by 19.9% or 49% after swelling by nitrobenzene or pyridine solvent, respectively. The swelling process did not change the morphologies and structures of the fibers. The pyridine solvent as the swelling agent improved the adsorption performance of the nanofiber membrane by about 45% in 1 hour. There was no detectable leached Zr in the remaining solution, indicating that the composite membrane was stable during the course. This work provides a new strategy for functional promotion of electrospun nanofiber membrane and will be helpful for environmentally friendly applications of nanocomposites in water remediation.","PeriodicalId":11785,"journal":{"name":"Environmental Pollutants and Bioavailability","volume":"31 1","pages":"496 - 500"},"PeriodicalIF":3.3,"publicationDate":"2022-10-19","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"73233338","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Single and combined toxic effects of clarithromycin and levofloxacin on Microcystis aeruginosa 克拉霉素与左氧氟沙星单独及联合对铜绿微囊藻的毒性作用
IF 3.3 4区 环境科学与生态学 Q2 BIOCHEMISTRY & MOLECULAR BIOLOGY Pub Date : 2022-10-06 DOI: 10.1080/26395940.2022.2130825
Yixiao Wu, Huijun Ding, L. Wan, Weihao Zhang, Yan Zhang, L. Yang, Chong Zhao
ABSTRACT This study compared the single and joint toxic effects of clarithromycin (CLA) and levofloxacin (LEV) on Microcystis aeruginosa. CLA was more toxic to algae than LEV, and the 96h-EC50s were 43.31 and 437.6 µg/L, respectively. The synergetic interaction of two antibiotics was detected. This synergetic action was also observed on Fv/Fm, chlorophyll a, and phycobiliprotein. The increase in reactive oxygen species (ROS) and malonaldehyde demonstrated that antibiotic exposure caused severe oxidative stress, which can destroy the membrane system, hinder photosynthesis and finally inhibit cell growth. The antioxidant enzyme activities were improved significantly, especially in the joint exposure treatment, which indicates that the antioxidant defense system can be activated to scavenge ROS. The release of microcystins (MCs) was accelerated under single or combined antibiotic exposure. The promotion of MCs discharge from cyanobacteria caused by the co-occurrence of CLA and LEV in water environment may pose a severe ecological risk to ecosystem.
摘要本研究比较了克拉霉素(CLA)和左氧氟沙星(LEV)单独和联合对铜绿微囊藻的毒性作用。CLA对藻类的毒性大于LEV, 96h- ec50分别为43.31µg/L和437.6µg/L。检测两种抗生素的协同相互作用。在Fv/Fm、叶绿素a和藻胆蛋白上也观察到这种协同作用。活性氧(ROS)和丙二醛的增加表明,抗生素暴露引起严重的氧化应激,破坏膜系统,阻碍光合作用,最终抑制细胞生长。抗氧化酶活性显著提高,特别是在联合暴露处理中,这表明抗氧化防御系统可以被激活,清除ROS。微囊藻毒素(MCs)的释放在单一或联合抗生素暴露下加速。水环境中CLA和LEV的共存促进蓝藻MCs的排放,可能对生态系统造成严重的生态风险。
{"title":"Single and combined toxic effects of clarithromycin and levofloxacin on Microcystis aeruginosa","authors":"Yixiao Wu, Huijun Ding, L. Wan, Weihao Zhang, Yan Zhang, L. Yang, Chong Zhao","doi":"10.1080/26395940.2022.2130825","DOIUrl":"https://doi.org/10.1080/26395940.2022.2130825","url":null,"abstract":"ABSTRACT This study compared the single and joint toxic effects of clarithromycin (CLA) and levofloxacin (LEV) on Microcystis aeruginosa. CLA was more toxic to algae than LEV, and the 96h-EC50s were 43.31 and 437.6 µg/L, respectively. The synergetic interaction of two antibiotics was detected. This synergetic action was also observed on Fv/Fm, chlorophyll a, and phycobiliprotein. The increase in reactive oxygen species (ROS) and malonaldehyde demonstrated that antibiotic exposure caused severe oxidative stress, which can destroy the membrane system, hinder photosynthesis and finally inhibit cell growth. The antioxidant enzyme activities were improved significantly, especially in the joint exposure treatment, which indicates that the antioxidant defense system can be activated to scavenge ROS. The release of microcystins (MCs) was accelerated under single or combined antibiotic exposure. The promotion of MCs discharge from cyanobacteria caused by the co-occurrence of CLA and LEV in water environment may pose a severe ecological risk to ecosystem.","PeriodicalId":11785,"journal":{"name":"Environmental Pollutants and Bioavailability","volume":"10 1","pages":"482 - 495"},"PeriodicalIF":3.3,"publicationDate":"2022-10-06","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"73902823","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 2
Biodegradation of oxidized high-density polyethylene and oxo-degradable plastic using microalgae Dunaliella salina 利用盐藻降解氧化高密度聚乙烯和氧降解塑料
IF 3.3 4区 环境科学与生态学 Q2 BIOCHEMISTRY & MOLECULAR BIOLOGY Pub Date : 2022-09-30 DOI: 10.1080/26395940.2022.2128884
Hadiyanto Hadiyanto, A. Khoironi, I. Dianratri, K. Huda, S. Suherman, F. Muhammad
ABSTRACT This research aimed to evaluate the effectiveness of microalgae Dunaliella salina in the biodegradation process of oxidized oxium and HDPE plastics. Microalgae and microplastic interactions were evaluated in two 1 L glass bioreactors containing D. salina with oxium microplastics and oxidized HDPE at various concentrations (100 mg/500 mL, 200 mg/500 mL, and 300 mg/500 mL) for 15 d. The results showed a more significant decrease in alkene functional groups in oxium plastics than in HDPE. In addition, there was a change in the oxium functional group with the formation of carbonyl, ether, and primary alcohol. The growth rate of D. salina decreased significantly after interaction with oxidized HDPE microplastics compared to oxium interaction. We established that oxium plastics have a faster biodegradation ability owing to the addition of additives to the plastic. However, oxidation pre-treatment with H2O2 on HDPE plastic can also accelerate the plastic degradation process.
摘要本研究旨在评价微藻Dunaliella salina在氧化氧和HDPE塑料生物降解过程中的有效性。在两个1 L含盐藻的玻璃生物反应器中,研究了微藻与微塑料和氧化HDPE在不同浓度(100 mg/500 mL、200 mg/500 mL和300 mg/500 mL)下的相互作用。结果表明,氧化塑料中烯烃官能团的减少比HDPE更显著。此外,氧官能团随着羰基、醚和伯醇的形成而发生变化。与氧化HDPE微塑料相互作用相比,氧化HDPE微塑料与盐藻的生长速率明显降低。我们确定,由于在塑料中添加了添加剂,氧塑料具有更快的生物降解能力。然而,用H2O2对HDPE塑料进行氧化预处理也会加速塑料的降解过程。
{"title":"Biodegradation of oxidized high-density polyethylene and oxo-degradable plastic using microalgae Dunaliella salina","authors":"Hadiyanto Hadiyanto, A. Khoironi, I. Dianratri, K. Huda, S. Suherman, F. Muhammad","doi":"10.1080/26395940.2022.2128884","DOIUrl":"https://doi.org/10.1080/26395940.2022.2128884","url":null,"abstract":"ABSTRACT This research aimed to evaluate the effectiveness of microalgae Dunaliella salina in the biodegradation process of oxidized oxium and HDPE plastics. Microalgae and microplastic interactions were evaluated in two 1 L glass bioreactors containing D. salina with oxium microplastics and oxidized HDPE at various concentrations (100 mg/500 mL, 200 mg/500 mL, and 300 mg/500 mL) for 15 d. The results showed a more significant decrease in alkene functional groups in oxium plastics than in HDPE. In addition, there was a change in the oxium functional group with the formation of carbonyl, ether, and primary alcohol. The growth rate of D. salina decreased significantly after interaction with oxidized HDPE microplastics compared to oxium interaction. We established that oxium plastics have a faster biodegradation ability owing to the addition of additives to the plastic. However, oxidation pre-treatment with H2O2 on HDPE plastic can also accelerate the plastic degradation process.","PeriodicalId":11785,"journal":{"name":"Environmental Pollutants and Bioavailability","volume":"9 1","pages":"469 - 481"},"PeriodicalIF":3.3,"publicationDate":"2022-09-30","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"77972040","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 5
Acute dermal effects of solar UV irradiation and efficacy of sunscreen use 太阳紫外线照射对皮肤的急性影响和防晒霜的使用效果
IF 3.3 4区 环境科学与生态学 Q2 BIOCHEMISTRY & MOLECULAR BIOLOGY Pub Date : 2022-09-29 DOI: 10.1080/26395940.2022.2128883
Yi-Chun Lin, Yu-Chieh Chen, B. Hwang, Chen-Peng Chen
ABSTRACT The Global Solar Ultraviolet (UV) Index provides limited information on health effects due to over-exposure. This study investigated the change in skin physiology in response to solar UV irradiation and the protective efficacy of a sunscreen. Fourteen female participants were divided into two groups, sunscreen users and non-users, and for 8 weeks they received solar irradiation and were monitored for change in the erythema-index (E-index), melanin-index, skin capillary blood flow, skin moisture, transepidermal water loss (TEWL), and skin temperature. The E-index and TEWL responded proportionally to solar radiation and could serve as indices of acute health effects from UV exposure. In the sun-radiated area, the E-index and TEWL measured on the forearm of the non-users were 111.3% and 138.4% of the levels determined for the users, respectively. Although thermal sensation and thermo-physiology were correlated, physiological monitoring was preferred over thermal sensation survey in evaluating the impact of solar UV irradiation.
全球太阳紫外线(UV)指数提供了有限的关于过度暴露对健康影响的信息。本研究探讨了太阳紫外线照射下皮肤生理机能的变化和防晒霜的保护功效。14名女性参与者被分为使用防晒霜和不使用防晒霜两组,她们接受8周的太阳照射,并监测红斑指数(E-index)、黑色素指数、皮肤毛细血管血流、皮肤水分、经皮失水(TEWL)和皮肤温度的变化。e -指数和TEWL与太阳辐射成正比,可作为紫外线照射对急性健康影响的指标。在阳光照射区域,非使用者前臂的e指数和TEWL分别为使用者的111.3%和138.4%。虽然热感觉与热生理相关,但在评价太阳紫外线照射的影响时,生理监测优于热感觉调查。
{"title":"Acute dermal effects of solar UV irradiation and efficacy of sunscreen use","authors":"Yi-Chun Lin, Yu-Chieh Chen, B. Hwang, Chen-Peng Chen","doi":"10.1080/26395940.2022.2128883","DOIUrl":"https://doi.org/10.1080/26395940.2022.2128883","url":null,"abstract":"ABSTRACT The Global Solar Ultraviolet (UV) Index provides limited information on health effects due to over-exposure. This study investigated the change in skin physiology in response to solar UV irradiation and the protective efficacy of a sunscreen. Fourteen female participants were divided into two groups, sunscreen users and non-users, and for 8 weeks they received solar irradiation and were monitored for change in the erythema-index (E-index), melanin-index, skin capillary blood flow, skin moisture, transepidermal water loss (TEWL), and skin temperature. The E-index and TEWL responded proportionally to solar radiation and could serve as indices of acute health effects from UV exposure. In the sun-radiated area, the E-index and TEWL measured on the forearm of the non-users were 111.3% and 138.4% of the levels determined for the users, respectively. Although thermal sensation and thermo-physiology were correlated, physiological monitoring was preferred over thermal sensation survey in evaluating the impact of solar UV irradiation.","PeriodicalId":11785,"journal":{"name":"Environmental Pollutants and Bioavailability","volume":"5 1","pages":"456 - 468"},"PeriodicalIF":3.3,"publicationDate":"2022-09-29","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"86450649","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Migration characteristics of oil pollutants into soil pores influenced by surface wettability 表面润湿性对石油污染物向土壤孔隙迁移特性的影响
IF 3.3 4区 环境科学与生态学 Q2 BIOCHEMISTRY & MOLECULAR BIOLOGY Pub Date : 2022-09-28 DOI: 10.1080/26395940.2022.2128885
Lingqi Lin, Yulin Pu, Di Wang, Xi Guo, Peng Wang, Zhong Lu
ABSTRACT Pore-scale modeling plays an indispensable role in unveiling the migration mechanism of oil pollutants into the water-saturated soil. Navier Stokes equations and conservation of mass, coupled with the phase field method, are employed to investigate the effect of soil wettability on oil pollutants migration into the soil porous media. The results show that the oil-water interface in the migration process does not advance evenly in three wetting states. When the model system is in oil-wetting state, oil pollutants obviously migrate at a higher speed. Through monitoring the evolution of oil front location and analyzing the velocity distribution vertical to the flow direction at the central axis of the model, the channel corresponding to the peak velocity is the dominant flow channel for the oil pollutants. This study will have the potential ability in obtaining the pore-scale migration regulation of oil pollutions as well as more accurately predicting the pollution range.
孔隙尺度模拟对于揭示含油污染物进入饱和水土壤的运移机理具有不可缺少的作用。采用Navier Stokes方程和质量守恒方程,结合相场法研究了土壤润湿性对石油污染物向土壤多孔介质迁移的影响。结果表明:在三种润湿状态下,运移过程中油水界面的推进并不均匀;当模型系统处于油润湿状态时,油类污染物运移速度明显加快。通过监测油锋位置的演变,分析模型中轴线处垂直于流向的流速分布,发现峰值流速所对应的通道是油污染物的主导流动通道。本研究将有可能获得油类污染在孔隙尺度上的运移规律,更准确地预测污染范围。
{"title":"Migration characteristics of oil pollutants into soil pores influenced by surface wettability","authors":"Lingqi Lin, Yulin Pu, Di Wang, Xi Guo, Peng Wang, Zhong Lu","doi":"10.1080/26395940.2022.2128885","DOIUrl":"https://doi.org/10.1080/26395940.2022.2128885","url":null,"abstract":"ABSTRACT Pore-scale modeling plays an indispensable role in unveiling the migration mechanism of oil pollutants into the water-saturated soil. Navier Stokes equations and conservation of mass, coupled with the phase field method, are employed to investigate the effect of soil wettability on oil pollutants migration into the soil porous media. The results show that the oil-water interface in the migration process does not advance evenly in three wetting states. When the model system is in oil-wetting state, oil pollutants obviously migrate at a higher speed. Through monitoring the evolution of oil front location and analyzing the velocity distribution vertical to the flow direction at the central axis of the model, the channel corresponding to the peak velocity is the dominant flow channel for the oil pollutants. This study will have the potential ability in obtaining the pore-scale migration regulation of oil pollutions as well as more accurately predicting the pollution range.","PeriodicalId":11785,"journal":{"name":"Environmental Pollutants and Bioavailability","volume":"21 1","pages":"446 - 455"},"PeriodicalIF":3.3,"publicationDate":"2022-09-28","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"87719904","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Effects of Cr6+ stress on chromium chemical speciation distribution and bacterial community structure in the Coix lacryma-jobi L. constructed wetlands Cr6+胁迫对人工湿地铬化学形态分布及细菌群落结构的影响
IF 3.3 4区 环境科学与生态学 Q2 BIOCHEMISTRY & MOLECULAR BIOLOGY Pub Date : 2022-09-27 DOI: 10.1080/26395940.2022.2128427
Zirui Fang, Qianyun Wang, Cunqi Zhang, Sulian Li, Shuai Li, Xueli Wang, Xiran Cheng, Zhenli He, Zhigang Li
ABSTRACT In this study, micro Coix lacryma-jobi L. vertical flow constructed wetlands with 0, 10 and 30 mg/L Cr6+ (in the form of K2Cr7O2) in the water sources were constructed to study the purification efficiency of chromium-contaminated wastewater, bacterial community diversity, chromium chemical speciation distribution and other indicators. The results showed that the constructed wetlands had high purification efficiency for chromium-contaminated wastewater. The removal rate of Cr6+ reached 99.61% and 95.45% in 10 and 30 mg/L Cr6+ treatment. The bacterial diversity index was unaffected by Cr6+ treatment; however, the bacterial richness index declined dramatically as Cr6+ treatment concentration increased. The bacterial community structure was influenced by the substrates pH, moisture content, organic matter and total chromium content. The abundance of Burkholderiaceae (uncultured) and Saccharimonadales (uncultured) were positively correlated with non-residual chromium content. The results contributed to understand the effect of chromium on bacterial community structure by considering the chromium chemical speciation.
摘要本研究通过在水源中构建0、10、30 mg/L Cr6+(以K2Cr7O2的形式)垂直流人工湿地,研究其对铬污染废水的净化效果、细菌群落多样性、铬化学形态分布等指标。结果表明,人工湿地对含铬废水具有较高的净化效果。10和30 mg/L Cr6+的去除率分别为99.61%和95.45%。细菌多样性指数不受Cr6+处理的影响;但随着Cr6+处理浓度的增加,细菌丰富度指数显著下降。细菌群落结构受基质pH、含水量、有机质和总铬含量的影响。burkholderaceae(未培养)和Saccharimonadales(未培养)的丰度与非残留铬含量呈正相关。研究结果有助于从铬的化学形态角度了解铬对细菌群落结构的影响。
{"title":"Effects of Cr6+ stress on chromium chemical speciation distribution and bacterial community structure in the Coix lacryma-jobi L. constructed wetlands","authors":"Zirui Fang, Qianyun Wang, Cunqi Zhang, Sulian Li, Shuai Li, Xueli Wang, Xiran Cheng, Zhenli He, Zhigang Li","doi":"10.1080/26395940.2022.2128427","DOIUrl":"https://doi.org/10.1080/26395940.2022.2128427","url":null,"abstract":"ABSTRACT In this study, micro Coix lacryma-jobi L. vertical flow constructed wetlands with 0, 10 and 30 mg/L Cr6+ (in the form of K2Cr7O2) in the water sources were constructed to study the purification efficiency of chromium-contaminated wastewater, bacterial community diversity, chromium chemical speciation distribution and other indicators. The results showed that the constructed wetlands had high purification efficiency for chromium-contaminated wastewater. The removal rate of Cr6+ reached 99.61% and 95.45% in 10 and 30 mg/L Cr6+ treatment. The bacterial diversity index was unaffected by Cr6+ treatment; however, the bacterial richness index declined dramatically as Cr6+ treatment concentration increased. The bacterial community structure was influenced by the substrates pH, moisture content, organic matter and total chromium content. The abundance of Burkholderiaceae (uncultured) and Saccharimonadales (uncultured) were positively correlated with non-residual chromium content. The results contributed to understand the effect of chromium on bacterial community structure by considering the chromium chemical speciation.","PeriodicalId":11785,"journal":{"name":"Environmental Pollutants and Bioavailability","volume":"138 1","pages":"433 - 445"},"PeriodicalIF":3.3,"publicationDate":"2022-09-27","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"84790225","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 1
Study on influence mechanism of biochar on soil nitrogen conversion 生物炭对土壤氮转化的影响机理研究
IF 3.3 4区 环境科学与生态学 Q2 BIOCHEMISTRY & MOLECULAR BIOLOGY Pub Date : 2022-09-22 DOI: 10.1080/26395940.2022.2125445
Pingnan Zhao, Shen Wang, Dong Liu, Hongxu Li, Song Han, Ming Li
ABSTRACT Straw had huge annual production, burning it in the air will cause serious air pollution. Burning straw into biochar and returning biochar to the field will not only make effective use of straw resources, but also improve soil quality. Different preparation conditions and addition levels of biochar were used to investigate the ammonia nitrogen, nitrate nitrogen, and total nitrogen contents in the soil leaching solution. The results showed that biochar had a favorable adsorption effect on ammonia nitrogen, the cumulative leaching of ammonia nitrogen reduced by 80.16% in the 2% and 400°C biochar addition treatment compared to that without adding biochar. The final leaching solution electrical conductivity value of the experimental group of biochar prepared at 500°C with 1% addition was the highest at 445 μS/cm. Sequencing of microorganisms revealed that biochar altered the structure and abundance of the soil microbial community, particularly increased the relative abundance of nitrifying bacteria.
摘要秸秆年生产量巨大,在空气中焚烧秸秆会造成严重的空气污染。将秸秆焚烧成生物炭,再将生物炭还田,既能有效利用秸秆资源,又能改善土壤质量。采用不同制备条件和添加量的生物炭对土壤浸出液中氨氮、硝态氮和全氮含量进行了研究。结果表明,生物炭对氨氮具有良好的吸附效果,添加2%和400℃的生物炭处理下,氨氮的累积浸出量比未添加生物炭的处理降低了80.16%。500℃、添加量1%制备的生物炭试验组最终浸出液电导率值最高,为445 μS/cm。微生物测序结果显示,生物炭改变了土壤微生物群落的结构和丰度,特别是增加了硝化细菌的相对丰度。
{"title":"Study on influence mechanism of biochar on soil nitrogen conversion","authors":"Pingnan Zhao, Shen Wang, Dong Liu, Hongxu Li, Song Han, Ming Li","doi":"10.1080/26395940.2022.2125445","DOIUrl":"https://doi.org/10.1080/26395940.2022.2125445","url":null,"abstract":"ABSTRACT Straw had huge annual production, burning it in the air will cause serious air pollution. Burning straw into biochar and returning biochar to the field will not only make effective use of straw resources, but also improve soil quality. Different preparation conditions and addition levels of biochar were used to investigate the ammonia nitrogen, nitrate nitrogen, and total nitrogen contents in the soil leaching solution. The results showed that biochar had a favorable adsorption effect on ammonia nitrogen, the cumulative leaching of ammonia nitrogen reduced by 80.16% in the 2% and 400°C biochar addition treatment compared to that without adding biochar. The final leaching solution electrical conductivity value of the experimental group of biochar prepared at 500°C with 1% addition was the highest at 445 μS/cm. Sequencing of microorganisms revealed that biochar altered the structure and abundance of the soil microbial community, particularly increased the relative abundance of nitrifying bacteria.","PeriodicalId":11785,"journal":{"name":"Environmental Pollutants and Bioavailability","volume":"1 1","pages":"419 - 432"},"PeriodicalIF":3.3,"publicationDate":"2022-09-22","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"83948027","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 8
Effects of the exogenous N-acylhomoserine lactones on the performances of microalgal-bacterial granular consortia 外源n -酰基高丝氨酸内酯对微藻-细菌颗粒菌群性能的影响
IF 3.3 4区 环境科学与生态学 Q2 BIOCHEMISTRY & MOLECULAR BIOLOGY Pub Date : 2022-09-15 DOI: 10.1080/26395940.2022.2123046
Wanlin Lyu, Shujia Zhang, Yijia Xie, Rongfan Chen, Xiaoling Hu, Bin Wang, Wenbin Guo, Hongyu Wang, Jie Xing, Daochun Zhou
ABSTRACT Chlorella sorokiniana, the dominant microalgal strain with fast growth rate and high nutrients’ adsorption rate, was selected from the mature MBGS system. After adding C6-HSL and 3-oxo-C12-HSL to the MBGS consortia formed by combining it with mature AGS, it could also be found that C6-HSL accelerated the denitrification rate and improved the removal rate of TIN and TP effectively. Besides, the promoting effect of C6-HSL was slightly higher than that of 3-oxo-C12-HSL. By adjusting the concentration of C6-HSL (5 × 10−9, 7.5 × 10−7 and 2.5 × 10−5mol/L), the results revealed that adding 5 × 10−9mol/L C6-HSL significantly improved the efficiency of nitrogen and phosphorus removal in MBGS consortia. However, adding higher concentration of C6-HSL (7.5 × 10−7mol/L) would lead to deterioration of TIN and COD degradation. The content of EPS secreted by bacteria was regulated by different concentrations of AHLs, and the PS/PN value decreased with the increasing trend of C6-HSL concentration. GRAPIHCAL ABSTRACT
摘要从成熟的MBGS体系中筛选出生长速度快、营养物质吸附率高的优势微藻小球藻(Chlorella sorokiniana)。将C6-HSL和3-氧- c12 - hsl加入到与成熟AGS结合形成的MBGS联合体中,也可以发现C6-HSL有效地加快了反硝化速度,提高了TIN和TP的去除率。此外,C6-HSL的促进作用略高于3-oxo-C12-HSL。通过调整C6-HSL的浓度(5 × 10−9、7.5 × 10−7和2.5 × 10−5mol/L),结果表明,添加5 × 10−9mol/L的C6-HSL显著提高了MBGS菌群的脱氮除磷效率。而C6-HSL浓度越高(7.5 × 10−7mol/L), TIN和COD的降解效果越差。细菌分泌的EPS含量受不同浓度ahl的调控,PS/PN值随C6-HSL浓度的增加而降低。GRAPIHCAL文摘
{"title":"Effects of the exogenous N-acylhomoserine lactones on the performances of microalgal-bacterial granular consortia","authors":"Wanlin Lyu, Shujia Zhang, Yijia Xie, Rongfan Chen, Xiaoling Hu, Bin Wang, Wenbin Guo, Hongyu Wang, Jie Xing, Daochun Zhou","doi":"10.1080/26395940.2022.2123046","DOIUrl":"https://doi.org/10.1080/26395940.2022.2123046","url":null,"abstract":"ABSTRACT Chlorella sorokiniana, the dominant microalgal strain with fast growth rate and high nutrients’ adsorption rate, was selected from the mature MBGS system. After adding C6-HSL and 3-oxo-C12-HSL to the MBGS consortia formed by combining it with mature AGS, it could also be found that C6-HSL accelerated the denitrification rate and improved the removal rate of TIN and TP effectively. Besides, the promoting effect of C6-HSL was slightly higher than that of 3-oxo-C12-HSL. By adjusting the concentration of C6-HSL (5 × 10−9, 7.5 × 10−7 and 2.5 × 10−5mol/L), the results revealed that adding 5 × 10−9mol/L C6-HSL significantly improved the efficiency of nitrogen and phosphorus removal in MBGS consortia. However, adding higher concentration of C6-HSL (7.5 × 10−7mol/L) would lead to deterioration of TIN and COD degradation. The content of EPS secreted by bacteria was regulated by different concentrations of AHLs, and the PS/PN value decreased with the increasing trend of C6-HSL concentration. GRAPIHCAL ABSTRACT","PeriodicalId":11785,"journal":{"name":"Environmental Pollutants and Bioavailability","volume":"263 1","pages":"407 - 418"},"PeriodicalIF":3.3,"publicationDate":"2022-09-15","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"83506074","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 2
期刊
Environmental Pollutants and Bioavailability
全部 Acc. Chem. Res. ACS Applied Bio Materials ACS Appl. Electron. Mater. ACS Appl. Energy Mater. ACS Appl. Mater. Interfaces ACS Appl. Nano Mater. ACS Appl. Polym. Mater. ACS BIOMATER-SCI ENG ACS Catal. ACS Cent. Sci. ACS Chem. Biol. ACS Chemical Health & Safety ACS Chem. Neurosci. ACS Comb. Sci. ACS Earth Space Chem. ACS Energy Lett. ACS Infect. Dis. ACS Macro Lett. ACS Mater. Lett. ACS Med. Chem. Lett. ACS Nano ACS Omega ACS Photonics ACS Sens. ACS Sustainable Chem. Eng. ACS Synth. Biol. Anal. Chem. BIOCHEMISTRY-US Bioconjugate Chem. BIOMACROMOLECULES Chem. Res. Toxicol. Chem. Rev. Chem. Mater. CRYST GROWTH DES ENERG FUEL Environ. Sci. Technol. Environ. Sci. Technol. Lett. Eur. J. Inorg. Chem. IND ENG CHEM RES Inorg. Chem. J. Agric. Food. Chem. J. Chem. Eng. Data J. Chem. Educ. J. Chem. Inf. Model. J. Chem. Theory Comput. J. Med. Chem. J. Nat. Prod. J PROTEOME RES J. Am. Chem. Soc. LANGMUIR MACROMOLECULES Mol. Pharmaceutics Nano Lett. Org. Lett. ORG PROCESS RES DEV ORGANOMETALLICS J. Org. Chem. J. Phys. Chem. J. Phys. Chem. A J. Phys. Chem. B J. Phys. Chem. C J. Phys. Chem. Lett. Analyst Anal. Methods Biomater. Sci. Catal. Sci. Technol. Chem. Commun. Chem. Soc. Rev. CHEM EDUC RES PRACT CRYSTENGCOMM Dalton Trans. Energy Environ. Sci. ENVIRON SCI-NANO ENVIRON SCI-PROC IMP ENVIRON SCI-WAT RES Faraday Discuss. Food Funct. Green Chem. Inorg. Chem. Front. Integr. Biol. J. Anal. At. Spectrom. J. Mater. Chem. A J. Mater. Chem. B J. Mater. Chem. C Lab Chip Mater. Chem. Front. Mater. Horiz. MEDCHEMCOMM Metallomics Mol. Biosyst. Mol. Syst. Des. Eng. Nanoscale Nanoscale Horiz. Nat. Prod. Rep. New J. Chem. Org. Biomol. Chem. Org. Chem. Front. PHOTOCH PHOTOBIO SCI PCCP Polym. Chem.
×
引用
GB/T 7714-2015
复制
MLA
复制
APA
复制
导出至
BibTeX EndNote RefMan NoteFirst NoteExpress
×
0
微信
客服QQ
Book学术公众号 扫码关注我们
反馈
×
意见反馈
请填写您的意见或建议
请填写您的手机或邮箱
×
提示
您的信息不完整,为了账户安全,请先补充。
现在去补充
×
提示
您因"违规操作"
具体请查看互助需知
我知道了
×
提示
现在去查看 取消
×
提示
确定
Book学术官方微信
Book学术文献互助
Book学术文献互助群
群 号:481959085
Book学术
文献互助 智能选刊 最新文献 互助须知 联系我们:info@booksci.cn
Book学术提供免费学术资源搜索服务,方便国内外学者检索中英文文献。致力于提供最便捷和优质的服务体验。
Copyright © 2023 Book学术 All rights reserved.
ghs 京公网安备 11010802042870号 京ICP备2023020795号-1