首页 > 最新文献

Comprehensive Reviews in Food Science and Food Safety最新文献

英文 中文
Targeted Modification of Dietary Fiber for Increasing Soluble Dietary Fiber and Its Application in Foods 膳食纤维定向改性提高可溶性膳食纤维含量及其在食品中的应用。
IF 14.1 1区 农林科学 Q1 FOOD SCIENCE & TECHNOLOGY Pub Date : 2026-02-08 DOI: 10.1111/1541-4337.70423
Shirong Wang, Jing Liu, Xuejiao Wang, Shao-Quan Liu, Yuyun Lu, Shujie Wang, Yuhong Guo, Xingwei Wang, Jianxin Cao

The high proportion of insoluble dietary fiber (IDF) in natural plant materials critically limits the solubility, functionality, and processing performance of dietary fiber (DF), making the conversion of IDF to soluble dietary fiber (SDF) a key focus in current research. Although numerous physical, chemical, and biological modification technologies have been developed, most studies focus on treatment outcomes but fail to adequately address two key determinants: the intrinsic properties of DF, specifically the typical composition of DFs from different sources, cellulose crystalline regions, and the inherent structural recalcitrance resulting from lignocellulosic network cross-linking; and the synergistic effects of parameters, referring to the impact of processing variables (such as power, pressure, and enzyme type) on DFs from various sources. This review provides a systematic comparison of mainstream and emerging modification strategies, highlighting their mechanisms, advantages, and limitations across diverse DF matrices. Based on this, lignocellulose is utilized as a representative IDF model to explain how its dense, multilayered architecture acts as the primary barrier to efficient SDF generation. Furthermore, this review synthesizes advances in the targeted disruption of lignocellulosic components, including targeted lignin degradation and the depolymerization of cellulose and hemicellulose, to propose strategies for overcoming IDF recalcitrance. Finally, the application potential of these modification pathways in improving DF utilization in foods is evaluated, enabling innovative formats such as personalized nutrition, 3D-printed products, and biodegradable materials. Overall, this review integrates technique-level insights with structure-guided strategies, offering a mechanistic framework and practical roadmap for achieving efficient, directional IDF modification and SDF enhancement.

天然植物材料中不溶性膳食纤维(IDF)的高比例严重限制了膳食纤维(DF)的溶解度、功能和加工性能,使IDF转化为可溶性膳食纤维(SDF)成为当前研究的重点。尽管已经开发了许多物理、化学和生物改性技术,但大多数研究都集中在处理结果上,但未能充分解决两个关键决定因素:DF的内在特性,特别是来自不同来源的DF的典型组成,纤维素晶体区域,以及由木质纤维素网络交联引起的固有结构顽抗;参数的协同效应,是指加工变量(如功率、压力、酶型)对各种来源的DFs的影响。这篇综述提供了主流和新兴的修饰策略的系统比较,强调了它们在不同DF矩阵中的机制、优势和局限性。基于此,木质纤维素被用作具有代表性的IDF模型,以解释其致密的多层结构如何成为有效生成SDF的主要障碍。此外,本文综述了靶向破坏木质纤维素组分的研究进展,包括靶向木质素降解和纤维素和半纤维素的解聚,并提出了克服IDF抗性的策略。最后,评估了这些改性途径在提高食品中DF利用率方面的应用潜力,从而实现个性化营养、3d打印产品和可生物降解材料等创新形式。总体而言,本综述将技术层面的见解与结构导向策略相结合,为实现高效、定向的IDF修改和SDF增强提供了一个机制框架和实用路线图。
{"title":"Targeted Modification of Dietary Fiber for Increasing Soluble Dietary Fiber and Its Application in Foods","authors":"Shirong Wang,&nbsp;Jing Liu,&nbsp;Xuejiao Wang,&nbsp;Shao-Quan Liu,&nbsp;Yuyun Lu,&nbsp;Shujie Wang,&nbsp;Yuhong Guo,&nbsp;Xingwei Wang,&nbsp;Jianxin Cao","doi":"10.1111/1541-4337.70423","DOIUrl":"10.1111/1541-4337.70423","url":null,"abstract":"<div>\u0000 \u0000 <p>The high proportion of insoluble dietary fiber (IDF) in natural plant materials critically limits the solubility, functionality, and processing performance of dietary fiber (DF), making the conversion of IDF to soluble dietary fiber (SDF) a key focus in current research. Although numerous physical, chemical, and biological modification technologies have been developed, most studies focus on treatment outcomes but fail to adequately address two key determinants: the intrinsic properties of DF, specifically the typical composition of DFs from different sources, cellulose crystalline regions, and the inherent structural recalcitrance resulting from lignocellulosic network cross-linking; and the synergistic effects of parameters, referring to the impact of processing variables (such as power, pressure, and enzyme type) on DFs from various sources. This review provides a systematic comparison of mainstream and emerging modification strategies, highlighting their mechanisms, advantages, and limitations across diverse DF matrices. Based on this, lignocellulose is utilized as a representative IDF model to explain how its dense, multilayered architecture acts as the primary barrier to efficient SDF generation. Furthermore, this review synthesizes advances in the targeted disruption of lignocellulosic components, including targeted lignin degradation and the depolymerization of cellulose and hemicellulose, to propose strategies for overcoming IDF recalcitrance. Finally, the application potential of these modification pathways in improving DF utilization in foods is evaluated, enabling innovative formats such as personalized nutrition, 3D-printed products, and biodegradable materials. Overall, this review integrates technique-level insights with structure-guided strategies, offering a mechanistic framework and practical roadmap for achieving efficient, directional IDF modification and SDF enhancement.</p>\u0000 </div>","PeriodicalId":155,"journal":{"name":"Comprehensive Reviews in Food Science and Food Safety","volume":"25 2","pages":""},"PeriodicalIF":14.1,"publicationDate":"2026-02-08","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"146140426","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"农林科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Techniques to Detect and Quantify the Bacterial Metalloprotease AprX in Bovine Milk: A Review 牛乳中细菌金属蛋白酶AprX的检测与定量技术综述
IF 14.1 1区 农林科学 Q1 FOOD SCIENCE & TECHNOLOGY Pub Date : 2026-02-08 DOI: 10.1111/1541-4337.70415
Aritra Sinha, Alan L. Kelly

The heat-stable metalloprotease AprX, secreted by psychrotrophic Pseudomonas spp., is a major cause of quality deterioration in dairy products, particularly ultrahigh temperature (UHT) milk. This review synthesizes the evolution and current state of detection and quantification techniques for AprX in bovine milk, covering traditional immunological assays, enzymatic activity measurements, and zymography, alongside modern molecular approaches such as PCR-based methods, mass spectrometry, and advanced biosensors. Highly sensitive systems, including indirect ELISA (LOD 21.0 ng/mL), multiplex qPCR, and biosensor platforms, have enhanced the ability to detect AprX activity at low concentrations. Comparative analysis evaluates these methods in terms of sensitivity, specificity, turnaround time, cost, ease of use, and industrial applicability. Emerging directions such as multiomics integration, biosensor miniaturization, and artificial intelligence-driven data interpretation are also discussed. By critically assessing available and emerging tools, this review supports dairy scientists and industry stakeholders in selecting optimal strategies to detect, monitor, and mitigate AprX-associated spoilage in milk and dairy products.

由嗜冷假单胞菌分泌的热稳定性金属蛋白酶AprX是导致乳制品质量恶化的主要原因,尤其是超高温牛奶。本文综述了牛乳中AprX的检测和定量技术的发展和现状,包括传统的免疫学分析、酶活性测量和酶谱分析,以及现代分子方法,如基于pcr的方法、质谱分析和先进的生物传感器。包括间接ELISA (LOD 21.0 ng/mL)、多重qPCR和生物传感器平台在内的高灵敏度系统增强了检测低浓度AprX活性的能力。比较分析从敏感性、特异性、周转时间、成本、易用性和工业适用性等方面评价这些方法。本文还讨论了多组学集成、生物传感器小型化和人工智能驱动的数据解释等新兴方向。通过对现有和新兴工具的批判性评估,本综述支持乳制品科学家和行业利益相关者选择最佳策略,以检测、监测和减轻牛奶和乳制品中与aprx相关的腐败。
{"title":"Techniques to Detect and Quantify the Bacterial Metalloprotease AprX in Bovine Milk: A Review","authors":"Aritra Sinha,&nbsp;Alan L. Kelly","doi":"10.1111/1541-4337.70415","DOIUrl":"10.1111/1541-4337.70415","url":null,"abstract":"<p>The heat-stable metalloprotease AprX, secreted by psychrotrophic <i>Pseudomonas</i> spp., is a major cause of quality deterioration in dairy products, particularly ultrahigh temperature (UHT) milk. This review synthesizes the evolution and current state of detection and quantification techniques for AprX in bovine milk, covering traditional immunological assays, enzymatic activity measurements, and zymography, alongside modern molecular approaches such as PCR-based methods, mass spectrometry, and advanced biosensors. Highly sensitive systems, including indirect ELISA (LOD 21.0 ng/mL), multiplex qPCR, and biosensor platforms, have enhanced the ability to detect AprX activity at low concentrations. Comparative analysis evaluates these methods in terms of sensitivity, specificity, turnaround time, cost, ease of use, and industrial applicability. Emerging directions such as multiomics integration, biosensor miniaturization, and artificial intelligence-driven data interpretation are also discussed. By critically assessing available and emerging tools, this review supports dairy scientists and industry stakeholders in selecting optimal strategies to detect, monitor, and mitigate AprX-associated spoilage in milk and dairy products.</p>","PeriodicalId":155,"journal":{"name":"Comprehensive Reviews in Food Science and Food Safety","volume":"25 2","pages":""},"PeriodicalIF":14.1,"publicationDate":"2026-02-08","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.ncbi.nlm.nih.gov/pmc/articles/PMC12884017/pdf/","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"146140464","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"农林科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
A Comprehensive Review of Wooden Breast Myopathy in Broilers: Impacts, Detection, Processing, and Future Perspectives 肉鸡木制乳房肌病的综合综述:影响、检测、处理和未来展望。
IF 14.1 1区 农林科学 Q1 FOOD SCIENCE & TECHNOLOGY Pub Date : 2026-02-08 DOI: 10.1111/1541-4337.70414
Liubin Yang, Mengyue Zhou, Wei Guo, Haizhou Wu

Wooden breast (WB) myopathy is a major muscle disorder in fast-growing broilers, affecting the entire poultry production chain and causing substantial economic losses. Current mitigation strategies rely primarily on carcass-level identification, grading, and processing treatments. However, existing studies remain fragmented and insufficiently integrated, limiting effective problem-solving. In this review, we summarize and compare reported WB identification and classification methods in terms of detection principles, industrial adaptability, accuracy, cost, scalability, technological maturity, and limitations. Overall, near-infrared (NIR) spectroscopy achieves high accuracy (95%–100%), whereas imaging-based methods show greater potential for real-time, on-site application. We further review major postmortem strategies to improve WB meat quality and compare their underlying principles, key effects, applicable product types, optimization outcomes, costs, and limitations. Evidence shows that papain treatment significantly improves the quality of intact WB fillets (p < 0.05), while functional additives and protein glycation significantly enhance the processing quality of WB meat products (p < 0.05). Finally, in light of current research gaps, future efforts should focus on reducing the impact of WB through genetic marker screening and environmental control, the establishment of standardized identification criteria, AI-assisted modeling, and the development of WB-specific formulations and processing equipment. By systematically integrating WB pathophysiology, detection technologies, and postmortem processing interventions, this review provides a cohesive framework that is currently lacking in WB research and may guide both mechanistic studies and industrial practice.

木胸(WB)肌病是速生肉鸡的一种主要肌肉疾病,影响整个家禽生产链并造成重大经济损失。目前的缓解策略主要依赖于胴体水平的识别、分级和处理处理。然而,现有的研究仍然支离破碎,缺乏充分的整合,限制了有效的解决问题。在本文中,我们从检测原理、行业适应性、准确性、成本、可扩展性、技术成熟度和局限性等方面对已有的WB识别和分类方法进行了总结和比较。总体而言,近红外(NIR)光谱学达到了很高的精度(95%-100%),而基于成像的方法在实时、现场应用方面显示出更大的潜力。我们进一步回顾了改善WB肉质的主要宰后策略,并比较了其基本原理、关键效果、适用产品类型、优化结果、成本和局限性。结果表明,木瓜蛋白酶处理显著提高了白豆肉片的完整品质(p < 0.05),功能添加剂和蛋白糖化处理显著提高了白豆肉制品的加工品质(p < 0.05)。最后,鉴于目前的研究差距,未来的工作应侧重于通过遗传标记筛选和环境控制,建立标准化的鉴定标准,人工智能辅助建模以及开发特定的WB配方和加工设备来减少WB的影响。通过系统地整合脑白质病理生理学、检测技术和死后处理干预,本综述提供了目前脑白质研究中缺乏的一个有衔接的框架,可以指导机制研究和工业实践。
{"title":"A Comprehensive Review of Wooden Breast Myopathy in Broilers: Impacts, Detection, Processing, and Future Perspectives","authors":"Liubin Yang,&nbsp;Mengyue Zhou,&nbsp;Wei Guo,&nbsp;Haizhou Wu","doi":"10.1111/1541-4337.70414","DOIUrl":"10.1111/1541-4337.70414","url":null,"abstract":"<div>\u0000 \u0000 <p>Wooden breast (WB) myopathy is a major muscle disorder in fast-growing broilers, affecting the entire poultry production chain and causing substantial economic losses. Current mitigation strategies rely primarily on carcass-level identification, grading, and processing treatments. However, existing studies remain fragmented and insufficiently integrated, limiting effective problem-solving. In this review, we summarize and compare reported WB identification and classification methods in terms of detection principles, industrial adaptability, accuracy, cost, scalability, technological maturity, and limitations. Overall, near-infrared (NIR) spectroscopy achieves high accuracy (95%–100%), whereas imaging-based methods show greater potential for real-time, on-site application. We further review major postmortem strategies to improve WB meat quality and compare their underlying principles, key effects, applicable product types, optimization outcomes, costs, and limitations. Evidence shows that papain treatment significantly improves the quality of intact WB fillets (<i>p</i> &lt; 0.05), while functional additives and protein glycation significantly enhance the processing quality of WB meat products (<i>p</i> &lt; 0.05). Finally, in light of current research gaps, future efforts should focus on reducing the impact of WB through genetic marker screening and environmental control, the establishment of standardized identification criteria, AI-assisted modeling, and the development of WB-specific formulations and processing equipment. By systematically integrating WB pathophysiology, detection technologies, and postmortem processing interventions, this review provides a cohesive framework that is currently lacking in WB research and may guide both mechanistic studies and industrial practice.</p>\u0000 </div>","PeriodicalId":155,"journal":{"name":"Comprehensive Reviews in Food Science and Food Safety","volume":"25 2","pages":""},"PeriodicalIF":14.1,"publicationDate":"2026-02-08","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"146140466","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"农林科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Designing Protein Gels for Nutrient Delivery: From Formulation to Digestion 设计用于营养输送的蛋白质凝胶:从配方到消化。
IF 14.1 1区 农林科学 Q1 FOOD SCIENCE & TECHNOLOGY Pub Date : 2026-02-08 DOI: 10.1111/1541-4337.70424
Xue Dong, Yong Wang, Xiao Dong Chen, Cordelia Selomulya

Protein gels have diverse applications in food industry, with plant proteins as potential alternatives to animal-derived products. The applications of protein gels mainly depend on gel properties while gel digestibility affects the delivery and release of nutrients. However, the relationship and synergistic influences among gelation mechanism, gel properties, and digestive characteristics, relevant to formulate gelation strategies of animal or plant proteins, have never been systematically discussed. This review provides insights into the relationship between molecular mechanism and gel properties, and effects on delayed or rapid digestibility and delivery of bioactive ingredients. Gel digestibility and delivery of bioactive ingredients can be controlled by altering gel properties and microstructure with various gel compositions and treatments. The encapsulation and delivery systems of bioactive ingredients based on protein gels were described. Finally, a comparison between in vitro static and dynamic digestion methods was conducted to evaluate suitability, limitations, and accuracy for assessing the digestibility and nutrient release of protein gels. Dynamic in vitro digestion systems mimic closely the physiological conditions of human digestion tract compared to that of in vitro static method. The comprehensive understanding of protein gel digestion with structural design and formulation strategies, offers practical insights for developing tailored protein-rich food systems with controlled digestive behavior relevant to satiety-enhancing foods and delivery systems with targeted outcomes such as elderly nutrition.

蛋白质凝胶在食品工业中有多种应用,植物蛋白是动物源性产品的潜在替代品。蛋白质凝胶的应用主要取决于凝胶的性质,而凝胶的消化率影响营养物质的输送和释放。然而,与制定动物或植物蛋白凝胶化策略相关的凝胶机制、凝胶性质和消化特性之间的关系和协同影响尚未得到系统的讨论。本文综述了分子机制与凝胶性质的关系,以及对生物活性成分的延迟或快速消化和递送的影响。凝胶的消化率和生物活性成分的递送可以通过改变凝胶的性质和微观结构来控制。介绍了基于蛋白质凝胶的生物活性成分的包封和递送系统。最后,比较了体外静态消化法和动态消化法在评估蛋白质凝胶消化率和养分释放方面的适用性、局限性和准确性。与体外静态消化系统相比,动态体外消化系统更接近于模拟人体消化道的生理状况。通过结构设计和配方策略对蛋白质凝胶消化的全面理解,为开发量身定制的富含蛋白质的食物系统提供了实用的见解,这些系统具有与增强饱腹感的食物相关的消化行为控制,以及具有老年人营养等目标结果的输送系统。
{"title":"Designing Protein Gels for Nutrient Delivery: From Formulation to Digestion","authors":"Xue Dong,&nbsp;Yong Wang,&nbsp;Xiao Dong Chen,&nbsp;Cordelia Selomulya","doi":"10.1111/1541-4337.70424","DOIUrl":"10.1111/1541-4337.70424","url":null,"abstract":"<p>Protein gels have diverse applications in food industry, with plant proteins as potential alternatives to animal-derived products. The applications of protein gels mainly depend on gel properties while gel digestibility affects the delivery and release of nutrients. However, the relationship and synergistic influences among gelation mechanism, gel properties, and digestive characteristics, relevant to formulate gelation strategies of animal or plant proteins, have never been systematically discussed. This review provides insights into the relationship between molecular mechanism and gel properties, and effects on delayed or rapid digestibility and delivery of bioactive ingredients. Gel digestibility and delivery of bioactive ingredients can be controlled by altering gel properties and microstructure with various gel compositions and treatments. The encapsulation and delivery systems of bioactive ingredients based on protein gels were described. Finally, a comparison between in vitro static and dynamic digestion methods was conducted to evaluate suitability, limitations, and accuracy for assessing the digestibility and nutrient release of protein gels. Dynamic in vitro digestion systems mimic closely the physiological conditions of human digestion tract compared to that of in vitro static method. The comprehensive understanding of protein gel digestion with structural design and formulation strategies, offers practical insights for developing tailored protein-rich food systems with controlled digestive behavior relevant to satiety-enhancing foods and delivery systems with targeted outcomes such as elderly nutrition.</p>","PeriodicalId":155,"journal":{"name":"Comprehensive Reviews in Food Science and Food Safety","volume":"25 2","pages":""},"PeriodicalIF":14.1,"publicationDate":"2026-02-08","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.ncbi.nlm.nih.gov/pmc/articles/PMC12884030/pdf/","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"146140389","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"农林科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Harnessing Cold Plasma for Rice Grain Processing: A Systematic Review on Functional, Structural, and Nutritional Properties 利用冷等离子体加工大米:功能、结构和营养特性的系统综述。
IF 14.1 1区 农林科学 Q1 FOOD SCIENCE & TECHNOLOGY Pub Date : 2026-02-06 DOI: 10.1111/1541-4337.70409
Javaneh Karimi, Sahand Sohrabi, Zahra Teymouri, Amene Nematollahi, Leila Zare, Saeedeh Karimlar, Neda Mollakhalili-Meybodi, Ehsan Sadeghi

Rice (Oryza sativa, Oryza glaberrima) is a globally essential staple, providing vital nutrients such as carbohydrates, fiber, proteins, vitamins, and minerals. However, conventional processing methods (e.g., milling, parboiling) often degrade its physicochemical and nutritional properties, causing loss of essential components.This systematic review critically examines the potential of cold plasma (CP), an emerging non-thermal technology, for enhancing rice quality. Following PRISMA guidelines, an extensive literature search was conducted using databases including PubMed, Scopus, Web of Science, and Google Scholar. The review highlights the effects of CP on rice grain structure, starch and protein behavior, and key techno-functional and nutritional attributes. CP treatment improves water absorption, reduces cooking time, and modifies starch gelatinization and pasting profiles. It also enhances protein solubility, emulsification properties, and textural characteristics, thus enhancing the sensory and functional profile of rice-based products. From a nutritional approach, CP contributes to increased nutrient bioavailability and reduction of anti-nutritional factors, while also offering microbial decontamination and shelf-life extension. CP represents a promising, energy and cost-efficient alternative to conventional thermal processing. Its ability to preserve and enhance nutritional and functional properties without compromising impact on sensory quality makes it an ideal tool in sustainable rice grain processing and value-added grain innovation.

水稻(Oryza sativa, Oryza glaberrima)是全球必不可少的主食,提供重要的营养物质,如碳水化合物、纤维、蛋白质、维生素和矿物质。然而,传统的加工方法(如碾磨、煮熟)往往会降低其物理化学和营养特性,导致基本成分的损失。这篇系统综述批判性地探讨了冷等离子体(CP)这一新兴的非热技术在提高大米品质方面的潜力。按照PRISMA的指导方针,使用PubMed、Scopus、Web of Science和谷歌Scholar等数据库进行了广泛的文献检索。综述了粗CP对水稻籽粒结构、淀粉和蛋白质行为、关键技术功能和营养特性的影响。CP处理提高了吸水率,减少了烹饪时间,并改变了淀粉糊化和糊化特性。它还可以提高蛋白质的溶解度、乳化性能和质地特征,从而增强大米产品的感官和功能特征。从营养角度来看,CP有助于提高营养物质的生物利用度,减少抗营养因子,同时还提供微生物净化和延长保质期。CP代表了一种有前途的、能源和成本效益的传统热加工替代方案。它能够在不影响感官质量的情况下保持和增强营养和功能特性,使其成为可持续稻米加工和增值谷物创新的理想工具。
{"title":"Harnessing Cold Plasma for Rice Grain Processing: A Systematic Review on Functional, Structural, and Nutritional Properties","authors":"Javaneh Karimi,&nbsp;Sahand Sohrabi,&nbsp;Zahra Teymouri,&nbsp;Amene Nematollahi,&nbsp;Leila Zare,&nbsp;Saeedeh Karimlar,&nbsp;Neda Mollakhalili-Meybodi,&nbsp;Ehsan Sadeghi","doi":"10.1111/1541-4337.70409","DOIUrl":"10.1111/1541-4337.70409","url":null,"abstract":"<div>\u0000 \u0000 <p>Rice (Oryza sativa, Oryza glaberrima) is a globally essential staple, providing vital nutrients such as carbohydrates, fiber, proteins, vitamins, and minerals. However, conventional processing methods (e.g., milling, parboiling) often degrade its physicochemical and nutritional properties, causing loss of essential components.This systematic review critically examines the potential of cold plasma (CP), an emerging non-thermal technology, for enhancing rice quality. Following PRISMA guidelines, an extensive literature search was conducted using databases including PubMed, Scopus, Web of Science, and Google Scholar. The review highlights the effects of CP on rice grain structure, starch and protein behavior, and key techno-functional and nutritional attributes. CP treatment improves water absorption, reduces cooking time, and modifies starch gelatinization and pasting profiles. It also enhances protein solubility, emulsification properties, and textural characteristics, thus enhancing the sensory and functional profile of rice-based products. From a nutritional approach, CP contributes to increased nutrient bioavailability and reduction of anti-nutritional factors, while also offering microbial decontamination and shelf-life extension. CP represents a promising, energy and cost-efficient alternative to conventional thermal processing. Its ability to preserve and enhance nutritional and functional properties without compromising impact on sensory quality makes it an ideal tool in sustainable rice grain processing and value-added grain innovation.</p>\u0000 </div>","PeriodicalId":155,"journal":{"name":"Comprehensive Reviews in Food Science and Food Safety","volume":"25 2","pages":""},"PeriodicalIF":14.1,"publicationDate":"2026-02-06","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"146123063","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"农林科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Innovative Progress of Marine Polysaccharide-Based Intelligent Food Packaging Materials: From Film-Forming Mechanisms to Intelligent Responses and Industrialization Challenges 海洋多糖智能食品包装材料的创新进展:从成膜机理到智能响应和产业化挑战。
IF 14.1 1区 农林科学 Q1 FOOD SCIENCE & TECHNOLOGY Pub Date : 2026-02-06 DOI: 10.1111/1541-4337.70413
Hongkun Xue, Junyao Feng, Bozhao Zhang, Kaifang Xie, Xiaojun Liao, Jiaqi Tan

With the intensification of the global plastic pollution crisis and the escalation of consumers’ concern for food safety, marine polysaccharide-based intelligent food packaging (MPIFP) materials have become a research hotspot in the field of food science due to their renewability, degradability, and multifunctionality. Marine polysaccharides are mainly used to construct functionalized network structures through three cross-linking methods (physical, chemical, and enzymatic cross-linking), thereby forming films. In addition, traditional and novel preparation techniques offer diverse options for the preparation of marine polysaccharide-based films (MPFs). The introduction of indicators, sensors, and data carriers can endow MPFs with intelligent response properties, which contribute to them demonstrating great potential in monitoring food quality, extending shelf life, and providing consumer information. Currently, MPIFP has commercial cases. However, the industrialization of MPIFP still faces many challenges. Hence, this paper systematically reviews the molecular properties of marine polysaccharides and introduces the film-forming mechanisms and preparation techniques of MPFs. In addition, this review illustrates the innovative applications of MPFs in intelligent packaging. Furthermore, this paper systematically reviews the current status of intelligent packaging technology in the commercial field, as well as the advantages and industrialization challenges of MPFs. This review innovatively integrates the film-forming mechanism of marine polysaccharides, advanced preparation techniques, and their multifunctional integrated applications in indicators, sensors, and data carriers, and addresses the practical issues of industrialization, which provides cross-disciplinary and full-chain theoretical references and practical guidance for the material design, process optimization, and commercialization path of MPFs.

随着全球塑料污染危机的加剧和消费者对食品安全关注的升级,海洋多糖基智能食品包装材料因其可再生、可降解、多功能性等优点成为食品科学领域的研究热点。海洋多糖主要通过三种交联方法(物理交联、化学交联和酶交联)构建功能化的网络结构,从而形成薄膜。此外,传统的和新型的制备技术为制备海洋多糖基薄膜提供了多种选择。引入指标、传感器和数据载体可以赋予mpf智能响应特性,这有助于它们在监测食品质量、延长保质期和提供消费者信息方面显示出巨大的潜力。目前,MPIFP有商业案例。然而,MPIFP的产业化仍面临诸多挑战。因此,本文系统地综述了海洋多糖的分子性质,并介绍了MPFs的成膜机理和制备技术。此外,本文综述了mpf在智能包装中的创新应用。此外,本文系统回顾了智能包装技术在商业领域的发展现状,以及mpf的优势和产业化面临的挑战。本文创新性地整合了海洋多糖的成膜机理、先进的制备技术及其在指标、传感器、数据载体等方面的多功能集成应用,解决了产业化的实际问题,为mpf的材料设计、工艺优化和商业化路径提供了跨学科、全链的理论参考和实践指导。
{"title":"Innovative Progress of Marine Polysaccharide-Based Intelligent Food Packaging Materials: From Film-Forming Mechanisms to Intelligent Responses and Industrialization Challenges","authors":"Hongkun Xue,&nbsp;Junyao Feng,&nbsp;Bozhao Zhang,&nbsp;Kaifang Xie,&nbsp;Xiaojun Liao,&nbsp;Jiaqi Tan","doi":"10.1111/1541-4337.70413","DOIUrl":"10.1111/1541-4337.70413","url":null,"abstract":"<div>\u0000 \u0000 <p>With the intensification of the global plastic pollution crisis and the escalation of consumers’ concern for food safety, marine polysaccharide-based intelligent food packaging (MPIFP) materials have become a research hotspot in the field of food science due to their renewability, degradability, and multifunctionality. Marine polysaccharides are mainly used to construct functionalized network structures through three cross-linking methods (physical, chemical, and enzymatic cross-linking), thereby forming films. In addition, traditional and novel preparation techniques offer diverse options for the preparation of marine polysaccharide-based films (MPFs). The introduction of indicators, sensors, and data carriers can endow MPFs with intelligent response properties, which contribute to them demonstrating great potential in monitoring food quality, extending shelf life, and providing consumer information. Currently, MPIFP has commercial cases. However, the industrialization of MPIFP still faces many challenges. Hence, this paper systematically reviews the molecular properties of marine polysaccharides and introduces the film-forming mechanisms and preparation techniques of MPFs. In addition, this review illustrates the innovative applications of MPFs in intelligent packaging. Furthermore, this paper systematically reviews the current status of intelligent packaging technology in the commercial field, as well as the advantages and industrialization challenges of MPFs. This review innovatively integrates the film-forming mechanism of marine polysaccharides, advanced preparation techniques, and their multifunctional integrated applications in indicators, sensors, and data carriers, and addresses the practical issues of industrialization, which provides cross-disciplinary and full-chain theoretical references and practical guidance for the material design, process optimization, and commercialization path of MPFs.</p>\u0000 </div>","PeriodicalId":155,"journal":{"name":"Comprehensive Reviews in Food Science and Food Safety","volume":"25 2","pages":""},"PeriodicalIF":14.1,"publicationDate":"2026-02-06","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"146122988","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"农林科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Cold Plasma for Fungal and Mycotoxin Control in Low-Moisture-Content Agri-Food Products: Mechanisms and Applications 冷等离子体在低水分农产品中的真菌和霉菌毒素控制:机制和应用。
IF 14.1 1区 农林科学 Q1 FOOD SCIENCE & TECHNOLOGY Pub Date : 2026-02-02 DOI: 10.1111/1541-4337.70410
Qiaoyun Wei, Yue Wang, Lan Jiang, Jing Qian, Xiaowei Sheng, Shuang Deng, Jianhao Zhang, Jin Wang

Fungal and mycotoxin contamination can occur during multiple stages of low-moisture-content (LMC) agri-food products production, processing, and storage, posing severe threats to global food safety and trade exchanges. Therefore, its effective decontamination is a critical measure for ensuring food safety and public health. In recent years, plasma technology, as a promising solution, has been widely applied in food and agricultural processing fields due to its advantages of low cost, simple operation, high efficiency, and minimal residue. This review outlines the key factors influencing the generation, migration, and interaction of cold plasma, including plasma excitation conditions, environmental conditions, and sample characteristics. Furthermore, it elucidates the efficacy and mechanisms of plasma treatment in inactivating fungi and degrading mycotoxins. The latest decontamination applications of plasma technology across diverse LMC agri-food products are comprehensively analyzed, alongside their impact on product quality properties. Synergistic approaches combining plasma with other technologies are also evaluated to highlight their comparative advantages. Finally, the current limitations of the technology are critically analyzed, and a forward-looking perspective is provided by outlining its prospects and proposing constructive suggestions. This review aims to assist researchers in comprehensively understanding the mechanisms of plasma technology and its recent advances in practical applications, highlighting its feasibility and prospects in the food processing field, thereby promoting its transition beyond laboratory constraints toward large-scale industrial implementation.

真菌和霉菌毒素污染可能发生在低水分农产品生产、加工和储存的多个阶段,对全球食品安全和贸易交流构成严重威胁。因此,对其进行有效的去污处理是保障食品安全和公众健康的关键措施。近年来,等离子体技术以其成本低、操作简单、效率高、残留少等优点,在食品和农产品加工领域得到了广泛的应用。本文综述了影响冷等离子体产生、迁移和相互作用的关键因素,包括等离子体激发条件、环境条件和样品特性。此外,它阐明了血浆治疗在灭活真菌和降解真菌毒素方面的功效和机制。全面分析了等离子体技术在不同LMC农产品中的最新去污应用,以及它们对产品质量特性的影响。还评估了将等离子体与其他技术相结合的协同方法,以突出其比较优势。最后,批判性地分析了该技术目前的局限性,并通过概述其前景和提出建设性建议提供了前瞻性的观点。本文旨在帮助研究人员全面了解等离子体技术的机理及其在实际应用中的最新进展,强调其在食品加工领域的可行性和前景,从而促进其从实验室限制向大规模工业应用的过渡。
{"title":"Cold Plasma for Fungal and Mycotoxin Control in Low-Moisture-Content Agri-Food Products: Mechanisms and Applications","authors":"Qiaoyun Wei,&nbsp;Yue Wang,&nbsp;Lan Jiang,&nbsp;Jing Qian,&nbsp;Xiaowei Sheng,&nbsp;Shuang Deng,&nbsp;Jianhao Zhang,&nbsp;Jin Wang","doi":"10.1111/1541-4337.70410","DOIUrl":"10.1111/1541-4337.70410","url":null,"abstract":"<div>\u0000 \u0000 <p>Fungal and mycotoxin contamination can occur during multiple stages of low-moisture-content (LMC) agri-food products production, processing, and storage, posing severe threats to global food safety and trade exchanges. Therefore, its effective decontamination is a critical measure for ensuring food safety and public health. In recent years, plasma technology, as a promising solution, has been widely applied in food and agricultural processing fields due to its advantages of low cost, simple operation, high efficiency, and minimal residue. This review outlines the key factors influencing the generation, migration, and interaction of cold plasma, including plasma excitation conditions, environmental conditions, and sample characteristics. Furthermore, it elucidates the efficacy and mechanisms of plasma treatment in inactivating fungi and degrading mycotoxins. The latest decontamination applications of plasma technology across diverse LMC agri-food products are comprehensively analyzed, alongside their impact on product quality properties. Synergistic approaches combining plasma with other technologies are also evaluated to highlight their comparative advantages. Finally, the current limitations of the technology are critically analyzed, and a forward-looking perspective is provided by outlining its prospects and proposing constructive suggestions. This review aims to assist researchers in comprehensively understanding the mechanisms of plasma technology and its recent advances in practical applications, highlighting its feasibility and prospects in the food processing field, thereby promoting its transition beyond laboratory constraints toward large-scale industrial implementation.</p>\u0000 </div>","PeriodicalId":155,"journal":{"name":"Comprehensive Reviews in Food Science and Food Safety","volume":"25 2","pages":""},"PeriodicalIF":14.1,"publicationDate":"2026-02-02","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"146103262","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"农林科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
The Prebiotic and Techno-Functional Potential of Microbial Exopolysaccharides for Human Health and Food Systems 微生物胞外多糖对人体健康和食品系统的益生元和技术功能潜力。
IF 14.1 1区 农林科学 Q1 FOOD SCIENCE & TECHNOLOGY Pub Date : 2026-01-31 DOI: 10.1111/1541-4337.70406
Md. Abdur Razzak, Hye Kim, Md. Ariful Haque, Min Ji Jang, Sehyeon Song, Anishka Talari, Lakshmi Devi Chittepu, Seockmo Ku

Microbial exopolysaccharides (EPS) represent a diverse class of biopolymers holding considerable promise as functional food ingredients. This review analyzes the dual function of microbial EPS as a candidate for prebiotic agents and techno-functional additives. Differentiating between broad chemical categories and validated functional ingredients is critical. Many EPS are resistant to digestion; however, only those that meet the criteria established by the International Scientific Association for Probiotics and Prebiotics (ISAPP)—notably, selective utilization by host microorganisms that confer health benefits—are classified as prebiotics. This review examines the “EPS-microbiota-host axis,” demonstrating how specific prebiotic EPS influence gut ecology to produce short-chain fatty acids (SCFAs). These metabolites regulate immunomodulatory and systemic metabolic homeostasis, which may have therapeutic benefits for conditions including diabetes and obesity. It is essential to differentiate microbiota-mediated effects from direct biological mechanisms associated with “bioactive EPS,” including immune receptor modulation, which operate independently of fermentation and should not be equated with postbiotics. Beyond health, the structural complexity underpinning these activities confers significant techno-functional utility. We explore EPS as natural emulsifiers, rheology modifiers, and biodegradable packaging materials, emphasizing their stabilizing roles in dairy and bakery systems. Finally, we examine techno-economic barriers, particularly production scalability, that hinder widespread adoption and discuss the potential of synthetic biology to engineer “designer” polysaccharides. This synthesis clarifies the precise roles of microbial EPS as sustainable, multifunctional ingredients in developing next-generation healthy foods.

微生物胞外多糖(EPS)代表了一类具有相当前景的功能性食品成分的生物聚合物。本文综述了微生物EPS作为益生元制剂和技术功能添加剂的双重功能。区分广泛的化学类别和经过验证的功能成分至关重要。许多EPS难以消化;然而,只有那些符合国际益生菌和益生元科学协会(ISAPP)制定的标准的益生元才被归类为益生元,特别是那些被宿主微生物选择性利用并赋予健康益处的益生元。本文综述了“EPS-微生物-宿主轴”,展示了特定益生元EPS如何影响肠道生态产生短链脂肪酸(SCFAs)。这些代谢物调节免疫调节和全身代谢稳态,这可能对包括糖尿病和肥胖在内的疾病有治疗益处。必须将微生物介导的效应与与“生物活性EPS”相关的直接生物学机制区分开来,包括免疫受体调节,后者独立于发酵作用,不应等同于后生物效应。除了健康之外,支撑这些活动的结构复杂性赋予了重要的技术功能效用。我们将探讨EPS作为天然乳化剂、流变调节剂和可生物降解的包装材料,强调其在乳制品和烘焙系统中的稳定作用。最后,我们研究了阻碍广泛采用的技术经济障碍,特别是生产可扩展性,并讨论了合成生物学设计“设计”多糖的潜力。这一合成阐明了微生物EPS作为可持续的多功能成分在开发下一代健康食品中的确切作用。
{"title":"The Prebiotic and Techno-Functional Potential of Microbial Exopolysaccharides for Human Health and Food Systems","authors":"Md. Abdur Razzak,&nbsp;Hye Kim,&nbsp;Md. Ariful Haque,&nbsp;Min Ji Jang,&nbsp;Sehyeon Song,&nbsp;Anishka Talari,&nbsp;Lakshmi Devi Chittepu,&nbsp;Seockmo Ku","doi":"10.1111/1541-4337.70406","DOIUrl":"10.1111/1541-4337.70406","url":null,"abstract":"<p>Microbial exopolysaccharides (EPS) represent a diverse class of biopolymers holding considerable promise as functional food ingredients. This review analyzes the dual function of microbial EPS as a candidate for prebiotic agents and techno-functional additives. Differentiating between broad chemical categories and validated functional ingredients is critical. Many EPS are resistant to digestion; however, only those that meet the criteria established by the International Scientific Association for Probiotics and Prebiotics (ISAPP)—notably, selective utilization by host microorganisms that confer health benefits—are classified as prebiotics. This review examines the “EPS-microbiota-host axis,” demonstrating how specific prebiotic EPS influence gut ecology to produce short-chain fatty acids (SCFAs). These metabolites regulate immunomodulatory and systemic metabolic homeostasis, which may have therapeutic benefits for conditions including diabetes and obesity. It is essential to differentiate microbiota-mediated effects from direct biological mechanisms associated with “bioactive EPS,” including immune receptor modulation, which operate independently of fermentation and should not be equated with postbiotics. Beyond health, the structural complexity underpinning these activities confers significant techno-functional utility. We explore EPS as natural emulsifiers, rheology modifiers, and biodegradable packaging materials, emphasizing their stabilizing roles in dairy and bakery systems. Finally, we examine techno-economic barriers, particularly production scalability, that hinder widespread adoption and discuss the potential of synthetic biology to engineer “designer” polysaccharides. This synthesis clarifies the precise roles of microbial EPS as sustainable, multifunctional ingredients in developing next-generation healthy foods.</p>","PeriodicalId":155,"journal":{"name":"Comprehensive Reviews in Food Science and Food Safety","volume":"25 2","pages":""},"PeriodicalIF":14.1,"publicationDate":"2026-01-31","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.ncbi.nlm.nih.gov/pmc/articles/PMC12860486/pdf/","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"146096789","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"农林科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Additional Cover: Cover Image, Volume 25, Issue 1 附加封面:第25卷第1期封面图片
IF 14.1 1区 农林科学 Q1 FOOD SCIENCE & TECHNOLOGY Pub Date : 2026-01-28 DOI: 10.1111/1541-4337.70416
Guotao Xue, Tao Zhou, Mengqi Li, Qiang Yu, Zhiyan Deng, Junzhi Lin, Chuan Zheng, Li Han, Dingkun Zhang, Haozhou Huang

The cover image is based on the Comprehensive Review Sweet Aftertaste (Huigan) in Foods: Evaluation and Processing Impacts for Enhanced Flavor Design and Applications by Guotao Xue et al., https://doi.org/10.1111/1541-4337.70378.

封面图片来源于薛国涛等人的综合综述《食品中的甜余味:强化风味设计与应用的评价与加工影响》https://doi.org/10.1111/1541-4337.70378。
{"title":"Additional Cover: Cover Image, Volume 25, Issue 1","authors":"Guotao Xue,&nbsp;Tao Zhou,&nbsp;Mengqi Li,&nbsp;Qiang Yu,&nbsp;Zhiyan Deng,&nbsp;Junzhi Lin,&nbsp;Chuan Zheng,&nbsp;Li Han,&nbsp;Dingkun Zhang,&nbsp;Haozhou Huang","doi":"10.1111/1541-4337.70416","DOIUrl":"https://doi.org/10.1111/1541-4337.70416","url":null,"abstract":"<p>The cover image is based on the Comprehensive Review <i>Sweet Aftertaste (Huigan) in Foods: Evaluation and Processing Impacts for Enhanced Flavor Design and Applications</i> by Guotao Xue et al., https://doi.org/10.1111/1541-4337.70378.\u0000\u0000 <figure>\u0000 <div><picture>\u0000 <source></source></picture><p></p>\u0000 </div>\u0000 </figure></p>","PeriodicalId":155,"journal":{"name":"Comprehensive Reviews in Food Science and Food Safety","volume":"25 1","pages":""},"PeriodicalIF":14.1,"publicationDate":"2026-01-28","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://ift.onlinelibrary.wiley.com/doi/epdf/10.1111/1541-4337.70416","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"146176492","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"农林科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Quality Analysis and Detection of Adulterants and Contaminations in Milk/Milk Powder by Raman Spectroscopy 牛奶/奶粉中掺假和污染物的拉曼光谱质量分析与检测。
IF 14.1 1区 农林科学 Q1 FOOD SCIENCE & TECHNOLOGY Pub Date : 2026-01-24 DOI: 10.1111/1541-4337.70403
B. Sudarshan Acharya, Sreerag Nair, Abdul Ajees Abdul Salam
<p>Milk and milk powder are central to global nutrition, yet remain vulnerable to adulteration and contamination. Adulteration using water, urea, ammonium sulfate, thiocyanates, detergents, melamine, or compositional changes with whey and carbohydrate fillers undermines nutritional quality, reduces consumer confidence, and challenges regulatory control, particularly in infant formula products. A field-ready analytical platform that is rapid, nondestructive, and capable of multi-adulterant surveillance is urgently needed across diverse dairy matrices. This review consolidates advances in Raman spectroscopy for milk and milk powder authentication reported from 2015 to early 2025, covering conventional Raman, surface-enhanced Raman spectroscopy (SERS), Fourier-transform Raman, hyperspectral Raman imaging, confocal/mapping approaches, and portable systems. We critically evaluate preprocessing and chemometrics such as principal component analysis, partial least squares regression, and partial least squares discriminant analysis, as well as machine-learning and deep-learning pipelines for classification and quantification. Species-specific applications including cow, buffalo, goat, camel, donkey, human breast milk (macronutrients, sex-linked profiles, microplastics, antibiotics), and milk powder workflows are compared with attention to matrix effects, fluorescence interference, and validation practices. Raman enables chemically specific fingerprints of proteins, lipids, and carbohydrates, whereas common adulterants present diagnostic bands. SERS substrates routinely extend sensitivity to ppm–ppb levels and suppress fluorescence, supporting rapid detection of melamine, urea, ammonium sulfate, thiocyanates, benzoate, and selected antibiotics. Hyperspectral imaging provides spatially resolved maps, differentiating multi-adulterant mixtures and thermo-structural behavior in powders. Chemometric models achieve high accuracy for classification and concentration prediction, whereas deep-learning architectures improve robustness under nonlinear matrix variation and instrument drift. Challenges persist in substrate reproducibility, calibration transfer, fluorescence in lipid-rich systems, and detection of emerging adulterants and trace preservatives under field conditions. Future progress will hinge on multi-excitation instruments with adaptive laser power control, universal SERS substrates integrating plasmonic metals, dielectric shells, and molecular recognition, and standard operating procedure grade preprocessing. Industrial reliability requires calibration-transfer strategies, rigorous validation, and explainable artificial intelligence to link decisions to chemically meaningful features, supporting regulatory acceptance and auditability. Portable Raman and SERS systems can aid nutritional profiling and contaminant surveillance in breast milk, whereas Fourier-transform Raman and hyperspectral imaging mitigate fluorescence and map heterogeneity in powders.
牛奶和奶粉是全球营养的核心,但仍然容易受到掺假和污染的影响。使用水、尿素、硫酸铵、硫氰酸盐、洗涤剂、三聚氰胺或改变乳清和碳水化合物填充物的成分进行掺假会破坏营养质量,降低消费者信心,并对监管控制构成挑战,特别是在婴儿配方奶粉产品中。一个现场准备的分析平台,是快速的,非破坏性的,并能够多种掺假监测是迫切需要在不同的乳制品矩阵。本文综述了2015年至2025年初拉曼光谱在牛奶和奶粉认证方面的进展,包括传统拉曼光谱、表面增强拉曼光谱(SERS)、傅里叶变换拉曼光谱、高光谱拉曼成像、共聚焦/映射方法和便携式系统。我们批判性地评估预处理和化学计量学,如主成分分析、偏最小二乘回归和偏最小二乘判别分析,以及用于分类和量化的机器学习和深度学习管道。物种特异性应用包括牛、水牛、山羊、骆驼、驴、人母乳(常量营养素、性别连锁谱、微塑料、抗生素)和奶粉工作流程,与基质效应、荧光干扰和验证实践的关注进行了比较。拉曼光谱使得蛋白质、脂类和碳水化合物的化学指纹图谱具有特异性,而常见的掺假物则呈现诊断谱带。SERS底物常规地将灵敏度扩展到ppm-ppb水平并抑制荧光,支持快速检测三聚氰胺、尿素、硫酸铵、硫氰酸酯、苯甲酸酯和选定的抗生素。高光谱成像提供空间分辨图,区分多掺杂混合物和粉末的热结构行为。化学计量模型在分类和浓度预测方面实现了高精度,而深度学习架构在非线性矩阵变化和仪器漂移下提高了鲁棒性。挑战仍然存在于底物再现性、校准转移、富脂系统中的荧光以及现场条件下新出现的掺假和微量防腐剂的检测。未来的进展将取决于具有自适应激光功率控制的多激励仪器,集成等离子体金属、介电壳和分子识别的通用SERS衬底,以及标准操作程序级预处理。工业可靠性需要校准转移策略、严格的验证和可解释的人工智能,以将决策与化学有意义的特征联系起来,支持监管接受和可审计性。便携式拉曼和SERS系统可以帮助母乳中的营养分析和污染物监测,而傅里叶变换拉曼和高光谱成像可以减轻粉末中的荧光和地图异质性。拉曼光谱,增强了SERS、高光谱成像和智能分析,为乳制品认证提供了一个快速、无损、无标签和可扩展的平台。持续的创新将使实时、现场检测单一和多种掺杂物成为可能,增强消费者信心、工业质量保证和法规遵从性,同时推进全球食品安全。
{"title":"Quality Analysis and Detection of Adulterants and Contaminations in Milk/Milk Powder by Raman Spectroscopy","authors":"B. Sudarshan Acharya,&nbsp;Sreerag Nair,&nbsp;Abdul Ajees Abdul Salam","doi":"10.1111/1541-4337.70403","DOIUrl":"10.1111/1541-4337.70403","url":null,"abstract":"&lt;p&gt;Milk and milk powder are central to global nutrition, yet remain vulnerable to adulteration and contamination. Adulteration using water, urea, ammonium sulfate, thiocyanates, detergents, melamine, or compositional changes with whey and carbohydrate fillers undermines nutritional quality, reduces consumer confidence, and challenges regulatory control, particularly in infant formula products. A field-ready analytical platform that is rapid, nondestructive, and capable of multi-adulterant surveillance is urgently needed across diverse dairy matrices. This review consolidates advances in Raman spectroscopy for milk and milk powder authentication reported from 2015 to early 2025, covering conventional Raman, surface-enhanced Raman spectroscopy (SERS), Fourier-transform Raman, hyperspectral Raman imaging, confocal/mapping approaches, and portable systems. We critically evaluate preprocessing and chemometrics such as principal component analysis, partial least squares regression, and partial least squares discriminant analysis, as well as machine-learning and deep-learning pipelines for classification and quantification. Species-specific applications including cow, buffalo, goat, camel, donkey, human breast milk (macronutrients, sex-linked profiles, microplastics, antibiotics), and milk powder workflows are compared with attention to matrix effects, fluorescence interference, and validation practices. Raman enables chemically specific fingerprints of proteins, lipids, and carbohydrates, whereas common adulterants present diagnostic bands. SERS substrates routinely extend sensitivity to ppm–ppb levels and suppress fluorescence, supporting rapid detection of melamine, urea, ammonium sulfate, thiocyanates, benzoate, and selected antibiotics. Hyperspectral imaging provides spatially resolved maps, differentiating multi-adulterant mixtures and thermo-structural behavior in powders. Chemometric models achieve high accuracy for classification and concentration prediction, whereas deep-learning architectures improve robustness under nonlinear matrix variation and instrument drift. Challenges persist in substrate reproducibility, calibration transfer, fluorescence in lipid-rich systems, and detection of emerging adulterants and trace preservatives under field conditions. Future progress will hinge on multi-excitation instruments with adaptive laser power control, universal SERS substrates integrating plasmonic metals, dielectric shells, and molecular recognition, and standard operating procedure grade preprocessing. Industrial reliability requires calibration-transfer strategies, rigorous validation, and explainable artificial intelligence to link decisions to chemically meaningful features, supporting regulatory acceptance and auditability. Portable Raman and SERS systems can aid nutritional profiling and contaminant surveillance in breast milk, whereas Fourier-transform Raman and hyperspectral imaging mitigate fluorescence and map heterogeneity in powders. ","PeriodicalId":155,"journal":{"name":"Comprehensive Reviews in Food Science and Food Safety","volume":"25 1","pages":""},"PeriodicalIF":14.1,"publicationDate":"2026-01-24","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.ncbi.nlm.nih.gov/pmc/articles/PMC12831472/pdf/","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"146040024","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"农林科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
期刊
Comprehensive Reviews in Food Science and Food Safety
全部 Acc. Chem. Res. ACS Applied Bio Materials ACS Appl. Electron. Mater. ACS Appl. Energy Mater. ACS Appl. Mater. Interfaces ACS Appl. Nano Mater. ACS Appl. Polym. Mater. ACS BIOMATER-SCI ENG ACS Catal. ACS Cent. Sci. ACS Chem. Biol. ACS Chemical Health & Safety ACS Chem. Neurosci. ACS Comb. Sci. ACS Earth Space Chem. ACS Energy Lett. ACS Infect. Dis. ACS Macro Lett. ACS Mater. Lett. ACS Med. Chem. Lett. ACS Nano ACS Omega ACS Photonics ACS Sens. ACS Sustainable Chem. Eng. ACS Synth. Biol. Anal. Chem. BIOCHEMISTRY-US Bioconjugate Chem. BIOMACROMOLECULES Chem. Res. Toxicol. Chem. Rev. Chem. Mater. CRYST GROWTH DES ENERG FUEL Environ. Sci. Technol. Environ. Sci. Technol. Lett. Eur. J. Inorg. Chem. IND ENG CHEM RES Inorg. Chem. J. Agric. Food. Chem. J. Chem. Eng. Data J. Chem. Educ. J. Chem. Inf. Model. J. Chem. Theory Comput. J. Med. Chem. J. Nat. Prod. J PROTEOME RES J. Am. Chem. Soc. LANGMUIR MACROMOLECULES Mol. Pharmaceutics Nano Lett. Org. Lett. ORG PROCESS RES DEV ORGANOMETALLICS J. Org. Chem. J. Phys. Chem. J. Phys. Chem. A J. Phys. Chem. B J. Phys. Chem. C J. Phys. Chem. Lett. Analyst Anal. Methods Biomater. Sci. Catal. Sci. Technol. Chem. Commun. Chem. Soc. Rev. CHEM EDUC RES PRACT CRYSTENGCOMM Dalton Trans. Energy Environ. Sci. ENVIRON SCI-NANO ENVIRON SCI-PROC IMP ENVIRON SCI-WAT RES Faraday Discuss. Food Funct. Green Chem. Inorg. Chem. Front. Integr. Biol. J. Anal. At. Spectrom. J. Mater. Chem. A J. Mater. Chem. B J. Mater. Chem. C Lab Chip Mater. Chem. Front. Mater. Horiz. MEDCHEMCOMM Metallomics Mol. Biosyst. Mol. Syst. Des. Eng. Nanoscale Nanoscale Horiz. Nat. Prod. Rep. New J. Chem. Org. Biomol. Chem. Org. Chem. Front. PHOTOCH PHOTOBIO SCI PCCP Polym. Chem.
×
引用
GB/T 7714-2015
复制
MLA
复制
APA
复制
导出至
BibTeX EndNote RefMan NoteFirst NoteExpress
×
0
微信
客服QQ
Book学术公众号 扫码关注我们
反馈
×
意见反馈
请填写您的意见或建议
请填写您的手机或邮箱
×
提示
您的信息不完整,为了账户安全,请先补充。
现在去补充
×
提示
您因"违规操作"
具体请查看互助需知
我知道了
×
提示
现在去查看 取消
×
提示
确定
Book学术官方微信
Book学术文献互助
Book学术文献互助群
群 号:604180095
Book学术
文献互助 智能选刊 最新文献 互助须知 联系我们:info@booksci.cn
Book学术提供免费学术资源搜索服务,方便国内外学者检索中英文文献。致力于提供最便捷和优质的服务体验。
Copyright © 2023 Book学术 All rights reserved.
ghs 京公网安备 11010802042870号 京ICP备2023020795号-1