首页 > 最新文献

Journal of environmental radioactivity最新文献

英文 中文
Inter-site comparison of radiocesium flux via litterfall more than a decade after the Fukushima nuclear accident 福岛核事故发生十多年后,废弃物中放射性元素通量的站点间比较。
IF 2.1 3区 环境科学与生态学 Q3 ENVIRONMENTAL SCIENCES Pub Date : 2025-12-23 DOI: 10.1016/j.jenvrad.2025.107880
Wataru Sakashita , Satoru Miura , Yoshiki Shinomiya
To accurately predict the long-term dynamics of radiocesium (137Cs) in forests contaminated by the nuclear accident, it is important to monitor 137Cs fluxes in forest ecosystems more than ten years after the accident. Among these fluxes, 137Cs transfer via litterfall—a major pathway by which trees return 137Cs to the soil—is one of the key processes to observe. However, in forests more than a decade after the Fukushima accident, observations of litterfall remain limited, and the extent of site-to-site variation has not been evaluated. In this study, we conducted new observations of litterfall over a two-year period from December 1, 2022, to November 28 or 29, 2024, at three Japanese cedar forest sites and three deciduous broad-leaved forest sites in Fukushima Prefecture, and obtained annual 137Cs fluxes via litterfall. Our results revealed that, in Japanese cedar forests, between 0.080% and 0.29% of the initial 137Cs deposition was transferred via litterfall, whereas in deciduous broad-leaved forests, the proportion ranged from 0.22% to 0.37%. Based on the evaluation of site-to-site variation using box plots, including previously reported values, the median proportion of 137Cs flux via litterfall relative to the initial deposition was 0.29% (95% confidence interval: 0.11–0.77%) in Japanese cedar forests and 0.33% (95% confidence interval: 0.27–0.41%) in deciduous broad-leaved forests. The results also indicated that the site-to-site variation tended to be relatively greater in Japanese cedar forests. These findings are expected to support modeling efforts aimed at predicting the distribution of 137Cs in forest ecosystems by providing a basis for evaluating the variability and uncertainty of 137Cs transfer between trees and soil as model parameters.
为了准确预测核事故污染森林中放射性铯(137Cs)的长期动态,有必要在事故发生后十多年监测森林生态系统中的放射性铯(137Cs)通量。在这些通量中,137Cs通过凋落物(树木将137Cs返回土壤的主要途径)的转移是需要观察的关键过程之一。然而,在福岛事故发生十多年后的森林中,对凋落物的观测仍然有限,而且还没有对不同地点的变化程度进行评估。本研究从2022年12月1日至2024年11月28日或29日,在福岛县3个日本雪松林和3个落叶阔叶林站点进行了为期2年的新凋落物观测,获得了凋落物的年137Cs通量。结果表明,在日本杉林中,通过凋落物转移的137Cs初始沉降量为0.080% ~ 0.29%,而在落叶阔叶林中,这一比例为0.22% ~ 0.37%。利用箱形图评价凋落物中137Cs通量相对于初始沉降的中位数比例,在日本杉林为0.29%(95%可信区间:0.11 ~ 0.77%),在落叶阔叶林为0.33%(95%可信区间:0.27 ~ 0.41%)。结果还表明,杉木林的点间差异相对较大。这些发现有望通过为评估作为模型参数的137Cs在树木和土壤之间转移的变异性和不确定性提供依据,支持旨在预测森林生态系统中137Cs分布的建模工作。
{"title":"Inter-site comparison of radiocesium flux via litterfall more than a decade after the Fukushima nuclear accident","authors":"Wataru Sakashita ,&nbsp;Satoru Miura ,&nbsp;Yoshiki Shinomiya","doi":"10.1016/j.jenvrad.2025.107880","DOIUrl":"10.1016/j.jenvrad.2025.107880","url":null,"abstract":"<div><div>To accurately predict the long-term dynamics of radiocesium (<sup>137</sup>Cs) in forests contaminated by the nuclear accident, it is important to monitor <sup>137</sup>Cs fluxes in forest ecosystems more than ten years after the accident. Among these fluxes, <sup>137</sup>Cs transfer via litterfall—a major pathway by which trees return <sup>137</sup>Cs to the soil—is one of the key processes to observe. However, in forests more than a decade after the Fukushima accident, observations of litterfall remain limited, and the extent of site-to-site variation has not been evaluated. In this study, we conducted new observations of litterfall over a two-year period from December 1, 2022, to November 28 or 29, 2024, at three Japanese cedar forest sites and three deciduous broad-leaved forest sites in Fukushima Prefecture, and obtained annual <sup>137</sup>Cs fluxes via litterfall. Our results revealed that, in Japanese cedar forests, between 0.080% and 0.29% of the initial <sup>137</sup>Cs deposition was transferred via litterfall, whereas in deciduous broad-leaved forests, the proportion ranged from 0.22% to 0.37%. Based on the evaluation of site-to-site variation using box plots, including previously reported values, the median proportion of <sup>137</sup>Cs flux via litterfall relative to the initial deposition was 0.29% (95% confidence interval: 0.11–0.77%) in Japanese cedar forests and 0.33% (95% confidence interval: 0.27–0.41%) in deciduous broad-leaved forests. The results also indicated that the site-to-site variation tended to be relatively greater in Japanese cedar forests. These findings are expected to support modeling efforts aimed at predicting the distribution of <sup>137</sup>Cs in forest ecosystems by providing a basis for evaluating the variability and uncertainty of <sup>137</sup>Cs transfer between trees and soil as model parameters.</div></div>","PeriodicalId":15667,"journal":{"name":"Journal of environmental radioactivity","volume":"292 ","pages":"Article 107880"},"PeriodicalIF":2.1,"publicationDate":"2025-12-23","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145827798","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
A new approach to assessing and mapping geogenic radon hazard 地质氡危害评价与制图新方法。
IF 2.1 3区 环境科学与生态学 Q3 ENVIRONMENTAL SCIENCES Pub Date : 2025-12-22 DOI: 10.1016/j.jenvrad.2025.107882
Egor I. Kaygorodov , Petr S. Miklyaev , Tatiana B. Petrova
Radon in buildings is the second most significant risk factor for lung cancer after smoking. Indoor radon concentrations are largely controlled by so-called geogenic radon, which forms in soils and rocks containing radium-226. Mapping the geogenic radon hazard is an urgent task that makes it possible to make managerial decisions in the field of radon standardization. In particular, mapping the geogenic radon hazard makes it possible to identify radon priority areas, which is a requirement of EURATOM BSS. There are different ways to mapping the geogenic radon hazard, and they all have their advantages and limitations.
In this paper, a method for assessing and mapping Diffusion Radon Potential is proposed. This is a new approach to assessing and city-scale mapping geogenic radon hazard of the territories based on the analysis of data on radium concentration and radon diffusion length in shallow soils. An original method for estimating the diffusion coefficient is proposed. It has been shown that in many cases radon transport in soils can be described by a diffusion transport model with a diffusion length from 0.9 m in weakly permeable clays to 2.4 m in well-understood dry sediments. An example of mapping the diffusive radon potential is given using the example of Pyatigorsk and Moscow.
建筑物中的氡是肺癌的第二大危险因素,仅次于吸烟。室内氡浓度主要受所谓的地质氡控制,它形成于含有镭-226的土壤和岩石中。地质氡危害制图是一项紧迫的任务,为氡标准化管理决策提供了可能。特别是,测绘地质氡危害使确定氡优先区域成为可能,这是EURATOM BSS的一项要求。测绘地质氡危害的方法多种多样,各有优缺点。本文提出了一种估算扩散氡势的方法。通过对浅层土壤中镭浓度和氡扩散长度数据的分析,提出了在城市尺度上进行国土地质氡危害评价和制图的新方法。提出了一种估算扩散系数的新方法。研究表明,在许多情况下,氡在土壤中的传输可以用扩散传输模型来描述,扩散长度从弱渗透性粘土中的0.9 m到熟知的干沉积物中的2.4 m。以皮亚季戈尔斯克和莫斯科为例,给出了氡扩散势的作图。
{"title":"A new approach to assessing and mapping geogenic radon hazard","authors":"Egor I. Kaygorodov ,&nbsp;Petr S. Miklyaev ,&nbsp;Tatiana B. Petrova","doi":"10.1016/j.jenvrad.2025.107882","DOIUrl":"10.1016/j.jenvrad.2025.107882","url":null,"abstract":"<div><div>Radon in buildings is the second most significant risk factor for lung cancer after smoking. Indoor radon concentrations are largely controlled by so-called geogenic radon, which forms in soils and rocks containing radium-226. Mapping the geogenic radon hazard is an urgent task that makes it possible to make managerial decisions in the field of radon standardization. In particular, mapping the geogenic radon hazard makes it possible to identify radon priority areas, which is a requirement of EURATOM BSS. There are different ways to mapping the geogenic radon hazard, and they all have their advantages and limitations.</div><div>In this paper, a method for assessing and mapping Diffusion Radon Potential is proposed. This is a new approach to assessing and city-scale mapping geogenic radon hazard of the territories based on the analysis of data on radium concentration and radon diffusion length in shallow soils. An original method for estimating the diffusion coefficient is proposed. It has been shown that in many cases radon transport in soils can be described by a diffusion transport model with a diffusion length from 0.9 m in weakly permeable clays to 2.4 m in well-understood dry sediments. An example of mapping the diffusive radon potential is given using the example of Pyatigorsk and Moscow.</div></div>","PeriodicalId":15667,"journal":{"name":"Journal of environmental radioactivity","volume":"292 ","pages":"Article 107882"},"PeriodicalIF":2.1,"publicationDate":"2025-12-22","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145819321","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
238U and 234U relationships in groundwater of Itararé Group, São Paulo State, Brazil 巴西圣保罗州itarar<s:1>组地下水中238U和234U的关系
IF 2.1 3区 环境科学与生态学 Q3 ENVIRONMENTAL SCIENCES Pub Date : 2025-12-19 DOI: 10.1016/j.jenvrad.2025.107881
Carlos Pinto Fracalossi , Peter Christian Hackspacher , Daniel Marcos Bonotto
This paper describes a novel database for the dissolved uranium concentration and 234U/238U activity ratio (AR) in groundwater samples (16), with a focus on those occurring in the Itararé Group in São Paulo State, Brazil. Such a geological unit takes a major role in the multilayered Tubarão Aquifer System (TAS), which has been extensively exploited, primarily due to water use for industrial purposes, agriculture, and human consumption, which has resulted in a drastic lowering of the groundwater static level. As a consequence, efforts have been made by the use of different approaches to understand the processes related to the groundwater flow after infiltration in the recharge area, inclusive by the use of the natural U-isotopes 238U and 234U as reported in this paper. Therefore, hydrogeochemical diagrams utilizing both parameters (dissolved U concentration and AR) were constructed from data obtained by alpha spectrometry, aiming to find trends associated with the groundwater flow direction, as well as with processes involving the mixture of different water sources.
本文描述了一个新的地下水样品中溶解铀浓度和234U/238U活度比(AR)的数据库(16),重点是巴西圣保罗州itarar群的地下水样品。这样一个地质单元在多层的tubar含水层系统(TAS)中起着重要作用,该系统已被广泛开发,主要是由于工业、农业和人类消费用水,这导致地下水静态水平急剧下降。因此,人们通过使用不同的方法来了解地下水在补给区入渗后的流动过程,包括本文所报道的使用天然铀同位素238U和234U。因此,利用α光谱法获得的数据构建了利用这两个参数(溶解U浓度和AR)的水文地球化学图,旨在找到与地下水流向相关的趋势,以及涉及不同水源混合的过程。
{"title":"238U and 234U relationships in groundwater of Itararé Group, São Paulo State, Brazil","authors":"Carlos Pinto Fracalossi ,&nbsp;Peter Christian Hackspacher ,&nbsp;Daniel Marcos Bonotto","doi":"10.1016/j.jenvrad.2025.107881","DOIUrl":"10.1016/j.jenvrad.2025.107881","url":null,"abstract":"<div><div>This paper describes a novel database for the dissolved uranium concentration and <sup>234</sup>U/<sup>238</sup>U activity ratio (AR) in groundwater samples (16), with a focus on those occurring in the Itararé Group in São Paulo State, Brazil. Such a geological unit takes a major role in the multilayered Tubarão Aquifer System (TAS), which has been extensively exploited, primarily due to water use for industrial purposes, agriculture, and human consumption, which has resulted in a drastic lowering of the groundwater static level. As a consequence, efforts have been made by the use of different approaches to understand the processes related to the groundwater flow after infiltration in the recharge area, inclusive by the use of the natural U-isotopes <sup>238</sup>U and <sup>234</sup>U as reported in this paper. Therefore, hydrogeochemical diagrams utilizing both parameters (dissolved U concentration and AR) were constructed from data obtained by alpha spectrometry, aiming to find trends associated with the groundwater flow direction, as well as with processes involving the mixture of different water sources.</div></div>","PeriodicalId":15667,"journal":{"name":"Journal of environmental radioactivity","volume":"292 ","pages":"Article 107881"},"PeriodicalIF":2.1,"publicationDate":"2025-12-19","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145787106","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Origin of an elevated radioxenon episode: A comparative study between the Swedish radioxenon array and the CTBT International Monitoring System 放射性氙升高事件的起因:瑞典放射性氙阵列与全面禁止核试验条约国际监测系统的比较研究。
IF 2.1 3区 环境科学与生态学 Q3 ENVIRONMENTAL SCIENCES Pub Date : 2025-12-17 DOI: 10.1016/j.jenvrad.2025.107875
Sofie Liljegren , J. Ole Ross , Sofia Brander
Between late November and early December 2022, large airborne activity concentrations of radioxenon were detected by multiple stations in the CTBT International Monitoring System (IMS) and the Swedish radioxenon array, which consisted of four operational radioxenon measurement units at the time. Over 100 samples containing 133Xe were recorded during this period, with 133mXe found concurrently in about a dozen samples. The consistent 133mXe to 133Xe activity ratio, and investigations with backward atmospheric transport models (ATM), suggests a sustained release of radioxenon from a single source for about two weeks. A grid of forward ATMs was computed, and model results were matched with observations to identify potential source regions and estimate the source term. We compare locating power of the sparse, globally distributed IMS network with the compact, local Swedish radioxenon array. In this specific case, the use of the array data both significantly improved the source localization area, and helped exclude local sources, when compared to exclusively using IMS observations. Additionally the 133mXe to 133Xe activity ratio was investigated for source characterization, and was found to be consistent with the start of a nuclear reactor cycle.
在2022年11月底至12月初期间,全面禁试条约国际监测系统(IMS)的多个站点和瑞典放射性氙阵列(当时由四个运行中的放射性氙测量单元组成)检测到大量的机载放射性氙活动浓度。在此期间,超过100个含有133Xe的样本被记录下来,其中大约有12个样本同时含有133mXe。一致的133mXe和133Xe活度比,以及对反向大气输送模式(ATM)的研究表明,单一来源的放射性氙持续释放约两周。计算前向自动取款机网格,并将模型结果与观测结果进行匹配,以识别潜在的源区域并估计源项。我们比较了稀疏的、全球分布的IMS网络与紧凑的、瑞典本地的放射性氙阵列的定位能力。在这种特殊情况下,与完全使用IMS观测结果相比,阵列数据的使用不仅显著改善了源定位区域,而且有助于排除本地源。此外,133mXe与133Xe的活度比也被研究用于源表征,并发现与核反应堆循环的开始一致。
{"title":"Origin of an elevated radioxenon episode: A comparative study between the Swedish radioxenon array and the CTBT International Monitoring System","authors":"Sofie Liljegren ,&nbsp;J. Ole Ross ,&nbsp;Sofia Brander","doi":"10.1016/j.jenvrad.2025.107875","DOIUrl":"10.1016/j.jenvrad.2025.107875","url":null,"abstract":"<div><div>Between late November and early December 2022, large airborne activity concentrations of radioxenon were detected by multiple stations in the CTBT International Monitoring System (IMS) and the Swedish radioxenon array, which consisted of four operational radioxenon measurement units at the time. Over 100 samples containing <span><math><mrow><msup><mrow></mrow><mrow><mn>133</mn></mrow></msup><mtext>Xe</mtext></mrow></math></span> were recorded during this period, with <span><math><msup><mrow></mrow><mrow><mn>133</mn><mtext>m</mtext></mrow></msup></math></span>Xe found concurrently in about a dozen samples. The consistent <span><math><msup><mrow></mrow><mrow><mn>133</mn><mtext>m</mtext></mrow></msup></math></span>Xe to <span><math><mrow><msup><mrow></mrow><mrow><mn>133</mn></mrow></msup><mtext>Xe</mtext></mrow></math></span> activity ratio, and investigations with backward atmospheric transport models (ATM), suggests a sustained release of radioxenon from a single source for about two weeks. A grid of forward ATMs was computed, and model results were matched with observations to identify potential source regions and estimate the source term. We compare locating power of the sparse, globally distributed IMS network with the compact, local Swedish radioxenon array. In this specific case, the use of the array data both significantly improved the source localization area, and helped exclude local sources, when compared to exclusively using IMS observations. Additionally the <span><math><msup><mrow></mrow><mrow><mn>133</mn><mtext>m</mtext></mrow></msup></math></span>Xe to <span><math><mrow><msup><mrow></mrow><mrow><mn>133</mn></mrow></msup><mtext>Xe</mtext></mrow></math></span> activity ratio was investigated for source characterization, and was found to be consistent with the start of a nuclear reactor cycle.</div></div>","PeriodicalId":15667,"journal":{"name":"Journal of environmental radioactivity","volume":"292 ","pages":"Article 107875"},"PeriodicalIF":2.1,"publicationDate":"2025-12-17","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145781247","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Tritium baseline concentration and the origins of water and solute in precipitation elucidated from monthly data in Osaka, Japan 从日本大阪的月资料分析降水中氚基线浓度和水及溶质的来源
IF 2.1 3区 环境科学与生态学 Q3 ENVIRONMENTAL SCIENCES Pub Date : 2025-12-13 DOI: 10.1016/j.jenvrad.2025.107878
Chonlada Pitakchaianan , Kanyanan Kosinarkaranun , Pantiwa Kumsut , Ryuta Hazama , Anawat Rittirong , Koichi Sakakibara , Koki Kashiwaya , Yoshimune Ogata , Yuka Kato , Naofumi Akata , Wanwisa Sudprasert
This research aimed to establish current baseline level of tritium in precipitation in Osaka, Japan, and to investigate their seasonal behavior in relation to stable hydrogen and oxygen isotope compositions and major chemical components. Monthly precipitation samples were collected from January 2020 to December 2024 and tritium and stable isotope analyses were conducted with high analytical precision. The tritium concentration ranged from 0.19 ± 0.03 to 0.53 ± 0.05 Bq L−1 with a mean concentration of 0.32 ± 0.08 Bq L−1, showing a clear seasonal trend with higher concentrations in spring and lower in summer. The isotope ratios of δD and δ18O ranged from −91.98 to −16.95 ‰ and from −12.71 to −3.50 ‰, respectively, both following a similar seasonal pattern of higher values in spring and lower in summer. The d-excess value ranged from 2.0 to 30.2 ‰, exhibiting a clear seasonal trend of higher values in winter and lower in summer. The most common ions found in the rainwater were Cl, Na+, and Ca2+, with mean concentrations of 30.58 ± 33.86, 30.47 ± 32.88, and 27.80 ± 23.89 μeq L−1, respectively. The new findings of this study provide updated baseline data on tritium concentrations and stable hydrogen and oxygen isotope compositions in Osaka precipitation, establish Local Meteoric Water Lines (LMWLs) for the region, and offer important hydrological information for assessing the environmental impact of routine nuclear activities and potential accidental releases.
本研究旨在建立目前日本大阪降水中氚的基线水平,并研究其与稳定氢、氧同位素组成和主要化学成分的季节性行为。从2020年1月至2024年12月,每月采集降水样本,进行了高精度的氚和稳定同位素分析。氚浓度范围为0.19±0.03 ~ 0.53±0.05 Bq L−1,平均浓度为0.32±0.08 Bq L−1,具有明显的春季高、夏季低的季节变化趋势。δD和δ18O的同位素比值分别为- 91.98 ~ - 16.95‰和- 12.71 ~ - 3.50‰,具有春季高、夏季低的季节特征。d-excess值在2.0 ~ 30.2‰之间,呈明显的冬高夏低的季节变化趋势。雨水中最常见的离子是Cl−、Na+和Ca2+,平均浓度分别为30.58±33.86、30.47±32.88和27.80±23.89 μeq L−1。本研究的新发现提供了大阪降水中氚浓度和稳定氢、氧同位素组成的最新基线数据,为该地区建立了当地大气水线(LMWLs),并为评估常规核活动和潜在意外释放的环境影响提供了重要的水文信息。
{"title":"Tritium baseline concentration and the origins of water and solute in precipitation elucidated from monthly data in Osaka, Japan","authors":"Chonlada Pitakchaianan ,&nbsp;Kanyanan Kosinarkaranun ,&nbsp;Pantiwa Kumsut ,&nbsp;Ryuta Hazama ,&nbsp;Anawat Rittirong ,&nbsp;Koichi Sakakibara ,&nbsp;Koki Kashiwaya ,&nbsp;Yoshimune Ogata ,&nbsp;Yuka Kato ,&nbsp;Naofumi Akata ,&nbsp;Wanwisa Sudprasert","doi":"10.1016/j.jenvrad.2025.107878","DOIUrl":"10.1016/j.jenvrad.2025.107878","url":null,"abstract":"<div><div>This research aimed to establish current baseline level of tritium in precipitation in Osaka, Japan, and to investigate their seasonal behavior in relation to stable hydrogen and oxygen isotope compositions and major chemical components. Monthly precipitation samples were collected from January 2020 to December 2024 and tritium and stable isotope analyses were conducted with high analytical precision. The tritium concentration ranged from 0.19 ± 0.03 to 0.53 ± 0.05 Bq L<sup>−1</sup> with a mean concentration of 0.32 ± 0.08 Bq L<sup>−1</sup>, showing a clear seasonal trend with higher concentrations in spring and lower in summer. The isotope ratios of δD and δ<sup>18</sup>O ranged from −91.98 to −16.95 ‰ and from −12.71 to −3.50 ‰, respectively, both following a similar seasonal pattern of higher values in spring and lower in summer. The d-excess value ranged from 2.0 to 30.2 ‰, exhibiting a clear seasonal trend of higher values in winter and lower in summer. The most common ions found in the rainwater were Cl<sup>−</sup>, Na<sup>+</sup>, and Ca<sup>2+</sup>, with mean concentrations of 30.58 ± 33.86, 30.47 ± 32.88, and 27.80 ± 23.89 μeq L<sup>−1</sup>, respectively. The new findings of this study provide updated baseline data on tritium concentrations and stable hydrogen and oxygen isotope compositions in Osaka precipitation, establish Local Meteoric Water Lines (LMWLs) for the region, and offer important hydrological information for assessing the environmental impact of routine nuclear activities and potential accidental releases.</div></div>","PeriodicalId":15667,"journal":{"name":"Journal of environmental radioactivity","volume":"292 ","pages":"Article 107878"},"PeriodicalIF":2.1,"publicationDate":"2025-12-13","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145734196","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Evidence of Fukushima fallout in the area affected by wildfires in Kamaishi (Iwate Prefecture, Tohoku Region, Japan): Implications for future environmental research using radionuclide tracers 在釜石(日本东北地区岩手县)受野火影响地区的福岛沉降物证据:对未来使用放射性核素示踪剂进行环境研究的影响
IF 2.1 3区 环境科学与生态学 Q3 ENVIRONMENTAL SCIENCES Pub Date : 2025-12-11 DOI: 10.1016/j.jenvrad.2025.107876
Olivier Evrard , Naoya Takahashi , Hotaka Sato , Ryoga Ohta , Anthony Foucher , Thomas Chalaux-Clergue , Pierre-Alexis Chaboche
Significant deposition of radiocesium including 134Cs and 137Cs occurred in March 2011 following the Fukushima nuclear accident across vast regions of Northeastern Japan. However, as most studies focused on fallout that took place in the Fukushima Prefecture, much less information is available on the situation that prevails further to the North, in other parts of the Tohoku Region of Japan. In this context, the current research investigated the occurrence of fallout radionuclides (including natural 210Pbxs as well as artificial 134Cs and 137Cs) in burned and unburned soil profiles as well as in a range of surface soil and sediment samples collected in the region of Kamaishi (Iwate Prefecture, Tohoku Region, Japan) affected by wildfires in 2017. Results show that 210Pbxs and 137Cs may be used as tracers of sediment sources across landscapes affected by wildfires in this region. Furthermore, the soil profile analysis demonstrated that all analysed fallout radionuclides were found enriched in the burned vs. unburned profiles, due to the incorporation of radionuclides trapped by vegetation into the ash after the fire. The detection of 134Cs in the uppermost 0–5 cm depth layer in all investigated soil profiles also allowed to demonstrate the occurrence of significant Fukushima fallout of 134Cs and 137Cs in this region (roughly of the same order of magnitude as the fallout associated with the nuclear atmospheric tests in the 1960s). In the future, both sources of fallout should be considered to provide relevant interpretations when examining radionuclide data found in environmental samples collected in vast regions of Northeastern Japan. The analysis of 134Cs should also be encouraged to document the sources of fallout in these regions as long as this short-lived radionuclide remains detectable (i.e., theoretically by 2031).
2011年3月,在福岛核事故发生后,包括134Cs和137Cs在内的放射性铯在日本东北部的广大地区大量沉积。然而,由于大多数研究都集中在福岛县发生的放射性尘降物上,关于日本东北地区其他地区更北地区的情况的信息要少得多。在此背景下,本研究调查了2017年受野火影响的日本东北地区岩手县(Kamaishi)地区燃烧和未燃烧的土壤剖面以及一系列表层土壤和沉积物样本中放射性沉降核素(包括天然210Pbxs以及人工134Cs和137Cs)的发生情况。结果表明,210Pbxs和137Cs可以作为该地区野火影响景观中沉积物源的示踪剂。此外,土壤剖面分析表明,所有分析的沉降物放射性核素在燃烧剖面和未燃烧剖面中都被发现富集,这是由于火灾后植被捕获的放射性核素混入了灰烬中。在所有调查的土壤剖面的最上层0-5厘米深度层中检测到134Cs,也证明在该地区发生了大量的134Cs和137Cs的福岛沉降物(大致与20世纪60年代大气核试验相关沉降物的数量级相同)。今后,在检查在日本东北部广大地区收集的环境样本中发现的放射性核素数据时,应考虑这两种沉降物来源,以提供相关的解释。还应鼓励对134Cs的分析,以记录这些地区的沉降物来源,只要这种短寿命的放射性核素仍然可检测到(即理论上到2031年)。
{"title":"Evidence of Fukushima fallout in the area affected by wildfires in Kamaishi (Iwate Prefecture, Tohoku Region, Japan): Implications for future environmental research using radionuclide tracers","authors":"Olivier Evrard ,&nbsp;Naoya Takahashi ,&nbsp;Hotaka Sato ,&nbsp;Ryoga Ohta ,&nbsp;Anthony Foucher ,&nbsp;Thomas Chalaux-Clergue ,&nbsp;Pierre-Alexis Chaboche","doi":"10.1016/j.jenvrad.2025.107876","DOIUrl":"10.1016/j.jenvrad.2025.107876","url":null,"abstract":"<div><div>Significant deposition of radiocesium including <sup>134</sup>Cs and <sup>137</sup>Cs occurred in March 2011 following the Fukushima nuclear accident across vast regions of Northeastern Japan. However, as most studies focused on fallout that took place in the Fukushima Prefecture, much less information is available on the situation that prevails further to the North, in other parts of the Tohoku Region of Japan. In this context, the current research investigated the occurrence of fallout radionuclides (including natural <sup>210</sup>Pb<sub>xs</sub> as well as artificial <sup>134</sup>Cs and <sup>137</sup>Cs) in burned and unburned soil profiles as well as in a range of surface soil and sediment samples collected in the region of Kamaishi (Iwate Prefecture, Tohoku Region, Japan) affected by wildfires in 2017. Results show that <sup>210</sup>Pb<sub>xs</sub> and <sup>137</sup>Cs may be used as tracers of sediment sources across landscapes affected by wildfires in this region. Furthermore, the soil profile analysis demonstrated that all analysed fallout radionuclides were found enriched in the burned vs. unburned profiles, due to the incorporation of radionuclides trapped by vegetation into the ash after the fire. The detection of <sup>134</sup>Cs in the uppermost 0–5 cm depth layer in all investigated soil profiles also allowed to demonstrate the occurrence of significant Fukushima fallout of <sup>134</sup>Cs and <sup>137</sup>Cs in this region (roughly of the same order of magnitude as the fallout associated with the nuclear atmospheric tests in the 1960s). In the future, both sources of fallout should be considered to provide relevant interpretations when examining radionuclide data found in environmental samples collected in vast regions of Northeastern Japan. The analysis of <sup>134</sup>Cs should also be encouraged to document the sources of fallout in these regions as long as this short-lived radionuclide remains detectable (i.e., theoretically by 2031).</div></div>","PeriodicalId":15667,"journal":{"name":"Journal of environmental radioactivity","volume":"292 ","pages":"Article 107876"},"PeriodicalIF":2.1,"publicationDate":"2025-12-11","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145734195","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Spatiotemporal variations and environmental behavior of activity concentrations of natural and artificial radionuclides in soils of Fukuoka, Japan (1980–2019) 1980-2019年日本福冈地区土壤天然和人工放射性核素活性浓度时空变化及环境行为
IF 2.1 3区 环境科学与生态学 Q3 ENVIRONMENTAL SCIENCES Pub Date : 2025-12-11 DOI: 10.1016/j.jenvrad.2025.107828
Yukinori Narazaki , Akihiro Sakoda , Yoichi Ishikawa , Junji Yamanaka , Toshiya Tamari , Naofumi Akata , Noriyuki Momoshima
The distribution of ambient radiation dose rates and radionuclide activity concentrations in soil was clarified over a wide area of Fukuoka Prefecture, located in western Japan, as of 2019. Locations with ambient radiation dose rates exceeding 100 nGy/h were identified. In areas with high ambient radiation dose rates, elevated activity concentrations of natural radionuclides (40K, 226Ra, and 232Th) were observed. The activity concentration of 90Sr in surface soil (0–5 cm) ranged from 0.15 to 2.0 Bq/kg dw, and 137Cs activity concentrations ranged from ND to 8.4 Bq/kg dw. 238Pu was not detected. The activity concentration of 239+240Pu ranged from 0.014 to 0.36 Bq/kg dw.
In a long-term, depth-specific study at fixed point, the eluviation rates of 90Sr, 137Cs, and 239+240Pu in surface soil were 1.6 %, 8.4 %, and 6.5 % per year, respectively. These tendencies differed significantly from previously reported migration rates. Additionally, in some cases, the activity concentration of 137Cs in the surface soil was lower than that of 90Sr, and 137Cs was no longer detected in the subsurface soil (5–20 cm). These observations are thought to result from the movement of surface soil due to weathering, erosion, and surface runoff, or the exposure of subsurface soil.
90Sr and 239+240Pu in the soil primarily originated from past atmospheric nuclear tests. On the other hand, 137Cs showed additional influence from the Chernobyl nuclear power plant accident. No contributions of 90Sr, 137Cs, or 239+240Pu to Fukuoka Prefecture's soil from the Fukushima Daiichi nuclear power plant accident were observed.
截至2019年,在日本西部福冈县的广大地区,环境辐射剂量率和土壤中放射性核素活性浓度的分布得到了澄清。确定了环境辐射剂量率超过100毫希/小时的地点。在环境辐射剂量率高的地区,观察到天然放射性核素(40K、226Ra和232Th)的活性浓度升高。土壤表层(0 ~ 5 cm) 90Sr活性浓度为0.15 ~ 2.0 Bq/kg dw, 137Cs活性浓度为ND ~ 8.4 Bq/kg dw。238未检测到pu。239+240Pu的活性浓度为0.014 ~ 0.36 Bq/kg dw。在定点的长期深度研究中,表层土壤90Sr、137Cs和239+240Pu的年淋失率分别为1.6%、8.4%和6.5%。这些趋势与以前报告的移徙率有很大不同。此外,在某些情况下,表层土壤中137Cs的活性浓度低于90Sr,在5-20 cm的地下土壤中不再检测到137Cs。这些观测结果被认为是由于风化、侵蚀和地表径流引起的地表土壤运动或地下土壤暴露造成的。土壤中的90Sr和239+240Pu主要来自过去的大气核试验。另一方面,137Cs受到切尔诺贝利核电站事故的额外影响。从福岛第一核电站事故中未观察到90Sr、137Cs或239+240Pu对福冈县土壤的贡献。
{"title":"Spatiotemporal variations and environmental behavior of activity concentrations of natural and artificial radionuclides in soils of Fukuoka, Japan (1980–2019)","authors":"Yukinori Narazaki ,&nbsp;Akihiro Sakoda ,&nbsp;Yoichi Ishikawa ,&nbsp;Junji Yamanaka ,&nbsp;Toshiya Tamari ,&nbsp;Naofumi Akata ,&nbsp;Noriyuki Momoshima","doi":"10.1016/j.jenvrad.2025.107828","DOIUrl":"10.1016/j.jenvrad.2025.107828","url":null,"abstract":"<div><div>The distribution of ambient radiation dose rates and radionuclide activity concentrations in soil was clarified over a wide area of Fukuoka Prefecture, located in western Japan, as of 2019. Locations with ambient radiation dose rates exceeding 100 nGy/h were identified. In areas with high ambient radiation dose rates, elevated activity concentrations of natural radionuclides (<sup>40</sup>K, <sup>226</sup>Ra, and <sup>232</sup>Th) were observed. The activity concentration of <sup>90</sup>Sr in surface soil (0–5 cm) ranged from 0.15 to 2.0 Bq/kg dw, and <sup>137</sup>Cs activity concentrations ranged from ND to 8.4 Bq/kg dw. <sup>238</sup>Pu was not detected. The activity concentration of <sup>239+240</sup>Pu ranged from 0.014 to 0.36 Bq/kg dw.</div><div>In a long-term, depth-specific study at fixed point, the eluviation rates of <sup>90</sup>Sr, <sup>137</sup>Cs, and <sup>239+240</sup>Pu in surface soil were 1.6 %, 8.4 %, and 6.5 % per year, respectively. These tendencies differed significantly from previously reported migration rates. Additionally, in some cases, the activity concentration of <sup>137</sup>Cs in the surface soil was lower than that of <sup>90</sup>Sr, and <sup>137</sup>Cs was no longer detected in the subsurface soil (5–20 cm). These observations are thought to result from the movement of surface soil due to weathering, erosion, and surface runoff, or the exposure of subsurface soil.</div><div><sup>90</sup>Sr and <sup>239+240</sup>Pu in the soil primarily originated from past atmospheric nuclear tests. On the other hand, <sup>137</sup>Cs showed additional influence from the Chernobyl nuclear power plant accident. No contributions of <sup>90</sup>Sr, <sup>137</sup>Cs, or <sup>239+240</sup>Pu to Fukuoka Prefecture's soil from the Fukushima Daiichi nuclear power plant accident were observed.</div></div>","PeriodicalId":15667,"journal":{"name":"Journal of environmental radioactivity","volume":"292 ","pages":"Article 107828"},"PeriodicalIF":2.1,"publicationDate":"2025-12-11","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145734197","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Assessment of radon and carrier gases in an underground gold mining company in Ghana 加纳地下金矿公司氡和载气的评估。
IF 2.1 3区 环境科学与生态学 Q3 ENVIRONMENTAL SCIENCES Pub Date : 2025-12-02 DOI: 10.1016/j.jenvrad.2025.107851
Rita kpordzro , Francis Otoo , Oscar K. Adukpo , Eric T. Glover , Anthony S.K. Amable
Previous studies in Ghanaian mines have largely focused on radon concentration and associated health risk, with limited investigation into the role of carrier gases that influence radon transport from bedrock. This study evaluates radon (222Rn) levels, carrier gases (CO2, H2S, CH4), and their associated health risks in an underground section of the AngloGold Ashanti mine. Measurements were conducted in two phases using CR-39 solid-state nuclear track detectors and a Ventis Pro5 multi-gas detector. The average radon concentration across both phases was 214 ± 16 Bq·m−3, with phase-specific means of 245 ± 8 Bq·m−3 and 184 ± 6 Bq·m−3. Based on ICRP 137, the annual effective dose and excess lifetime cancer risk were estimated at 0.6 ± 0.2 mSv y−1 and 1.5 × 10−3 per million persons/year, respectively, both below ICRP and NCRP safety limits. Concentrations of all carrier gases remained within OSHA and Chart Industries recommended exposure limits. Principal component analysis indicated that methane and hydrogen sulfide significantly influence radon distribution with Eigenvalue >1, Overall, the findings suggest that the current levels of radon and carrier gases in the mine do not pose significant health risks to underground workers.
以前对加纳矿山的研究主要集中在氡浓度和相关的健康风险上,对影响基岩氡输送的载气的作用进行了有限的调查。本研究评估了AngloGold Ashanti矿井地下部分的氡(222Rn)水平、载气(CO2、H2S、CH4)及其相关健康风险。使用CR-39固体核径迹探测器和Ventis Pro5多气体探测器分两阶段进行测量。两相平均氡浓度分别为214±16 Bq·m-3和184±6 Bq·m-3。根据ICRP 137,估计年有效剂量和超额终身癌症风险分别为0.6±0.2 mSv -1和1.5 × 10-3 /百万人/年,均低于ICRP和NCRP的安全限值。所有载气浓度保持在OSHA和Chart Industries推荐的暴露限值之内。主成分分析表明,甲烷和硫化氢显著影响氡分布,特征值为>1。总体而言,研究结果表明,矿井中目前的氡和载气水平不会对井下工人构成重大健康风险。
{"title":"Assessment of radon and carrier gases in an underground gold mining company in Ghana","authors":"Rita kpordzro ,&nbsp;Francis Otoo ,&nbsp;Oscar K. Adukpo ,&nbsp;Eric T. Glover ,&nbsp;Anthony S.K. Amable","doi":"10.1016/j.jenvrad.2025.107851","DOIUrl":"10.1016/j.jenvrad.2025.107851","url":null,"abstract":"<div><div>Previous studies in Ghanaian mines have largely focused on radon concentration and associated health risk, with limited investigation into the role of carrier gases that influence radon transport from bedrock. This study evaluates radon (<sup>222</sup>Rn) levels, carrier gases (CO<sub>2</sub>, H<sub>2</sub>S, CH<sub>4</sub>), and their associated health risks in an underground section of the AngloGold Ashanti mine. Measurements were conducted in two phases using CR-39 solid-state nuclear track detectors and a Ventis Pro5 multi-gas detector. The average radon concentration across both phases was 214 ± 16 Bq·m<sup>−3</sup>, with phase-specific means of 245 ± 8 Bq·m<sup>−3</sup> and 184 ± 6 Bq·m<sup>−3</sup>. Based on ICRP 137, the annual effective dose and excess lifetime cancer risk were estimated at 0.6 ± 0.2 mSv y<sup>−1</sup> and 1.5 × 10<sup>−3</sup> per million persons/year, respectively, both below ICRP and NCRP safety limits. Concentrations of all carrier gases remained within OSHA and Chart Industries recommended exposure limits. Principal component analysis indicated that methane and hydrogen sulfide significantly influence radon distribution with Eigenvalue &gt;1, Overall, the findings suggest that the current levels of radon and carrier gases in the mine do not pose significant health risks to underground workers.</div></div>","PeriodicalId":15667,"journal":{"name":"Journal of environmental radioactivity","volume":"292 ","pages":"Article 107851"},"PeriodicalIF":2.1,"publicationDate":"2025-12-02","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145668633","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Downscaled simulation approach for near-field nuclear facility pollutant atmospheric transport and dispersion using a coupled WRF–CFD downscaling model framework 基于耦合WRF-CFD模型框架的核设施近场污染物大气输送和扩散降尺度模拟方法
IF 2.1 3区 环境科学与生态学 Q3 ENVIRONMENTAL SCIENCES Pub Date : 2025-12-01 DOI: 10.1016/j.jenvrad.2025.107864
Zhengming Li , Yongjun Ye , Xinyu Liu , Zhongkun Wang
Nuclear facilities can release radioactive pollutants into the atmosphere during daily operations and accidents. These pollutants are transported and dispersed through atmospheric processes, eventually depositing on the surface and posing potential risks to ecosystems and public health. Accurately describing their atmospheric dispersion is therefore essential for scientific assessments of radioactive impact. In this study, a one-way downscaling model framework of atmospheric dispersion of pollutants was developed, which coupled the mesoscale Weather Research and Forecasting (WRF) model with a microscale computational fluid dynamics (CFD) model. To enhance the microscale model and make it inherit the flow field characteristics of the mesoscale model, closure constants of the microscale turbulence model were adjusted according to the planetary boundary layer scheme in the mesoscale model. The simulation performance of the WRF-CFD downscaling model framework and its adjusted model was evaluated by meteorological observations and an SF6 tracer experiment conducted in Fuqing Nuclear Power Plant. The results demonstrated that WRF reasonably reproduced the mesoscale wind field and provided reliable inflow conditions for the CFD simulations. The coupled WRF-CFD downscaling model had high accuracy and reliability in reproducing wind profiles and concentration field distributions, while the adjustment strategy for turbulence model closure constants could effectively enhance the simulation performance of the downscaling model. Although wind shear-induced plume swing introduced spatial deviations between the simulation results based on steady RANS and the measured values in far-field regions, the model still captured peak concentration magnitudes comparable to measurements. Overall, the proposed downscaling strategy enabled reliable high-resolution simulations of pollutant transport and dispersion in the near-field atmosphere of nuclear facilities. The turbulence constant adjustment improved model performance, while limitations remain in steady-state RANS for resolving plume swing. Future work is needed to explore transient approaches to better capture shear-induced plume variability. This study provided a new approach for the detailed investigation of pollutant transport and dispersion in the real atmospheric environment, as well as a practical and scientifically robust tool for environmental impact assessment and emergency preparedness in nuclear facility management.
核设施在日常运行和事故中会向大气中释放放射性污染物。这些污染物通过大气过程运输和扩散,最终沉积在地表,对生态系统和公众健康构成潜在风险。因此,准确描述它们在大气中的扩散对放射性影响的科学评估至关重要。本文建立了大气污染物扩散的单向降尺度模式框架,该框架将中尺度天气研究与预报(WRF)模式与微尺度计算流体动力学(CFD)模式耦合在一起。为了增强微尺度模式并使其继承中尺度模式的流场特征,根据中尺度模式中的行星边界层格式对微尺度湍流模式的闭合常数进行了调整。通过福清核电站的气象观测和SF6示踪剂实验,对WRF-CFD降尺度模型框架及其调整模型的模拟性能进行了评价。结果表明,WRF能较好地再现中尺度风场,为CFD模拟提供了可靠的入流条件。耦合WRF-CFD降尺度模型在再现风廓线和浓度场分布方面具有较高的精度和可靠性,而湍流模型闭合常数的调整策略可以有效地提高降尺度模型的模拟性能。尽管风切变引起的羽流摆动导致基于稳定RANS的模拟结果与远场区域的实测值之间存在空间偏差,但该模型仍然捕获了与实测值相当的峰值浓度量级。总体而言,所提出的降尺度策略能够对核设施近场大气中的污染物输送和扩散进行可靠的高分辨率模拟。湍流常数调整提高了模型的性能,但稳态RANS在解决羽流摆动方面仍然存在局限性。未来的工作需要探索瞬态方法,以更好地捕捉剪切引起的羽流变化。该研究为深入研究污染物在真实大气环境中的运移和扩散提供了新的途径,也为核设施管理中的环境影响评价和应急准备提供了实用、科学、可靠的工具。
{"title":"Downscaled simulation approach for near-field nuclear facility pollutant atmospheric transport and dispersion using a coupled WRF–CFD downscaling model framework","authors":"Zhengming Li ,&nbsp;Yongjun Ye ,&nbsp;Xinyu Liu ,&nbsp;Zhongkun Wang","doi":"10.1016/j.jenvrad.2025.107864","DOIUrl":"10.1016/j.jenvrad.2025.107864","url":null,"abstract":"<div><div>Nuclear facilities can release radioactive pollutants into the atmosphere during daily operations and accidents. These pollutants are transported and dispersed through atmospheric processes, eventually depositing on the surface and posing potential risks to ecosystems and public health. Accurately describing their atmospheric dispersion is therefore essential for scientific assessments of radioactive impact. In this study, a one-way downscaling model framework of atmospheric dispersion of pollutants was developed, which coupled the mesoscale Weather Research and Forecasting (WRF) model with a microscale computational fluid dynamics (CFD) model. To enhance the microscale model and make it inherit the flow field characteristics of the mesoscale model, closure constants of the microscale turbulence model were adjusted according to the planetary boundary layer scheme in the mesoscale model. The simulation performance of the WRF-CFD downscaling model framework and its adjusted model was evaluated by meteorological observations and an SF<sub>6</sub> tracer experiment conducted in Fuqing Nuclear Power Plant. The results demonstrated that WRF reasonably reproduced the mesoscale wind field and provided reliable inflow conditions for the CFD simulations. The coupled WRF-CFD downscaling model had high accuracy and reliability in reproducing wind profiles and concentration field distributions, while the adjustment strategy for turbulence model closure constants could effectively enhance the simulation performance of the downscaling model. Although wind shear-induced plume swing introduced spatial deviations between the simulation results based on steady RANS and the measured values in far-field regions, the model still captured peak concentration magnitudes comparable to measurements. Overall, the proposed downscaling strategy enabled reliable high-resolution simulations of pollutant transport and dispersion in the near-field atmosphere of nuclear facilities. The turbulence constant adjustment improved model performance, while limitations remain in steady-state RANS for resolving plume swing. Future work is needed to explore transient approaches to better capture shear-induced plume variability. This study provided a new approach for the detailed investigation of pollutant transport and dispersion in the real atmospheric environment, as well as a practical and scientifically robust tool for environmental impact assessment and emergency preparedness in nuclear facility management.</div></div>","PeriodicalId":15667,"journal":{"name":"Journal of environmental radioactivity","volume":"292 ","pages":"Article 107864"},"PeriodicalIF":2.1,"publicationDate":"2025-12-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145623202","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Uranium and thorium levels in urine and hair of coal miners and local residents in Shanxi, China 中国山西煤矿工人和当地居民尿液和头发中的铀和钍含量。
IF 2.1 3区 环境科学与生态学 Q3 ENVIRONMENTAL SCIENCES Pub Date : 2025-11-30 DOI: 10.1016/j.jenvrad.2025.107861
Yuhan Xie , Yuxin Qian , Yao Zhang , Liangliang Yin , Ning Guo , Yanqin Ji
Uranium and thorium are naturally occurring radionuclides that may pose health risks when released into the environment through coal mining activities. This study aimed to investigate the levels of uranium and thorium exposure among coal miners and nearby residents in Shanxi, China. Urine and hair samples were collected from 51 participants, including 30 coal miners and 21 nearby residents. The concentrations of uranium and thorium were measured using inductively coupled plasma mass spectrometer. Subgroup analysis was performed to investigate the effects of environmental and occupational factors. Both urine and hair samples showed uranium and thorium concentrations higher than typical baseline values, indicating environmental and occupational exposure. Uranium levels in urine were notably higher in coal miners, especially among those with shorter work duration, suggesting recent or ongoing exposure. Thorium concentrations displayed limited variability and did not significantly differ between miners and residents. Uranium exposure appears to be closely linked to mining operations and environmental contamination in the region, whereas thorium exposure remains relatively uniform across groups. These findings underscore the need for further investigation into the long-term health effects of uranium and thorium exposure in coal mining areas and call for targeted interventions to reduce exposure risks.
铀和钍是天然存在的放射性核素,如果通过煤矿开采活动释放到环境中,可能对健康构成威胁。本研究旨在调查中国山西煤矿工人和附近居民的铀和钍暴露水平。研究人员收集了51名参与者的尿液和毛发样本,其中包括30名煤矿工人和21名附近居民。用电感耦合等离子体质谱仪测定了铀和钍的浓度。采用亚组分析探讨环境和职业因素的影响。尿液和头发样本显示铀和钍浓度高于典型基线值,表明环境和职业暴露。煤矿工人尿液中的铀含量明显较高,尤其是那些工作时间较短的矿工,这表明他们最近或正在接触铀。钍浓度表现出有限的可变性,在矿工和居民之间没有显著差异。铀暴露似乎与该区域的采矿作业和环境污染密切相关,而钍暴露在各群体之间仍然相对一致。这些发现强调需要进一步调查煤矿地区铀和钍暴露对健康的长期影响,并呼吁采取有针对性的干预措施以减少暴露风险。
{"title":"Uranium and thorium levels in urine and hair of coal miners and local residents in Shanxi, China","authors":"Yuhan Xie ,&nbsp;Yuxin Qian ,&nbsp;Yao Zhang ,&nbsp;Liangliang Yin ,&nbsp;Ning Guo ,&nbsp;Yanqin Ji","doi":"10.1016/j.jenvrad.2025.107861","DOIUrl":"10.1016/j.jenvrad.2025.107861","url":null,"abstract":"<div><div>Uranium and thorium are naturally occurring radionuclides that may pose health risks when released into the environment through coal mining activities. This study aimed to investigate the levels of uranium and thorium exposure among coal miners and nearby residents in Shanxi, China. Urine and hair samples were collected from 51 participants, including 30 coal miners and 21 nearby residents. The concentrations of uranium and thorium were measured using inductively coupled plasma mass spectrometer. Subgroup analysis was performed to investigate the effects of environmental and occupational factors. Both urine and hair samples showed uranium and thorium concentrations higher than typical baseline values, indicating environmental and occupational exposure. Uranium levels in urine were notably higher in coal miners, especially among those with shorter work duration, suggesting recent or ongoing exposure. Thorium concentrations displayed limited variability and did not significantly differ between miners and residents. Uranium exposure appears to be closely linked to mining operations and environmental contamination in the region, whereas thorium exposure remains relatively uniform across groups. These findings underscore the need for further investigation into the long-term health effects of uranium and thorium exposure in coal mining areas and call for targeted interventions to reduce exposure risks.</div></div>","PeriodicalId":15667,"journal":{"name":"Journal of environmental radioactivity","volume":"291 ","pages":"Article 107861"},"PeriodicalIF":2.1,"publicationDate":"2025-11-30","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145654631","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
期刊
Journal of environmental radioactivity
全部 Acc. Chem. Res. ACS Applied Bio Materials ACS Appl. Electron. Mater. ACS Appl. Energy Mater. ACS Appl. Mater. Interfaces ACS Appl. Nano Mater. ACS Appl. Polym. Mater. ACS BIOMATER-SCI ENG ACS Catal. ACS Cent. Sci. ACS Chem. Biol. ACS Chemical Health & Safety ACS Chem. Neurosci. ACS Comb. Sci. ACS Earth Space Chem. ACS Energy Lett. ACS Infect. Dis. ACS Macro Lett. ACS Mater. Lett. ACS Med. Chem. Lett. ACS Nano ACS Omega ACS Photonics ACS Sens. ACS Sustainable Chem. Eng. ACS Synth. Biol. Anal. Chem. BIOCHEMISTRY-US Bioconjugate Chem. BIOMACROMOLECULES Chem. Res. Toxicol. Chem. Rev. Chem. Mater. CRYST GROWTH DES ENERG FUEL Environ. Sci. Technol. Environ. Sci. Technol. Lett. Eur. J. Inorg. Chem. IND ENG CHEM RES Inorg. Chem. J. Agric. Food. Chem. J. Chem. Eng. Data J. Chem. Educ. J. Chem. Inf. Model. J. Chem. Theory Comput. J. Med. Chem. J. Nat. Prod. J PROTEOME RES J. Am. Chem. Soc. LANGMUIR MACROMOLECULES Mol. Pharmaceutics Nano Lett. Org. Lett. ORG PROCESS RES DEV ORGANOMETALLICS J. Org. Chem. J. Phys. Chem. J. Phys. Chem. A J. Phys. Chem. B J. Phys. Chem. C J. Phys. Chem. Lett. Analyst Anal. Methods Biomater. Sci. Catal. Sci. Technol. Chem. Commun. Chem. Soc. Rev. CHEM EDUC RES PRACT CRYSTENGCOMM Dalton Trans. Energy Environ. Sci. ENVIRON SCI-NANO ENVIRON SCI-PROC IMP ENVIRON SCI-WAT RES Faraday Discuss. Food Funct. Green Chem. Inorg. Chem. Front. Integr. Biol. J. Anal. At. Spectrom. J. Mater. Chem. A J. Mater. Chem. B J. Mater. Chem. C Lab Chip Mater. Chem. Front. Mater. Horiz. MEDCHEMCOMM Metallomics Mol. Biosyst. Mol. Syst. Des. Eng. Nanoscale Nanoscale Horiz. Nat. Prod. Rep. New J. Chem. Org. Biomol. Chem. Org. Chem. Front. PHOTOCH PHOTOBIO SCI PCCP Polym. Chem.
×
引用
GB/T 7714-2015
复制
MLA
复制
APA
复制
导出至
BibTeX EndNote RefMan NoteFirst NoteExpress
×
0
微信
客服QQ
Book学术公众号 扫码关注我们
反馈
×
意见反馈
请填写您的意见或建议
请填写您的手机或邮箱
×
提示
您的信息不完整,为了账户安全,请先补充。
现在去补充
×
提示
您因"违规操作"
具体请查看互助需知
我知道了
×
提示
现在去查看 取消
×
提示
确定
Book学术官方微信
Book学术文献互助
Book学术文献互助群
群 号:604180095
Book学术
文献互助 智能选刊 最新文献 互助须知 联系我们:info@booksci.cn
Book学术提供免费学术资源搜索服务,方便国内外学者检索中英文文献。致力于提供最便捷和优质的服务体验。
Copyright © 2023 Book学术 All rights reserved.
ghs 京公网安备 11010802042870号 京ICP备2023020795号-1