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Theoretical Investigation of α-decay Chains of Fm-isotopes fm同位素α-衰变链的理论研究
Pub Date : 2022-06-20 DOI: 10.15415/jnp.2022.92020
T. M. Joshua, Shilpa Rana, N. Jain, M. Bhuyan, K. Anwar, Raj Kumar, N. Abdullah
Background: The theoretical and experimental investigations of decay properties of heavy and superheavy nuclei are crucial to explore the nuclear structure and reaction dynamics. Purpose: The aim of this study is to probe the α-decay properties of 243Fm and 245Fm isotopic chains using relativistic mean-field (RMF) approach within the framework of preformed cluster-decay model (PCM). Methods: The RMF densities are folded with the relativistic R3Y NN potential to deduce the nuclear interaction potential between the α particle and daughter nucleus. The penetration probability is calculated within the WKB approximation. Results: The α-decay half-lives of even-odd 243Fm and 245Fm isotopes and their daughter nuclei are obtained from the preformed cluster-decay model. These theoretically calculated half-lives are found to be in good agreement with the recent experimental measurements. Conclusions: The novel result here is the applicability of the scaling factor within the PCM as a signature for shell/sub-shell closures in α-decay studies. As such, we have also demonstrated that N=137, 139 and Z=94 corresponding to 231,233Pu could be shell/sub-shell closures. The least T1/2 is found at 243,245Fm which indicate their individual stability and α-decay as their most probable decay mode.
背景:重核和超重核衰变性质的理论和实验研究对于探索核结构和反应动力学至关重要。目的:在预成形簇衰变模型(PCM)框架下,利用相对论平均场(RMF)方法研究243Fm和245Fm同位素链的α-衰变特性。方法:将RMF密度与相对论性R3Y NN势进行折叠,推导出α粒子与子核之间的核相互作用势。在WKB近似范围内计算侵彻概率。结果:通过预形成的团簇衰变模型,得到了243Fm和245Fm的偶奇同位素及其子核的α-衰变半衰期。这些理论计算的半衰期与最近的实验测量结果非常吻合。结论:这里的新结果是PCM内的比例因子作为α-衰变研究中壳/子壳闭合的标志的适用性。因此,我们也证明了231,233Pu对应的N=137, 139和Z=94可能是壳层/子壳层闭包。在243,245Fm处发现最小的T1/2,这表明它们的个体稳定性和α-衰变是它们最可能的衰变模式。
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引用次数: 1
Evaluation of Natural Radioactivity Levels and Exhalation rate of 222Rn and 220Rn in the Soil Samples from the Kuthiran Hills, Kerala, India 印度喀拉拉邦Kuthiran山土壤样品中222Rn和220Rn天然放射性水平及呼出率的评价
Pub Date : 2022-06-20 DOI: 10.15415/jnp.2022.92034
V. C V, Antony Joseph
Background: Exposure to radon and its decay products is one of the important contributors of radiation doses to human population. Radon exhalation study is important for understanding the contribution of the soil towards the total radioactivity concentration found inside the dwellings. Purpose: The aim of the present study is to investigate the radioactivity levels and radium and radon exhalation rates in soil samples collected from Kuthiran hills and nearby places in Thrissur district, Kerala state, India. On the basis of this data, radiological health hazard parameters are also evaluated. Methods: About 18 soil samples were collected from the study location. The radium, thorium and potassium activity concentrations were analyzed by HPGe gamma ray spectrometer. The “can technique” using LR-115 type II plastic track detectors have been used for the measurement of radon exhalation rate in soil samples. Results: The mean values of activity concentrations of 226Ra, 232Th and 40K were 64.60 Bqkg-1, 109.03 Bqkg-1and 972.67 Bqkg-1 respectively. The mean value of radon mass exhalation rate is 9.19 mBqkg-1h-1 and thoron surface exhalation rate is and 237.9 mBqm-2s-1. The radium equivalent activity concentration of all the soil samples was below the level of 370 Bqkg-1, recommended for building materials, by OECD 1979 (Organization for Economic Cooperation and Development). Conclusions: The results show that the study area is safe, as far as the health hazard effects of radium and radon exhalation rate are concerned. This data will be helpful in establishing new regulations and safety limits, related to the radiation dose and radon activity in Kuthiran hills.
背景:氡及其衰变产物的暴露是人类辐射剂量的重要来源之一。氡呼出研究对于了解土壤对住宅内总放射性浓度的贡献具有重要意义。目的:本研究的目的是调查在印度喀拉拉邦特里苏苏尔地区库蒂兰丘陵和附近地区收集的土壤样品的放射性水平和镭和氡的呼出率。在此基础上,还对放射性健康危害参数进行了评价。方法:在研究地点采集土壤样品18份。用HPGe能谱仪分析了镭、钍和钾的活性浓度。采用“can技术”,利用LR-115型II型塑料径迹检测器对土壤样品中的氡析出率进行了测量。结果:226Ra、232Th和40K活性浓度平均值分别为64.60 Bqkg-1、109.03 Bqkg-1和972.67 Bqkg-1。氡质量呼出率均值为9.19 mBqkg-1h-1,氡表面呼出率均值为237.9 mBqm-2s-1。所有土壤样品的镭当量活度浓度均低于经济合作与发展组织1979年为建筑材料建议的370 Bqkg-1水平。结论:从氡和镭对健康的危害效应来看,研究区是安全的。这些数据将有助于制定与库蒂兰山的辐射剂量和氡活度有关的新条例和安全限制。
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引用次数: 0
Charge Radius And Neutron Skin Thickness Of Platinum And Osmium Isotopes Near The Nuclear Drip Lines 核滴注线附近铂和锇同位素的电荷半径和中子皮厚
Pub Date : 2022-06-20 DOI: 10.15415/jnp.2022.92027
Anjana A V, Nicemon Thomas, A. Joseph
Background: The density distributions of exotic nuclei are different from that of stable nuclei. For stable nuclei, charge radii can be obtained through electron scattering experiments. The excessive neutrons in neutron-rich nuclei make a decoupling of neutron and proton distribution and as a result nuclear skin structures are appeared.Purpose: The charge radius and the way by which nucleons are distributed can provide information about size, surface thickness and shell structure of nuclei. The information collected from such nuclei can be used for astrophysical studies to understand the origin of heavy elements.Methods: In the present study, we have made an attempt to investigate the charge radii, rms radii and skin thickness of Pt and Os isotopes. Here, the calculations were made by using the HFB solver which utilizes HO single-particle basis and iteratively diagonalizes the HFB Hamiltonian based on the Skyrme forces.Results: Here we can observe an increase in charge radius, rms radius and skin thickness with neutron number. The charge radii calculated are in good agreement with the experimental data and predictions of RCHB model. A linear dependence of skin thickness on neutron number is observed with the change in slope is noticed around N =126.Conclusion: Using HFB theory, we have analyzed the charge radius and neutron skin thickness of Pt and Os isotopes. The drip line nuclei have larger charge radius in comparison to the stable nuclei. The redistribution of the nucleons due to addition of neutrons leads to the gradual increase in neutron skin. The sudden increase of skin thickness may be due to the extra stability and shell closure around the magic number.
背景:外来核的密度分布不同于稳定核。对于稳定原子核,电荷半径可以通过电子散射实验得到。富中子核中过多的中子使中子和质子的分布发生解耦,从而出现核表皮结构。目的:电荷半径和核子的分布方式可以提供原子核的大小、表面厚度和壳层结构的信息。从这些核中收集的信息可以用于天体物理学研究,以了解重元素的起源。方法:在本研究中,我们尝试研究了Pt和Os同位素的电荷半径、均方根半径和趋肤厚度。在这里,使用HFB求解器进行计算,该求解器利用HO单粒子基,并基于Skyrme力迭代对角化HFB哈密顿量。结果:随着中子数的增加,电荷半径、均方根半径和镀层厚度均有所增加。计算的电荷半径与实验数据和RCHB模型的预测结果吻合较好。观察到蒙皮厚度与中子数呈线性关系,在N =126附近出现斜率变化。结论:利用HFB理论分析了Pt和Os同位素的电荷半径和中子蒙皮厚度。与稳定原子核相比,滴线原子核的电荷半径更大。中子的加入使核子重新分布,使中子表皮逐渐增大。皮肤厚度的突然增加可能是由于额外的稳定性和壳闭合在魔术数周围。
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引用次数: 0
Radii of Thorium Nuclides Lying in Between the Drip Lines 滴油管之间钍核素的半径
Pub Date : 2022-06-20 DOI: 10.15415/jnp.2022.92031
U. E, Prof Antony Joseph
Background: Nuclear rms radii give information about the nuclear structure, nuclear shape, deformation etc. Microscopic methods are widely used for the study of nuclear structure properties. Hartree-Fock method with an effective interaction of Skyrme force is used for studying the nuclear structure properties.Purpose: To calculate the rms radii of proton and neutron for thorium nuclei, lying between the drip lines, by using the microscopic mean field theory. The nuclear rms radii data is useful for identifying the shape variation of thorium nuclei, from proton drip line to neutron drip line. It also helps to identify the trends in nuclear radii variation as we move towards the drip line. This nuclear data will be useful in designing experiments in future and also in understanding the behaviour of complex nuclei. Microscopic study of thorium nuclei is also important in the astrophysical environments.Methods: This study is based on the Skyrme interacting potential in the Hartree-Fock mean field theory. Iterative diagonalization method with the help of a computational code is used for solving the Hartree-Fock equation.Results: We have calculated the rms radii of neutron, proton and their total with SV, SLY4 and UDF2 parametrization of the Skyrme force. Neutron rms radii, proton rms radii and total rms radii of thorium nuclei are found to increase with neutron number. UDF2 parametrization shows an oscillatory nature in the rms radii. This may be due to the shape change of thorium nuclei when adding neutrons.Conclusions: The rms radii of thorium nuclei are found to increase with neutron number. The Skyrme force with UDF2 parametrization is the most suitable one for the structure studies of thorium nuclei.
背景:核均方根半径提供了核结构、核形状、核变形等信息。显微方法被广泛用于核结构性质的研究。采用具有Skyrme力有效相互作用的Hartree-Fock方法研究了核的结构性质。目的:用微观平均场理论计算滴线之间钍核的质子和中子的均方根半径。核均方根半径数据对于确定钍原子核从质子滴线到中子滴线的形状变化是有用的。它还有助于确定核半径变化的趋势,因为我们移动到滴油管。这些核数据对将来设计实验和理解复杂核的行为是有用的。钍核的微观研究在天体物理环境中也很重要。方法:基于Hartree-Fock平均场理论中的Skyrme相互作用势进行研究。在计算代码的帮助下,采用迭代对角化方法求解Hartree-Fock方程。结果:我们用SV、sl4和UDF2参数化计算出了中子、质子的均方根半径和总均方根半径。钍原子核的中子均方根半径、质子均方根半径和总均方根半径随中子数的增加而增大。UDF2参数化在均方根半径上显示出振荡性质。这可能是由于加入中子后钍原子核的形状发生了变化。结论:钍原子核的均方根半径随中子数的增加而增大。采用UDF2参数化的Skyrme力最适合于钍原子核的结构研究。
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引用次数: 0
Heavy Particle Accompanied Fission of 284Og - A Statistical Model Study 284Og重粒子伴随裂变的统计模型研究
Pub Date : 2021-08-31 DOI: 10.15415/jnp.2021.91003
S. Subramanian, S. Selvaraj
The structural characteristics of SHN can be investigated through the decay of SHN. In the present work ternary fission of SHN 284Og for two proton magic fixed third fragment 48Ca and 68Ni is studied at three different excitation energies 20, 35 and 50 MeV. Interestingly, 169Yb + 67Ni + 48Ca is having larger yield values and hence it is the most favoured way of fragmentation at intermediate excitation energy 35 MeV. It is observed that, asymmetric fission is favoured over symmetric fission at all the excitation for the third fragment 48Ca. Asymmetric fission is the most favoured with the fragment combination 148Sm + 68Ni + 68Ni for fixed A3 = 68Ni at all the excitations. Unlike the Ca third fragment, near symmetric fission is also favoured with 113Ag + 103Tc + 68Ni for A3 = 68Ni at all the three excitation energies.
通过SHN的衰变可以研究SHN的结构特性。本文研究了SHN 284Og在20mev、35mev和50mev三种激发能下对两个质子魔力固定的第三碎片48Ca和68Ni的三元裂变。有趣的是,169Yb + 67Ni + 48Ca具有更大的屈服值,因此在中等激发能35 MeV时,它是最有利的碎裂方式。我们观察到,在所有的激发下,非对称裂变都比对称裂变更有利。对于固定的A3 = 68Ni,在所有激发下均以148Sm + 68Ni + 68Ni的碎片组合最有利于非对称裂变。与Ca第三碎片不同的是,A3 = 68Ni在三种激发能下,113Ag + 103Tc + 68Ni也有利于近对称裂变。
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引用次数: 0
Comparative Analysis of Woods-Saxon and Yukawa Model Nuclear Potentials Woods-Saxon和Yukawa模型核势的比较分析
Pub Date : 2021-08-31 DOI: 10.15415/jnp.2021.91013
O. Sastri, Aditi Sharma, Swapna Gora, Richa Sharma
In this paper, we model the nuclear potential using Woods-Saxon and Yukawa interaction as the mean field in which each nucleon experiences a central force due to rest of the nucleons. The single particle energy states are obtained by solving the time independent Schrodinger wave equation using matrix diagonalization method with infinite spherical well wave-functions as the basis. The best fit model parameters are obtained by using variational Monte-Carlo algorithm wherein the relative mean-squared error, christened as chi-squared value, is minimized. The universal parameters obtained using Woods-Saxon potential are found to be matched with literature reported data resulting a chi-square value of 0.066 for neutron states and 0.069 for proton states whereas the chi-square value comes out to be 1.98 and 1.57 for neutron and proton states respectively by considering Yukawa potential. To further assess the performance of both the interaction potentials, the model parameters have been optimized for three different groups, light nuclei up to 16O - 56Ni, heavy nuclei 100Sn - 208Pb and all nuclei 16O - 208Pb. It is observed that Yukawa model performed reasonably well for light nuclei but did not give satisfactory results for the other two groups while Woods-Saxon potential gives satisfactory results for all magic nuclei across the periodic table. 
在本文中,我们使用伍兹-撒克逊和汤川相互作用作为平均场来模拟核势,其中每个核子经历由其余核子引起的中心力。以无限球面井波函数为基础,采用矩阵对角化方法求解与时间无关的薛定谔波方程,得到了单粒子的能量态。采用变分蒙特卡罗算法得到最佳拟合模型参数,其中相对均方误差(称为卡方值)最小。利用Woods-Saxon势得到的通用参数与文献报道的数据相匹配,中子态和质子态的卡方值分别为0.066和0.069,而考虑汤川势得到的中子态和质子态的卡方值分别为1.98和1.57。为了进一步评估这两种相互作用势的性能,对三种不同的原子核进行了模型参数优化,分别是轻核(16O - 56Ni)、重核(100Sn - 208Pb)和所有核(16O - 208Pb)。我们观察到汤川模型对轻核的表现相当好,但对其他两组的结果不满意,而伍兹-撒克逊势对周期表上所有的幻核都能给出满意的结果。
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引用次数: 2
Effect of the Width of Gaussian Wave Packets on the Stability of the Nuclei 高斯波包宽度对原子核稳定性的影响
Pub Date : 2021-08-31 DOI: 10.15415/jnp.2021.91002
S. Goyal
The role of the range of interaction on the stability of the nuclei propagating with and without momentum dependent interactions is analyzed within the framework of Quantum Molecular Dynamics (QMD) model. A detailed study is carried out by taking different equations of state (i.e., static soft and hard and the momentum dependent soft and hard) for the selected nuclei from 12C to 197Au. Comparison is done by using the standard and the double width of the Gaussian wave packets. We find that the effect of the double width of the Gaussian wave packets on the stability of the initial stage nuclei cannot be neglected. The nuclei having double width do not emit free nucleons for a long period of time. Also, the ground state properties of all the nuclei are described well. In the low mass region, the obtained nuclei are less bound but stable. Heavy mass nuclei have proper binding energy and are stable.
在量子分子动力学(QMD)模型的框架内,分析了相互作用范围对有动量依赖相互作用和没有动量依赖相互作用的原子核的稳定性的影响。采用不同的状态方程(即静态软、硬、动量依赖软、硬)对12C ~ 197Au范围内选定的核进行了详细的研究。采用高斯波包的标准宽度和双宽度进行了比较。我们发现高斯波包的双宽度对初始核稳定性的影响是不可忽视的。具有双宽度的原子核在很长一段时间内不释放自由核子。此外,所有原子核的基态性质都得到了很好的描述。在低质量区,得到的原子核束缚较少,但稳定。大质量原子核具有适当的结合能,是稳定的。
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引用次数: 0
Triton Scattering Phase-Shifts for S-wave using Morse Potential 基于莫尔斯电势的s波Triton散射相移
Pub Date : 2021-08-31 DOI: 10.15415/jnp.2021.91014
Anil Khachi, S. Awasthi, O. Sastri, L R Amruth Kumar
In this paper, the phase-shifts for neutron-dueteron (n-d) scattering have been determined using the molecular Morse potential as theoretical model of interaction. The Triton (n-d) 2S1/2 ground state initially has been chosen as -7.61 MeV to determine the model parameters using variational Monte-Carlo technique in combination with matrix methods numerical approach to solving the time independent Schrodinger equation (TISE). The obtained potential is incorporated into the phase function equation, which is solved using Runge-Kutta (RK) 4,5 order technique, to calculate the phaseshifts at various lab energies below 15 MeV, for which experimental data is available. The results have been compared with those obtained using another molecular potential named Manning-Rosen (MR) and have been observed to fare better. Finally, the Triton ground state has been chosen as its binding energy (BE), given by -8.481795 MeV, as determined from experimental atomic mass evaluation data and the calculations are repeated. It has been found that these phase-shifts from BE data are slightly better matched with experimental ones as compared to those obtained using -7.61 MeV ground state for Triton (n-d two-body system) modeled using Morse potential.
本文用分子莫尔斯势作为相互作用的理论模型,确定了中子-氘核(n-d)散射的相移。Triton (n-d) 2S1/2基态初始值为-7.61 MeV,采用变分蒙特卡罗技术结合矩阵方法求解时间无关薛定谔方程(TISE),确定模型参数。将得到的势代入相函数方程,利用龙格-库塔(RK) 4,5阶技术求解相函数方程,计算出15 MeV以下不同实验室能量下的相移,得到实验数据。结果已经与使用另一种称为曼宁-罗森(MR)的分子势得到的结果进行了比较,并且观察到效果更好。最后,选择Triton基态作为它的结合能(BE),由实验原子质量评价数据得到-8.481795 MeV,并进行了重复计算。与使用莫尔斯势模型模拟Triton (n-d两体系统)-7.61 MeV基态得到的相移相比,BE数据的相移与实验相移的匹配程度稍好一些。
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引用次数: 2
Comparative Analysis of 13,14C Induced Reactions on 232Th Target 232Th靶上13,14c诱导反应的比较分析
Pub Date : 2021-08-31 DOI: 10.15415/jnp.2021.91009
M. Kaur, BirBikram Singh, M. Sharma
We have investigated the pairing and magicity effect in context of a comparative study of 13,14C induced reactions on 232Th target at energies in the vicinity of Coulomb barrier. The fission distribution and related properties are explored in terms of the summed-up preformation probabilities. The barrierpenetrability is found to be higher for fragments emitted from 246Cm* formed in 14C+232Th reaction than those emitted in the fission of 245Cm*, leading to higher magnitude of cross-section for earlier case. The DCM calculated fusion-fission cross-sections using ΔR=0 fm are normalised to compare with the available experimental data. The calculations are done for spherical shape of fragments and it will be of further interest to explore the fission mass distribution after the inclusion of deformations.
本文研究了1314c在232Th靶上在库仑势垒附近诱导反应的配对效应和魔力效应。利用总结的预形成概率探讨了裂变分布及其相关性质。在14C+232Th反应中,246Cm*产生的碎片比245Cm*裂变产生的碎片具有更高的障壁穿透率,这导致了早期反应产生的截面大小更高。利用ΔR=0 fm计算的DCM计算的聚变-裂变截面归一化,并与现有的实验数据进行比较。这些计算是对碎片的球形进行的,进一步探索包含变形后的裂变质量分布将是有意义的。
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引用次数: 0
Decay Analysis of 197Tl* Compound Nucleus Formed in 16O + 181Ta Reaction at above Barrier Energy Ec.m.~100 MeV 16O + 181Ta反应中197Tl*复合核的衰变分析~ 100伏
Pub Date : 2021-08-31 DOI: 10.15415/jnp.2021.91017
G. Sarkar, M. Maiti, A. Kaur, M. Sharma
The decay dynamics of 197Tl* compound nucleus has been studied within the framework of the dynamical cluster-decay model (DCM) at above barrier energy Ec.m. ≈ 100 MeV using quadrupole deformed configuration of decay fragments. The influence of various nuclear radius parameters on the decay path and mass distributions has been investigated by analysing the fragmentation potential and preformation probability. It is observed that 197Tl* nucleus exhibits the triple-humped mass distribution, independent of nuclear radius choice. The most preferred fission fragments of both fission modes (symmetric and asymmetric) are identified, which lie in the neighborhood of spherical and deformed magic shell closures. Moreover, the modification in the barrier characteristics, such as interaction barrier and interaction radius, is observed with the variation in the radius parameter of decaying fragments and influences the penetrability and fission cross-sections. Finally, the fission cross-sections are calculated for considered choices of nuclear radii, and the results are compared with the available experimental data.
本文在动力学团簇衰变模型(DCM)的框架下,研究了197Tl*复合核在势垒能以上的衰变动力学。≈100 MeV,采用四极形变结构的衰变碎片。通过分析裂变势和预形成概率,研究了不同核半径参数对衰变路径和质量分布的影响。结果表明,197Tl*核的质量分布与核半径的选择无关,呈三峰状分布。确定了两种裂变模式(对称和非对称)中最优选的裂变碎片,它们位于球形和变形魔壳闭包附近。此外,随着衰变破片半径参数的变化,可以观察到势垒特性的变化,如相互作用势垒和相互作用半径,并影响穿透率和裂变截面。最后,在考虑核半径选择的情况下计算了裂变截面,并将计算结果与现有实验数据进行了比较。
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引用次数: 0
期刊
Journal of Nuclear Physics, Material Sciences, Radiation and Applications
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