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Recalculated Viola-Seaborg Coefficients for Partial Alpha Half-lives Based on AME2016 基于AME2016重新计算部分α半衰期的Viola-Seaborg系数
Pub Date : 2021-08-31 DOI: 10.15415/jnp.2021.91007
L. Kumar, Swapna Gora, V. Rana, Anil Khachi, O. Sastri
In this paper, the systematics for obtaining the Viola-Seaborg formula (VSF) for logarithmic partial alpha half-lives (Tα1/2) have been undertaken based on the NUBASE2016 evaluation. The constants Az and Bz in Geiger-Nuttal law for determination of Tα1/2  , are obtained using gs-gs transitions data, of even-even nuclei for two sets of nuclei with Z = 84 - 102 and Z = 86 - 98 with N > 126. The Viola-Seaborg co-efficients are determined for both the sets. The obtained parameters for both sets are tested on even-even nuclei for Z ranging from 104 - 118 and it is observed that first set parameters fare better. This formula for estimating α-decay half-lives of heavy nuclei can be extrapolated to predict those of super-heavy nuclei. The logarithmic half-lives Tα1/2 obtained for isotopes of Z = 121 and 122 using current modified VSF (AME2016) are compared with those obtained from theoretical considerations using Coulomb and proximity potential model (CPPM) and observed to be much larger. They are also much larger than those obtained from the previous coefficients based on AME2003 data.
本文基于NUBASE2016评价,对对数偏α半衰期(t - α1/2)的Viola-Seaborg公式(VSF)进行了系统求解。利用偶偶核的gs-gs跃迁数据,对Z = 84 ~ 102和Z = 86 ~ 98且N > 126的两组核,得到了测定Tα1/2的geiger - nunal定律常数Az和Bz。确定了两组的Viola-Seaborg系数。在Z值为104 ~ 118的偶偶核上对两组所得到的参数进行了测试,发现第一组参数效果更好。这个估算重核α衰变半衰期的公式可以外推到预测超重核的半衰期。用电流修正VSF (AME2016)计算得到的Z = 121和122同位素的对数半衰期Tα1/2与用库仑和接近电位模型(CPPM)理论计算得到的半衰期Tα1/2要大得多。它们也比以前基于AME2003数据得到的系数大得多。
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引用次数: 0
Neutron-Proton Scattering Phase Shifts in S-Channel using Phase Function Method for Various Two Term Potentials s通道中中子-质子散射的相移,用相函数法计算各种两项电位
Pub Date : 2021-08-31 DOI: 10.15415/jnp.2021.91015
Anil Khachi, L. Kumar, O. Sastri
The scattering phase shifts for n-p scattering have been modeled using various two term exponential type potentials such as Malfliet-Tjon, Manning-Rosen and Morse to study the phase shifts in the S-channels. As a first step, the model arameters for each of the potentials are determined by obtaining binding energy of the deuteron using matrix methods vis-a-vis Variational Monte-Carlo (VMC) technique to minimize the percentage error w.r.t. the experimental value. Then, the first order ODE as given by phase function method (PFM), is numerically solved using 5th order Runge-Kutta (RK-5) technique, by substituting the obtained potentials for calculating phase shifts for the bound 3S1 channel. Finally, the potential parameters are varied in least squares sense using VMC technique to obtain the scattering phase-shifts for each of the potentials in the 1S0 channel. The numerically obtained values are seen to be matching with those obtained using other analytical techniques and a comparative analysis with the experimental values up to 300 MeV is presented.
利用Malfliet-Tjon、Manning-Rosen和Morse等不同的两项指数型势对n-p散射的相移进行了建模,研究了s通道中的相移。首先,利用矩阵法相对于变分蒙特卡罗(VMC)技术获得氘核的结合能,从而确定每个势的模型参数,以最小化与实验值相对的百分比误差。然后,用五阶龙格-库塔(RK-5)技术对相函数法(PFM)给出的一阶ODE进行数值求解,将得到的势代入计算束缚3S1信道的相移。最后,利用VMC技术在最小二乘意义上改变电势参数,得到了1S0通道中每个电势的散射相移。数值计算得到的数值与其他分析方法得到的数值相匹配,并与实验值进行了比较分析,最高可达300 MeV。
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引用次数: 7
Surface modification of polyethylene terephthalate (PET) by corona discharge plasma 电晕放电等离子体对聚对苯二甲酸乙二醇酯(PET)表面进行改性
Pub Date : 2021-02-10 DOI: 10.15415/JNP.2021.82016
O. Flores, B. Campillo, F. Castillo, H. Martínez, J. Colin
Received: September 26, 2020 Accepted: January 09, 2021 Published Online: February 10, 2021 Surface modification of polyethylene terephthalate (PET) was studied by corona discharge plasma at different exposure times using air as working gas. The modification of the surface properties are characterized, those are morphology and wettability. Corona plasma treatment was found to modify the PET surface in both morphology and wettability. The corona discharge at atmospheric pressure is a heterogeneous with multiple current pulses, which generates an asymmetric pattern of erosion on the PET surface. The corona discharge treatment erodes the surface and therefore modifies the surface morphology. The roughness of the PET surface increases in the impact point of the corona discharge on the PET surface. An increase in the wettability of PET was also observed after corona discharge treatment at atmospheric pressure.
采用电冕放电等离子体,以空气为工作气体,研究了不同暴露时间下聚对苯二甲酸乙二醇酯(PET)的表面改性。对改性后的表面形貌和润湿性进行了表征。电晕等离子体处理可以改变PET表面的形态和润湿性。大气压下的电晕放电具有多脉冲电流的非均匀性,在PET表面产生不对称的侵蚀模式。电晕放电处理会腐蚀表面,从而改变表面形貌。在电晕放电对PET表面的冲击点处,PET表面的粗糙度增加。在常压下电晕放电处理后,PET的润湿性也有所增加。
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引用次数: 0
Surface Modification of Polypropylene by Atmospheric Pressure Plasma 常压等离子体对聚丙烯表面改性的研究
Pub Date : 2021-02-10 DOI: 10.15415/JNP.2021.82011
O. Xosocotla, H. Martínez, B. Campillo
Received: September 18, 2020 Accepted: January 06, 2021 Published Online: February 10, 2021 In this investigation, we studied the influence of atmospheric pressure plasma treatment on the surface properties of polypropylene (PP). The PP samples were treated for various durations using a gliding arc plasma source with air as a working gas. The formation of polar groups (–OH and C = O) on the PP surface after plasma treatment was evaluated and analyzed using Raman spectroscopy and attenuated total reflection–Fourier transform infrared spectroscopy. The contact angle was measured using polar and non-polar liquids to obtain the polar and dispersive components as well as the surface free energy of the PP before and after treatment. A sevenfold increase after treatment was observed for the polar component, while hydrophobicity decreased 73% after treatment. Finally, changes in topography were observed using atomic force microscopy (AFM) analysis before and after plasma treatment. AFM images showed that under atmospheric treatment, the PP surface underwent etching, reducing the surface roughness. Microhardness measurements of the films also revealed significant changes in mechanical properties after plasma treatment.
在本研究中,我们研究了常压等离子体处理对聚丙烯(PP)表面性能的影响。使用以空气为工作气体的滑动电弧等离子体源对PP样品进行不同时间的处理。利用拉曼光谱和衰减全反射-傅里叶变换红外光谱对等离子体处理后PP表面极性基团(-OH和C = O)的形成进行了评价和分析。用极性和非极性液体测量接触角,得到处理前后PP的极性和色散组分以及表面自由能。极性组分在处理后增加了7倍,而疏水性在处理后下降了73%。最后,利用原子力显微镜(AFM)分析等离子体处理前后的形貌变化。AFM图像显示,在大气处理下,PP表面发生蚀刻,表面粗糙度降低。薄膜的显微硬度测量也显示了等离子体处理后力学性能的显著变化。
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引用次数: 1
Hydrochemistry and Uranium Concentration in Brackish Groundwater from an Arid Zone, Chihuahua, Mexico 墨西哥奇瓦瓦干旱区微咸地下水的水化学和铀浓度
Pub Date : 2021-02-10 DOI: 10.15415/JNP.2021.82024
Rentería-Villalobos Marusia, Mendieta-Mendoza Aurora, Montero-Cabrera María Elena, Manjón-Collado Guillermo, Galván-Moreno José Antonio
In arid zones, the principal water supply is from groundwater, which can present high concentration of salts, heavy metals, and radioactive elements. The aim of the study was to determine isotopic uranium concentration in groundwater samples with high concentration of salts and its association with other chemical species. Samples were taken from wells with high salt content. The 238,234U radioisotope concentrations were determined by liquid scintillation and alpha-particle spectrometry. In addition, the physical-chemical parameters were recorded in situ; whereas the dissolved ions and elemental composition were measured by UV-Vis and X-ray fluorescence spectrophotometry, respectively. To obtain isotopic uranium concentrations, three radiochemistry procedures were carried out. An ANOVA test was performed to compare the results from procedures, as well as an analysis of Pearson correlation was used between parameters to obtain their associations. Statistically, the U isotopic concentrations did not show differences (p-value 0.82) between procedures. 238U and 234U showed mean concentrations of 6.7 mBq mL-1 and 16.6 mBq mL-1, respectively, with an Activity Ratioby up 7.2. The groundwater under study showed high concentration of TDS, calcium, sulphate, chloride, nitrate, and nitrite. Isotopic U concentrations tend to increase with NO3>Zn>Cl>Br>SO4>Cu>T>SDT>P; meanwhile their contents decrease with T>Cl->NO2>Fe. These findings help us to understand the uranium behavior in groundwater with high salt contents as well as the influence of agricultural supplies on chemical species presents in groundwater.
在干旱地区,主要的水供应来自地下水,地下水可能含有高浓度的盐、重金属和放射性元素。这项研究的目的是确定盐浓度高的地下水样品中的同位素铀浓度及其与其他化学物质的关系。样品取自含盐量高的井。用液体闪烁和α粒子光谱法测定了238,234U放射性同位素浓度。此外,现场记录了物理化学参数;用紫外可见分光光度法和x射线荧光分光光度法分别测定了溶解离子和元素组成。为了获得同位素铀浓度,进行了三个放射化学程序。采用方差分析(ANOVA)检验比较各过程的结果,并采用Pearson相关性分析参数之间的相关性,以获得其相关性。在统计学上,不同处理间铀同位素浓度无差异(p值0.82)。238U和234U的平均浓度分别为6.7 mBq mL-1和16.6 mBq mL-1,活性比为7.2。地下水中TDS、钙、硫酸盐、氯化物、硝酸盐和亚硝酸盐含量较高。同位素U浓度的增加趋势为NO3>Zn>Cl>Br>SO4>Cu>T>SDT>P;它们的含量依次为T>Cl >NO2>Fe。这些发现有助于我们了解高含盐量地下水中铀的行为以及农业供给对地下水中化学物质的影响。
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引用次数: 0
Formic Acid Ionization and Fragmentation by Multiphoton Absorption 甲酸电离与多光子吸收碎裂
Pub Date : 2021-02-10 DOI: 10.15415/JNP.2021.82026
C. Cisneros, T. Bautista, C. F. Betancourt, E. Prieto, A. Guerrero, I. Álvarez
Multiphoton absorption is an intensity dependent nonlinear effect related to the excitation of virtual intermediate states. In the present work, multiphoton ionization and dissociation of the formic acid molecule (HCOOH) by the interaction with photons from 532 Nd: YAG laser at different intensities are discussed, using different carrier gases. The induced fragmentation-ionization patterns show up to 17 fragments and dissociation channels are proposed. Some evidence of small clusters formation and conformational memory from the ratio of the detected products, CO+ and CO2+, on the light of the available results, it is possible to conclude that they arise from trans and cis formic acid. Our results are compared with those obtained in other laboratories under different experimental conditions, some of them show only partial agreement and differences are discussed. Following the Keldysh description it is possible, from our experimental parameters, characterize our results, in the multiphoton absorption regime.
多光子吸收是一种与虚中间态激发有关的强度依赖的非线性效应。本文讨论了在不同载流子气体下,不同强度的532 Nd: YAG激光光子与甲酸分子(HCOOH)相互作用的多光子电离和解离。诱导的碎片-电离模式显示多达17个碎片和解离通道。一些小簇形成和构象记忆的证据来自于检测到的产物CO+和CO2+的比例,根据现有的结果,有可能得出结论,它们是由反式和顺式甲酸产生的。我们的结果与其他实验室在不同实验条件下得到的结果进行了比较,有些结果只显示部分一致,并讨论了差异。根据Keldysh的描述,从我们的实验参数可以在多光子吸收状态下描述我们的结果。
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引用次数: 1
Study through Geant4, for Time Resolution characterization of different detectors arrays coupled with two SiPMs, as a function of: the scintillator plastic material, its volumetric dimensions and the location of the radiation emission source 通过Geant4,研究了不同探测器阵列耦合两个sipm的时间分辨率特性,作为闪烁体塑料材料,其体积尺寸和辐射发射源位置的函数
Pub Date : 2021-02-10 DOI: 10.15415/JNP.2021.82028
C. H. Z. Fernández, Hernández Aguilar Javier Efrén, E. Moreno-Barbosa
Received: September 24, 2020 Accepted: January 30, 2021 Published Online: February 10, 2021 The high time resolution detectors are relevant in those experiments or simulations were the particles to detect, have a very short time of flight (TOF), and due this it ́s required that the detections times are ranged between ns. & ps. Using Geant4 software, it was made thirty simulations of coupled detectors to plastic scintillators with two silicon photomultipliers (SiPMs) located on the scintillator’s central sides. To characterize the time resolution, it was required to quantify the optical photons that reach the Score in a certain time, which are generated by muons on the surface of the plastic scintillator. Different configurations of muon beams were simulated at energy of 1 GeV, to interact with the configuration of the scintillator material of its corresponding arrangement. The simulations were made varying three parameters: the scintillator material “BC404 & BC422”, its size, and the location of the radiation source. Fifteen simulations correspond to BC404 material & fifteen simulations to BC422 material respectively. The first five simulations consisted in varying the scintillator’s volumetric size and collocate the muons beam guided randomly distributed over it, the next five simulations differentiate from setting up a directly centered beam, and the last five simulations for guide the beam on the left lower corner of each scintillator. The best time resolution achieved was σ= 8.67 +/− 0.26 ps., reported by the detector with BC422 scintillator material which has a volume of 20x20x3 mm3.
接收日期:2020年9月24日接收日期:2021年1月30日发布日期:2021年2月10日高时间分辨率探测器在那些实验或模拟中是相关的,被检测的粒子具有非常短的飞行时间(TOF),因此它要求检测时间在ns之间。利用Geant4软件,用两个硅光电倍增管(SiPMs)安装在塑料闪烁体的中心两侧,对耦合探测器进行了30次模拟。为了表征时间分辨率,需要量化在一定时间内到达Score的光子,这些光子是由塑料闪烁体表面的μ子产生的。模拟了能量为1 GeV的不同结构的介子光束,并与相应排列的闪烁体材料的结构相互作用。通过改变闪烁体材料“BC404 & BC422”、闪烁体大小和辐射源位置三个参数进行了模拟。15次模拟分别对应BC404材料和BC422材料。前5个模拟是改变闪烁体的体积大小,并将随机分布在闪烁体上的μ介子束进行配置,后5个模拟是不同于设置一个正中心的光束,后5个模拟是将光束引导到每个闪烁体的左下角。采用体积为20x20x3 mm3的BC422闪烁体材料,获得的最佳时间分辨率为σ= 8.67 +/−0.26 ps.。
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引用次数: 0
Gamma Irradiation of Aqueos Solution of L-Aspartic Acid, L-Aspartic Acid in Solid State, and L-Aspartic Acid Adsorbed into Na-Montmorillonite: Its Relevance in Chemistry Prebiotic l -天冬氨酸、固态l -天冬氨酸和l -天冬氨酸吸附在na -蒙脱土中的伽马辐射:与化学益生元的相关性
Pub Date : 2021-02-10 DOI: 10.15415/JNP.2021.82012
A. Meléndez-López, M. F. García-Hurtado, J. Cruz-Castañeda, A. Negrón-Mendoza, S. Ramos-Bernal, A. Heredia
Aspartic acid is an amino acid present in the modern proteins, however, is considered a primitive amino acid hence its importance in prebiotic chemistry experiments studies. In some works of prebiotic chemistry have been studied the synthesis and the stability of organic matter under high energy sources, and the role of clays has been highlighted due to clays that can affect the reaction mechanisms in the radiolytic processes. The present work is focused on the study of the role of Namontmorillonite in the gamma radiolysis processes of L-aspartic acid. Gamma radiolysis processes were carried out in three different systems a) L-aspartic acid in aqueous solution; b) L-aspartic acid in solid-state; and c) L-aspartic acid adsorbed into Na-montmorillonite. L-aspartic acid was analyzed by high-performance liquid chromatography−electrospray ionization−mass spectrometry (HPLCESI-MS). The results showed that the decomposition of L-aspartic acid considerably decreased in the presence of clay thus highlighting the protector role of clays and favors the stability of organic matter even under the possible high energy conditions of primitive environments. The principal product ofgamma radiolysis of L-aspartic acid was succinic acid produced by deamination reaction. On the other hand, when aspartic acid was irradiated in solid-state the main product was the L-aspartic acid dimer. Both radiolysis products are important for chemical evolution processes for L-aspartic acid in primitive environments.
天冬氨酸是一种存在于现代蛋白质中的氨基酸,但被认为是一种原始氨基酸,因此在益生元化学实验研究中具有重要意义。在一些益生元化学的研究中,研究了高能量源下有机物的合成和稳定性,并强调了粘土在辐射分解过程中的作用,因为粘土可以影响反应机制。本文主要研究了纳蒙脱土在l -天冬氨酸γ辐射分解过程中的作用。在三种不同的体系中进行γ辐射分解过程a)水溶液中的l -天冬氨酸;b)固态l -天冬氨酸;c) l -天冬氨酸吸附在钠蒙脱土上。采用高效液相色谱-电喷雾电离-质谱法(HPLCESI-MS)对l -天冬氨酸进行分析。结果表明,在粘土存在的情况下,l -天冬氨酸的分解明显减少,从而突出了粘土的保护作用,即使在原始环境可能存在的高能量条件下,也有利于有机质的稳定。l -天冬氨酸辐射分解的主要产物是脱胺反应产生的琥珀酸。另一方面,当天冬氨酸以固态形式辐照时,主要产物是l -天冬氨酸二聚体。这两种辐射分解产物对l -天冬氨酸在原始环境下的化学演化过程具有重要意义。
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引用次数: 0
Charged Lepton Masses as a Possible CPV Source 带电轻子质量作为可能的CPV源
Pub Date : 2021-02-10 DOI: 10.15415/JNP.2021.82021
O. Félix-Beltrán, J. E. B. J. E. Barradas-Guevara, F. Gonzalez-Canales
We realize a model-independent study of the so-called Tri-Bi-Maximal pattern of leptonic flavor mixing. Different charged lepton mass matrix textures are studied. In particular, we are interested in those textures with a minimum number of parameters and that are able to reproduce the current experimental data on neutrino oscillation. The textures studied here form an equivalent class with two texture zeros. We obtain a Tri-Bi-Maximal pattern deviation in terms of the charged leptons masses, leading to a reactor angle and three CP violation phases non-zero. These lastest are one CP violation phase Dirac-like and two phases Majorana-like. Also, we can test the phenomenological implications of the numerical values obtained for the mixing angles and CP violation phases, on the neutrinoless double beta decay, and in the present and upcoming experiments on long-base neutrino oscillation, such as T2K, NOvA, and DUNE.
我们实现了所谓的轻子风味混合的三-双极大模式的模型独立研究。研究了不同的带电轻子质量矩阵结构。我们特别感兴趣的是那些具有最少参数的织构,它们能够再现当前中微子振荡的实验数据。这里研究的纹理形成了一个具有两个纹理零的等效类。我们在带电轻子质量方面得到了一个三-双极值模式偏差,导致了一个反应堆角度和三个CP违逆相非零。最新发现的是一个类似狄拉克的CP违背相和两个类似马约拉纳的相。此外,我们还可以在T2K、NOvA和DUNE等长基中微子振荡实验中,验证混合角和CP破坏相的数值在无中微子双β衰变中的现象学意义。
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引用次数: 0
Optimization of the Position of the CR-39 Polycarbonate Sheet Inside the Solid State Track Detector “Measuring Device” Through Computational Fluid Dynamics Technique 基于计算流体力学技术的CR-39聚碳酸酯片材在固体轨迹探测器“测量装置”内的位置优化
Pub Date : 2021-02-10 DOI: 10.15415/JNP.2021.82013
A. Lima Flores, R. Palomino-Merino, V. Castaño, J. Golzarri, G. Espinosa
The “measuring device” is one of the most reliable, efficient and economic indoor radon dosimeters that exist. This device was developed by the Proyecto de Aplicaciones de la Dosimetria (PAD) at the Physics Institute of UNAM (IF-UNAM) and consists of a transparent rigid plastic cup, a CR-39 polycarbonate sheet and a standard size metal clip that is used to hold the polycarbonate in the center of the cup. The cup is wrapped and covered with a low-density polyurethane protector in order to prevent the detector from being irradiated by ionizing particles found in the environment. In this work, an analysis was carried out that allowed to understand how the radon concentration on the polycarbonate sheet varies when its height is changed with respect to the base of the plastic cup, in order to understand what position increase the probability of interaction between radon and the surface of the detector. For the development of this work, four computational simulations were performed with the technique called Computational Fluid Dynamics (CFD). The results shows that as the CR-39 is positioned more closed to the base of the cup, the probability of interaction of the radon and the detector increase. Based on these results it is concluded that, when there is a limit in the time in which a measuring device can be placed in the zone where it is desired to quantify indoor radon, it is recommended to collocated the CR-39 at 1 cm with respect to the base of the cup.
该“测量装置”是目前最可靠、最高效、最经济的室内氡剂量计之一。该装置由UNAM物理研究所(IF-UNAM)的应用剂量学项目(PAD)开发,由一个透明的刚性塑料杯,CR-39聚碳酸酯片和一个标准尺寸的金属夹组成,用于将聚碳酸酯固定在杯中心。杯子用低密度聚氨酯保护器包裹和覆盖,以防止探测器被环境中发现的电离粒子照射。在这项工作中,进行了一项分析,以了解当聚碳酸酯片的高度相对于塑料杯的底座发生变化时,聚碳酸酯片上的氡浓度是如何变化的,以便了解什么位置增加了氡与探测器表面相互作用的概率。为了开展这项工作,使用计算流体动力学(CFD)技术进行了四次计算模拟。结果表明,CR-39的位置越靠近杯底,氡与探测器相互作用的概率越大。根据这些结果,得出的结论是,当测量装置可以放置在想要量化室内氡的区域的时间有限制时,建议将CR-39放置在距离杯底1厘米的位置。
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引用次数: 0
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Journal of Nuclear Physics, Material Sciences, Radiation and Applications
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