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Toward development of a low-temperature failure envelope of cases for high-burnup RIAs under PWR operational conditions 开发压水堆运行条件下高燃烧 RIA 的低温失效情况包络线
IF 1.9 3区 工程技术 Q1 NUCLEAR SCIENCE & TECHNOLOGY Pub Date : 2024-10-30 DOI: 10.1016/j.nucengdes.2024.113642
L. Aldeia Machado , K. Nantes , E. Merzari , L. Charlot , A. Motta , W. Walters
A Reactivity-Initiated Accident (RIA) is a design-basis accident that occurs when the reactor loses one of its control rods. A reactivity insertion will follow such events, drastically increasing the fuel pellet’s temperature and volume due to thermal expansion. The fuel pellet and the cladding will interact mechanically, which could lead to cladding failure. This work presents the development of cases where low-temperature failures are more likely to happen for high-burnup fuels under PWR operational conditions. A coupled computational model between the nuclear fuel performance code BISON, MOOSE’s Thermal-Hydraulic Module (MOOSE-THM), and MOOSE’s Stochastic Tools Modules (MOOSE-STM) was created to study the thermal-hydraulic behavior of a high-burnup fuel rodlet during the first stages of an RIA transient, allowing us to identify three scenarios: the system reached CHF, leading to high-temperature failure, the system failed due to PCMI, or the system survived the whole transient without failing. To address these scenarios, we performed a sensitivity analysis with more than 140,000 model replicates through MOOSE-STM varying parameters such as the power pulse width, power pulse total energy deposition, hydride rim thickness, coolant inlet temperature, and coolant inlet mass flux. We also compared two PCMI failure criteria in our analysis. Our results suggest that the hydride rim thickness and the power pulse width will be the key parameters impacting the failure type our system would undergo during the power transient. Using the data from our simulations, we constructed two failure maps, one for each PCMI failure criterion, showing how the failure type is affected by each parameter considered in the sensitivity analysis. We also provided a closed-form expression for the boundary between the PCMI and CHF failure types as a function of the hydride rim thickness and power pulse width.
反应性引发事故(RIA)是指反应堆失去一根控制棒时发生的基于设计的事故。这种事故发生后会发生反应性插入,由于热膨胀,燃料芯块的温度和体积会急剧增加。燃料芯块和包壳将发生机械相互作用,从而导致包壳失效。这项工作介绍了压水堆运行条件下高燃耗燃料更有可能发生低温失效的情况。我们创建了核燃料性能代码 BISON、MOOSE 热液压模块(MOOSE-THM)和 MOOSE 随机工具模块(MOOSE-STM)之间的耦合计算模型,以研究高燃耗燃料棒材在 RIA 瞬态第一阶段的热液压行为,从而确定了三种情况:系统达到 CHF,导致高温失效;系统因 PCMI 而失效;或系统在整个瞬态过程中存活而未失效。针对这些情况,我们通过 MOOSE-STM 对功率脉冲宽度、功率脉冲总能量沉积、氢化物边缘厚度、冷却剂入口温度和冷却剂入口质量通量等参数进行了超过 14 万次模型重复的敏感性分析。我们还在分析中比较了两种 PCMI 失效标准。我们的结果表明,氢化物边缘厚度和功率脉冲宽度将是影响系统在功率瞬态期间发生故障类型的关键参数。利用模拟数据,我们绘制了两张失效图,每张图针对一个 PCMI 失效标准,显示了失效类型如何受到敏感性分析中考虑的每个参数的影响。我们还提供了 PCMI 和 CHF 故障类型边界的闭式表达式,它是氢化物边缘厚度和功率脉冲宽度的函数。
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引用次数: 0
Sub-channel analysis of the influence of the ATF cladding corrosion on thermal hydraulic behaviors ATF 覆层腐蚀对热液压行为影响的子通道分析
IF 1.9 3区 工程技术 Q1 NUCLEAR SCIENCE & TECHNOLOGY Pub Date : 2024-10-30 DOI: 10.1016/j.nucengdes.2024.113668
Mingdong Kai , Jiejin Cai
Accident-tolerant fuel (ATF) enhances the accident tolerance of the fuels by improving its thermal properties and antioxidant radiation performance, thereby enabling the reactor to withstand severe accidents for a long time. This article applies and improves heat transfer and CHF models in the COBRA-EN by considering the impact of cladding surface corrosion on critical heat transfer between coolant and fuel rods. We conduct detailed and critical validation of the model constructed in this paper based on two benchmark experiments. We apply this model to study the thermal–hydraulic behaviors of ATFs under accident conditions. We obtain parameters such as the maximum fuel centerline temperature (MFCT), the maximum cladding surface temperature (MCT), the minimal departure from nucleate boiling ratio (MDNBR), the critical heat flux (CHF), and the average void fraction (AVF) for different ATFs. The results indicate that under most transient operating conditions, cladding corrosion delays the soaring time of the MFCT and MCT, and generally enhances CHF, with an average enhancement amplitude of over 0.15 MW/m2. At the same time, due to the effect of cladding corrosion, the MDNBR of the reactor has also been improved, which mitigates the impact of the accident to some extent.
事故耐受燃料(ATF)通过改善燃料的热性能和抗氧化辐射性能来提高燃料的事故耐受性,从而使反应堆能够长期承受严重事故。本文通过考虑包壳表面腐蚀对冷却剂和燃料棒之间临界传热的影响,应用并改进了 COBRA-EN 中的传热和 CHF 模型。我们基于两个基准实验对本文构建的模型进行了详细而关键的验证。我们应用该模型研究了 ATF 在事故条件下的热液压行为。我们获得了不同 ATF 的最大燃料中心线温度 (MFCT)、最大包壳表面温度 (MCT)、最小离核沸腾比 (MDNBR)、临界热通量 (CHF) 和平均空隙率 (AVF) 等参数。结果表明,在大多数瞬态运行条件下,包层腐蚀会延迟 MFCT 和 MCT 的沸腾时间,并普遍增强 CHF,平均增强幅度超过 0.15 MW/m2。同时,由于包壳腐蚀的影响,反应堆的 MDNBR 也得到了改善,在一定程度上减轻了事故的影响。
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引用次数: 0
New insight into fatigue life of modified 9Cr-1Mo steel in liquid lead–bismuth environment and life prediction considering environmental factors 对液态铅铋环境中改性 9Cr-1Mo 钢疲劳寿命的新认识以及考虑环境因素的寿命预测
IF 1.9 3区 工程技术 Q1 NUCLEAR SCIENCE & TECHNOLOGY Pub Date : 2024-10-30 DOI: 10.1016/j.nucengdes.2024.113648
Shouwen Shi , Wei Huang , Gaoyuan Xie , Weibin Li , Longyi Yang , Qiang Lin , Gang Chen , Xu Chen
The fatigue life of modified 9Cr-1Mo steel in liquid lead bismuth eutectic (LBE) at different strain amplitudes, temperatures and oxygen concentrations are analyzed. A liquid metal embrittlement (LME) factor of plastic strain is proposed to account for the reduced fatigue life induced by LME effect, which is also found to correlate well with tensile elongation in LBE. In low oxygen content LBE, the LME effect is influenced by temperature instead of plastic strain amplitude. While in high oxygen content LBE, the plastic LME factor is found to decrease exponentially with increasing plastic strain amplitude. Based on these findings, a fatigue life prediction model is proposed taking into account of different environmental influencing factors. In total, 86 data points are used with 70 % data points for independent validation only. Regardless of the discrepancy in fatigue life from different sources, good prediction results are still achieved with 98 % data points fall within ± 3 error band and 75 % data points fall within ± 2 error band.
分析了液态铅铋共晶(LBE)中改性 9Cr-1Mo 钢在不同应变振幅、温度和氧浓度下的疲劳寿命。提出了塑性应变的液态金属脆化(LME)因子,以解释 LME 效应引起的疲劳寿命降低,该因子还与 LBE 中的拉伸延伸率密切相关。在低氧含量的鳞片状结晶器中,LME效应受温度而不是塑性应变振幅的影响。而在高含氧量的鳞片板材中,塑性 LME 因子会随着塑性应变振幅的增大而呈指数下降。基于这些发现,我们提出了一个考虑到不同环境影响因素的疲劳寿命预测模型。总共使用了 86 个数据点,其中 70% 的数据点仅用于独立验证。尽管不同来源的疲劳寿命存在差异,但仍取得了良好的预测结果,98% 的数据点在±3 的误差范围内,75% 的数据点在±2 的误差范围内。
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引用次数: 0
Analysis of the experimental tests performed at NACIE-UP facility through a novel CFX-RELAP5 codes coupling 通过新型 CFX-RELAP5 代码耦合分析在 NACIE-UP 设施进行的实验测试
IF 1.9 3区 工程技术 Q1 NUCLEAR SCIENCE & TECHNOLOGY Pub Date : 2024-10-30 DOI: 10.1016/j.nucengdes.2024.113676
T. Del Moro , P. Cioli Puviani , B. Gonfiotti , I. Di Piazza , D. Martelli , C. Ciurluini , F. Giannetti , R. Zanino , M. Tarantino
The design and safety assessment of Lead-cooled Fast Reactors (LFRs), being one of the Generation IV technologies, must be supported by extensive experimental campaigns. Such activities are necessary to completely understand the physical phenomena involved in such reactors, as well as to properly develop new numerical tools or validate the pre-existent ones. From the experimental point of view, ENEA Research Center of Brasimone is one of the most active institutions, thanks to its experimental platforms and know-how maturated since the early 2000s. From the numerical point of view, Computational Fluid Dynamics (CFD) codes are the most suitable ones to analyze some phenomena expected in a Heavy Liquid Metal (HLM)-cooled reactor, such as the complex 3D phenomena occurring within the pools or the core fuel assemblies. In addition, the fluid thermal conduction, usually neglected in a System Thermal-Hydraulic (STH) code, can assume a significant importance in some transient scenarios, e.g., loss of flow accidents with transition from forced to natural circulation. However, the safety analysis of the LFRs should still rely on the use of STH codes because of their lower computational cost compared to the CFD codes, also considering the high number of transient evolutions to be analyzed for the purpose of the reactor licensing. At ENEA Brasimone, a novel coupling approach has been developed to couple the CFD code Ansys CFX with the STH code RELAP5/Mod3.3. The coupled tool aims at exploiting the advantages of the two families of codes. It adopts a multi-scale approach to simulate in detail some circuit components while performing system-level analysis, so as to keep an acceptable computational time. The coupling technique is based on ad-hoc user routines written in FORTRAN and implemented in Ansys CFX, which acts as the master code. The user routines take care of time step management, data exchange, RELAP5 execution, and error checking. The goal of this paper is to assess the simulation capabilities of the coupled tool by reproducing a forced-to-natural-circulation transition test, carried out at the NACIE-UP facility, with LBE as working fluid. The work has been realized in the framework of the IAEA Coordinate Research Project-I31038, named “Benchmark of Transition from Forced to Natural Circulation Experiment with Heavy Liquid Metal Loop”.
作为第四代技术之一,铅冷快堆的设计和安全评估必须得到大量实验活动的支持。这些活动对于全面了解此类反应堆所涉及的物理现象,以及正确开发新的数值工具或验证已有工具都是必不可少的。从实验角度来看,ENEA 布拉西蒙研究中心是最活跃的机构之一,这要归功于其自 2000 年代初以来成熟的实验平台和专业技术。从数值角度来看,计算流体动力学(CFD)代码是分析重液态金属(HLM)冷却反应堆中某些预期现象的最合适代码,例如在水池或堆芯燃料组件内发生的复杂三维现象。此外,通常在系统热工-水力(STH)代码中被忽略的流体热传导在某些瞬态情况下可能具有重要意义,例如从强制循环过渡到自然循环时的失流事故。然而,低温冷冻堆的安全分析仍应依赖于 STH 代码的使用,因为与 CFD 代码相比,STH 代码的计算成本更低,同时还考虑到反应堆许可所需的大量瞬态演化分析。ENEA Brasimone 开发了一种新颖的耦合方法,将 CFD 代码 Ansys CFX 与 STH 代码 RELAP5/Mod3.3 结合起来。该耦合工具旨在利用两个系列代码的优势。它采用多尺度方法,在进行系统级分析的同时详细模拟某些电路元件,从而保持可接受的计算时间。耦合技术基于用 FORTRAN 编写并在作为主代码的 Ansys CFX 中实现的临时用户例程。用户例程负责时间步长管理、数据交换、RELAP5 执行和错误检查。本文的目的是通过再现在 NACIE-UP 设备上进行的以 LBE 为工作流体的强制到自然循环过渡试验,评估耦合工具的模拟能力。这项工作是在国际原子能机构协调研究项目-I31038(名为 "使用重金属液环从强制循环到自然循环过渡试验的基准")的框架内完成的。
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引用次数: 0
Crack path analysis of spent nuclear fuel cladding using the strain energy-based Dijkstra algorithm 利用基于应变能的 Dijkstra 算法分析乏核燃料包壳的裂纹路径
IF 1.9 3区 工程技术 Q1 NUCLEAR SCIENCE & TECHNOLOGY Pub Date : 2024-10-30 DOI: 10.1016/j.nucengdes.2024.113661
Jee A Baik, Jung Jin Kim
The integrity of spent fuel cladding is crucial for preventing the release of radioactive materials, which pose significant risks to public safety and the environment. However, accurately predicting cracks in cladding tubes remains a challenge. This study proposes a novel method for predicting crack paths in spent nuclear fuel cladding tubes using the Dijkstra algorithm, based on strain energy. In this method, cladding images are segmented into cladding and hydride pixels, followed by a finite element analysis to calculate the strain energy. The Dijkstra algorithm utilizes this strain energy data from hydrides to predict crack paths in areas with low resistance to loading. The predicted path exhibited an accuracy of 92.78 % with respect to the initiation point of the actual crack path and was located within 200 μm of the actual crack path. The proposed method demonstrates a higher similarity to the actual crack path than conventional image-based methods. These results suggest that the safety assessment of spent nuclear fuel can be enhanced, enabling the development of effective management strategies for spent nuclear fuel.
乏燃料包壳的完整性对于防止放射性物质泄漏至关重要,而放射性物质泄漏会给公共安全和环境带来重大风险。然而,准确预测包壳管中的裂纹仍然是一项挑战。本研究提出了一种基于应变能、使用 Dijkstra 算法预测乏核燃料包壳管裂纹路径的新方法。在这种方法中,包壳图像被分割为包壳和氢化物像素,然后进行有限元分析以计算应变能。Dijkstra 算法利用来自氢化物的应变能数据来预测负载阻力较低区域的裂纹路径。与实际裂纹路径的起始点相比,预测路径的准确率为 92.78%,并且位于实际裂纹路径的 200 μm 范围内。与传统的基于图像的方法相比,所提出的方法与实际裂纹路径的相似度更高。这些结果表明,可以加强乏核燃料的安全评估,从而制定有效的乏核燃料管理策略。
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引用次数: 0
Simulating the time-dependent evolution of Alkali-Silica Reaction (ASR) strains in concrete 模拟混凝土中随时间变化的碱硅反应(ASR)应变
IF 1.9 3区 工程技术 Q1 NUCLEAR SCIENCE & TECHNOLOGY Pub Date : 2024-10-30 DOI: 10.1016/j.nucengdes.2024.113658
Gunay Gina Aliyeva , Yann Le Pape , Abhinav Gupta
Alkali-Silica Reaction (ASR) affects the resiliency of concrete structures by initiation of cracking in concrete which in turn leads to deterioration. There has been an increasing demand to understand the ASR-induced expansion and degradation in concrete. Continued safe operation of concrete structures requires an assessment of ASR-induced expansion and degradation. This paper attempts to understand the time-dependent evolution of ASR-induced expansion and degradation in concrete structures. A novel approach is proposed to simulate the ASR-induced expansion and degradation in concrete that is based on coupling the ASR-induced strains with the mechanical strains using a time-dependent piecewise evolution process at each instance of time. Data from an experimental study is used to develop the proposed approach. It is shown that the proposed approach is able to simulate the ASR-induced expansion and degradation in concrete reasonably well.
碱硅反应(ASR)会影响混凝土结构的韧性,使混凝土开裂,进而导致结构退化。人们越来越需要了解 ASR 引起的混凝土膨胀和退化。混凝土结构的持续安全运行需要对 ASR 引起的膨胀和退化进行评估。本文试图了解 ASR 引起的混凝土结构膨胀和退化随时间的变化。本文提出了一种模拟 ASR 引起的混凝土膨胀和降解的新方法,该方法基于 ASR 引起的应变与机械应变的耦合,在每个时间实例使用随时间变化的片断演化过程。实验研究的数据被用来开发所提出的方法。结果表明,所提出的方法能够很好地模拟 ASR 引起的混凝土膨胀和降解。
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引用次数: 0
Open-set recognition based on the combination of deep learning and hypothesis testing for detecting unknown nuclear faults 基于深度学习和假设检验相结合的开放集识别,用于检测未知核故障
IF 1.9 3区 工程技术 Q1 NUCLEAR SCIENCE & TECHNOLOGY Pub Date : 2024-10-30 DOI: 10.1016/j.nucengdes.2024.113654
Wei Pan , Jihong Shen , Bo Wang , Shujuan Wang , Zhanhao Sun
Most current fault diagnosis techniques for nuclear systems mainly rely on the closed-set assumption, which restricts the diagnosis model to select from a set of pre-established known fault classes. However, the nuclear system is a dynamic open system, and unknown faults that have never been seen can occur at any time. Therefore, it is very meaningful to design a diagnosis model that can recognize both known and unknown faults. This paper proposes a fault diagnosis method for open-set scenarios. Specifically, a modified loss function is used to train a convolutional neural network (CNN) to learn more compact feature representations of known classes. The features output by the last fully connected layer of the CNN are taken as the scores belonging to each known class, and a calibration model based on extreme value theory (EVT) is introduced to calibrate the scores. In addition, hypothesis testing is introduced for statistical inference. The threshold is determined according to the confidence level to distinguish the known faults from the unknown faults. Experiments conducted on two sets of nuclear system faults simulation data demonstrate that the proposed model not only identifies more unknown faults without compromising the accuracy of known fault classification but also selects more appropriate thresholds for different datasets, thereby enhancing the model’s generalization capability. Furthermore, experiments under varying degrees of openness also prove that our model exhibits higher robustness across different levels of openness.
目前大多数核系统的故障诊断技术主要依赖于封闭集假设,即限制诊断模型从一组预先确定的已知故障类别中进行选择。然而,核系统是一个动态开放的系统,从未见过的未知故障随时可能发生。因此,设计一个既能识别已知故障又能识别未知故障的诊断模型是非常有意义的。本文提出了一种开放式场景下的故障诊断方法。具体来说,使用修正的损失函数来训练卷积神经网络(CNN),以学习已知类别的更紧凑的特征表示。将卷积神经网络最后一层全连接层输出的特征作为属于每个已知类别的分数,并引入基于极值理论(EVT)的校准模型来校准分数。此外,还引入了假设检验进行统计推断。根据置信度确定阈值,以区分已知故障和未知故障。在两组核系统故障模拟数据上进行的实验表明,所提出的模型不仅能在不影响已知故障分类准确性的情况下识别出更多未知故障,还能为不同数据集选择更合适的阈值,从而增强模型的泛化能力。此外,在不同开放程度下的实验也证明,我们的模型在不同开放程度下表现出更高的鲁棒性。
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引用次数: 0
Numerical investigation against CABRI-E7 experiment by coupling fuel-pin failure module with FRTAC 通过将燃料销失效模块与 FRTAC 相结合,针对 CABRI-E7 试验进行数值研究
IF 1.9 3区 工程技术 Q1 NUCLEAR SCIENCE & TECHNOLOGY Pub Date : 2024-10-29 DOI: 10.1016/j.nucengdes.2024.113651
Yi Lei , Bin Zhang , Siqi Feng , Hao Yang , Shaowei Tang , Lin Sun
Fuel-pin failure hold considerable importance in safety evaluations of sodium-fast reactors (SFRs) as fuel swelling and cladding rupture are key phenomena in the early stages of core disruptive accidents (CDAs). For transients leading to pin failure, the failure modes and initial fuel disruption depend partly on pre-transient irradiation effects, such as fission-gas retention and release, fuel swelling, cladding deformation, and central void formation. With the increasingly stringent requirements on safety analysis, it is necessary to accurately evaluate the thermo-mechanical degradation of the fuel-pin resulting from pre-transient irradiation. Therefore, this study developed a fuel-pin failure module based on mechanistic models of pre-transient fuel-pin characterization and proposed an innovative approach by coupling this module with the self-developed Fast Reactor Transient Analysis Code (FRTAC). The results of the numerical simulation against the CABRI-E7 test are presented and discussed in this paper. The expected heat transfer mechanism between fuel and cladding was reproduced by the simulation, and the temperature distribution of the fuel pin agreed well with other reference analysis codes. Additionally, analyses based on elastoplastic mechanics theory and biaxial stress rupture criteria were conducted, with a specific focus on the thermal and mechanical failure of the fuel-pin. The overall code assessment indicated that the prediction error was within an acceptable range, demonstrating that the module’s reliability and its applicability to safety analyses of oxide fuel in CDAs of SFRs.
燃料膨胀和包壳破裂是堆芯破坏性事故(CDA)早期阶段的关键现象,因此燃料销失效在钠快堆的安全评估中占有相当重要的地位。对于导致引脚失效的瞬变,失效模式和初始燃料破坏部分取决于瞬变前的辐照效应,如裂变气体滞留和释放、燃料膨胀、包层变形和中心空隙形成。随着对安全分析的要求越来越严格,有必要对瞬态前辐照导致的燃料引脚热机械退化进行准确评估。因此,本研究基于瞬态前燃料引脚表征的机理模型开发了燃料引脚失效模块,并提出了一种将该模块与自主开发的快堆瞬态分析代码(FRTAC)耦合的创新方法。本文介绍并讨论了针对 CABRI-E7 试验的数值模拟结果。模拟再现了燃料和包壳之间预期的热传导机制,燃料针的温度分布与其他参考分析代码吻合。此外,还根据弹塑性力学理论和双轴应力断裂标准进行了分析,重点关注燃料销的热失效和机械失效。对代码的总体评估表明,预测误差在可接受范围内,这表明该模块的可靠性及其适用于对超小型反应堆 CDA 中的氧化物燃料进行安全分析。
{"title":"Numerical investigation against CABRI-E7 experiment by coupling fuel-pin failure module with FRTAC","authors":"Yi Lei ,&nbsp;Bin Zhang ,&nbsp;Siqi Feng ,&nbsp;Hao Yang ,&nbsp;Shaowei Tang ,&nbsp;Lin Sun","doi":"10.1016/j.nucengdes.2024.113651","DOIUrl":"10.1016/j.nucengdes.2024.113651","url":null,"abstract":"<div><div>Fuel-pin failure hold considerable importance in safety evaluations of sodium-fast reactors (SFRs) as fuel swelling and cladding rupture are key phenomena in the early stages of core disruptive accidents (CDAs). For transients leading to pin failure, the failure modes and initial fuel disruption depend partly on pre-transient irradiation effects, such as fission-gas retention and release, fuel swelling, cladding deformation, and central void formation. With the increasingly stringent requirements on safety analysis, it is necessary to accurately evaluate the thermo-mechanical degradation of the fuel-pin resulting from pre-transient irradiation. Therefore, this study developed a fuel-pin failure module based on mechanistic models of pre-transient fuel-pin characterization and proposed an innovative approach by coupling this module with the self-developed Fast Reactor Transient Analysis Code (FRTAC). The results of the numerical simulation against the CABRI-E7 test are presented and discussed in this paper. The expected heat transfer mechanism between fuel and cladding was reproduced by the simulation, and the temperature distribution of the fuel pin agreed well with other reference analysis codes. Additionally, analyses based on elastoplastic mechanics theory and biaxial stress rupture criteria were conducted, with a specific focus on the thermal and mechanical failure of the fuel-pin. The overall code assessment indicated that the prediction error was within an acceptable range, demonstrating that the module’s reliability and its applicability to safety analyses of oxide fuel in CDAs of SFRs.</div></div>","PeriodicalId":19170,"journal":{"name":"Nuclear Engineering and Design","volume":"429 ","pages":"Article 113651"},"PeriodicalIF":1.9,"publicationDate":"2024-10-29","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142535541","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Round-robin analysis of highly depleted lithium for Generation IV nuclear reactor applications 用于第四代核反应堆的高贫化锂循环分析
IF 1.9 3区 工程技术 Q1 NUCLEAR SCIENCE & TECHNOLOGY Pub Date : 2024-10-29 DOI: 10.1016/j.nucengdes.2024.113664
Sean R. Scott , Johnny Williams , Sara Mastromarino , Norbert Gajos , Christian Berry , Ian Anderson , Steven Shen , Trent R. Graham , Cole Hexel , Josh Wimpenny , Jacob Brookhart , Alan Kruizenga
Lithium reference materials containing unnaturally high abundances of 7Li are not currently available, which poses quality control problems for highly depleted lithium materials (i.e., depleted in 6Li) required for Generation IV nuclear reactors. This study presents an interlaboratory comparison of a lithium carbonate (NIST SRM924a) containing nominally natural isotopic abundances (∼92.4 % Li-7) and a highly depleted lithium hydroxide material (∼99.95 % Li-7). The natural lithium isotope abundances of NIST SRM924a are confirmed, and the 6Li/7Li ratio of the lithium hydroxide ranged from 0.000399 to 0.000436 with an average of 0.000428 ± 0.000023 (2SD, n = 9). Going forward this material can be used as quality control for analytical work involving highly depleted lithium.
目前还没有含有非天然高丰度 7Li 的锂参考材料,这给第四代核反应堆所需的高贫化锂材料(即贫化 6Li)带来了质量控制问题。本研究对一种碳酸锂(NIST SRM924a)和一种高贫化氢氧化锂材料(Li-7 含量为 99.95%)进行了实验室间比较,前者含有名义上的天然同位素丰度(Li-7 含量为 92.4%),后者则含有名义上的天然同位素丰度(Li-7 含量为 99.95%)。NIST SRM924a 的天然锂同位素丰度得到了证实,氢氧化锂的 6Li/7Li 比率介于 0.000399 至 0.000436 之间,平均值为 0.000428 ± 0.000023(2SD,n = 9)。今后,这种材料可用作涉及高贫化锂的分析工作的质量控制。
{"title":"Round-robin analysis of highly depleted lithium for Generation IV nuclear reactor applications","authors":"Sean R. Scott ,&nbsp;Johnny Williams ,&nbsp;Sara Mastromarino ,&nbsp;Norbert Gajos ,&nbsp;Christian Berry ,&nbsp;Ian Anderson ,&nbsp;Steven Shen ,&nbsp;Trent R. Graham ,&nbsp;Cole Hexel ,&nbsp;Josh Wimpenny ,&nbsp;Jacob Brookhart ,&nbsp;Alan Kruizenga","doi":"10.1016/j.nucengdes.2024.113664","DOIUrl":"10.1016/j.nucengdes.2024.113664","url":null,"abstract":"<div><div>Lithium reference materials containing unnaturally high abundances of <sup>7</sup>Li are not currently available, which poses quality control problems for highly depleted lithium materials (i.e., depleted in <sup>6</sup>Li) required for Generation IV nuclear reactors. This study presents an interlaboratory comparison of a lithium carbonate (NIST SRM924a) containing nominally natural isotopic abundances (∼92.4 % Li-7) and a highly depleted lithium hydroxide material (∼99.95 % Li-7). The natural lithium isotope abundances of NIST SRM924a are confirmed, and the <sup>6</sup>Li/<sup>7</sup>Li ratio of the lithium hydroxide ranged from 0.000399 to 0.000436 with an average of 0.000428 ± 0.000023 (2SD, n = 9). Going forward this material can be used as quality control for analytical work involving highly depleted lithium.</div></div>","PeriodicalId":19170,"journal":{"name":"Nuclear Engineering and Design","volume":"429 ","pages":"Article 113664"},"PeriodicalIF":1.9,"publicationDate":"2024-10-29","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142535542","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
CFD modeling methods applied to a lead-cooled fast reactor: A parametric study on conjugate heat transfer and thermal boundary conditions 应用于铅冷快堆的 CFD 建模方法:共轭传热和热边界条件的参数研究
IF 1.9 3区 工程技术 Q1 NUCLEAR SCIENCE & TECHNOLOGY Pub Date : 2024-10-28 DOI: 10.1016/j.nucengdes.2024.113649
Ivan K. Umezu , Dario M. Godino , Damián E. Ramajo , Claubia Pereira , Antonella L. Costa
Given the ever-increasing global demand for energy and the need to reduce greenhouse gas emissions, small modular reactors (SMRs), have emerged as potential options for increasing the contribution of nuclear energy, offering lower costs and faster deployment compared to traditional nuclear projects. In the context of this technological development, safety studies have become a priority, particularly for licensing new-generation systems such as metal-cooled fast reactors. This work models the steady-state operation of the lead-cooled SMR SEALER Arctic using Computational Fluid Dynamics. The entire primary circuit of the SEALER is modeled; the core is represented as a combination of porous media and heat sources, the pumps are represented as recirculating boundary conditions to account for momentum sources, and the steam generators are represented as porous media coupled with a temperature-dependent heat sink function. The main objective of this study is to simulate the SEALER under steady-state condition, while also accounting for the effects of heat conduction through its solid regions, and heat losses on the reactor vessel wall to the environment. For the former, the reactor is modeled with and without conductive solids and surfaces, using a conjugate heat transfer model. For the latter, natural convection and radiation heat transfer considerations are included as boundary conditions, and a parametric study is carried out with a range of external temperatures, and their effects on fuel and coolant temperatures are also discussed. Despite significant differences in local temperatures near the vessel walls, the impact on the peak fuel temperature and the average coolant temperature was less noticeable. Ultimately, the general operating parameters of the steady-state reactor design were verified, which is the first step before using the current model to evaluate fast transients and postulated events, where the thermal inertia of the solids and additional heat losses could play a crucial role on determining the system’s response to rapid temperature changes.
鉴于全球对能源需求的不断增长以及减少温室气体排放的需要,小型模块化反应堆(SMR)已成为增加核能贡献的潜在选择,与传统核项目相比,它成本更低,部署更快。在这一技术发展的背景下,安全研究已成为当务之急,尤其是对金属冷却快堆等新一代系统的许可研究。这项研究利用计算流体动力学建立了铅冷 SMR SEALER Arctic 稳态运行模型。对 SEALER 的整个一次回路进行了建模;堆芯表示为多孔介质和热源的组合,泵表示为再循环边界条件以考虑动量源,蒸汽发生器表示为多孔介质与温度相关的散热功能的耦合。本研究的主要目的是模拟稳态条件下的 SEALER,同时考虑通过其固体区域进行热传导的影响,以及反应器容器壁对环境的热损失。对于前者,使用共轭传热模型对有和无传导性固体和表面的反应器进行建模。对于后者,将自然对流和辐射传热因素作为边界条件,并对一系列外部温度进行了参数研究,还讨论了它们对燃料和冷却剂温度的影响。尽管容器壁附近的局部温度存在明显差异,但对燃料峰值温度和冷却剂平均温度的影响并不明显。最终,稳态反应堆设计的一般运行参数得到了验证,这是在使用当前模型评估快速瞬态和假定事件之前的第一步。
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Nuclear Engineering and Design
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