npj Quantum Materials最新文献

Dynamic axion insulators feature a time-dependent axion field that can be induced by antiferromagnetic resonance. Here, we show that a Josephson junction incorporating this dynamic axion insulator between two superconductors exhibits striking doubled Shapiro steps wherein all odd steps are completely suppressed in the joint presence of a DC bias and a static magnetic field. The resistively shunted junction simulation confirms that these doubled Shapiro steps originate from the distinctive axion electrodynamics driven by the antiferromagnetic resonance, which thus not only furnishes a hallmark to identify the dynamic axion insulator but also provides a method to evaluate its mass term. Furthermore, the experimentally feasible differential conductance is also determined. Our work holds significant importance in condensed matter physics and materials science for understanding the dynamic axion insulator, paving the way for its further exploration and applications.

The incommensurate charge density wave states (CDWs) can exhibit steady motion in the flow limit after depinning, behaving as a nonequilibrium system with time-dependent states. Since the moving CDW, like an electric current, breaks both time-reversal and inversion symmetries, one may speculate the emergence of nonreciprocal nonlinear responses from such motion. However, the moving CDW order parameter is intrinsically time-dependent in the lab frame, and it is known to be challenging to evaluate the responses of such a time-varying system. In this work, following the principle of Galilean relativity, we resolve this time-dependent hard problem in the lab frame by mapping the system to the comoving frame with static CDW states through the Galilean transformation. We explicitly show that the nonreciprocal nonlinear responses would be generated by the movement of CDW states through violating Galilean relativity.

Phonon polaritons are hybrid states of light and matter that are typically realised when optically active phonons couple strongly to photons. We suggest a new approach to realising phonon polaritons, by employing a transverse-pumping Raman scheme, as used in experiments on cold atoms in optical cavities. This approach allows hybridisation between an optical cavity mode and any Raman-active phonon mode. Moreover, this approach enables one to tune the effective phonon–photon coupling by changing the strength of the transverse pumping light. We show that such a system may realise a phonon-polariton condensate. To do this, we find the stationary states and use Floquet theory to determine their stability. We thus identify distinct superradiant and lasing states in which the polariton modes are macroscopically populated. We map out the phase diagram of these states as a function of pump frequencies and strengths. Using parameters for transition metal dichalcogenides, we show that realisation of these phases may be practicably obtainable. The ability to manipulate phonon mode frequencies and attain steady-state populations of selected phonon modes provides a new tool for engineering correlated states of electrons.

An experimental study found superconductivity in bilayer phase of La₃Ni₂O₇, with the highest superconducting transition temperature (T_c) ∼ 80 K under pressure. Recently, some reports claimed that there exists a competitive monolayer-trilayer structural phase in La₃Ni₂O₇ compounds. We perform the first-principles calculations and find that bilayer phase of La₃Ni₂O₇ is energetically favorable under pressure. Although extensive studies have been done to investigate the electronic correlation and potential superconducting pairing mechanism in bilayer phase of La₃Ni₂O₇, the phonon properties and electron-phonon coupling (EPC) in the high-pressure I4/mmm phase of La₃Ni₂O₇ are not reported. Using the density functional theory (DFT) combined with Wannier interpolation technique, we study the phonon properties and EPC in bilayer phase of La₃Ni₂O₇ under 29.5 GPa. Our findings reveal that EPC is insufficient to explain the observed superconducting T_c ∼ 80 K. And the calculated Fermi surface nesting may explain the experimentally observed charge density wave (CDW) transition in bilayer phase of La₃Ni₂O₇. Our calculations substantiate that bilayer phase of La₃Ni₂O₇ is an unconventional superconductor.

Nonlinear charge transport, such as nonreciprocal longitudinal resistance and nonlinear Hall effect, has attracted considerable interest in probing the symmetries and topological properties of new materials. Recent research has revealed significant nonreciprocal longitudinal resistance and nonlinear Hall effect in MnBi₂Te₄, an intrinsic magnetic topological insulator, induced by the quantum metric dipole. However, the inconsistent response with charge density and conflicting C_3z symmetry requirement necessitate a thorough understanding of factors affecting the nonlinear transport measurement. This study uncovers an experimental factor leading to significant nonlinear transport signals in MnBi₂Te₄, attributed to gate voltage oscillation from the application of large alternating current. Additionally, a methodology is proposed to suppress this effect by individually grounding the voltage electrodes during second-harmonic measurements. The investigation underscores the critical importance of assessing gate voltage oscillation’s impact before determining the intrinsic nature of nonlinear transport in 2D material devices with an electrically connected operative gate electrode.

Scanning tunneling spectroscopy (STS) and scanning tunneling microscopy (STM) are perhaps the most promising ways to detect the superconducting gap size and structure in the canonical unconventional superconductor Sr₂RuO₄ directly. However, in many cases, researchers have reported being unable to detect the gap at all in STM conductance measurements. Recently, an investigation of this issue on various local topographic structures on a Sr-terminated surface found that superconducting spectra appeared only in the region of small nanoscale canyons, corresponding to the removal of one RuO surface layer. Here, we analyze the electronic structure of various possible surface structures using first principles methods, and argue that bulk conditions favorable for superconductivity can be achieved when removal of the RuO layer suppresses the RuO₄ octahedral rotation locally. We further propose alternative terminations to the most frequently reported Sr termination where superconductivity surfaces should be observed.

The vacancy effect in quantum spin liquid (QSL) has been extensively studied. A finite density of random vacancies in the Kitaev model can lead to a pileup of low-energy density of states (DOS), which is generally experimentally determined by a scaling behavior of thermodynamic or magnetization quantities. Here, we report detailed muon spin relaxation (μSR) results of H₃LiIr₂O₆, a Kitaev QSL candidate with vacancies. The absence of magnetic order is confirmed down to 80 mK, and the spin fluctuations are found to be persistent at low temperatures. Intriguingly, the time-field scaling law of longitudinal-field (LF)-μSR polarization is observed down to 0.1 K. This indicates a dynamical scaling, whose critical exponent of 0.46 is excellently consistent with the scaling behavior of specific heat and magnetization data. All the observations point to the finite DOS with the form (N(E)sim {E}^{-nu }), which is expected for the Kitaev QSL in the presence of vacancies. Our μSR study provides a dynamical fingerprint of the power-law low-energy DOS and introduces a crucial new insight into the vacancy effect in QSL.

The layered van der Waals material ZrTe₅ is known as a candidate topological insulator (TI), however its topological phase and the relation with other properties such as an apparent Dirac semimetallic state is still a subject of debate. We employ a semiclassical multicarrier transport (MCT) model to analyze the magnetotransport of ZrTe₅ nanodevices at hydrostatic pressures up to 2 GPa. The temperature dependence of the MCT results between 10 and 300 K is assessed in the context of thermal activation, and we obtain the positions of conduction and valence band edges in the vicinity of the chemical potential. We find evidence of the closing and re-opening of the band gap with increasing pressure, which is consistent with a phase transition from weak to strong TI. This matches expectations from ab initio band structure calculations, as well as previous observations that CVT-grown ZrTe₅ is a weak TI in ambient conditions.

We study the transport properties of underdoped trilayer cuprate HgBa₂Ca₂Cu₃O_8+δ with doping level p = 0.10–0.12 in magnetic field up to 88 T. We report for the first time in a cuprate superconductor a dramatic change of the quantum oscillation spectrum versus temperature, which is accompanied by a sign change of the Hall effect below T ≈10 K. Based on numerical simulations, we infer a Fermi surface reconstruction in the inner plane from an antiferromagnetic state (hole pockets) to a biaxial charge density wave state (electron pockets). We show that both orders compete and share the same hotspots of the Fermi surface, and we discuss our result in the context of spin-fermion models.

Flat bands are intriguing platforms for correlated and topological physics. Various methods have been developed to create flat bands utilizing lattice geometry, but the investigation of orbital symmetry in multiorbital materials is a new area of focus. Here, we introduce a site symmetry-based approach to emerging multiorbital 2D and 3D flat bands on the kagome and pyrochlore lattices. As a conceptual advance, the one-orbital flat bands are shown to originate as mutual eigenstates of isolated molecular motifs. Further developing the mutual eigenstate method for multiple orbitals transforming differently under the site symmetries, we derive interorbital hopping generated flat bands from the antisymmetric interorbital Hamiltonian and introduce group-theoretic descriptions of the flat band wavefunctions. Realizations of multiorbital flat bands in realistic materials are shown to be possible in the Slater-Koster formalism. Our findings provide new directions for exploring flat-band electronic structures for novel correlated and topological quantum states.