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Strong magnon-magnon coupling and low dissipation rate in an all-magnetic-insulator heterostructure 全磁-绝缘体异质结构中的强磁-磁子耦合和低耗散率
IF 4.6 2区 物理与天体物理 Q2 PHYSICS, APPLIED Pub Date : 2024-09-09 DOI: 10.1103/physrevapplied.22.034017
Jiacheng Liu, Yuzan Xiong, Jingming Liang, Xuezhao Wu, Chen Liu, Shun Kong Cheung, Zheyu Ren, Ruizi Liu, Andrew Christy, Zehan Chen, Yifan Liu, Ferris Prima Nugraha, Xi-Xiang Zhang, Dennis Chi Wah Leung, Wei Zhang, Qiming Shao
Magnetic insulators, such as yttrium iron garnets (YIGs), are important for spin-wave or magnonic devices as their low damping enables low-power dissipation. Magnetic insulator heterostructures can offer larger design space for realizing exotic magnonic quantum states, provided that individual layers have low damping and their exchange coupling is strong and engineerable. Here, we show that, in a high-quality all-insulator thulium iron garnet (TmIG)/YIG bilayer system, TmIG exhibits an ultralow dissipation rate thanks to its low-damping, low-saturation magnetization and strong orbital momentum. The low dissipation rates in both YIG and TmIG, along with their significant coupling strength due to interfacial exchange coupling, enable strong and coherent magnon-magnon coupling. The coupling strength can be tuned by varying the magnetic insulator layer thickness and magnon modes, which is consistent with analytical calculations and micromagnetic simulations. Our results demonstrate TmIG/YIG as a novel platform for investigating hybrid magnonic phenomena and open opportunities for magnon devices comprising all-insulator heterostructures.
钇铁石榴石(YIGs)等磁绝缘体对于自旋波或磁子器件非常重要,因为它们的低阻尼可以实现低功耗耗散。磁绝缘体异质结构可以为实现奇异的磁子量子态提供更大的设计空间,前提是单个层具有低阻尼,而且它们之间的交换耦合很强,可以进行工程设计。在这里,我们展示了在高质量全绝缘体铥铁榴石(TmIG)/YIG 双层体系中,铥铁榴石因其低阻尼、低饱和磁化和强轨道动量而表现出超低耗散率。YIG 和 TmIG 中的低耗散率,以及它们因界面交换耦合而产生的显著耦合强度,实现了强大而连贯的磁子-磁子耦合。耦合强度可以通过改变磁绝缘层厚度和磁子模式来调节,这与分析计算和微磁模拟结果一致。我们的研究结果表明,TmIG/YIG 是研究混合磁子现象的新型平台,并为包含全绝缘体异质结构的磁子器件带来了机遇。
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引用次数: 0
Beyond quantum Shannon decomposition: Circuit construction for n-qubit gates based on block-ZXZ decomposition 超越量子香农分解:基于块-ZXZ分解的 n 量子位门电路构建
IF 4.6 2区 物理与天体物理 Q2 PHYSICS, APPLIED Pub Date : 2024-09-09 DOI: 10.1103/physrevapplied.22.034019
Anna M. Krol, Zaid Al-Ars
This paper proposes an optimized quantum block-ZXZ decomposition method that results in more optimal quantum circuits than the quantum Shannon decomposition, which was presented in 2005 by M. Möttönen, and J. J. Vartiainen [in Trends in quantum computing research, edited by S. Shannon (Nova Science Publishers, 2006) Chap. 7, p. 149, arXiv:quant-ph/0504100]. The decomposition is applied recursively to generic quantum gates, and can take advantage of existing and future small-circuit optimizations. Because our method uses only single-qubit gates and uniformly controlled rotation-Z gates, it can easily be adapted to use other types of multi-qubit gates. With the proposed decomposition, a general three-qubit gate can be decomposed using 19 cnot gates (rather than 20). For general n-qubit gates, the proposed decomposition generates circuits that have 22484n322n+53 cnot gates, which is less than the best-known exact decomposition algorithm by (4n21)/3 cnot gates.
本文提出了一种优化的量子块-ZXZ分解方法,它比 M. Möttönen 和 J. J. Vartiainen 于 2005 年提出的量子香农分解方法[见 S. Shannon 编辑的《量子计算研究趋势》(新星科学出版社,2006 年)第 7 章第 149 页,arXiv:quant-ph/0504100]能产生更优化的量子电路。该分解方法可递归应用于通用量子门,并能利用现有和未来的小电路优化。由于我们的方法只使用单量子比特门和均匀控制的旋转-Z 门,因此很容易调整为使用其他类型的多量子比特门。使用我们提出的分解方法,一般的三量子位门可以用 19 个 cnot 门(而不是 20 个)来分解。对于一般的 n-qubit 门,所提出的分解方法生成的电路有 22484n-322n+53 个 cnot 门,比最著名的精确分解算法少 (4n-2-1)/3 个 cnot 门。
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引用次数: 0
Optical determination of thermoelectric transport coefficients in a hot-carrier absorber 热载流子吸收器中热电传输系数的光学测定
IF 4.6 2区 物理与天体物理 Q2 PHYSICS, APPLIED Pub Date : 2024-09-09 DOI: 10.1103/physrevapplied.22.034018
Thomas Vezin, Hamidreza Esmaielpour, Laurent Lombez, Jean-François Guillemoles, Daniel Suchet
Hot-carrier solar cells offer potential for enhancing the energy-conversion efficiency of photovoltaic devices. Transport properties of such systems remain largely unexplored but could hinder their efficiency. In this work, we develop a suitable framework for describing the thermoelectric ambipolar transport of photogenerated hot carriers and derive analytical expressions for the ambipolar transport coefficients that are valid even in the degenerate case. We demonstrate that these transport coefficients can be measured from hyperspectral photoluminescence imaging. We validate this experimental determination by showing its consistency with the Boltzmann transport equation in the relaxation-time approximation.
热载流子太阳能电池为提高光伏设备的能量转换效率提供了潜力。此类系统的传输特性在很大程度上仍未得到探索,但可能会阻碍其效率的提高。在这项研究中,我们建立了一个合适的框架来描述光生热载流子的热电非极性传输,并推导出了非极性传输系数的分析表达式,这些表达式即使在退化情况下也有效。我们证明,这些传输系数可以通过高光谱光致发光成像来测量。我们通过证明其与弛豫时间近似的玻尔兹曼输运方程的一致性,验证了这一实验测定结果。
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引用次数: 0
Tunable sigmoid behavior of a magnon-based parametron using a Y3Fe5O12/Pt bilayer disk 利用 Y3Fe5O12/Pt 双层盘实现基于磁子的可调谐西格码行为的准子系统
IF 4.6 2区 物理与天体物理 Q2 PHYSICS, APPLIED Pub Date : 2024-09-09 DOI: 10.1103/physrevapplied.22.l031002
Geil Emdi, Tomosato Hioki, Takahiko Makiuchi, Eiji Saitoh
Sigmoidal curve behavior of 0 and π state probability in a magnon parametron, using yttrium iron garnet (Y3Fe5O12) thin disk, is systematically investigated. We demonstrate that the probability distribution can be tuned by bias and pump microwave power. Our numerical calculation that considers increasing damping due to four-magnon scattering processes reproduces the results well.
我们利用钇铁石榴石(Y3Fe5O12)薄片系统地研究了磁子准电子中 0 和 π 状态概率的西格玛曲线行为。我们证明,概率分布可以通过偏置和泵浦微波功率来调整。我们的数值计算考虑了四磁子散射过程导致的阻尼增加,很好地再现了结果。
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引用次数: 0
Tuning the thermal conductivity of a silicon membrane using nanopillars: From crystalline to amorphous pillars 利用纳米柱调节硅膜的导热性:从晶体柱到非晶柱
IF 4.6 2区 物理与天体物理 Q2 PHYSICS, APPLIED Pub Date : 2024-09-09 DOI: 10.1103/physrevapplied.22.034016
Lina Yang, Yixin Xu, Xianheng Wang, Yanguang Zhou
Tuning thermal transport in nanostructures is essential for many applications, such as thermal management and thermoelectrics. Nanophononic metamaterials (NPMs) have shown great potential for reducing thermal conductivity. In this work, the thermal conductivity of NPMs with crystalline Si (c-Si) pillar, crystalline Ge (c-Ge) pillar, and amorphous Si (a-Si) pillar are systematically investigated by a molecular dynamics method. An analysis of phonon dispersion and spectral energy density shows that phonon dispersions of a Si membrane are flattened due to local resonant hybridization induced by both crystalline and amorphous pillars. In addition, an a-Si pillar can cause a larger reduction in thermal conductivity compared with a c-Si pillar. Specifically, when the atomic mass of the atoms in the pillars increases, the thermal conductivity of NPMs with a crystalline pillar increases because of the weakened phonon hybridization. However, the thermal conductivity of NPMs with an amorphous pillar is almost unchanged. The analyses of the reduction of thermal conductivity show that both resonant hybridization and scattering mechanisms are important in NPMs with a crystalline pillar, while the scattering mechanism dominates in NPMs with an amorphous pillar and NPMs with a short crystalline pillar. The results of this work can provide meaningful insights into controlling thermal transport in NPMs by choosing the materials and atomic mass of pillars for specific applications.
调谐纳米结构中的热传输对于热管理和热电等许多应用至关重要。纳米声超材料(NPM)在降低热传导率方面显示出巨大的潜力。在这项研究中,采用分子动力学方法系统地研究了具有晶体硅(c-Si)柱、晶体锗(c-Ge)柱和非晶硅(a-Si)柱的纳米超材料的热导率。对声子频散和频谱能量密度的分析表明,由于晶体和非晶柱引起的局部共振杂化,硅膜的声子频散变得扁平。此外,与晶体硅柱相比,非晶硅柱会导致热导率大幅降低。具体来说,当支柱中原子的原子质量增加时,由于声子杂化减弱,具有晶柱的 NPM 的热导率会增加。然而,具有非晶柱的 NPM 的热导率几乎没有变化。对热导率降低的分析表明,共振杂化和散射机制在具有晶柱的 NPM 中都很重要,而在具有非晶柱的 NPM 和具有短晶柱的 NPM 中,散射机制占主导地位。这项工作的结果可为我们提供有意义的见解,帮助我们通过选择材料和原子质量的支柱来控制 NPM 中的热传输,从而满足特定应用的需要。
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引用次数: 0
Target-field design of surface permanent magnets 表面永磁体的靶场设计
IF 4.6 2区 物理与天体物理 Q2 PHYSICS, APPLIED Pub Date : 2024-09-06 DOI: 10.1103/physrevapplied.22.034015
Peter J. Hobson, Chris Morley, Alister Davis, Thomas Smith, Mark Fromhold
We present a target-field approach to analytically design magnetic fields using permanent magnets. We assume that their magnetization is bound to a two-dimensional surface and is composed of a complete basis of surface modes. By posing the Poisson’s equation relating the magnetic scalar potential to the magnetization using Green’s functions, we derive simple integrals that determine the magnetic field generated by each mode. This approach is demonstrated by deriving the governing integrals for optimizing axial magnetization on cylindrical and circular-planar surfaces. We approximate the governing integrals numerically and implement them into a regularized least-squares optimization routine to design permanent magnets that generate uniform axial and transverse target magnetic fields. The resulting uniform axial magnetic field profiles demonstrate more than a tenfold increase in uniformity across equivalent target regions compared to the field generated by an optimally separated axially magnetized pair of rings, as validated using finite element method simulations. We use a simple example to examine how two-dimensional surface magnetization profiles can be emulated using thin three-dimensional volumes and determine how many discrete intervals are required to accurately approximate a continuously varying surface pattern. Magnets designed using our approach may enable higher-quality bias fields for electric machines, nuclear fusion, fundamental physics, magnetic trapping, and beyond.
我们提出了一种利用永磁体分析设计磁场的目标场方法。我们假设永磁体的磁化绑定在一个二维表面上,并由表面模式的完整基础组成。通过利用格林函数提出磁标量势与磁化之间的泊松方程,我们得出了确定每个模式产生的磁场的简单积分。通过推导优化圆柱面和圆平面上轴向磁化的支配积分,我们证明了这种方法。我们对支配积分进行了数值近似,并将其应用到正则化最小二乘优化程序中,从而设计出能产生均匀轴向和横向目标磁场的永磁体。由此产生的均匀轴向磁场剖面与最佳分离的轴向磁化对环产生的磁场相比,在等效目标区域的均匀性提高了十倍以上,这一点已通过有限元法模拟得到验证。我们用一个简单的例子来研究如何使用薄三维体积来模拟二维表面磁化剖面,并确定需要多少个离散区间才能精确地近似连续变化的表面图案。使用我们的方法设计的磁体可以为电机、核聚变、基础物理学、磁捕捉等领域提供更高质量的偏置磁场。
{"title":"Target-field design of surface permanent magnets","authors":"Peter J. Hobson, Chris Morley, Alister Davis, Thomas Smith, Mark Fromhold","doi":"10.1103/physrevapplied.22.034015","DOIUrl":"https://doi.org/10.1103/physrevapplied.22.034015","url":null,"abstract":"We present a target-field approach to analytically design magnetic fields using permanent magnets. We assume that their magnetization is bound to a two-dimensional surface and is composed of a complete basis of surface modes. By posing the Poisson’s equation relating the magnetic scalar potential to the magnetization using Green’s functions, we derive simple integrals that determine the magnetic field generated by each mode. This approach is demonstrated by deriving the governing integrals for optimizing axial magnetization on cylindrical and circular-planar surfaces. We approximate the governing integrals numerically and implement them into a regularized least-squares optimization routine to design permanent magnets that generate uniform axial and transverse target magnetic fields. The resulting uniform axial magnetic field profiles demonstrate more than a tenfold increase in uniformity across equivalent target regions compared to the field generated by an optimally separated axially magnetized pair of rings, as validated using finite element method simulations. We use a simple example to examine how two-dimensional surface magnetization profiles can be emulated using thin three-dimensional volumes and determine how many discrete intervals are required to accurately approximate a continuously varying surface pattern. Magnets designed using our approach may enable higher-quality bias fields for electric machines, nuclear fusion, fundamental physics, magnetic trapping, and beyond.","PeriodicalId":20109,"journal":{"name":"Physical Review Applied","volume":null,"pages":null},"PeriodicalIF":4.6,"publicationDate":"2024-09-06","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142224222","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
First-principles nanocircuit model of open electromagnetic resonators 开放式电磁谐振器的第一原理纳米电路模型
IF 4.6 2区 物理与天体物理 Q2 PHYSICS, APPLIED Pub Date : 2024-09-05 DOI: 10.1103/physrevapplied.22.034014
Carlo Forestiere, Giovanni Miano, Andrea Alù
We derive from first principles a general circuit model for open, frequency dispersive electromagnetic resonators in the full-wave regime. This model extends the concepts of radiation impedance to the polarization current-density modes induced in open resonators by an arbitrary external excitation. Its physics-based elements offer physical insights into the scattering problem and enable efficient modeling of the resonance frequency and associated bandwidth for arbitrary scattering resonances, establishing a powerful platform for the design and optimization of nanophotonic circuits. Our findings offer compelling prospects for electromagnetic scattering and ultrafast nanophotonics, streamlining the analysis and design of nanoresonators with enhanced operational speeds, and outlining a physics-based model of their temporal dynamics.
我们从第一原理出发,推导出了全波状态下开放式频率色散电磁谐振器的一般电路模型。该模型将辐射阻抗的概念扩展到任意外部激励在开放式谐振器中诱导的极化电流密度模式。其基于物理学的元素提供了对散射问题的物理洞察力,并能对任意散射谐振的谐振频率和相关带宽进行有效建模,为纳米光子电路的设计和优化建立了一个强大的平台。我们的研究成果为电磁散射和超快纳米光子学提供了令人信服的前景,简化了具有更快运行速度的纳米谐振器的分析和设计,并概述了基于物理学的时间动力学模型。
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引用次数: 0
Electron cooling behavior in cascading semiconductor double-quantum-well structures 级联半导体双量子阱结构中的电子冷却行为
IF 4.6 2区 物理与天体物理 Q2 PHYSICS, APPLIED Pub Date : 2024-09-05 DOI: 10.1103/physrevapplied.22.034012
Xiangyu Zhu, Chloé Salhani, Guéric Etesse, Naomi Nagai, Marc Bescond, Francesca Carosella, Robson Ferreira, Gérald Bastard, Kazuhiko Hirakawa
We investigate evaporative electron cooling in cascading semiconductor double-quantum-well (QW) structures. In this cascading double QW structure (QW1 and QW2, where QW2 is on the anode side), one electron absorbs two longitudinal optical (LO) phonons as it travels from the cathode to the anode, for which efficient thermionic cooling is expected. By analyzing the high-energy tail of the photoluminescence spectra, the electron temperature in each QW is determined. When Al0.35Ga0.65As barriers are used, anomalous electron heating in QW2 due to hot electron distribution above the barrier is observed. By introducing taller barriers (Al0.7Ga0.3As) before QW2 to suppress hot electron distribution above the barrier, electron cooling in both QWs by several tens of kelvins is achieved. Furthermore, oscillatory anticorrelated electron temperature change in the two QWs that results from LO-phonon scattering is observed.
我们研究了级联半导体双量子阱(QW)结构中的蒸发电子冷却。在这种级联双量子阱结构(QW1 和 QW2,其中 QW2 位于阳极侧)中,一个电子在从阴极到阳极的过程中会吸收两个纵向光学(LO)声子,因此有望实现高效的热离子冷却。通过分析光致发光光谱的高能尾部,可以确定每个 QW 中的电子温度。当使用 Al0.35Ga0.65As 势垒时,由于势垒上方的热电子分布,在 QW2 中观察到异常的电子加热现象。通过在 QW2 之前引入较高的势垒(Al0.7Ga0.3As)来抑制势垒上方的热电子分布,两个 QW 中的电子冷却了几十开尔文。此外,还观察到两个 QW 中因 LO 光子散射而产生的振荡反相关电子温度变化。
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引用次数: 0
Two-dimensional P3¯m1Ca3N2, Ba3P2, and Ba3As2: Promising stable narrow-gap semiconductors for infrared and broadband photodetectors 二维 P3¯m1Ca3N2、Ba3P2 和 Ba3As2:有望用于红外和宽带光探测器的稳定窄隙半导体
IF 4.6 2区 物理与天体物理 Q2 PHYSICS, APPLIED Pub Date : 2024-09-05 DOI: 10.1103/physrevapplied.22.034013
Qing-Yuan Chen, Fei-Jie Huang, Ju-Qi Ruan, Yi-Fen Zhao, Xiong-Fei Zhang, Kai Xiong, Yao He, CLEO Collaboration
Exploring two-dimensional (2D) narrow-gap materials with exceptional stability and outstanding photoelectric performance has become a key focus in nano-optoelectronics. However, most existing 2D materials contain relatively large band gaps, and those with narrow band gaps tend to have inadequate stability. This study employed first-principles calculation to predict three alternative narrow-gap 2D binary group (<math display="inline" overflow="scroll" xmlns="http://www.w3.org/1998/Math/MathML"><msub><mi>II</mi><mn>3</mn></msub></math>-<math display="inline" overflow="scroll" xmlns="http://www.w3.org/1998/Math/MathML"><msub><mrow><mi mathvariant="normal">V</mi></mrow><mn>2</mn></msub></math>) materials in the <math display="inline" overflow="scroll" xmlns="http://www.w3.org/1998/Math/MathML"><mi>P</mi><mrow><mover><mn>3</mn><mo stretchy="false">¯</mo></mover></mrow><mi>m</mi><mn>1</mn></math> space group: <math display="inline" overflow="scroll" xmlns="http://www.w3.org/1998/Math/MathML"><msub><mi>Ca</mi><mn>3</mn></msub><msub><mrow><mi mathvariant="normal">N</mi></mrow><mn>2</mn></msub></math>, <math display="inline" overflow="scroll" xmlns="http://www.w3.org/1998/Math/MathML"><msub><mi>Ba</mi><mn>3</mn></msub><msub><mrow><mi mathvariant="normal">P</mi></mrow><mn>2</mn></msub></math>, and <math display="inline" overflow="scroll" xmlns="http://www.w3.org/1998/Math/MathML"><msub><mi>Ba</mi><mn>3</mn></msub><msub><mi>As</mi><mn>2</mn></msub></math>. All these materials exhibit excellent energetic, mechanical, dynamic, and thermal stability. Their mechanical properties reveal isotropic characteristics and demonstrate excellent in-plane stiffness and flexibility. Regarding electronic properties, monolayer <math display="inline" overflow="scroll" xmlns="http://www.w3.org/1998/Math/MathML"><msub><mi>Ca</mi><mn>3</mn></msub><msub><mrow><mi mathvariant="normal">N</mi></mrow><mn>2</mn></msub></math>, <math display="inline" overflow="scroll" xmlns="http://www.w3.org/1998/Math/MathML"><msub><mi>Ba</mi><mn>3</mn></msub><msub><mrow><mi mathvariant="normal">P</mi></mrow><mn>2</mn></msub></math>, and <math display="inline" overflow="scroll" xmlns="http://www.w3.org/1998/Math/MathML"><msub><mi>Ba</mi><mn>3</mn></msub><msub><mi>As</mi><mn>2</mn></msub></math> possess indirect narrow band gaps of <math display="inline" overflow="scroll" xmlns="http://www.w3.org/1998/Math/MathML"><mn>0.41</mn></math>, <math display="inline" overflow="scroll" xmlns="http://www.w3.org/1998/Math/MathML"><mn>0.61</mn></math>, and <math display="inline" overflow="scroll" xmlns="http://www.w3.org/1998/Math/MathML"><mn>0.68</mn></math> eV, respectively. Moreover, they exhibit high electron mobilities (about <math display="inline" overflow="scroll" xmlns="http://www.w3.org/1998/Math/MathML"><msup><mn>10</mn><mn>3</mn></msup></math>–<math display="inline" overflow="scroll" xmlns="http://www.w3.org/1998/Math/MathML"><msup><mn>10</mn><mn>4</mn></msup><mspace width="0.2em"></mspace><msup><mi>cm<
探索具有优异稳定性和出色光电性能的二维(2D)窄间隙材料已成为纳米光电子学的一个重点。然而,现有的大多数二维材料都含有相对较大的带隙,而带隙较窄的材料往往稳定性不足。本研究采用第一性原理计算,预测了 P3¯m1 空间群中三种可供选择的窄间隙二维二元基团(II3-V2)材料:Ca3N2、Ba3P2 和 Ba3As2。所有这些材料都表现出卓越的能量、机械、动态和热稳定性。它们的机械性能显示出各向同性的特点,并具有出色的面内刚度和柔韧性。在电子特性方面,单层 Ca3N2、Ba3P2 和 Ba3As2 分别具有 0.41、0.61 和 0.68 eV 的间接窄带隙。此外,它们还表现出很高的电子迁移率(约 103-104cm2V-1s-1),并且几乎各向同性。在光学特性方面,它们的吸收范围很广,从红外到可见光和紫外区,吸收系数非常高(约 104-105cm-1)。此外,它们的激子结合能高于在传统块体材料中观察到的激子结合能,同时又低于大多数其他二维材料,因而具有优异的光驱动性能。我们认为,这些替代性二维 P3¯m1Ca3N2、Ba3P2 和 Ba3As2 二元窄隙半导体将在红外光探测、安培极晶体管、医学成像、电极、光通信和遥感等纳米光电领域具有广阔的应用前景。
{"title":"Two-dimensional P3¯m1Ca3N2, Ba3P2, and Ba3As2: Promising stable narrow-gap semiconductors for infrared and broadband photodetectors","authors":"Qing-Yuan Chen, Fei-Jie Huang, Ju-Qi Ruan, Yi-Fen Zhao, Xiong-Fei Zhang, Kai Xiong, Yao He, CLEO Collaboration","doi":"10.1103/physrevapplied.22.034013","DOIUrl":"https://doi.org/10.1103/physrevapplied.22.034013","url":null,"abstract":"Exploring two-dimensional (2D) narrow-gap materials with exceptional stability and outstanding photoelectric performance has become a key focus in nano-optoelectronics. However, most existing 2D materials contain relatively large band gaps, and those with narrow band gaps tend to have inadequate stability. This study employed first-principles calculation to predict three alternative narrow-gap 2D binary group (&lt;math display=\"inline\" overflow=\"scroll\" xmlns=\"http://www.w3.org/1998/Math/MathML\"&gt;&lt;msub&gt;&lt;mi&gt;II&lt;/mi&gt;&lt;mn&gt;3&lt;/mn&gt;&lt;/msub&gt;&lt;/math&gt;-&lt;math display=\"inline\" overflow=\"scroll\" xmlns=\"http://www.w3.org/1998/Math/MathML\"&gt;&lt;msub&gt;&lt;mrow&gt;&lt;mi mathvariant=\"normal\"&gt;V&lt;/mi&gt;&lt;/mrow&gt;&lt;mn&gt;2&lt;/mn&gt;&lt;/msub&gt;&lt;/math&gt;) materials in the &lt;math display=\"inline\" overflow=\"scroll\" xmlns=\"http://www.w3.org/1998/Math/MathML\"&gt;&lt;mi&gt;P&lt;/mi&gt;&lt;mrow&gt;&lt;mover&gt;&lt;mn&gt;3&lt;/mn&gt;&lt;mo stretchy=\"false\"&gt;¯&lt;/mo&gt;&lt;/mover&gt;&lt;/mrow&gt;&lt;mi&gt;m&lt;/mi&gt;&lt;mn&gt;1&lt;/mn&gt;&lt;/math&gt; space group: &lt;math display=\"inline\" overflow=\"scroll\" xmlns=\"http://www.w3.org/1998/Math/MathML\"&gt;&lt;msub&gt;&lt;mi&gt;Ca&lt;/mi&gt;&lt;mn&gt;3&lt;/mn&gt;&lt;/msub&gt;&lt;msub&gt;&lt;mrow&gt;&lt;mi mathvariant=\"normal\"&gt;N&lt;/mi&gt;&lt;/mrow&gt;&lt;mn&gt;2&lt;/mn&gt;&lt;/msub&gt;&lt;/math&gt;, &lt;math display=\"inline\" overflow=\"scroll\" xmlns=\"http://www.w3.org/1998/Math/MathML\"&gt;&lt;msub&gt;&lt;mi&gt;Ba&lt;/mi&gt;&lt;mn&gt;3&lt;/mn&gt;&lt;/msub&gt;&lt;msub&gt;&lt;mrow&gt;&lt;mi mathvariant=\"normal\"&gt;P&lt;/mi&gt;&lt;/mrow&gt;&lt;mn&gt;2&lt;/mn&gt;&lt;/msub&gt;&lt;/math&gt;, and &lt;math display=\"inline\" overflow=\"scroll\" xmlns=\"http://www.w3.org/1998/Math/MathML\"&gt;&lt;msub&gt;&lt;mi&gt;Ba&lt;/mi&gt;&lt;mn&gt;3&lt;/mn&gt;&lt;/msub&gt;&lt;msub&gt;&lt;mi&gt;As&lt;/mi&gt;&lt;mn&gt;2&lt;/mn&gt;&lt;/msub&gt;&lt;/math&gt;. All these materials exhibit excellent energetic, mechanical, dynamic, and thermal stability. Their mechanical properties reveal isotropic characteristics and demonstrate excellent in-plane stiffness and flexibility. Regarding electronic properties, monolayer &lt;math display=\"inline\" overflow=\"scroll\" xmlns=\"http://www.w3.org/1998/Math/MathML\"&gt;&lt;msub&gt;&lt;mi&gt;Ca&lt;/mi&gt;&lt;mn&gt;3&lt;/mn&gt;&lt;/msub&gt;&lt;msub&gt;&lt;mrow&gt;&lt;mi mathvariant=\"normal\"&gt;N&lt;/mi&gt;&lt;/mrow&gt;&lt;mn&gt;2&lt;/mn&gt;&lt;/msub&gt;&lt;/math&gt;, &lt;math display=\"inline\" overflow=\"scroll\" xmlns=\"http://www.w3.org/1998/Math/MathML\"&gt;&lt;msub&gt;&lt;mi&gt;Ba&lt;/mi&gt;&lt;mn&gt;3&lt;/mn&gt;&lt;/msub&gt;&lt;msub&gt;&lt;mrow&gt;&lt;mi mathvariant=\"normal\"&gt;P&lt;/mi&gt;&lt;/mrow&gt;&lt;mn&gt;2&lt;/mn&gt;&lt;/msub&gt;&lt;/math&gt;, and &lt;math display=\"inline\" overflow=\"scroll\" xmlns=\"http://www.w3.org/1998/Math/MathML\"&gt;&lt;msub&gt;&lt;mi&gt;Ba&lt;/mi&gt;&lt;mn&gt;3&lt;/mn&gt;&lt;/msub&gt;&lt;msub&gt;&lt;mi&gt;As&lt;/mi&gt;&lt;mn&gt;2&lt;/mn&gt;&lt;/msub&gt;&lt;/math&gt; possess indirect narrow band gaps of &lt;math display=\"inline\" overflow=\"scroll\" xmlns=\"http://www.w3.org/1998/Math/MathML\"&gt;&lt;mn&gt;0.41&lt;/mn&gt;&lt;/math&gt;, &lt;math display=\"inline\" overflow=\"scroll\" xmlns=\"http://www.w3.org/1998/Math/MathML\"&gt;&lt;mn&gt;0.61&lt;/mn&gt;&lt;/math&gt;, and &lt;math display=\"inline\" overflow=\"scroll\" xmlns=\"http://www.w3.org/1998/Math/MathML\"&gt;&lt;mn&gt;0.68&lt;/mn&gt;&lt;/math&gt; eV, respectively. Moreover, they exhibit high electron mobilities (about &lt;math display=\"inline\" overflow=\"scroll\" xmlns=\"http://www.w3.org/1998/Math/MathML\"&gt;&lt;msup&gt;&lt;mn&gt;10&lt;/mn&gt;&lt;mn&gt;3&lt;/mn&gt;&lt;/msup&gt;&lt;/math&gt;–&lt;math display=\"inline\" overflow=\"scroll\" xmlns=\"http://www.w3.org/1998/Math/MathML\"&gt;&lt;msup&gt;&lt;mn&gt;10&lt;/mn&gt;&lt;mn&gt;4&lt;/mn&gt;&lt;/msup&gt;&lt;mspace width=\"0.2em\"&gt;&lt;/mspace&gt;&lt;msup&gt;&lt;mi&gt;cm&lt;","PeriodicalId":20109,"journal":{"name":"Physical Review Applied","volume":null,"pages":null},"PeriodicalIF":4.6,"publicationDate":"2024-09-05","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142224229","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Critical phenomenon of the ferromagnet Cr2Te3 with strong perpendicular magnetic anisotropy 具有强垂直磁各向异性的铁磁体 Cr2Te3 的临界现象
IF 4.6 2区 物理与天体物理 Q2 PHYSICS, APPLIED Pub Date : 2024-09-04 DOI: 10.1103/physrevapplied.22.034006
Aina Wang, Zan Du, Fanying Meng, Azizur Rahman, Wei Liu, Jiyu Fan, Chunlan Ma, Langsheng Ling, Chuanying Xi, Min Ge, Li Pi, Yuheng Zhang, Lei Zhang
Chromium telluride <math display="inline" overflow="scroll" xmlns="http://www.w3.org/1998/Math/MathML"><msub><mi>Cr</mi><mi>x</mi></msub><msub><mi>Te</mi><mi>y</mi></msub></math> has great potential applications in spintronics due to its intrinsic ferromagnetism and strong magnetic anisotropy. In this study, we systematically investigate magnetic properties of a ferromagnetic <math display="inline" overflow="scroll" xmlns="http://www.w3.org/1998/Math/MathML"><msub><mi>Cr</mi><mn>2</mn></msub><msub><mi>Te</mi><mn>3</mn></msub></math> single crystal with strong perpendicular magnetic anisotropy (PMA). Apart from ferromagnetic-to-paramagnetic (FM-PM) transitions at <math display="inline" overflow="scroll" xmlns="http://www.w3.org/1998/Math/MathML"><msub><mi>T</mi><mi>C</mi></msub><mo>∼</mo><mn>181</mn></math> K for both <math display="inline" overflow="scroll" xmlns="http://www.w3.org/1998/Math/MathML"><mi>H</mi><mo>/</mo><mo>/</mo><mi>c</mi></math> and <math display="inline" overflow="scroll" xmlns="http://www.w3.org/1998/Math/MathML"><mi>H</mi><mo>/</mo><mo>/</mo><mi>a</mi><mi>b</mi></math>, other exotic magnetic behaviors are revealed, such as a field-modulated first-order transition uncovered by the anisotropic magnetization, a canted FM coupling rather than previously reported spin-glass behavior demonstrated by the ac susceptibility. Furthermore, anisotropic magnetization reveals significant PMA stronger than any other <math display="inline" overflow="scroll" xmlns="http://www.w3.org/1998/Math/MathML"><mi>Cr</mi></math>-based transition metal chalcogenide, with a negligible saturation field for <math display="inline" overflow="scroll" xmlns="http://www.w3.org/1998/Math/MathML"><mi>H</mi><mo>/</mo><mo>/</mo><mi>c</mi></math> but a distinct one up to 155 kOe for <math display="inline" overflow="scroll" xmlns="http://www.w3.org/1998/Math/MathML"><mi>H</mi><mo>/</mo><mo>/</mo><mi>a</mi><mi>b</mi></math>. Critical exponents <math display="inline" overflow="scroll" xmlns="http://www.w3.org/1998/Math/MathML"><mi>β</mi><mo>=</mo><mn>0.340</mn><mo stretchy="false">(</mo><mn>5</mn><mo stretchy="false">)</mo></math>, <math display="inline" overflow="scroll" xmlns="http://www.w3.org/1998/Math/MathML"><mi>γ</mi><mo>=</mo><mn>1.114</mn><mo stretchy="false">(</mo><mn>1</mn><mo stretchy="false">)</mo></math>, and <math display="inline" overflow="scroll" xmlns="http://www.w3.org/1998/Math/MathML"><mi>δ</mi><mo>=</mo><mn>4.504</mn><mo stretchy="false">(</mo><mn>5</mn><mo stretchy="false">)</mo></math> are obtained for <math display="inline" overflow="scroll" xmlns="http://www.w3.org/1998/Math/MathML"><mi>H</mi><mo>/</mo><mo>/</mo><mi>c</mi></math>, which fall between the three-dimensional (3D)-<math display="inline" overflow="scroll" xmlns="http://www.w3.org/1998/Math/MathML"><mi>X</mi><mi>Y</mi></math> and 3D-Ising models indicative of anisotropic magnetic coupling. An <math display="inline" overflow="scroll" xmlns="http://www.w3.org/1998/Math/MathML"><mi>H</m
碲化铬 CrxTey 因其固有的铁磁性和强磁各向异性,在自旋电子学中具有巨大的应用潜力。在这项研究中,我们系统地研究了具有强垂直磁各向异性(PMA)的铁磁性 Cr2Te3 单晶体的磁特性。除了 H//c 和 H//ab 在 TC∼181 K 时的铁磁到顺磁(FM-PM)转变外,还揭示了其他奇特的磁性行为,如由各向异性磁化揭示的场调制一阶转变、倾斜的 FM 耦合,而不是之前报道的由交流电感所证明的自旋玻璃行为。此外,各向异性磁化揭示了比任何其他铬基过渡金属掺杂物更强的显著 PMA,H//c 的饱和磁场可忽略不计,但 H//ab 的饱和磁场高达 155 kOe。H//c 的临界指数 β=0.340(5)、γ=1.114(1) 和 δ=4.504(5) 介于三维(3D)-XY 和三维-Ising 模型之间,表明存在各向异性的磁耦合。针对 H//c 构建了 Cr2Te3 单晶的 H-T 相图,区分了悬臂 FM1、悬臂 FM2、强制 FM(FFM)和 PM 相。相图表明,在较低磁场下,向悬臂调频2的转变属于一阶类型,而在外加磁场的作用下,这一转变被抑制为二阶类型。多重相变和复杂的磁性结构被认为源于层内超交换(调频耦合)和层间直接相互作用(原子力显微镜耦合)之间的竞争。各种磁性构型和强 PMA 使 Cr2Te3 极有希望应用于自旋电子器件。
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Physical Review Applied
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